Young-Hoon Lee, Hee Jeong Park, Eunbin Park, Geumbi Na, Ji Hwan Kim, Se-Woong Baek, Seunghwan Bae, June Huh, Yung-Eun Sung, Seung-Ho Yu
{"title":"Geometry-independent uniform zinc deposition in sustainable aqueous zinc-ion batteries","authors":"Young-Hoon Lee, Hee Jeong Park, Eunbin Park, Geumbi Na, Ji Hwan Kim, Se-Woong Baek, Seunghwan Bae, June Huh, Yung-Eun Sung, Seung-Ho Yu","doi":"10.1039/d5ee05097a","DOIUrl":"https://doi.org/10.1039/d5ee05097a","url":null,"abstract":"To address challenges such as dendrite growth, hydrogen evolution, and corrosion that degrade the reversibility and uniform zinc deposition in aqueous zinc-ion batteries, extensive research has focused on developing inorganic co-solvent systems. However, many of the co-solvents under investigation are highly toxic. Herein, to overcome these limitations, we employed provitamin B5, an eco-friendly and biocompatible co-solvent commonly used in skin moisturizers. The formation of a unique provitamin B5–zinc ion complex in the electrolyte was confirmed through heteronuclear multiple bond correlation (HMBC), indicating strong interactions between provitamin B5 molecules and zinc ions. This complex significantly enhanced zinc ion diffusion, enabling uniform zinc deposition up to 3.2 cm in a capillary cell without dendritic growth and hydrogen evolution. As a result, these effects of provitamin B5 co-solvent exhibited outstanding cycling stability for 3500 hours at 1 mA cm<small><sup>−2</sup></small> under 1 mAh cm<small><sup>−2</sup></small> conditions, and even under a harsh 35% depth-of-discharge condition, it maintained stable operation for 600 hours. Moreover, the full cell under pouch cell conditions revealed a remarkable cycle retention of 90% with a Coulombic efficiency of 99.75% over 1000 cycles. This study offers a new platform to co-solvent engineering for highly reversible and sustainable aqueous-ion batteries.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"24 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-10-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145247394","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Hydrogen-Bond Network Sieve Enables Selective OH-/Cl- Discrimination for Stable Seawater Splitting at 2.0 A·cm-2","authors":"Yang Yu, Wei Zhou, Junshu Yuan, Xiaohan Zhou, Xiaoxiao Meng, Xuewei Zhang, Xuhan Li, Naiyuan Xue, Yingjian Chen, Xiao Xia, Mengyao Gu, Juan Chen, Xingxing Wang, Fei Sun, Jihui Gao, Guangbo Zhao","doi":"10.1039/d5ee04595a","DOIUrl":"https://doi.org/10.1039/d5ee04595a","url":null,"abstract":"Direct seawater electrolysis offers a sustainable route to producing green hydrogen, but it suffers from severe chloride corrosion at conventional anodes. Challenging the long-standing electrostatic repulsion model for chloride suppression, we reveal that interfacial hydrogen-bond networks govern selective OH- transport while excluding Cl-. Through integrated ab initio molecular dynamics and in-situ Raman spectroscopy, we demonstrate that structured water layers near the anode form a dynamic H-bond sieve: OH- undergoes barrier-free transfer by reconfiguring the H-bond network, while Cl- faces high rejection due to its inability to reorganize interfacial water. Leveraging this mechanism, we engineer an interfacial H-bond buffer using SO42- and CO32- anions. SO42- reinforces the H-bond network to block Cl-, while CO32- acts as an OH- pump to mitigate depletion at high current densities. The optimized buffer enables a CoFe LDH anode to achieve exceptional activity (overpotential of 291.4 mV at 300 mA·cm-2) and stability (550 h at 2.0 A·cm-2). Integrated into an anion-exchange membrane electrolyzer, the system delivers industrially relevant performance (2.51 V @ 1.0 A·cm-2, 4.85 kWh·Nm-3 H2) with 1000h stability. This work establishes a transformative H-bond-mediated ion-sieving paradigm for corrosion-resistant seawater electrochemistry.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"32 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-10-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145241698","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Song Kyu Kang, Minho Kim, Seochan Hong, Jae-Hong Lim, Gwan Hyeon Park, Junhyuk Ji, Jeongbin Cho, Hansol Bae, Won Bae Kim
{"title":"Magneto-conversion anode design for unlocking high energy density and dendrite-free hybrid lithium–ion/lithium–metal batteries","authors":"Song Kyu Kang, Minho Kim, Seochan Hong, Jae-Hong Lim, Gwan Hyeon Park, Junhyuk Ji, Jeongbin Cho, Hansol Bae, Won Bae Kim","doi":"10.1039/d5ee02644j","DOIUrl":"https://doi.org/10.1039/d5ee02644j","url":null,"abstract":"By coupling intercalation with controlled lithium (Li) metal plating, hybrid Li–ion/Li–metal anodes offer a promising route toward higher energy-density and dendrite-free Li batteries. However, conventional graphite-based electroactive hosts inherently suffer from limited capacity and sluggish Li plating kinetics, which constrain further advancement. Here, we introduce a novel magnetically tailored conversion strategy that integrates