Journal of Environmental Sciences-china最新文献

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Transcriptomic and biochemical analysis of the mechanism of sodium gluconate promoting the degradation of benzo [a] pyrene by Bacillus subtilis MSC4 葡萄糖酸钠促进枯草芽孢杆菌 MSC4 降解苯并 [a] 芘的转录组和生化分析机制
2区 环境科学与生态学
Journal of Environmental Sciences-china Pub Date : 2024-04-25 DOI: 10.1016/j.jes.2024.04.021
Rui Chen , Tangbing Cui
{"title":"Transcriptomic and biochemical analysis of the mechanism of sodium gluconate promoting the degradation of benzo [a] pyrene by Bacillus subtilis MSC4","authors":"Rui Chen ,&nbsp;Tangbing Cui","doi":"10.1016/j.jes.2024.04.021","DOIUrl":"10.1016/j.jes.2024.04.021","url":null,"abstract":"<div><p>Benzo[a]pyrene (B[a]P) is a carcinogenic environmental pollutant widely present in the environment and can enter the human body through the food chain. It is therefore essential to treat and remediate the B[a]P-contaminated environment. Microbial remediation of B[a]P-contaminated environments is considered to be one of the most effective strategies, and the addition of biostimulants is a feasible method to further improve the effectiveness of microbial remediation. In this study, we used <em>Bacillus subtilis</em> MSC4 to screen for the stimulation of sodium gluconate, which promoted B[a]P degradation. Based on biochemical and transcriptomic analyses, Sodium gluconate was found to significantly increase the biomass of MSC4 and the expression of most genes involved in B[a]P degradation. Activities of central carbon metabolism, fatty acid β-oxidation and oxidative phosphorylation were all promoted. The significant increase in acid-induced oxalate decarboxylase expression indicates a decrease in intracellular pH, which promoted the synthesis of acetoin and lactate. Genes involved in the nitrogen cycle, especially nitrification and denitrification, were significantly up-regulated, contributing to B[a]P degradation. Genes involved in the synthesis of enzyme cofactors, including thiamine, molybdenum cofactors, NAD and heme, were up-regulated, which contributes to increasing enzyme activity in metabolic pathways. Up-regulation of genes in flagella assembly, chemotaxis, and lipopeptide synthesis is beneficial for the dissolution and uptake of B[a]P. Genes related to the sugar transport system were upregulated, which facilitates the transport and absorption of monosaccharides and oligosaccharides by MSC4. This study provides a theoretical basis for the further application of sodium gluconate in the treatment of PAH-contaminated sites.</p></div>","PeriodicalId":15788,"journal":{"name":"Journal of Environmental Sciences-china","volume":"152 ","pages":"Pages 39-53"},"PeriodicalIF":0.0,"publicationDate":"2024-04-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140795336","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Stable partial nitrification was achieved for nitrogen removal from municipal wastewater by gel immobilization: A pilot-scale study 通过凝胶固定化技术实现了稳定的部分硝化,从而去除城市污水中的氮:中试规模研究
2区 环境科学与生态学
Journal of Environmental Sciences-china Pub Date : 2024-04-24 DOI: 10.1016/j.jes.2024.04.020
Xin Hu , Hong Yang , Xiaoyue Fang , Xuyan Liu , Jiawei Wang , Xiaotong Wang , Yongsheng Bai , Bojun Su
{"title":"Stable partial nitrification was achieved for nitrogen removal from municipal wastewater by gel immobilization: A pilot-scale study","authors":"Xin Hu ,&nbsp;Hong Yang ,&nbsp;Xiaoyue Fang ,&nbsp;Xuyan Liu ,&nbsp;Jiawei Wang ,&nbsp;Xiaotong Wang ,&nbsp;Yongsheng Bai ,&nbsp;Bojun Su","doi":"10.1016/j.jes.2024.04.020","DOIUrl":"10.1016/j.jes.2024.04.020","url":null,"abstract":"<div><p>As an energy and carbon saving process for nitrogen removal from wastewater, the partial nitrification and denitrification process (PN/D) has been extensively researched. However, achieving stable PN in municipal wastewater has always been challenging. In this study, a gel immobilized PN/D nitrogen removal process (GI-PN/D) was established. A 94d pilot-scale experiment was conducted