Journal of Quantitative Spectroscopy & Radiative Transfer最新文献

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Global carbon monoxide retrieval from the hyperspectral infrared atmospheric sounder-II onboard FengYun-3E in a dawn-dusk sun-synchronous orbit 从黎明-黄昏太阳同步轨道上的风云- 3e上的高光谱红外大气探测仪- ii获取全球一氧化碳
IF 2.3 3区 物理与天体物理
Journal of Quantitative Spectroscopy & Radiative Transfer Pub Date : 2024-12-30 DOI: 10.1016/j.jqsrt.2024.109336
Zhao-Cheng Zeng
{"title":"Global carbon monoxide retrieval from the hyperspectral infrared atmospheric sounder-II onboard FengYun-3E in a dawn-dusk sun-synchronous orbit","authors":"Zhao-Cheng Zeng","doi":"10.1016/j.jqsrt.2024.109336","DOIUrl":"10.1016/j.jqsrt.2024.109336","url":null,"abstract":"<div><div>This study presents an information content analysis of the retrieval of global carbon monoxide (CO) from the 2<sup>nd</sup> generation of Hyperspectral Infrared Atmospheric Sounder on board Fengyun-3E (FY-3E/HIRAS-II), which is the world's first dawn-dusk orbiting meteorological satellite for civilian use with equatorial overpass times at about 5:30am/pm. Using the distinctive absorption features of CO around 2145 cm-1 in the infrared band, a retrieval algorithm based on optimal estimation is first developed to retrieve the CO profiles from FY-3E/HIRAS-II. The thermal contrast, defined as the temperature difference between the surface and the lower atmosphere, is then examined for the FY-3E/HIRAS-II observations to investigate the potential sensitivity of the observations. Retrievals of CO columns on four representative days over four seasons reveal strong enhancements from global wildfire emissions. Furthermore, the information content from the spectra, quantified by the degree of freedom for signal (DOFS), is assessed using the retrievals. The retrievals are compared with model simulations, which show good agreement. Finally, synthetic experiments are performed to investigate the impacts of thermal contrast and the vertical structure of wildfire-induced CO enhancement on the observational sensitivity. The result highlights the effectiveness of observing wildfire-induced CO enhancement during the dawn and dusk hours, even when thermal contrast conditions are not favorable. This study demonstrates the capability of FY-3E/HIRAS-II to monitor global CO, which sheds light on the potential benefits of adding dawn-dusk orbit observations to the current global air quality observations from mid-morning and early-afternoon orbit constellations.</div></div>","PeriodicalId":16935,"journal":{"name":"Journal of Quantitative Spectroscopy & Radiative Transfer","volume":"333 ","pages":"Article 109336"},"PeriodicalIF":2.3,"publicationDate":"2024-12-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142929289","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Atmospheric Chemistry Experiment (ACE) satellite observations of aerosols and SO2 emissions from the 2024 Ruang volcanic eruption 2024年阮氏火山喷发气溶胶和SO[公式省略]排放的大气化学实验(ACE)卫星观测
IF 2.3 3区 物理与天体物理
Journal of Quantitative Spectroscopy & Radiative Transfer Pub Date : 2024-12-28 DOI: 10.1016/j.jqsrt.2024.109333
Randika Dodangodage , Peter F. Bernath , Matthew Wyatt , Chris Boone
{"title":"Atmospheric Chemistry Experiment (ACE) satellite observations of aerosols and SO2 emissions from the 2024 Ruang volcanic eruption","authors":"Randika Dodangodage ,&nbsp;Peter F. Bernath ,&nbsp;Matthew Wyatt ,&nbsp;Chris Boone","doi":"10.1016/j.jqsrt.2024.109333","DOIUrl":"10.1016/j.jqsrt.2024.109333","url":null,"abstract":"<div><div>Indonesia’s Ruang volcano erupted on April 16, 2024, with subsequent eruptions on April 17 and 30. The resulting plume was observed rising to altitudes of up to 12 km. 10 days after the eruption of the Ruang volcano in April 2024, the Atmospheric Chemistry Experiment (ACE) observed notable increases in SO<span><math><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub></math></span> volume mixing ratios and aerosol extinction at an altitude of approximately 20 km. It was confirmed that the aerosols present were sulfate aerosols from their infrared spectra. The composition and size of the stratospheric sulfate aerosol particles were determined by fitting the infrared transmission spectra. The sulfate aerosols observed in the plume were about 64% (by weight) sulfuric acid, and the droplets had an average median radius of 0.127 <span><math><mi>μ</mi></math></span>m.