Advanced Sensor and Energy Materials最新文献

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Unveiling the synthesis, characteristics, electrical conductivity, photocatalytic activity, and electrochemical activity of eco-friendly zinc oxide nanoparticles 揭示环保型纳米氧化锌的合成、特性、导电性、光催化活性和电化学活性
Advanced Sensor and Energy Materials Pub Date : 2024-05-15 DOI: 10.1016/j.asems.2024.100105
Redwanul Islam , Suprio Shantanu Saha , Reana Raen , Nayeemul Islam , Torikul Islam
{"title":"Unveiling the synthesis, characteristics, electrical conductivity, photocatalytic activity, and electrochemical activity of eco-friendly zinc oxide nanoparticles","authors":"Redwanul Islam ,&nbsp;Suprio Shantanu Saha ,&nbsp;Reana Raen ,&nbsp;Nayeemul Islam ,&nbsp;Torikul Islam","doi":"10.1016/j.asems.2024.100105","DOIUrl":"10.1016/j.asems.2024.100105","url":null,"abstract":"<div><p>The <em>Nigella Sativa</em> seeds were utilized for the environment-friendly zinc oxide nanoparticles (ZnO NPs), as evident by the observation of a white precipitate. Numerous analytical techniques, such as XRD, FTIR, UV–vis, SEM, and EDX, were utilized to describe the specimen's structural, optical, and electrical properties. XRD analysis was used to confirm that the ZnO NPs were crystalline. An absorbance peak at 401 nm was observed in the UV–vis, indicating that the ZnO NPs have a 2.91 eV bandgap. Functional groups are present in ZnO NPs, as seen by the FTIR graph. The nanoparticles' spherical form and average size of 37.9 nm were confirmed by the SEM image. EDX analysis confirmed the composition of the nanoparticles, with zinc accounting for 73.17% and oxygen for 26.83%. ZnO NPs demonstrated excellent electrical conductivity because of their higher surface-to-volume ratio. Additionally, the synthesis of ZnO NPs exhibited effective degradation of methylene blue dye. These results point to potential applications in several domains, including electronics, biomedical devices, industry, and agriculture, and they call for immediate follow-up research.</p></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"3 3","pages":"Article 100105"},"PeriodicalIF":0.0,"publicationDate":"2024-05-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773045X24000165/pdfft?md5=694b8a30b8b6232e98fb18669ace6289&pid=1-s2.0-S2773045X24000165-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141052514","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Three-in-one DNA nanowheels for simultaneous tumor regression and drug resistance prevention in breast cancer model 在乳腺癌模型中同时实现肿瘤消退和抗药性预防的三合一 DNA 纳米轮
Advanced Sensor and Energy Materials Pub Date : 2024-05-13 DOI: 10.1016/j.asems.2024.100104
Ping Li , Chun-Feng Feng , Peng-Fei Lyu , Fei Liu , Hui-Sheng Li , Li-Qun Zhang
{"title":"Three-in-one DNA nanowheels for simultaneous tumor regression and drug resistance prevention in breast cancer model","authors":"Ping Li ,&nbsp;Chun-Feng Feng ,&nbsp;Peng-Fei Lyu ,&nbsp;Fei Liu ,&nbsp;Hui-Sheng Li ,&nbsp;Li-Qun Zhang","doi":"10.1016/j.asems.2024.100104","DOIUrl":"10.1016/j.asems.2024.100104","url":null,"abstract":"<div><p>Herein, we proposed novel three-in-one DNA nanowheels with simultaneous chemo and gene therapy to treat tumor, especially to prevent simultaneous drug resistance, which could be disassembled <em>via</em> a cascaded hybridization reactions triggered by the highly expressed microRNA in cancer cells for smart and efficient cancer therapy. Typically, with breast cancer as a model, microRNA 21 could trigger the self-disassembly of DNA nanowheel 1 <em>via</em> hybridization with a specially designed oligonucleotide (anti-microRNA 21) in DNA nanowheel 1, releasing another special oligonucleotide (Contact sequence) to trigger the self-disassembly of DNA nanowheel 2 with releasing of a special oligonucleotide (anti-Contact sequence) to trigger the self-disassembly of DNA nanowheel 1 cyclically, and thus the cascaded hybridization reactions with three-in-one anti-cancer functions could be generated based on three main therapeutic effects <em>via</em> releasing doxorubicin to inhibit macromolecular biosynthesis, antisense oligonucleotide of microRNA 21 to activate the apoptotic cell pathway and antisense oligonucleotide of MDR1 to prevent the drug resistance respectively. As expected, the proposed method showed improved therapeutic efficacy on the cancer cells with about 80% apoptosis ratio, especially on the drug resistant cancer cells with about 75% apoptosis ratio, compared with that in the conventional anti-cancer systems of about 70% on cancer cells and below 40% on drug resistant cancer cells, respectively. Most importantly, this strategy opened the door for generation of complex functional DNA-based structures for target triggering drugs releasing system combining with chemo- and gene-therapy to generate tumor regression and prevent drug resistance with an optimized therapeutic efficacy, providing a new avenue for efficient cancer treatment, especially drug resistant cancers.