Advanced Energy Materials最新文献

{"title":"Impurity Impacts of Recycling NMC Cathodes","authors":"Zifei Meng, Xiaotu Ma, Jiahui Hou, Yadong Zheng, Yan Wang","doi":"10.1002/aenm.202405383","DOIUrl":"https://doi.org/10.1002/aenm.202405383","url":null,"abstract":"The skyrocketing demands for electric vehicles cause large quantities of spent lithium-ion batteries (LIBs) and pressure on the global supply chain, leading to raw materials shortages and cost increases. In LIBs, LiNi_xMn_yCo_zO₂(NMC) cathodes are one of the major cathode materials. Thus, recycling NMC cathodes from spent lithium-ion batteries is emerging because they contain abundant valuable materials, which can be considered unique “mineral” sources. Impurities are one of the main concerns for introducing recovered materials back into new battery manufacture because impurities are typically considered to impair the properties of recovered materials. However, some impurities can beneficially act as dopants or coatings. To comprehensively understand the effects of different impurities and treat impurities properly, this review summarizes the origin and species of possible impurities which can be introduced during different pretreatment processes, analyzes the methods to remove impurities, and discusses the effects of impurities on the regeneration process and recovered materials. This work also outlines future perspectives for fundamental research about impurities and relevant challenges of the recycling industry, helps academia and manufacturers to create new impurity standards of recovered cathode materials, and suggests opportunities for achieving a circular economy for the lithium-ion batteries industry.","PeriodicalId":111,"journal":{"name":"Advanced Energy Materials","volume":"9 1","pages":""},"PeriodicalIF":27.8,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142992517","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Stable and Efficient Perovskite Photovoltaics via a Three-In-One Passivating Approach by Aminoacetonitrile Hydrochloride","authors":"Yinjiang Liu, Tengfei Kong, Yang Zhang, Zihan Zhao, Weiting Chen, Wenli Liu, Peng Gao, Xu-Dong Wang, Dongqin Bi","doi":"10.1002/aenm.202404638","DOIUrl":"https://doi.org/10.1002/aenm.202404638","url":null,"abstract":"Reducing defect density is of significant importance for enhancing the power conversion efficiency (PCE) and stability of perovskite solar cells (PSCs). While most previous outstanding studies have focused on individual layers within the perovskite device structure. Herein, a three-in-one strategy using the aminoacetonitrile hydrochloride (AmiHCl) molecule to reduce the defects in the bulk and surface of perovskite. The results of the study found that the AmiHCl bottom modification can decrease the number of buried interface holes, doping into bulk perovskite can modulate crystallization via a strong interaction between AmiHCl and perovskite components, and the upper interface modification can inhibit the formation of vacancies by creating hydrogen bonds with A-site cations. This approach yields PSCs with an efficiency of 25.90% and a high fill factor (<i>FF)</i> of 88.54%. Additionally, the modified PSCs show significantly enhanced operational stability, with the PCE retaining more than 90.0% of the initial value after 1350 h of maximum power point tracking.","PeriodicalId":111,"journal":{"name":"Advanced Energy Materials","volume":"206 1","pages":""},"PeriodicalIF":27.8,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142992520","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Functionalized Interlayers in Self-Powered Organic Photodiodes for Enhanced