</div></div>","PeriodicalId":16935,"journal":{"name":"Journal of Quantitative Spectroscopy & Radiative Transfer","volume":"333 ","pages":"Article 109333"},"PeriodicalIF":2.3,"publicationDate":"2024-12-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142929288","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Ro-vibrational levels of acetylene isotopologues calculated from new potential energy surface 由新势能面计算的乙炔同位素的反振动能级
IF 2.3 3区 物理与天体物理
Journal of Quantitative Spectroscopy & Radiative Transfer Pub Date : 2024-12-28 DOI: 10.1016/j.jqsrt.2024.109337
Alexander E. Protasevich, Andrei V. Nikitin
{"title":"Ro-vibrational levels of acetylene isotopologues calculated from new potential energy surface","authors":"Alexander E. Protasevich,&nbsp;Andrei V. Nikitin","doi":"10.1016/j.jqsrt.2024.109337","DOIUrl":"10.1016/j.jqsrt.2024.109337","url":null,"abstract":"<div><div>Ro-vibrational energy levels of acetylene isotopologues are reported using variational nuclear motion calculations from empirically optimized full six-dimensional potential energy surface (PES) in the ground electronic state. This surface is based on pure ab initio PES of H<sup>12</sup>C<sup>12</sup>CH which took into account the triple, quadruple and quintuple excitations as well as relativistic and diagonal Born-Oppenheimer corrections (DBOC). Variational calculations of the motion of nuclei for all isotopologues were carried out using one exact kinetic energy operator in which only the masses of the atoms were changed. Experimental values of 1529 ro-vibrational levels up to <em>J</em> = 10 of the main isotopologue were used to empirically adjust some 58 lower-order parameters of the PES. The unweighted average RMS for empirically optimized PES is 0.0953 cm<sup>−1</sup>. Ro-vibrational energy levels of H<sup>12</sup>C<sup>12</sup>CH, H<sup>13</sup>C<sup>13</sup>CH, D<sup>12</sup>C<sup>12</sup>CD, D<sup>13</sup>C<sup>13</sup>CD, H<sup>12</sup>C<sup>13</sup>CH, H<sup>12</sup>C<sup>12</sup>CD, H<sup>12</sup>C<sup>13</sup>CD, H<sup>13</sup>C<sup>12</sup>CD, D<sup>12</sup>C<sup>13</sup>CD up to <em>J</em> = 10 were calculated in the ground electronic state. Calculated ro-vibrational energy levels of H<sup>12</sup>C<sup>12</sup>CH, H<sup>13</sup>C<sup>13</sup>CH, D<sup>12</sup>C<sup>12</sup>CD, H<sup>12</sup>C<sup>13</sup>CH, H<sup>12</sup>C<sup>12</sup>CD isotopologues were compared with high precision empirical energy levels available in literature.</div></div>","PeriodicalId":16935,"journal":{"name":"Journal of Quantitative Spectroscopy & Radiative Transfer","volume":"333 ","pages":"Article 109337"},"PeriodicalIF":2.3,"publicationDate":"2024-12-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142929287","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The contribution of scattered radiation to the upward radiance of a city 散射辐射对城市向上辐射的贡献
IF 2.3 3区 物理与天体物理
Journal of Quantitative Spectroscopy & Radiative Transfer Pub Date : 2024-12-26 DOI: 10.1016/j.jqsrt.2024.109330
Jaromír Petržala, Ladislav Kómar
{"title":"The contribution of scattered radiation to the upward radiance of a city","authors":"Jaromír Petržala,&nbsp;Ladislav Kómar","doi":"10.1016/j.jqsrt.2024.109330","DOIUrl":"10.1016/j.jqsrt.2024.109330","url":null,"abstract":"<div><div>Remote sensing of nighttime urban light emissions becomes a common part of light pollution modeling. Radiance data gathered by various satellites scanning the Earth surface serve as important inputs for estimating the upward luminous flux of a city, which then allows to evaluate the level of light pollution in its surroundings. The easiest way is to assume the measured radiance of a city pixel as belonging to its direct radiation. However, this radiance is ”contaminated” by scattered radiation coming from the light emitting