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Perovskite Solar Cells and Light Emitting Diodes: Materials Chemistry, Device Physics and Relationship 钙钛矿太阳能电池与发光二极管：材料化学、器件物理及其关系
IF 62.1 1区 化学
Chemical Reviews Pub Date : 2025-05-21 DOI: 10.1021/acs.chemrev.4c00663
Ligang Yuan, Qifan Xue, Feng Wang, Ning Li, Geoffrey I. N. Waterhouse, Christoph J. Brabec, Feng Gao, Keyou Yan
{"title":"Perovskite Solar Cells and Light Emitting Diodes: Materials Chemistry, Device Physics and Relationship","authors":"Ligang Yuan, Qifan Xue, Feng Wang, Ning Li, Geoffrey I. N. Waterhouse, Christoph J. Brabec, Feng Gao, Keyou Yan","doi":"10.1021/acs.chemrev.4c00663","DOIUrl":"https://doi.org/10.1021/acs.chemrev.4c00663","url":null,"abstract":"Solution-processed perovskite solar cells (PSCs) and perovskite light emitting diodes (PeLEDs) represent promising next-generation optoelectronic technologies. This Review summarizes recent advancements in the application of metal halide perovskite materials for PSC and PeLED devices to address the efficiency, stability and scalability issues. Emphasis is placed on material chemistry strategies used to control and engineer the composition, deposition process, interface and micro-nanostructure in solution-processed perovskite films, leading to high-quality crystalline thin films for optimal device performance. Furthermore, we retrospectively compare the device physics of PSCs and PeLEDs, their working principles and their energy loss mechanisms, examining the similarities and differences between the two types of devices. The reciprocity relationship suggests that a great PSC should also be a great PeLED, motivating the search for interconverting photoelectric bifunctional devices with maximum radiative recombination and negligible non-radiative recombination. Specific requirements of PSCs and PeLEDs in terms of bandgap, thickness, band alignment and charge transport to achieve this target are discussed in detail. Further challenges and issues are also illustrated, together with prospects for future development. Understanding these fundamentals, embracing recent breakthroughs and exploring future prospects pave the way toward the rational design and development of high-performance PSC and PeLED devices.","PeriodicalId":32,"journal":{"name":"Chemical Reviews","volume":"2 1","pages":""},"PeriodicalIF":62.1,"publicationDate":"2025-05-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144114501","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Residue-Specific Incorporation of Noncanonical Amino Acids in Auxotrophic Hosts: Quo Vadis? 非规范氨基酸在营养不良宿主体内的残留特异性掺入：现状？
IF 51.4 1区 化学
Chemical Reviews Pub Date : 2025-05-16 DOI: 10.1021/acs.chemrev.4c0028010.1021/acs.chemrev.4c00280
Žana Marin, Claudia Lacombe, Simindokht Rostami, Arshia Arasteh Kani, Andrea Borgonovo, Monika Cserjan-Puschmann, Jürgen Mairhofer, Gerald Striedner and Birgit Wiltschi*, 
{"title":"Residue-Specific Incorporation of Noncanonical Amino Acids in Auxotrophic Hosts: Quo Vadis?","authors":"Žana Marin,&nbsp;Claudia Lacombe,&nbsp;Simindokht Rostami,&nbsp;Arshia Arasteh Kani,&nbsp;Andrea Borgonovo,&nbsp;Monika Cserjan-Puschmann,&nbsp;Jürgen Mairhofer,&nbsp;Gerald Striedner and Birgit Wiltschi*,&nbsp;","doi":"10.1021/acs.chemrev.4c0028010.1021/acs.chemrev.4c00280","DOIUrl":"https://doi.org/10.1021/acs.chemrev.4c00280https://doi.org/10.1021/acs.chemrev.4c00280","url":null,"abstract":"<p >The residue-specific incorporation of noncanonical amino acids in auxotrophic hosts allows the global exchange of a canonical amino acid with its noncanonical analog. Noncanonical amino acids are not encoded by the standard genetic code, but they carry unique side chain chemistries, e.g., to perform bioorthogonal conjugation reactions or to manipulate the physicochemical properties of a protein such as folding and stability. The method was introduced nearly 70 years ago and is still in widespread use because of its simplicity and robustness. In our study, we review the trends in the field during the last two decades. We give an overview of the application of the method for artificial post-translational protein modifications and the selective functionalization and directed immobilization of proteins. We highlight the trends in the use of noncanonical amino acids for the analysis of nascent proteomes and the engineering of enzymes and biomaterials, and the progress in the biosynthesis of amino acid analogs. We also discuss the challenges for the scale-up of the technique.</p>","PeriodicalId":32,"journal":{"name":"Chemical Reviews","volume":"125 10","pages":"4840–4932 4840–4932"},"PeriodicalIF":51.4,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acs.chemrev.4c00280","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144146633","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Residue-Specific Incorporation of Noncanonical Amino Acids in Auxotrophic Hosts: Quo Vadis? 非规范氨基酸在营养不良宿主体内的残留特异性掺入：现状？
IF 62.1 1区 化学
Chemical Reviews Pub Date : 2025-05-16 DOI: 10.1021/acs.chemrev.4c00280