Near-Infrared Sensing","authors":"Yongju Lee, Swarup Biswas, Dong Hyun Nam, Jae Won Park, Hyowon Jang, Hyojeong Choi, Juhwan Kim, Dong-Wook Park, Hyeok Kim","doi":"10.1002/aenm.202403532","DOIUrl":"https://doi.org/10.1002/aenm.202403532","url":null,"abstract":"There is a growing interest in fabricated organic material-based photodiodes (OPDs) since they are lightweight, flexible, and cost-effective to manufacture. Notably, they exhibit near-infrared photo-sensing capabilities that are self-powered, a feature attributed to the tunable optical properties of organic semiconductor (OSC) materials. Nonetheless, the application of OPDs in the semiconductor industry encounters challenges compared to their inorganic counterparts, such as low sensitivity and limited durability. In this study, a self-powered OPD using a poly[4,8-bis(5-(2-ethylhexyl)thiophen-2-yl)benzo [1,2-b:4,5-b′]dithiophene-2,6-diyl-alt-(4-(2-ethylhexyl)-3-fluorothieno[3,4-b]thiophene-)-2-carboxylate-2-6-diyl)]:biaxial active layer of phenyl-C70-butyric acid methyl ester (PTB7-Th:PC₇₀BM) and an organic hole transport layer (HTL) composed of poly(3,4-ethylenedioxythiophene) and poly(styrene sulfonate) (PPY:PSS) is developed. These results highlight the effectiveness of PPY:PSS as an HTL, demonstrating distinct improvements in efficiency, photosensitivity, photo-detectivity, and operational stability of the OPD when the weight ratio between the PPY and PSS is 1:2.","PeriodicalId":111,"journal":{"name":"Advanced Energy Materials","volume":"32 1","pages":""},"PeriodicalIF":27.8,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142992555","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Ambient-Printed Methylammonium-Free Perovskite Solar Cells Enabled by Multiple Molecular Interactions","authors":"Lei Lang, Zicheng Ding, Yachao Du, Nan Wu, Pengchi Liu, Ru Qin, Shuang Wang, Zhichao Wang, Yongchao Tu, Xiujie Liu, Zheng Zhang, Yongshuai Gong, Dongxue Liu, Kui Zhao, Shengzhong (Frank) Liu","doi":"10.1002/aenm.202405423","DOIUrl":"https://doi.org/10.1002/aenm.202405423","url":null,"abstract":"The ambient printing of high-performance and stable perovskite solar cells (PSCs) is crucial for enabling low-cost and energy-efficient industrial fabrication. However, producing high-quality perovskite films via ambient printing remains challenging due to direct exposure to air, which easily induces additional stacking defects and triggers perovskite degradation compared to films fabricated by traditional spin-coating under inert conditions. Here, a multiple molecular interaction strategy is introduced to address this challenge by incorporating a 2-thiazole formamidine hydrochloride (TC) additive, effectively suppressing defect formation during ambient printing. The specific interactions between TC and precursor components, i.e., multiple hydrogen bonds and coordination interactions, could promote the crystallization of α-phase perovskites and reduce cation and anion vacancies simultaneously when drying in air. These endows high-quality ambient-printed perovskite films with large crystalline grains with eliminated nanovoids and low trap-densities, which improve charge carrier dynamics and prevent perovskite decomposition and hydration under thermal/humidity stress during long-term annealing/ambient storage. The unencapsulated PSCs show a high efficiency of 23.72% with good stability, i.e., realizing 92% and 95% efficiency retention after 672 h of annealing at 85 °C in a N₂ atmosphere and after 2088 h of storage in ambient air.","PeriodicalId":111,"journal":{"name":"Advanced Energy Materials","volume":"33 