Environmental Science and Ecotechnology最新文献

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Demystifying polyphosphate-accumulating organisms relevant to wastewater treatment: A review of their phylogeny, metabolism, and detection 揭开与废水处理有关的聚磷酸盐积累生物的神秘面纱:系统发育、新陈代谢和检测综述
IF 12.6 1区 环境科学与生态学
Environmental Science and Ecotechnology Pub Date : 2024-01-04 DOI: 10.1016/j.ese.2024.100387
Lucia Ruiz-Haddad , Muhammad Ali , Mario Pronk , Mark C.M. van Loosdrecht , Pascal E. Saikaly
{"title":"Demystifying polyphosphate-accumulating organisms relevant to wastewater treatment: A review of their phylogeny, metabolism, and detection","authors":"Lucia Ruiz-Haddad ,&nbsp;Muhammad Ali ,&nbsp;Mario Pronk ,&nbsp;Mark C.M. van Loosdrecht ,&nbsp;Pascal E. Saikaly","doi":"10.1016/j.ese.2024.100387","DOIUrl":"10.1016/j.ese.2024.100387","url":null,"abstract":"<div><p>Currently, the most cost-effective and efficient method for phosphorus (P) removal from wastewater is enhanced biological P removal (EPBR) via polyphosphate-accumulating organisms (PAOs). This study integrates a literature review with genomic analysis to uncover the phylogenetic and metabolic diversity of the relevant PAOs for wastewater treatment. The findings highlight significant differences in the metabolic capabilities of PAOs relevant to wastewater treatment. Notably, <em>Candidatus</em> Dechloromonas and <em>Candidatus</em> Accumulibacter can synthesize polyhydroxyalkanoates, possess specific enzymes for ATP production from polyphosphate, and have electrochemical transporters for acetate and C4-dicarboxylates. In contrast, <em>Tetrasphaera, Candidatus</em> Phosphoribacter, <em>Knoellia,</em> and <em>Phycicoccus</em> possess PolyP-glucokinase and electrochemical transporters for sugars/amino acids. Additionally, this review explores various detection methods for polyphosphate and PAOs in activated sludge wastewater treatment plants. Notably, FISH-Raman spectroscopy emerges as one of the most advanced detection techniques. Overall, this review provides critical insights into PAO research, underscoring the need for enhanced strategies in biological phosphorus removal.</p></div>","PeriodicalId":34434,"journal":{"name":"Environmental Science and Ecotechnology","volume":null,"pages":null},"PeriodicalIF":12.6,"publicationDate":"2024-01-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2666498424000012/pdfft?md5=dfb1e924dceed7a49a7adc8fb7101cc0&pid=1-s2.0-S2666498424000012-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139393429","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Exploring research on ecotechnology through artificial intelligence and bibliometric maps 通过人工智能和文献计量图探索生态技术研究
IF 12.6 1区 环境科学与生态学
Environmental Science and Ecotechnology Pub Date : 2024-01-04 DOI: 10.1016/j.ese.2023.100386
Ricardo Ruiz-Sánchez , Ricardo Arencibia-Jorge , Julia Tagüeña , José Luis Jiménez-Andrade , Humberto Carrillo-Calvet
{"title":"Exploring research on ecotechnology through artificial intelligence and bibliometric maps","authors":"Ricardo Ruiz-Sánchez ,&nbsp;Ricardo Arencibia-Jorge ,&nbsp;Julia Tagüeña ,&nbsp;José Luis Jiménez-Andrade ,&nbsp;Humberto Carrillo-Calvet","doi":"10.1016/j.ese.2023.100386","DOIUrl":"10.1016/j.ese.2023.100386","url":null,"abstract":"<div><p>Ecotechnology, quintessential for crafting sustainable socio-environmental strategies, remains tantalizingly uncharted. Our analysis, steered by the nuances of machine learning and augmented by bibliometric insights, delineates the expansive terrain of this domain, elucidates pivotal research themes and conundrums, and discerns the vanguard nations in this field. Furthermore, we deftly connect our discoveries to the United Nations' 2030 Sustainable Development Goals, thereby accentuating the profound societal ramifications of ecotechnology.</p></div>","PeriodicalId":34434,"journal":{"name":"Environmental Science and Ecotechnology","volume":null,"pages":null},"PeriodicalIF":12.6,"publicationDate":"2024-01-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2666498423001515/pdfft?md5=5abdf9eeb7a603c814c404b4ab1ea67d&pid=1-s2.0-S2666498423001515-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139395149","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Health risk ranking of antibiotic resistance genes in the Yangtze River 长江中抗生素耐药基因的健康风险排序
