Nature Sustainability最新文献_第9页

Recycled micro-sized silicon anode for high-voltage lithium-ion batteries 用于高压锂离子电池的回收微型硅负极

IF 25.7 1区环境科学与生态学

Nature Sustainability Pub Date : 2024-07-16 DOI: 10.1038/s41893-024-01393-9

Tao Liu, Tiantian Dong, Mengying Wang, Xiaofan Du, Youlong Sun, Gaojie Xu, Huanrui Zhang, Shanmu Dong, Guanglei Cui

{"title":"Recycled micro-sized silicon anode for high-voltage lithium-ion batteries","authors":"Tao Liu, Tiantian Dong, Mengying Wang, Xiaofan Du, Youlong Sun, Gaojie Xu, Huanrui Zhang, Shanmu Dong, Guanglei Cui","doi":"10.1038/s41893-024-01393-9","DOIUrl":"10.1038/s41893-024-01393-9","url":null,"abstract":"Silicon (Si) anode is widely viewed as a game changer for lithium-ion batteries (LIBs) due to its much higher capacity than the prevalent graphite and availability in sufficient quantity and quality. Most Si anode designs are nanostructured to overcome the large volume variation during cycling, but this comes at the expense of manufacturability, cost advantage and other merits. Here we demonstrate that micro-sized Si (μm-Si) recycled from photovoltaic waste can serve as anode material, exhibiting an average Coulombic efficiency of 99.94% and retaining 83.13% of its initial capacity after 200 cycles through the rational electrolyte design. With a formulated ether electrolyte of 3 M LiPF6 in 1,3-dioxane (DX)/1,2-diethoxyethane (DEE), NCM811||μm-Si pouch cells survive 80 cycles and deliver an energy density of 340.7 Wh kg−1 even under harsh conditions. Responsible for the impressive electrochemical performance is a unique SEI chemistry where the flexible polymer-dominated outer layer well holds fractured Si particles together and the rigid Li2O/LiF-rich inner layer serves to facilitate ionic conduction and suppress side reactions. Our work not only suggests a more sustainable supply source for Si particles but also addresses the major problems facing μm-Si anode materials. Silicon (Si) has emerged as a promising next-generation anode material. Here the authors recycle photovoltaic waste for micro-sized Si that can pair with high-voltage cathode for high-performance Li-ion pouch cells.","PeriodicalId":19056,"journal":{"name":"Nature Sustainability","volume":"7 8","pages":"1057-1066"},"PeriodicalIF":25.7,"publicationDate":"2024-07-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141644043","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Sustainable urban transformations based on integrated microgrid designs 基于综合微电网设计的可持续城市转型

IF 25.7 1区环境科学与生态学

Nature Sustainability Pub Date : 2024-07-16 DOI: 10.1038/s41893-024-01395-7

Sadeeb S. Ottenburger, Rob Cox, Badrul H. Chowdhury, Dmytro Trybushnyi, Ehmedi Al Omar, Sujay A. Kaloti, Ulrich Ufer, Witold-R. Poganietz, Weijia Liu, Evgenia Deines, Tim O. Müller, Stella Möhrle, Wolfgang Raskob

{"title":"Sustainable urban transformations based on integrated microgrid designs","authors":"Sadeeb S. Ottenburger, Rob Cox, Badrul H. Chowdhury, Dmytro Trybushnyi, Ehmedi Al Omar, Sujay A. Kaloti, Ulrich Ufer, Witold-R. Poganietz, Weijia Liu, Evgenia Deines, Tim O. Müller, Stella Möhrle, Wolfgang Raskob","doi":"10.1038/s41893-024-01395-7","DOIUrl":"10.1038/s41893-024-01395-7","url":null,"abstract":"The impacts of natural hazards on infrastructure, enhanced by climate change, are increasingly more severe emphasizing the necessity of resilient energy grids. Microgrids, tailored energy systems for specific neighbourhoods and districts, play a pivotal role in sustaining energy supply during main grid outages. These solutions not only mitigate economic losses and well-being disruptions against escalating hazards but also enhance city resilience in alignment with Sustainable Development Goal (SDG) 11. However, disregarding socioeconomic factors in defining microgrid boundaries risks perpetuating inequalities and impeding progress towards other SDG 11 targets, including fair democratic participation. Our approach integrates social and technical indicators to bolster urban microgrid planning. Through a case study in a US county, we illustrate how integrated microgrid planning effectively intertwines urban resilience, well-being and equity while promoting sustainable development. This study underscores the importance of integrated microgrid planning for sustainable and resilient urban transformation amid environmental and societal challenges. Improving the resilience of energy systems to natural hazards cannot rely only on strengthening technical aspects of energy grids. This study shows how integrating technical and socioeconomic dimensions in the design of microgrids can enhance the resilience and equity of energy systems and promote well-being.","PeriodicalId":19056,"journal":{"name":"Nature Sustainability","volume":"7 8","pages":"1067-1079"},"PeriodicalIF":25.7,"publicationDate":"2024-07-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s41893-024-01395-7.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141643599","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Sustainable power generation from sewage with engineered microorganisms as electrocatalysts 利用工程微生物作为电催化剂从污水中进行可持续发电