ferromagnetic transition metal oxides with an interfacial conductive carbon layer under an external magnetic field to significantly increase the energy-density and reversibility of the electrode. The converted ferromagnetic nanoparticles, embedded within a lithiophilic Li<small><sub>2</sub></small>O matrix, regulate spatially uniform Li<small><sup>+</sup></small> flux and homogenize nucleation barriers <em>via</em> magnetically modulated ionic pathways and interfacial Li kinetics. Concurrently, the intrinsic spin-polarized surface capacitance of the ferromagnetic conversion chemistry is exploited to enhance charge storage and reversibility. <em>Operando</em> X-ray micro-imaging and computational modelling reveal dynamic evolution of Li deposition, showing that micromagnetic fields from magnetized ferromagnetic nanoparticles induce Lorentz force-driven ionic redistribution, guiding compact and dendrite-free Li growth, even at high deposition rates. As a result, a superior reversible capacity of 1400 mAh g<small><sup>−1</sup></small> is achieved with outstanding cyclability, maintaining a Coulombic efficiency over 99% after 300 cycles and further validating its practical viability in stable full-cell configurations. These insights suggest a new paradigm in hybrid anode design by bridging conversion chemistry with magnetically modulated interfacial Li dynamics.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"56 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-10-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145241809","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Yilin Ding, ZheYue Mei, Wenjing Zhang, Xueke Wu, Yaqi Zhang, Di Gao, Fan Lan, Run Li, Xungang Diao, Rufan Zhang
{"title":"Intelligent Electrochromic Photothermal Regulation for Integrated Building Energy Saving","authors":"Yilin Ding, ZheYue Mei, Wenjing Zhang, Xueke Wu, Yaqi Zhang, Di Gao, Fan Lan, Run Li, Xungang Diao, Rufan Zhang","doi":"10.1039/d5ee02750k","DOIUrl":"https://doi.org/10.1039/d5ee02750k","url":null,"abstract":"As the demand for energy-efficient buildings surges, it is of utmost importance to develop efficient and integrated intelligent energy-conservation technologies. This research presents a comprehensive intelligent energy-saving system that combines electrochromic dynamic photothermal regulation windows (DPRW) with selective dynamic radiative cooling regulators (SDRCR) using electrochromic technology. The DPRW enables independent solar transmittance modulation (ΔT=~92%/~82% at visible/near-infrared band) and mid-infrared emissivity switching (Δε=~0.6), leading to a temperature ~14°C lower than that of normal windows. The SDRCR provides customizable colors while guaranteeing selective emissivity modulation (Δεmax=0.6/0.64) within the atmospheric transparent windows (8-13 μm, 16-23 μm), facilitating dynamic thermal management with a temperature regulation of ~5°C for cooling/insulation and overcoming static radiative cooling limitations. EnergyPlus simulations suggest a potential annual energy saving of up to 99.5 MJ/m² and ~80% reduction in cooling energy consumption in hot climates. This study is the first to introduce electrochromic technology into an integrated building system and offers a novel solution for intelligent buildings through multi-band spectral control, achieving a balance among energy efficiency, aesthetic flexibility, and environmental adaptability.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"50 15 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-10-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145241496","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pierfrancesco Ombrini, Shakul Pathak, Dimitrios Ntagkras, Santosh K. Pal, Pranav Karanth, Fokko M. Mulder, Marnix Wagemaker, Martin Z. Bazant, Alexandros Vasileiadis
{"title":"Modeling Single-Crystal Electrodes as a Network of Primary Particles","authors":"Pierfrancesco Ombrini, Shakul Pathak, Dimitrios Ntagkras, Santosh K. Pal, Pranav Karanth, Fokko M. Mulder, Marnix Wagemaker, Martin Z. Bazant, Alexandros Vasileiadis","doi":"10.1039/d5ee04131g","DOIUrl":"https://doi.org/10.1039/d5ee04131g","url":null,"abstract":"Predicting lithium-ion battery behavior is critical for advancing next-generation energy storage. Conventional Doyle–Fuller–Newman models can simulate many materials, but they fail in phase-separating single-crystal systems, such as lithium iron phosphate (LiFePO4), where the electrical connectivity of primary particles limits charge transport. We redefine the electrode as a network of reactive primary particles, each governed by validated electrochemical kinetics and interconnected through tomographic-informed contact resistances. Without empirical tuning, the model predicts voltage responses of LiFePO4 electrodes across temperatures, rates, loadings, and dynamic load conditions using a single fitted physical parameter. It also captures and explains charge-discharge asymmetries and hysteresis. By bridging particle-scale physics up to cell-level performance, while retaining computational efficiency, this physics-based framework provides a foundation for the design, and control of single-crystal electrode systems.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"37 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-10-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145241495","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Cheng Liu, Vlad Martin-Diaconescu, Ashley Phillip Black-Serra, Siavash Khabazian, Bernat Mundet, Krzysztof Matlak, Lorenzo Stievano, Andrea Sorrentino, Laura Simonelli, Dino Tonti