</p></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"3 3","pages":"Article 100104"},"PeriodicalIF":0.0,"publicationDate":"2024-05-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773045X24000153/pdfft?md5=ac5e863c59149740a770207108aac21b&pid=1-s2.0-S2773045X24000153-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141045037","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Pencil drawn interdigitated capacitive sensors on wood substrate 铅笔绘制的木质基底互嵌电容式传感器
Advanced Sensor and Energy Materials Pub Date : 2024-04-22 DOI: 10.1016/j.asems.2024.100103
{"title":"Pencil drawn interdigitated capacitive sensors on wood substrate","authors":"","doi":"10.1016/j.asems.2024.100103","DOIUrl":"10.1016/j.asems.2024.100103","url":null,"abstract":"<div><p>This research presents the fabrication and characterization of an interdigitated capacitive (IDC) sensor on a wooden substrate using pencil traces. The resistance of the pencil traces decreased from 100 kΩ to 5 kΩ as the pencil grade shifted from HB to 8B. Concurrently, capacitance measurements revealed an increase from approximately 5 pF for a 5-finger IDC made with HB pencil to around 32 pF for an 8B pencil counterpart. Increasing the number of pencil traces from 10 to 50 resulted in a significant decrease in resistance and a proportional increase in capacitance. Application of the IDC sensor demonstrated notable changes in capacitance upon proximity and touch, with a significant decrease upon removal. The interdigitated capacitance sensor exhibits good proximity effects and contact sensitivity in touch, with capacitance increasing exponentially from 0.3 pF (7 cm) to 1.2 pF (direct contact), highlighting its ability to detect objects with high precision. Additionally, environmental factors such as temperature and humidity influence capacitance values. These findings underscore the potential of pencil-drawn IDC sensors for responsive and adaptable applications in various fields.</p></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"3 4","pages":"Article 100103"},"PeriodicalIF":0.0,"publicationDate":"2024-04-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773045X24000141/pdfft?md5=7636fc9618b2d2125a50e0329f4d402b&pid=1-s2.0-S2773045X24000141-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140778500","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Evaluating the impact of delayed centrifugation on protein profiles analyzed by LC/MS in serum and plasma samples 评估延迟离心对通过 LC/MS 分析血清和血浆样本中蛋白质概况的影响
Advanced Sensor and Energy Materials Pub Date : 2024-04-15 DOI: 10.1016/j.asems.2024.100101
Jingyi Si , Yifan Gao , Binjian Yan , Xizhong Shen , Changfeng Zhu , Qunyan Yao
{"title":"Evaluating the impact of delayed centrifugation on protein profiles analyzed by LC/MS in serum and plasma samples","authors":"Jingyi Si ,&nbsp;Yifan Gao ,&nbsp;Binjian Yan ,&nbsp;Xizhong Shen ,&nbsp;Changfeng Zhu ,&nbsp;Qunyan Yao","doi":"10.1016/j.asems.2024.100101","DOIUrl":"https://doi.org/10.1016/j.asems.2024.100101","url":null,"abstract":"<div><p>The pre-analytical steps in blood-based liquid biopsy, involving sample collection techniques and storage conditions, play a critical role in ensuring the integrity and reliability of collected samples. These steps have a directly impact on the accuracy and reliability of test results and are therefore of utmost importance. Mass spectrometry (MS)-based proteomics is an exceptionally powerful tool in the field of liquid biopsy. It enables the comprehensive analysis of the protein content within biological specimens, providing valuable insights into the underlying mechanisms and pathogenesis of diseases. In this study, we aim to explore the variations in the protein landscape between serum and plasma specimens and evaluate the impact of delayed centrifugation on LC/MS-analyzed protein profiles. We seek to provide recommendations on optimal pre-analytical protocols for MS-based proteomics studies. This will enhance the accuracy and reliability of liquid biopsy for precision medicine, ultimately leading to improved patient outcomes.