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Leucite-Coesite ceramic coatings for metal-based dental restorations: Structural and thermoluminescence analysis 金属基牙齿修复体用白晶石-钴石陶瓷涂层:结构和热释光分析
IF 2.8 3区 物理与天体物理
Radiation Physics and Chemistry Pub Date : 2025-06-04 DOI: 10.1016/j.radphyschem.2025.113037
Esma Başak Gül Aygün , A. Barad , Abeer S. Altowyan , J. Hakami , M. Topaksu , N. Can
{"title":"Leucite-Coesite ceramic coatings for metal-based dental restorations: Structural and thermoluminescence analysis","authors":"Esma Başak Gül Aygün ,&nbsp;A. Barad ,&nbsp;Abeer S. Altowyan ,&nbsp;J. Hakami ,&nbsp;M. Topaksu ,&nbsp;N. Can","doi":"10.1016/j.radphyschem.2025.113037","DOIUrl":"10.1016/j.radphyschem.2025.113037","url":null,"abstract":"<div><h3>Leucite</h3><div>and Coesite-based ceramic materials have garnered significant attention for their potential use in dental restorations due to their enhanced mechanical strength, thermal stability, and aesthetic properties. This study investigates the structural, microstructural, and thermoluminescence (TL) properties of a Leucite-Coesite ceramic coating designed for metal-based dental applications. A comprehensive characterization was performed using X-ray diffraction (XRD), scanning electron microscopy (SEM), Fourier-transform infrared spectroscopy (FTIR), and TL analysis to assess crystallinity, phase composition, and luminescence behavior. Energy-dispersive X-ray spectroscopy (EDX) confirmed the presence of key elements, while FTIR revealed characteristic Si–O and Al–O vibrational modes, indicating a stable aluminosilicate structure. TL analysis revealed a dose-dependent response with distinct glow peaks, suggesting potential applications in radiation dosimetry. The TL intensity exhibited a moderate increase with heating rate (∼10 %), deviating from classical first-order kinetics. This behavior may reflect non-classical recombination mechanisms involving spatial correlations between traps and recombination centers. Glow Curve Deconvolution (GCD) analysis identified nine distinct TL peaks with activation energy values ranging from 0.80 eV to 1.42 eV. These results indicate the presence of well-separated kinetic components with consistent parameter estimates. These findings highlight the complex charge carrier dynamics in Leucite-Coesite ceramics and underscore their potential for both restorative dentistry and radiation dosimetry.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"237 ","pages":"Article 113037"},"PeriodicalIF":2.8,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144221724","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Design and evaluation of borate glasses doped with multiple components for effective low-energy radiation shielding 多组分掺杂硼酸盐玻璃的低能量有效屏蔽设计与评价
IF 2.8 3区 物理与天体物理
Radiation Physics and Chemistry Pub Date : 2025-06-04 DOI: 10.1016/j.radphyschem.2025.113030
M.I. Sayyed , S. Yasmin , M.R.I. Faruque , S. Abdullah , K.A. Mahmoud , M.U. Khandaker , Yasser Maghrbi , M. Elsafi
{"title":"Design and evaluation of borate glasses doped with multiple components for effective low-energy radiation shielding","authors":"M.I. Sayyed ,&nbsp;S. Yasmin ,&nbsp;M.R.I. Faruque ,&nbsp;S. Abdullah ,&nbsp;K.A. Mahmoud ,&nbsp;M.U. Khandaker ,&nbsp;Yasser Maghrbi ,&nbsp;M. Elsafi","doi":"10.1016/j.radphyschem.2025.113030","DOIUrl":"10.1016/j.radphyschem.2025.113030","url":null,"abstract":"<div><div>The present study aims at examining the low-energy radiation shielding properties of a Bi<sub>2</sub>O<sub>3</sub>- and ZnO-doped borosilicate [(61-x) B<sub>2</sub>O<sub>3</sub>–10ZnO–10BaO–5TiO<sub>2</sub>-(14+x) Bi<sub>2</sub>O<sub>3</sub>; x = 4, 8, 12, and 16 mol%] glass system. The mechanical characteristics of the produced glasses were evaluated using the Makishima–Mackenzie theory. The study shows that substituting part of B<sub>2</sub>O<sub>3</sub> with Bi<sub>2</sub>O<sub>3</sub> reduces the microhardness and mechanical moduli of the glasses.