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Thermomechanical properties of stereolithographic 3D-printed zinc oxide nanocomposites 立体光刻三维打印氧化锌纳米复合材料的热力学特性
IF 1.9 4区 材料科学
MRS Communications Pub Date : 2024-07-01 DOI: 10.1557/s43579-024-00602-y
Vincent Joseph Garcia, Xiang Cheng, Lihan Rong, Tania E. Lara-Ceniceros, Emmanuel Ricohermoso, José Bonilla-Cruz, Richard D. Espiritu, Rigoberto C. Advincula
{"title":"Thermomechanical properties of stereolithographic 3D-printed zinc oxide nanocomposites","authors":"Vincent Joseph Garcia, Xiang Cheng, Lihan Rong, Tania E. Lara-Ceniceros, Emmanuel Ricohermoso, José Bonilla-Cruz, Richard D. Espiritu, Rigoberto C. Advincula","doi":"10.1557/s43579-024-00602-y","DOIUrl":"https://doi.org/10.1557/s43579-024-00602-y","url":null,"abstract":"<p>Stereolithography (SLA) is a highly versatile additive manufacturing technique that utilizes various ink formulations to fabricate 3D-printed nanocomposite structures with desired properties. Zinc oxide (ZnO) is a promising candidate due to its excellent mechanical and thermal stability, and compatibility with various polymeric matrices. In this work, varying ink formulations containing ZnO nanoparticles, along with employing appropriate post-printing curing parameters to fabricate SLA 3D-printed acrylate-based nanocomposites with improved mechanical and thermal properties, were reported. This study can significantly contribute to expanding its potential use in practical applications such as biomedical and structural applications.</p><h3 data-test=\"abstract-sub-heading\">Graphical Abstract</h3>\u0000","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"2012 1","pages":""},"PeriodicalIF":1.9,"publicationDate":"2024-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141518647","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A prospective on machine learning challenges, progress, and potential in polymer science 展望机器学习在聚合物科学中的挑战、进展和潜力
IF 1.9 4区 材料科学
MRS Communications Pub Date : 2024-07-01 DOI: 10.1557/s43579-024-00587-8
Daniel C. Struble, Bradley G. Lamb, Boran Ma
{"title":"A prospective on machine learning challenges, progress, and potential in polymer science","authors":"Daniel C. Struble, Bradley G. Lamb, Boran Ma","doi":"10.1557/s43579-024-00587-8","DOIUrl":"https://doi.org/10.1557/s43579-024-00587-8","url":null,"abstract":"<h3 data-test=\"abstract-sub-heading\">Abstract</h3><p>Artificial intelligence and machine learning (ML) continue to see increasing interest in science and engineering every year. Polymer science is no different, though implementation of data-driven algorithms in this subfield has unique challenges barring widespread application of these techniques to the study of polymer systems. In this Prospective, we discuss several critical challenges to implementation of ML in polymer science, including polymer structure and representation, high-throughput techniques and limitations, and limited data availability. Promising studies targeting resolution of these issues are explored, and contemporary research demonstrating the potential of ML in polymer science despite existing obstacles are discussed. Finally, we present an outlook for ML in polymer science moving forward.</p><h3 data-test=\"abstract-sub-heading\">Graphical Abstract</h3>","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"6 1","pages":""},"PeriodicalIF":1.9,"publicationDate":"2024-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141503803","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Architectural engineering of nanocomposite electrodes for energy storage 用于储能的纳米复合电极的建筑工程
IF 1.9 4区 材料科学
MRS Communications Pub Date : 2024-07-01 DOI: 10.1557/s43579-024-00601-z
Kara A. Randall, Mirina E. Enderlin, Paraskevi Flouda
{"title":"Architectural engineering of nanocomposite electrodes for energy storage","authors":"Kara A. Randall, Mirina E. Enderlin, Paraskevi Flouda","doi":"10.1557/s43579-024-00601-z","DOIUrl":"https://doi.org/10.1557/s43579-024-00601-z","url":null,"abstract":"<p>The design of electrode architecture plays a crucial role in advancing the development of next generation energy storage devices, such as lithium-ion batteries and supercapacitors. Nevertheless, existing literature lacks a comprehensive examination of the property tradeoffs stemming from different electrode architectures. This prospective seeks to bridge this gap by focusing on the diverse nanocomposite electrode architectures. Furthermore, the challenges related to designing well-defined electrode architectures for enhanced energy storage are discussed. Finally, this review addresses the interdisciplinary nature of this field by examining the integration of advanced characterization and fabrication techniques, and machine learning methodologies for electrode optimization.