</p></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"3 2","pages":"Article 100101"},"PeriodicalIF":0.0,"publicationDate":"2024-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773045X24000128/pdfft?md5=493e773c29b819f9ead66dea824ec007&pid=1-s2.0-S2773045X24000128-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140650503","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Heteroatom self-doped graphitic carbon materials from Sargassum thunbergii with improved supercapacitance performance 具有更好超级电容性能的马尾藻自掺杂杂原子石墨碳材料
Advanced Sensor and Energy Materials Pub Date : 2024-04-12 DOI: 10.1016/j.asems.2024.100102
Hui Xu , Lina Dong , Bing Zhang , Kun Wang , Jiafeng Meng , Yanwei Tong , Hua Wang
{"title":"Heteroatom self-doped graphitic carbon materials from Sargassum thunbergii with improved supercapacitance performance","authors":"Hui Xu ,&nbsp;Lina Dong ,&nbsp;Bing Zhang ,&nbsp;Kun Wang ,&nbsp;Jiafeng Meng ,&nbsp;Yanwei Tong ,&nbsp;Hua Wang","doi":"10.1016/j.asems.2024.100102","DOIUrl":"https://doi.org/10.1016/j.asems.2024.100102","url":null,"abstract":"<div><p>It is well-known that high specific surface area and improved pore structure is significantly desired for the application of supercapacitor based on biomass-based activated carbon. Herein, <em>Sargassum thunbergii</em> was selected as carbon precursor. Then, a simple and environmentally friendly method was designed to synthesize heteroatom self-doped porous carbon materials via synchronous activation and graphitization by using K<sub>2</sub>FeO<sub>4</sub>. Our results demonstrated that activation temperature plays an important role in porous structure, morphology, and degree of graphitization, thus affecting the performance of supercapacitance. <em>Sargassum thunbergii</em>-based graphitized porous carbons STGPC-2 sample (calcination temperature at 700 °C) has a large specific surface area (1641.98 m<sup>2</sup> g<sup>−1</sup>), pore volume (0.91 cm<sup>3</sup> g<sup>−1</sup>), high microporosity (<em>V</em><sub>micro</sub> = 0.62 cm<sup>3</sup> g<sup>−1</sup>, more than 68%), and a certain degree of graphitization. In three-electrode system, The STGPC-2 electrode exhibited a high specific capacitance of 325.5 F g<sup>−1</sup> at 0.5 A g<sup>−1</sup> and displays high rate capability (248 F g<sup>−1</sup> at 10 A g<sup>−1</sup> in 6 M KOH electrolyte). The symmetric STGPC-2 supercapacitor exhibits energy density as high as 21.3 Wh kg<sup>−1</sup> (at a power density of 450 W kg<sup>−1</sup>) and excellent long-term cycling stability (97% capacitance retention after 3000 cycles) in 1 M Na<sub>2</sub>SO<sub>4</sub> electrolyte.</p></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"3 2","pages":"Article 100102"},"PeriodicalIF":0.0,"publicationDate":"2024-04-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773045X2400013X/pdfft?md5=bd62eca1a8a03cd062b2029088d24f3c&pid=1-s2.0-S2773045X2400013X-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140893606","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Needle−tip effect promoted flexible electrochemical sensor for detecting chloride ions in food by in−situ deposited silver dendrimers 利用原位沉积银树枝形分子促进针尖效应的柔性电化学传感器检测食品中的氯离子
Advanced Sensor and Energy Materials Pub Date : 2024-04-10 DOI: 10.1016/j.asems.2024.100100
Huang Dai , Huilin Hu , Zhiyong Gong , Jing Shu , Jiahua Wang , Xiaodan Liu , Fuwei Pi , Qiao Wang , Shuo Duan , Yingli Wang