IF 12.6 1区 环境科学与生态学
Environmental Science and Ecotechnology Pub Date : 2024-01-03 DOI: 10.1016/j.ese.2024.100388
Chunxia Jiang , Zelong Zhao , Hans-Peter Grossart , Feng Ju , Yi Zhao , Geoffrey Michael Gadd , Ewa Korzeniewska , Yuyi Yang
{"title":"Health risk ranking of antibiotic resistance genes in the Yangtze River","authors":"Chunxia Jiang ,&nbsp;Zelong Zhao ,&nbsp;Hans-Peter Grossart ,&nbsp;Feng Ju ,&nbsp;Yi Zhao ,&nbsp;Geoffrey Michael Gadd ,&nbsp;Ewa Korzeniewska ,&nbsp;Yuyi Yang","doi":"10.1016/j.ese.2024.100388","DOIUrl":"10.1016/j.ese.2024.100388","url":null,"abstract":"<div><p>Antibiotic resistance is an escalating global health concern, exacerbated by the pervasive presence of antibiotic resistance genes (ARGs) in natural environments. The Yangtze River, the world's third-longest river, traversing areas with intense human activities, presents a unique ecosystem for studying the impact of these genes on human health. Here, we explored ARGs in the Yangtze River, examining 204 samples from six distinct habitats of approximately 6000 km of the river, including free-living and particle-associated settings, surface and bottom sediments, and surface and bottom bank soils. Employing shotgun sequencing, we generated an average of 13.69 Gb reads per sample. Our findings revealed a significantly higher abundance and diversity of ARGs in water-borne bacteria compared to other habitats. A notable pattern of resistome coalescence was observed within similar habitat types. In addition, we developed a framework for ranking the risk of ARG and a corresponding method for calculating the risk index. Applying them, we identified water-borne bacteria as the highest contributors to health risks, and noted an increase in ARG risks in particle-associated bacteria correlating with heightened anthropogenic activities. Further analysis using a weighted ARG risk index pinpointed the Chengdu–Chongqing and Yangtze River Delta urban agglomerations as regions of elevated health risk. These insights provide a critical new perspective on ARG health risk assessment, highlighting the urgent need for strategies to mitigate the impact of ARGs on human health and to preserve the ecological and economic sustainability of the Yangtze River for future human use.</p></div>","PeriodicalId":34434,"journal":{"name":"Environmental Science and Ecotechnology","volume":null,"pages":null},"PeriodicalIF":12.6,"publicationDate":"2024-01-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2666498424000024/pdfft?md5=642220b1cdd44d6baa25dbbce5f992fe&pid=1-s2.0-S2666498424000024-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139395526","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Copper-based electro-catalytic nitrate reduction to ammonia from water: Mechanism, preparation, and research directions 铜基电催化硝酸盐从水中还原成氨:机理、制备和研究方向
IF 12.6 1区 环境科学与生态学
Environmental Science and Ecotechnology Pub Date : 2023-12-28 DOI: 10.1016/j.ese.2023.100383
Jinshan Wei , Yi Li , Hexing Lin , Xihui Lu , Chucheng Zhou, Ya-yun Li
{"title":"Copper-based electro-catalytic nitrate reduction to ammonia from water: Mechanism, preparation, and research directions","authors":"Jinshan Wei ,&nbsp;Yi Li ,&nbsp;Hexing Lin ,&nbsp;Xihui Lu ,&nbsp;Chucheng Zhou,&nbsp;Ya-yun Li","doi":"10.1016/j.ese.2023.100383","DOIUrl":"10.1016/j.ese.2023.100383","url":null,"abstract":"<div><p>Global water bodies are increasingly imperiled by nitrate pollution, primarily originating from industrial waste, agricultural runoffs, and urban sewage. This escalating environmental crisis challenges traditional water treatment paradigms and necessitates innovative solutions. Electro-catalysis, especially utilizing copper-based catalysts, known for their efficiency, cost-effectiveness, and