using real municipal wastewater with an ammonia concentration of 43.5 ± 5.3 mg N/L at a temperature range of 11.3–28.7℃. The nitrogen removal performance and associated pathways, shifts in the microbial community as well as sludge yield were investigated. The results were as follows: the effluent TN and COD were 0.6 ± 0.4 mg/L and 31.1 ± 3.8 mg/L respectively, and the NAR exceeding 95 %. GI-PN/D achieved deep nitrogen removal of municipal wastewater through stable PN without taking any other measures. The primary pathways for nitrogen removal were identified as denitrification, simultaneous nitrification-denitrification, and aerobic denitrification. High-throughput sequencing analysis revealed that the immobilized fillers facilitated the autonomous enrichment of functional bacteria in each reactor, effectively promoting the dominance and stability of the microbial communities. In addition, GI-PN/D had the characteristic of low sludge yield, with an average sludge yield of 0.029 kg SS/kg COD. This study provides an effective technical for nitrogen removal from municipal wastewater through PN.</p></div>","PeriodicalId":15788,"journal":{"name":"Journal of Environmental Sciences-china","volume":"151 ","pages":"Pages 529-539"},"PeriodicalIF":0.0,"publicationDate":"2024-04-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140768558","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Research progress and application of carbon sequestration in industrial flue gas by microalgae: A review 微藻在工业烟气中固碳的研究进展与应用:综述
2区 环境科学与生态学
Journal of Environmental Sciences-china Pub Date : 2024-04-23 DOI: 10.1016/j.jes.2024.04.018
Rui Wang , Xue Wang , Tingyu Zhu
{"title":"Research progress and application of carbon sequestration in industrial flue gas by microalgae: A review","authors":"Rui Wang ,&nbsp;Xue Wang ,&nbsp;Tingyu Zhu","doi":"10.1016/j.jes.2024.04.018","DOIUrl":"10.1016/j.jes.2024.04.018","url":null,"abstract":"<div><p>Global warming caused by the emission of CO<sub>2</sub> in industrial flue gas has attracted more and more attention. Therefore, to fix CO<sub>2</sub> with high efficiency and environmentally friendly had become the hot research field. Compared with the traditional coal-fired power plant flue gas emission reduction technology, carbon fixation and emission reduction by microalgae is considered as a promising technology due to the advantages of simple process equipment, convenient operation and environmental protection. When the flue gas is treated by microalgae carbon fixation and emission reduction technology, microalgae cells can fix CO<sub>2</sub> in the flue gas through photosynthesis, and simultaneously absorb NO<sub>x</sub> and SO<sub>x</sub> as nitrogen and sulfur sources required for growth. Meanwhile, they can also absorb mercury, selenium, arsenic, cadmium, lead and other heavy metal ions in the flue gas to obtain microalgae biomass. The obtained microalgae biomass can be further transformed into high value-added products, which has broad development prospects. This paper reviews the mechanisms and pathways of CO<sub>2</sub> sequestration, the mechanism and impacts of microalgal emission reduction of flue gas pollutants, and the applications of carbon sequestration in industrial flue gas by microalgae. Finally, this paper provides some guidelines and prospects for the research and application of green emission reduction technology for industrial flue gas.</p></div>","PeriodicalId":15788,"journal":{"name":"Journal of Environmental Sciences-china","volume":"152 ","pages":"Pages 14-28"},"PeriodicalIF":0.0,"publicationDate":"2024-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140772869","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High summer background O3 levels in the desert of northwest China 中国西北沙漠地区夏季背景臭氧浓度较高
2区 环境科学与生态学
Journal of Environmental Sciences-china Pub Date : 2024-04-23 DOI: 10.1016/j.jes.2024.04.015
Xinbing Ren , Fang Wang , Bayi Wu , Shaoting Zhang , Lei Zhang , Xingjun Zhou , Yuanzhe Ren , Yongjing Ma , Feng Hao , Yongli Tian , Jinyuan Xin