Žana Marin, Claudia Lacombe, Simindokht Rostami, Arshia Arasteh Kani, Andrea Borgonovo, Monika Cserjan-Puschmann, Jürgen Mairhofer, Gerald Striedner, Birgit Wiltschi
{"title":"Residue-Specific Incorporation of Noncanonical Amino Acids in Auxotrophic Hosts: Quo Vadis?","authors":"Žana Marin, Claudia Lacombe, Simindokht Rostami, Arshia Arasteh Kani, Andrea Borgonovo, Monika Cserjan-Puschmann, Jürgen Mairhofer, Gerald Striedner, Birgit Wiltschi","doi":"10.1021/acs.chemrev.4c00280","DOIUrl":"https://doi.org/10.1021/acs.chemrev.4c00280","url":null,"abstract":"The residue-specific incorporation of noncanonical amino acids in auxotrophic hosts allows the global exchange of a canonical amino acid with its noncanonical analog. Noncanonical amino acids are not encoded by the standard genetic code, but they carry unique side chain chemistries, e.g., to perform bioorthogonal conjugation reactions or to manipulate the physicochemical properties of a protein such as folding and stability. The method was introduced nearly 70 years ago and is still in widespread use because of its simplicity and robustness. In our study, we review the trends in the field during the last two decades. We give an overview of the application of the method for artificial post-translational protein modifications and the selective functionalization and directed immobilization of proteins. We highlight the trends in the use of noncanonical amino acids for the analysis of nascent proteomes and the engineering of enzymes and biomaterials, and the progress in the biosynthesis of amino acid analogs. We also discuss the challenges for the scale-up of the technique.","PeriodicalId":32,"journal":{"name":"Chemical Reviews","volume":"77 1","pages":""},"PeriodicalIF":62.1,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144066773","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Selective Noncovalent Catalysis with Small Molecules 小分子选择性非共价催化
IF 62.1 1区 化学
Chemical Reviews Pub Date : 2025-05-15 DOI: 10.1021/acs.chemrev.5c00121
Marcus H. Sak, Eric N. Jacobsen
{"title":"Selective Noncovalent Catalysis with Small Molecules","authors":"Marcus H. Sak, Eric N. Jacobsen","doi":"10.1021/acs.chemrev.5c00121","DOIUrl":"https://doi.org/10.1021/acs.chemrev.5c00121","url":null,"abstract":"In catalysis, selectivity reflects the energetic preference for the formation of a single product out of multiple possible reaction outcomes. The classic steric biasing approach in small-molecule catalysis employs steric destabilization of the undesired competing transition states to achieve energetic differentiation. In contrast, enzymes achieve high levels of rate acceleration and selectivity by accelerating the pathway leading to the major product, often through networks of attractive, stabilizing noncovalent interactions. This Review showcases selective noncovalent catalysis (NCC) with small organic molecules and transition-metal complexes. We collect and highlight examples whereby selectivity was documented experimentally to arise from selective stabilization of the transition state leading to the major product. We also showcase how synergistic experimental and computational investigations have enabled the elucidation of specific noncovalent interactions responsible for selective stabilization.","PeriodicalId":32,"journal":{"name":"Chemical Reviews","volume":"130 1","pages":""},"PeriodicalIF":62.1,"publicationDate":"2025-05-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144066775","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 51.4 1区 化学
Chemical Reviews Pub Date : 2025-05-14
Raavi, Angela N. Koehler and Arturo J. Vegas*, 
{"title":"","authors":"Raavi,&nbsp;Angela N. Koehler and Arturo J. Vegas*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":32,"journal":{"name":"Chemical Reviews","volume":"125 9","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":51.4,"publicationDate":"2025-05-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acs.chemrev.4c00469","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144446305","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Photolithographic Patterning of Organic Semiconductors for Organic Field-Effect Transistors. 用于有机场效应晶体管的有机半导体光刻图像化。
IF 62.1 1区 化学
Chemical Reviews Pub Date : 2025-05-14 DOI: 10.1021/acs.chemrev.4c00446
Yang Li,Renzhong Chen