surroundings of the pixel. In principle, this diffuse light contribution can influence the estimate of the emitted flux. In this paper, we developed a model to assess how important such a contribution can be for cities of different shapes and sizes. The numerical simulations for real city patterns obtained from the VIIRS-DNB database reveal, that scattered radiation could make up on average about 10%–20% of the total upward radiance of a pixel under quite obvious aerosol conditions. We have also derived two simplified models for idealized city patterns which enable relatively simple estimation of the diffuse radiation contribution without the need of complex simulations for realistic cities.</div></div>","PeriodicalId":16935,"journal":{"name":"Journal of Quantitative Spectroscopy & Radiative Transfer","volume":"333 ","pages":"Article 109330"},"PeriodicalIF":2.3,"publicationDate":"2024-12-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142929290","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Global distributions of multi-layer and multi-phase clouds and their cloud radiative effects 多层多相云的全球分布及其云辐射效应
IF 2.3 3区 物理与天体物理
Journal of Quantitative Spectroscopy & Radiative Transfer Pub Date : 2024-12-26 DOI: 10.1016/j.jqsrt.2024.109334
Bingqi Yi , Ruiyi Li , Zhiyong Yang
{"title":"Global distributions of multi-layer and multi-phase clouds and their cloud radiative effects","authors":"Bingqi Yi ,&nbsp;Ruiyi Li ,&nbsp;Zhiyong Yang","doi":"10.1016/j.jqsrt.2024.109334","DOIUrl":"10.1016/j.jqsrt.2024.109334","url":null,"abstract":"<div><div>Accurate and reliable knowledge about how clouds with various layers and phases are vertically and horizontally distributed over the globe has been lacking, which hinders the understanding about the impacts of various sub-types of clouds. This study utilizes the cloud retrieval products from the CloudSat/CALIPSO satellite observations from 2007 to 2010 to analyze the global distributions of multi-layer and multi-phase clouds as well as their cloud radiative effects (CRE) at the top of the atmosphere (TOA), at the surface, and within the atmosphere. We separate and aggregate cloudy satellite footprints by the number of cloud layers, and further consider the different combinations of cloud phases for the one-layer and multi-layer clouds. The globally averaged total cloud fraction is 72.52 %, with the one-layer and multi-layer clouds take up 49.39 % and 23.13 %, respectively. The one-layer water, ice, and mixed-phase cloud fractions are 21.93 %, 19.42 %, and 8.04 %, respectively. The two-layer and three-layer clouds most frequently occur with one ice layer at the top. The heights of cloud top and bottom as well as the cloud thickness are correspondingly derived for all sub-types of clouds. The globally averaged TOA net total CRE is −18.25 W m<sup>−2</sup>, with −14.63 W m<sup>−2</sup> attributed to one-layer clouds and −3.62 W m<sup>−2</sup> to multi-layer clouds. At the surface, the global annual average net total CRE is −25.01 W m<sup>−2</sup>, and the one-layer and multi-layer clouds contribute −17.24 W m<sup>−2</sup> and −7.77 W m<sup>−2</sup>, respectively. Clouds generally exert a net heating effect within the atmosphere. Our findings provide valuable insights into the detailed layer and phase structures of clouds and could serve as the reference for evaluating cloud structure and radiation simulations.</div></div>","PeriodicalId":16935,"journal":{"name":"Journal of Quantitative Spectroscopy & Radiative Transfer","volume":"333 ","pages":"Article 109334"},"PeriodicalIF":2.3,"publicationDate":"2024-12-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142889185","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Absorption spectroscopy of AlO including photodissociation 含光解作用的AlO吸收光谱
IF 2.3 3区 物理与天体物理
Journal of Quantitative Spectroscopy & Radiative Transfer Pub Date : 2024-12-25 DOI: 10.1016/j.jqsrt.2024.109335
Tianrui Bai , Lynette Edline Momo Jeulefack , Songfeng Li , Jie Cheng , Shuidong Dai , Linhua Liu , Fei Li
