Atmospheric Measurement Techniques最新文献

{"title":"High-resolution wind speed measurements with quadcopter uncrewed aerial systems: calibration and verification in a wind tunnel with an active grid","authors":"Johannes Kistner, Lars Neuhaus, Norman Wildmann","doi":"10.5194/amt-17-4941-2024","DOIUrl":"https://doi.org/10.5194/amt-17-4941-2024","url":null,"abstract":"Abstract. As a contribution to closing observational gaps in the atmospheric boundary layer (ABL), the Simultaneous Wind measurement with Uncrewed Flight Systems in 3D (SWUF-3D) fleet of uncrewed aerial systems (UASs) is utilized for in situ measurements of turbulence. To date, the coefficients for the transformation terms used in our algorithm for deriving wind speeds from avionic data have only been determined via calibration flights in the free field. Therefore, we present in this work calibration and verification under laboratory conditions. The UAS measurements are performed in a wind tunnel equipped with an active grid and constant temperature anemometers (CTAs) as a reference. Calibration is performed in x- and y-coordinate directions of the UAS body frame at wind speeds of 2 … 18 m s−1. For systematic verification of the measurement capabilities and identification of limitations, different measurement scenarios like gusts, velocity steps, and turbulence are generated with the active grid. Furthermore, the measurement accuracy under different angles of sideslip (AoSs) and wind speeds is investigated, and we examined whether the calibration coefficients can be ported to other UASs in the fleet. Our analyses show that the uncertainty in measuring the wind speed depends on the wind speed magnitude and increases with extreme velocity changes and with higher wind speeds, resulting in a root-mean-square error (RMSE) of less than 0.2 m s−1 for steady wind speeds. Applying the calibration coefficients from one UAS to others within the fleet results in comparable accuracies. Flights in gusts of different strengths yield an RMSE of up to 0.6 m s−1. The maximal RMSE occurs in the most extreme velocity steps (i.e., a lower speed of 5 m s−1 and an amplitude of 10 m s−1) and exceeds 1.3 m s−1. For variances below approx. 0.5 and 0.3 m2 s−2, the maximal resolvable frequencies of the turbulence are about 2 and 1 Hz, respectively. The results indicate successful calibration but with susceptibility to high AoSs in high wind speeds, no necessity for wind tunnel calibration for individual UASs, and the need for further research regarding turbulence analysis.","PeriodicalId":8619,"journal":{"name":"Atmospheric Measurement Techniques","volume":"36 1","pages":""},"PeriodicalIF":3.8,"publicationDate":"2024-08-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198389","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Retrieving cloud base height and geometric thickness using the oxygen A-band channel of GCOM-C/SGLI","authors":"Takashi M. Nagao, Kentaroh Suzuki, Makoto Kuji","doi":"10.5194/amt-2024-141","DOIUrl":"https://doi.org/10.5194/amt-2024-141","url":null,"abstract":"<strong>Abstract.</strong> Measurements with a 763 nm channel, located within the oxygen A-band and equipped on the Second-generation Global Imager (SGLI) onboard the JAXA’s Global Change Observation Mission – Climate (GCOM-C) satellite, have the potential to retrieve cloud base height (CBH) and cloud geometric thickness (CGT) through passive remote sensing. This study implemented an algorithm to retrieve the CBH using the SGLI 763 nm channel in combination with several other SGLI channels in the visible, shortwave infrared, and thermal infrared regions. In addition to CBH, the algorithm can simultaneously retrieve other key cloud properties, including cloud optical thickness (COT), cloud effective radius, ice COT fraction as the cloud thermodynamic phase, cloud top height (CTH), and CGT. Moreover, the algorithm can be seamlessly applied to global clouds comprised of liquid, ice, and mixed phases. The SGLI-retrieved CBH exhibited quantitative consistency with CBH data obtained from the ground-based ceilometer network, ship-borne ceilometer, satellite-borne radar and lidar observations, as evidenced by sufficiently high correlations and small biases. These results provide practical evidence that the retrieval of CBH is indeed possible using the SGLI 763 nm channel. Moreover, the results lend