{"title":"Photolithographic Patterning of Organic Semiconductors for Organic Field-Effect Transistors.","authors":"Yang Li,Renzhong Chen","doi":"10.1021/acs.chemrev.4c00446","DOIUrl":"https://doi.org/10.1021/acs.chemrev.4c00446","url":null,"abstract":"Over the past 25 years, three major photolithography strategies have been employed for patterning organic semiconductors in organic field-effect transistors (OFETs): modified photolithography (MPL), orthogonal photolithography (OPL), and direct photolithography (DPL). This Review examines key studies to highlight the strengths and weaknesses of each strategy. Two DPL methods, in particular, show great promise: organic azide/diazirine cross-linkers (Z-cross-linkers) and UV-cross-linkable organic semiconducting blends (X-blends). These methods not only simplify the photolithography process significantly but also enhance the chemical and physical resistance of patterned organic semiconductors against photolithographic chemicals and tandem solution-depositions. Consequently, these advancements enable the fabrication of organic integrated circuits entirely through solution processes. In conclusion, photolithography of organic semiconductors serves a dual purpose: it facilitates the patterning of active layers for OFETs and acts as an enabling technology for fabricating sophisticated and cost-effective organic integrated circuits.","PeriodicalId":32,"journal":{"name":"Chemical Reviews","volume":"13 1","pages":""},"PeriodicalIF":62.1,"publicationDate":"2025-05-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143945569","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 51.4 1区 化学
Chemical Reviews Pub Date : 2025-05-14
{"title":"","authors":"","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":32,"journal":{"name":"Chemical Reviews","volume":"125 9","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":51.4,"publicationDate":"2025-05-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/crv125i009_1934703","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144342027","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 51.4 1区 化学
Chemical Reviews Pub Date : 2025-05-14
Tong Jiang, Jinghong Zhang, Moritz K. A. Baumgarten, Meng-Fu Chen, Hieu Q. Dinh, Aadithya Ganeshram, Nishad Maskara, Anton Ni and Joonho Lee*, 
{"title":"","authors":"Tong Jiang,&nbsp;Jinghong Zhang,&nbsp;Moritz K. A. Baumgarten,&nbsp;Meng-Fu Chen,&nbsp;Hieu Q. Dinh,&nbsp;Aadithya Ganeshram,&nbsp;Nishad Maskara,&nbsp;Anton Ni and Joonho Lee*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":32,"journal":{"name":"Chemical Reviews","volume":"125 9","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":51.4,"publicationDate":"2025-05-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acs.chemrev.4c00508","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144446308","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Photolithographic Patterning of Organic Semiconductors for Organic Field-Effect Transistors 用于有机场效应晶体管的有机半导体光刻图像化
IF 51.4 1区 化学
Chemical Reviews Pub Date : 2025-05-14 DOI: 10.1021/acs.chemrev.4c0044610.1021/acs.chemrev.4c00446
Yang Li*,  and , Renzhong Chen, 
{"title":"Photolithographic Patterning of Organic Semiconductors for Organic Field-Effect Transistors","authors":"Yang Li*,&nbsp; and ,&nbsp;Renzhong Chen,&nbsp;","doi":"10.1021/acs.chemrev.4c0044610.1021/acs.chemrev.4c00446","DOIUrl":"https://doi.org/10.1021/acs.chemrev.4c00446https://doi.org/10.1021/acs.chemrev.4c00446","url":null,"abstract":"<p >Over the past 25 years, three major photolithography strategies have been employed for patterning organic semiconductors in organic field-effect transistors (OFETs): modified photolithography (MPL), orthogonal photolithography (OPL), and direct photolithography (DPL). This Review examines key studies to highlight the strengths and weaknesses of each strategy. Two DPL methods, in particular, show great promise: organic azide/diazirine cross-linkers (Z-cross-linkers) and UV-cross-linkable organic semiconducting blends (X-blends). These methods not only simplify the photolithography process significantly but also enhance the chemical and physical resistance of patterned organic semiconductors against photolithographic chemicals and tandem solution-depositions. Consequently, these advancements enable the fabrication of organic integrated circuits entirely through solution processes. In conclusion, photolithography of organic semiconductors serves a dual purpose: it facilitates the patterning of active layers for OFETs and acts as an enabling technology for fabricating sophisticated and cost-effective organic integrated circuits.</p>","PeriodicalId":32,"journal":{"name":"Chemical Reviews","volume":"125 10","pages":"4933–4973 4933–4973"},"PeriodicalIF":51.4,"publicationDate":"2025-05-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144146548","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 51.4 1区 化学
Chemical Reviews Pub Date : 2025-05-14
Shuai Liu, Jun Zhou, Lu Yu, Yingle Liu, Yangen Huang, Yao Ouyang, Guo-Kai Liu, Xiu-Hua Xu and Norio Shibata, 
{"title":"","authors":"Shuai Liu,&nbsp;Jun Zhou,&nbsp;Lu Yu,&nbsp;Yingle Liu,&nbsp;Yangen Huang,&nbsp;Yao Ouyang,&nbsp;Guo-Kai Liu,&nbsp;Xiu-Hua Xu and Norio Shibata,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":32,"journal":{"name":"Chemical Reviews","volume":"125 9","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":51.4,"publicationDate":"2025-05-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acs.chemrev.4c00661","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144446309","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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