{"title":"Absorption spectroscopy of AlO including photodissociation","authors":"Tianrui Bai ,&nbsp;Lynette Edline Momo Jeulefack ,&nbsp;Songfeng Li ,&nbsp;Jie Cheng ,&nbsp;Shuidong Dai ,&nbsp;Linhua Liu ,&nbsp;Fei Li","doi":"10.1016/j.jqsrt.2024.109335","DOIUrl":"10.1016/j.jqsrt.2024.109335","url":null,"abstract":"<div><div>Photodissociation of AlO may be important for the aluminium chemistry in various astrophysical regions. The photodissociation cross sections and rates of AlO were investigated over the temperature range from 0 to 15000 K in this work. Firstly, the state-resolved cross sections at the wavelength of 50 − 5000 nm for transitions from the ground and first excited states were calculated using <em>ab initio</em> potential energy curves and transition dipole moments. The temperature-dependent cross sections were then obtained by assuming a Boltzmann distribution to describe the population of the initial state. Several common radiation fields (interstellar, solar and blackbody radiation field) were selected as the radiation fields, and then the photodissociation rates in different radiation fields were obtained. The photodissociation rates in all studied radiation fields exhibit a positive correlation with increasing temperature. This finding indicates that the total photodissociation rates are sensitive to the temperature. In addition, the photodissociation rates in the solar radiation field are higher than those in the interstellar radiation fields, indicating that photodissociation rate is associated with the type of radiation field in which the molecule is exposed. The calculated photodissociation cross sections and rates of AlO are useful to investigate the chemical evolution of the aluminum element in the interstellar environment.</div></div>","PeriodicalId":16935,"journal":{"name":"Journal of Quantitative Spectroscopy & Radiative Transfer","volume":"333 ","pages":"Article 109335"},"PeriodicalIF":2.3,"publicationDate":"2024-12-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142929291","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Deep sub-wavelength scale focusing of heat flux radiated by magneto-optical nanoemitters in the presence of an external magnetic-field 外磁场存在下磁光纳米发射器辐射热流的深亚波长尺度聚焦
IF 2.3 3区 物理与天体物理
Journal of Quantitative Spectroscopy & Radiative Transfer Pub Date : 2024-12-24 DOI: 10.1016/j.jqsrt.2024.109322
Louis Rihouey, Philippe Ben-Abdallah, Riccardo Messina
{"title":"Deep sub-wavelength scale focusing of heat flux radiated by magneto-optical nanoemitters in the presence of an external magnetic-field","authors":"Louis Rihouey,&nbsp;Philippe Ben-Abdallah,&nbsp;Riccardo Messina","doi":"10.1016/j.jqsrt.2024.109322","DOIUrl":"10.1016/j.jqsrt.2024.109322","url":null,"abstract":"<div><div>We introduce a theoretical framework to describe the heat flux radiated in the near-field regime by a set of magneto-optical thermal nanoemitters close to a substrate in the presence of an external magnetic field. Then, we investigate the particular case of a single emitter and we demonstrate that the external field can induce both an amplification of the heat exchanged between emittter and substrate and a focusing of the Poynting field at the substrate interface at deep sub-wavelength scale. These effects open up promising perspectives for the development of heat-assisted magnetic-recording technology.</div></div>","PeriodicalId":16935,"journal":{"name":"Journal of Quantitative Spectroscopy & Radiative Transfer","volume":"333 ","pages":"Article 109322"},"PeriodicalIF":2.3,"publicationDate":"2024-12-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142929293","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Updating the carbon dioxide line list in HITEMP 更新HITEMP中的二氧化碳行列表
IF 2.3 3区 物理与天体物理
Journal of Quantitative Spectroscopy & Radiative Transfer Pub Date : 2024-12-24 DOI: 10.1016/j.jqsrt.2024.109324
Robert J. Hargreaves , Iouli E. Gordon , Xinchuan Huang , Geoffrey C. Toon , Laurence S. Rothman