credence to the future use of SGLI CBH data, including the estimation of the surface downward longwave radiative flux from clouds. Nevertheless, issues remain that must be addressed to enhance the value of SGLI-derived cloud retrieval products. These include the systematic bias of SGLI CTH related to cirrus clouds and the bias of SGLI CBH caused by multi-layer clouds.","PeriodicalId":8619,"journal":{"name":"Atmospheric Measurement Techniques","volume":"43 1","pages":""},"PeriodicalIF":3.8,"publicationDate":"2024-08-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198390","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"ampycloud: an open-source algorithm to determine cloud base heights and sky coverage fractions from ceilometer data","authors":"Frédéric P. A. Vogt, Loris Foresti, Daniel Regenass, Sophie Réthoré, Néstor Tarin Burriel, Mervyn Bibby, Przemysław Juda, Simone Balmelli, Tobias Hanselmann, Pieter du Preez, Dirk Furrer","doi":"10.5194/amt-17-4891-2024","DOIUrl":"https://doi.org/10.5194/amt-17-4891-2024","url":null,"abstract":"Abstract. Ceilometers are used routinely at aerodromes worldwide to derive the height and sky coverage fraction of cloud layers. This information, possibly combined with direct observations by human observers, contributes to the production of meteorological aerodrome reports (METARs). Here, we present ampycloud, a new algorithm, and its associated Python package for automatic processing of ceilometer data with the aim of determining the sky coverage fraction and base height of cloud layers above aerodromes. The ampycloud algorithm was developed at the Swiss Federal Office of Meteorology and Climatology (MeteoSwiss) as part of the AMAROC (AutoMETAR/AutoReport rOund the Clock) program to help in the fully automatic production of METARs at Swiss civil aerodromes. ampycloud is designed to work with no direct human supervision. The algorithm consists of three distinct, sequential steps that rely on agglomerative clustering methods and Gaussian mixture models to identify distinct cloud layers from individual cloud base hits reported by ceilometers. The robustness of the ampycloud algorithm stems from the first processing step, which is simple and reliable. It constrains the two subsequent processing steps that are more sensitive but also better suited to handling complex cloud distributions. The software implementation of the ampycloud algorithm takes the form of an eponymous, pip-installable Python package developed on GitHub and made publicly accessible.","PeriodicalId":8619,"journal":{"name":"Atmospheric Measurement Techniques","volume":"47 1","pages":""},"PeriodicalIF":3.8,"publicationDate":"2024-08-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142225284","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system","authors":"Tianle Pan, Andrew T. Lambe, Weiwei Hu, Yicong He, Minghao Hu, Huaishan Zhou, Xinming Wang, Qingqing Hu, Hui Chen, Yue Zhao, Yuanlong Huang, Doug R. Worsnop, Zhe Peng, Melissa A. Morris, Douglas A. Day, Pedro Campuzano-Jost, Jose-Luis Jimenez, Shantanu H. Jathar","doi":"10.5194/amt-17-4915-2024","DOIUrl":"https://doi.org/10.5194/amt-17-4915-2024","url":null,"abstract":"Abstract. Oxidation flow reactors (OFRs) have been extensively utilized to examine the formation of secondary organic aerosol (SOA). However, the UV lamps typically employed to initiate the photochemistry in OFRs can result in an elevated reactor temperature when their implications are not thoroughly evaluated. In this study, we conducted a comprehensive investigation into the temperature distribution within an Aerodyne potential aerosol mass OFR (PAM-OFR) and then examined the subsequent effects on flow and chemistry due to lamp heating. A lamp-induced temperature increase was observed, which was a function of lamp-driving voltage, number of lamps, lamp types, OFR residence time, and positions within the PAM-OFR. Under typical PAM-OFR operational conditions (e.g., < 5 d of equivalent atmospheric OH exposure under low-NOx conditions), the temperature increase typically ranged from 1–5 °C. Under extreme (but less frequently encountered) conditions, the heating could reach up to 15 °C. The influences of the increased temperature over ambient conditions on the flow distribution, gas, and condensed-phase chemistry within PAM-OFR were evaluated. Our findings indicate that the increase