Advanced Materials Technologies最新文献

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Optimizing Metamaterial Inverse Design with 3D Conditional Diffusion Model and Data Augmentation (Adv. Mater. Technol. 14/2025) 基于三维条件扩散模型和数据增强的超材料逆向设计优化[j]。抛光工艺。14/2025)
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-07-21 DOI: 10.1002/admt.202570074
Xiaoyang Zheng, Junichiro Shiomi, Takayuki Yamada
{"title":"Optimizing Metamaterial Inverse Design with 3D Conditional Diffusion Model and Data Augmentation (Adv. Mater. Technol. 14/2025)","authors":"Xiaoyang Zheng,&nbsp;Junichiro Shiomi,&nbsp;Takayuki Yamada","doi":"10.1002/admt.202570074","DOIUrl":"10.1002/admt.202570074","url":null,"abstract":"<p><b>Metamaterial Design</b></p><p>In article number 2500293, Xiaoyang Zheng, Takayuki Yamada, and Junichiro Shiomi propose a novel 3D conditional diffusion model (3D-CDM), combined with a data augmentation technique to expand the small dataset, aimed at enhancing the inverse design of voxel-based metamaterials. The 3D-CDM generates realistic 3D metamaterials with targeted properties, outperforming existing methods in both fidelity and diversity.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 14","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-07-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202570074","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144673089","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High Magnetic Sensitivity at the Coercive Field Induced by Shear Horizontal SAW in Polycrystalline FeGa Films 剪切水平SAW在多晶FeGa薄膜矫顽力场下的高磁灵敏度
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-07-12 DOI: 10.1002/admt.202500746
Juan Diego Aguilera, Rocio Ranchal, Fernando Gálvez, Jose Miguel Colino, Isabel Gràcia, Stella Vallejos, Antonio Hernando, Pilar Marín, Patricia de la Presa, Daniel Matatagui
{"title":"High Magnetic Sensitivity at the Coercive Field Induced by Shear Horizontal SAW in Polycrystalline FeGa Films","authors":"Juan Diego Aguilera,&nbsp;Rocio Ranchal,&nbsp;Fernando Gálvez,&nbsp;Jose Miguel Colino,&nbsp;Isabel Gràcia,&nbsp;Stella Vallejos,&nbsp;Antonio Hernando,&nbsp;Pilar Marín,&nbsp;Patricia de la Presa,&nbsp;Daniel Matatagui","doi":"10.1002/admt.202500746","DOIUrl":"10.1002/admt.202500746","url":null,"abstract":"<p>A Love wave device is designed to generate surface acoustic waves (SAWs) with strong shear-horizontal polarization, interacting with a polycrystalline Fe<sub>72</sub>Ga<sub>28</sub> magnetostrictive layer. The shear strain induced by these waves at a frequency of ≈160 MHz, coupled with magnetoelastic effects, leads to domain magnetization oscillation, resulting in unique responses that are particularly pronounced near the coercive field. Experimental results reveal that the response of the sensor is highly sensitive to the angle between the applied magnetic field and the wave propagation direction, with profiles that can vary significantly depending on this angle, with some configurations resulting in practically opposite responses. A particularly relevant case arises when the magnetic field is aligned with the Love wave propagation direction. In this case, the sensor response shows mainly a monotonic increase with the magnetic field, except near the coercive field, where a sharp peak emerges and then abruptly collapses, resulting in a magnetic sensitivity of ≈5 Hz/nT (0.031 ppm nT<sup>−1</sup>). This high sensitivity near the coercive field opens the door to the development of high-performance sensors, simplifying electronics while leveraging the key advantages of SAW technology, including low power consumption, compact size, real-time response, and portability. A theoretical model is also discussed to further understand the underlying phenomena and optimize the design of next-generation devices, which hold significant potential for sensor applications across various fields.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 18","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-07-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://advanced.onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202500746","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145101082","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Ultra-Sensitive Wireless Capacitive Nanocomposite-Based Pressure Sensors for Health Monitoring 用于健康监测的超灵敏无线电容纳米复合压力传感器
