Journal of Cleaner Production最新文献

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Measuring Circularity in the Construction Industry: A Systematic Literature Review from the Stakeholder Perspective 建筑业循环度测量:基于利益相关者视角的系统文献综述
IF 11.1 1区 环境科学与生态学
Journal of Cleaner Production Pub Date : 2025-01-22 DOI: 10.1016/j.jclepro.2025.144805
Luyuan Peng, Wen-Jun Cao
{"title":"Measuring Circularity in the Construction Industry: A Systematic Literature Review from the Stakeholder Perspective","authors":"Luyuan Peng, Wen-Jun Cao","doi":"10.1016/j.jclepro.2025.144805","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.144805","url":null,"abstract":"The implementation of the circular economy (CE) in the construction industry has become a feasible solution for achieving sustainable development while reducing environmental impact. It is essential to systematically monitor, manage, and evaluate circularity within the construction industry based on the needs and interests of stakeholders, as this can provide evidence for circular practices. However, the integration of CE increases complexities in the stakeholder network of the construction industry. Many stakeholders lack clarity about their roles, requirements, and aspirations in circular projects, leading to ineffective, hesitant, and ambiguous utilization of various circular measurement methods. To address those problems, this paper adopts a systematic literature review approach to conduct a comprehensive and critical review of measuring circularity from a stakeholder perspective. The paper categorizes stakeholders into 7 key groups and identifies their needs and dilemmas at specific stages of the circular project life cycle. Additionally, this study reviews the current development of circularity measurements at different stages of the circular project life cycle and discusses how well they align with stakeholders' needs and dilemmas. Finally, this study finds that there have been various attempts, but several essential prerequisites for comprehensive measurement are missing or incomplete. Several recommendations for measuring circularity that align more closely with stakeholder needs and address their current dilemmas are proposed. These findings are intended to enhance the evaluation, regulation, and oversight of CE in the construction industry, as well as to promote CE implementation.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"28 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142991975","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Nonlinear effects of urban multidimensional characteristics on air pollution heterogeneity in China's urban agglomerations 城市多维特征对中国城市群大气污染异质性的非线性影响
IF 11.1 1区 环境科学与生态学
Journal of Cleaner Production Pub Date : 2025-01-22 DOI: 10.1016/j.jclepro.2025.144813
Yikai Yang, Luoman Ouyang, Zhiqiang Wu, Qingrui Minyag Jiang, Renlu Qiao
{"title":"Nonlinear effects of urban multidimensional characteristics on air pollution heterogeneity in China's urban agglomerations","authors":"Yikai Yang, Luoman Ouyang, Zhiqiang Wu, Qingrui Minyag Jiang, Renlu Qiao","doi":"10.1016/j.jclepro.2025.144813","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.144813","url":null,"abstract":"Air pollution remains a pervasive global threat, with far-reaching implications for both environmental sustainability and public health. While considerable research has examined the relationship between PM<sub>2.5</sub> concentrations and their driving factors, the nonlinear contributions of these factors, especially across different urban contexts, remain insufficiently explored. This study seeks to bridge this gap by applying interpretable machine learning (XGBoost) to investigate the nonlinear impacts of meteorological, socio-economic, environmental, and architectural variables on PM<sub>10</sub> and PM<sub>2.5</sub> levels. Specifically, we aim to understand how these factors' contributions differ across three major urban agglomerations (UAs) in China. Our findings reveal notable spatial heterogeneity, with meteorological variables, such as temperature, AOD, and evapotranspiration playing a predominant role in the BTH region, while architectural factors have a more significant impact in the PRD, contributing more than 60%. In the YRD, increasing standard deviation of building height (SDBH) to 20-40m and average mean building height (MBH) to 15-20m are associated with lower PM<sub>10</sub> concentrations. Notably, the impact of socio-economic activities on air pollution was also observed. For example, as NPP_VIIRS increased from 15 to 120, PM<sub>2.5</sub> concentrations in the PRD region decreased from 14 μg/m³ to 11.5 μg/m³, a novel finding not previously highlighted in related studies. Furthermore, the relationship between GDP and PM<sub>2.5</sub> concentrations follows a nonlinear pattern, initially rising and then declining, a pattern consistently observed across all UAs. Overall, this study underscores the spatial heterogeneity in the relationship between air pollutants and their driving factors, offering insights for region-specific pollution control strategies and broader global environmental management frameworks.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"45 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143020149","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
