Advanced Energy and Sustainability Research最新文献_第5页

A Novel Methodology for the Accelerated Desalination of Seawater Utilizing Up- and Down-Conversion Phosphors 利用上下转换荧光粉加速海水淡化的新方法

IF 6.2

Advanced Energy and Sustainability Research Pub Date : 2025-01-13 DOI: 10.1002/aesr.202400242

Ernesto Valadez-Renteria, Jorge Oliva, Haggeo Desirena, Christian Gomez-Solis, Vicente Rodriguez-Gonzalez

{"title":"A Novel Methodology for the Accelerated Desalination of Seawater Utilizing Up- and Down-Conversion Phosphors","authors":"Ernesto Valadez-Renteria, Jorge Oliva, Haggeo Desirena, Christian Gomez-Solis, Vicente Rodriguez-Gonzalez","doi":"10.1002/aesr.202400242","DOIUrl":"https://doi.org/10.1002/aesr.202400242","url":null,"abstract":"Solar evaporators are fabricated by coating coconut/agave fibers with graphene. Those ones are utilized to desalinate seawater brought from Vallarta beach, Mexico. The graphene-based evaporators exposed to sunlight produce a maximum evaporation rate/efficiency of 2.13 kg m−2 h−1/83%. The addition of Fe2O3 particles to the evaporators enhances the evaporation rate/efficiency up to 2.36 kg m−2 h−1/88.5%. The higher presence of oxygen vacancies defects in the evaporators made with Fe2O3 improves the absorption of light in the UV-Vis range, which in turn, accelerates the desalination of seawater. Moreover, the performance of the solar evaporators is evaluated in absence of solar light. In this case, upconversion (UC) and downconversion (DC) phosphors are attached to the evaporators and such phosphors are excited with near-infrared (980 nm) or ultraviolet (360 nm) light. Consequently, green light is produced by DC/UC, which is absorbed by the evaporators to be heated and the seawater evaporation is induced. The maximum evaporation rate/efficiency produced by the evaporators is 0.738 kg m−2 h−1/84.9%. In general, this research offers a novel strategy to continue the desalination of seawater in absence of solar light or in cloudy days. This can be useful to design new types of desalination plants without using complex/expensive filtration systems.","PeriodicalId":29794,"journal":{"name":"Advanced Energy and Sustainability Research","volume":"6 2","pages":""},"PeriodicalIF":6.2,"publicationDate":"2025-01-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/aesr.202400242","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143362852","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Cyano-Borazine Photosensitizers for Dye-Sensitized Solar Cells 染料敏化太阳能电池用氰硼嗪光敏剂

IF 6.2

Advanced Energy and Sustainability Research Pub Date : 2025-01-13 DOI: 10.1002/aesr.202400344

Sanchari Chowdhury, Vivek Chandrakant Wakchure, El Czar Galleposo, Davide Bonifazi, Rubén D. Costa

{"title":"Cyano-Borazine Photosensitizers for Dye-Sensitized Solar Cells","authors":"Sanchari Chowdhury, Vivek Chandrakant Wakchure, El Czar Galleposo, Davide Bonifazi, Rubén D. Costa","doi":"10.1002/aesr.202400344","DOIUrl":"https://doi.org/10.1002/aesr.202400344","url":null,"abstract":"Implementing novel metal-free and strongly absorbing donor–acceptor sensitizers without carboxylic acid anchoring groups are still a frontier in dye-sensitized solar cells (DSSCs). Herein, the facile synthesis of a strongly absorbing sensitizer combining three 1,1,4,4-tetracyanobuta-1,3-diene (TCBD) anchoring moieties with a borazine core instead of the classical cyano anchoring groups, such as tetracyanoquinodimethane (TCNQ) and tetracyanoethylene (TCNE), and the dimethyl-phenyl amino donor group, is disclosed. This results in a 1.6-fold increase in solar energy conversion efficiency compared to DSSCs with the reference sensitizers (TCBD-dimethyl-amino-phenyl core) and the prior art cyano-sensitizers with TCNE and TCNG anchors. The advantages of the TCBD-borazine design are twofold: 1) threefold increase in absorption extinction coefficient as well as 2) a reduction in back electron transfer and aggregation behavior upon dye adsorption onto the semiconducting electrode, resulting in 45% and 23% improvement in open-circuit voltage (Voc) and short-circuit current density (Jsc), respectively, compared to those of the prior art. Overall, this work highlights an easy-to-design of cyano-sensitizer that results in a significant improvement of solar energy conversion when using borazine frameworks for the first time.","PeriodicalId":29794,"journal":{"name":"Advanced Energy and Sustainability Research","volume":"6 5","pages":""},"PeriodicalIF":6.2,"publicationDate":"2025-01-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/aesr.202400344","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143909140","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