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-07-12 DOI: 10.1002/admt.202501316
Seyedamin Hashemi, Saman Ebrahimibasabi, Mostafa Sajjadi, Naghmeh Shahraki, Delaram Tamjid Shabestari, Maryam Golshahi, Saeed Zeinolabedinzadeh, Hamed Arami, Layla Khalifehzadeh
{"title":"Ultra-Sensitive Wireless Capacitive Nanocomposite-Based Pressure Sensors for Health Monitoring","authors":"Seyedamin Hashemi,&nbsp;Saman Ebrahimibasabi,&nbsp;Mostafa Sajjadi,&nbsp;Naghmeh Shahraki,&nbsp;Delaram Tamjid Shabestari,&nbsp;Maryam Golshahi,&nbsp;Saeed Zeinolabedinzadeh,&nbsp;Hamed Arami,&nbsp;Layla Khalifehzadeh","doi":"10.1002/admt.202501316","DOIUrl":"https://doi.org/10.1002/admt.202501316","url":null,"abstract":"<p>Wireless pressure sensing plays a crucial role in a wide range of applications, including robotics, wearables, and health monitoring. These sensors are of particular interest in healthcare, especially for monitoring physiological pressures such as intraocular, blood, bladder, and intracranial pressure (ICP), offering significant potential for clinical use. However, improving the sensitivity and in vivo performance of these sensors remains a key challenge. In this paper, a novel approach is introduced to enhance the sensitivity of wireless capacitive pressure sensors by utilizing a nanocomposite dielectric layer. Biocompatible zinc oxide (ZnO) nanoparticles are incorporated into styrene-ethylene-butylene-styrene (SEBS) at different concentrations to fabricate a nanocomposite pyramid-structured dielectric layer. Sensors with a 0.7%-ZnO (v/v) nanocomposite dielectric layer exhibit a 4.3-fold improvement in sensitivity compared to ones with a pure SEBS dielectric layer. The sensitivity of the fabricated sensors reaches a notably high value of 45 MHz mmHg⁻¹ within the pressure range of up to 25 mmHg. Additionally, a new pickup probe is developed that extends the wireless reading distance by 40% over conventional probes. Furthermore, in vivo studies are conducted, demonstrating reliable detection of ICP changes in murine models. This design enables wireless sensing without complex electronics, offering enhanced sensitivity, stability, and clinical potential.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 19","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-07-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145230758","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High-Speed Microscopy and Optofluidic Modulation of Dynamic Oscillations in Liquid Metal Microdroplets 液态金属微滴动态振荡的高速显微镜和光流控调制
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-07-12 DOI: 10.1002/admt.202500910
Chenggang Li, Mingzhang Xiong, Yi Qiao, Zushun Xu, Jing Zeng, Wen Fan
{"title":"High-Speed Microscopy and Optofluidic Modulation of Dynamic Oscillations in Liquid Metal Microdroplets","authors":"Chenggang Li,&nbsp;Mingzhang Xiong,&nbsp;Yi Qiao,&nbsp;Zushun Xu,&nbsp;Jing Zeng,&nbsp;Wen Fan","doi":"10.1002/admt.202500910","DOIUrl":"https://doi.org/10.1002/admt.202500910","url":null,"abstract":"<p>Autonomous interfacial oscillations of gallium-based liquid metals hold great promise for soft robotics and adaptive photonic devices, yet their rapid transient dynamics remain insufficiently characterized due to the limitations of conventional imaging techniques. Here, a high-speed microscopy study of self-sustained, asymmetric oscillations in eutectic gallium–indium (EGaIn) microdroplets partially immersed in hydrochloric acid (HCl) solution is presented. Using a cost-effective smartphone-based imaging platform capable of 7680 frames per second, a pronounced temporal asymmetry in the oscillation cycle, consisting of a rapid 3 