How supply chain finance promote carbon emission reduction in manufacturing firms—Evidence from Chinese market 供应链金融如何促进制造业企业碳减排——来自中国市场的证据
IF 11.1 1区 环境科学与生态学
Journal of Cleaner Production Pub Date : 2025-01-22 DOI: 10.1016/j.jclepro.2025.144849
Long Xue, Shijie Ai
{"title":"How supply chain finance promote carbon emission reduction in manufacturing firms—Evidence from Chinese market","authors":"Long Xue, Shijie Ai","doi":"10.1016/j.jclepro.2025.144849","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.144849","url":null,"abstract":"This paper provides evidence of the role of supply chain finance (hereinafter referred to as SCF) in the development of the manufacturing industry in China. As the world's largest manufacturing country and the second-largest economy, China presents a unique case for this study. Utilizing data from A-share manufacturing companies in Shanghai and Shenzhen from 2008 to 2021, we examine the impact of SCF on carbon emission reduction among manufacturing enterprises in China. The study finds that SCF contributes to reducing carbon emissions in manufacturing companies. After conducting a series of robustness tests and controlling for potential endogeneity issues, this conclusion remains valid. Regarding the transmission mechanism, SCF's contribution to carbon emission reduction in manufacturing firms occurs through the pathways of corporate financial availability and green technology innovation. Further research shows that the promotion effect of SCF on carbon emission reduction of manufacturing enterprises is more obvious in areas with strong environmental regulations and high level of digital economy development, as well as manufacturing enterprises with high supply chain concentration and strong management ability.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"10 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142991919","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
How is carbon storage in plateau–plain transition zone influenced? Evidence from Minjiang River Basin, China 高原-平原过渡带对碳储量有何影响?来自中国岷江流域的证据
IF 11.1 1区 环境科学与生态学
Journal of Cleaner Production Pub Date : 2025-01-22 DOI: 10.1016/j.jclepro.2025.144766
Menglin Qin, Xinyu Wu, Yijia Zhou, Xiaoyue Li, Hongbo Jiang, Dingding Luo, Yuting Liu, Ouyang Huiting
{"title":"How is carbon storage in plateau–plain transition zone influenced? Evidence from Minjiang River Basin, China","authors":"Menglin Qin, Xinyu Wu, Yijia Zhou, Xiaoyue Li, Hongbo Jiang, Dingding Luo, Yuting Liu, Ouyang Huiting","doi":"10.1016/j.jclepro.2025.144766","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.144766","url":null,"abstract":"Topographic transition zones are vital for global carbon storage and are sensitive to climate change, playing a key role in achieving global carbon neutrality goals. However, previous studies have not adequately addressed the characteristics of these zones from a comprehensive macroscopic perspective. To fill this gap, this study examines the Minjiang River Basin (MRB), which exemplifies a typical plateau–plain transition zone, dividing it into three areas: upstream, midstream, and downstream. Carbon density values were estimated based on land use and soil attribute data from 2000 to 2020, and the spatiotemporal distribution and changes in carbon storage were analyzed using the Integrated Valuation of Ecosystem Services and Trade-offs model along with Standard Deviation Ellipse Analysis. Sixteen natural economic indicators from 52 districts and counties were selected to construct a geographically and temporally weighted regression model, exploring the spatiotemporal heterogeneity of influencing factors across the basin. The results revealed the following: (1) From 2000 to 2020, total carbon storage in the MRB decreased by 5.563×10<sup>6</sup> t, with the midstream region accounting for 83.93% of this decline. (2) The dominant factors influencing carbon storage were nighttime light (NL) and relative humidity, with average influence intensities of -0.181 and 0.111, respectively. (3) Influencing factors exhibited significant spatiotemporal heterogeneity; the upstream area was most adversely affected by NL, with a maximum regression coefficient of -3.29. In contrast, the midstream and downstream areas experienced relatively weak influences, primarily from the positive effects of annual production value in the primary industry and soil pH, which had maximum regression coefficients of 0.437 and 0.747, respectively. These findings provide robust data for assessing regional carbon sequestration capacity in the MRB and offer a theoretical basis for conducting ecological protection and managing human activities in areas with complex terrain.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"10 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142991917","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