IF 25.7 1区环境科学与生态学

Nature Sustainability Pub Date : 2024-07-16 DOI: 10.1038/s41893-024-01383-x

Yangdi Niu, Deming Xue, Xianqi Dai, Gaofu Guo, Xiaoli Yang, Lin Yang, Zhengyu Bai

{"title":"Sustainable power generation from sewage with engineered microorganisms as electrocatalysts","authors":"Yangdi Niu, Deming Xue, Xianqi Dai, Gaofu Guo, Xiaoli Yang, Lin Yang, Zhengyu Bai","doi":"10.1038/s41893-024-01383-x","DOIUrl":"10.1038/s41893-024-01383-x","url":null,"abstract":"Microbial fuel cells (MFCs) are an emerging technology that could degrade contaminants and produce electricity simultaneously with the assistance of microorganisms. However, key challenges remain for their practical implementation, including the lack of efficient and cost-effective catalysts at the cathode. Here we take advantage of a sustainable cathode biocatalyst to construct a high-performance MFC that allows fast treatment of sewage and competitive power output. Our catalyst design is built on the Escherichia coli cell, which, upon coupled gene and nano engineering, shows excellent oxygen reduction reaction activity (current density of 3.32 mA cm−2 and onset potential of 0.63 V versus the reversible hydrogen electrode) and accelerates the depollution of organic matter in sewage sludge. Remarkably, glucose consumption reaches a level as high as 19.4 mM in 100 h with a maximum power density of 334 μW cm−2. Combined characterizations and theoretical calculations reveal that the enabling chemistry is the unique configuration of the iron centre of intermembranous cytochrome c in cells. Our study not only opens a new path for the rational design of electrocatalysts but also suggests the feasibility of addressing environmental issues using MFCs. This study presents a microorganism electrocatalyst for the cathode of a microbial fuel cell that allows simultaneous electricity generation and treatment of sewage.","PeriodicalId":19056,"journal":{"name":"Nature Sustainability","volume":"7 9","pages":"1182-1189"},"PeriodicalIF":25.7,"publicationDate":"2024-07-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141641129","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Nature-inspired microfabrication 受大自然启发的微加工技术

IF 25.7 1区环境科学与生态学

Nature Sustainability Pub Date : 2024-07-10 DOI: 10.1038/s41893-024-01386-8

Jing Meng, Feng Ryan Wang

引用次数: 0

A bioinspired permeable junction approach for sustainable device microfabrication 可持续设备微细加工的生物启发渗透结方法

IF 25.7 1区环境科学与生态学

Nature Sustainability Pub Date : 2024-07-10 DOI: 10.1038/s41893-024-01389-5

Chuanwang Yang, Pengju Li, Chen Wei, Aleksander Prominski, Jingcheng Ma, Changxu Sun, Jiping Yue, Zhe Cheng, Jing Zhang, Brennan Ashwood, Wen Li, Jiuyun Shi, Kun Hou, Fengyuan Shi, Philip Griffin, Lihua Jin, Bozhi Tian