</div><div>Additionally, radiation shielding factors were determined to investigate the relationship between Bi<sub>2</sub>O<sub>3</sub> and B<sub>2</sub>O<sub>3</sub> content and the glasses' low-energy gamma-ray shielding performance, as well as the influence of the radiation source energy on the glass properties. The results demonstrated a positive correlation between increasing Bi<sub>2</sub>O<sub>3</sub> concentration and the linear attenuation coefficients (LAC) of the glasses.</div><div>The glass sample containing 18 mol% Bi<sub>2</sub>O<sub>3</sub> led to the lowest LAC values, whereas the sample with 30 mol% Bi<sub>2</sub>O<sub>3</sub> led to the highest. Furthermore, the mean free path (MFP) of the glasses was compared to that of commercial glasses to assess their effectiveness in low-energy radiation protection. The glass with the highest Bi<sub>2</sub>O<sub>3</sub> content had the lowest MFP and thus provided better protection than some commercial alternatives.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"237 ","pages":"Article 113030"},"PeriodicalIF":2.8,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144253945","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Estimation of S-values using the Digimouse phantom for radionuclides commonly under preclinical investigation for treatment of early and terminal stages of hepatocellular cancer 使用digimmouse幻影估计放射性核素的s值,通常在临床前研究中用于治疗早期和晚期肝细胞癌
IF 2.8 3区 物理与天体物理
Radiation Physics and Chemistry Pub Date : 2025-06-04 DOI: 10.1016/j.radphyschem.2025.113039
R. Yerrou , J. El Bakkali , T. El Bardouni , B. Ahannout , Y. Ben Lazrak , A. Akka , A. Nouayti , C. Benkabdi
{"title":"Estimation of S-values using the Digimouse phantom for radionuclides commonly under preclinical investigation for treatment of early and terminal stages of hepatocellular cancer","authors":"R. Yerrou ,&nbsp;J. El Bakkali ,&nbsp;T. El Bardouni ,&nbsp;B. Ahannout ,&nbsp;Y. Ben Lazrak ,&nbsp;A. Akka ,&nbsp;A. Nouayti ,&nbsp;C. Benkabdi","doi":"10.1016/j.radphyschem.2025.113039","DOIUrl":"10.1016/j.radphyschem.2025.113039","url":null,"abstract":"<div><div>Hepatocellular carcinoma (HCC) is a major therapeutic challenge due to its complex biology and the need for targeted radionuclide therapy. This study aims to evaluate and compare the S-values of radionuclides that have been investigated for HCC radionuclide therapy including 131I, 90Y, 188Re, 166Ho, 125I, and 67Cu. Using the InterDosi code version 1.3 in conjunction with the Digimouse voxelized phantom, we calculated S-values for two HCC radionuclide therapy scenarios representing the early and terminal stages of the disease by considering a small tumor in the liver and the whole liver as separate radiation sources. The results highlight significant variations in dose distribution, which affect both therapeutic efficacy and the protection of healthy tissues. Indeed, in the first scenario while the small tumor in the liver is irradiated, both 67Cu and 131I exhibited high S-values, with variations between them of less than 10 %. Notably, 67Cu enabled a substantial reduction in dose absorption in neighboring organs, reducing exposure by 54 %–71 % compared with 131I, making it a safer option for treatment. Whereas, in the second scenario in which the whole liver is irradiated, 90Y and 188Re had the highest S-values, delivering homogeneous doses throughout the liver, but also resulting in higher exposure of surrounding organs. In contrast, 67Cu showed moderate S-values while significantly reducing doses to non-target organs, with kidney exposure reduced by 97.9 % compared to 90Y. We conclude that 67Cu appears to be a promising candidate for optimizing HCC radionuclide therapy minimizing toxicity to healthy tissues while maintaining high radiation therapeutic efficacy.