HYDROTHERMAL CARBONIZATION – A CRITICAL OVERVIEW OF ITS ENVIRONMENTAL AND ECONOMIC SUSTAINABILITY 热液碳化-其环境和经济可持续性的关键概述
IF 11.1 1区 环境科学与生态学
Journal of Cleaner Production Pub Date : 2025-01-22 DOI: 10.1016/j.jclepro.2025.144838
Matheus Cavali, Aline Perin Dresch, Igor Marcon Belli, Nelson Libardi Junior, Adenise Lorenci Woiciechowski, Sebastião Roberto Soares, Armando Borges de Castilhos Junior
{"title":"HYDROTHERMAL CARBONIZATION – A CRITICAL OVERVIEW OF ITS ENVIRONMENTAL AND ECONOMIC SUSTAINABILITY","authors":"Matheus Cavali, Aline Perin Dresch, Igor Marcon Belli, Nelson Libardi Junior, Adenise Lorenci Woiciechowski, Sebastião Roberto Soares, Armando Borges de Castilhos Junior","doi":"10.1016/j.jclepro.2025.144838","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.144838","url":null,"abstract":"Circular economy and waste valorization are intertwined concepts crucial for sustainable development. From this perspective, the search for environmentally friendly processes that supply energy and materials from waste is growing. Hydrothermal carbonization (HTC) is a promising thermochemical process that converts waste into a solid product named hydrochar. Hydrochar, given its physicochemical characteristics, has the potential for several applications (e.g., energy production, soil amendment, and adsorption of water pollutants), which has boosted the research interest in HTC. Several studies have focused on optimizing HTC conditions and evaluating the environmental and economic aspects of this process through life cycle assessment (LCA) and techno-economic analysis (TEA), respectively. However, despite the increasing number of review articles about feedstocks, optimal conditions, and reaction mechanisms of HTC, a critical review focused on HTC sustainability is lacking in the literature. Therefore, this review provides a critical outlook on LCA and TEA studies concerning HTC to verify its environmental and economic sustainability from a broad perspective. Overall, some studies have demonstrated the environmental and economic feasibility of HTC, as evidenced by the current technology readiness level (TRL) of this thermochemical process, which has reached industrial implementation in the last decade. Moreover, this waste valorization approach can evolve into a multi-product biorefinery, in addition to becoming a potential contributor to the achievement of some Sustainable Development Goals (SDGs).","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"42 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142992042","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Mapping socio-environmental policy integration in the European Union: A multilayer network approach 绘制欧盟社会环境政策一体化:多层网络方法
IF 11.1 1区 环境科学与生态学
Journal of Cleaner Production Pub Date : 2025-01-22 DOI: 10.1016/j.jclepro.2025.144792
Roy Cerqueti, Giovanna Ferraro, Raffaele Mattera, Saverio Storani
{"title":"Mapping socio-environmental policy integration in the European Union: A multilayer network approach","authors":"Roy Cerqueti, Giovanna Ferraro, Raffaele Mattera, Saverio Storani","doi":"10.1016/j.jclepro.2025.144792","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.144792","url":null,"abstract":"This paper faces the relevant task of assessing the integration of European countries when dealing with three paradigmatic socio-environmental themes: Circular Economy (CE), Energy Transition (ET), and Social Justice (SJ). Specifically, we aim to explore whether a similar behavior in facing one of the considered aspects is mirrored by similarity in the others. We move from a dataset composed of five variables for CE, two for ET, and three for SJ, representing yearly data for the quinquennium 2016-2020 and European countries. We build a multilayer network based on the ten variables having countries as nodes. Each layer/variable has weighted links based on countries’ similarity. Inter-layer links are created through a community detection exercise over the individual layers. This approach allows us to evaluate analogies, leading to the assessment of intra- and inter-layer policy integration. We find a relatively low level of integration at the European level and a high sensitivity to the number of detected communities, thus revealing the role of countries’ heterogeneity in driving integration.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"50 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143020147","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Towards Sustainable Chemical Process Design: Revisiting the Integration of Life Cycle Assessment 迈向可持续化工过程设计:重新审视生命周期评估的整合
IF 11.1 1区 环境科学与生态学
Journal of Cleaner Production Pub Date : 2025-01-22 DOI: 10.1016/j.jclepro.2025.144831
Bartolomeus Häussling Löwgren, Christian Hoffmann, Martina G. Vijver, Bernhard Steubing, Giuseppe Cardellini
