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Perovskite computed tomography imager and three-dimensional reconstruction Perovskite 计算机断层扫描成像仪和三维重建
IF 32.3 1区 物理与天体物理
Nature Photonics Pub Date : 2024-08-16 DOI: 10.1038/s41566-024-01506-y
Yuhong He, Jinmei Song, Mingbian Li, Kostiantyn Sakhatskyi, Weijun Li, Xiaopeng Feng, Bai Yang, Maksym Kovalenko, Haotong Wei
{"title":"Perovskite computed tomography imager and three-dimensional reconstruction","authors":"Yuhong He, Jinmei Song, Mingbian Li, Kostiantyn Sakhatskyi, Weijun Li, Xiaopeng Feng, Bai Yang, Maksym Kovalenko, Haotong Wei","doi":"10.1038/s41566-024-01506-y","DOIUrl":"10.1038/s41566-024-01506-y","url":null,"abstract":"Indirect scintillator computed tomography (CT) imaging suffers from reduced image contrast and high-dose X-ray exposure due to inevitable light losses and multiple energy conversion steps. Here we report a direct lead-halide perovskite CT imager through low-cost spray-coating processes. Detector arrays with 980 μm absorber thickness and <10 nm surface roughness yield uniform X-ray response with detection quantum efficiency of 80% and noise-equivalent dose of 153 pGyair. The perovskite CT imager affords the three-dimensional reconstruction of a tooth under a low effective dose of 5.5 μSv, about two orders of magnitude smaller than dental cone-beam CT, and low-contrast detectability by resolving a 5 Hounsfield unit difference within a 5 mm region of interest. A direct lead-halide perovskite CT imager has been demonstrated. The detector arrays have 980 μm absorber thickness and exhibit detection quantum efficiency of 80% and noise-equivalent dose of 153 pGyair.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 10","pages":"1052-1058"},"PeriodicalIF":32.3,"publicationDate":"2024-08-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141992023","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Multi-spectral reflection matrix for ultrafast 3D label-free microscopy 用于超快三维无标记显微镜的多光谱反射矩阵
IF 32.3 1区 物理与天体物理
Nature Photonics Pub Date : 2024-08-16 DOI: 10.1038/s41566-024-01479-y
Paul Balondrade, Victor Barolle, Nicolas Guigui, Emeric Auriant, Nathan Rougier, Claude Boccara, Mathias Fink, Alexandre Aubry
{"title":"Multi-spectral reflection matrix for ultrafast 3D label-free microscopy","authors":"Paul Balondrade, Victor Barolle, Nicolas Guigui, Emeric Auriant, Nathan Rougier, Claude Boccara, Mathias Fink, Alexandre Aubry","doi":"10.1038/s41566-024-01479-y","DOIUrl":"10.1038/s41566-024-01479-y","url":null,"abstract":"Label-free microscopy exploits light scattering to obtain a three-dimensional image of biological tissues. However, light propagation is affected by aberrations and multiple scattering, which drastically degrade the image quality and limit the penetration depth. Multi-conjugate adaptive optics and time-gated matrix approaches have been developed to compensate for aberrations but the associated frame rate is extremely limited for three-dimensional imaging. Here we develop a multi-spectral matrix approach to solve these fundamental problems. On the basis of a sparse illumination scheme and an interferometric measurement of the reflected wave field at multiple wavelengths, the focusing process can be optimized in post-processing for any voxel by addressing independently each frequency component of the reflection matrix. A proof-of-concept experiment shows a three-dimensional image of an opaque human cornea over a 0.1 mm3 field of view at a 290 nm resolution and a 1 Hz frame rate. This work paves the way towards a fully digital microscope allowing real-time, in vivo, quantitative and deep inspection of tissues. Based on the acquisition of a multi-spectral reflection matrix at a high frame rate, a fully digital microscope overcomes aberrations and multiple scattering to provide a three-dimensional image of an ex vivo opaque cornea at a resolution of 0.29 μm and 0.5 μm in the transverse and axial directions, respectively.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 10","pages":"1097-1104"},"PeriodicalIF":32.3,"publicationDate":"2024-08-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141992022","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Author Correction: Sub-femtonewton force sensing in solution by super-resolved photonic force microscopy 作者更正:利用超分辨光子力显微镜感测溶液中的亚微顿力
IF 32.3 1区 物理与天体物理
Nature Photonics Pub Date : 2024-08-15 DOI: 10.1038/s41566-024-01518-8