eco-friendliness, offer a promising avenue for the electro-catalytic reduction of nitrate to ammonia. In this review, we systematically consolidate current research on diverse copper-based catalysts, including pure Cu, Cu alloys, oxides, single-atom entities, and composites. Furthermore, we assess their catalytic performance, operational mechanisms, and future research directions to find effective, long-term solutions to water purification and ammonia synthesis. Electro-catalysis technology shows the potential in mitigating nitrate pollution and has strategic importance in sustainable environmental management. As to the application, challenges regarding complexity of the real water, the scale-up of the commerical catalysts, and the efficient collection of produced NH<sub>3</sub> are still exist. Following reseraches of catalyst specially on long term stability and <em>in situ</em> mechanisms are proposed.</p></div>","PeriodicalId":34434,"journal":{"name":"Environmental Science and Ecotechnology","volume":null,"pages":null},"PeriodicalIF":12.6,"publicationDate":"2023-12-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2666498423001485/pdfft?md5=42a929de2f9565776f40be0fb64ff9ee&pid=1-s2.0-S2666498423001485-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139190533","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dynamic membrane filtration accelerates electroactive biofilms in bioelectrochemical systems 动态膜过滤加速生物电化学系统中的电活性生物膜
IF 12.6 1区 环境科学与生态学
Environmental Science and Ecotechnology Pub Date : 2023-12-27 DOI: 10.1016/j.ese.2023.100375
Jinning Wang , Mei Chen , Jiayao Zhang , Xinyi Sun , Nan Li , Xin Wang
{"title":"Dynamic membrane filtration accelerates electroactive biofilms in bioelectrochemical systems","authors":"Jinning Wang ,&nbsp;Mei Chen ,&nbsp;Jiayao Zhang ,&nbsp;Xinyi Sun ,&nbsp;Nan Li ,&nbsp;Xin Wang","doi":"10.1016/j.ese.2023.100375","DOIUrl":"https://doi.org/10.1016/j.ese.2023.100375","url":null,"abstract":"<div><p>Bioelectrochemical systems (BES) have emerged as a dual-function technology for treating wastewater and recovering energy. A vital element of BES is the rapid formation and maintenance of electroactive biofilms (EABs). Previous attempts to accelerate EAB formation and improve electroactivities focused on enhancing the bacterial adhesion process while neglecting the rate-limiting step of the bacterial transport process. Here, we introduce membrane filtration into BES, establishing a dynamic membrane filtration system that enhances overall performance. We observed that optimal membrane flux considerably reduced the startup time for EAB formation. Specifically, EABs established under a 25 L m<sup>−2</sup> h<sup>−1</sup> flux (EAB<sub>25 LMH</sub>) had a formation time of 43.8 ± 1.3 h, notably faster than the 51.4 ± 1.6 h in the static state (EAB<sub>0 LMH</sub>). Additionally, EAB<sub>25 LMH</sub> exhibited a significant increase in maximum current density, approximately 2.2 times higher than EAB<sub>0 LMH</sub>. Pearson correlation analysis indicated a positive relationship between current densities and biomass quantities and an inverse correlation with startup time. Microbial analysis revealed two critical findings: (i) variations in maximum current densities across different filtration conditions were associated with redox-active substances and biomass accumulation, and (ii) the incorporation of a filtration process in EAB formation enhanced the proportion of viable cells and encouraged a more diverse range of electroactive bacteria. Moreover, the novel electroactive membrane demonstrated sustained current production and effective solid-liquid separation during prolonged operation, indicating its potential as a viable alternative in membrane-based systems. This approach not only provides a new operational model for BES but also holds promise for expanding its application in future wastewater treatment solutions.</p></div>","PeriodicalId":34434,"journal":{"name":"Environmental Science and Ecotechnology","volume":null,"pages":null},"PeriodicalIF":12.6,"publicationDate":"2023-12-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2666498423001400/pdfft?md5=b5372c62be2272b0b273dfa3596fc7ff&pid=1-s2.0-S2666498423001400-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139419288","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Advanced wastewater treatment with microalgae-indigenous bacterial interactions 利用微藻与土著细菌的相互作用进行高级废水处理