in temperature altered the flow field, resulting in a diminished tail on the residence time distribution and corresponding oxidant exposure due to faster recirculation. According to simulation results from a radical chemistry box model, the variation in absolute oxidant concentration within PAM-OFR due to temperature increase was minimal (< 5 %). The temperature influences on seed organic aerosol (OA) and newly formed secondary OA were also investigated, suggesting that an increase in temperature can impact the yield, size, and oxidation levels of representative biogenic and anthropogenic SOA types. Recommendations for temperature-dependent SOA yield corrections and PAM-OFR operating protocols that mitigate lamp-induced temperature enhancement and fluctuations are presented. We recommend blowing air around the reactor's exterior with fans during PAM-OFR experiments to minimize the temperature increase within PAM-OFR. Temperature increases are substantially lower for OFRs utilizing less powerful lamps compared to the Aerodyne version.","PeriodicalId":8619,"journal":{"name":"Atmospheric Measurement Techniques","volume":"35 1","pages":""},"PeriodicalIF":3.8,"publicationDate":"2024-08-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198388","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Estimating hourly ground-level aerosols using GEMS aerosol optical depth: A machine learning approach","authors":"Sungmin O, Ji Won Yoon, Seon Ki Park","doi":"10.5194/amt-2024-142","DOIUrl":"https://doi.org/10.5194/amt-2024-142","url":null,"abstract":"<strong>Abstract.</strong> The Geostationary Environment Monitoring Spectrometer (GEMS) is the world's first ultraviolet–visible instrument for air quality monitoring in geostationary orbit. Since its launch in 2020, GEMS has provided hourly daytime air quality information over Asia. However, to date, validation and applications of these data are lacking. Here we evaluate the effectiveness of the first 1.5-year GEMS aerosol optical depth (AOD) data in estimating ground-level particulate matter (PM) concentrations at an hourly scale. To do so, we employ random forest models and use GEMS AOD data and meteorological variables as input features to estimate PM10 and PM2.5 concentrations, respectively, in South Korea. The model-estimated PM concentrations are strongly correlated with ground measurements, but they exhibit negative biases, particularly during high aerosol loading months. Our results indicate that GEMS AOD values represent underestimates compared to ground-measured AOD values, possibly leading to negative biases in the final PM estimates. Further, we demonstrate that more training data could significantly improve random forest model performance, thus indicating the potential of GEMS for high-resolution surface PM prediction when sufficient data are accumulated over the coming years. Our results will serve as a reference to aid the evaluation of future GEMS AOD retrieval algorithm improvements and also provide initial guidance for data users.","PeriodicalId":8619,"journal":{"name":"Atmospheric Measurement Techniques","volume":"69 1","pages":""},"PeriodicalIF":3.8,"publicationDate":"2024-08-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198391","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Direct calibration using atmospheric particles and performance evaluation of PSM 2.0 for sub-10 nm particle measurements","authors":"Yiliang Liu, Arttu Yli-Kujala, Fabian Schmidt-Ott, Sebastian Holm, Lauri Ahonen, Tommy Chan, Joonas Enroth, Joonas Vanhanen, Runlong Cai, Tuukka Petäjä, Markku Kulmala, Yang Chen, Juha Kangasluoma","doi":"10.5194/egusphere-2024-2603","DOIUrl":"https://doi.org/10.5194/egusphere-2024-2603","url":null,"abstract":"<strong>Abstract.</strong> Particle Size Magnifier is widely used for the measuring nano-sized particles. Here we calibrated the newly developed Particle Size Magnifier version 2.0 (PSM 2.0). 