International Journal of Energy Research最新文献

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High-Accuracy Bandgap Prediction and Classification in Hybrid and Inorganic Halide Perovskites Using Advanced Machine Learning Techniques 利用先进的机器学习技术对杂化和无机卤化物钙钛矿进行高精度带隙预测和分类
IF 4.3 3区 工程技术
International Journal of Energy Research Pub Date : 2025-07-28 DOI: 10.1155/er/1215175
Alireza Sabagh Moeini, Fatemeh Shariatmadar Tehrani, Alireza Naeimi-Sadigh
{"title":"High-Accuracy Bandgap Prediction and Classification in Hybrid and Inorganic Halide Perovskites Using Advanced Machine Learning Techniques","authors":"Alireza Sabagh Moeini,&nbsp;Fatemeh Shariatmadar Tehrani,&nbsp;Alireza Naeimi-Sadigh","doi":"10.1155/er/1215175","DOIUrl":"https://doi.org/10.1155/er/1215175","url":null,"abstract":"<div>\u0000 <p>Hybrid and inorganic halide perovskites (HP) have garnered significant attention for their applications in solar cells, LEDs, and sensors due to their exceptional electronic and optical properties. The accurate prediction and classification of bandgaps in these materials are crucial for advancing their technological potential. Traditional methods like Density Functional Theory (DFT) are computationally expensive, motivating the use of machine learning (ML) as a faster and more efficient alternative. In this study, we analyze 7382 hybrid and inorganic HP using a diverse set of ML models to classify materials based on whether they exhibit zero or nonzero bandgaps, and to predict their bandgap values. For regression tasks, AdaBoost Regressor (ABR), decision tree regressor (DTR), and gradient boosting regressor (GBR) were employed, while gradient boosting machines (GBM), decision tree (DT), and Multilayer Perceptron (MLP) were used for classification. Evaluation metrics for prediction included mean absolute error (MAE), mean squared error (MSE), and the <i>R</i><sup>2</sup>. For classification, metrics, such as accuracy, precision, recall, F1-score, area under the ROC curve (AUC-ROC), and area under the precision-recall curve (AUC-PR) were utilized. Results indicate that ABR achieved the highest prediction accuracy (MSE ≈ 0.074 eV, MAE ≈ 0.088 eV, <i>R</i><sup>2</sup> ≈ 91.1% for direct bandgaps; MSE ≈ 0.041 eV, MAE ≈ 0.076 eV, <i>R</i><sup>2</sup> ≈ 93.4% for indirect bandgaps). In classification, the GBM model outperformed others, achieving 96% and 97% accuracy for direct and indirect bandgaps, respectively. Feature analysis revealed that elemental properties, such as valence and group of constituent elements, particularly their mean and standard deviation, play a dominant role in bandgap determination. These findings highlight the potential of ML-driven approaches in accelerating perovskite material discovery and optimizing their electronic properties for future optoelectronic applications.</p>\u0000 </div>","PeriodicalId":14051,"journal":{"name":"International Journal of Energy Research","volume":"2025 1","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-07-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1155/er/1215175","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144714955","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Introducing a Sustainable Novel Double Absorber Perovskite Solar Cell Using CsSnI3 and La2NiMnO6: A Strategy to Achieve 32.73% Efficiency 采用CsSnI3和La2NiMnO6的新型可持续双吸收钙钛矿太阳能电池:实现32.73%效率的策略
IF 4.3 3区 工程技术
International Journal of Energy Research Pub Date : 2025-07-27 DOI: 10.1155/er/6693434
Basra Sultana, Md Masum Mia, Lamia Ben Farhat, Ameni Brahmia, Okba Saidani, Md. Ferdous Rahman
{"title":"Introducing a Sustainable Novel Double Absorber Perovskite Solar Cell Using CsSnI3 and La2NiMnO6: A Strategy to Achieve 32.73% Efficiency","authors":"Basra Sultana,&nbsp;Md Masum Mia,&nbsp;Lamia Ben Farhat,&nbsp;Ameni Brahmia,&nbsp;Okba Saidani,&nbsp;Md. Ferdous Rahman","doi":"10.1155/er/6693434","DOIUrl":"https://doi.org/10.1155/er/6693434","url":null,"abstract":"<div>\u0000 <p>This study focuses on improving device performance by introducing an innovative double perovskite active layer (DPAL). The proposed design incorporates a DPAL made of CsSnI<sub>3</sub> and La<sub>2</sub>NiMnO<sub>6</sub> (LNMO), combined with a tungsten disulfide (WS<sub>2</sub>) electron transport layer (ETL). Using