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Front Cover: Advances in Tandem Strategies for CO2 Electroreduction: From Electrocatalysts to Reaction System Design (ChemCatChem 6/2025)
IF 3.8 3区 化学
ChemCatChem Pub Date : 2025-03-17 DOI: 10.1002/cctc.202580601
Peng-Fei Sui, Yi-Cheng Wang, Xiaolei Wang, Subiao Liu, Jing-Li Luo
{"title":"Front Cover: Advances in Tandem Strategies for CO2 Electroreduction: From Electrocatalysts to Reaction System Design (ChemCatChem 6/2025)","authors":"Peng-Fei Sui,&nbsp;Yi-Cheng Wang,&nbsp;Xiaolei Wang,&nbsp;Subiao Liu,&nbsp;Jing-Li Luo","doi":"10.1002/cctc.202580601","DOIUrl":"https://doi.org/10.1002/cctc.202580601","url":null,"abstract":"<p><b>The Front Cover</b> highlights recent advances in tandem strategies for CO<sub>2</sub> electrochemical reduction, spanning electrocatalyst design to reaction systems. The Review by J.-L. Luo and co-workers (DOI: 10.1002/cctc.202401604) summarizes tandem catalysts from the atomic to the macroscale, internal product upgrades during tandem reactions, and tandem multi-physical fields. Various tandem systems, including two-step electrochemical, electrochemical–thermochemical, and electrochemical–microbial tandem systems are discussed, offering insights into rational tandem design and guidance for developing efficient energy conversion systems.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":141,"journal":{"name":"ChemCatChem","volume":"17 6","pages":""},"PeriodicalIF":3.8,"publicationDate":"2025-03-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cctc.202580601","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143632610","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Cover Feature: Unveiling the Catalytic Activity of Nickel(II) Complexes of Pentadentate Ligands in Aromatic Oxidations (ChemCatChem 6/2025)
IF 3.8 3区 化学
ChemCatChem Pub Date : 2025-03-17 DOI: 10.1002/cctc.202580602
Anjana Rajeev, Sethuraman Muthuramalingam, Visvesvarar Pitchai Murugan, Miquel Costas, Prabha Vadivelu, Muniyandi Sankaralingam
{"title":"Cover Feature: Unveiling the Catalytic Activity of Nickel(II) Complexes of Pentadentate Ligands in Aromatic Oxidations (ChemCatChem 6/2025)","authors":"Anjana Rajeev,&nbsp;Sethuraman Muthuramalingam,&nbsp;Visvesvarar Pitchai Murugan,&nbsp;Miquel Costas,&nbsp;Prabha Vadivelu,&nbsp;Muniyandi Sankaralingam","doi":"10.1002/cctc.202580602","DOIUrl":"https://doi.org/10.1002/cctc.202580602","url":null,"abstract":"<p><b>The Cover Feature</b> depicts the hydroxylation of benzene to phenol in the presence of a nickel pentadentate catalyst and hydrogen peroxide. The highly inert nature of the C─H bonds of benzene is represented by a spherical cage secured with a locked chain. However, the powerful nickel catalyst and oxidant act as a key, facilitating the selective oxidation of one of the C─H bonds to produce phenol. More information can be found in the Research Article by M. Sankaralingam and co-workers (DOI: 10.1002/cctc.202401645).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":141,"journal":{"name":"ChemCatChem","volume":"17 6","pages":""},"PeriodicalIF":3.8,"publicationDate":"2025-03-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cctc.202580602","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143632693","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Front Cover: Development of Bifunctional Catalysts for CO2 Capture and Conversion at Low Temperatures Under an Electric Field (ChemCatChem 5/2025)
IF 3.8 3区 化学
ChemCatChem Pub Date : 2025-03-06 DOI: 10.1002/cctc.202580501
Keidai Tomozawa, Prof. Dr. Nao Tsunoji, Rin Suwa, Prof. Dr. Masahiro Sadakane, Prof. Dr. Tadaharu Ueda, Prof. Dr. Shuhei Ogo
