Advanced Sensor and Energy Materials最新文献

Editorial: Recent advances in biosensor and energy storage materials 编辑：生物传感器和储能材料的最新进展

Advanced Sensor and Energy Materials Pub Date : 2025-04-22 DOI: 10.1016/j.asems.2025.100151

Juewen Liu

引用次数: 0

Wearable electrochemical sensor for real-time sweat monitoring powered by Li–S battery: Rapid ion-electron transduction driven by high-entropy Prussian blue analogues 用于实时汗液监测的可穿戴电化学传感器，由锂-S 电池供电：高熵普鲁士蓝类似物驱动的快速离子-电子转换

Advanced Sensor and Energy Materials Pub Date : 2025-03-18 DOI: 10.1016/j.asems.2025.100150

Zhong-Hui Sun , Qiu-Ling Huang , Zhan-Chao Li , Wei Zheng , Yan Mao , Dong-Xue Han , Gang Huang

{"title":"Wearable electrochemical sensor for real-time sweat monitoring powered by Li–S battery: Rapid ion-electron transduction driven by high-entropy Prussian blue analogues","authors":"Zhong-Hui Sun , Qiu-Ling Huang , Zhan-Chao Li , Wei Zheng , Yan Mao , Dong-Xue Han , Gang Huang","doi":"10.1016/j.asems.2025.100150","DOIUrl":"10.1016/j.asems.2025.100150","url":null,"abstract":"<div><div>The portable electrochemical sensors couple with high-energy density batteries lay the foundation for intelligent electronic devices capable of real-time and long-term monitoring of signals at the molecular level. Currently, high-entropy materials play a crucial role in advanced energy storage system and electroanalytical chemistry due to their powerful multi active centers and lattice strain fields. Herein, we propose high-entropy Prussian blue analogues (HE-PBA) as a bidirectional catalyst to reduce the activation energy of sulfur redox reaction, alleviate polysulfides shuttle, and inhibit lithium dendritic growth in Li–S battery. Furthermore, benefited from hierarchical HE-PBA with multiple redox active sites, superior ion-selective effect, high ionic/electrical conductivity and hydrophobicity, thus contributing to splendid ion-electron transducer capability as solid contact layer in wearable potentiometric electrochemical sensors. As a result, an advanced wearable electronic device integrates LSB as a power source with potentiometric electrochemical sensor unit equipped with ion selective electrode, enabling real-time monitoring of K<sup>+</sup> concentration in sweat metabolite during outdoor exercise. In a word, this work demonstrates a tremendous potential of designing multifunctional electrode materials for advanced energy storage and electrochemical sensing applications through high entropy strategies.</div></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"4 2","pages":"Article 100150"},"PeriodicalIF":0.0,"publicationDate":"2025-03-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143828520","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Mid-infrared integrated spectroscopic sensor based on chalcogenide glasses: Optical characterization and sensing applications 基于硫系玻璃的中红外集成光谱传感器：光学特性和传感应用

Advanced Sensor and Energy Materials Pub Date : 2025-03-18 DOI: 10.1016/j.asems.2025.100149

S. Meziani , A. Hammouti , L. Bodiou , N. Lorrain , R. Chahal , A. Bénardais , R. Courson , J. Troles , C. Boussard-Plédel , V. Nazabal , J. Charrier