the Solar Cell Capacitance Simulator Structures (SCAPS-1D) software tool, a novel double absorber solar cell was computationally analyzed. Comparative results show that the DPAL-based perovskite solar cell (PSC) outperforms single active layer PSCs. The study also investigates how factors, such as active layer thickness, defect density, and interface defects affect performance, along with the influence of temperature and doping density on efficiency. The proposed design achieves a power conversion efficiency (PCE) of 32.73%, with a short-circuit current density (<i>J</i><sub>SC</sub>) of 36.51 mA/cm<sup>2</sup>, an open-circuit voltage (<i>V</i><sub>OC</sub>) of 1.05 V, and a fill factor (FF) of 85.28%. In comparison, single absorber designs based on LNMO and CsSnI<sub>3</sub> yield PCEs of 20.26% and 30.57%, respectively. This DPAL-based solar cell shows great potential for advancing highly efficient PSC development in the future.</p>\u0000 </div>","PeriodicalId":14051,"journal":{"name":"International Journal of Energy Research","volume":"2025 1","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-07-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1155/er/6693434","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144714847","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Performance and Energy Analysis of Solar Water Heating Plant in Area of High Solar Radiation: Case of Study in Northern Chile 太阳高辐射地区太阳能热水厂性能及能源分析——以智利北部为例
IF 4.3 3区 工程技术
International Journal of Energy Research Pub Date : 2025-07-26 DOI: 10.1155/er/9912440
Svetlana Ushak, Stephan Pierre Louis, Sergio Pablo, Paula E. Marín, M. Judith Cruz, Mario Grageda
{"title":"Performance and Energy Analysis of Solar Water Heating Plant in Area of High Solar Radiation: Case of Study in Northern Chile","authors":"Svetlana Ushak,&nbsp;Stephan Pierre Louis,&nbsp;Sergio Pablo,&nbsp;Paula E. Marín,&nbsp;M. Judith Cruz,&nbsp;Mario Grageda","doi":"10.1155/er/9912440","DOIUrl":"https://doi.org/10.1155/er/9912440","url":null,"abstract":"<div>\u0000 <p>This study focuses on the analysis of the efficiency and the energy performance of a solar water heating (SWH) plant located in the North of Chile, characterized by an instantaneous global solar radiation reaching around 1000 W/m<sup>2</sup>. The methodology combined experimental measurements in an indirect active solar system with systematic variations in operating parameters, including the evaluation of different flow rates in both the primary and secondary circuits, a comparative analysis of storage system volumes (100 L vs. 200 L) and an assessment of domestic hot water (DHW) consumption management. Precise temperature and flow rate measurements were used to determine performance indicators such as collector efficiency, charging efficiency, and overall plant efficiency. The experimental results reveal that the higher flow rates translate into greater efficiency, reaching a 72% with a flow rate of the 0.63 m<sup>3</sup>/h compared to the 46% obtained with a flow rate of the 0.35 m<sup>3</sup>/h. Also, under similar operating conditions, the larger capacity tank (200 L) reaches a lower maximum temperature during the charging (60°C vs. 75°C for the tank of 100 L). However, despite the lower temperature reached, the largest capacity tank (200 L) manages to recover 55% more of DHW. This analysis highlights the importance of considering the efficiency, the storage capacity, and the consumption management to optimize SWH systems in environments with high solar radiation, such as Northern Chile. Furthermore, the exploration of innovative technologies, such as the use of phase change materials (PCM), is suggested to further improve the efficiency of the thermal storage system.</p>\u0000 </div>","PeriodicalId":14051,"journal":{"name":"International Journal of Energy Research","volume":"2025 1","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-07-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1155/er/9912440","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144705624","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Rapid Prediction of Local Mean Age of Air for Energy-Efficient Ventilation Systems Using Permutation Feature Importance 利用置换特征重要性快速预测节能通风系统局部平均风龄
IF 4.3 3区 工程技术