{"title":"Needle−tip effect promoted flexible electrochemical sensor for detecting chloride ions in food by in−situ deposited silver dendrimers","authors":"Huang Dai ,&nbsp;Huilin Hu ,&nbsp;Zhiyong Gong ,&nbsp;Jing Shu ,&nbsp;Jiahua Wang ,&nbsp;Xiaodan Liu ,&nbsp;Fuwei Pi ,&nbsp;Qiao Wang ,&nbsp;Shuo Duan ,&nbsp;Yingli Wang","doi":"10.1016/j.asems.2024.100100","DOIUrl":"10.1016/j.asems.2024.100100","url":null,"abstract":"<div><p>Salt plays a crucial role in food processing and consumption, and the rapid detection of chloride ions in food and feed has great significance for practical applications. In this work, Ag−based nanomaterials were deposited on the surface of a flexible integrated electrochemical sensor for the detection of Cl<sup>−</sup> in food. In order to enhance the detection performance, a unique needle−tip structure was formed by manipulating the electro−engraving process during the electrodeposition growth. Theoretical calculations and electrochemical investigations have demonstrated that the dendrimer’s rich tip structure significantly enhanced its electrochemical performance. A sensitive and flexible integrated electrochemical sensor was creatively developed for the detection of Cl<sup>−</sup> using needle−tip effect−promoted Ag micro dendrimers. The sensor achieved quantitative detection of Cl<sup>−</sup> over a dynamic range of 10.0 μM–100.0 mM, with a low limit of detection of 0.148 μM. The flexible electrochemical sensor proposed in this work exhibited good repeatability, selectivity and recoveries in real food samples.</p></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"3 4","pages":"Article 100100"},"PeriodicalIF":0.0,"publicationDate":"2024-04-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773045X24000116/pdfft?md5=7f1732a8a93054fff68eb3a6c33e9d2c&pid=1-s2.0-S2773045X24000116-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141997598","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Editorial for special issue: Electrochemical sensing and imaging 特刊编辑:电化学传感与成像
Advanced Sensor and Energy Materials Pub Date : 2024-03-21 DOI: 10.1016/j.asems.2024.100099
{"title":"Editorial for special issue: Electrochemical sensing and imaging","authors":"","doi":"10.1016/j.asems.2024.100099","DOIUrl":"10.1016/j.asems.2024.100099","url":null,"abstract":"","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"3 3","pages":"Article 100099"},"PeriodicalIF":0.0,"publicationDate":"2024-03-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773045X24000104/pdfft?md5=6295c498bc908c19532df6942037e748&pid=1-s2.0-S2773045X24000104-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140268220","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Coating tetrahedral DNA framework with endosomolytic peptides for improved stability and cytosolic delivery 在四面体 DNA 框架上涂覆内溶酶体肽,提高稳定性和细胞输送能力
Advanced Sensor and Energy Materials Pub Date : 2024-03-05 DOI: 10.1016/j.asems.2024.100098
Jinjun He , Xiang Ji , Zihui Xu , Wei He , Yan Zhao , Lele Sun , Lan Ma
{"title":"Coating tetrahedral DNA framework with endosomolytic peptides for improved stability and cytosolic delivery","authors":"Jinjun He ,&nbsp;Xiang Ji ,&nbsp;Zihui Xu ,&nbsp;Wei He ,&nbsp;Yan Zhao ,&nbsp;Lele Sun ,&nbsp;Lan Ma","doi":"10.1016/j.asems.2024.100098","DOIUrl":"10.1016/j.asems.2024.100098","url":null,"abstract":"<div><p>DNA nanostructures have emerged as promising carriers for drug delivery. However, challenges such as low stability, poor cellular uptake efficiency, and vulnerability to lysosomal degradation still hinder their therapeutic potential. In this study, we demonstrate the coating of tetrahedral DNA frameworks (TDF) with the endosomolytic peptide L17E through electrostatic interactions to address these issues. Our findings highlight that L17E coating substantially enhances the stability of TDFs and improves their uptake efficiency into RAW264.7 cells through endocytosis and macropinocytosis. Moreover, L17E coating enables efficient endosomal release of TDFs. Finally, we employed L17E-coated TDF to deliver osteogenic growth peptide and demonstrated its potential applications in inhibiting periodontitis both in vitro and in vivo. This straightforward and cost-effective strategy holds promise for advancing the biomedical applications of DNA nanostructures.</p></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"3 2","pages":"Article 100098"},"PeriodicalIF":0.0,"publicationDate":"2024-03-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773045X24000098/pdfft?md5=663ff88ef1140bb1f77c4c3c37915cd5&pid=1-s2.0-S2773045X24000098-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140091702","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Nanofibers enabled advanced gas sensors: A review 纳米纤维实现了先进的气体传感器:综述
Advanced Sensor and Energy Materials Pub Date : 2024-02-24 DOI: 10.1016/j.asems.2024.100093
Kening Lang , Tianyi Liu , Daniel J. Padilla , Marriana Nelson , Christopher W. Landorf , Rishi J. Patel , Mark L. Ballentine , Alan J. Kennedy , Wu-Sheng Shih , Adam Scotch , Jiadeng Zhu