{"title":"Unveiling Capacity Limitations of MnO2 in Rechargeable Zn Chemistry","authors":"Cheng Liu, Vlad Martin-Diaconescu, Ashley Phillip Black-Serra, Siavash Khabazian, Bernat Mundet, Krzysztof Matlak, Lorenzo Stievano, Andrea Sorrentino, Laura Simonelli, Dino Tonti","doi":"10.1039/d5ee03588k","DOIUrl":"https://doi.org/10.1039/d5ee03588k","url":null,"abstract":"Aqueous Zn–MnO2 batteries with mildly acidic electrolytes show attractive experimental capacities, however the underlying mechanisms remain elusive, particularly regarding the interactions of Zn2+ and H+ with MnO2, as well as the formation of Mn2+ and Zn4SO4(OH)6·xH2O (ZSH). Although these products are compatible with a two-electron dissolution mechanism, the observed first-discharge capacity is limited to approximately 300 mAh g-1MnO2, close to that of a one-electron reaction. To address this contradiction, commonly used α-MnO2 nanowires were chosen as cathode material and investigated by a systematic multimodal and multiscale approach under operando or ex situ conditions to analyze the processes that occur during the first discharge. MnO2 dissolution into Mn2+ and ZSH precipitation were confirmed, and the formation of a disordered phase at the nanowire surface with the accumulation of Mn(III) was detected. An in-depth analysis indicates that such Mn(III) species correspond to protonated corner-sharing MnO2 octahedra, which, unlike the edge-sharing ones, are hindered from undergoing disproportion, limiting the MnO2 dissolution and explaining the reduced capacity. This comprehensive mechanistic understanding opens new pathways for the selection of the most appropriate MnO2 phases and the optimization of electrodes to improve the performance of aqueous Zn–MnO2 battery systems.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"9 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-10-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145241498","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Competitive Coordination Effect to Simultaneously Achieve High-Energy and Stable Cycles in Li-Metal Pouch Cell under –40°C","authors":"Xingxing Meng, Xiao Zhang, Litong Shi, Zhe Chen, Jiashen Meng, Feixiang Ding, Xiong Liu, Baokang Zhang, Qian Wang, Liqiang Mai, Chaojiang Niu","doi":"10.1039/d5ee03522h","DOIUrl":"https://doi.org/10.1039/d5ee03522h","url":null,"abstract":"Lithium metal batteries (LMBs) are expected to have significant advantages under extreme low-temperature conditions (i.e., −40°C), mainly due to the much short ion transport pathway and deposition/stripping mechanism of Li metal anode. However, high-energy-density Li-metal pouch cells capable of stable operation at −40°C have rarely been reported due to the harsh condition under extremely low-temperature. Herein, a Li-metal pouch cell suitable for use at −40°C was designed, and coupled with a newly developed electrolyte, to simultaneously achieve high energy and stable cycling performance. The low-temperature capability of the LMBs is activated by a competitive coordination effect in the first solvation sheaths. The competitive coordination between Li+ and dimethyl carbonate (DMC) and 1, 2-dimethoxyethane (DME) weakens the interaction between Li+ and the solvent, widens the voltage window, and facilitates the formation of robust inorganic-rich interfaces under low-temperature conditions. Notably, a low-temperature Li-metal pouch cell was designed and assembled with an energy at 300 Wh kg−1. When tested at the extremely low temperature of −40°C, the Li-metal pouch cell can retain 77% of its energy output, with 93% capacity retention after 70 cycles. This work paves the way for low-temperature LMBs with competitive energy density and stable cycle life.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"33 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-10-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145241500","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Unified contact layers design for highly efficient segmented PbTe/Bi2Te3 thermoelectric devices","authors":"Linmao Wen, Li Yin, Xiaofang Li, Shanghao Chen, Tianyu Zhang, Jinxuan Cheng, Baopeng Ma, Yunzi Ren, Liming Xiao, Feng Cao, Jun Mao, Qian Zhang","doi":"10.1039/d5ee04306a","DOIUrl":"https://doi.org/10.1039/d5ee04306a","url":null,"abstract":"The development of segmented thermoelectric devices is often constrained by complex fabrication processes and the lack of interfacial materials compatible across different segments. Here, we demonstrate a unified contact layer