{"title":"A bioinspired permeable junction approach for sustainable device microfabrication","authors":"Chuanwang Yang, Pengju Li, Chen Wei, Aleksander Prominski, Jingcheng Ma, Changxu Sun, Jiping Yue, Zhe Cheng, Jing Zhang, Brennan Ashwood, Wen Li, Jiuyun Shi, Kun Hou, Fengyuan Shi, Philip Griffin, Lihua Jin, Bozhi Tian","doi":"10.1038/s41893-024-01389-5","DOIUrl":"10.1038/s41893-024-01389-5","url":null,"abstract":"Microfabrication, the process of fabricating small structures usually in micrometre scale, has wide practical applications but confronts sustainability challenges due to the substantial chemical and energy consumption during the patterning and transfer stages. Here we introduce a bioinspired permeable junction approach involving patterning on biopolymer matrices with a salt-assisted photochemical synthesis to advance sustainable microfabrication. This approach leverages an ‘actuator-inhibitor-neutralizer’ process for on-demand adhesion and delamination. Utilizing water as a green actuation agent, our method realizes instantaneous delamination (<1 s) for patterned device transfer, far exceeding the efficacy of traditional technologies. This advancement boosts the roll-to-roll production speed and minimizes the consumption of energy and hazardous chemicals. The combination of sustainable substrates and hazards-free processing substantially lowers greenhouse gas emissions and reduces environmental impacts for device fabrication compared with traditional microfabrication methods. This approach is widely applicable to various device fabrication processes, ranging from bioelectronic devices to catalytic robotics. Overall, this work addresses the sustainability challenges of microfabrication, paving the way to environmentally friendly device fabrication. Microfabrication has an essential role in device fabrication but is accompanied by unfavourable environmental footprint. This study presents a bioinspired permeable junction approach for sustainable microfabrication, which eliminates the use of hazardous chemicals and minimizes energy consumption.","PeriodicalId":19056,"journal":{"name":"Nature Sustainability","volume":"7 9","pages":"1190-1203"},"PeriodicalIF":25.7,"publicationDate":"2024-07-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141662649","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

The impact of genetically modified crops on bird diversity 转基因作物对鸟类多样性的影响

IF 25.7 1区环境科学与生态学

Nature Sustainability Pub Date : 2024-07-09 DOI: 10.1038/s41893-024-01390-y

Dennis Engist, Laura Melissa Guzman, Ashley Larsen, Trevor Church, Frederik Noack

{"title":"The impact of genetically modified crops on bird diversity","authors":"Dennis Engist, Laura Melissa Guzman, Ashley Larsen, Trevor Church, Frederik Noack","doi":"10.1038/s41893-024-01390-y","DOIUrl":"10.1038/s41893-024-01390-y","url":null,"abstract":"Biodiversity provides essential ecosystem services to agriculture, including pest control and pollination, yet it is declining at an alarming rate, largely due to the agricultural sector. The introduction of genetically modified (GM) crops in the United States marked a major transformation of agricultural production, as over 90% of US corn, soybean and cotton areas are now planted with GM varieties. This shift in crop cultivation has substantially altered crop management practices, most notably the types and quantities of pesticides used. Despite the magnitude of these changes, the impact on biodiversity is still poorly understood. Here we estimate the causal impact of GM crops on bird diversity in the United States and compare bird communities through time in areas with different levels of exposure to GM crops. We find that insectivorous birds benefit from GM crop adoption and that this benefit is largest in cotton. In contrast, herbivorous birds weakly decrease with GM crop adoption. Thus, while GM crop adoption has a small positive effect on overall abundance of birds, the effect is heterogeneous across species groups, with potentially important consequences for bird community composition and associated ecosystem services in agricultural landscapes. The effects of genetically modified (GM) crops on biodiversity is not well understood, yet could have important implications due to the many ecosystem services provided by biodiversity to agricultural landscapes. This study evaluates the impact of GM crops on bird diversity in the United States.","PeriodicalId":19056,"journal":{"name":"Nature Sustainability","volume":"7 9","pages":"1149-1159"},"PeriodicalIF":25.7,"publicationDate":"2024-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141666101","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Genetically modified crops benefit insectivorous birds but are detrimental to others 转基因作物有利于食虫鸟类，但对其他鸟类不利

IF 25.7 1区环境科学与生态学

Nature Sustainability Pub Date : 2024-07-09 DOI: 10.1038/s41893-024-01391-x

引用次数: 0

A sustainable no-kill sea urchin aquaculture method to obtain caviar 获取鱼子酱的可持续无杀生海胆养殖方法