1–10 nm particles with different compositions were used, including metal particles, organic particles generated in the laboratory and atmospheric particles collected in Helsinki and Hyytiälä, respectively. Noticeable difference among the calibration curves was observed. Atmospheric particles from Hyytiälä required higher DEG supersaturation to be activated compared to metal particles (standard calibration particles) and other types of particles. This suggests that chemical composition differences introduce measurement uncertainties and highlight the importance of in-situ calibration. The size resolution of PSM 2.0 was characterized using metal particles. The maximum size resolution was observed at 2–3 nm. PSM 2.0 was then operated in Hyytiälä in parallel with a Half-mini Differential Mobility Particle Sizer (DMPS). During new particle formation (NPF) events, comparable total particle concentrations were observed between Half-mini DMPS and PSM 2.0 based on Hyytiälä atmospheric particle calibration. Meanwhile, applying the calibration with metal particles to atmospheric measurements would cause an overestimation of 3–10 nm particles. In terms of the particle size distributions, similar patterns were observed between DMPS and PSM when using the calibration of Hyytiälä atmospheric particles. In summary, PSM 2.0 is a powerful instrument for measuring sub-10 nm particles and can achieve more precise particle size distribution measurements with proper calibration.","PeriodicalId":8619,"journal":{"name":"Atmospheric Measurement Techniques","volume":"13 1","pages":""},"PeriodicalIF":3.8,"publicationDate":"2024-08-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142225254","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Tracking Traveling Ionospheric Disturbances through Doppler-shifted AM radio transmissions","authors":"Claire Trop, James LaBelle, Philip Erickson, Shun-Rong Zhang, David McGaw, Terrence Kovacs","doi":"10.5194/egusphere-2024-2383","DOIUrl":"https://doi.org/10.5194/egusphere-2024-2383","url":null,"abstract":"<strong>Abstract.</strong> Six specialized radio receivers were developed to measure the Doppler shift of amplitude modulation (AM) broadcast radio carrier signals due to ionospheric effects. Five were deployed approximately on a circle at a one-hop distance from an 810-kHz clear-channel AM transmitter in Schenectady, New York, and the sixth was located close to the transmitter, providing a reference recording. Clear-channel AM signals from New York City and Connecticut were also received. The experiment confirmed detection of travelling ionospheric disturbances (TIDs) and measurement of their horizontal phase velocities through monitoring variations of the Doppler shift of reflected AM signals imparted by vertical motions of the ionosphere. Comparison of thirteen events with simultaneous global navigation satellite system (GNSS) based TID measurements showed generally good agreement between the two techniques, with differences attributable to differing sensitivities of the techniques to wave altitude and characteristics within a complex wave environment. Detected TIDs had mostly southward phase velocities, and in 4 cases they were associated with auroral disturbances that could plausibly be their sources. A purely automated software technique for event detection and phase velocity measurement was developed and applied to one year of data, revealing that AM Doppler sounding is much more effective when using transmitter signals in the upper part of the AM band (above 1 MHz) and demonstrating that the AM Doppler technique has promise to scale to large numbers of receivers covering continent-wide spatial scales.","PeriodicalId":8619,"journal":{"name":"Atmospheric Measurement Techniques","volume":"27 1","pages":""},"PeriodicalIF":3.8,"publicationDate":"2024-08-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142225255","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"High-altitude balloon-launched uncrewed aircraft system measurements of atmospheric turbulence and qualitative comparison with infrasound microphone response","authors":"Anisa N. Haghighi, Ryan D. Nolin, Gary D. Pundsack, Nick Craine, Aliaksei Stratsilatau, Sean C. C. Bailey","doi":"10.5194/amt-17-4863-2024","DOIUrl":"https://doi.org/10.5194/amt-17-4863-2024","url":null,"abstract":"Abstract. This study investigates the use of a balloon-launched uncrewed aircraft system (UAS) for the measurement of turbulence in the troposphere and lower stratosphere. The UAS was a glider which could conduct an automated descent following a designated flight trajectory and was equipped with in situ sensors for measuring thermodynamic and kinematic atmospheric properties. In addition, this aircraft was equipped with an infrasonic microphone to assess its suitability for the remote