Xuchen Shan, Lei Ding, Dajing Wang, Shihui Wen, Jinlong Shi, Chaohao Chen, Yang Wang, Hongyan Zhu, Zhaocun Huang, Shen S. J. Wang, Xiaolan Zhong, Baolei Liu, Peter John Reece, Wei Ren, Weichang Hao, Xunyu Lu, Jie Lu, Qian Peter Su, Lingqian Chang, Lingdong Sun, Dayong Jin, Lei Jiang, Fan Wang
{"title":"Author Correction: Sub-femtonewton force sensing in solution by super-resolved photonic force microscopy","authors":"Xuchen Shan, Lei Ding, Dajing Wang, Shihui Wen, Jinlong Shi, Chaohao Chen, Yang Wang, Hongyan Zhu, Zhaocun Huang, Shen S. J. Wang, Xiaolan Zhong, Baolei Liu, Peter John Reece, Wei Ren, Weichang Hao, Xunyu Lu, Jie Lu, Qian Peter Su, Lingqian Chang, Lingdong Sun, Dayong Jin, Lei Jiang, Fan Wang","doi":"10.1038/s41566-024-01518-8","DOIUrl":"10.1038/s41566-024-01518-8","url":null,"abstract":"","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 9","pages":"998-998"},"PeriodicalIF":32.3,"publicationDate":"2024-08-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s41566-024-01518-8.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142137899","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Gate-tunable optical anisotropy in wafer-scale, aligned carbon nanotube films 晶圆级排列碳纳米管薄膜中的栅极可调光学各向异性
IF 32.3 1区 物理与天体物理
Nature Photonics Pub Date : 2024-08-14 DOI: 10.1038/s41566-024-01504-0
Jason Lynch, Evan Smith, Adam Alfieri, Baokun Song, Matthew Klein, Christopher E. Stevens, Cindy Yueli Chen, Chavez FK. Lawrence, Cherie R. Kagan, Honggang Gu, Shiyuan Liu, Lian-Mao Peng, Shivashankar Vangala, Joshua R. Hendrickson, Deep Jariwala
{"title":"Gate-tunable optical anisotropy in wafer-scale, aligned carbon nanotube films","authors":"Jason Lynch, Evan Smith, Adam Alfieri, Baokun Song, Matthew Klein, Christopher E. Stevens, Cindy Yueli Chen, Chavez FK. Lawrence, Cherie R. Kagan, Honggang Gu, Shiyuan Liu, Lian-Mao Peng, Shivashankar Vangala, Joshua R. Hendrickson, Deep Jariwala","doi":"10.1038/s41566-024-01504-0","DOIUrl":"10.1038/s41566-024-01504-0","url":null,"abstract":"Telecommunications and polarimetry both require the active control of the polarization of light. Currently, this is done by combining intrinsically anisotropic materials with tunable isotropic materials into heterostructures using complicated fabrication techniques owing to the lack of scalable materials that possess both properties. Tunable birefringent and dichromic materials are scarce and rarely available in high-quality thin films over wafer scales. Here we report semiconducting, highly aligned, single-walled carbon nanotubes (SWCNTs) over 4″ wafers with normalized birefringence and dichroism values of 0.09 and 0.58, respectively. The real and imaginary parts of the refractive index of these SWCNT films are tuned by up to 5.9% and 14.3% in the infrared at 2,200 nm and 1,660 nm, respectively, using electrostatic doping. Our results suggest that aligned SWCNTs are among the most anisotropic and tunable optical materials known and open new avenues for their application in integrated photonics and telecommunications. Using electrostatic doping, the real and imaginary parts of the refractive index along the extraordinary axis of semiconducting, highly aligned, single-walled carbon nanotubes over 4″ wafers can be tuned by up to 5.9% and 14.3% in the infrared at 2,200 nm and 1,660 nm, respectively.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 11","pages":"1176-1184"},"PeriodicalIF":32.3,"publicationDate":"2024-08-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141980915","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Observation of Floquet states and their dephasing in colloidal nanoplatelets driven by visible pulses 观察可见光脉冲驱动的胶体纳米微粒中的 Floquet 状态及其相消现象
IF 32.3 1区 物理与天体物理
Nature Photonics Pub Date : 2024-08-13 DOI: 10.1038/s41566-024-01505-z
Yuxuan Li, Yupeng Yang, Yuan Liu, Jingyi Zhu, Kaifeng Wu
{"title":"Observation of Floquet states and their dephasing in colloidal nanoplatelets driven by visible pulses","authors":"Yuxuan Li, Yupeng Yang, Yuan Liu, Jingyi Zhu, Kaifeng Wu","doi":"10.1038/s41566-024-01505-z","DOIUrl":"10.1038/s41566-024-01505-z","url":null,"abstract":"Coherent interaction between light and matter generates photon-dressed replicas of the original electronic levels (that is, Floquet states). This opens up a so-called field of Floquet engineering that applies electromagnetic fields to create new non-equilibrium phases of solid-state materials. The direct observation of such Floquet states, which often requires low-temperature, high-vacuum housing of the interrogated materials and low-energy infrared photons or microwaves