IF 12.6 1区 环境科学与生态学
Environmental Science and Ecotechnology Pub Date : 2023-12-21 DOI: 10.1016/j.ese.2023.100374
Xue Li , Shengnan Li , Peng Xie , Xi Chen , Yuhao Chu , Haixing Chang , Jian Sun , Qing Li , Nanqi Ren , Shih-Hsin Ho
{"title":"Advanced wastewater treatment with microalgae-indigenous bacterial interactions","authors":"Xue Li ,&nbsp;Shengnan Li ,&nbsp;Peng Xie ,&nbsp;Xi Chen ,&nbsp;Yuhao Chu ,&nbsp;Haixing Chang ,&nbsp;Jian Sun ,&nbsp;Qing Li ,&nbsp;Nanqi Ren ,&nbsp;Shih-Hsin Ho","doi":"10.1016/j.ese.2023.100374","DOIUrl":"10.1016/j.ese.2023.100374","url":null,"abstract":"<div><p>Microalgal-indigenous bacterial wastewater treatment (MBWT) emerges as a promising approach for the concurrent removal of nitrogen (N) and phosphorus (P). Despite its potential, the prevalent use of MBWT in batch systems limits its broader application. Furthermore, the success of MBWT critically depends on the stable self-adaptation and synergistic interactions between microalgae and indigenous bacteria, yet the underlying biological mechanisms are not fully understood. Here we explore the viability and microbial dynamics of a continuous flow microalgae-indigenous bacteria advanced wastewater treatment system (CFMBAWTS) in processing actual secondary effluent, with a focus on varying hydraulic retention times (HRTs). The research highlights a stable, mutually beneficial relationship between indigenous bacteria and microalgae. Microalgae and indigenous bacteria can create an optimal environment for each other by providing essential cofactors (like iron, vitamins, and indole-3-acetic acid), oxygen, dissolved organic matter, and tryptophan. This collaboration leads to effective microbial growth, enhanced N and P removal, and energy generation. The study also uncovers crucial metabolic pathways, functional genes, and patterns of microbial succession. Significantly, the effluent NH<sub>4</sub><sup>+</sup>-N and P levels complied with the Chinese national Class-II, Class-V, Class-IA, and Class-IB wastewater discharge standards when the HRT was reduced from 15 to 6 h. Optimal results, including the highest rates of CO<sub>2</sub> fixation (1.23 g L<sup>−1</sup>), total energy yield (32.35 kJ L<sup>−1</sup>), and the maximal lipid (33.91%) and carbohydrate (41.91%) content, were observed at an HRT of 15 h. Overall, this study not only confirms the feasibility of CFMBAWTS but also lays a crucial foundation for enhancing our understanding of this technology and propelling its practical application in wastewater treatment plants.</p></div>","PeriodicalId":34434,"journal":{"name":"Environmental Science and Ecotechnology","volume":null,"pages":null},"PeriodicalIF":12.6,"publicationDate":"2023-12-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2666498423001394/pdfft?md5=858f2940b113a32c89fe8f9af8a4355b&pid=1-s2.0-S2666498423001394-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139012953","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Electrogenic sulfur oxidation mediated by cable bacteria and its ecological effects 电缆细菌介导的电氧化硫及其生态效应
IF 12.6 1区 环境科学与生态学
Environmental Science and Ecotechnology Pub Date : 2023-12-19 DOI: 10.1016/j.ese.2023.100371
Zhenyu Wang , Leonid Digel , Yongqiang Yuan , Hui Lu , Yonggang Yang , Carsten Vogt , Hans-Hermann Richnow , Lars Peter Nielsen