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"237 ","pages":"Article 113039"},"PeriodicalIF":2.8,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144237656","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effects of Er2O3 doping on the physical properties and gamma/neutron shielding performance of borate-tellurite glasses: PHITS Monte Carlo simulations Er2O3掺杂对硼酸碲酸盐玻璃物理性能和屏蔽性能的影响:PHITS蒙特卡罗模拟
IF 2.8 3区 物理与天体物理
Radiation Physics and Chemistry Pub Date : 2025-06-04 DOI: 10.1016/j.radphyschem.2025.113042
M.S. Al-Buriahi , Norah Alomayrah , S.S. Owoeye , Norah Salem Alsaiari
{"title":"Effects of Er2O3 doping on the physical properties and gamma/neutron shielding performance of borate-tellurite glasses: PHITS Monte Carlo simulations","authors":"M.S. Al-Buriahi ,&nbsp;Norah Alomayrah ,&nbsp;S.S. Owoeye ,&nbsp;Norah Salem Alsaiari","doi":"10.1016/j.radphyschem.2025.113042","DOIUrl":"10.1016/j.radphyschem.2025.113042","url":null,"abstract":"<div><div>Presently, there have been consistent research towards designing and testing of novel materials with high radiation shielding potential. This present study investigates the effects of Erbium oxide (Er<sub>2</sub>O<sub>3</sub>) doping on the physical and radiation shielding features of mixed telluro-borate glasses containing B<sub>2</sub>O<sub>3</sub>–TeO<sub>2</sub>–PbO–BaO–Bi<sub>2</sub>O<sub>3</sub>-xEr<sub>2</sub>O<sub>3</sub>, (with x = 0.5, 1.0 and 2.0 mol %). The produced glasses (BTE0.5, BTE1 and BTE2) were studied for their physical and radiation shielding properties. The results showed that the density of the glasses increased from 3.97 to 4.25 g/cm<sup>3</sup>, while molar volume decreased from 4.25 to 3.95 cm<sup>3</sup>/mol at increasing Er<sub>2</sub>O<sub>3</sub> addition from 0.5 to 2.0 mol %. The measured mass attenuation coefficient (MAC) validated by XCOM and PHITS (with no significant difference between the two validated data) showed that MAC values generally increased from BTE0.5 to BTE2 at all energy levels between 0.015 and 15 MeV. This suggest that increasing Er<sub>2</sub>O<sub>3</sub> in the BTE composition enhanced shielding effectiveness. Sample BTE2 exhibited lowest half-value layer (HVL) followed by BTE1 and BTE0.5 at lower energies, which indicates that increasing Er<sub>2</sub>O<sub>3</sub> content improves shielding efficiency at low energies. However, at increased photon energies, the differences in the samples decline, suggesting that all the samples (BTE0.5, BTE1 and BTE2) are likewise effective for high-energy radiation shielding. The fast neutron removal cross-section (<em>Σ</em><sub><em>R</em></sub>) also improves at increasing Er<sub>2</sub>O<sub>3</sub> content with values ranged from 0.10235, 0.10374, and 10672 cm<sup>−1</sup> for BTE0.5, BTE1, and BTE2, respectively. In the overall, sample BTE containing higher Er<sub>2</sub>O<sub>3</sub> content (BTE2) showed promising properties comparable with other shielding materials highlighting its potential for gamma/neutron shielding applications.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"237 ","pages":"Article 113042"},"PeriodicalIF":2.8,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144242864","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Cations distribution, optical and radiation shielding investigations of ZnAl2O4 doped with different metals: Ni, Mn and Mg Ni、Mn、Mg不同金属掺杂ZnAl2O4的阳离子分布、光学和辐射屏蔽研究
IF 2.8 3区 物理与天体物理
Radiation Physics and Chemistry Pub Date : 2025-06-04 DOI: 10.1016/j.radphyschem.2025.113036
Zein K. Heiba , Noura M. Farag , Saif A. Mouhammad , Ali Badawi , Mohamed Bakr Mohamed