detection of clear-air turbulence. The capabilities of the UAS and sensing systems were tested during three flights conducted in New Mexico, USA, in 2021. It was found that the profiles of temperature, humidity, and horizontal winds measured during descent were in broad agreement with those made by radiosonde data published by the US National Weather Service, separated by up to 380 km spatially and by 3 to 5 h temporally. Winds measured during controlled flight descent were consistent with the winds measured by global-positioning-system-derived velocity during balloon ascent. During controlled descent with this particular payload, a nominal vertical resolution on the order of 1 m was achieved for temperature, relative humidity, and pressure with a nominal vertical resolution of the wind velocity vector on the order of 0.1 m; the aircraft had a glide slope angle from 1 to 4° during this time. Analysis approaches were developed that provided turbulent kinetic energy and dissipation rate, but it was found that the corresponding Richardson number was sensitive to the methodology used to determine the vertical gradients from a single flight. The low-frequency content of the infrasonic microphone signal was observed to qualitatively align with long-wavelength wind velocity fluctuations detected at high altitude. Moreover, the microphone measured more broadband frequency content when the aircraft approached turbulence produced by the boundary layer.","PeriodicalId":8619,"journal":{"name":"Atmospheric Measurement Techniques","volume":"11 1","pages":""},"PeriodicalIF":3.8,"publicationDate":"2024-08-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142225253","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Atmospheric H2 observations from the NOAA Cooperative Global Air Sampling Network","authors":"Gabrielle Pétron, Andrew M. Crotwell, John Mund, Molly Crotwell, Thomas Mefford, Kirk Thoning, Bradley Hall, Duane Kitzis, Monica Madronich, Eric Moglia, Donald Neff, Sonja Wolter, Armin Jordan, Paul Krummel, Ray Langenfelds, John Patterson","doi":"10.5194/amt-17-4803-2024","DOIUrl":"https://doi.org/10.5194/amt-17-4803-2024","url":null,"abstract":"Abstract. The NOAA Global Monitoring Laboratory (GML) measures atmospheric hydrogen (H2) in grab samples collected weekly as flask pairs at over 50 sites in the Cooperative Global Air Sampling Network. Measurements representative of background air sampling show higher H2 in recent years at all latitudes. The marine boundary layer (MBL) global mean H2 was 552.8 ppb in 2021, 20.2 ± 0.2 ppb higher compared to 2010. A 10 ppb or more increase over the 2010–2021 average annual cycle was detected in 2016 for MBL zonal means in the tropics and in the Southern Hemisphere. Carbon monoxide measurements in the same-air samples suggest large biomass burning events in different regions likely contributed to the observed interannual variability at different latitudes. The NOAA H2 measurements from 2009 to 2021 are now based on the World Meteorological Organization Global Atmospheric Watch (WMO GAW) H2 mole fraction calibration scale, developed and maintained by the Max Planck Institute for Biogeochemistry (MPI-BGC), Jena, Germany. GML maintains eight H2 primary calibration standards to propagate the WMO scale. These are gravimetric hydrogen-in-air mixtures in electropolished stainless steel cylinders (Essex Industries, St. Louis, MO), which are stable for H2. These mixtures were calibrated at the MPI-BGC, the WMO Central Calibration Laboratory (CCL) for H2, in late 2020 and span the range 250–700 ppb. We have used the CCL assignments to propagate the WMO H2 calibration scale to NOAA air measurements performed using gas chromatography and helium pulse discharge detector instruments since 2009. To propagate the scale, NOAA uses a hierarchy of secondary and tertiary standards, which consist of high-pressure whole-air mixtures in aluminum cylinders, calibrated against the primary and secondary standards, respectively. Hydrogen at the parts per billion level has a tendency to increase in aluminum cylinders over time. We fit the calibration histories of these standards with zero-, first-, or second-order polynomial functions of time and use the time-dependent mole fraction assignments on the WMO scale to reprocess all tank air and flask air H2 measurement records. The robustness of the scale