{"title":"Updating the carbon dioxide line list in HITEMP","authors":"Robert J. Hargreaves ,&nbsp;Iouli E. Gordon ,&nbsp;Xinchuan Huang ,&nbsp;Geoffrey C. Toon ,&nbsp;Laurence S. Rothman","doi":"10.1016/j.jqsrt.2024.109324","DOIUrl":"10.1016/j.jqsrt.2024.109324","url":null,"abstract":"<div><div>An updated carbon dioxide line list for the HITEMP spectroscopic database is presented. This line list covers the 0–17<!--> <!-->697 cm<sup>−1</sup> (<span><math><mo>&gt;</mo></math></span>565 nm) spectral range and is built upon the AI-3000K semi-empirical line list for <sup>12</sup>C<sup>16</sup>O<sub>2</sub>, <sup>13</sup>C<sup>16</sup>O<sub>2</sub>, <sup>16</sup>O<sup>12</sup>C<sup>18</sup>O, and <sup>16</sup>O<sup>12</sup>C<sup>17</sup>O (Huang et al., 2023), combined with HITRAN2020 data, additional isotopologues, and further improvements described in this work. In order to make the line list practical for applications, over 36 billion individual transitions of the original AI-3000K line list have been separated into “strong” and “weak”. “Strong” transitions were adapted directly, while the weak transitions were then combined into so-called “effective” lines. The latter can accurately account for the intensity contribution of underlying weak AI-3000K transitions while reducing the database by over two orders of magnitude (to <span><math><mo>∼</mo></math></span>326 million). In addition, pressure broadening parameters have been revised for this work to improve applicability at high temperatures. The line list has been added to HITEMP and is suitable for modeling the spectrum of carbon dioxide at temperatures up to 3000 K.</div><div>Multiple validations have been carried out against terrestrial CO<sub>2</sub> retrievals, as well as high-resolution experimental measurements of CO<sub>2</sub> at different temperatures (up to 2000 K). The updated HITEMP line list includes 12 isotopologues of CO<sub>2</sub> and is provided in the standard HITRAN/HITEMP format, which is accepted by many community tools. It is demonstrated to be practical, accurate, and sufficiently complete for high-temperature environments. This work will be suitable for various high-temperature spectroscopic applications including exoplanet retrievals and remote sensing of combustion environments.</div></div>","PeriodicalId":16935,"journal":{"name":"Journal of Quantitative Spectroscopy & Radiative Transfer","volume":"333 ","pages":"Article 109324"},"PeriodicalIF":2.3,"publicationDate":"2024-12-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142929292","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Statistical simulation of the angular distribution of reflected solar radiation in optically anisotropic ice-crystal clouds: Horizontally oriented particles 光学各向异性冰晶云中反射太阳辐射角分布的统计模拟:水平取向粒子
IF 2.3 3区 物理与天体物理
Journal of Quantitative Spectroscopy & Radiative Transfer Pub Date : 2024-12-22 DOI: 10.1016/j.jqsrt.2024.109327
Tatiana Zhuravleva
{"title":"Statistical simulation of the angular distribution of reflected solar radiation in optically anisotropic ice-crystal clouds: Horizontally oriented particles","authors":"Tatiana Zhuravleva","doi":"10.1016/j.jqsrt.2024.109327","DOIUrl":"10.1016/j.jqsrt.2024.109327","url":null,"abstract":"<div><div>The results of statistical modeling of the angular characteristics of reflected solar radiation in the atmosphere containing a layer of ice crystal clouds with anisotropy caused by the orientation of particles in space are presented. Numerical experiments are carried out using (1) original algorithm of the Monte Carlo method for calculating characteristics of unpolarized solar radiation taking into account the multiple scattering, reflection from the underlying surface, and attenuation by aerosol particles and due to molecular scattering and (2) optical model of anisotropic medium, composed of horizontally oriented hexagonal plates or Parry columns (visible range), developed previously in Institute of Atmospheric Optics, Siberian Branch, Russian Academy of Sciences, Tomsk, Russia. We discuss the patterns of formation of reflected solar radiation without taking into account the aerosol-molecular component of the atmosphere and surface reflection; these simulation results make it possible to identify the specific features of