From Graphene Oxide to N-Doped Graphene: Understanding the Doping Process 从氧化石墨烯到氮掺杂石墨烯：了解掺杂过程

IF 6.2

Advanced Energy and Sustainability Research Pub Date : 2025-01-06 DOI: 10.1002/aesr.202400310

José Manuel Ruiz-Marizcal, José Israel Paez-Ornelas, Héctor Noé Fernández-Escamilla, Eduardo Antonio Murillo-Bracamontes, Gabriel Alonso-Núñez, Eduardo G. Perez-Tijerina, Noboru Takeuchi, José Manuel Romo-Herrera

{"title":"From Graphene Oxide to N-Doped Graphene: Understanding the Doping Process","authors":"José Manuel Ruiz-Marizcal, José Israel Paez-Ornelas, Héctor Noé Fernández-Escamilla, Eduardo Antonio Murillo-Bracamontes, Gabriel Alonso-Núñez, Eduardo G. Perez-Tijerina, Noboru Takeuchi, José Manuel Romo-Herrera","doi":"10.1002/aesr.202400310","DOIUrl":"https://doi.org/10.1002/aesr.202400310","url":null,"abstract":"N-doped carbon nanostructures have gained attention as an alternative electrocatalyst for diverse reactions. They are making attractive the scalable methods to achieve enough material. However, optimizing the appropriate nitrogen species in the N-doped graphitic electrocatalysts is critical. Here, the N-doping process to obtain N-doped graphene starting from graphene oxide (GO) as the precursor to contributing toward this goal is explored. The role of doping temperatures and doping times on nitrogen incorporation into the graphene sheets, the subsequent desorption, and the influence of the oxygen (O) species from the GO during the N-doping process are analyzed. The experimental evidence is combined with first-principles density functional theory calculations to understand key characteristics of the N-doping process, particularly emphasizing the proportion of N species obtained. Finally, the critical sensitivity to N species proportions present in the electrocatalysts is illustrated by evaluating the activity and selectivity for the oxygen reduction reaction with a set of three different samples designed.","PeriodicalId":29794,"journal":{"name":"Advanced Energy and Sustainability Research","volume":"6 4","pages":""},"PeriodicalIF":6.2,"publicationDate":"2025-01-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/aesr.202400310","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143770498","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Ameliorating Device Efficiency of Perovskite Solar Cells via Low-Cost Interfacial Modification between SnO2 and Perovskite Absorber 通过低成本改性SnO2与钙钛矿吸收体之间的界面改善钙钛矿太阳能电池的器件效率

IF 6.2

Advanced Energy and Sustainability Research Pub Date : 2025-01-05 DOI: 10.1002/aesr.202570001

Ching-Ying Wang, Sheng-Hsiung Yang

引用次数: 0

Data-Driven Innovation in Metal-Organic Frameworks Photocatalysis: Bridging Gaps for CO2 Capture and Conversion with FAIR Principles 数据驱动的金属有机框架光催化创新：用公平原则弥合二氧化碳捕获和转化的差距

IF 6.2

Advanced Energy and Sustainability Research Pub Date : 2024-12-30 DOI: 10.1002/aesr.202400325