{"title":"High summer background O3 levels in the desert of northwest China","authors":"Xinbing Ren ,&nbsp;Fang Wang ,&nbsp;Bayi Wu ,&nbsp;Shaoting Zhang ,&nbsp;Lei Zhang ,&nbsp;Xingjun Zhou ,&nbsp;Yuanzhe Ren ,&nbsp;Yongjing Ma ,&nbsp;Feng Hao ,&nbsp;Yongli Tian ,&nbsp;Jinyuan Xin","doi":"10.1016/j.jes.2024.04.015","DOIUrl":"10.1016/j.jes.2024.04.015","url":null,"abstract":"<div><p>Generally speaking, the precursors of ozone (O<sub>3</sub>), nitrogen oxides and volatile organic compounds are very low in desert areas due to the lack of anthropogenic emissions and natural emissions, and thus O<sub>3</sub> concentrations are relatively low. However, high summer background concentrations of about 100 µg/m<sup>3</sup> or 60 ppb were found in the Alxa Desert in the highland of northwest China based on continuous summer observations from 2019 to 2021, which was higher than the most of natural background areas or clean areas in world for summer O<sub>3</sub> background concentrations. The high O<sub>3</sub> background concentrations were related to surface features and altitude. Heavy-intensity anthropogenic activity areas in desert areas can cause increased O<sub>3</sub> concentrations or pollution, but also generated O<sub>3</sub> depleting substances such as nitrous oxide, which eventually reduced the regional O<sub>3</sub> baseline values. Nitrogen dioxide (NO<sub>2</sub>) also had a dual effect on O<sub>3</sub> generation, showing promotion at low concentrations and inhibition at high concentrations. In addition, sand-dust weather reduced O<sub>3</sub> clearly, but O<sub>3</sub> eventually stabilized around the background concentration values and did not vary with sand-dust particulate matter.</p></div>","PeriodicalId":15788,"journal":{"name":"Journal of Environmental Sciences-china","volume":"151 ","pages":"Pages 516-528"},"PeriodicalIF":0.0,"publicationDate":"2024-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140797069","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Analyzing carbon emissions and influencing factors in Chengdu-Chongqing urban agglomeration counties 成渝城市群县域碳排放及其影响因素分析
2区 环境科学与生态学
Journal of Environmental Sciences-china Pub Date : 2024-04-21 DOI: 10.1016/j.jes.2024.04.019
Ji Zhang , Heng Lu , Wenfu Peng , Lindan Zhang
{"title":"Analyzing carbon emissions and influencing factors in Chengdu-Chongqing urban agglomeration counties","authors":"Ji Zhang ,&nbsp;Heng Lu ,&nbsp;Wenfu Peng ,&nbsp;Lindan Zhang","doi":"10.1016/j.jes.2024.04.019","DOIUrl":"10.1016/j.jes.2024.04.019","url":null,"abstract":"<div><p>Majority of carbon emissions originate from fossil energy consumption, thus necessitating calculation and monitoring of carbon emissions from energy consumption. In this study, we utilized energy consumption data from Sichuan Province and Chongqing Municipality for the years 2000 to 2019 to estimate their statistical carbon emissions. We then employed nighttime light data to downscale and infer the spatial distribution of carbon emissions at the county level within the Chengdu-Chongqing urban agglomeration. Furthermore, we analyzed the spatial pattern of carbon emissions at the county level using the coefficient of variation and spatial autocorrelation, and we used the Geographically and Temporally Weighted Regression (GTWR) model to analyze the influencing factors of carbon emissions at this scale. The results of this study are as follows: (1) from 2000 to 2019, the overall carbon emissions in the Chengdu-Chongqing urban agglomeration showed an increasing trend followed by a decrease, with an average annual growth rate of 4.24%. However, in recent years, it has stabilized, and 2012 was the peak year for carbon emissions in the Chengdu-Chongqing urban agglomeration; (2) carbon emissions exhibited significant spatial clustering, with high-high clustering observed in the core urban areas of Chengdu and Chongqing and low-low clustering in the southern counties of the Chengdu-Chongqing urban agglomeration; (3) factors such as GDP, population (Pop), urbanization rate (Ur), and industrialization structure (Ic) all showed a significant influence on carbon emissions; (4) the spatial heterogeneity of each influencing factor was evident.