{"title":"Cations distribution, optical and radiation shielding investigations of ZnAl2O4 doped with different metals: Ni, Mn and Mg","authors":"Zein K. Heiba ,&nbsp;Noura M. Farag ,&nbsp;Saif A. Mouhammad ,&nbsp;Ali Badawi ,&nbsp;Mohamed Bakr Mohamed","doi":"10.1016/j.radphyschem.2025.113036","DOIUrl":"10.1016/j.radphyschem.2025.113036","url":null,"abstract":"<div><div>Nanocrystalline ZnAl<sub>2</sub>O<sub>4</sub> undoped and doped with different metals (Ni, Mn and Mg) has been prepared applying the solid-state reaction method. Analysis of synchrotron x-ray diffraction patterns revealed the formation of a major phase with a cubic spinel structure, <span><math><mrow><mi>F</mi><mspace></mspace><mi>d</mi><mover><mn>3</mn><mo>‾</mo></mover><mi>m</mi></mrow></math></span>, alongside tiny phases unobservable without synchrotron radiation. Incorporation of the dopant elements into the ZnAl<sub>2</sub>O<sub>4</sub> lattice is confirmed by FTIR and Raman spectroscopic analysis. Rietveld structural analysis revealed a partial inverse structure for the pure ZnAl<sub>2</sub>O<sub>4</sub> sample with an inversion parameter of 0.146 which increased upon doping with Mg or Ni but reduced upon doping with Mn. UV–Vis diffuse reflectance revealed a significant increase in absorption, especially in the visible region upon doping with Mn or Ni, with a substantial reduction in the optical bandgap from 4.0 eV to 1.62, 1.9 eV respectively. The reduction in the bandgap energies was confirmed by excitation and emission photoluminescence (PL) measurements. The PL intensity was almost totally quenched for samples containing Ni or Mn. The undoped and doped samples displayed violet-blue colors, with different intensities. At 0.015 MeV, the linear (LAC) and mass attenuation coefficient (MAC) values for undoped and doped ZnAl<sub>2</sub>O<sub>4</sub> samples with Ni, Mn, or Mg are (127.1, 233.0, 205.7, 169.0 cm<sup>−1</sup>) and (31.9, 58.1, 50.9, and 43.0 cm<sup>2</sup>/g), respectively. The half value layers (HVL) and tenth value layers (TVL) values decreased when ZnAl<sub>2</sub>O<sub>4</sub> was doped with either Ni, Mn or Mg at both low and high photon energy. ZnAl<sub>2</sub>O<sub>4</sub> doped with Ni exhibited the smallest mean free path (MFP) value throughout both lower and higher photon energy ranges. Compared to ZnAl<sub>2</sub>O<sub>4</sub>, the samples containing doped samples display elevated effective atomic number (Z<sub>eff</sub>) values. The impact of doping on the fast neutron removal cross-section (FNRCS), exposure buildup factor (EBF) and energy absorption buildup factor (EABF) parameters was also explored. The quenched intensity of PL emission and the reduction in the bandgap energy, obtained via Ni or Mn doping, signify that the samples are appropriate for photocatalytic applications.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"237 ","pages":"Article 113036"},"PeriodicalIF":2.8,"publicationDate":"2025-06-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144242736","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Investigations on electrical, optical and thermal properties of Yb2O3 doped-borate glasses: radiation-shielding features using the Phy-X software Yb2O3掺杂硼酸盐玻璃的电学、光学和热学性能研究:利用Phy-X软件研究辐射屏蔽特性
IF 2.8 3区 物理与天体物理
Radiation Physics and Chemistry Pub Date : 2025-06-03 DOI: 10.1016/j.radphyschem.2025.113022
Ali M. Ibrahim , Homaisara A. Mohammed , Ayman El-Amin