{"title":"Front Cover: Development of Bifunctional Catalysts for CO2 Capture and Conversion at Low Temperatures Under an Electric Field (ChemCatChem 5/2025)","authors":"Keidai Tomozawa,&nbsp;Prof. Dr. Nao Tsunoji,&nbsp;Rin Suwa,&nbsp;Prof. Dr. Masahiro Sadakane,&nbsp;Prof. Dr. Tadaharu Ueda,&nbsp;Prof. Dr. Shuhei Ogo","doi":"10.1002/cctc.202580501","DOIUrl":"https://doi.org/10.1002/cctc.202580501","url":null,"abstract":"<p><b>The Front Cover</b> highlights greener systems for CO<sub>2</sub> capture and reduction into CO (CCR) by using bifunctional catalysts. The synergistic effects of a direct-current electric field and developed Na-modified Pt nanoparticles on TiO<sub>2</sub> as a bifunctional catalyst realized selective CO production through CCR under low-temperature isothermal conditions. More information can be found in the Research Article by S. Ogo and co-workers (DOI: 10.1002/cctc.202401775).\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":141,"journal":{"name":"ChemCatChem","volume":"17 5","pages":""},"PeriodicalIF":3.8,"publicationDate":"2025-03-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cctc.202580501","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143564996","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
ChemCatChem: From Europe for the World
IF 3.8 3区 化学
ChemCatChem Pub Date : 2025-03-06 DOI: 10.1002/cctc.202500219
Sandra González-Gallardo, Rosemary Puls
{"title":"ChemCatChem: From Europe for the World","authors":"Sandra González-Gallardo,&nbsp;Rosemary Puls","doi":"10.1002/cctc.202500219","DOIUrl":"https://doi.org/10.1002/cctc.202500219","url":null,"abstract":"<p>As a society journal, co-owned by the cooperative of societies that make up Chemistry Europe. <i>ChemCatChem</i> plays a significant role in the dissemination of catalysis research and is committed to supporting researchers at every stage of their careers. In this Editorial, we present our new Editorial and Early Career Advisory Boards.</p>","PeriodicalId":141,"journal":{"name":"ChemCatChem","volume":"17 5","pages":""},"PeriodicalIF":3.8,"publicationDate":"2025-03-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cctc.202500219","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143564998","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Roots and Wings for a Better World at the 18th International Congress on Catalysis in Lyon, France
IF 3.8 3区 化学
ChemCatChem Pub Date : 2025-03-06 DOI: 10.1002/cctc.202500167
Dr. Céline Chizallet, Dr. Clément Camp, David Farrusseng, Prof. Pascal Fongarland, Dr. Dorothée Laurenti, Dr. Axel Löfberg, Dr. Françoise Maugé, Dr. Hélène Olivier-Bourbigou, Dr. Catherine Pinel, Dr. Nathalie Tanchoux
{"title":"Roots and Wings for a Better World at the 18th International Congress on Catalysis in Lyon, France","authors":"Dr. Céline Chizallet,&nbsp;Dr. Clément Camp,&nbsp;David Farrusseng,&nbsp;Prof. Pascal Fongarland,&nbsp;Dr. Dorothée Laurenti,&nbsp;Dr. Axel Löfberg,&nbsp;Dr. Françoise Maugé,&nbsp;Dr. Hélène Olivier-Bourbigou,&nbsp;Dr. Catherine Pinel,&nbsp;Dr. Nathalie Tanchoux","doi":"10.1002/cctc.202500167","DOIUrl":"https://doi.org/10.1002/cctc.202500167","url":null,"abstract":"<p>With the motto “Roots and Wings for a Better World”, the 18<sup>th</sup> International Congress on Catalysis, held in Lyon, France, from July 14<sup>th</sup> to 19<sup>th</sup>, 2024, has been an invaluable forum for the catalysis community to share its most advanced results. The dense and high-quality scientific program along with a vibrant exhibition and friendly social events have made this edition highly memorable.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":141,"journal":{"name":"ChemCatChem","volume":"17 6","pages":""},"PeriodicalIF":3.8,"publicationDate":"2025-03-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143632765","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Cover Feature: N-Doped Ti3C2Tx MXene-regulated Metal-oxide Facilitates the Efficient Electrocatalytic CO2 Reduction to CO (ChemCatChem 5/2025)
IF 3.8 3区 化学
ChemCatChem Pub Date : 2025-03-06 DOI: 10.1002/cctc.202580502
Hui-Hui Cao, Zhen-Hong He, Pan-Pan Guo, Yue Tian, Xin Wang, Kuan Wang, Weitao Wang, Huan Wang, Yang Yang, Zhao-Tie Liu