</p></div>","PeriodicalId":15788,"journal":{"name":"Journal of Environmental Sciences-china","volume":"151 ","pages":"Pages 640-651"},"PeriodicalIF":0.0,"publicationDate":"2024-04-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140790775","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Impacts of emission reduction and meteorological conditions on air quality improvement from 2016 to 2020 in the Northeast Plain, China 2016-2020 年减排和气象条件对中国东北平原空气质量改善的影响
2区 环境科学与生态学
Journal of Environmental Sciences-china Pub Date : 2024-04-21 DOI: 10.1016/j.jes.2024.04.017
Xueling Yang , Qiyuan Wang , Lang Liu , Jie Tian , Hailing Xie , Luyao Wang , Yue Cao , Steven Sai Hang Ho
{"title":"Impacts of emission reduction and meteorological conditions on air quality improvement from 2016 to 2020 in the Northeast Plain, China","authors":"Xueling Yang ,&nbsp;Qiyuan Wang ,&nbsp;Lang Liu ,&nbsp;Jie Tian ,&nbsp;Hailing Xie ,&nbsp;Luyao Wang ,&nbsp;Yue Cao ,&nbsp;Steven Sai Hang Ho","doi":"10.1016/j.jes.2024.04.017","DOIUrl":"10.1016/j.jes.2024.04.017","url":null,"abstract":"<div><p>The Northeast Plain in China ranks among the top five regions that have been significantly impacted by haze pollution. To effectively control pollution, it is crucial to accurately assess the effects of emission reduction measures. In this study, we analyzed surveillance data and found substantial decreases (ranging from 19.0% to 50.1%) in average annual mass concentrations of key pollutants (such as CO, SO<sub>2</sub>, NO<sub>2</sub>, and PM<sub>2.5</sub>) in the Northeast Plain from 2016 to 2020. To precisely determine the contributions of meteorological conditions and emission reductions to the improvement of air quality in the Northeast Plain, we conducted three scenario simulations. By comparing source emissions in December 2016 and 2020 using the WRF-Chem model (except for SO<sub>2</sub>), we observed significant reductions of 21.3%, 8.8%, and 9.8% in mass concentrations of PM<sub>2.5</sub>, NO<sub>2</sub>, and CO, respectively, from 2016 to 2020. This highlights the essential role that meteorological conditions play in determining air quality in the Northeast Plain. Moreover, further reducing source emissions by 30% in December 2016 resulted in subsequent reductions of 25.3%, 29.0%, 4.5%, and 30.3% in mass concentrations of PM<sub>2.5</sub>, SO<sub>2</sub>, NO<sub>2</sub>, and CO, respectively, under the same meteorological conditions. Notably, source emission reduction was effective for PM<sub>2.5</sub>, SO<sub>2</sub>, and CO, but not for NO<sub>2</sub>. The improvement in air quality in the Northeast Plain from 2016 to 2020 can be attributed to the combined effects of improved meteorological conditions and reduced pollution sources.</p></div>","PeriodicalId":15788,"journal":{"name":"Journal of Environmental Sciences-china","volume":"151 ","pages":"Pages 484-496"},"PeriodicalIF":0.0,"publicationDate":"2024-04-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140771413","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Biogenic emission as a potential source of atmospheric aromatic hydrocarbons: Insights from a cyanobacterial bloom-occurring eutrophic lake 作为大气芳香烃潜在来源的生物排放:从发生蓝藻水华的富营养化湖泊中获得的启示
2区 环境科学与生态学
Journal of Environmental Sciences-china Pub Date : 2024-04-20 DOI: 10.1016/j.jes.2024.04.011
Hua Fang , Ting Wu , Shutan Ma , Yuqing Miao , Xinming Wang
