Energy & Environmental Science最新文献

{"title":"Enhancing the kinetics and reversibility of copper batteries via anionic chemistry","authors":"Qianwei Zhou, Linyu Hu, Huajun Zhang, Dongxu Hu, Guoqiang Liu, Maowen Xu, Hong Jin Fan, Zhimeng Liu, Chunlong Dai, Xin He","doi":"10.1039/d5ee00492f","DOIUrl":"https://doi.org/10.1039/d5ee00492f","url":null,"abstract":"Aqueous rechargeable batteries face the challenges of gas evolution side reactions on metal anodes. While copper metal offers a compelling candidate electrode due to its redox potential being above that of the hydrogen generation reaction, the role of coordinating anions in Cu-ion deposition/stripping is not clearly understood. Here, the influence of anions on the behavior of Cu during electrochemical processes is systematically investigated. Among various anions, perchlorate (ClO<small>₄</small><small>⁻</small>) enables the best reversibility and fastest deposition/stripping kinetics by preventing the formation of the Cu<small>₂</small>O by-product. A Cu‖Cu symmetric cell with a 0.5 m Cu(ClO<small>₄</small>)<small>₂</small> electrolyte achieves over 7000 hours of stable cycling at 1 mA cm<small>⁻²</small>, outperforming as a new benchmark for Cu electrodes. Moreover, a 3 m Cu(ClO<small>₄</small>)<small>₂</small> electrolyte lowers the freezing point to −112 °C by disrupting the hydrogen-bond network between water molecules. This electrolyte exhibits high ionic conductivity by the weak interaction between Cu<small>²⁺</small> and ClO<small>₄</small><small>⁻</small> ions. Our assembled planar Cu–MnO<small>₂</small> micro-battery through a dual-plating strategy demonstrates stable cycling for over 350 cycles and low-temperature performance down to −60 °C.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"56 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-05-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143910189","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Molecular Engineering of Residual Lithium Compounds for Stable LiNi0.92Co0.05Mn0.03O2 Cathodes","authors":"Weihong Jiang, Xianshu Wang, Xuerui Yang, Yun Zhao, Jun Yao, Xiaoping Yang, Wei Luo, Liang Luo, Jianguo Duan, Peng Dong, Yingjie Zhang, Baohua Li, Ding WANG","doi":"10.1039/d5ee00282f","DOIUrl":"https://doi.org/10.1039/d5ee00282f","url":null,"abstract":"Residual lithium compounds (RLCs) on the surface of high-nickel layered oxides aggravate battery capacity decay, irreversible phase transformation and safety hazards, hindering the development of high-energy density lithium-ion batteries (LIBs). Conventional physical and chemical methods not only increase the steps required to address RLCs but also fail to fully resolve the issues. Herein, we use the alkaline characteristics of RLCs to convert harmful RLCs into functional molecular layer during slurry preparation process, facilitating the formation of a stable cathode electrolyte interfacial (CEI) layer. As a proof of concept, 2,5-thiophenediylbisboronic acid (TDBA) is selected for surface molecular engineering of single-crystal LiNi0.92Co0.05Mn0.03O2 cathode through neutralization with RLCs. After in situ electrochemical reaction, the uniform and stable CEI forms and provides high Li+ diffusivity and mechanical strength, effectively suppressing cathode particle cracking and electrolyte decomposition. As a result, the cell with modified LiNi0.92Co0.05Mn0.03O2 cathode achieves a high retention of 83.23% over 600 cycles at 1 C and excellent capacity at 10 C (169.9 m Ah g-1) and a charge cutoff voltage of 4.3 V. Even at high voltages (4.4 V, 4.5, 4.6 V) or 60 ℃, it still contributes to much better cycling stability and longevity. The fabricated modified LiNi0.92Co0.05Mn0.03O2ǁgraphite pouch cell stably cycle over 450 times (&gt; 92% capacity retention) at 1 C. Our work presents a novel molecular engineering method that effectively re-decouples RLCs and CEI film in high-nickel layered oxides, emphasizing the significance of interface design for advancing battery and great potential for strategy applications.