</p><h3 data-test=\"abstract-sub-heading\">Graphical abstract</h3><p>Designing electrodes with controlled architecture and leveraging emerging tools such as <i>in situ</i> characterization, additive manufacturing methods, and machine learning facilitates the advancement of energy storage systems.</p>\u0000","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"209 1","pages":""},"PeriodicalIF":1.9,"publicationDate":"2024-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141518644","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Enhanced syngas (H2/CO) production by Co/CeO2 nanorods catalyst through dry reforming of methane 利用 Co/CeO2 纳米棒催化剂通过甲烷干转化提高合成气（H2/CO）产量
IF 1.9 4区 材料科学
MRS Communications Pub Date : 2024-06-28 DOI: 10.1557/s43579-024-00585-w
Jorge Reyna-Alvarado, Oscar A. López-Galán, Jorge Trimmer, Oscar Recalde-Benitez, Leopoldo Molina, Albina Gutiérrez-Martínez, Raúl Pérez-Hernández, Manuel Ramos
{"title":"Enhanced syngas (H2/CO) production by Co/CeO2 nanorods catalyst through dry reforming of methane","authors":"Jorge Reyna-Alvarado, Oscar A. López-Galán, Jorge Trimmer, Oscar Recalde-Benitez, Leopoldo Molina, Albina Gutiérrez-Martínez, Raúl Pérez-Hernández, Manuel Ramos","doi":"10.1557/s43579-024-00585-w","DOIUrl":"https://doi.org/10.1557/s43579-024-00585-w","url":null,"abstract":"<p>This study presents the synthesis and characterization of the Co supported on CeO<sub>2</sub> nanorods (NR) catalyst to investigate catalytic performance towards efficient hydrogen production. The catalyst was characterized by transmission electron microscopy, energy-dispersive X-ray spectroscopy, and X-ray diffraction. Temperature-programmed reduction measurements showed that the Co/CeO<sub>2</sub>-NR active phase was reduced below 500°C. Adding Co to CeO<sub>2</sub>-NR enhances the basicity of the raw CeO<sub>2</sub>-NR and greatly improves the conversion to 70% for CO<sub>2</sub> and 55% for CH<sub>4</sub>. In addition, density functional theory calculations using Halgren–Lipscomb indicate electron donation from Co to CeO<sub>2</sub>-NR promotes feasible breaking of C–H bonds.</p><h3 data-test=\"abstract-sub-heading\">Graphical abstract</h3>\u0000","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"14 1","pages":""},"PeriodicalIF":1.9,"publicationDate":"2024-06-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141503804","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Supramolecular hydrogels for sustained extracellular vesicle delivery 用于细胞外囊泡持续输送的超分子水凝胶
IF 1.9 4区 材料科学
MRS Communications Pub Date : 2024-06-27 DOI: 10.1557/s43579-024-00589-6
Neil Patel, Elijah Avery, Eun Ji Chung
{"title":"Supramolecular hydrogels for sustained extracellular vesicle delivery","authors":"Neil Patel, Elijah Avery, Eun Ji Chung","doi":"10.1557/s43579-024-00589-6","DOIUrl":"https://doi.org/10.1557/s43579-024-00589-6","url":null,"abstract":"<p>Extracellular vesicles (EVs) have been explored as promising drug delivery platforms and cell-free therapies for a range of diseases. Despite their therapeutic potential, challenges persist in achieving sustained EV delivery. Here, we integrate EVs into a supramolecular and injectable hydrogel-based drug delivery system based on dodecyl- or octadecyl-modified hydroxypropyl methylcellulose (HPMC-C12 or -C18) that form non-covalent crosslinks with liposomes. Hydrogel mechanics and EV-release kinetics were tunable by varying liposome concentrations. Using mesenchymal stem cell-derived EVs (MSC-EVs), we confirm effective, hydrogel-mediated sustained EV delivery and uptake and a ~ 20% greater anti-inflammatory response in pathogenic vascular smooth muscle cells than bolus EV-only treatment.</p><h3 data-test=\"abstract-sub-heading\">Graphical abstract</h3>\u0000","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"19 1","pages":""},"PeriodicalIF":1.9,"publicationDate":"2024-06-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141518645","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Biodegradable hydrogels with tunable cross-linking structures regulate Al oxidation in Al–air batteries 具有可调交联结构的可生物降解水凝胶调节铝-空气电池中的铝氧化作用
IF 1.9 4区 材料科学
MRS Communications Pub Date : 2024-06-27 DOI: 10.1557/s43579-024-00598-5
Muqing Ren, Yichao Shi, Langqiu Xiao, Anqian Sun, Eric Johnston, Thomas E. Mallouk, Mark Allen, James H. Pikul
