MRS CommunicationsPub Date : 2026-01-01Epub Date: 2025-12-08DOI: 10.1557/s43579-025-00860-4
Brinthan Kanesalingam, Can Yildirim, Leora Dresselhaus-Marais
{"title":"Advances in artificial intelligence-based approaches to enhance dark field X-ray microscopy analysis.","authors":"Brinthan Kanesalingam, Can Yildirim, Leora Dresselhaus-Marais","doi":"10.1557/s43579-025-00860-4","DOIUrl":"10.1557/s43579-025-00860-4","url":null,"abstract":"<p><p>Dark field X-ray microscopy (DFXM) has emerged as a powerful technique for characterizing dislocations in bulk crystalline materials, whose high penetration depth and non-destructive evaluation offer unique advantages over traditional electron microscopy methods. The interpretation and analysis of the DFXM data presents significant challenges that have limited its broader adoption. Here we review our recent advances using artificial intelligence (AI) methods to enhance DFXM analysis, particularly focusing on dislocation characterization. We discuss the development of physics-informed AI approaches that combine theoretical understanding with data science techniques to enable both time-resolved dislocation dynamics studies and dimensional reduction of complex DFXM datasets. Our work demonstrates how semi-automated workflows, guided by dislocation theory and employing techniques such as wavelet transforms and Bayesian inference, can effectively track and analyze dislocation behavior across multiple time scales. These methodologies have been successfully applied to various materials science challenges, from studying thermally activated dislocation motion to characterizing dislocation networks. By presenting our works that integrate physics-based modeling into AI capabilities, we demonstrate how our and other works can extract new important quantitative dislocation data from DFXM measurements.</p><p><strong>Graphical abstract: </strong></p>","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"16 1","pages":"144-154"},"PeriodicalIF":2.7,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC13002649/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147499690","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
MRS CommunicationsPub Date : 2026-01-01Epub Date: 2026-02-17DOI: 10.1557/s43579-026-00936-9
Laurel Hilger, Alexandra Marnot, Blair Brettmann
{"title":"Composition consistency as a critical quality attribute for material extrusion additive manufacturing.","authors":"Laurel Hilger, Alexandra Marnot, Blair Brettmann","doi":"10.1557/s43579-026-00936-9","DOIUrl":"10.1557/s43579-026-00936-9","url":null,"abstract":"<p><p>Additive manufacturing (AM) of dense pastes is attracting interest across many fields and while the combination of a high loading of functional particles with a flowable continuous phase is promising, the heterogeneous system makes material and process design difficult. Prior work has focused on assessing printability by examining their extrudability and shape retention. However, for dense pastes, the inks are susceptible to separation of particles from binder, so we consider composition consistency as a critical quality attribute. This composition consistency attribute provides a framework for quality assessment of material extrusion AM inks and processes.</p><p><strong>Graphical abstract: </strong></p><p><strong>Supplementary information: </strong>The online version contains supplementary material available at 10.1557/s43579-026-00936-9.</p>","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"16 3","pages":"566-574"},"PeriodicalIF":2.7,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC13337734/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148405363","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Synchronized modulation Kelvin probe force microscopy for surface photovoltage studies in optoelectronic systems.","authors":"Zeinab Eftekhari, Ariane Ufer, Ursula Wurstbauer, Rebecca Saive","doi":"10.1557/s43579-025-00899-3","DOIUrl":"10.1557/s43579-025-00899-3","url":null,"abstract":"<p><p>We introduce synchronized modulation Kelvin probe force microscopy (SM-KPFM), an in-operando technique that synchronizes external stimulus modulation, such as illumination or bias, with the scanning direction of the atomic force microscope to minimize artifacts from drift, thermal effects, and probe degradation. In synchronized illumination KPFM, the sample is illuminated during retrace and dark during trace, enabling real-time comparison of surface potentials within a single raster frame. At the example of a silicon photodiode and a molybdenum disulfide bilayer on gold, these superior properties are demonstrated, yielding drift-free, accurate surface photovoltage maps and clearer insights into photovoltaic effects.</p><p><strong>Graphical abstract: </strong></p><p><strong>Supplementary information: </strong>The online version contains supplementary material available at 10.1557/s43579-025-00899-3.</p>","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"16 1","pages":"180-186"},"PeriodicalIF":2.7,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC13002633/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147499661","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