{"title":"Cover Feature: N-Doped Ti3C2Tx MXene-regulated Metal-oxide Facilitates the Efficient Electrocatalytic CO2 Reduction to CO (ChemCatChem 5/2025)","authors":"Hui-Hui Cao,&nbsp;Zhen-Hong He,&nbsp;Pan-Pan Guo,&nbsp;Yue Tian,&nbsp;Xin Wang,&nbsp;Kuan Wang,&nbsp;Weitao Wang,&nbsp;Huan Wang,&nbsp;Yang Yang,&nbsp;Zhao-Tie Liu","doi":"10.1002/cctc.202580502","DOIUrl":"https://doi.org/10.1002/cctc.202580502","url":null,"abstract":"<p><b>The Cover Feature</b> shows the electrocatalytic CO<sub>2</sub> reduction reaction (ECO<sub>2</sub>RR), which is crucial for converting CO<sub>2</sub> into valuable chemicals. In their Research Article (DOI: 10.1002/cctc.202401133), Z.-H. He, Z.-T. Liu and co-workers report the synthesis of a ZnO catalyst supported on N-doped Ti<sub>3</sub>C<sub>2</sub>T<sub>x</sub> MXene (ZnO/N-Ti<sub>3</sub>C<sub>2</sub>T<sub>x</sub>) by a simple incipient wetness impregnation method. The FECO reached 96.4% with a current density of 7.2 mA cm<sup>–2</sup> at –0.967 V (vs. RHE) in a 0.5 M KCl electrolyte. These results rank among the top values for similar catalytic systems in aqueous electrolytes and H-type cells.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":141,"journal":{"name":"ChemCatChem","volume":"17 5","pages":""},"PeriodicalIF":3.8,"publicationDate":"2025-03-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cctc.202580502","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143564997","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Trapping Hydrogen: Confined Catalysis for Improved Alcohol Amination Selectivity
IF 3.8 3区 化学
ChemCatChem Pub Date : 2025-03-05 DOI: 10.1002/cctc.202401941
Julio C. S. Terra, Jackson DeWolfe, Jesus A. Valdez, Audrey Moores
{"title":"Trapping Hydrogen: Confined Catalysis for Improved Alcohol Amination Selectivity","authors":"Julio C. S. Terra,&nbsp;Jackson DeWolfe,&nbsp;Jesus A. Valdez,&nbsp;Audrey Moores","doi":"10.1002/cctc.202401941","DOIUrl":"https://doi.org/10.1002/cctc.202401941","url":null,"abstract":"<p>Confined chemistry is a powerful tool in catalysis. In this study, we report hierarchical structures with controlled morphology able to trap labile intermediates and improve a catalytic cascade reaction. We used alcohol amination via hydrogen borrowing as model, a process that gives substituted amines from alcohols and does not require the addition of hydrogen to reduce the imines or the use of coupling agents. A common problem however in those systems is the loss of the borrowed hydrogen atoms, leading to stagnation of the product at the imine stage. To this end, we encapsulated Al<sub>2</sub>O<sub>3</sub>/Ru(OH)<sub>x</sub> nanocatalysts inside mesoporous silica in a yolk-shell architecture and were able to trap the hydrogens to increase the amine yield from 12% to 82%, with a three-fold increase in selectivity without the need of any additive. We found the presence of mesopores in the silica shells to be essential to enable access to the catalytic sites and the yolk-shell gap size to be the key parameter influencing the reactivity of the catalytic system. To the best of our knowledge, this is the first report of a confined hydrogen borrowing reaction, an approach that can be extended to the other types of cascade reactions that produce labile intermediates.</p>","PeriodicalId":141,"journal":{"name":"ChemCatChem","volume":"17 6","pages":""},"PeriodicalIF":3.8,"publicationDate":"2025-03-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143632926","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Two-Dimensional Ti3C2 MXene Supported RuCo Catalyst for Improving the NH3 Yield of Electrocatalytic Nitrate Reduction Reaction
IF 3.8 3区 化学
ChemCatChem Pub Date : 2025-03-04 DOI: 10.1002/cctc.202401549
Qianqian Hua, Zhen Yuan, Feng Li, Yidi Liu, Liguo Gao, Xiaoying Dong, Xuefeng Ren, Tingli Ma, Junjiang Bao, Anmin Liu