{"title":"Nanofibers enabled advanced gas sensors: A review","authors":"Kening Lang ,&nbsp;Tianyi Liu ,&nbsp;Daniel J. Padilla ,&nbsp;Marriana Nelson ,&nbsp;Christopher W. Landorf ,&nbsp;Rishi J. Patel ,&nbsp;Mark L. Ballentine ,&nbsp;Alan J. Kennedy ,&nbsp;Wu-Sheng Shih ,&nbsp;Adam Scotch ,&nbsp;Jiadeng Zhu","doi":"10.1016/j.asems.2024.100093","DOIUrl":"https://doi.org/10.1016/j.asems.2024.100093","url":null,"abstract":"<div><p>The advancement of gas sensor technology over the past decades has led to remarkable progress and achievements in pollution control and environmental protection. Compared with other sensing materials, electrospun nanofibers have attracted significant attention, which is mainly due to their unique characteristics, including but not limited to high surface area, easy structure design, facile facility setup, multifunctional properties, etc., making them outstanding candidates for potential applications in this field. This review provides an overview of the applications of electrospun nanofibers in gas sensors, concentrating on carbon monoxide, hydrogen, carbon dioxide, hydrogen sulfide, ammonia, nitrogen oxides, oxygen, and volatile organic compounds. It begins with a brief introduction to sensing materials and the advantages of electrospun nanofibers along with their ongoing research. The principles and progress of electrospinning are then discussed. Afterward, the corresponding properties of electrospun nanofibers in diverse gas sensors are thoroughly reviewed. Finally, a future vision regarding challenges and perspectives in this area is proposed. This review provides an extensive and comprehensive reference to utilize advanced electrospun nanofibers to generate novel sensors, facilitating their performance in high-demand areas.</p></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"3 2","pages":"Article 100093"},"PeriodicalIF":0.0,"publicationDate":"2024-02-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773045X24000049/pdfft?md5=9bc3dc0e18a0f9bbcdd72792c2abab1d&pid=1-s2.0-S2773045X24000049-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140052420","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Functionalized MXene fiber electrode for the electrochemical sensing of urinary ammonia 用于电化学检测尿氨的功能化 MXene 纤维电极
Advanced Sensor and Energy Materials Pub Date : 2024-02-02 DOI: 10.1016/j.asems.2024.100091
{"title":"Functionalized MXene fiber electrode for the electrochemical sensing of urinary ammonia","authors":"","doi":"10.1016/j.asems.2024.100091","DOIUrl":"10.1016/j.asems.2024.100091","url":null,"abstract":"<div><p>The development of technologically advanced fiber-based flexible microelectrodes has been of extensive research interest in healthcare systems because of their unique construction and synergistic effect on multifunctional properties. In this work, we constructed functional MXene fiber (MXF) by a simple and versatile wet spinning method, and then, a well-aligned ZIF-67 nanoarray was grown in situ on the surface. Using the chemical vapor deposition (CVD) method, carbon nanotubes (CNTs) were produced on MXF via the pyrolysis of ZIF-67 and melamine. Finally, Pt nanoparticles were electrodeposited on the CNTs forest, and a Pt@CNTs/MXF electrode was obtained. Owing to the plethora of surface active sites and the synergistic effects between MXene, CNTs, and Pt nanoparticles, the as-fabricated fiber electrode enabled the precise detection of ammonia under alkaline conditions via differential pulse voltammetry (DPV), which exhibited a linear range of 0.1 μM–10 mM and a detection limit of 73.2 nM. Due to their good performance in ammonia detection, Pt@CNTs/MXF electrodes could be adopted to determine the ammonia concentration in urine for clinical estimation, which provides a practical approach for the diagnosis of urinary ammonia-associated diseases.</p></div>","PeriodicalId":100036,"journal":{"name":"Advanced Sensor and Energy Materials","volume":"3 4","pages":"Article 100091"},"PeriodicalIF":0.0,"publicationDate":"2024-02-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773045X24000025/pdfft?md5=178ff2e2268690d230f9d5db61430805&pid=1-s2.0-S2773045X24000025-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139685771","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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