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"2 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-05-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143910190","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Charge carrier management for highly efficient perovskite/Si tandem solar cells with poly-Si based passivating contacts","authors":"Xuzheng Liu, Michael Rienäcker, Mohammad Gholipoor, Lingyi Fang, Tonghan Zhao, Benjamin Hacene, Julian Petermann, Ruijun Cai, Hang Hu, Thomas Feeney, Faranak Sadegh, Paul Fassl, Renjun Guo, Uli Lemmer, Robby Peibst, Ulrich Wilhelm Paetzold","doi":"10.1039/d5ee01486g","DOIUrl":"https://doi.org/10.1039/d5ee01486g","url":null,"abstract":"Integrating wide-bandgap organic-inorganic lead halide perovskite absorber layers with Si bottom solar cells into tandem architectures offers significant potential for increasing power conversion efficiency (PCE). However, achieving high-performance monolithic tandem devices remains challenging, particularly when processing perovskite top cells on top of industrial silicon bottom cells, featuring polycrystalline silicon on oxide (POLO) passivating contacts, as implemented in “TOPCon” solar cells. Here, we employ an advanced silicon bottom cell architecture incorporating full-area electron-selective POLO front contacts and laser-structured hole-selective POLO back contacts. We perform the N<small>₂</small> annealing at an elevated temperature of silicon bottom cells, effectively curing sputter-induced damage in the full-area electron-selective POLO contact of the recombination junction and enhancing the interface between transparent conductive oxide and the n-type doped poly-Si layer. Additionally, this annealing treatment likely improves the rear small-area contact between the aluminum and the p+ poly-Si. Furthermore, we investigate how the nickel oxide layer regulates the substrate morphology and affects the charge carrier mechanisms for the top perovskite solar cells. These strategies remarkably promote charge carrier management, achieving a monolithic perovskite/POLO-Si tandem solar cell with a PCE of 31%. Moreover, the unencapsulated tandem cell retained 93% of its initial efficiency after operating for 240 hours at maximum power point under one sun intensity, 25°C, and 30% relative humidity (ISOS-L-1), the extrapolated T80 lifetime is estimated to be 740 hours.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"46 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-05-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143910186","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Catalytic ultrasound-driven synthesis of syngas from CO2 saturated water","authors":"Lina Chen, Yi Qin, Claire T. Coulthard, Zoë R. Turner, Chunping Chen, James Kwan, Dermot O’Hare","doi":"10.1039/d5ee01202c","DOIUrl":"https://doi.org/10.1039/d5ee01202c","url":null,"abstract":"Conventional catalytic CO<small>₂</small> reduction into value-added products often encounters challenges such as high energy barriers and complex operational setups. Here, we introduce a sonocatalysis approach to CO<small>₂</small> reduction in water under ambient conditions. In an acoustic cavitation-induced high-energy local environment, the Cu nanoparticles incorporated on the ZnAl-layered double oxide create a favorable energy barrier for CO<small>₂</small> reduction in water, a CO production rate of 23.8 μmol<small>_CO</small> g<small>⁻¹</small> h<small>⁻¹</small> with over 85% selectivity was achieved by ultrasonic irradiation of a CO<small>₂</small>-saturated aqueous solution at room temperature. Furthermore, more acoustic cavitation was produced with 5% CO<small>₂</small> in argon dissolved in water, resulting in a higher CO productivity of 252.7 μmol<small>_CO</small> g<small>⁻¹</small> h<small>⁻¹</small>, 11 times larger than pure CO<small>₂</small>. Hydrogen production also increased with acoustic cavitation, creating a syngas mixture with a CO to H<small>₂</small> ratio of 1.2 to 2.2. This approach produces a high sonochemical efficiency of 211.1 μmol kJ<small>⁻¹</small> g<small>⁻¹</small> L<small>⁻¹</small> for the ultrasound-driven fuel production from CO<small>₂</small> and water. These results highlight the use of cavitation to provide an alternative approach to CO<small>₂</small> conversion.