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Russian Journal of Physical Chemistry A最新文献

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Remote Ignition of an Open Gas Well Fountain Using Laser Radiation 利用激光辐射远程点燃露天气井喷泉
IF 0.7 4区 化学
Russian Journal of Physical Chemistry A Pub Date : 2024-11-18 DOI: 10.1134/S0036024424702200
S. V. Gvozdev, V. Yu. Dubrovsky, A. G. Krasyukov, R. E. Romanov, D. D. Metlyaev, A. Yu. Lysikov, V. K. Rerikh, G. V. Smirnov, M. D. Taran
{"title":"Remote Ignition of an Open Gas Well Fountain Using Laser Radiation","authors":"S. V. Gvozdev,&nbsp;V. Yu. Dubrovsky,&nbsp;A. G. Krasyukov,&nbsp;R. E. Romanov,&nbsp;D. D. Metlyaev,&nbsp;A. Yu. Lysikov,&nbsp;V. K. Rerikh,&nbsp;G. V. Smirnov,&nbsp;M. D. Taran","doi":"10.1134/S0036024424702200","DOIUrl":"10.1134/S0036024424702200","url":null,"abstract":"<p>A vertical methane fountain with sand particles of different sizes is simulated under laboratory conditions. The authors determine the intensity and duration of exposure to laser radiation with wavelength λ = 1.07 µm on sand particles needed for the stable ignition of an air–methane mixture. A cinematogram is presented of the ignition of a mixture on a laboratory model. The temperature of the gas mixture’s ignition, the time needed for radiation to heat particles to this temperature, and the maximum speeds of different particle sizes in the gas flow are estimated at ∼0.1 m<sup>3</sup>/s for laboratory conditions and ∼17 m<sup>3</sup>/s for a real emergency gas well. The angular velocity of the beam’s movement that is needed to keep particles with the highest speed in the zone of the beam while igniting the air–methane mixture is determined for a safe distance from the gas fountain. The main characteristics of a possible future laser complex capable of quickly solving the problem of remotely igniting a fountain of an emergency gas well are determined.</p>","PeriodicalId":767,"journal":{"name":"Russian Journal of Physical Chemistry A","volume":"98 12","pages":"2905 - 2907"},"PeriodicalIF":0.7,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142672370","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Platinum–Chromium–Nickel Catalysts of Bicyclohexyl Dehydrogenation, Supported on Oxidized Sibunit Carbon 以氧化锡本碳为载体的双环己基脱氢铂-铬-镍催化剂
IF 0.7 4区 化学
Russian Journal of Physical Chemistry A Pub Date : 2024-11-18 DOI: 10.1134/S0036024424701942
A. N. Kalenchuk, V. I. Bogdan, L. M. Kustov, Teng Hev
{"title":"Platinum–Chromium–Nickel Catalysts of Bicyclohexyl Dehydrogenation, Supported on Oxidized Sibunit Carbon","authors":"A. N. Kalenchuk,&nbsp;V. I. Bogdan,&nbsp;L. M. Kustov,&nbsp;Teng Hev","doi":"10.1134/S0036024424701942","DOIUrl":"10.1134/S0036024424701942","url":null,"abstract":"<p>Bicyclohexyl dehydrogenation using PtCrNi-containing catalysts supported on oxidized Sibunit carbon is studied as a key stage of hydrogen storage and evolution systems using liquid organic hydrogen carriers. It is shown that modifying platinum with nickel and chromium raises the specific activity of the catalyst considerably, relative to the evolution of hydrogen at a low content of the noble metal (0.1 wt % Pt). It is found that using an oxidized Sibunit carbon support to synthesize active supported Pt catalysts for bicyclohexyl dehydrogenation does not produce products of side reactions.</p>","PeriodicalId":767,"journal":{"name":"Russian Journal of Physical Chemistry A","volume":"98 12","pages":"2723 - 2726"},"PeriodicalIF":0.7,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142672434","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Enthalpy of Formation of Mixed Nickel(II) Complexes with L-Histidine and Oliglycines L 组氨酸和低聚甘氨酸混合镍（II）络合物的形成焓
IF 0.7 4区 化学
Russian Journal of Physical Chemistry A Pub Date : 2024-11-18 DOI: 10.1134/S0036024424701966
G. G. Gorboletova, S. A. Bychkova