as the driver, has been challenging. Here we report the observation of Floquet states in CdSe nanoplatelets, which are the colloidal analogue of quantum wells, under ambient conditions using femtosecond transient absorption. A sub-bandgap visible photon dresses a heavy-hole state (|hh1〉) to a Floquet state (|hh1 + ℏωL〉) that can hybridize with the first quantized electron state (|e1〉). This enables us to probe the Floquet state using a near-infrared photon through its transition to the second quantized electron state (|e2〉). Dephasing of the Floquet state into the real population of |e1〉 is also directly observed with a dephasing time of a few hundred femtoseconds, which is well reproduced by our density matrix simulations. Researchers demonstrate the ambient-condition observation of Floquet states in CdSe nanoplatelets, a colloidal analogue of quantum wells.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 10","pages":"1044-1051"},"PeriodicalIF":32.3,"publicationDate":"2024-08-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141974152","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Chiral topological light for detection of robust enantiosensitive observables 用于检测稳健对映敏感观测值的手性拓扑光
IF 32.3 1区 物理与天体物理
Nature Photonics Pub Date : 2024-08-13 DOI: 10.1038/s41566-024-01499-8
Nicola Mayer, David Ayuso, Piero Decleva, Margarita Khokhlova, Emilio Pisanty, Misha Ivanov, Olga Smirnova
{"title":"Chiral topological light for detection of robust enantiosensitive observables","authors":"Nicola Mayer, David Ayuso, Piero Decleva, Margarita Khokhlova, Emilio Pisanty, Misha Ivanov, Olga Smirnova","doi":"10.1038/s41566-024-01499-8","DOIUrl":"10.1038/s41566-024-01499-8","url":null,"abstract":"The topological response of matter to electromagnetic fields is a highly demanded property in materials design and metrology due to its robustness against noise and decoherence, stimulating recent advances in ultrafast photonics. Embedding topological properties into the enantiosensitive optical response of chiral molecules could therefore enhance the efficiency and robustness of chiral optical discrimination. Here we achieve such a topological embedding by introducing the concept of chiral topological light—a light beam which displays chirality locally, with an azimuthal distribution of its handedness described globally by a topological charge. The topological charge is mapped onto the azimuthal intensity modulation of the non-linear optical response, where enantiosensitivity is encoded into its spatial rotation. The spatial rotation is robust against intensity fluctuations and imperfect local polarization states of the driving field. Our theoretical results show that chiral topological light enables detection of percentage-level enantiomeric excesses in randomly oriented mixtures of chiral molecules, opening a way to new, extremely sensitive and robust chiro-optical spectroscopies with attosecond time resolution. The concept of chiral topological light—a polychromatic light with chiral closed 3D polarization trajectories, space-varying with the azimuthal angle—is introduced and used for efficient sensing in chiral molecules, showcasing an example of successful application of topological concepts in optics.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 11","pages":"1155-1160"},"PeriodicalIF":32.3,"publicationDate":"2024-08-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s41566-024-01499-8.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141974153","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Bose–Einstein condensation of photons in a vertical-cavity surface-emitting laser 垂直腔表面发射激光器中光子的玻色-爱因斯坦凝聚
IF 32.3 1区 物理与天体物理
Nature Photonics Pub Date : 2024-08-12 DOI: 10.1038/s41566-024-01478-z
Maciej Pieczarka, Marcin Gębski, Aleksandra N. Piasecka, James A. Lott, Axel Pelster, Michał Wasiak, Tomasz Czyszanowski