{"title":"Electrogenic sulfur oxidation mediated by cable bacteria and its ecological effects","authors":"Zhenyu Wang ,&nbsp;Leonid Digel ,&nbsp;Yongqiang Yuan ,&nbsp;Hui Lu ,&nbsp;Yonggang Yang ,&nbsp;Carsten Vogt ,&nbsp;Hans-Hermann Richnow ,&nbsp;Lars Peter Nielsen","doi":"10.1016/j.ese.2023.100371","DOIUrl":"10.1016/j.ese.2023.100371","url":null,"abstract":"<div><p>At the sediment-water interfaces, filamentous cable bacteria transport electrons from sulfide oxidation along their filaments towards oxygen or nitrate as electron acceptors. These multicellular bacteria belonging to the family Desulfobulbaceae thus form a biogeobattery that mediates redox processes between multiple elements. Cable bacteria were first reported in 2012. In the past years, cable bacteria have been found to be widely distributed across the globe. Their potential in shaping the surface water environments has been extensively studied but is not fully elucidated. In this review, the biogeochemical characteristics, conduction mechanisms, and geographical distribution of cable bacteria, as well as their ecological effects, are systematically reviewed and discussed. Novel insights for understanding and applying the role of cable bacteria in aquatic ecology are summarized.</p></div>","PeriodicalId":34434,"journal":{"name":"Environmental Science and Ecotechnology","volume":null,"pages":null},"PeriodicalIF":12.6,"publicationDate":"2023-12-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2666498423001369/pdfft?md5=e9a6edc0a6e3f22e0424e4bd79e15139&pid=1-s2.0-S2666498423001369-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138991497","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Global WWTP Microbiome-based Integrative Information Platform: From experience to intelligence 基于微生物组的全球污水处理厂综合信息平台:从经验到智慧
IF 12.6 1区 环境科学与生态学
Environmental Science and Ecotechnology Pub Date : 2023-12-18 DOI: 10.1016/j.ese.2023.100370
Fuzhong Xiong , Zhiguo Su , Yushi Tang , Tianjiao Dai , Donghui Wen
{"title":"Global WWTP Microbiome-based Integrative Information Platform: From experience to intelligence","authors":"Fuzhong Xiong ,&nbsp;Zhiguo Su ,&nbsp;Yushi Tang ,&nbsp;Tianjiao Dai ,&nbsp;Donghui Wen","doi":"10.1016/j.ese.2023.100370","DOIUrl":"10.1016/j.ese.2023.100370","url":null,"abstract":"<div><p>Domestic and industrial wastewater treatment plants (WWTPs) are facing formidable challenges in effectively eliminating emerging pollutants and conventional nutrients. In microbiome engineering, two approaches have been developed: a top-down method focusing on domesticating seed microbiomes into engineered ones, and a bottom-up strategy that synthesizes engineered microbiomes from microbial isolates. However, these approaches face substantial hurdles that limit their real-world applicability in wastewater treatment engineering. Addressing this gap, we propose the creation of a Global WWTP Microbiome-based Integrative Information Platform, inspired by the untapped microbiome and engineering data from WWTPs and advancements in artificial intelligence (AI). This open platform integrates microbiome and engineering information globally and utilizes AI-driven tools for identifying seed microbiomes for new plants, providing technical upgrades for existing facilities, and deploying microbiomes for accidental pollution remediation. Beyond its practical applications, this platform has significant scientific and social value, supporting multidisciplinary research, documenting microbial evolution, advancing Wastewater-Based Epidemiology, and enhancing global resource sharing. Overall, the platform is expected to enhance WWTPs’ performance in pollution control, safeguarding a harmonious and healthy future for human society and the natural environment.</p></div>","PeriodicalId":34434,"journal":{"name":"Environmental Science and Ecotechnology","volume":null,"pages":null},"PeriodicalIF":12.6,"publicationDate":"2023-12-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2666498423001357/pdfft?md5=a349c8d5d0487701d45669b8c9e8adbf&pid=1-s2.0-S2666498423001357-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138993047","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Protect the oceans from Japan's radioisotope dumping 保护海洋免受日本放射性同位素倾倒的危害
IF 12.6 1区 环境科学与生态学
Environmental Science and Ecotechnology Pub Date : 2023-12-18 DOI: 10.1016/j.ese.2023.100369