{"title":"Biogenic emission as a potential source of atmospheric aromatic hydrocarbons: Insights from a cyanobacterial bloom-occurring eutrophic lake","authors":"Hua Fang ,&nbsp;Ting Wu ,&nbsp;Shutan Ma ,&nbsp;Yuqing Miao ,&nbsp;Xinming Wang","doi":"10.1016/j.jes.2024.04.011","DOIUrl":"10.1016/j.jes.2024.04.011","url":null,"abstract":"<div><p>As important precursors of ozone (O<sub>3</sub>) and secondary organic aerosol (SOA), reactive aromatic hydrocarbons (AHs) have typically been classified as anthropogenic air pollutants. However, biogenic emission can also be a potential source of atmospheric AHs. Herein, field observations in a eutrophic lake were combined with laboratory incubation experiments to investigate the biogenic AH emission. Field work showed that the water-air fluxes of AHs measured at sites with high cyanobacteria abundance could reach an order of magnitude greater than those at sites with low cyanobacteria abundance, suggesting that cyanobacteria could be the important contributor to measured AHs. Laboratory incubation experiments further confirmed the AH emission of cyanobacteria and revealed that the emission could change significantly over the lifespan of cyanobacteria and varied to their growing conditions. By combining field observations and laboratory incubation experiments, it has been suggested that the emission of different AH species from cyanobacteria could be modulated by variable biogeochemical mechanisms and that the biochemical process of toluene could be different from that of other AHs. This study investigates AH emissions from inland aquatic ecosystem and suggests that biogenic emission could be a potential source of atmospheric AHs.</p></div>","PeriodicalId":15788,"journal":{"name":"Journal of Environmental Sciences-china","volume":"151 ","pages":"Pages 497-504"},"PeriodicalIF":0.0,"publicationDate":"2024-04-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140790524","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Interannual succession of phytoplankton community in a canyon-shaped drinking water reservoir during the initial impoundment period: Taxonomic versus functional groups 峡谷型饮用水水库浮游植物群落在蓄水初期的年际演替:分类群与功能群
2区 环境科学与生态学
Journal of Environmental Sciences-china Pub Date : 2024-04-20 DOI: 10.1016/j.jes.2024.04.013
Yi Hou , Ya Cheng , Kai Li , Meng Yang , Kangzhe Huang , Gang Ji , Ruikang Xue , Tinglin Huang , Gang Wen
{"title":"Interannual succession of phytoplankton community in a canyon-shaped drinking water reservoir during the initial impoundment period: Taxonomic versus functional groups","authors":"Yi Hou ,&nbsp;Ya Cheng ,&nbsp;Kai Li ,&nbsp;Meng Yang ,&nbsp;Kangzhe Huang ,&nbsp;Gang Ji ,&nbsp;Ruikang Xue ,&nbsp;Tinglin Huang ,&nbsp;Gang Wen","doi":"10.1016/j.jes.2024.04.013","DOIUrl":"https://doi.org/10.1016/j.jes.2024.04.013","url":null,"abstract":"<div><p>During the initial impoundment period of a canyon-shaped reservoir, the water body fluctuated violently regarding water level, hydrological condition, and thermal stratification. These variations may alter the structure of phytoplankton community, resulting in algal blooms and seriously threatening the ecological security of the reservoir. It is of great significance to understand the continuous changes of phytoplankton in the initial impoundment period for the protection of reservoir water quality. Therefore, a two-year in-situ monitoring study was conducted on water quality and phytoplankton in a representative canyon-shaped reservoir named Sanhekou and the interannual changes of phytoplankton community and its response to environmental changes during the initial impoundment period were discussed at taxonomic versus functional classification levels. The results showed that the total nitrogen and permanganate index levels were relatively high in the first year due to rapid water storage and heavy rainfall input, and the more stable hydrological conditions in the second year promoted the increase of algae density and the transformation of community, and the proportion of cyanobacteria increased significantly. The succession order of phytoplankton in the first year of the initial impoundment period was Chlorophyta-Bacillariophyta-Chlorophyta, or J/F/X1-P/MP/W1-A/X1/MP, respectively. And the succession order in the second year was Cyanobacteria/Chlorophyta-Bacillariophyta-Chlorophyta, or L<sub>M</sub>/G/P-P/A/X1-X1/J/G. Water temperature, relative water column stability, mixing depth, and pH were crucial factors affecting phytoplankton community succession. This study revealed the interannual succession law and driving factors of phytoplankton in the initial impoundment period and provided an important reference for the operation management and ecological protection of canyon-shaped reservoirs.