{"title":"Bose–Einstein condensation of photons in a vertical-cavity surface-emitting laser","authors":"Maciej Pieczarka, Marcin Gębski, Aleksandra N. Piasecka, James A. Lott, Axel Pelster, Michał Wasiak, Tomasz Czyszanowski","doi":"10.1038/s41566-024-01478-z","DOIUrl":"10.1038/s41566-024-01478-z","url":null,"abstract":"Many bosons can occupy a single quantum state without a limit. It is described by the quantum-mechanical Bose–Einstein statistic, which allows Bose–Einstein condensation at low temperatures and high particle densities. Photons, historically the first considered bosonic gas, were late to show this phenomenon, observed in rhodamine-filled microcavities and doped fibre cavities. These findings have raised the question of whether condensation is also common in other laser systems with potential technological applications. Here we show the Bose–Einstein condensation of photons in a broad-area vertical-cavity surface-emitting laser with a slight cavity-gain spectral detuning. We observed a Bose–Einstein condensate in the fundamental transversal optical mode at a critical phase-space density. The experimental results follow the equation of state for a two-dimensional gas of bosons in thermal equilibrium, although the extracted spectral temperatures were lower than the device’s. This is interpreted as originating from the driven-dissipative nature of the photon gas. In contrast, non-equilibrium lasing action is observed in the higher-order modes in more negatively detuned device. Our work opens the way for the potential exploration of superfluid physics of interacting photons mediated by semiconductor optical nonlinearities. It also shows great promise for enabling single-mode high-power emission from a large-aperture device. Bose–Einstein condensation of photons is demonstrated in a large-aperture electrically driven InGaAs vertical-cavity surface-emitting laser diode at room temperature. The observed photon Bose–Einstein condensate exhibits the fundamental transversal optical mode at a critical phase-space density.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 10","pages":"1090-1096"},"PeriodicalIF":32.3,"publicationDate":"2024-08-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s41566-024-01478-z.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141918855","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Bose–Einstein condensation of light in a semiconductor quantum well microcavity 光在半导体量子阱微腔中的玻色-爱因斯坦凝聚
IF 32.3 1区 物理与天体物理
Nature Photonics Pub Date : 2024-08-12 DOI: 10.1038/s41566-024-01491-2
Ross C. Schofield, Ming Fu, Edmund Clarke, Ian Farrer, Aristotelis Trapalis, Himadri S. Dhar, Rick Mukherjee, Toby Severs Millard, Jon Heffernan, Florian Mintert, Robert A. Nyman, Rupert F. Oulton
{"title":"Bose–Einstein condensation of light in a semiconductor quantum well microcavity","authors":"Ross C. Schofield, Ming Fu, Edmund Clarke, Ian Farrer, Aristotelis Trapalis, Himadri S. Dhar, Rick Mukherjee, Toby Severs Millard, Jon Heffernan, Florian Mintert, Robert A. Nyman, Rupert F. Oulton","doi":"10.1038/s41566-024-01491-2","DOIUrl":"10.1038/s41566-024-01491-2","url":null,"abstract":"When particles with integer spin accumulate at low temperature and high density, they undergo Bose–Einstein condensation (BEC). Atoms, magnons, solid-state excitons, surface plasmon polaritons and excitons coupled to light exhibit BEC, which results in high coherence due to massive occupation of the respective system’s ground state. Surprisingly, photons were shown to exhibit BEC recently in organic-dye-filled optical microcavities, which—owing to the photon’s low mass—occurs at room temperature. Here we demonstrate that photons within an inorganic semiconductor microcavity also thermalize and undergo BEC. Although semiconductor lasers are understood to operate out of thermal equilibrium, we identify a region of good thermalization in our system where we can clearly distinguish laser action from BEC. Semiconductor microcavities are a robust system for exploring the physics and applications of quantum statistical photon condensates. In practical terms, photon BECs offer their critical behaviour at lower thresholds than lasers. Our study shows two further advantages: the lack of dark electronic states in inorganic semiconductors allows these BECs to be sustained continuously; and quantum wells offer stronger photon–photon scattering. We measure an unoptimized interaction parameter ( $$tilde{{{{{g}}}}}$$  ≳ 10–3), which is large enough to access the rich physics of interactions within BECs, such as superfluid light. Photon Bose–Einstein condensation is observed in a semiconductor laser, where thermalization and condensation of photons occur using an InGaAs quantum well and an open microcavity. The distinction between regimes of photon Bose–Einstein condensation and conventional lasing are clearly identified.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 10","pages":"1083-1089"},"PeriodicalIF":32.3,"publicationDate":"2024-08-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s41566-024-01491-2.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141918854","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