IF 25.7 1区环境科学与生态学

Nature Sustainability Pub Date : 2024-07-08 DOI: 10.1038/s41893-024-01372-0

Arnold Rakaj, Luca Grosso, Alessandra Fianchini, Stefano Cataudella

{"title":"A sustainable no-kill sea urchin aquaculture method to obtain caviar","authors":"Arnold Rakaj, Luca Grosso, Alessandra Fianchini, Stefano Cataudella","doi":"10.1038/s41893-024-01372-0","DOIUrl":"10.1038/s41893-024-01372-0","url":null,"abstract":"Sea urchin aquaculture represents a promising tool to promote blue economy principles that are geared towards the sustainable production of low-trophic-level organisms with high market and nutritional value. However, although sea urchin aquaculture has been practised for several decades, this sector has not yet achieved sustainable production and large-scale development outside China, mainly due to problems linked with long-term rearing cycles of most commercial sea urchin species. Here we present a method of sea urchin caviar production, called ‘raking’, that represents a technological advancement both in terms of the production approach and the final product. Raking is a no-kill method for the harvesting of caviar (sea urchin eggs) from female-only batches, meaning that the same sea urchins are used through several production cycles (three per year). Raking was compared with a traditional gonad enhancement method (known as ‘bulking’, where gonads are the final market product), and it proved to be more profitable through multi-cycle production, more sustainable without needing to kill the sea urchins to obtain the market product and able to overcome important biological and economic constraints of traditional sea urchin aquaculture. Sea urchin gonads are high-demand culinary delicacies, and depleted wild populations of these echinoderms have spurred efforts to culture them sustainably. This study presents a sea urchin aquaculture method that produces ‘caviar’ made of eggs produced by female batches, without needing to kill the sea urchins.","PeriodicalId":19056,"journal":{"name":"Nature Sustainability","volume":"7 8","pages":"1038-1047"},"PeriodicalIF":25.7,"publicationDate":"2024-07-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141667695","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

An innovative, sustainable, no-kill sea urchin aquaculture method 创新、可持续、无杀戮的海胆养殖方法

IF 25.7 1区环境科学与生态学

Nature Sustainability Pub Date : 2024-07-08 DOI: 10.1038/s41893-024-01378-8

引用次数: 0

Atmospheric emissions of respirable quartz from industrial activities in China 中国工业活动向大气排放的可吸入石英

IF 25.7 1区环境科学与生态学

Nature Sustainability Pub Date : 2024-07-08 DOI: 10.1038/s41893-024-01388-6

Qiuting Yang, Guorui Liu, Lili Yang, Jianghui Yun, Xiaoyue Zhang, Chenyan Zhao, Minghui Zheng, Guibin Jiang

{"title":"Atmospheric emissions of respirable quartz from industrial activities in China","authors":"Qiuting Yang, Guorui Liu, Lili Yang, Jianghui Yun, Xiaoyue Zhang, Chenyan Zhao, Minghui Zheng, Guibin Jiang","doi":"10.1038/s41893-024-01388-6","DOIUrl":"10.1038/s41893-024-01388-6","url":null,"abstract":"Quartz is classified as a group 1 carcinogen by the International Agency for Research on Cancer. Atmospheric emissions of respirable quartz in particulate matter released from industrial activities are important for evaluating human exposure. Here we quantified the mass concentrations of quartz as a constituent of particulate matter collected from 118 full-scale industrial plants, comprising 13 main source categories, with the aim of identifying primary industrial contributors. The sources with the highest quartz mass concentrations are waste incineration and electric-arc furnace steelmaking, with average values of 16,924 μg g−1 and 12,005 μg g−1, respectively. Total atmospheric emissions of quartz from the investigated industrial sources are 24,581.3 t. Cement kiln co-processing solid waste, coking plants, pig-iron blast furnaces, iron-ore sintering and steelmaking electric-arc furnaces were identified as the major industrial sources contributing to quartz emissions in China. Quartz emissions arising from the 13 industrial sources could generate up to 77.2% increment in cancer risk for China owing to the high density of these activities. These results provide important fundamental data to assess exposure risks in the general population and enhance sustainability of industrial development. Quartz is a well-known carcinogen of particular concern to industrial workers exposed to particulate quartz. Industrial atmospheric emissions across multiple sectors, however, are found to include respirable quartz, posing a threat to the public health of surrounding populations.","PeriodicalId":19056,"journal":{"name":"Nature Sustainability","volume":"7 9","pages":"1120-1127"},"PeriodicalIF":25.7,"publicationDate":"2024-07-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141669069","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0