{"title":"Investigations on electrical, optical and thermal properties of Yb2O3 doped-borate glasses: radiation-shielding features using the Phy-X software","authors":"Ali M. Ibrahim ,&nbsp;Homaisara A. Mohammed ,&nbsp;Ayman El-Amin","doi":"10.1016/j.radphyschem.2025.113022","DOIUrl":"10.1016/j.radphyschem.2025.113022","url":null,"abstract":"<div><div>The addition of Yb<sub>2</sub>O<sub>3</sub> cations to borate glasses significantly improves their electrical and optical properties. The capability of glass composition makes it further useful for a huge range of applications. The electrical properties, optical properties, XRD and DSC analysis have been studied. Furthermore, Yb<sub>2</sub>O<sub>3</sub> doped borate glasses are synthesized using melt quenching technique. All glasses are demonstrated to be completely amorphous. The glasses exhibits two glass transition temperatures, which nearly increase with Yb<sub>2</sub>O<sub>3</sub>-addition. The DC conduction activation energies are between 0.7845 and 0.7097 eV. The conductivity reduces with incorporation of Yb<sub>2</sub>O<sub>3</sub>. The most important optical parameters including direct and indirect band gap are estimated. The maximum and minimum energy gaps are found 2.84 and 2.79 eV at Yb<sub>2</sub>O<sub>3</sub> content 0 and 6 mol%, respectively, but the band gap increases with the addition of Yb<sub>2</sub>O<sub>3</sub>. There is also an ultraviolet limit from 246 to 381 nm, which the highest transparency is observed in the both ranges visible and infrared for samples glasses. With increasing Yb<sub>2</sub>O<sub>3</sub> content, the transmittance decreases up to Yb<sub>2</sub>O<sub>3</sub> = 7.5 mol% and then increases. The Phy-X program is utilized to calculate the properties of the shielding versus gamma radiation, the mass attenuation coefficient (MAC), half-value layer (HVL), linear attenuation coefficient (LAC), the effective atomic number (Z<sub>eff</sub>) and the mean free path (MFP). The optimal radiation shielding properties are observed for the glass containing 7.5 mol%of Yb<sub>2</sub>O<sub>3</sub>.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"237 ","pages":"Article 113022"},"PeriodicalIF":2.8,"publicationDate":"2025-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144253548","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Elastic modulus, nuclear radiation transmission properties of Fe-based/contained novel alloys for critical radiation applications 关键辐射应用铁基/含铁新型合金的弹性模量、核辐射透射性能
IF 2.8 3区 物理与天体物理
Radiation Physics and Chemistry Pub Date : 2025-06-03 DOI: 10.1016/j.radphyschem.2025.113026
Ghada ALMisned , Gulfem Susoy , Duygu Sen Baykal , Hessa Alkarrani , Ömer Güler , Shams A.M. Issa , Hesham M.H. Zakaly , H.O. Tekin
{"title":"Elastic modulus, nuclear radiation transmission properties of Fe-based/contained novel alloys for critical radiation applications","authors":"Ghada ALMisned ,&nbsp;Gulfem Susoy ,&nbsp;Duygu Sen Baykal ,&nbsp;Hessa Alkarrani ,&nbsp;Ömer Güler ,&nbsp;Shams A.M. Issa ,&nbsp;Hesham M.H. Zakaly ,&nbsp;H.O. Tekin","doi":"10.1016/j.radphyschem.2025.113026","DOIUrl":"10.1016/j.radphyschem.2025.113026","url":null,"abstract":"<div><div>This study explores the gamma-ray and neutron shielding properties and mechanical performance of eight Fe-based alloys with varying elemental compositions and densities. Different parameters such as mass attenuation coefficients, linear attenuation coefficients, half-value layer, tenth-value layer, mean free path, fast neutron removal cross-sections, transmission factors were analysed using PHITS and Phy-X/PSD codes. Moreover, elastic modulus values were calculated for each alloy sample. Our results reveal that the S9 alloy, with high density and tungsten contribution, exhibited superior shielding and mechanical properties, achieving the lowest TF, HVL, and TVL values. In contrast, the low-density S1 alloy performed weakest, reflecting its lighter elemental composition. Intermediate alloys like MAR-302 and Cupero-Nickel showed balanced performance, suitable for moderate shielding needs. Strong correlations between elemental compositions, particularly high-Z elements like tungsten and boron, and shielding efficiency were observed. It can be concluded that optimizing elemental composition and density is critical for designing alloys with enhanced multifunctional properties.