An 8 × 160 Gb s−1 all-silicon avalanche photodiode chip 8 × 160 Gb s-1 全硅雪崩光电二极管芯片
IF 32.3 1区 物理与天体物理
Nature Photonics Pub Date : 2024-08-09 DOI: 10.1038/s41566-024-01495-y
Yiwei Peng, Yuan Yuan, Wayne V. Sorin, Stanley Cheung, Zhihong Huang, Chaerin Hong, Di Liang, Marco Fiorentino, Raymond G. Beausoleil
{"title":"An 8 × 160 Gb s−1 all-silicon avalanche photodiode chip","authors":"Yiwei Peng, Yuan Yuan, Wayne V. Sorin, Stanley Cheung, Zhihong Huang, Chaerin Hong, Di Liang, Marco Fiorentino, Raymond G. Beausoleil","doi":"10.1038/s41566-024-01495-y","DOIUrl":"10.1038/s41566-024-01495-y","url":null,"abstract":"In response to growing demands on data traffic, silicon (Si) photonics has emerged as a promising technology for ultra-high-speed and low-cost optical interconnects. However, achieving high-performance photodetectors with Si photonics requires integrating narrower-bandgap materials, resulting in more complex fabrication processes, higher costs and yield issues. To address this challenge, we demonstrate an all-Si receiver (RX) based on a cost-efficient, eight-channel, double-microring-resonator, avalanche photodiode. It has an aggregate data rate of 1.28 Tb s−1. All channels show excellent uniformity in their device performance with a responsivity of 0.4 A W−1, an ultra-low dark current of 1 nA, a high bandwidth of 40 GHz at −8 V and a $$k$$ value of 0.28. To the best of our knowledge, this is the first demonstration of an all-Si RX supporting a record-high transmission data rate of 160 Gb s−1 per channel, along with an ultra-low electrical crosstalk of less than −50 dB. This all-Si optical RX can compete with the commercial heterojunction-based RXs and promises ~40% chip cost saving, thus paving the way to realizing >3.2 Tb s−1 interconnects for future optical networks. Researchers demonstrate a receiver based on an all-Si eight-channel avalanche photodiode, which operates at a data rate of 160 Gb s−1 per channel and has an aggregate rate of 1.28 Tb s−1.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 9","pages":"928-934"},"PeriodicalIF":32.3,"publicationDate":"2024-08-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141909226","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Colossal in-plane optical anisotropy in a two-dimensional van der Waals crystal 二维范德华晶体中巨大的面内光学各向异性
IF 32.3 1区 物理与天体物理
Nature Photonics Pub Date : 2024-08-08 DOI: 10.1038/s41566-024-01501-3
Qiangbing Guo, Qiuhong Zhang, Tan Zhang, Jun Zhou, Shumin Xiao, Shijie Wang, Yuan Ping Feng, Cheng-Wei Qiu
{"title":"Colossal in-plane optical anisotropy in a two-dimensional van der Waals crystal","authors":"Qiangbing Guo, Qiuhong Zhang, Tan Zhang, Jun Zhou, Shumin Xiao, Shijie Wang, Yuan Ping Feng, Cheng-Wei Qiu","doi":"10.1038/s41566-024-01501-3","DOIUrl":"10.1038/s41566-024-01501-3","url":null,"abstract":"Polarization, a fundamental property of light, has been widely exploited from quantum physics to high-dimensional optics. Materials with intrinsic optical anisotropy, such as dichroism and birefringence, are central to light polarization control, including the development of polarizers, waveplates, mirrors and phase-matching elements. Therefore, materials with strong optical anisotropy have been long-sought. Recently, two-dimensional van der Waals crystals show high optical anisotropy but are mostly restricted to the out-of-plane direction, which is challenging to access in optical engineering. Here we report a two-dimensional van der Waals material, NbOCl2, that exhibits sharp electronic and structural contrast between its in-plane orthogonal axes. Colossal in-plane optical anisotropy—linear dichroism (up to 99% in ultraviolet) and birefringence (0.26–0.46 within a wide visible–near-infrared transparency window)—is experimentally demonstrated. Our findings provide a powerful and easy-to-access recipe for ultracompact integrated polarization industries. A two-dimensional van der Waals material, NbOCl2, that simultaneously exhibits near-unity linear dichroism (~99%) over 100 nm bandwidth in ultraviolet regime and large birefringence (0.26–0.46) within a wide visible–near-infrared transparency window is reported.","PeriodicalId":18926,"journal":{"name":"Nature Photonics","volume":"18 11","pages":"1170-1175"},"PeriodicalIF":32.3,"publicationDate":"2024-08-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141904675","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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