Claudia Bizzarri, Manuel Tsotsalas

{"title":"Data-Driven Innovation in Metal-Organic Frameworks Photocatalysis: Bridging Gaps for CO2 Capture and Conversion with FAIR Principles","authors":"Claudia Bizzarri, Manuel Tsotsalas","doi":"10.1002/aesr.202400325","DOIUrl":"https://doi.org/10.1002/aesr.202400325","url":null,"abstract":"Metal-organic frameworks (MOFs) have emerged as key materials for carbon capture and conversion, particularly in photocatalytic CO2 reduction. However, inconsistent reporting of essential parameters in the literature hinders informed decisions about material selection and optimization. This perspective highlights the need for a user-friendly, centralized database supported by automated data extraction using natural language processing tools to streamline comparisons of MOF materials. By consolidating crucial data from scientific literature, such a database promotes efficient decision-making in material selection for CO2 capture and utilization. Emphasizing the significance of open-source initiatives and the principles of FAIR data—ensuring data are Findable, Accessible, Interoperable, and Reusable—a collaborative approach to data management and sharing is advocated for. Making the database-accessible worldwide enhances data quality and reliability, fostering innovation and progress in CO2 capture and conversion using MOF materials. Additionally, such databases are valuable in creating artificial intelligence tools to assist researchers in the discovery and synthesis of MOF materials for CO2 capture and conversion.","PeriodicalId":29794,"journal":{"name":"Advanced Energy and Sustainability Research","volume":"6 5","pages":""},"PeriodicalIF":6.2,"publicationDate":"2024-12-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/aesr.202400325","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143909546","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Optical Properties of Spin-Coated Solution Processed MoS2 旋转镀膜溶液处理二硫化钼的光学性质

IF 6.2

Advanced Energy and Sustainability Research Pub Date : 2024-12-28 DOI: 10.1002/aesr.202400392

Muntaser Almansoori, Sabina Abdul Hadi, Ayman Rezk, Khalid Askar, Ammar Nayfeh

引用次数: 0

On the Reversibility of Sustainable Symmetric Aqueous Organic Redox Flow Batteries 可持续对称有机水氧化还原液流电池的可逆性研究

IF 6.2

Advanced Energy and Sustainability Research Pub Date : 2024-12-27 DOI: 10.1002/aesr.202400324

Saeed Mardi, Ujwala Ail, Mikhail Vagin, Jaywant Phopase, Reverant Crispin

引用次数: 0

Novel Quantification Method for Lithium Ion Battery Electrolyte Solvents in Aqueous Recycling Samples Using Solid-Phase Extraction/Gas Chromatography-Flame Ionization Detection 固相萃取/气相色谱-火焰电离检测法定量回收水样品中锂离子电池电解质溶剂

IF 6.2

Advanced Energy and Sustainability Research Pub Date : 2024-12-24 DOI: 10.1002/aesr.202400311

Julius Buchmann, Yixin Song, Simon Wiemers-Meyer, Martin Winter, Sascha Nowak

{"title":"Novel Quantification Method for Lithium Ion Battery Electrolyte Solvents in Aqueous Recycling Samples Using Solid-Phase Extraction/Gas Chromatography-Flame Ionization Detection","authors":"Julius Buchmann, Yixin Song, Simon Wiemers-Meyer, Martin Winter, Sascha Nowak","doi":"10.1002/aesr.202400311","DOIUrl":"https://doi.org/10.1002/aesr.202400311","url":null,"abstract":"Efficient recycling processes of lithium ion batteries are critical for advancing the sustainability of this technology. Yet, the quantitative analysis of potential electrolyte residues in wastewaters generated in the recycling process can be challenging. This study introduces a robust method that combines solid-phase extraction with gas chromatography-flame ionization detection for quantifying organic carbonate electrolyte solvents and their degradation products in aqueous samples. A quantitative extraction of all target analytes is achieved using the polystyrene-divinylbenzene-based stationary phase LiChrolut EN. Method optimization and limitations are evaluated by varying mass loading, load and elution volume, enabling preconcentration factors >250 for linear and oligomeric carbonates. More hydrophilic cyclic carbonates exhibit lower preconcentration potential due to reduced retention on the cartridge. However, limits of quantification in the water sample in a range of a few hundred ppb are achieved for cyclic carbonates (186 ppb for ethylene carbonate, 119 ppb for vinylene carbonate) and down to the single-digit ppb range for linear and oligomeric carbonates. Additionally, effective matrix elimination is demonstrated through the removal of ionic compounds, such as conductive salts, while the extraction efficiency is independent of the matrix. In conclusion, a robust quantification method is developed, suitable for monitoring wastewater treatment processes and environmental samples.","PeriodicalId":29794,"journal":{"name":"Advanced Energy and Sustainability Research","volume":"6 2","pages":""},"PeriodicalIF":6.2,"publicationDate":"2024-12-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/aesr.202400311","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143363055","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Sustainable Production of Graphene from Solar-Driven Expanded Graphite 由太阳能驱动的膨胀石墨可持续生产石墨烯