radiative transfer, caused exclusively by the effects of anisotropy of ice-crystal clouds. The factors that determine the influence of the surface reflection and aerosol attenuation on halo phenomena are described. It is shown that, as the surface albedo increases, the near-isotropic radiation field is formed outside the main halo lines and the intensity of different halo lines decreases down to the level when these lines or their components become almost invisible against the background of the contribution formed by surface-reflected radiation. Our radiation code is to be used for a research into the optical phenomena, observed from the Earth's surface and space, and, in particular, for an additional study of scattering by oriented ice crystals near the specular reflection direction (solar glint).</div></div>","PeriodicalId":16935,"journal":{"name":"Journal of Quantitative Spectroscopy & Radiative Transfer","volume":"333 ","pages":"Article 109327"},"PeriodicalIF":2.3,"publicationDate":"2024-12-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142889186","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Using convolutional neural networks to predict the optical properties of coated black carbon 利用卷积神经网络预测涂覆黑碳的光学性质
IF 2.3 3区 物理与天体物理
Journal of Quantitative Spectroscopy & Radiative Transfer Pub Date : 2024-12-22 DOI: 10.1016/j.jqsrt.2024.109326
Zhenhai Qin, Jinhong Wu, Haihui Wang, Yongming Zhang, Qixing Zhang
{"title":"Using convolutional neural networks to predict the optical properties of coated black carbon","authors":"Zhenhai Qin,&nbsp;Jinhong Wu,&nbsp;Haihui Wang,&nbsp;Yongming Zhang,&nbsp;Qixing Zhang","doi":"10.1016/j.jqsrt.2024.109326","DOIUrl":"10.1016/j.jqsrt.2024.109326","url":null,"abstract":"<div><div>Black carbon (BC) is a type of light absorbing substances in atmosphere, which has a significant impact on regional and global radiation balance. When evaluating the climatic effects of BC, the complex morphology of BC poses a challenge for large-scale climate models to proceed with the calculations. In this study, we developed a deep convolutional neural network (CNN) that combines residual links with one-dimensional multi-scale dilated convolutions. Using the multiple sphere T-matrix (MSTM), the extinction efficiency (<em>Q<sub>ext</sub></em>), absorption efficiency (<em>Q<sub>abs</sub></em>), scattering efficiency (<em>Q<sub>sca</sub></em>), and asymmetry factor (<em>g</em>) for coated BC were evaluated under different fractal dimensions, monomer radii, refractive indices, and incident wavelengths, by considering the volume fraction of thinly coated BC and thickly coated BC in the range from 20 % to 60 % and 2 % to 10 %, respectively. The optical properties of small particles were then treated as the training set to train the CNN, and the trained CNN was used to output the optical properties of large particles. By comparing the <em>Q<sub>ext</sub>, Q<sub>abs</sub>, Q<sub>sca</sub></em>, and <em>g</em> predicted by the CNN with those obtained from the MSTM, we found that the CNN has superior predictive capabilities for the optical properties of coated BC, and the newly established CNN exhibited broad applicability in predicting the optical properties of coated BC. Although relative deviations are observed in predicting the optical properties of small particles using the CNN, the errors for large particle predictions are essentially &lt;1 %, with the mean absolute errors and root mean square errors being lower than 0.029 and 0.043, respectively. This study demonstrates that the CNN has great potential for further development. Future research should focus on how to use less data to predict more accurate results for the range of computational parameters for BC.</div></div>","PeriodicalId":16935,"journal":{"name":"Journal of Quantitative Spectroscopy & Radiative Transfer","volume":"333 ","pages":"Article 109326"},"PeriodicalIF":2.3,"publicationDate":"2024-12-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142889188","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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