{"title":"Mid-infrared integrated spectroscopic sensor based on chalcogenide glasses: Optical characterization and sensing applications","authors":"S. Meziani , A. Hammouti , L. Bodiou , N. Lorrain , R. Chahal , A. Bénardais , R. Courson , J. Troles , C. Boussard-Plédel , V. Nazabal , J. Charrier","doi":"10.1016/j.asems.2025.100149","DOIUrl":"10.1016/j.asems.2025.100149","url":null,"abstract":"<div><div>A mid-infrared (mid-IR) spectroscopic sensor is developed using a chalcogenide glasses (ChGs) platform with a broad transmission band. The ridge ChGs waveguides were patterned via standard i-line photolithography and reactive ion etching, following the deposition of guiding and confinement layers through RF magnetron sputtering. The waveguides exhibit a wide transparency range from <em>λ</em> = 3.94–8.95 μm, with minimum propagation losses value of 2.5 dB/cm at <em>λ</em> = 7.58 μm. To validate the feasibility of the suggested sensor, a spectroscopic gas sensing experiment was performed using CO<sub>2</sub>, resulting in an estimated limit of detection (LoD) of 1.16%v at <em>λ</em> = 4.28 μm, achieved with an external confinement factor <em>Γ</em> of 6.5%. Additionally, liquid sensing experiment was carried out using isopropanol, obtaining a LoD of 300 ppmv at <em>λ</em> = 7.25 μm.</div></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"4 3","pages":"Article 100149"},"PeriodicalIF":0.0,"publicationDate":"2025-03-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143937792","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Corrigendum to “Needle−tip effect promoted flexible electrochemical sensor for detecting chloride ions in food by in−situ deposited silver dendrimers” [Adv Sensor Energy Mater 3 (2024) 100100] “针尖效应促进的柔性电化学传感器用于原位沉积银树突物检测食品中的氯离子”的勘误表[Adv传感器能量物质3 (2024)100100]

Advanced Sensor and Energy Materials Pub Date : 2025-03-10 DOI: 10.1016/j.asems.2024.100130

Huang Dai , Huilin Hu , Zhiyong Gong , Jing Shu , Jiahua Wang , Xiaodan Liu , Fuwei Pi , Qiao Wang , Shuo Duan , Yingli Wang

引用次数: 0

Enhanced multienzyme-like and antibacterial activity by copper atomically dispersed into molybdenum disulfide for accelerated wound healing 铜原子分散到二硫化钼中加速伤口愈合，增强了多酶样和抗菌活性

Advanced Sensor and Energy Materials Pub Date : 2025-03-08 DOI: 10.1016/j.asems.2025.100148

Jiahao Shen , Junli Liu , Yunxiao Yi , Chenhui He , Hengyu Liu , Linrong Shi , Jin Liu , Pingen Shi , Hui Liu , Xuanmeng He , Yi Feng , Xingjian Song , Shaowei Chen

{"title":"Enhanced multienzyme-like and antibacterial activity by copper atomically dispersed into molybdenum disulfide for accelerated wound healing","authors":"Jiahao Shen , Junli Liu , Yunxiao Yi , Chenhui He , Hengyu Liu , Linrong Shi , Jin Liu , Pingen Shi , Hui Liu , Xuanmeng He , Yi Feng , Xingjian Song , Shaowei Chen","doi":"10.1016/j.asems.2025.100148","DOIUrl":"10.1016/j.asems.2025.100148","url":null,"abstract":"<div><div>Bacterial and viral infections have been a global challenge, exacerbated by rampant antibiotic overuse. It is thus of fundamental and technological significance to develop effective antibacterial agents. Herein, copper is atomically dispersed into a MoS<sub>2</sub> matrix via the chelation of ammonium tetrathiomolybdate [(NH<sub>4</sub>)<sub>2</sub>MoS<sub>4</sub>]. Meticulous control of the copper content enables uniform atomic dispersion and optimizes active site accessibility, both critical factors for a range of catalytic activities that mimic native enzymes like peroxidase, superoxide dismutase and glutathione oxidase. Among the series, the Cu/MoS<sub>2</sub>-3 sample, with a Cu:Mo molar ratio of ca. 0.3, exhibits the best activity, with a maximum rate of 14.3 × 10<sup>−18</sup> M s<sup>–</sup><sup>1</sup> in the peroxidase-like reaction with H<sub>2</sub>O<sub>2</sub> and rate constant of 2.56 × 10<sup>−3</sup> s<sup>−1</sup> that are at least one order of magnitude greater than those of MoS<sub>2</sub>. These unique properties endow the resultant Cu/MoS<sub>2</sub> composites with a remarkable antimicrobial activity. Experimentally, with the addition of 1 mM H<sub>2</sub>O<sub>2</sub>, 99% of Gram-positive <em>Staphylococcus aureus</em> and Gram-negative <em>Escherichia coli</em> can be eliminated within 10 min by Cu/MoS<sub>2</sub> (50 μg/mL). Such a peroxidase-like activity of Cu/MoS<sub>2</sub> can facilitate wound healing and inflammation reduction in a <em>Staphylococcus aureus</em> infected wound model. Results from this study highlight the unique significance of atomic dispersion in the structural engineering of high-performance bactericidal agents for biomedical applications.</div></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"4 2","pages":"Article 100148"},"PeriodicalIF":0.0,"publicationDate":"2025-03-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143792342","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Metal-bearing nanomaterials for oral antibacteria: Mechanisms and applications 含金属纳米口腔抗菌材料：机理与应用