propagation over multiple years is evaluated with the regular analysis of target air cylinders and with long-term same-air measurement comparison efforts with WMO GAW partner laboratories. Long-term calibrated, globally distributed, and freely accessible measurements of H2 and other gases and isotopes continue to be essential to track and interpret regional and global changes in the atmosphere composition. The adoption of the WMO H2 calibration scale and subsequent reprocessing of NOAA atmospheric data constitute a significant improvement in the NOAA H2 measurement records.","PeriodicalId":8619,"journal":{"name":"Atmospheric Measurement Techniques","volume":"69 1","pages":""},"PeriodicalIF":3.8,"publicationDate":"2024-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198392","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Partition between supercooled liquid droplets and ice crystals in mixed-phase clouds based on airborne in situ observations","authors":"Flor Vanessa Maciel, Minghui Diao, Ching An Yang","doi":"10.5194/amt-17-4843-2024","DOIUrl":"https://doi.org/10.5194/amt-17-4843-2024","url":null,"abstract":"Abstract. The onset of ice nucleation in mixed-phase clouds determines the lifetime and microphysical properties of ice clouds. In this work, we develop a novel method that differentiates between various phases of mixed-phase clouds, such as clouds dominated by pure liquid or pure ice segments, compared with those having ice crystals surrounded by supercooled liquid water droplets or vice versa. Using this method, we examine the relationship between the macrophysical and microphysical properties of Southern Ocean mixed-phase clouds at −40 to 0 °C (e.g. stratiform and cumuliform clouds) based on the in situ aircraft-based observations during the US National Science Foundation Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) flight campaign. The results show that the exchange between supercooled liquid water and ice crystals from a macrophysical perspective, represented by the increasing spatial ratio of regions containing ice crystals relative to the total in-cloud region (defined as ice spatial ratio), is positively correlated with the phase exchange from a microphysical perspective, represented by the increasing ice water content (IWC), decreasing liquid water content (LWC), increasing ice mass fraction, and increasing ice particle number fraction (IPNF). The mass exchange between liquid and ice becomes more significant during phase 3 when pure ice cloud regions (ICRs) start to appear. Occurrence frequencies of cloud thermodynamic phases show a significant phase change from liquid to ice at a similar temperature (i.e. −17.5 °C) among three types of definitions of mixed-phase clouds based on ice spatial ratio, ice mass fraction, or IPNF. Aerosol indirect effects are quantified for different phases using number concentrations of aerosols greater than 100 or 500 nm (N&gt;100 and N&gt;500, respectively). N&gt;500 shows stronger positive correlations with ice spatial ratios compared with N&gt;100. This result indicates that larger aerosols potentially contain ice-nucleating particles (INPs), which facilitate the formation of ice crystals in mixed-phase clouds. The impact of N&gt;500 is also more significant in phase 2 when ice crystals just start to appear in the mixed phase compared with phase 3 when pure ICRs have formed, possibly due to the competing aerosol indirect effects on primary and secondary ice production in phase 3. The thermodynamic and dynamic conditions are quantified for each phase. The results show stronger in-cloud turbulence and higher updraughts in phases 2 and 3 when liquid and ice coexist compared with pure liquid or ice (phases 1 and 4, respectively). The highest updraughts and turbulence are seen in phase 3 when supercooled liquid droplets are surrounded by ice crystals. These results indicate both updraughts and turbulence support the maintenance of supercooled liquid water amongst ice crystals. Overall, these results illustrate the varying effects of aerosols, thermodynamics, and dynamics through various s","PeriodicalId":8619,"journal":{"name":"Atmospheric Measurement Techniques","volume":"5 1","pages":""},"PeriodicalIF":3.8,"publicationDate":"2024-08-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142198424","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}