{"title":"Enthalpy of Formation of Mixed Nickel(II) Complexes with L-Histidine and Oliglycines","authors":"G. G. Gorboletova,&nbsp;S. A. Bychkova","doi":"10.1134/S0036024424701966","DOIUrl":"10.1134/S0036024424701966","url":null,"abstract":"<p>Potentiometry and calorimetry are used to study the Ni<sup>2+</sup>–diglycine–L-histidine system in an aqueous solution at <i>T</i> = 298.15 K (KNO<sub>3</sub>). The composition and stability of the mixed ligand complex Ni(GG)(His) are defined with potentiometric measurements. The study is performed at ratios Ni : (GG + His) = 1 : 4 and 1 : 6. The concentrations of diglycine and L-histidine are in ratios of 3 : 1 and 5 : 1. The values of <span>(log beta )</span> obtained at different ratios of diglycine and L-histidine agree well with one another. Thermal effects are measured in the ampoule of a mixing calorimeter with an isothermal shell, a thermistor temperature sensor, and automatic recording of the temperature/time curve. The thermal effects of mixing solutions of Ni(NO<sub>3</sub>)<sub>2</sub>, diglycine, and L-histidine in the ratio <span>(c_{{{text{Ni}}}}^{0})</span> : <span>(c_{{{text{GG}}}}^{0})</span> : <span>(c_{{{text{His}}}}^{0})</span> = 1 : 3 : 1 are measured to determine the enthalpy of formation of a Ni(GG)(His) particle. The experiments are performed at ionic strengths of 0.2, 0.5, and 1.0 (mol/L). The standard thermodynamic characteristics (Δ<sub>r</sub><i>H</i>°, Δ<sub>r</sub><i>G</i>°, Δ<sub>r</sub><i>S</i>°) of the formation of a mixed-ligand complex are determined. A comparative analysis of the obtained data is performed using thermodynamic characteristics of mixed-ligand complexation in the Ni<sup>2+</sup>–glycine–L-histidine and Ni<sup>2+</sup>–triglycine–L-histidine studied earlier. Structures of forming complexes are proposed.</p>","PeriodicalId":767,"journal":{"name":"Russian Journal of Physical Chemistry A","volume":"98 12","pages":"2735 - 2740"},"PeriodicalIF":0.7,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142672534","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Studying Intermolecular Interactions in Binary Systems of Butyl Acetate-Dibutyl Phthalate and Butyl Acetate-Dioctyl Phthalate 研究乙酸丁酯-邻苯二甲酸二丁酯和乙酸丁酯-邻苯二甲酸二辛酯二元体系中的分子间相互作用
IF 0.7 4区 化学
Russian Journal of Physical Chemistry A Pub Date : 2024-11-18 DOI: 10.1134/S003602442470198X
D. I. Polevshchikov, V. V. Loskutov
{"title":"Studying Intermolecular Interactions in Binary Systems of Butyl Acetate-Dibutyl Phthalate and Butyl Acetate-Dioctyl Phthalate","authors":"D. I. Polevshchikov,&nbsp;V. V. Loskutov","doi":"10.1134/S003602442470198X","DOIUrl":"10.1134/S003602442470198X","url":null,"abstract":"<p>Studies of intermolecular interactions in butyl acetate-dibutyl phthalate and butyl acetate-dioctyl phthalate systems show that except for excess volume, deviations of properties from an ideal mixture are reduced as the temperature rises. Results indicate considerable van der Waals forces and confirm the effect the size of molecules has on the properties of binary mixtures. Experimental data on density, refractive index, viscosity, excess molar volume, and other properties are presented for systems and pure substances.</p>","PeriodicalId":767,"journal":{"name":"Russian Journal of Physical Chemistry A","volume":"98 12","pages":"2748 - 2756"},"PeriodicalIF":0.7,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142672537","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effect of Regimes of Processing Pulsed Flows of Plasma on the Corrosion Properties of Structural Steels 处理脉冲等离子体流的制度对结构钢腐蚀特性的影响
IF 0.7 4区 化学
Russian Journal of Physical Chemistry A Pub Date : 2024-11-18 DOI: 10.1134/S0036024424702212
A. K. Kutukov, A. V. Mironov, S. E. Panin, N. A. Danilina, V. V. Gaponova
{"title":"Effect of Regimes of Processing Pulsed Flows of Plasma on the Corrosion Properties of Structural Steels","authors":"A. K. Kutukov,&nbsp;A. V. Mironov,&nbsp;S. E. Panin,&nbsp;N. A. Danilina,&nbsp;V. V. Gaponova","doi":"10.1134/S0036024424702212","DOIUrl":"10.1134/S0036024424702212","url":null,"abstract":"<p>An investigation is performed of the effect the treatment of a pulsed plasma flow has on samples of two shapes (flat and cylindrical) made of structural steels (St45, 40Kh, 65G, ShKh15, 40KhN2MA). Processing is done under different conditions with varying parameters (pulse duration, capacitor bank charging voltage, and the type of working gas). Data show that after treatment, corrosion resistance increases for most of the considered grades of steel. The most effective processing parameters are established for each grade of steel.</p>","PeriodicalId":767,"journal":{"name":"Russian Journal of Physical Chemistry A","volume":"98 12","pages":"2908 - 2913"},"PeriodicalIF":0.7,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142672529","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Theoretical Investigation of the Properties of Magnetic W-Doped InSb Using TB-mBJ Approximation 使用 TB-mBJ 近似法对掺杂 W 的 InSb 的磁性能进行理论研究