ms contraction driven by surface oxidation, followed by a 86 ms recovery governed by acid-mediated oxide dissolution at the triple-phase boundary, is uncovered. The system supports stable, high-frequency oscillations, sustaining up to 31 Hz for over 30 min, a performance that contrasts markedly with previously reported behavior in alkaline environments. As proof of concept, a Janus EGaIn-HCl droplet functioning as an autonomous optical modulator, producing tunable laser reflection and interference patterns without external input, is demonstrated. The oscillation frequency is readily tunable via HCl concentration, offering a strategy for environmentally regulated, redox-driven soft matter dynamics. These findings support the development of intelligent, self-regulating soft devices for chemical-to-mechanical energy conversion as well as adaptive photonics.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 19","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-07-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145230819","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Thermal Annealing Enhances Piezoelectricity and Regenerative Potential of PVDF-TrFE Nanofiber Scaffolds. 热处理增强PVDF-TrFE纳米纤维支架的压电性和再生潜能。
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-07-09 DOI: 10.1002/admt.202401513
Maksym Krutko, Holly M Poling, Maulee Sheth, Supasek Kongsomros, Andrew E Bryan, Manju Sharma, Akaljot Singh, Hasan A Reza, Kathryn A Wikenheiser-Brokamp, Takanori Takebe, Michael A Helmrath, Greg M Harris, Leyla Esfandiari
{"title":"Thermal Annealing Enhances Piezoelectricity and Regenerative Potential of PVDF-TrFE Nanofiber Scaffolds.","authors":"Maksym Krutko, Holly M Poling, Maulee Sheth, Supasek Kongsomros, Andrew E Bryan, Manju Sharma, Akaljot Singh, Hasan A Reza, Kathryn A Wikenheiser-Brokamp, Takanori Takebe, Michael A Helmrath, Greg M Harris, Leyla Esfandiari","doi":"10.1002/admt.202401513","DOIUrl":"https://doi.org/10.1002/admt.202401513","url":null,"abstract":"<p><p>This study investigates bioelectric stimulation's role in tissue regeneration by enhancing the piezoelectric properties of tissue-engineered grafts using annealed poly(vinylidene fluoride-trifluoroethylene) (PVDF-TrFE) scaffolds. Annealing at temperatures of 80°C, 100°C, 120°C, and 140°C is assessed for its impact on material properties and physiological utility. Analytical techniques such as Differential Scanning Calorimetry (DSC), Fourier-Transform Infrared Spectroscopy (FTIR), and X-ray Diffraction (XRD) reveal increased crystallinity with higher annealing temperatures, peaking in β-phase content and crystallinity at 140°C. Scanning Electron Microscopy (SEM) shows that 140°C annealed scaffolds have enhanced lamellar structures, increased porosity, and maximum piezoelectric response. Mechanical tests indicate that 140°C annealing improved elastic modulus, tensile strength, and substrate stiffness, aligning these properties with physiological soft tissues. In vitro assessments in Schwann cells demonstrate favorable responses, with increased cell proliferation, contraction, and extracellular matrix attachment. Additionally, genes linked to extracellular matrix production, vascularization, and calcium signaling are upregulated. The foreign body response in C57BL/6 mice, evaluated through Hematoxylin and Eosin (H&E) and Picrosirius Red staining, shows no differences between scaffold groups, supporting the potential for future functional evaluation of the annealed group in tissue repair.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":" ","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC12380390/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144938517","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Coffee Ground Matrix Frame-Based Transient Battery for Environmentally Sustainable Sensor Applications (Adv. Mater. Technol. 13/2025) 环境可持续传感器应用的基于咖啡粉矩阵框架的瞬态电池。抛光工艺。13/2025)
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-07-07 DOI: 10.1002/admt.202570068