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"19 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-05-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143910187","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Design of Strong and Weak Intermolecular Interactions to Engineer Buried Interfaces in Inverted Wide-Bandgap Perovskite Solar Cells","authors":"Hui Li, Davide Regaldo, Chunsheng Jack Wu, Mirko Prato, Antonella Treglia, Heyong Wang, Wolfram Hempel, Michele Sessolo, Yang Zhou, Andrea Olivati, Annamaria Petrozza","doi":"10.1039/d5ee01110h","DOIUrl":"https://doi.org/10.1039/d5ee01110h","url":null,"abstract":"The interfaces between the charge extraction layers and the perovskite layer are critical in defining the performance and stability of wide-bandgap (WBG) perovskite solar cells (PSCs). They govern multiple critical factors affecting the operation of photovoltaic devices such as the energetics of the contact, and the crystallization process of the thin film, thus its structural and electronic quality. Self-assembled monolayers (SAMs) have emerged as promising candidates as hole-selective materials for inverted PSCs, thanks to the flexibility provided by the large library of their functional groups. Herein, we outline a molecular hybridization strategy through the incorporation of the histamine molecule into the [4-(3,6-dimethyl-9H-carbazol-9yl)butyl]phosphonic acid (Me-4PACz), which is one of the most common hole extracting layers. Playing with intermolecular strong and weak interactions, we can contextually act on multiple processes. The proton transfer from the phosphonic acid group of the Me-4PACz to the ethylamine functional group of histamine enables the design of the interface dipole to facilitate hole extraction and minimize recombination losses. Then, the protonated amines balance the nucleation of halide components and stabilize the halide ions in the perovskite, avoiding their migration. Thus, three-dimensional nanovoids and tensile stress at the bottom surface were reduced, stabilizing the buried interface. Finally, the π-π interactions between the imidazole moiety and Me-4PACz improve the molecular assembling of the SAM, reducing disorder at the interfacial contact. The general impact of these results has been tested on PSCs based on lead mix-halide perovskites with two different bandgaps. The inverted WBG PSCs with 1.77 eV bandgap present a power conversion efficiency (PCE) of 20.34%, and maintains 95.5% of the initial PCE after 1000 hours of continuous illumination. The highly challenging WBG PSCs with 1.83 eV bandgap deliver a PCE of 18.99% with a Voc as high as 1.364 V-ranking among the highest reported PCEs and Voc values for such large bandgap.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"18 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-05-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143910191","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Efficient charge separation at localized 2D ferroelectric domains in perovskite solar cells","authors":"Jihoo Lim, Seungmin Lee, Hongjae Shim, Lei Wang, Hyeonah Cho, Jincheol Kim, Claudio Cazorla, Yong-Jin Kim, Hanul Min, Minwoo Lee, Xiaojing Hao, S. Ravi P. Silva, Jan Seidel, Dohyung Kim, Jun Hong Noh, Jae Sung Yun","doi":"10.1039/d5ee00640f","DOIUrl":"https://doi.org/10.1039/d5ee00640f","url":null,"abstract":"Ferroelectric properties can be utilized for efficient charge carrier separation through spontaneous electric polarization. Here, we reveal the potential of ferroelectric-assisted charge separation in 2D perovskites in conjunction with conventional p–n junction photovoltaics. We fabricate high-quality perovskite devices in which a ferroelectric 2D perovskite layer with oppositely polarized regions is locally formed on top of a 3D perovskite layer. Such distinct regions are created near the grain boundary and grain interior regions within the perovskites, and their polarity can be manipulated under bias voltage and light illumination. This configuration promotes distinct potential offsets between the two regions and acts as an excellent electron–hole pair separator. Our findings offer promising opportunities for the design of ferroelectric and p–n junction hybrid photovoltaic devices, resulting in a power conversion efficiency of 26.0%, with an independently certified efficiency of 25.2%.