IF 0.7 4区 化学
Russian Journal of Physical Chemistry A Pub Date : 2024-11-18 DOI: 10.1134/S0036024424702054
Drioua Mohamed, Badaoui Abdelhamid, Elkeurti Mohammed, Boudia Keltoum
{"title":"Theoretical Investigation of the Properties of Magnetic W-Doped InSb Using TB-mBJ Approximation","authors":"Drioua Mohamed,&nbsp;Badaoui Abdelhamid,&nbsp;Elkeurti Mohammed,&nbsp;Boudia Keltoum","doi":"10.1134/S0036024424702054","DOIUrl":"10.1134/S0036024424702054","url":null,"abstract":"<p>Our current study employs the spin-polarized density functional theory (DFT) using the all-electron full potential linear augmented plane-wave method (FP-LAPW) to examine the structural, electronic, and magnetic properties of InSb doped with Tungsten (In<span>(_{{1 - x}})</span>W<sub><i>x</i></sub>Sb with <i>x</i> = 0.125, 0.25) in the zinc blende crystal structure. We used, for the electronic exchange and correlation energy, the generalized gradient approximation (GGA) with the Wu-Cohen (WC) functional, improved with the Tran–Blaha modified Becke–Johnson (TB-mBJ) approach for the electronic properties. The obtained results show that this calculation method allows for reliable band gap values. The estimated structural properties match well with existing experimental results. The value of the total magnetic moment is around 3.00 µB for the investigated compounds, and because of their half-metallic ferromagnetic properties, they are regarded prospective candidates for spintronic applications.</p>","PeriodicalId":767,"journal":{"name":"Russian Journal of Physical Chemistry A","volume":"98 12","pages":"2810 - 2815"},"PeriodicalIF":0.7,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142672685","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Thermodynamics of the Sorption of Quinoline Derivatives, 1,2,3,4-Tetrahydroquinoline and Pyridazino[4,5-c]Quinoline Under Conditions of RP HPLC RP HPLC 条件下喹啉衍生物、1,2,3,4-四氢喹啉和哒嗪并[4,5-c]喹啉的吸附热力学
IF 0.7 4区 化学
Russian Journal of Physical Chemistry A Pub Date : 2024-11-18 DOI: 10.1134/S003602442470208X
A. V. Kapitonov, S. A. Ryzhkin, S. V. Kurbatova, M. N. Zemtsova
{"title":"Thermodynamics of the Sorption of Quinoline Derivatives, 1,2,3,4-Tetrahydroquinoline and Pyridazino[4,5-c]Quinoline Under Conditions of RP HPLC","authors":"A. V. Kapitonov,&nbsp;S. A. Ryzhkin,&nbsp;S. V. Kurbatova,&nbsp;M. N. Zemtsova","doi":"10.1134/S003602442470208X","DOIUrl":"10.1134/S003602442470208X","url":null,"abstract":"<p>The authors analyze temperature dependences of the retention of derivatives of quinoline, 1,2,3,4-tetrahydroquinoline, and pyridazino[4,5-c]quinoline under conditions of reversed-phase high-performance liquid chromatography on octadecyl silica gel. The thermodynamic characteristics of sorption of these compounds are calculated. The change in the enthalpies of sorption are found to depend on the content of acetonitrile in the water–acetonitrile eluent.</p>","PeriodicalId":767,"journal":{"name":"Russian Journal of Physical Chemistry A","volume":"98 12","pages":"2828 - 2837"},"PeriodicalIF":0.7,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142672467","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Experimental Modeling of Boron-10 Isotope Enrichment during Chemical Exchange in a Liquid–Liquid System 液-液系统化学交换过程中硼-10 同位素富集的实验模型
IF 0.7 4区 化学
Russian Journal of Physical Chemistry A Pub Date : 2024-11-18 DOI: 10.1134/S0036024424702182
P. I. Ivanov, A. V. Khoroshilov, N. S. Panyukova
{"title":"Experimental Modeling of Boron-10 Isotope Enrichment during Chemical Exchange in a Liquid–Liquid System","authors":"P. I. Ivanov,&nbsp;A. V. Khoroshilov,&nbsp;N. S. Panyukova","doi":"10.1134/S0036024424702182","DOIUrl":"10.1134/S0036024424702182","url":null,"abstract":"<p>The authors continue their set of studies on the separation of boron isotopes by means of chemical exchange in liquid–liquid systems using tri-<i>n</i>-octylamine as the main component of the organic phase. Degree of separation <i>K</i> = 1.0961 ± 0.0016 was obtained using experimental modeling of the operation of a rectangular cascade for separating boron isotopes in a 30-h long period of separation in the mode of product extraction. The obtained data are used to determine period τ = 19–21 h of concentration needed to reach a steady state when operating with product extraction at maximum degree of separation <i>K</i><sub>m</sub> = 1.109. The time needed to reach a steady state is τ = 130–160 h when operating in the mode without product extraction, which corresponds to maximum degree of separation <i>K</i><sub>m</sub> = 1.131.