{"title":"Towards Sustainable Chemical Process Design: Revisiting the Integration of Life Cycle Assessment","authors":"Bartolomeus Häussling Löwgren, Christian Hoffmann, Martina G. Vijver, Bernhard Steubing, Giuseppe Cardellini","doi":"10.1016/j.jclepro.2025.144831","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.144831","url":null,"abstract":"Life-cycle assessment (LCA) is essential for sustainable chemical process design. However, current integrations treat LCA as a top-level environmental assessment tool, risking superficial integration and perpetuating conventional process design assumptions. This contribution reviews how LCA is integrated with model-based chemical process design. It focuses on current practices, challenges in goal and scope, modelling, computational, and interpretation integration, and discusses the integration of LCA's core features alongside profit-driven assumptions.The contribution identified more than 100 articles via a hybrid search method and reviewed 53 based on a saturation curve, resulting in 25 metrics to assess process design and LCA integration. To assist practitioners, a comprehensive classification of computational integrations is provided. The review highlights the following gaps: most studies (74%) focus only on cradle-to-gate phases, neglect use and end-of-life phases (89%) and do not define the function (92%). However, including a user function perspective could enhance the integration of use and end-of-life scenarios, supporting circular strategies and sufficiency measures. Additionally, environmental externalities are systematically excluded during model linkage, and most studies concentrate on energy utilities (75%) and material inputs (70%), whereas emissions (26%), waste, and wastewater (25%) are frequently overlooked, which emphasises the dominance of economic factors in current design studies.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"137 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143020144","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Clean production of microalgae high-value lipid fraction: Influence of different pretreatments on chemical and cytotoxic profiles of Chlorella vulgaris supercritical extracts and life cycle assessment 微藻高价值脂质组分的清洁生产:不同预处理对小球藻超临界提取物化学和细胞毒性的影响及生命周期评价
IF 11.1 1区 环境科学与生态学
Journal of Cleaner Production Pub Date : 2025-01-22 DOI: 10.1016/j.jclepro.2025.144823
Jelena Vladic, Sanja Radman, Zeljko Zizak, Irina Besu, Igor Jerkovic, Lais Galileu Speranza, Ahmad Furqan Hala, Strahinja Kovacevic, Hugo Perreira, Luisa Gouveia
{"title":"Clean production of microalgae high-value lipid fraction: Influence of different pretreatments on chemical and cytotoxic profiles of Chlorella vulgaris supercritical extracts and life cycle assessment","authors":"Jelena Vladic, Sanja Radman, Zeljko Zizak, Irina Besu, Igor Jerkovic, Lais Galileu Speranza, Ahmad Furqan Hala, Strahinja Kovacevic, Hugo Perreira, Luisa Gouveia","doi":"10.1016/j.jclepro.2025.144823","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.144823","url":null,"abstract":"Microalgae have emerged as a promising natural resource rich in bioactive compounds. Health-beneficial properties of microalgae, coupled with advantageous characteristics such as high biomass productivity, adaptability, robustness, and carbon dioxide mitigation, position them as a viable solution for global sustainable food production. This study explored clean and environmentally friendly processes to enhance the recovery of lipid bioactive fractions. Microwave (MW), enzymatic (ENZ), and ultrasound (US) pretreatments were applied to improve environmentally friendly extraction of lipid-based components using supercritical CO<sub>2</sub>. The effects of these pretreatments on extraction yield, chemical profiles, and cytotoxic properties of <em>Chlorella vulgaris</em> (Cv) and smooth <em>C. vulgaris</em> (sCv) extracts were investigated. Additionally, a Life Cycle Assessment (LCA) was conducted to evaluate environmental impacts. MW pretreatment achieved the highest yield increases, from 2.58 times (Cv) to 3.15 times (sCv). UHPLC-ESI-HRMS analysis revealed shifts in the distribution of pigments and derivatives caused by pretreatments, with ENZ extracts showing the most pronounced changes: pigments increased from 9.24% (control Cv) to 40.92% (Cv) and from 12.52% (control sCv) to 71.12% (sCv). Cv extracts exhibited greater activity against MDA-MB-453 cells, while sCv extracts from US pretreatment demonstrated the strongest effect on HeLa cells. The LCA indicated reduced environmental impacts of the pretreatment-enhanced processes up to 65% compared to the control. A scenario analysis was presented to show further possible impact reduction by recirculating the CO<sub>2</sub> solvent and substituting the energy source. These findings provide valuable insights into sustainable and scalable green processes for recovering microalgal bioactive components.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"74 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143020146","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Synergistic Effect of Bimetallic Bioelectrocatalysis and Endogenous Soluble Electron Mediators for Functional Regulation of Electroactive Biofilms 双金属生物电催化与内源性可溶性电子介质在电活性生物膜功能调控中的协同作用
IF 11.1 1区 环境科学与生态学