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"139 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-05-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143910188","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Highly Dense Atomic Fe-Ni Dual Metal Sites for Efficient CO2 to CO Electrolyzers at Industrial Current Densities","authors":"Manman Qi, Michael J. Zachman, Yingxin Li, Yachao Zeng, Sooyeon Hwang, Jiashun Liang, Mason Lyons, Qian Zhao, Yu Mao, Yuyan Shao, Zhenxing Feng, Ziyun Wang, Yong Zhao, Gang Wu","doi":"10.1039/d5ee01081k","DOIUrl":"https://doi.org/10.1039/d5ee01081k","url":null,"abstract":"Carbon-supported, atomically dispersed, nitrogen-coordinated metal sites (e.g., Fe and Ni) are arguably the most promising catalysts for the electrochemical reduction of CO2 to CO due to their unique catalytic properties and the use of earth-abundant elements. However, single metal sites are constrained by their structural simplicity, causing either too weak or too strong absorption/desorption of multiple critical intermediates (e.g., *COOH and *CO). Current catalysts also suffer from ultra-low loadings (&lt; 1.0 wt.%) of atomic metal active sites in catalysts, leading to inadequate performance for CO2-to-CO conversion. Here, we develop dual Ni/Fe metal site catalysts with significantly increased atomically dispersed metal loadings (up to 4.8 wt.%). We developed a gas-phase chemical vapor deposition (CVD) approach to introduce single Ni sites into Fe2O3/ZIF-8 precursors, followed by an optimal thermal activation. The optimized CVD-Ni/Fe-N-C catalyst exhibited remarkable electrocatalytic performance for the CO2 reduction to CO in a continuous membrane-electrode-assembly electrolyzer, achieving a maximum CO Faradaic efficiency (FECO) of 96% at a current density of 700 mA cm−2 in a near-neutral electrolyte. Furthermore, a desirable but challenging acidic flow-cell electrolyzer was designed using this dual metal site catalyst to improve CO2 utilization, accomplishing a FECO of up to 95% at a CO partial current density close to 600 mA cm−2. Density functional theory (DFT) calculations suggest a synergetic effect between Fe-Ni pairs facilitating *COOH intermediate formation and *CO desorption simultaneously during CO2 to CO conversion. This is key to breaking the linear scaling relationship of conventional single-metal site catalysts during the CO2 reduction reaction.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"35 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-05-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143910160","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Cascade electrocatalysis via integrating ruthenium clusters and yttrium single atoms for boosted alkaline hydrogen evolution","authors":"Haotian Zhang, Haoran Guo, Fuhui Zhang, Jinyang Zhang, Yizhuo Cheng, Yanqing Ma, Lei Ma, Limin Qi","doi":"10.1039/d5ee00810g","DOIUrl":"https://doi.org/10.1039/d5ee00810g","url":null,"abstract":"Anion-exchange-membrane water electrolysis (AEMWE) has emerged as a highly prospective technology for large-scale hydrogen production. However, its widespread application is severely restricted by the sluggish kinetics of alkaline hydrogen evolution reaction (HER). Inspired by enzymatic cascade reactions, this work proposes a novel cascade electrocatalysis mechanism for alkaline HER on a supported metal catalyst comprising Ru clusters and Y single atoms simultaneously immobilized on a N-doped carbon support (Ru-YNC). Specifically, oxophilic Y single atoms serve as preferential water adsorption and dissociation centers, and the generated hydrogen adsorption intermediates are promptly captured and reduced by adjacent Ru clusters owing to the different adsorption properties of Ru and Y species, thereby remarkably accelerating the alkaline HER kinetics. Consequently, the Ru-YNC exhibits an overpotential of only 22 mV at 10 mA cm-2 in 1.0 M KOH. The assembled AEMWE electrolyzer delivers a current density of 1000 mA cm-2 and a remarkable noble metal mass activity of 52.07 A mgnoble metal-1 at a cell voltage of 1.87 V. Furthermore, it shows outstanding durability over 1000 h at 500 mA cm-2 with a degradation rate of only 40 μV h-1. This work provides new insights into catalyst design and mechanism exploration for electrochemical alkaline HER.