</p></div>","PeriodicalId":15788,"journal":{"name":"Journal of Environmental Sciences-china","volume":"151 ","pages":"Pages 454-468"},"PeriodicalIF":0.0,"publicationDate":"2024-04-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140650565","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Impact of aerosol-radiation interaction and heterogeneous chemistry on the winter decreasing PM2.5 and increasing O3 in Eastern China 2014–2020 气溶胶-辐射相互作用和异质化学对 2014-2020 年华东地区冬季 PM2.5 下降和 O3 上升的影响
2区 环境科学与生态学
Journal of Environmental Sciences-china Pub Date : 2024-04-18 DOI: 10.1016/j.jes.2024.04.010
Yasong Li , Tijian Wang , Qin'geng Wang , Mengmeng Li , Yawei Qu , Hao Wu , Min Xie
{"title":"Impact of aerosol-radiation interaction and heterogeneous chemistry on the winter decreasing PM2.5 and increasing O3 in Eastern China 2014–2020","authors":"Yasong Li ,&nbsp;Tijian Wang ,&nbsp;Qin'geng Wang ,&nbsp;Mengmeng Li ,&nbsp;Yawei Qu ,&nbsp;Hao Wu ,&nbsp;Min Xie","doi":"10.1016/j.jes.2024.04.010","DOIUrl":"https://doi.org/10.1016/j.jes.2024.04.010","url":null,"abstract":"<div><p>In the context of the prevalent winter air quality issues in China marked by declining PM<sub>2.5</sub> and rising O<sub>3</sub>, this study employed a modified WRF-Chem model to examine the aerosol radiation interaction (ARI), heterogeneous chemistry (AHC), and their combined impact (ALL) on the variations in O<sub>3</sub> and PM<sub>2.5</sub> during the 2014–2020 in eastern China. Our analysis confirmed that ARI curtailed O<sub>3</sub> while elevating PM<sub>2.5</sub>. AHC reduced O<sub>3</sub> through heterogeneous absorption of NO<sub>x</sub> and hydroxides while notably fostering fine-grained sulfate, resulting in a PM<sub>2.5</sub> increase. Emission reductions mitigated the inhibitory impact of ARI on meteorological fields and photolysis rates. Emission reduction individually without aerosol feedback led to a 5.43 ppb O<sub>3</sub> increase and a 22.89 µg/m<sup>3</sup> PM<sub>2.5</sub> decrease. ARI and AHC amplified the emission-reduction-induced (ERI) O<sub>3</sub> rise by 1.83 and 0.31 ppb, respectively. The response of ARI to emission diminution brought about a modest PM<sub>2.5</sub> increase of 0.31 µg/m<sup>3</sup>. Conversely, AHC, acting as the primary contributor, caused a noteworthy PM<sub>2.5</sub> decrease of 4.60 µg/m<sup>3</sup>. As efforts concentrate on reducing PM<sub>2.5</sub>, the promotion of ARI on PM<sub>2.5</sub> counterbalanced the efficacy of emission reduction and the AHC-induced strengthening of PM<sub>2.5</sub> decrease. The ALL magnified the ERI O<sub>3</sub> increase by 38.9% and PM<sub>2.5</sub> decrease by 18.7%. Sensitivity experiments with different degrees of emission reduction demonstrated a consistent linear relationship between the ALL-induced enhancement of O<sub>3</sub> increase and PM<sub>2.5</sub> decrease to the ERI PM<sub>2.5</sub> decline. Our investigation revealed the complex connection between emissions and aerosol feedback in influencing air quality.</p></div>","PeriodicalId":15788,"journal":{"name":"Journal of Environmental Sciences-china","volume":"151 ","pages":"Pages 469-483"},"PeriodicalIF":0.0,"publicationDate":"2024-04-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140649651","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Removal of arsenic from water by silver nanoparticles and Fe-Ce mixed oxide supported on polymeric anion exchanger 聚合物阴离子交换器上支持的银纳米粒子和铁铈混合氧化物去除水中的砷
2区 环境科学与生态学
Journal of Environmental Sciences-china Pub Date : 2024-04-18 DOI: 10.1016/j.jes.2024.04.009
Li Li , Su-juan Yu , Rong-gang Zheng , Qing-cun Li , Rui Liu , Jing-fu Liu
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