T. Elkeles, P. García-Sánchez, Wu Yue, A. Ramos, G. Yossifon
{"title":"Dielectrophoretic Force Equilibrium of Complex Particles","authors":"T. Elkeles, P. García-Sánchez, Wu Yue, A. Ramos, G. Yossifon","doi":"10.1103/PHYSREVAPPLIED.14.054047","DOIUrl":"https://doi.org/10.1103/PHYSREVAPPLIED.14.054047","url":null,"abstract":"In contrast to the commonly used spherical Janus particles, here we used engineered Janus particles that are fabricated using photolithography technique for precise control over their geometry and coated regions. Specifically, we studied a lollipop-shaped complex particle where its head is coated with gold while its tail is left bare. Due to their distinct electrical properties (i.e. electrical polarizability) the particle exhibits force equilibrium where opposite dielectrophoretic forces acting on its head and tail exactly cancel each other to yield a stable equilibrium position. This was realized in a quadrupolar electrode array where the equilibrium position of the engineered particle could be tuned by the frequency. This stands in contrast to the standard dielectrophoretic behavior where the particle shifts positions from either the center of the quad to the very edge of the electrodes when shifting from a negative to positive dielectrophoretic response, respectively. This opens new opportunities for positioning control of such complex particles for self-assembly, biosensing, biomimetic spermatozoa and more.","PeriodicalId":8472,"journal":{"name":"arXiv: Soft Condensed Matter","volume":"1 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-07-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"89798418","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Microphase separation in active filament systems maintained by cyclic dynamics of cluster size and order","authors":"L. Huber, T. Krüger, Erwin Frey","doi":"10.1103/PHYSREVRESEARCH.3.013280","DOIUrl":"https://doi.org/10.1103/PHYSREVRESEARCH.3.013280","url":null,"abstract":"The onset of polar flocking in active matter is discontinuous, akin to gas-liquid phase transitions, except that the steady state exhibits microphase separation into polar clusters. While these features have been observed in theoretical models and experiments, little is known about the underlying mesoscopic processes at the cluster level. Here we show that emergence and maintenance of polar order are governed by the interplay between the assembly and disassembly dynamics of clusters with varying size and degree of polar order. Using agent-based simulations of propelled filaments in a parameter regime relevant for actomyosin motility assays, we monitor the temporal evolution of cluster statistics and the transport processes of filaments between clusters. We find that, over a broad parameter range, the emergence of order is determined by nucleation and growth of polar clusters, where the nucleation threshold depends not only on the cluster size but also on its polar moment. Growth involves cluster self-replication, and polar order is established by cluster growth and fragmentation. Maintenance of the microphase-separated, polar-ordered state results from a cyclic dynamics in cluster size and order, driven by an interplay between cluster nucleation, coagulation, fragmentation and evaporation of single filaments. These findings are corroborated by a kinetic model for the cluster dynamics that includes these elementary cluster-level processes. It consistently reproduces the cluster statistics as well as the cyclic turnover from disordered to ordered clusters and back. Such cyclic kinetic processes could represent a general mechanism for the maintenance of order in active matter systems.","PeriodicalId":8472,"journal":{"name":"arXiv: Soft Condensed Matter","volume":"120 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"86136235","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
L. Jing, J. Ottino, Richard M. Lueptow, P. Umbanhowar
{"title":"Rising and sinking intruders in dense granular flows","authors":"L. Jing, J. Ottino, Richard M. Lueptow, P. Umbanhowar","doi":"10.1103/PHYSREVRESEARCH.2.022069","DOIUrl":"https://doi.org/10.1103/PHYSREVRESEARCH.2.022069","url":null,"abstract":"We computationally determine the force on single spherical intruder particles in sheared granular flows as a function of particle size, particle density, shear rate, overburden pressure, and gravitational acceleration. The force scales similarly to, but deviates from, the buoyancy force predicted by Archimedes' principle. The deviation depends only on the intruder to bed particle size ratio, but not the density ratio or flow conditions. We propose a simple force model that successfully predicts whether intruders rise or sink, knowing only the size and density ratios, for a variety of flow configurations in physical experiments.","PeriodicalId":8472,"journal":{"name":"arXiv: Soft Condensed Matter","volume":"98 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-06-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"77611805","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