International Journal of Energy Research Pub Date : 2025-07-26 DOI: 10.1155/er/3878472
Sanghun Shin, Keuntae Baek, Hongyun So
{"title":"Rapid Prediction of Local Mean Age of Air for Energy-Efficient Ventilation Systems Using Permutation Feature Importance","authors":"Sanghun Shin,&nbsp;Keuntae Baek,&nbsp;Hongyun So","doi":"10.1155/er/3878472","DOIUrl":"https://doi.org/10.1155/er/3878472","url":null,"abstract":"<div>\u0000 <p>Prediction of local mean age of air (MAA) is a key technology that can enhance the comfort, health, and productivity of indoor residents by adjusting and optimizing the indoor environmental conditions. In this study, we developed a deep neural network (DNN)-based regression model to predict indoor air quality (IAQ) and proposed a permutation feature importance (PFI)-based explainable artificial intelligence (XAI) model to implement efficient ventilation systems in a hospital ward utilizing this regression model. The rapid prediction of the MAA in the space near each patient in the ward, depending on the location of the heating, ventilation, and air conditioning (HVAC) inlets and fluid velocity, were successfully measured through data-driven deep learning model training. Consequently, the proposed MAA prediction model achieved average <i>R</i>-squared values of 0.9506 and 0.9220 for MAA<sub>1</sub> and MAA<sub>2</sub>, respectively. In addition, the DNN model demonstrated rapid predictive performance (~0.4 ms/prediction), highlighting the possibility of real-time monitoring compared to conventional methods. Furthermore, the contribution of the location and fluid velocity of the HVAC system to the MAA in the space near the patient was analyzed using PFI. These results support the rapid virtual sensing and recommendation method that has the potential to be applied in future IAQ management, human healthcare, and energy management systems.</p>\u0000 </div>","PeriodicalId":14051,"journal":{"name":"International Journal of Energy Research","volume":"2025 1","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-07-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1155/er/3878472","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144705446","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Unraveling a Novel CsSnI3 and CsSnGeI3 Double Absorber Perovskite Solar Cell 新型CsSnI3和CsSnGeI3双吸收钙钛矿太阳能电池的研究
IF 4.3 3区 工程技术
International Journal of Energy Research Pub Date : 2025-07-26 DOI: 10.1155/er/1804390
Md. Ferdous Rahman, Rihan Akter, Md. Faruk Hossain, Nacer Badi, Ahmad Irfan
{"title":"Unraveling a Novel CsSnI3 and CsSnGeI3 Double Absorber Perovskite Solar Cell","authors":"Md. Ferdous Rahman,&nbsp;Rihan Akter,&nbsp;Md. Faruk Hossain,&nbsp;Nacer Badi,&nbsp;Ahmad Irfan","doi":"10.1155/er/1804390","DOIUrl":"https://doi.org/10.1155/er/1804390","url":null,"abstract":"<div>\u0000 <p>The demanding need for sustainable energy solutions has driven notable progress in solar cell technology, with perovskite solar cells (PSCs) emerging as a promising option. This research introduces a novel method to boost PSC efficiency by incorporating a double perovskite active layer (DPAL) design featuring CsSnGeI<sub>3</sub> and CsSnI<sub>3</sub> having energy bandgap of 1.5 and 1.3 eV, respectively. Through comprehensive simulation and optimization applying SCAPS-1D software, this work investigates the effects of absorber layer thickness, defect density, and doping concentration on the photovoltaic (PV) performance of the proposed PSCs. The results reveal that the DPAL structure (FTO/PCBM/CsSnGeI<sub>3</sub>/CsSnI<sub>3</sub>/Au) achieves impressive power conversion efficiency (PCE) of 31.31%, significantly surpassing single absorber designs. The optimized configuration exhibits a short-circuit current density (<i>J</i><sub>SC</sub>) of 35.31 mA/cm<sup>2</sup>, an open-circuit voltage (<i>V</i><sub>OC</sub>) of 1.01 V, and a fill factor (FF) of 87.63%. In comparison, CsSnGeI<sub>3</sub> and CsSnI<sub>3</sub>-based single absorbers achieved PCEs of 27.33% and 28.10%, respectively. These findings demonstrate the potential of the DPAL approach in enhancing light absorption, charge carrier separation, and transport. This study not only deepens the understanding of PSC design and optimization but also lays the groundwork for advanced solar cells designed to achieve higher efficiency and greater environmental sustainability.</p>\u0000 </div>","PeriodicalId":14051,"journal":{"name":"International Journal of Energy Research","volume":"2025 1","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-07-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1155/er/1804390","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144705625","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Food Waste Biomass-Derived Hydrochar by Hydrothermal Carbonization for Solid Biofuel Production 利用水热炭化法生产固体生物燃料的食物垃圾生物质衍生碳氢化合物