IF 6.2

Advanced Energy and Sustainability Research Pub Date : 2024-12-24 DOI: 10.1002/aesr.202400274

Shanavas Shajahan, Rami Elkaffas, Dhinesh Babu Velusamy, Dalaver H. Anjum, Yarjan Abdul Samad

{"title":"Sustainable Production of Graphene from Solar-Driven Expanded Graphite","authors":"Shanavas Shajahan, Rami Elkaffas, Dhinesh Babu Velusamy, Dalaver H. Anjum, Yarjan Abdul Samad","doi":"10.1002/aesr.202400274","DOIUrl":"https://doi.org/10.1002/aesr.202400274","url":null,"abstract":"\u0000Scalable synthesis of graphene sheets is challenging due to the complex production processes. Few-layered graphene sheets with high lateral sizes (4–5 μm) through a state-of-the-art solar irradiation-driven liquid-phase exfoliation technique are achieved. The sunlight is directly used on the intercalated graphite flakes for just 0.5 s to achieve the graphite expansion. Using focused sunlight makes our solar expansion technique sustainable with zero energy demand (0 J). The total energy spent to produce 1 kg of graphene through this technique is only around 2.135 MJ. The produced graphene sheets show significant electrical conductivity (1586 S cm−1) and high in-plane thermal conductivity (196.3 W mK−1). The electromagnetic interference (EMI) shielding properties of solar graphene are evaluated in the X-band region, and it shows a very high shielding effectiveness of about 71.5 dB at a thickness of ≈80 μm with an absolute EMI shielding effectiveness of about 11983.7 dB cm2 g−1. Overall, this work provides a viable approach for the efficient, scalable production of graphene with reduced energy consumption and cost, contributing to the sustainable production of graphene.","PeriodicalId":29794,"journal":{"name":"Advanced Energy and Sustainability Research","volume":"6 3","pages":""},"PeriodicalIF":6.2,"publicationDate":"2024-12-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/aesr.202400274","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143555212","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Recent Advances in Iron-Containing Perovskites for Supercapacitors 超级电容器用含铁钙钛矿的研究进展

IF 6.2

Advanced Energy and Sustainability Research Pub Date : 2024-12-24 DOI: 10.1002/aesr.202400289

Celal Avcıoğlu, Suna Avcıoğlu

{"title":"Recent Advances in Iron-Containing Perovskites for Supercapacitors","authors":"Celal Avcıoğlu, Suna Avcıoğlu","doi":"10.1002/aesr.202400289","DOIUrl":"https://doi.org/10.1002/aesr.202400289","url":null,"abstract":"The growing energy demands in transportation and portable electronics necessitate advancements in energy storage technologies. Supercapacitors, with their exceptional power density, rapid charge–discharge capabilities, and long cycle life, provide a compelling solution for energy storage applications. However, their inherent low energy density remains a persistent challenge. To overcome this limitation, perovskite oxides, particularly those containing iron, have emerged as promising electrode materials. These materials leverage their unique structure, compositional flexibility, rich redox chemistry, and pseudocapacitive attributes. This concise overview aims to provide insights into the development of iron-containing perovskite oxides and their design principles. The discussion covers fundamental aspects of supercapacitors, iron-containing perovskite structures, synthetic methodologies, defect engineering, and the construction of composites. The overview concludes by providing a perspective, particularly regarding the challenges in designing efficient and stable supercapacitors based on iron-containing perovskite oxides.","PeriodicalId":29794,"journal":{"name":"Advanced Energy and Sustainability Research","volume":"6 3","pages":""},"PeriodicalIF":6.2,"publicationDate":"2024-12-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/aesr.202400289","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143555214","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0