V. Sharma, H. Srinivasan, V. García Sakai, S. Mitra
{"title":"Caffeine modulates the dynamics of DODAB membranes: Role of the physical state of the bilayer","authors":"V. Sharma, H. Srinivasan, V. García Sakai, S. Mitra","doi":"10.1063/5.0027953","DOIUrl":"https://doi.org/10.1063/5.0027953","url":null,"abstract":"Caffeine (1,3,7-trimethylxanthine), an ingredient of coffee, is used worldwide as a psychostimulant, antioxidant, and adjuvant analgesic. To gain insights into the action mechanism of caffeine, we report on its effects on the phase behaviour and microscopic dynamics of a dioctadecyldimethylammonium bromide (DODAB) lipid membrane, as studied quasielastic neutron scattering (QENS). Tracking the elastic scattering intensity as a function of temperature showed that caffeine does not alter the phase behaviour of the DODAB membrane and that transition temperatures remain almost unaltered. However, QENS measurements revealed caffeine significantly modulates the microscopic dynamics of the lipids in the system, and that the effects depend on the structural arrangement of the lipids in the membrane. In the coagel phase, caffeine acts as a plasticizing agent which enhances the membrane dynamics. However, in the fluid phase the opposite effect is observed; caffeine behaves like a stiffening agent, restricting the lipid dynamics. Further analysis of the QENS data indicates that in the fluid phase, caffeine restricts both lateral and internal motions of the lipids in the membrane. The present study illustrates how caffeine regulates the fluidity of the membrane by modulating the dynamics of constituent lipids depending on the physical state of the bilayer.","PeriodicalId":8472,"journal":{"name":"arXiv: Soft Condensed Matter","volume":"75 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-06-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"87029652","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Confinement-induced demixing and crystallization","authors":"Gerhard Jung, Charlotte F. Petersen","doi":"10.1103/physrevresearch.2.033207","DOIUrl":"https://doi.org/10.1103/physrevresearch.2.033207","url":null,"abstract":"We simulate a strongly size-disperse hard-sphere fluid confined between two parallel, hard walls. We find that confinement induces crystallization into n-layered hexagonal lattices and a novel honeycomb-shaped structure, facilitated by fractionation. The onset of freezing prevents the formation of a stable glass phase and occurs at much smaller packing fraction than in bulk. Varying the wall separation triggers solid-to-solid transitions and a systematic change of the size-distribution of crystalline particles, which we rationalize using a semi-quantitative theory. We show that the crystallization can be exploited in a wedge geometry to demix particles of different sizes.","PeriodicalId":8472,"journal":{"name":"arXiv: Soft Condensed Matter","volume":"5 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-06-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"80366108","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Quantitatively consistent scale-spanning model for same-material tribocharging","authors":"G. Grosjean, S. Wald, J. Sobarzo, S. Waitukaitis","doi":"10.1103/physrevmaterials.4.082602","DOIUrl":"https://doi.org/10.1103/physrevmaterials.4.082602","url":null,"abstract":"By rigorously accounting for mesoscale spatial correlations in donor/acceptor surface properties, we develop a scale-spanning model for same-material tribocharging. We find that mesoscale correlations affect not only the magnitude of charge transfer but also the fluctuations-suppressing otherwise overwhelming charge-transfer variability that is not observed experimentally. We furthermore propose a generic theoretical mechanism by which the mesoscale features might emerge, which is qualitatively consistent with other proposals in the literature.","PeriodicalId":8472,"journal":{"name":"arXiv: Soft Condensed Matter","volume":"60 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-06-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"76212788","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
E. Mompó, M. A. López-Castaño, A. Lasanta, F. Vega Reyes, A. Torrente
{"title":"Memory effects in a gas of viscoelastic particles","authors":"E. Mompó, M. A. López-Castaño, A. Lasanta, F. Vega Reyes, A. Torrente","doi":"10.1063/5.0050804","DOIUrl":"https://doi.org/10.1063/5.0050804","url":null,"abstract":"We study a granular gas of viscoelastic particles, i.e, the kinetic energy loss upon collision, characteristic of granular materials, is a function of the particles relative velocities at impact. In order to characterize thermal memory in this system, we study the temperature relaxation curves when the granular gas is subject to sudden thermostat changes (the gas is heated homogeneously by means of a white noise). Results show that the system may display anomalous cooling and heating velocities at early times. In particular, a significant Mpemba effect is present; i.e., an