IF 4.3 3区 工程技术
International Journal of Energy Research Pub Date : 2025-07-25 DOI: 10.1155/er/8452650
Januario Da Costa Hossi, Michael Wark, Kevin Graham Harding
{"title":"Food Waste Biomass-Derived Hydrochar by Hydrothermal Carbonization for Solid Biofuel Production","authors":"Januario Da Costa Hossi,&nbsp;Michael Wark,&nbsp;Kevin Graham Harding","doi":"10.1155/er/8452650","DOIUrl":"https://doi.org/10.1155/er/8452650","url":null,"abstract":"<div>\u0000 <p>Energy catalyzes economic development, with research into energy technologies essential for identifying alternatives that could mitigate against the reliance on fossil energy and its aggravating environmental impacts. This study explored the conversion of food waste (FW) biomass into hydrochar achieved via hydrothermal carbonization (HTC) technology. The research focused on evaluating the merits and demerits of using mixed FW feedstock, especially rice, potatoes, vegetables, and/or animal byproducts such as meat and fish at varying water-to-biomass ratios and through the implementation of water recirculation in the HTC process. This approach aimed to decrease water consumption while assessing its impact on the fuel characteristics of the resultant hydrochar. The hydrochar produced demonstrated an enhanced carbon content, which is conducive to combustion, while also exhibiting improved fuel properties such as elevated heating values, improved energy densities, and reduced volatile components. Conditions exceeding 200°C, with a reaction time of 6 h, were found to be sufficient to attain an average carbon content of above 70% and a heating value of around 30 MJ/kg. Moreover, decreasing the water-to-biomass ratio enabled a reduction in initial water usage by up to 50%, without significantly impairing the carbon content and fuel attributes of the hydrochar. Thermogravimetric analysis (TGA) indicated a comparatively elevated combustion temperature of 600°C for the hydrochar generated at an HTC temperature of 220°C, which corresponded with a substantial increase in the carbon content of hydrochar up to 70.65% from initial 48% in the parent biomass. Consequently, the hydrochar generated from FW under different HTC reaction conditions, including water volume reduction and recirculation, demonstrated the potential for minimal water consumption. This method represents a promising strategy for enhancing HTC as a renewable energy technology.</p>\u0000 </div>","PeriodicalId":14051,"journal":{"name":"International Journal of Energy Research","volume":"2025 1","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-07-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1155/er/8452650","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144695892","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Synergistic Effects of F Doping and CNT Incorporation in ZnMn2O4 Cathode Materials to Achieve High-Performance Aqueous Zinc-Ion Batteries ZnMn2O4正极材料中F掺杂与碳纳米管掺入的协同效应制备高性能水性锌离子电池
IF 4.3 3区 工程技术
International Journal of Energy Research Pub Date : 2025-07-25 DOI: 10.1155/er/5520873
Boram Lee, Min Gu Kang, Shin Ae Song, Ju Young Woo, Jeong Cheol Seo, Yongho Choa, Yun-Seok Jun, Wook Ahn, Sung Nam Lim