{"title":"Two-Dimensional Ti3C2 MXene Supported RuCo Catalyst for Improving the NH3 Yield of Electrocatalytic Nitrate Reduction Reaction","authors":"Qianqian Hua,&nbsp;Zhen Yuan,&nbsp;Feng Li,&nbsp;Yidi Liu,&nbsp;Liguo Gao,&nbsp;Xiaoying Dong,&nbsp;Xuefeng Ren,&nbsp;Tingli Ma,&nbsp;Junjiang Bao,&nbsp;Anmin Liu","doi":"10.1002/cctc.202401549","DOIUrl":"https://doi.org/10.1002/cctc.202401549","url":null,"abstract":"<p>To enhance the electrochemical synthesis of ammonia performance by accelerating the reaction kinetics of electrocatalytic Nitrate reduction reaction (NO<sub>3</sub><sup>−</sup>RR), it is crucial to develop electrocatalysts with high acitiity and selectivity of NO<sub>3</sub><sup>−</sup>RR. Herein, a Ru-doped Co-Ti<sub>3</sub>C<sub>2</sub> catalyst was prepared for NO<sub>3</sub><sup>−</sup>RR in this work. In 0.1 M KOH &amp; 0.1 M KNO<sub>3</sub> electrolyte, the Ru doped Co-Ti<sub>3</sub>C<sub>2</sub> (nRu:nCo = 2:8, RuCo-Ti<sub>3</sub>C<sub>2</sub>-2:8) achieved a Faraday efficiency (FE) of 96.48% and an ammonia yield of 2261.99 µg cm<sup>−2</sup> h<sup>−1</sup> at −0.4 V vs. RHE. Compared with the Co-MXene catalyst and the Ru doped Co-Ti<sub>3</sub>C<sub>2</sub> catalysts of other compositions, RuCo-Ti<sub>3</sub>C<sub>2</sub>-2:8 exhibited better ammonia yield and high FE. Moreover, the RuCo-Ti<sub>3</sub>C<sub>2</sub>-2:8 catalyst exhibited excellent stability of electrocatalytic NO<sub>3</sub><sup>−</sup>RR.</p>","PeriodicalId":141,"journal":{"name":"ChemCatChem","volume":"17 6","pages":""},"PeriodicalIF":3.8,"publicationDate":"2025-03-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143632931","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Metal-Organic Framework–Specific Catalysis
IF 3.8 3区 化学
ChemCatChem Pub Date : 2025-02-19 DOI: 10.1002/cctc.202402102
Marco Bengsch, Dr. Constanze N. Neumann
{"title":"Metal-Organic Framework–Specific Catalysis","authors":"Marco Bengsch,&nbsp;Dr. Constanze N. Neumann","doi":"10.1002/cctc.202402102","DOIUrl":"https://doi.org/10.1002/cctc.202402102","url":null,"abstract":"<p>The precision with which atoms can be positioned in 3D space through reticular chemistry imbues metal-organic frameworks (MOFs) with the potential to access catalytic performance beyond what is possible with classical heterogeneous manifolds. In this paper, we highlight illustrative examples in which MOF-based catalysts integrate adsorption and catalysis, optimize cooperation, bypass high-energy intermediates, bring about active site regeneration, stabilize unusual active sites or use extended environment effects in order to break new ground in catalyst design.</p>","PeriodicalId":141,"journal":{"name":"ChemCatChem","volume":"17 6","pages":""},"PeriodicalIF":3.8,"publicationDate":"2025-02-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cctc.202402102","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143632979","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Cover Feature: Coupling Conversion of CO2 and High-Carbon Alkane to CO and Gasoline (ChemCatChem 4/2025)
IF 3.8 3区 化学
ChemCatChem Pub Date : 2025-02-18 DOI: 10.1002/cctc.202580402
Shenghui Tao, Dr. Shimin Liu, Liping Zhang, Dr. Teng Li, Bowen Qiu, Guomin Li, Prof. Feng Shi, Prof. Xinjiang Cui
{"title":"Cover Feature: Coupling Conversion of CO2 and High-Carbon Alkane to CO and Gasoline (ChemCatChem 4/2025)","authors":"Shenghui Tao,&nbsp;Dr. Shimin Liu,&nbsp;Liping Zhang,&nbsp;Dr. Teng Li,&nbsp;Bowen Qiu,&nbsp;Guomin Li,&nbsp;Prof. Feng Shi,&nbsp;Prof. Xinjiang Cui","doi":"10.1002/cctc.202580402","DOIUrl":"https://doi.org/10.1002/cctc.202580402","url":null,"abstract":"<p><b>The Cover Feature</b> depicts the coupling reaction of CO<sub>2</sub> and <i>n</i>-C<sub>16</sub> to CO and gasoline at the bifunctional sites of a Ni/β catalyst. In their Research Article (DOI: 10.1002/cctc.202401546), F. Shi, X. Cui, and co-workers report a promising approach to CO<sub>2</sub> utilization—coupling transformation of CO<sub>2</sub> and <i>n</i>-C<sub>16</sub> to gasoline. The Brønsted acid was responsible for <i>n</i>-C<sub>16</sub> activation, and Ni catalyzed the RWGS reaction and captured the H<sub>2</sub> species produced during aromatization, thereby increasing the yield of aromatics and the octane value of gasoline.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":141,"journal":{"name":"ChemCatChem","volume":"17 4","pages":""},"PeriodicalIF":3.8,"publicationDate":"2025-02-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/cctc.202580402","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143439130","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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