initially hotter/cooler granular gas can cool down/heat up faster than an in comparison cooler/hotter granular gas. Moreover, a non-monotonic relaxation of the granular temperature can also be observed (also known as Kovacs effect) when the granular gas undergoes a certain protocol that sets it at a temperature equal to its long-time value. We study our system via three independent methods: theoretical solution, molecular dynamics simulations and exact numerical solution of the kinetic equation (obtained by means of the Direct Monte Carlo simulation method). We find a good agreement between all three methods.","PeriodicalId":8472,"journal":{"name":"arXiv: Soft Condensed Matter","volume":"25 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-05-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"85523357","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Eduardo Vitral, S. Mukherjee, P. Leo, J. Viñals, M. Paul, Zhi-Feng Huang
{"title":"Spiral defect chaos in Rayleigh-Bénard convection: Asymptotic and numerical studies of azimuthal flows induced by rotating spirals","authors":"Eduardo Vitral, S. Mukherjee, P. Leo, J. Viñals, M. Paul, Zhi-Feng Huang","doi":"10.1103/physrevfluids.5.093501","DOIUrl":"https://doi.org/10.1103/physrevfluids.5.093501","url":null,"abstract":"Rotating spiral patterns in Rayleigh-Benard convection are known to induce azimuthal flows, which raises the question of how different neighboring spirals interact with each other in spiral chaos, and the role of hydrodynamics in this regime. Far from the core, we show that spiral rotations lead to an azimuthal body force that is irrotational and of magnitude proportional to the topological index of the spiral and its angular frequency. The force, although irrotational, cannot be included in the pressure field as it would lead to a nonphysical, multivalued pressure. We calculate the asymptotic dependence of the resulting flow, and show that it leads to a logarithmic dependence of the azimuthal velocity on distance r away from the spiral core in the limit of negligible damping coefficient. This solution dampens to approximately $1/r$ when accounting for no-slip boundary conditions for the convection cell's plate. This flow component can provide additional hydrodynamic interactions among spirals including those observed in spiral defect chaos. We show that the analytic prediction for the azimuthal velocity agrees with numerical results obtained from both two-dimensional generalized Swift-Hohenberg and three-dimensional Boussinesq models, and find that the velocity field is affected by the size and charges of neighboring spirals. Numerically, we identify a correlation between the appearance of spiral defect chaos and the balancing between the mean-flow advection and the diffusive dynamics related to roll unwinding.","PeriodicalId":8472,"journal":{"name":"arXiv: Soft Condensed Matter","volume":"11 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-05-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"88634324","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"How does the presence of stevia glycosides impact surface bubbles stability?","authors":"Jonas Miguet, Yuan Fang, F. Rouyer, E. Rio","doi":"10.1016/j.colsurfa.2020.125093","DOIUrl":"https://doi.org/10.1016/j.colsurfa.2020.125093","url":null,"abstract":"","PeriodicalId":8472,"journal":{"name":"arXiv: Soft Condensed Matter","volume":"12 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-05-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"87716346","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
M. Leoni, M. Paoluzzi, Sarah Eldeen, A. Estrada, Lauren Nguyen, M. Alexandrescu, Karin Sherb, W. Ahmed
{"title":"Surfing and crawling macroscopic active particles under strong confinement: Inertial dynamics","authors":"M. Leoni, M. Paoluzzi, Sarah Eldeen, A. Estrada, Lauren Nguyen, M. Alexandrescu, Karin Sherb, W. Ahmed","doi":"10.1103/physrevresearch.2.043299","DOIUrl":"https://doi.org/10.1103/physrevresearch.2.043299","url":null,"abstract":"We study two types of active (self-propelled) macroscopic particles under confinement: camphor surfers and hexbug crawlers, using a combined experimental, theoretical, and numerical approach. Unlike widely studied microscopic active particles and swimmers, where thermal forces are often important and inertia is negligible, our macroscopic particles exhibit complex dynamics due expressly to active non-thermal noise combined with inertial effects. Hard confinement induces accumulation at a finite distance within the boundary and gives rise to three distinguishable dynamical states; both depending on activity and inertia. These surprisingly complex dynamics arise already at the single particle level -- highlighting the importance of inertia in macroscopic active matter.","PeriodicalId":8472,"journal":{"name":"arXiv: Soft Condensed Matter","volume":"26 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-05-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"74518373","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}