{"title":"Synergistic Effects of F Doping and CNT Incorporation in ZnMn2O4 Cathode Materials to Achieve High-Performance Aqueous Zinc-Ion Batteries","authors":"Boram Lee,&nbsp;Min Gu Kang,&nbsp;Shin Ae Song,&nbsp;Ju Young Woo,&nbsp;Jeong Cheol Seo,&nbsp;Yongho Choa,&nbsp;Yun-Seok Jun,&nbsp;Wook Ahn,&nbsp;Sung Nam Lim","doi":"10.1155/er/5520873","DOIUrl":"https://doi.org/10.1155/er/5520873","url":null,"abstract":"<div>\u0000 <p>Mn-based materials are promising cathode candidates for aqueous Zn-ion batteries (AZIBs) because of their high-voltage platforms, environmental friendliness, and nontoxicity. However, their practical applications are limited by the rapid capacity decay caused by their slow electrochemical reaction kinetics and intrinsically poor conductivity. In this study, <i>F</i>-doped ZnMn<sub>2</sub>O<sub>4</sub> (ZMO) (F-ZMO) microspheres incorporated with carbon nanotubes (CNTs) were synthesized and investigated to overcome these limitations. <i>F</i>-doping induced structural modifications by generating oxygen defects, which improved the ion diffusion and electronic conductivity. In addition, it improved the structure stability owing to the formation of strong metal-<i>F</i> bonds. These doping effects led to enhanced rate performance and cycle stability. Furthermore, the incorporation of CNTs complemented the insufficient electrical conductivity of the cathode material. The resulting F-ZMO/carbon nanotube (CNT) composites exhibited superior charge–transfer kinetics. Consequently, they achieved an enhanced discharge capacity of 122.2 mAh g<sup>−1</sup> at a high current density of 2.0 A g<sup>−1</sup>, demonstrating significantly improved performance compared to those of ZMO and ZMO/CNT. These findings highlight the synergistic effect of <i>F</i>-doping and CNT incorporation in enhancing the electrochemical properties of ZMO cathodes and provide critical insights into the development of high-performance cathode materials for AZIBs.</p>\u0000 </div>","PeriodicalId":14051,"journal":{"name":"International Journal of Energy Research","volume":"2025 1","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-07-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1155/er/5520873","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144695893","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Conceptual Design of a Micro Nuclear Energy System With Integrated Heat Pipe Cooled Reactor and Molten Salt Heat Storage 热管冷却堆与熔盐蓄热一体化微型核能系统的概念设计
IF 4.3 3区 工程技术
International Journal of Energy Research Pub Date : 2025-07-24 DOI: 10.1155/er/6804154
Dong Huang, Fanchen Li, Youqi Zheng
{"title":"Conceptual Design of a Micro Nuclear Energy System With Integrated Heat Pipe Cooled Reactor and Molten Salt Heat Storage","authors":"Dong Huang,&nbsp;Fanchen Li,&nbsp;Youqi Zheng","doi":"10.1155/er/6804154","DOIUrl":"https://doi.org/10.1155/er/6804154","url":null,"abstract":"<div>\u0000 <p>Micro nuclear energy system has the advantages of low investment and flexible deployment, which contribute to wide application prospects. However, in comparison to the large nuclear power plants, micro nuclear energy system is situated closer to users and requires higher safety performance. This paper proposes a new conceptual design of a micro nuclear energy system with high thermal inertia. It is based on a heat pipe cooled reactor and an integrated heat storage system along with a supercritical carbon dioxide (SCO<sub>2</sub>) Brayton cycle. The system can achieve 34.45% energy conversion efficiency and 1.2 MW electric power output. A heat pipe cooled reactor with uranium dioxide (UO<sub>2</sub>) fuel and sodium heat pipe was designed. It was connected by the condensation section of heat pipes to a molten salt heat storage system. The SCO<sub>2</sub> Brayton cycle was used to ensure a compact system layout. Using a newly developed analysis platform, three transient conditions including the load reduction, reactivity insertion, and loss of heat sink were discussed. The results indicate that, with the intermediate heat storage, the micro nuclear energy system has better tolerance of the transient thermal shocks. The peak temperature in the core is reduced for all conditions. Particularly in the process of loss of heat sink, the peak temperature in the core can be reduced by more than 70 K.</p>\u0000 </div>","PeriodicalId":14051,"journal":{"name":"International Journal of Energy Research","volume":"2025 1","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1155/er/6804154","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144695880","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Ionic Liquid-Protected Edge Plane of Graphite to Overcome Initial Irreversible Capacity Loss for Improved Lithium-Ion Batteries 离子液体保护石墨边缘平面克服改进锂离子电池初始不可逆容量损失