MRS CommunicationsPub Date : 2026-01-01Epub Date: 2026-04-22DOI: 10.1557/s43579-026-00940-z
Claudia Gollner, Aaron Lindenberg, Tony F Heinz
{"title":"Time-domain terahertz emission spectroscopy on van der Waals materials.","authors":"Claudia Gollner, Aaron Lindenberg, Tony F Heinz","doi":"10.1557/s43579-026-00940-z","DOIUrl":"10.1557/s43579-026-00940-z","url":null,"abstract":"<p><strong>Abstract: </strong>Time-domain terahertz (THz) emission spectroscopy provides a direct method to probe transient photo-currents by recording the emitted terahertz electric field. Although the basic principles of THz surface emission have been understood for more than 30 years, the constant progress in ultrafast laser science to ever shorter pulses, the development of new materials and enhanced sensitivity promote THz emission spectroscopy as a reliable method to gain insights into charge carrier dynamics with unprecedented precision. It provides a versatile tool to study ultrafast processes, such as plasmon-driven hot carriers, dynamics of Dirac fermions, interfacial charge transfer, coherent phonon emission and quantum beating, to name only a few. However, despite the rapidly growing body of research on van der Waals materials, especially in their low-dimensional limit, THz emission spectroscopy has only been applied to a limited extent in these material systems. In this prospective, we review time-domain THz emission spectroscopy as a complementary approach to probe ultrafast charge carrier dynamics and the material's nonlinear response. After a description of the experimental method, we report on THz emission spectroscopy of bulk and 2D van der Waals materials with special focus on graphene and transition metal dichalcogenide layers.</p><p><strong>Graphical abstract: </strong></p>","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"16 3","pages":"659-671"},"PeriodicalIF":2.7,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC13337885/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"148405313","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
MRS CommunicationsPub Date : 2025-01-01Epub Date: 2025-08-18DOI: 10.1557/s43579-025-00788-9
George H Creasey, Andreas Kafizas, Anna Hankin
{"title":"Investigating the beneficial effects of a WO<sub>3</sub> seed layer on the mechanical and photoelectrochemical stability of WO<sub>3</sub>|BiVO<sub>4</sub>|NiFeOOH photoanodes under operational conditions.","authors":"George H Creasey, Andreas Kafizas, Anna Hankin","doi":"10.1557/s43579-025-00788-9","DOIUrl":"10.1557/s43579-025-00788-9","url":null,"abstract":"<p><p>Scalable and durable photoelectrodes are essential for technological breakthroughs in photoelectrochemical systems, yet the fragility of nanostructured photocatalyst materials in industrially relevant operating conditions is rarely explored. Herein, we advance understanding of the importance of morphology and temperature on stability and performance of nanostructured WO<sub>3</sub>|BiVO<sub>4</sub>|NiFeOOH photoanodes. The integration of a planar WO<sub>3</sub> seed layer beneath nanostructured WO<sub>3</sub>, improved mechanical stability at 40°C with flowing electrolyte approximately twofold compared with materials where a seed layer was not integrated. This work provides a pathway through which robust photoelectrode systems can be engineered to enable the advancement of up-scaled photoelectrochemical water splitting.</p><p><strong>Graphical abstract: </strong></p><p><strong>Supplementary information: </strong>The online version contains supplementary material available at 10.1557/s43579-025-00788-9.</p>","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"15 4","pages":"721-730"},"PeriodicalIF":2.3,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12484363/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145213181","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
MRS CommunicationsPub Date : 2025-01-01Epub Date: 2024-12-02DOI: 10.1557/s43579-024-00678-6
Siddharth R Krishnan, Robert Langer, Daniel G Anderson