{"title":"Biodegradable hydrogels with tunable cross-linking structures regulate Al oxidation in Al–air batteries","authors":"Muqing Ren, Yichao Shi, Langqiu Xiao, Anqian Sun, Eric Johnston, Thomas E. Mallouk, Mark Allen, James H. Pikul","doi":"10.1557/s43579-024-00598-5","DOIUrl":"https://doi.org/10.1557/s43579-024-00598-5","url":null,"abstract":"<p>Internet of Things (IoT) devices and small robots would benefit from higher-energy-density and disposable primary Al–air batteries, but corrosion and side reactions on the Al anode limit the widespread application of this chemistry. This paper studies how the physical and chemical characteristics of double-network hydrogel (DNH) electrolytes affect the anode oxidation, discharge morphology, and performance of Al–air batteries. The chemically crosslinked and physical–chemical crosslinked DNHs were made from biodegradable materials and showed enhanced corrosion inhibition compared to aqueous KOH solution, reducing the corrosion rate by 58% to 21 mmpy. An Al–air battery with a PVA-PAAM DNH extracted over 300 mAh cm<sup>−2</sup> from Al at 10 mA cm<sup>−2</sup>.</p><h3 data-test=\"abstract-sub-heading\">Graphical abstract</h3>\u0000","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"32 1","pages":""},"PeriodicalIF":1.9,"publicationDate":"2024-06-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141518646","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Progress and prospects of quantum emission from perovskites 过氧化物量子发射的进展与前景
IF 1.9 4区 材料科学
MRS Communications Pub Date : 2024-06-26 DOI: 10.1557/s43579-024-00597-6
Arka Chatterjee, Sadie Brasel, Autumn Bruncz, Wenjing Wu, Shengxi Huang
{"title":"Progress and prospects of quantum emission from perovskites","authors":"Arka Chatterjee, Sadie Brasel, Autumn Bruncz, Wenjing Wu, Shengxi Huang","doi":"10.1557/s43579-024-00597-6","DOIUrl":"https://doi.org/10.1557/s43579-024-00597-6","url":null,"abstract":"<p>Quantum emissions, such as single photon emission (SPE) and superradiance (SR), are fundamental ingredients of quantum optical technology. The quest for efficient, controllable, and scalable quantum emitters is crucial for successfully implementing various quantum technologies, such as quantum computing, secure quantum communication and high-precision metrology. Recently, perovskite quantum dots (PQDs) have emerged as highly efficient sources of quantum emission due to their excellent optical properties, including near 100% quantum yield, high optical absorbance, and tunable bandgaps covering the entire visible range. This Prospective introduces the principles of quantum emissions, including SPE and SR, and summarizes recent progress in exploring quantum emissions in PQDs. We focus on the prospects, advantages, and challenges associated with the quantum emissions from PQDs. This Prospective concludes with an outlook on PQDs in advancing future quantum technologies.</p><h3 data-test=\"abstract-sub-heading\">Graphical abstract</h3>\u0000","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"53 1","pages":""},"PeriodicalIF":1.9,"publicationDate":"2024-06-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141503805","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Transmission-scanning electron microscopy of interface fracture of ferrite deformation twins 铁素体变形孪晶界面断裂的透射扫描电子显微镜观察
IF 1.9 4区 材料科学
MRS Communications Pub Date : 2024-06-25 DOI: 10.1557/s43579-024-00595-8
Abdalrhaman Koko, T. James Marrow
{"title":"Transmission-scanning electron microscopy of interface fracture of ferrite deformation twins","authors":"Abdalrhaman Koko, T. James Marrow","doi":"10.1557/s43579-024-00595-8","DOIUrl":"https://doi.org/10.1557/s43579-024-00595-8","url":null,"abstract":"<p>Deformation twins in the ferrite matrix of an age-hardened duplex stainless steel have been observed using on-axis transmission Kikuchi diffraction (TKD) in a scanning electron microscope. This provided details of the lattice misorientation and dislocation arrangement, including the dislocation-free zone at the twin tip. These observations provide evidence for the link between microcracking of the irregular twin/parent interface and relaxation of the residual strains that arise from twin growth, offering new insights into fracture mechanics in these materials.</p><h3 data-test=\"abstract-sub-heading\">Graphical abstract</h3>\u0000","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"27 1","pages":""},"PeriodicalIF":1.9,"publicationDate":"2024-06-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141518566","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Additive engineering in ether-based electrolyte for lithium metal battery 锂金属电池醚基电解质中的添加剂工程