1","pages":""},"PeriodicalIF":27.8,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142992518","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Functional Alloy Collector Capable of Sustainable Lithium Compensation for Anode-Free Batteries by a Controlled Lithium-Prestorage Technology","authors":"Yao Liu, Cheng Zeng, Mingtao Hu, Haoyue Liang, Xinqi Wei, Xinyu Ji, Shuhao Wang, Xizheng Liu, Yanming Cui, Jiu Lin, Tianyou Zhai, Huiqiao Li","doi":"10.1002/aenm.202405960","DOIUrl":"https://doi.org/10.1002/aenm.202405960","url":null,"abstract":"With higher energy density and reduced cost, anode-free battery has attracted great attention from both academic and industry. However, the development of anode-free batteries is hindered by their poor cycle life due to the continuous irreversible lithium (Li) consumption at the anode side. Here, a surface-functionalized alloy foil, which can gradually release active lithium to the cell upon cycling, used as the collector for anode-free batteries is proposed. The alloy foil is prestored with a certain amount of active lithium via a simple wet contacting reaction between the metal foil and liquid lithium source reagent. The prestored lithium amount can be precisely controlled by reagent concentration and contact time. When the foil is used as the anode, its alloyed surface demonstrates a low nucleation barrier for lithium deposition and a more uniform deposition behavior. More importantly, the alloy collector can rationally release active lithium to sustainably compensate for the irreversible Li consumption upon the cycling of a full cell, thus greatly prolonging the cycle life of the anode-free battery by 10 times. Besides, this technique can be extended to diverse metal collectors demonstrating its broad applicability.","PeriodicalId":111,"journal":{"name":"Advanced Energy Materials","volume":"11 1","pages":""},"PeriodicalIF":27.8,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142992519","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Confining Surface Oxygen Redox in Double Perovskites for Enhanced Oxygen Evolution Reaction Activity and Stability","authors":"Natasha Hales, Jinzhen Huang, Benjamin Heckscher Sjølin, Alvaro Garcia-Padilla, Camelia Nicoleta Borca, Thomas Huthwelker, Ivano E. Castelli, Radim Skoupy, Adam H. Clark, Michal Andrzejewski, Nicola Casati, Thomas J. Schmidt, Emiliana Fabbri","doi":"10.1002/aenm.202404560","DOIUrl":"https://doi.org/10.1002/aenm.202404560","url":null,"abstract":"Nickel-based double perovskites AA′BB′O₆ are an underexplored class of oxygen evolution reaction (OER) catalysts, in which B-site substitution is used to tune electronic and structural properties. BaSrNiWO₆, with a B-site comprised of alternating Ni and W, exhibits high oxygen evolution activity, attributed to the evolution of a highly OER active surface phase. The redox transformation of Ni²⁺(3d⁸) to Ni³⁺(3d⁷) combined with partial W dissolution into the electrolyte from the linear Ni(3d)-O(2p)-W(5d) chains drives an in situ reconstruction of the surface to an amorphized, NiO-like layer, promoting oxygen redox in the OER mechanism. However, the high valence W⁶⁺(5d⁰) acts as a stabilizing electronic influence in the bulk, preventing the mobilization of lattice oxygen which is bound in highly covalent W─O bonds. It is proposed that the surface generated during the OER can support a lattice oxygen evolution mechanism (LOEM) in which oxygen vacancies are created and preferentially refilled by electrolytic OH⁻, while bulk O species remain stable. This surface LOEM (sLOEM) allows BaSrNiWO₆ to retain structural integrity during OER catalysis. With a Tafel slope of 45 mV dec⁻¹ in 0.1 <span>m</span> KOH, BaSrNiWO₆ illustrates the potential of Ni-based double perovskites to offer both OER efficiency and bulk stability in alkaline electrolysis.","PeriodicalId":111,"journal":{"name":"Advanced Energy Materials","volume":"8 1","pages":""},"PeriodicalIF":27.8,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142992516","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Host–Guest Complexation of α-Cyclodextrin and Triiodide Ions for Enhanced Performance of Ionic Thermoelectric Capacitors","authors":"Shih-Ting Kao, Ching-Chieh Hsu, Shao-Huan Hong, U-Ser Jeng, Chia-Hsin Wang, Shih-Huang Tung, Cheng-Liang Liu","doi":"10.1002/aenm.202405502","DOIUrl":"https://doi.org/10.1002/aenm.202405502","url":null,"abstract":"Ionic thermoelectric materials have emerged as a promising avenue for harvesting low-grade waste heat, with significant potential for applications in wearable electronics. This study introduces a novel design for ionic thermoelectric capacitors (ITECs) by incorporating host–guest complexation between α–cyclodextrin (α-CD) and triiodide ions (I₃⁻). The strong host–guest complexation between α-CD and I₃⁻ confines the diffusion of I₃⁻ within the cylindrical cavities of α-CD, as evidenced by UV–vis spectroscopy and ¹³C-NMR analysis. This confinement enhances the ion mobility difference between I₃⁻ and sodium ions, which in turn significantly boosts the ionic thermopower of the polyvinyl alcohol/α-CD/NaI hydrogels. Accordingly, the optimized sample achieves an impressive positive ionic thermopower of 14.24 mV K⁻¹ and a high ionic power factor of 477.2 µW K⁻² m⁻¹. Furthermore, the stretchable ITEC demonstrates a substantial power density of 5.9 mW m⁻². When integrated into a 3-leg device, a stable thermovoltage of 176 mV is generated under a temperature gradient of 4.4 K, thus highlighting the potential of this system for efficient thermal energy harvesting.","PeriodicalId":111,"journal":{"name":"Advanced Energy Materials","volume":"120 1","pages":""},"PeriodicalIF":27.8,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142992522","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Boosting Li-Metal Anode Performance with Lithiophilic Li–Zn Seeds in a 2D Reduced Graphene Oxide Scaffold (Adv. Energy Mater. 3/2025)","authors":"Xiaoze Zhou, Shuaiqi Wang, Yaru Li, Yi Yang, Xiao Xiao, Gang Chen","doi":"10.1002/aenm.202570015","DOIUrl":"https://doi.org/10.1002/aenm.202570015","url":null,"abstract":"<b>Li-Metal Anodes</b>","PeriodicalId":111,"journal":{"name":"Advanced Energy Materials","volume":"10 1","pages":""},"PeriodicalIF":27.8,"publicationDate":"2025-01-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142991620","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Dual Strategies of Na+ Electrolyte Additives and Dendrites Protective Ti3C2TX-MXene/Zn Anode with 2D MXene Nanosheet Encased Niobium Pyrophosphate (NbP2O7) Composite Binder-Free Cathode for Stable Zinc-Ion Storage (Adv. Energy Mater. 3/2025)","authors":"Amar M. Patil, Hyo-Min You, Arti A. Jadhav, Jongwoo Hong, Sushanta K. Das, Suprimkumar D. Dhas, Tae Jin Lim, Eunbyoul Lee, Kyung Yoon Chung, Kyeounghak Kim, Seong Chan Jun","doi":"10.1002/aenm.202570013","DOIUrl":"https://doi.org/10.1002/aenm.202570013","url":null,"abstract":"<b>Zinc-Ion Capacitors</b>","PeriodicalId":111,"journal":{"name":"Advanced Energy Materials","volume":"37 1","pages":""},"PeriodicalIF":27.8,"publicationDate":"2025-01-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142991619","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Phase Transition Behavior During Sintering Process of Li-Rich Materials","authors":"Mengke Zhang, Jiayang Li, Qi Pang, Weibo