Journal of Cleaner Production Pub Date : 2025-01-22 DOI: 10.1016/j.jclepro.2025.144789
Xu Pan, Ye Chen, Qing Wen, Cunguo Lin, Haiping Gao, Zhenghui Qiu, Liuqingying Yang
{"title":"Synergistic Effect of Bimetallic Bioelectrocatalysis and Endogenous Soluble Electron Mediators for Functional Regulation of Electroactive Biofilms","authors":"Xu Pan, Ye Chen, Qing Wen, Cunguo Lin, Haiping Gao, Zhenghui Qiu, Liuqingying Yang","doi":"10.1016/j.jclepro.2025.144789","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.144789","url":null,"abstract":"Microbial fuel cells (MFCs) are green power generation devices that convert chemical energy into electricity. The energy conversion efficiency and power generation performance of MFCs are primarily influenced by the extracellular electron transfer (EET) process mediated by electroactive bacteria. In this study, Zr, N-codoped carbon (Zr-NC) and Fe, Zr, N-codoped carbon (Fe-Zr-NC) materials were derived from amino-modified Zr and Fe-Zr metal organic frameworks (MOF), respectively, and were considered as high-performance bioelectrocatalysts to optimize the multi-electron EET pathway and the interfacial charge transfer kinetics. Compared to Zr-NC MFC, the maximum power density of Fe-Zr-NC MFC increased from 3.62 to 5.25 W/m<sup>2</sup>, and the coulombic efficiency increased from 18.23% to 26.37%. In addition, Fe-Zr-NC improved the total capacitive behavior contribution of bioanode, increasing the limiting storage capacity of biocapacitor from 4207.46 to 10582.28 C/m<sup>2</sup>. Furthermore, the exchange current density of the Fe-Zr-NC bioanode increased from 0.65 to 1.43 mA/cm<sup>2</sup>, while the charge transfer resistance decreased from 3.72 Ω to 1.08 Ω. Electrochemical measurements and density functional theory (DFT) suggested that the charge redistribution of Fe atoms at the bimetallic catalytic sites increased the interfacial potential difference of the terminal conductive protein and the strong adsorption of flavin species, thus regulating the dominant EET pathway and charge transfer kinetics. High-throughput sequencing results and PICRUSt2 indicated the affinity of Fe-Zr-NC bioelectrocatalyst for functional microorganisms, facilitating the enrichment of exoelectrogens and the secretion of soluble electron mediators. Fe-Zr-NC can serve as a novel bioelectrocatalyst with high performance and stability for the improvement of MFCs or biocapacitors, leading to higher power output and energy conversion efficiency.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"37 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142991918","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Pore-Scale Dynamics of Steam Assisted Gravity Drainage with Hydrocarbon Solvents (HC-SAGD) for Technically and Environmentally Efficient Heavy Oil Recovery 烃类溶剂蒸汽辅助重力泄油(HC-SAGD)在稠油开采中的孔隙尺度动力学研究
IF 11.1 1区 环境科学与生态学
Journal of Cleaner Production Pub Date : 2025-01-22 DOI: 10.1016/j.jclepro.2025.144833
Jingjing Huang, Tayfun Babadagli
{"title":"Pore-Scale Dynamics of Steam Assisted Gravity Drainage with Hydrocarbon Solvents (HC-SAGD) for Technically and Environmentally Efficient Heavy Oil Recovery","authors":"Jingjing Huang, Tayfun Babadagli","doi":"10.1016/j.jclepro.2025.144833","DOIUrl":"https://doi.org/10.1016/j.jclepro.2025.144833","url":null,"abstract":"Steam Assisted Gravity Drainage (SAGD) is the primary in-situ heavy oil and bitumen recovery method in Canada. Improvement of the efficiency of this method is essential for new and matured SAGD projects to minimize the project cost and the amount of carbon emitted for steam generation. Adding hydrocarbon (HC) solvents to steam can effectively improve the recovery efficiency of SAGD by improving the recovery per amount of the steam used. The optimization of this process requires further clarifications and understandings on the fluid-steam-rock interactions, especially at the pore scale. For this purpose, a visual two-dimensional physical porous media model was constructed and HC additive-assisted SAGD (HC-SAGD) process was studied. Heptane was selected to represent the HC phase as it its boiling point is close to water. The effects of physicochemical properties of the oil-steam-water-heptane and fluid-rock interactions on the growth of the steam chamber and oil drainage were visually analyzed. The oil recovery efficiency, energy efficiency and carbon emission intensity of HC-SAGD and SAGD were compared for different scenarios to suggest optimal operational conditions. It was shown that the introduction of HC can reduce carbon emission intensity to that of the half of conventional SAGD while improving heavy oil recovery. It was also observed that the technical and economic benefits of solvent addition to steam in the SAGD process could be much higher than previously anticipated.","PeriodicalId":349,"journal":{"name":"Journal of Cleaner Production","volume":"81 1","pages":""},"PeriodicalIF":11.1,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143020145","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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