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"237 ","pages":"Article 113026"},"PeriodicalIF":2.8,"publicationDate":"2025-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144222253","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A novel method for Cu-64 radioisotope production by secondary neutrons irradiation of natural ZnO and enriched 64ZnO targets 用次级中子辐照天然氧化锌和富集64ZnO靶制备Cu-64放射性同位素的新方法
IF 2.8 3区 物理与天体物理
Radiation Physics and Chemistry Pub Date : 2025-06-03 DOI: 10.1016/j.radphyschem.2025.113008
Kartika Fajarwati , Wahyu Setia Budi , Ngurah Ayu Ketut Umiati , Imam Kambali
{"title":"A novel method for Cu-64 radioisotope production by secondary neutrons irradiation of natural ZnO and enriched 64ZnO targets","authors":"Kartika Fajarwati ,&nbsp;Wahyu Setia Budi ,&nbsp;Ngurah Ayu Ketut Umiati ,&nbsp;Imam Kambali","doi":"10.1016/j.radphyschem.2025.113008","DOIUrl":"10.1016/j.radphyschem.2025.113008","url":null,"abstract":"<div><div>This work presents the PHITS simulation and experimental studies of copper-64 (Cu-64) radioisotope by secondary neutron irradiation of <sup>64</sup>ZnO and <sup>nat</sup>ZnO targets. The secondary neutrons are generated from 11-MeV proton bombardment of titanium (Ti) primary targets with a proton beam of 15 μA and irradiation time of 5 min. The PHITS calculated results show that the 11-MeV proton bombarded Ti target generates a total neutron flux of 3.38x10<sup>9</sup> n/cm<sup>2</sup>s, which then theoretically produces a saturated Cu-64 yield of 35 kBq/g and 25 kBq/g following neutron irradiation of enriched <sup>64</sup>ZnO and natural ZnO targets, respectively. The PHITS simulation results very well agree with the experimental data.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"237 ","pages":"Article 113008"},"PeriodicalIF":2.8,"publicationDate":"2025-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144221718","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Radiation protection assessment of patient activation and dosimetry in Boron Neutron Capture Therapy 硼中子俘获治疗中患者激活和剂量学的辐射防护评估
IF 2.8 3区 物理与天体物理
Radiation Physics and Chemistry Pub Date : 2025-06-03 DOI: 10.1016/j.radphyschem.2025.112900
Giovanni Garini , Chiara Magni , Ian Postuma , Setareh Fatemi , Ricardo Ramos , Barbara Marcaccio , Cristina Pezzi , Laura Bagnale , Sandro Sandri , Gianfranco De Matteis , Giuseppe Paolisso , Valerio Vercesi , Silva Bortolussi
{"title":"Radiation protection assessment of patient activation and dosimetry in Boron Neutron Capture Therapy","authors":"Giovanni Garini ,&nbsp;Chiara Magni ,&nbsp;Ian Postuma ,&nbsp;Setareh Fatemi ,&nbsp;Ricardo Ramos ,&nbsp;Barbara Marcaccio ,&nbsp;Cristina Pezzi ,&nbsp;Laura Bagnale ,&nbsp;Sandro Sandri ,&nbsp;Gianfranco De Matteis ,&nbsp;Giuseppe Paolisso ,&nbsp;Valerio Vercesi ,&nbsp;Silva Bortolussi","doi":"10.1016/j.radphyschem.2025.112900","DOIUrl":"10.1016/j.radphyschem.2025.112900","url":null,"abstract":"<div><div>Boron Neutron Capture Therapy (BNCT) is a form of radiotherapy based on the irradiation of the tumor with a low energy neutron beam, after the administration of a selective drug enriched in boron-10. The therapy exploits the high cross section of thermal neutron capture in boron, generating two low-range charged particles. The availability of accelerators able to generate high-intensity neutron beams via proton nuclear interaction is boosting the construction of new clinical centers. One of these is under development in Italy, using a 5 MeV, 30 mA proton radiofrequency