Nagaraju Mukurala, Hyeon Bin Jo, Han Min Kim, Hyeon Jong Lee, Geun Lee, Sung Hun Jin
{"title":"Coffee Ground Matrix Frame-Based Transient Battery for Environmentally Sustainable Sensor Applications (Adv. Mater. Technol. 13/2025)","authors":"Nagaraju Mukurala,&nbsp;Hyeon Bin Jo,&nbsp;Han Min Kim,&nbsp;Hyeon Jong Lee,&nbsp;Geun Lee,&nbsp;Sung Hun Jin","doi":"10.1002/admt.202570068","DOIUrl":"10.1002/admt.202570068","url":null,"abstract":"<p><b>Sustainable Transient Batteries</b></p><p>This artwork highlights a biodegradable transient battery built from coffee ground-derived matrix frames and Mg-AZ31/MoO<sub>3</sub> electrodes. The device delivers stable voltage and high energy density, with full degradation in 60 days. Repurposing organic waste into energy storage components, this eco-friendly platform advances sustainable electronics for environmental sensors and transient systems. More information can be found in article number 2500066 by Sung Hun Jin and co-workers.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 13","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-07-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202570068","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144573352","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A Paraffin-Based Photoresin: 3D Printing of Paraffin for Encapsulation-Free Shape-Stabilized Paraffin-Based Phase Change Materials (Adv. Mater. Technol. 13/2025) 石蜡基光树脂:用于无封装形状稳定石蜡基相变材料的石蜡3D打印抛光工艺。13/2025)
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-07-07 DOI: 10.1002/admt.202570070
Swathi Krishna Subhash, Qingchuan Song, Paul H. Kamm, Santiago Franco, Yunong Chen, Dorothea Helmer, Uwe Pelz, Frederik Kotz-Helmer, Peter Woias, Bastian E. Rapp
{"title":"A Paraffin-Based Photoresin: 3D Printing of Paraffin for Encapsulation-Free Shape-Stabilized Paraffin-Based Phase Change Materials (Adv. Mater. Technol. 13/2025)","authors":"Swathi Krishna Subhash,&nbsp;Qingchuan Song,&nbsp;Paul H. Kamm,&nbsp;Santiago Franco,&nbsp;Yunong Chen,&nbsp;Dorothea Helmer,&nbsp;Uwe Pelz,&nbsp;Frederik Kotz-Helmer,&nbsp;Peter Woias,&nbsp;Bastian E. Rapp","doi":"10.1002/admt.202570070","DOIUrl":"10.1002/admt.202570070","url":null,"abstract":"<p><b>Paraffin-Based Photoresins</b></p><p>In article number 2500617, Frederik Kotz-Helmer and co-workers demonstrate a low-cost approach for preparing shape-stabilized paraffin-based phase change materials using high resolution 3D printing.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 13","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-07-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202570070","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144573983","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effective Molecular Alignment of Semiconducting Polymer and Its Application to Photopatterned Stretchable Transistors (Adv. Mater. Technol. 13/2025) 半导体聚合物的有效分子取向及其在光模式可拉伸晶体管中的应用。抛光工艺。13/2025)
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-07-07 DOI: 10.1002/admt.202570071
Yasutaka Kuzumoto, Sung-Gyu Kang, Hyunbum Kang, Sangah Gam, Hyungjun Kim, Ji Young Jung, Suk Gyu Hahm, EunA Kim, Youngsik Shin, Seon-Jeong Lim, Youngjun Yun, Gae Hwang Lee
{"title":"Effective Molecular Alignment of Semiconducting Polymer and Its Application to Photopatterned Stretchable Transistors (Adv. Mater. Technol. 13/2025)","authors":"Yasutaka Kuzumoto,&nbsp;Sung-Gyu Kang,&nbsp;Hyunbum Kang,&nbsp;Sangah Gam,&nbsp;Hyungjun Kim,&nbsp;Ji Young Jung,&nbsp;Suk Gyu Hahm,&nbsp;EunA Kim,&nbsp;Youngsik Shin,&nbsp;Seon-Jeong Lim,&nbsp;Youngjun Yun,&nbsp;Gae Hwang Lee","doi":"10.1002/admt.202570071","DOIUrl":"10.1002/admt.202570071","url":null,"abstract":"<p><b>Photopatterned Stretchable Transistors</b></p><p>In article number 2500068, Youngjun Yun, Gae Hwang Lee, and co-workers present intrinsically stretchable organic transistors with high mobility and low off-current, achieved through multi-scale polymer alignment, photopatterning, and film transfer. These transistors exhibit reliable electrical performance under strain, making a key step toward stretchable electronics.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 13","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-07-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202570071","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144573984","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Strain Amplification via Helically Braided Fiber Reinforced Sleeve for Soft Material Energy Harvesting (Adv. Mater. Technol. 13/2025) 基于螺旋编织纤维增强套管的软材料能量收集应变放大技术。抛光工艺。13/2025)