{"title":"Materials approaches for next-generation encapsulated cell therapies.","authors":"Siddharth R Krishnan, Robert Langer, Daniel G Anderson","doi":"10.1557/s43579-024-00678-6","DOIUrl":"10.1557/s43579-024-00678-6","url":null,"abstract":"<p><p>Transplanted cells can act as living drug factories capable of secreting therapeutic proteins <i>in vivo</i>, with applications in the treatment of Type 1 diabetes (T1D), blood borne disease, vision disorders, and degenerative neural disease, potentially representing functional cures for chronic conditions. However, attack from the host immune system represents a major challenge, requiring chronic immunosuppression to enable long-lived cell transplantation <i>in vivo</i>. Encapsulating cells in engineered biomaterials capable of excluding components of the host immune system while allowing for the transport of therapeutic proteins, oxygen, nutrients, metabolites, and waste products represents a potential solution. However, the foreign-body response can lead to isolation from native vasculature and hypoxia leading to cell death. In this prospective article, we highlight materials-based solutions to three important challenges in the field: (i) improving biocompatibility and reducing fibrosis; (ii) enhancing transport of secreted protein drugs and key nutrients and oxygen <i>via</i> engineered, semipermeable membranes; and (iii) improving oxygenation. These efforts draw on several disciplines in materials' research, including polymer science, surfaces, membranes, biomaterials' microfabrication, and flexible electronics. If successful, these efforts could lead to new therapies for chronic disease and are a rich space for both fundamental materials' discovery and applied translational science.</p><p><strong>Graphical abstract: </strong></p>","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"15 1","pages":"21-33"},"PeriodicalIF":1.8,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11825545/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143433540","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
MRS CommunicationsPub Date : 2025-01-01Epub Date: 2025-07-31DOI: 10.1557/s43579-025-00780-3
Mitchell R Donoughue, Joshua D Anderson, Dev I Thawani, Jean Corraliza-Rodriguez, Anna Mathis, Monique S McClain
{"title":"Additive manufacturing and rheological characterization of ceramic matrix composite inks with high fiber volume loadings.","authors":"Mitchell R Donoughue, Joshua D Anderson, Dev I Thawani, Jean Corraliza-Rodriguez, Anna Mathis, Monique S McClain","doi":"10.1557/s43579-025-00780-3","DOIUrl":"10.1557/s43579-025-00780-3","url":null,"abstract":"<p><p>Additive manufacturing of fiber-filled ceramic matrix composites (CMCs) can be used to tune local properties <i>via</i> controlled fiber orientation. Increasing the loading of fibers in additively manufactured CMCs is needed to improve the fracture toughness, yet printing CMCs with high fiber loadings (> 20 vol%) remains challenging. In this work, the combination of viscous silicon oxycarbide preceramic resins, short carbon fibers (50 µm × 7 µm), and Vibration-Assisted Printing enable printing of a mixture with 39.4-vol.% carbon fiber (total loading of 43.3 vol%) with omnidirectional fibers within the bead.</p><p><strong>Graphical abstract: </strong></p><p><strong>Supplementary information: </strong>The online version contains supplementary material available at 10.1557/s43579-025-00780-3.</p>","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"15 4","pages":"674-681"},"PeriodicalIF":2.3,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12484376/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145213175","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
MRS CommunicationsPub Date : 2025-01-01Epub Date: 2025-05-13DOI: 10.1557/s43579-025-00726-9
Thomas Defferriere, Harry L Tuller
{"title":"Optoionics: New opportunity for ionic conduction-based radiation detection.","authors":"Thomas Defferriere, Harry L Tuller","doi":"10.1557/s43579-025-00726-9","DOIUrl":"10.1557/s43579-025-00726-9","url":null,"abstract":"<p><p>Optoionics, involving light-modulated ionic transport in ionic solids, parallels optoelectronics in semiconductors and offers novel device design opportunities across various fields. Among these opportunities, grain boundary phenomena related to radiation-induced electron/hole pair generation and charge trapping at the boundaries causing a modulation in ionic current could enable fast, sensitive, and reversible radiation detectors. The robustness of ionic solids in chemical, structural, and thermal aspects in turn makes them scalable and robust alternatives to traditional semiconductor detectors. This article explores the theoretical underpinnings, experimental breakthroughs, and design considerations needed to optimize such optoionic devices.</p><p><strong>Graphical abstract: </strong></p>","PeriodicalId":19016,"journal":{"name":"MRS Communications","volume":"15 3","pages":"523-532"},"PeriodicalIF":1.8,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12241152/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144626753","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}