Advanced Sensor and Energy Materials Pub Date : 2025-03-03 DOI: 10.1016/j.asems.2025.100141

Ke Quan , Yuqing Zeng , Sijia Gao , Yanli Lei , Le Yang , Yibo Zhou , Lucky Poh Wah Goh , Zhihe Qing

{"title":"Metal-bearing nanomaterials for oral antibacteria: Mechanisms and applications","authors":"Ke Quan , Yuqing Zeng , Sijia Gao , Yanli Lei , Le Yang , Yibo Zhou , Lucky Poh Wah Goh , Zhihe Qing","doi":"10.1016/j.asems.2025.100141","DOIUrl":"10.1016/j.asems.2025.100141","url":null,"abstract":"<div><div>The prevalent oral diseases, such as dental caries, chronic gingivitis, and periodontitis, which are primarily caused by pathogenic bacteria, pose significant public health risks and impose substantial economic burdens. However, conventional treatment strategies for oral pathogens rely on mechanical debridement and antibiotic treatment, which remain unsatisfactory and contribute to the emergence of antimicrobial resistance pathogens. The escalating crisis of antibiotic resistance and the intricate microbial communities in oral niches urgently demand innovative antimicrobial strategies that can overcome these issues. Metal-bearing nanomaterials (MBNs), as an integration of metallic components with other substances such as polymers or inorganic materials, have demonstrated improved antimicrobial effectiveness while mitigating the toxicity associated with pure metals in oral environments. This review provides an innovative overview of designing and utilizing MBNs for oral antimicrobial applications, bridging the gap between nanomaterial design and clinical dentistry needs while guiding the development of next-generation antimicrobials in the post-antibiotic era. Firstly, we categorize and elucidate the main antibacterial mechanisms of metallic components in MBNs. Furthermore, a comprehensive summary is provided on the up-to-date advancements in using MBNs for oral antibacterial purposes, highlighting the pivotal role of metals in enhancing antibacterial properties. Finally, we discuss the existing challenges and potential future developments to establish a theoretical foundation for ongoing progress and clinical approval.</div></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"4 2","pages":"Article 100141"},"PeriodicalIF":0.0,"publicationDate":"2025-03-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143843783","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Editorial: Recent approaches in biosensors and wearable sensors 社论：生物传感器和可穿戴传感器的最新进展

Advanced Sensor and Energy Materials Pub Date : 2025-03-01 DOI: 10.1016/j.asems.2025.100143

Chengyi Xiong

引用次数: 0

Simple surface modification of poly(methyl methacrylate) microfluidic microplates for enhanced ultrasensitive multiplexed detection of infectious diseases 聚甲基丙烯酸甲酯微流控微孔板的简单表面修饰，增强了传染病的超灵敏多路检测

Advanced Sensor and Energy Materials Pub Date : 2025-02-28 DOI: 10.1016/j.asems.2025.100142