</p>","PeriodicalId":767,"journal":{"name":"Russian Journal of Physical Chemistry A","volume":"98 12","pages":"2891 - 2896"},"PeriodicalIF":0.7,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142672532","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Mechanism of the Cojoint Effect of Components of the Ni/HMOR/({text{SO}}_{4}^{{2 - }})–ZrO2 Catalytic System on the Hydroconversion of Aromatic Hydrocarbons Ni/HMOR/({text{SO}}_{4}^{{2 - }})-ZrO2 催化体系各组分对芳香烃加氢转化的协同效应机理
IF 0.7 4区 化学
Russian Journal of Physical Chemistry A Pub Date : 2024-11-18 DOI: 10.1134/S0036024424701930
S. I. Abasov, E. S. Isaeva, S. B. Agaeva, M. T. Mamedova, A. A. Iskenderova, A. A. Imanova
{"title":"Mechanism of the Cojoint Effect of Components of the Ni/HMOR/({text{SO}}_{4}^{{2 - }})–ZrO2 Catalytic System on the Hydroconversion of Aromatic Hydrocarbons","authors":"S. I. Abasov,&nbsp;E. S. Isaeva,&nbsp;S. B. Agaeva,&nbsp;M. T. Mamedova,&nbsp;A. A. Iskenderova,&nbsp;A. A. Imanova","doi":"10.1134/S0036024424701930","DOIUrl":"10.1134/S0036024424701930","url":null,"abstract":"<p>Composite catalyst (CC) Ni/HMOR/<span>({text{SO}}_{4}^{{2 - }})</span>–ZrO<sub>2</sub> is used to study the hydroconversion of benzene and toluene at atmospheric pressure, a temperature of 180°C, WHSV = 2 h<sup>−1</sup>, and Н<sub>2</sub>/ArH = 8. The conversion of benzene is as high as 58.2%. Adding an alkyl substituent raises conversion to 78.5%. It is shown that the primary conversion of toluene is similar to the conversion of benzene through selective aromatic ring hydrogenation with its subsequent isomerization, ring reduction, and hydrocleavage. Components of the catalytic system are inactive in the hydroconversion of aromatic hydrocarbons. Synergism emerges in the hydrogenating CC activity due to the cojoint effect which individual inactive <span>({text{SO}}_{4}^{{2 - }})</span>–ZrO<sub>2</sub> and Ni/HMOR components of this system have on the reaction. The probable mechanism of the hydrogenation of aromatic hydrocarbons is discussed. It is hypothesized that hydrogenating activity synergism results from the radical reaction becoming one of an ion radical.</p>","PeriodicalId":767,"journal":{"name":"Russian Journal of Physical Chemistry A","volume":"98 12","pages":"2717 - 2722"},"PeriodicalIF":0.7,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142672432","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Some Features of Non-Exchangeable Sorption of Tryptophan: The Role of Polar and π–π Interactions 色氨酸不可交换吸附的一些特点：极性和 π-π 相互作用的作用
IF 0.7 4区 化学
Russian Journal of Physical Chemistry A Pub Date : 2024-11-18 DOI: 10.1134/S0036024424701991
O. N. Khokhlova, E. R. Kashirtseva, V. Yu. Khokhlov, S. A. Lisitsyna
{"title":"Some Features of Non-Exchangeable Sorption of Tryptophan: The Role of Polar and π–π Interactions","authors":"O. N. Khokhlova,&nbsp;E. R. Kashirtseva,&nbsp;V. Yu. Khokhlov,&nbsp;S. A. Lisitsyna","doi":"10.1134/S0036024424701991","DOIUrl":"10.1134/S0036024424701991","url":null,"abstract":"<p>The non-exchangeable sorption of tryptophan by the AV-17-2P anion exchanger from solutions of different compositions was studied. The sorption of the amino acid was shown to be independent of the nature of the accompanying component. This was explained by quantum-chemical modeling, which gave variants of attachment and energy characteristics of the bonds formed in the sorbent phase during non-exchangeable sorption of tryptophan by a highly basic anion exchanger in the salt form. The polar interactions play the major role, and π–π interactions produce an additional effect during the non-exchangeable sorption of amino acids on highly basic aromatic anion exchangers.</p>","PeriodicalId":767,"journal":{"name":"Russian Journal of Physical Chemistry A","volume":"98 12","pages":"2757 - 2762"},"PeriodicalIF":0.7,"publicationDate":"2024-11-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142672536","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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