IF 1.9 4区 材料科学
MRS Communications Pub Date : 2024-06-25 DOI: 10.1557/s43579-024-00592-x
Jiayi Zhang, Laisuo Su
{"title":"Additive engineering in ether-based electrolyte for lithium metal battery","authors":"Jiayi Zhang, Laisuo Su","doi":"10.1557/s43579-024-00592-x","DOIUrl":"https://doi.org/10.1557/s43579-024-00592-x","url":null,"abstract":"<p>Lithium metal batteries (LMBs) outperform lithium-ion batteries in the aspect of energy density as they use lithium metal as the anode that has extremely high energy density and low potential. However, the development of LMBs is hampered by uncontrollable Li plating morphology and inferior Coulombic efficiency (CE) during cycling. In the past decade, electrolyte development has been recognized as one of the most effective strategies to tackle these two challenges. Much progress has been made through designing advanced electrolytes, especially ether-based electrolytes, in developing LMBs. Herein, we focus on summarizing the use of additives in ether-based electrolytes to enable high-performance LMBs. The impact of additives in electrolytes on lithium metal anode (LMA) protection, cathode protection, extreme temperature operation, and fast charging for LMBs are systematically discussed. The review reveals the significance of additive engineering in developing advanced electrolytes for high-energy–density LMBs.</p><h3 data-test=\"abstract-sub-heading\">Graphical abstract</h3>\u0000","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"133 1","pages":""},"PeriodicalIF":1.9,"publicationDate":"2024-06-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141518651","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Advancements in oxidative chemical vapor deposition (oCVD) with liquid oxidant: A true dry vacuum manufacturing approach for optoelectronic devices 使用液态氧化剂的氧化化学气相沉积 (oCVD) 取得进展：用于光电设备的真正干式真空制造方法
IF 1.9 4区 材料科学
MRS Communications Pub Date : 2024-06-25 DOI: 10.1557/s43579-024-00593-w
Meysam Heydari Gharahcheshmeh
{"title":"Advancements in oxidative chemical vapor deposition (oCVD) with liquid oxidant: A true dry vacuum manufacturing approach for optoelectronic devices","authors":"Meysam Heydari Gharahcheshmeh","doi":"10.1557/s43579-024-00593-w","DOIUrl":"https://doi.org/10.1557/s43579-024-00593-w","url":null,"abstract":"<p>Conducting polymers have attracted significant interest due to their unique properties, including metal-like conductivity, ionic conductivity, optical transparency, and mechanical flexibility. Poly(3,4-ethylene-dioxythiophene):poly(styrene sulfone) (PEDOT:PSS) is commonly utilized as the hole transport layer (HTL) in optoelectronic devices. However, its high acidity, primarily attributed to the low pH of PSS, poses challenges such as counter electrode etching, detrimental interactions with the photoactive layer, and device instability. To address these issues, researchers are exploring alternative HTL materials and deposition methods. Oxidative chemical vapor deposition (oCVD) has emerged as a promising technique to fabricate high-quality PEDOT thin films without PSS, enhancing device stability. The selection of an appropriate oxidant is crucial in oCVD, as it significantly influences film properties and performance. The utilization of liquid oxidants enables direct integration of conductive polymer thin films into devices through a one-step, dry process, eliminating the need for post-deposition rinsing and ensuring compatibility with solvent-sensitive and temperature-sensitive substrates. Moreover, precise control over liquid oxidant flow rates provides advantages over solid oxidants. This prospective article provides an overview of recent advancements in engineering the texture and nanostructure of conducting polymers to boost electrical conductivity and enhance optoelectronic performance. Additionally, it provides a comprehensive overview of recent progress in oCVD method, focusing on the use of liquid oxidants. Furthermore, the prospective article underscores the significance of oCVD in the efficient fabrication of PEDOT thin films without PSS, thus playing a pivotal role in the development of stable optoelectronic devices.</p><h3 data-test=\"abstract-sub-heading\">Graphical Abstract</h3>\u0000","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"198 1","pages":""},"PeriodicalIF":1.9,"publicationDate":"2024-06-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141518649","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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