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-07-07 DOI: 10.1002/admt.202570069
Emily Duan, Syed Ahmed Jaseem, Jeong Yong Kim, Michael D. Dickey, Matthew Bryant
{"title":"Strain Amplification via Helically Braided Fiber Reinforced Sleeve for Soft Material Energy Harvesting (Adv. Mater. Technol. 13/2025)","authors":"Emily Duan,&nbsp;Syed Ahmed Jaseem,&nbsp;Jeong Yong Kim,&nbsp;Michael D. Dickey,&nbsp;Matthew Bryant","doi":"10.1002/admt.202570069","DOIUrl":"10.1002/admt.202570069","url":null,"abstract":"<p><b>Soft Material Energy Harvesting</b></p><p>In article number 2402033, Matthew Bryant and co-workers introduce a braided fiber-reinforced sleeve that amplifies strain in soft materials. This approach improves the performance of strain sensors and energy harvesters, demonstrated with hydrogel-based electrical double layer supercapacitors to enhance sensor sensitivity and mechanical strength in wave energy harvesting.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 13","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-07-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/admt.202570069","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144573982","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Environmentally Robust Semiconducting Carbon Nanotube Extraction with Cellulose Acetate in Polar Solvents 在极性溶剂中用醋酸纤维素萃取半导体碳纳米管
IF 6.4 3区 材料科学
Advanced Materials Technologies Pub Date : 2025-07-05 DOI: 10.1002/admt.202501246
Kazuhiro Yoshida, Daichi Suzuki, Elia Marin, Yoshiyuki Nonoguchi
{"title":"Environmentally Robust Semiconducting Carbon Nanotube Extraction with Cellulose Acetate in Polar Solvents","authors":"Kazuhiro Yoshida,&nbsp;Daichi Suzuki,&nbsp;Elia Marin,&nbsp;Yoshiyuki Nonoguchi","doi":"10.1002/admt.202501246","DOIUrl":"10.1002/admt.202501246","url":null,"abstract":"<p>Semiconducting carbon nanotubes (CNTs) are recognized as candidates for next-generation electronics and energy applications, where scalable and reproducible post-synthesis extraction of semiconducting CNTs is still required. In this study, purifying semiconducting CNTs using cellulose acetate (CA) as a surfactant in polar organic solvents is proposed that can tolerate environmental impurities such as water. Dispersion experiments with up to 1 v/v% water added to the polar organic solvent showed no significant deterioration in the purity and yield of the semiconducting CNTs. This process requires no dry hydrophobic solvents, in contrast to widely used extraction methods with conducting polymers. Controlling the solubility of CA with an ethyl lactate-tetrahydrofuran mixture helped differentiate between the colloidal stabilities of semiconducting and metallic CNTs and increased the purity of semiconducting CNTs. The semiconducting CNTs purified in this study demonstrated significant conductivity switching characteristics in electric double-layer transistors and large thermoelectric power factors used for thermal-electrical energy conversion. This study lays the groundwork for bridging the gap between the material preparation stages and practical applications of semiconducting CNTs.</p>","PeriodicalId":7292,"journal":{"name":"Advanced Materials Technologies","volume":"10 18","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-07-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145100902","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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