IF 4.3 3区 工程技术
International Journal of Energy Research Pub Date : 2025-07-24 DOI: 10.1155/er/8122951
Hui Gyeong Park, Chi Keung Song, Jongchul Lim, Woo-Jin Song, Jung-Soo Lee
{"title":"Ionic Liquid-Protected Edge Plane of Graphite to Overcome Initial Irreversible Capacity Loss for Improved Lithium-Ion Batteries","authors":"Hui Gyeong Park,&nbsp;Chi Keung Song,&nbsp;Jongchul Lim,&nbsp;Woo-Jin Song,&nbsp;Jung-Soo Lee","doi":"10.1155/er/8122951","DOIUrl":"https://doi.org/10.1155/er/8122951","url":null,"abstract":"&lt;div&gt;\u0000 &lt;p&gt;Lithium-ion batteries (LIBs) are considered indispensable in contemporary life because of their appropriate power density, rechargeability, and exceptional energy density. In recent decades, the crucial role of graphite (Gt) as the primary material for LIB anodes has been established. Although extensive research has been conducted to find alternatives with higher power and energy densities, Gt continues to be selected as the predominant material for commercial LIBs. During the operation of LIBs, the Gt reacts with the electrolyte to form a solid–electrolyte interphase (SEI). This complex and structurally disordered SEI layer acts as a barrier that suppresses undesirable reactions but also increases resistance, which in turn affects the LIB performance. Ionic liquids (ILs) are providing a promising solution for improving LIB performance owing to their nonflammability, low vapor pressure, tunability, and large electrochemical window. In this study, we examined the functionalization of Gt edges by employing 4-bromobenzoic acid (4BAc) via a direct Friedel–Crafts acylation reaction in a polyphosphoric acid (PPA)/phosphorous pentoxide (P&lt;sub&gt;2&lt;/sub&gt;O&lt;sub&gt;5&lt;/sub&gt;) medium. Additionally, we investigated the attachment of IL monomers to modified Gt to control the SEI layer formation. Our research findings demonstrated that IL-modified Gt exhibit significantly improved electrochemical cycle stability and durability, effectively addressing the capacity degradation and limitations of conventional Gt anodes “to” LIBs, indispensable in modern life, owe their ubiquity to their high energy density, rechargeability, and optimal power performance. Among anode materials, Gt has remained the cornerstone of commercial LIBs for decades due to its stability and cost-effectiveness. Despite extensive efforts to identify superior alternatives with enhanced power and energy densities, Gt’s dominance persists. However, during LIB operation, Gt reacts with electrolytes to form a structurally disordered SEI layer. While this layer prevents undesirable side reactions, it also increases resistance, thereby limiting LIB performance. In this study, we introduce a novel approach to address these challenges by functionalizing Gt edges using 4BAc via a direct Friedel–Crafts acylation reaction in a PPA/P&lt;sub&gt;2&lt;/sub&gt;O&lt;sub&gt;5&lt;/sub&gt; medium. Furthermore, IL monomers were grafted onto the modified Gt surface to regulate SEI layer formation. This dual-functionalization strategy uniquely leverages the nonflammability, tunability, and wide electrochemical window of ILs to enhance anode performance. Our findings reveal that IL-modified Gt significantly improves electrochemical cycle stability and durability, mitigating capacity degradation, and resistance issues associated with conventional Gt anodes. This work offers a groundbreaking pathway to overcoming key limitations in LIB technology, advancing the development of next-generation energy storage systems.&lt;/p&gt;\u0000 ","PeriodicalId":14051,"journal":{"name":"International Journal of Energy Research","volume":"2025 1","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1155/er/8122951","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144688246","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Hybrid Renewable Energy and Smart App-Based Management for Efficient and Sustainable EV Charging Infrastructure 混合可再生能源和基于智能应用程序的高效可持续电动汽车充电基础设施管理
IF 4.3 3区 工程技术
International Journal of Energy Research Pub Date : 2025-07-24 DOI: 10.1155/er/5872792
Ammar Ahmed Alkahtani, Ali Q. Al-Shetwi, Mohamed A. El-Hameed, Ibrahem E. Atawi, Fahad A. Sahli, Mousa H. Adaqriri
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