Chengjun Li, Huan Zhong, Lingyu Meng, Mengjie Wu, Wenjing Ning, Su Shiung Lam, Jun Luo, Christian Sonne
{"title":"Protect the oceans from Japan's radioisotope dumping","authors":"Chengjun Li,&nbsp;Huan Zhong,&nbsp;Lingyu Meng,&nbsp;Mengjie Wu,&nbsp;Wenjing Ning,&nbsp;Su Shiung Lam,&nbsp;Jun Luo,&nbsp;Christian Sonne","doi":"10.1016/j.ese.2023.100369","DOIUrl":"10.1016/j.ese.2023.100369","url":null,"abstract":"","PeriodicalId":34434,"journal":{"name":"Environmental Science and Ecotechnology","volume":null,"pages":null},"PeriodicalIF":12.6,"publicationDate":"2023-12-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2666498423001345/pdfft?md5=bf73c09d30618b52b378b243ca87ed09&pid=1-s2.0-S2666498423001345-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139015830","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Enhancing photocatalytic CO2 reduction with TiO2-based materials: Strategies, mechanisms, challenges, and perspectives 利用基于二氧化钛的材料加强光催化二氧化碳还原:战略、机制、挑战和前景
IF 12.6 1区 环境科学与生态学
Environmental Science and Ecotechnology Pub Date : 2023-12-16 DOI: 10.1016/j.ese.2023.100368
Zhimin Yuan , Xianglin Zhu , Xianqiang Gao , Changhua An , Zheng Wang , Cheng Zuo , Dionysios D. Dionysiou , Hong He , Zaiyong Jiang
{"title":"Enhancing photocatalytic CO2 reduction with TiO2-based materials: Strategies, mechanisms, challenges, and perspectives","authors":"Zhimin Yuan ,&nbsp;Xianglin Zhu ,&nbsp;Xianqiang Gao ,&nbsp;Changhua An ,&nbsp;Zheng Wang ,&nbsp;Cheng Zuo ,&nbsp;Dionysios D. Dionysiou ,&nbsp;Hong He ,&nbsp;Zaiyong Jiang","doi":"10.1016/j.ese.2023.100368","DOIUrl":"10.1016/j.ese.2023.100368","url":null,"abstract":"<div><p>The concentration of atmospheric CO<sub>2</sub> has exceeded 400 ppm, surpassing its natural variability and raising concerns about uncontrollable shifts in the carbon cycle, leading to significant climate and environmental impacts. A promising method to balance carbon levels and mitigate atmospheric CO<sub>2</sub> rise is through photocatalytic CO<sub>2</sub> reduction. Titanium dioxide (TiO<sub>2</sub>), renowned for its affordability, stability, availability, and eco-friendliness, stands out as an exemplary catalyst in photocatalytic CO<sub>2</sub> reduction. Various strategies have been proposed to modify TiO<sub>2</sub> for photocatalytic CO<sub>2</sub> reduction and improve catalytic activity and product selectivity. However, few studies have systematically summarized these strategies and analyzed their advantages, disadvantages, and current progress. Here, we comprehensively review recent advancements in TiO<sub>2</sub> engineering, focusing on crystal engineering, interface design, and reactive site construction to enhance photocatalytic efficiency and product selectivity. We discuss how modifications in TiO<sub>2</sub>'s optical characteristics, carrier migration, and active site design have led to varied and selective CO<sub>2</sub> reduction products. These enhancements are thoroughly analyzed through experimental data and theoretical calculations. Additionally, we identify current challenges and suggest future research directions, emphasizing the role of TiO<sub>2</sub>-based materials in understanding photocatalytic CO<sub>2</sub> reduction mechanisms and in designing effective catalysts. This review is expected to contribute to the global pursuit of carbon neutrality by providing foundational insights into the mechanisms of photocatalytic CO<sub>2</sub> reduction with TiO<sub>2</sub>-based materials and guiding the development of efficient photocatalysts.</p></div>","PeriodicalId":34434,"journal":{"name":"Environmental Science and Ecotechnology","volume":null,"pages":null},"PeriodicalIF":12.6,"publicationDate":"2023-12-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2666498423001333/pdfft?md5=af73bd14b8adedefc9fbc700d2bf8c20&pid=1-s2.0-S2666498423001333-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"138987199","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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