Advanced Industrial and Engineering Polymer Research最新文献

筛选
英文 中文
Corrigendum regarding updated Declaration of Competing Interest statement in previously published articles 关于先前发表的文章中更新的竞争利益声明的勘误表
IF 12
Advanced Industrial and Engineering Polymer Research Pub Date : 2026-04-01 DOI: 10.1016/j.aiepr.2026.03.005
{"title":"Corrigendum regarding updated Declaration of Competing Interest statement in previously published articles","authors":"","doi":"10.1016/j.aiepr.2026.03.005","DOIUrl":"10.1016/j.aiepr.2026.03.005","url":null,"abstract":"","PeriodicalId":7186,"journal":{"name":"Advanced Industrial and Engineering Polymer Research","volume":"9 2","pages":"Pages 399-400"},"PeriodicalIF":12.0,"publicationDate":"2026-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147584272","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A comprehensive review on the influence of fused deposition modelling process parameters upon thermoplastic composite materials 熔融沉积成型工艺参数对热塑性复合材料影响的综述
IF 12
Advanced Industrial and Engineering Polymer Research Pub Date : 2026-04-01 Epub Date: 2025-11-27 DOI: 10.1016/j.aiepr.2025.11.006
Vijayvignesh Namasivayam Sukumaar , Sanjay Mavinkere Rangappa , Yucheng Liu , Suchart Siengchin
{"title":"A comprehensive review on the influence of fused deposition modelling process parameters upon thermoplastic composite materials","authors":"Vijayvignesh Namasivayam Sukumaar ,&nbsp;Sanjay Mavinkere Rangappa ,&nbsp;Yucheng Liu ,&nbsp;Suchart Siengchin","doi":"10.1016/j.aiepr.2025.11.006","DOIUrl":"10.1016/j.aiepr.2025.11.006","url":null,"abstract":"<div><div>This review critically examines how key fused deposition modelling (FDM) process parameters, such as nozzle and bed temperature, layer thickness, infill density, raster orientation, print speed and cooling rate, affect the mechanical and thermal performance of thermoplastic composite materials. The central research questions addressed include: (i) individual and interacting parameters influence tensile, flexural, impact and thermal properties (ii) how reinforcement type and morphology mediate process-structure-property relationships and (iii) what strategies can optimize these parameters for enhanced functional performance. The review synthesizes findings from recent literature to reveal that parameter optimization can significantly improve interlayer adhesion, reduce porosity and enhance crystallinity, thereby increasing strength, stiffness and thermal stability. Critical challenges are discussed, including anisotropy, void formation and limited reproducibility across build conditions. Finally, emerging research directions are outlined, including process optimization through data-driven and machine learning approaches, sustainable composite development and industrial scale-up through standardized process control. This review provides a consolidated framework for researchers and engineers to design and optimize FDM processing parameters for advanced thermoplastic composites.</div></div>","PeriodicalId":7186,"journal":{"name":"Advanced Industrial and Engineering Polymer Research","volume":"9 2","pages":"Pages 281-303"},"PeriodicalIF":12.0,"publicationDate":"2026-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147584418","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Stress-free two-way shape memory polyurethane with high reversible strain and excellent mechanical properties for intelligent actuators 无应力双向形状记忆聚氨酯,具有高可逆应变和优异的机械性能,用于智能执行器
IF 12
Advanced Industrial and Engineering Polymer Research Pub Date : 2026-04-01 Epub Date: 2025-11-17 DOI: 10.1016/j.aiepr.2025.11.004
Zhongzheng Zhu, Qitan Zheng, Junyi Yao, Siyu Liu, Hezhou Liu, Hua Li
{"title":"Stress-free two-way shape memory polyurethane with high reversible strain and excellent mechanical properties for intelligent actuators","authors":"Zhongzheng Zhu,&nbsp;Qitan Zheng,&nbsp;Junyi Yao,&nbsp;Siyu Liu,&nbsp;Hezhou Liu,&nbsp;Hua Li","doi":"10.1016/j.aiepr.2025.11.004","DOIUrl":"10.1016/j.aiepr.2025.11.004","url":null,"abstract":"<div><div>Stress-free two-way shape memory polymers (2W SMPs), capable of reversible transformation between two distinct shapes, hold great promise as actuator components for applications in soft robotics and other intelligent devices. However, fabricating stress-free 2W SMPs with superior mechanical properties and high reversible actuation through a simple processing method remains a significant challenge. To address this issue, we propose a strategy that utilizes hydrogen bonds to construct the skeleton phase for the fabrication of stress-free 2W SMPs. By introducing N, N-bis(2-hydroxyethyl) oxamide (BHO) chain extenders rich in amide groups, strong hydrogen bond interactions are formed in the microdomains. After programming, these temperature-sensitive hydrogen bonds generate internal stress. This stress drives crystallization-induced elongation of the semi-crystalline polymer and enables reversible actuation without the need for external stress. The resulting materials exhibit both high reversible strain (22.6 %) and excellent mechanical properties (tensile strength of 45.78 MPa and fracture strain of 1992.52 %). Furthermore, the dynamic tunability of hydrogen bonds imparts the polymer network with outstanding two-way shape memory programmability. After erasing the original programmed state at high temperature and then reprogramming it, the material can be endowed with different reversible strain behaviors, thereby allowing reuse in various application scenarios. This strategy provides an effective approach for the fabrication of high-performance stress-free 2W SMPs, which is expected to advance the development of intelligent actuation materials.