design using TiTe2 for p-type PbTe/(Bi, Sb)2Te3 (BST) segmented thermoelectric devices guided by thermodynamic phase diagram analysis and validated through experimental investigations. The TiTe2 exhibits matched thermal expansion, exceptional chemical inertness, and low contact resistivity with both PbTe and BST. This enables a one-step spark plasma sintering (SPS) process that replaces conventional multi-step soldering, reducing interfacial parasitic resistance to below 5% of total device resistance. The optimized p-type segmented single leg achieved a record energy conversion efficiency of 15.3% at a temperature difference (ΔT) of 450 K, while a two-pair module achieved an efficiency of 13.5% at a ΔT of 500 K, outperforming conventional PbTe-based devices. The proposed interface design and simplified fabrication protocol provide a robust framework for advancing next-generation thermoelectric module development.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"23 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-10-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145241499","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Wenjun Peng, Jianan Wei, Hongbing Li, Wei Feng, Mengting Liu, Tianyang Xu, Shudi Qiu, Chong Liu, Michael Wagner, Andreas Distler, Christoph J Brabec, Yaohua Mai, Fei Guo
{"title":"Balancing the supersaturation rate and coordination capability for upscaling high-performance perovskite photovoltaics","authors":"Wenjun Peng, Jianan Wei, Hongbing Li, Wei Feng, Mengting Liu, Tianyang Xu, Shudi Qiu, Chong Liu, Michael Wagner, Andreas Distler, Christoph J Brabec, Yaohua Mai, Fei Guo","doi":"10.1039/d5ee03888j","DOIUrl":"https://doi.org/10.1039/d5ee03888j","url":null,"abstract":"Transferring the well-established perovskite ink formulations from antisolvent spin coating to scalable deposition techniques remains a great challenge, primarily owing to the strikingly different crystallization kinetics involved in the two processes. Here, we discover that a balanced trade-off between supersaturation rate and coordination capability plays an essential role in regulating crystallization kinetics of the perovskite films deposited by scalable methods. In comparison to the commonly used DMF/DMSO solvent mixture, incorporating a small volume of NMP promotes rapid α-phase perovskite nucleation together with controllable crystal growth. Consequently, high-quality crystalline perovskite films with large grains and voids-free buried interface are readily obtained by blade coating. On these bases, inverted perovskite solar cells (0.09 cm2) and mini-modules (21.84 cm2) achieve high efficiencies of 25.38% and 23.22%, respectively. Furthermore, the unencapsulated solar cells deliver remarkable durability under maximum power point (MPP) tracking, maintaining 87% of their initial efficiency over 1000 h. This work provides an important avenue to bridge the gap between lab-scale cells to fab-scale perovskite photovoltaic modules.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"18 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-10-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145209824","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Trace molecular chelation engineering of a self-healing hybrid interphase for highly stable aqueous zinc-ion batteries","authors":"Hongbo Wu, Gongxun Lu, Chang Dong, Tao Yang, Zeyang Sun, Zhijin Ju, Chengbin Jin, Ouwei Sheng, Dexin Yang, Tianyu Shen, Haojie Ji, Jian Zhang, Guangmin Zhou, Xuefeng Zhang","doi":"10.1039/d5ee05118e","DOIUrl":"https://doi.org/10.1039/d5ee05118e","url":null,"abstract":"Aqueous Zn-ion batteries (AZIBs) hold promise for grid-scale storage due to their intrinsic safety and low cost, yet face critical irreversible anode degradation from dendritic proliferation and parasitic reactions. Here, we introduce a molecular chelation-driven interfacial engineering strategy using trace polyglutamate sodium (PS) to construct a dynamically selfhealing hybrid interphase on Zn anodes. PS reorganizes interfacial water networks and chelates Zn 2+ , forming an adaptive hydrogel-like PS-Zn layer (PSZ), which further in situ generates an inorganic solid-electrolyte interphase (SEI). This synergistic PSZ-SEI layer provides robust electrode shielding, precise hydration regulation, and continuous self-repair. Consequently, Zn||Zn symmetric cells achieve >4500 h cycling, Zn||Na 2 V 6 O 16 •3H 2 O full cells exhibit stable cycling for 1000 cycles in coin cells and 180 cycles in pouch cells (N/P ratio = 1.62) under high cathode loading (~12 mg cm -2 ). The universality of this approach is further demonstrated in Zn||I 2 batteries over 5000 cycles. This ppm-level dynamic interface control resolves long-standing interfacial conflicts in practical AZIBs.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"37 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-10-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145203828","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
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