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"18 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-05-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143910161","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Opportunities and Challenges for Emerging Inorganic Chalcogenide-Silicon Tandem Solar Cells","authors":"Vijay C Karade, Mingrui He, Abasi Abudulimu, Zhaoning Song, Yeonwoo Park, Donghoon Song, Yanfa Yan, Jin Hyeok Kim, Randy Ellingson, Jae Ho Yun, Xiaojing Hao, Seung Wook Shin, Mahesh P. Suryawanshi","doi":"10.1039/d4ee04526b","DOIUrl":"https://doi.org/10.1039/d4ee04526b","url":null,"abstract":"This review highlights the promise of emerging inorganic chalcogenide-silicon (Si) tandem solar cells (TSCs) to overcome the power conversion efficiency (PCE) and long-term stability limitations of single-junction solar cells, advancing them toward early commercialization. First, we cover the fundamentals of TSCs, including basic concepts, design considerations, and key requirements. The unique optoelectronic properties of proven and emerging chalcogenide absorber materials are then thoroughly examined to evaluate whether they are suitable candidates for the top cell in tandem configurations. Furthermore, we highlight the critical factors that limit PCE when compared to III-V-, Si-, and perovskite-based tandem and single-junction solar cells. In light of limitations, we discuss the challenges and solutions for the fabrication process, device performance, long-term stability, and outdoor testing of chalcogenide-Si TSCs. Finally, we provide perspectives on future research directions and potential pathways for the early commercialization of these emerging inorganic chalcogenide-Si tandem technologies.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"4 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-05-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143897673","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Built-in Single-Ion-Conducting Polymer Bridges for Superior Ion Transport Enabling Long-Life and High-Voltage Lithium-Metal Batteries","authors":"Jiajun Gong, Qimin Peng, Shunshun Zhao, Taolue Wen, Haojie Xu, Weiting Ma, Zhicheng Yao, Yong Chen, Guoxiu Wang, Shimou Chen","doi":"10.1039/d5ee01338k","DOIUrl":"https://doi.org/10.1039/d5ee01338k","url":null,"abstract":"Composite polymer electrolyte (CPE)-based Li metal batteries have emerged as the most promising candidates for next-generation batteries. However, intrinsic incompatibility between composite phases severely compromises electrolyte performance. Herein, we propose a built-in single-ion-conductor bridge that seamlessly links the garnet-type oxide phase with PVDF-based polymer matrixes, enabling excellent composite compatibility and superior Li⁺ fluxes throughout the bulk electrolyte. The 2‐acrylamido‐2‐methylpropanesulfonic acid molecule is chosen to in-situ convert the inert surface layer of garnet fast‐ion conductors into a molecular single‐ion-conducting layer with rapid ionic transport, effectively bridging ion transport among multiple components. The resulting CPE exhibits remarkable long-cycling stability under extreme conditions (e.g., high voltage of 4.5 V, high loading of 10.2 mg cm−2, and low temperature of –30 °C). Specifically, the assembled Li||LiNi0.9Co0.05Mn0.05O2 pouch cells delivered a stable cycling for 1200 cycles at 0.5 C. Moreover, the strategy is readily applicable to sodium metal batteries, achieving decay-free performance over 2200 cycles. Thus, it offers a promising approach for fabricating high-performance solid-state batteries.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":"95 1","pages":""},"PeriodicalIF":32.5,"publicationDate":"2025-05-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143897671","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}