Hua, Yuting Deng, Manqi Tang, Weikong Pang, Zhenguo Wu, Benhe Zhong, Yao Xiao, Lang Qiu, Xiaodong Guo","doi":"10.1002/aenm.202406031","DOIUrl":"https://doi.org/10.1002/aenm.202406031","url":null,"abstract":"Phase transition serves as an ordinary behavior occurring during the high-temperature calcination process, while it becomes quite complicated in Li-rich materials composed of rhombohedral phase LiTMO&lt;sub&gt;2&lt;/sub&gt; (TM: Ni, Mn) with &lt;i&gt;R&lt;/i&gt;&lt;span data-altimg=\"/cms/asset/8075c819-931b-4ff7-b149-7f022f6f6fe5/aenm202406031-math-0001.png\"&gt;&lt;/span&gt;&lt;mjx-container ctxtmenu_counter=\"2\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"&gt;&lt;mjx-math aria-hidden=\"true\" location=\"graphic/aenm202406031-math-0001.png\"&gt;&lt;mjx-semantics&gt;&lt;mjx-mover data-semantic-children=\"0,1\" data-semantic- data-semantic-role=\"integer\" data-semantic-speech=\"ModifyingAbove 3 With bar\" data-semantic-type=\"overscore\"&gt;&lt;mjx-over style=\"padding-bottom: 0.105em; margin-bottom: -0.544em;\"&gt;&lt;mjx-mo data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"overaccent\" data-semantic-type=\"operator\"&gt;&lt;mjx-stretchy-h style=\"width: 0.5em;\"&gt;&lt;mjx-ext&gt;&lt;mjx-c&gt;&lt;/mjx-c&gt;&lt;/mjx-ext&gt;&lt;/mjx-stretchy-h&gt;&lt;/mjx-mo&gt;&lt;/mjx-over&gt;&lt;mjx-base&gt;&lt;mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\"&gt;&lt;mjx-c&gt;&lt;/mjx-c&gt;&lt;/mjx-mn&gt;&lt;/mjx-base&gt;&lt;/mjx-mover&gt;&lt;/mjx-semantics&gt;&lt;/mjx-math&gt;&lt;mjx-assistive-mml display=\"inline\" unselectable=\"on\"&gt;&lt;math altimg=\"urn:x-wiley:16146832:media:aenm202406031:aenm202406031-math-0001\" display=\"inline\" location=\"graphic/aenm202406031-math-0001.png\" xmlns=\"http://www.w3.org/1998/Math/MathML\"&gt;&lt;semantics&gt;&lt;mover accent=\"true\" data-semantic-=\"\" data-semantic-children=\"0,1\" data-semantic-role=\"integer\" data-semantic-speech=\"ModifyingAbove 3 With bar\" data-semantic-type=\"overscore\"&gt;&lt;mn data-semantic-=\"\" data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\"&gt;3&lt;/mn&gt;&lt;mo data-semantic-=\"\" data-semantic-parent=\"2\" data-semantic-role=\"overaccent\" data-semantic-type=\"operator\"&gt;¯&lt;/mo&gt;&lt;/mover&gt;${bar{3}}$&lt;/annotation&gt;&lt;/semantics&gt;&lt;/math&gt;&lt;/mjx-assistive-mml&gt;&lt;/mjx-container&gt;&lt;i&gt;m&lt;/i&gt; space group and monoclinic phase Li&lt;sub&gt;2&lt;/sub&gt;TMO&lt;sub&gt;3&lt;/sub&gt; with &lt;i&gt;C&lt;/i&gt;2/&lt;i&gt;m&lt;/i&gt; space group. Yet to be firmly elucidated is how the precursor transforms into LiTMO&lt;sub&gt;2&lt;/sub&gt; (&lt;i&gt;R&lt;/i&gt;&lt;span data-altimg=\"/cms/asset/0575498d-35a3-4359-92fa-12776aeebbb1/aenm202406031-math-0002.png\"&gt;&lt;/span&gt;&lt;mjx-container ctxtmenu_counter=\"3\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" role=\"application\" sre-explorer- style=\"font-size: 103%; position: relative;\" tabindex=\"0\"&gt;&lt;mjx-math aria-hidden=\"true\" location=\"graphic/aenm202406031-math-0002.png\"&gt;&lt;mjx-semantics&gt;&lt;mjx-mover data-semantic-children=\"0,1\" data-semantic- data-semantic-role=\"integer\" data-semantic-speech=\"ModifyingAbove 3 With bar\" data-semantic-type=\"overscore\"&gt;&lt;mjx-over style=\"padding-bottom: 0.105em; margin-bottom: -0.544em;\"&gt;&lt;mjx-mo data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"overaccent\" data-se","PeriodicalId":111,"journal":{"name":"Advanced Energy Materials","volume":"84 1","pages":""},"PeriodicalIF":27.8,"publicationDate":"2025-01-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142992557","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}