accelerator coupled to a beryllium target, funded by the Complementary Plan to the Recovery and Resilience National Plan, under the project ANTHEM. The present study focuses on radiation protection aspects of patients undergoing BNCT, specifically on the activation of their organs and tissues. A criterion to establish the relevance of such activation after BNCT has been proposed. Based on the current Italian regulatory framework, the level of patient activation following BNCT treatment does not pose a significant radiological concern, even shortly after irradiation. Another aspect is the activation of patient’s excretions, which can impact on the design of the building and requires a process for the discharge. The described study contributes to the radiation protection study for the ANTHEM BNCT centre in Italy.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"237 ","pages":"Article 112900"},"PeriodicalIF":2.8,"publicationDate":"2025-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144231417","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Advancing neutron and photon shielding for space technology and electronic protection: Investigation of Nylon-Based and non-nylon-based polymers as soft protection materials through PHITS code 推进空间技术和电子防护中的中子和光子屏蔽:通过PHITS代码研究尼龙基和非尼龙基聚合物作为软防护材料
IF 2.8 3区 物理与天体物理
Radiation Physics and Chemistry Pub Date : 2025-06-03 DOI: 10.1016/j.radphyschem.2025.113025
Hessa Alkarrani , Ghada Almisned , Hesham M.H. Zakaly , Gokhan Kilic , Shams A.M. Issa , Duygu Sen Baykal , Antoaneta Ene , H.O. Tekin
{"title":"Advancing neutron and photon shielding for space technology and electronic protection: Investigation of Nylon-Based and non-nylon-based polymers as soft protection materials through PHITS code","authors":"Hessa Alkarrani ,&nbsp;Ghada Almisned ,&nbsp;Hesham M.H. Zakaly ,&nbsp;Gokhan Kilic ,&nbsp;Shams A.M. Issa ,&nbsp;Duygu Sen Baykal ,&nbsp;Antoaneta Ene ,&nbsp;H.O. Tekin","doi":"10.1016/j.radphyschem.2025.113025","DOIUrl":"10.1016/j.radphyschem.2025.113025","url":null,"abstract":"<div><div>This study investigates the neutron and photon attenuation properties of various Nylon-Based and Non-Nylon-Based Polymers as soft protection materials for space technology and related applications. We analyzed the material densities, mass and linear attenuation coefficients, half-value layers, mean free paths, effective atomic numbers, effective electron densities, fast neutron effective removal cross-sections, and energy absorption buildup factor values of several polymers through PHITS code and other computational tools. Nylon Type 11 (Rilsan) emerged as a standout, offering substantial resistance to neutron radiation, highlighting its potential in sectors where neutron shielding is paramount. Conversely, Polyvinyl Chloride (PVC), characterized by its unique composition, demonstrated superior gamma-ray attenuation capabilities, making it an attractive option for environments predominantly exposed to gamma radiation. Our results showed that the efficacy of PVC in gamma shielding and Nylon Type 11's (Rilsan) notable neutron attenuation, demonstrating their potential as lightweight and environmentally sustainable alternatives for specific applications where lead's heavy weight poses a challenge. While lead remains superior in gamma shielding due to its high atomic number and density, the tested polymers offer practical advantages in applications requiring weight reduction and environmental considerations.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"237 ","pages":"Article 113025"},"PeriodicalIF":2.8,"publicationDate":"2025-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144231554","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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