Sharma T. Sanjay , Sapna Kannan , XiuJun Li

{"title":"Simple surface modification of poly(methyl methacrylate) microfluidic microplates for enhanced ultrasensitive multiplexed detection of infectious diseases","authors":"Sharma T. Sanjay , Sapna Kannan , XiuJun Li","doi":"10.1016/j.asems.2025.100142","DOIUrl":"10.1016/j.asems.2025.100142","url":null,"abstract":"<div><div>Novel strategies for the simultaneous and portable detection of multiple analytes are highly favorable for clinical diagnosis and healthcare. Conventional colorimetric enzyme-linked immunosorbent assay (ELISA) is a widely used laboratory technique for medical diagnostics, quality control, and research applications. However, nonspecific absorption of proteins may lead to a reduction of functional sites, resulting in high background and low sensitivity in ELISA. Herein, we report a simple method of functionalization of poly(methyl methacrylate) (PMMA) with polylysine to be used as the microfluidic microplate substrate for enhanced ELISA, enabling rapid, ultrasensitive, and multiplexed detection of infectious diseases. FTIR and fluorescence microscopy characterization confirmed high amine densities on polylysine-modified PMMA surface, resulting in high detection sensitivity of the colorimetric ELISA on the PMMA microdevice. The ultrasensitive polylysine-modified microplate can immobilize protein within 20 min and results of the assay can be viewed by the naked eye or scanned through a simple desktop scanner for quantitative analysis within 90 min. A sandwich-type immunoassay for the rapid and sensitive detection of immunoglobulin G (IgG), hepatitis B surface antigen (HBsAg), and hepatitis B core antigen (HBcAg) was demonstrated as a proof-of-concept for multiplexed detection. The limits of detection (LOD) of 200.0 pg/mL for IgG, 180.0 pg/mL for HBsAg, and 300.0 pg/mL for HBcAg were achieved, without any specialized equipment like a microplate reader. The surface-modified microchip exhibited about 10-fold higher sensitivity than traditional microplates. This surface-modified microplate has tremendous potential as a point-of-care multiplexed testing platform for many applications ranging from clinical diagnosis to environmental monitoring, particularly in resource-limited settings.</div></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"4 2","pages":"Article 100142"},"PeriodicalIF":0.0,"publicationDate":"2025-02-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143847360","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

3D-printed microneedles for sensing applications: Emerging topics and future trends 用于传感应用的3d打印微针：新兴主题和未来趋势

Advanced Sensor and Energy Materials Pub Date : 2025-02-27 DOI: 10.1016/j.asems.2025.100139

Kelcilene B.R. Teodoro , Tamires S. Pereira , Ana Laura M.M. Alves , Francisco V. dos Santos , Fabrício A. dos Santos , Daniel S. Correa

{"title":"3D-printed microneedles for sensing applications: Emerging topics and future trends","authors":"Kelcilene B.R. Teodoro , Tamires S. Pereira , Ana Laura M.M. Alves , Francisco V. dos Santos , Fabrício A. dos Santos , Daniel S. Correa","doi":"10.1016/j.asems.2025.100139","DOIUrl":"10.1016/j.asems.2025.100139","url":null,"abstract":"<div><div>3D-printed microneedles (MNs) have revolutionized the biomedical sector, enabling applications in aesthetic treatments, vaccine delivery, diagnostics, and real-time biomarker analysis. These minimally invasive structures advance the development of sensors and biosensors for diverse applications, including human, veterinary, agricultural, and environmental domains. Recent trends favor MNs made from polymers and nanomaterials over traditional metals, addressing challenges related to cost, biocompatibility, and scalability. In this context, this review explores recent advancements on different MNs-based sensors, fabricated by 3D printing, highlighting innovations, shortcomings and also pointing future opportunities to expand their applications in medical, agricultural and environmental domains. Initially, we discuss the general aspects of planning an efficient MN's design (encompassing possible types and required properties), as well as the choice of materials and manufacturing techniques for 3D printing polymeric MNs. Next, we examine the relationship between printing techniques, the manufactured MNs, and their integration with sensors, followed by examples of studies that explore this connection. Key innovations include the use of biodegradable resins, nanocomposites, artificial intelligence, and machine learning for design optimization. While biomedical applications dominate, we highlight significant opportunities for MNs in agriculture and environmental monitoring through tailored manufacturing approaches.</div></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"4 2","pages":"Article 100139"},"PeriodicalIF":0.0,"publicationDate":"2025-02-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143934927","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Fluorescent graphene quantum dots: Properties regulation, sensing applications, and future prospects 荧光石墨烯量子点：特性调控、传感应用及未来展望

Advanced Sensor and Energy Materials Pub Date : 2025-02-26 DOI: 10.1016/j.asems.2025.100140

Ru Wu , Yue Cao , Zixuan Chen , Jun-Jie Zhu

引用次数: 0