</div></div>","PeriodicalId":7186,"journal":{"name":"Advanced Industrial and Engineering Polymer Research","volume":"9 2","pages":"Pages 316-326"},"PeriodicalIF":12.0,"publicationDate":"2026-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147584445","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Self-healing carbohydrate polymers: Synthesis, properties, mechanisms, and applications 自愈性碳水化合物聚合物:合成、性质、机理及应用
IF 12
Advanced Industrial and Engineering Polymer Research Pub Date : 2026-04-01 Epub Date: 2025-12-30 DOI: 10.1016/j.aiepr.2025.12.003
Fateme Veghari Atigh , Mohammad Reza Saeb , Mehdi Salami-Kalajahi
{"title":"Self-healing carbohydrate polymers: Synthesis, properties, mechanisms, and applications","authors":"Fateme Veghari Atigh ,&nbsp;Mohammad Reza Saeb ,&nbsp;Mehdi Salami-Kalajahi","doi":"10.1016/j.aiepr.2025.12.003","DOIUrl":"10.1016/j.aiepr.2025.12.003","url":null,"abstract":"<div><div>Carbohydrate polymers, also known as polysaccharides, such as alginate, chitosan, cellulose, and hyaluronic acid have emerged as versatile platforms for self-healing materials, because of their natural abundance, biocompatibility, and abundant functional groups. They may also exhibit antimicrobial activity mediated by reversible physical and/or chemical interactions, potentially enabling partial or autonomous self-repair following mechanical or chemical damage. In parallel with the growing demand for sustainable and adaptive materials, carbohydrate polymers have been recognized not merely for biomedical applications but also for environmental remediation, soft electronics, and active packaging. Despire substantial progress, the field remains partially fragmented. In this review, we systematically examine recent developments in extrinsic self-healing strategies (<em>e.g</em>., microcapsules and vascular networks) as well as intrinsic mechanisms, including hydrogen bonding; ionic and metal–ligand interactions, and host–guest recognition; π–π stacking; hydrophobic associations; and dynamic covalent chemistries such as Schiff-base formation, disulfide exchange, and borate ester linkage. We further analyze how polymer blending, copolymerization, and chemical or enzymatic modifications modulate healing kinetics, mechanical recovery, and responsiveness to external stimuli. Applications such as wound dressings, drug delivery systems, water purification membranes, and edible films are highlighted, alongside persistent challenges in scalability, long-term performance, and mechanical robustness. Looking ahead, the future of self-healing carbohydrate polymers depends on the degree to which the molecular-level design integrates with real-world functionality, also developing standardized evaluation methods, and fostering interdisciplinary collaboration. Addressing these aspects may accelerate translation from laboratory-scale outcomes to practical, large-scale applications, ultimately establishing these polymers as cornerstones of sustainable and intelligent material technologies.</div></div>","PeriodicalId":7186,"journal":{"name":"Advanced Industrial and Engineering Polymer Research","volume":"9 2","pages":"Pages 208-237"},"PeriodicalIF":12.0,"publicationDate":"2026-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147584503","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A novel flexible clamping method with adaptive error compensation for enhancing precision in polymer injection molding 基于自适应误差补偿的柔性装模方法提高了聚合物注射成型的精度
IF 12
Advanced Industrial and Engineering Polymer Research Pub Date : 2026-04-01 Epub Date: 2026-01-07 DOI: 10.1016/j.aiepr.2025.12.005
Qing-wen Yuan , Hong-yi Qu , Yong-kui Ren , Wei-bin Fu , Jin-ping Qu
{"title":"A novel flexible clamping method with adaptive error compensation for enhancing precision in polymer injection molding","authors":"Qing-wen Yuan ,&nbsp;Hong-yi Qu ,&nbsp;Yong-kui Ren ,&nbsp;Wei-bin Fu ,&nbsp;Jin-ping Qu","doi":"10.1016/j.aiepr.2025.12.005","DOIUrl":"10.1016/j.aiepr.2025.12.005","url":null,"abstract":"<div><div>Injection-molded optical products are widely used in various fields, but the clamping errors of traditional injection molding clamping systems are particularly detrimental to the manufacture of high-precision optical devices. Herein, a flexible adaptive clamping method was developed to dynamically compensate for clamping error through the isostatic pressure-driven floating structure. The adaptive clamping characteristics, specifically the relationship between the floating angle and the clamping force, were investigated through both theoretical modeling and laser interferometry experiments. And the feasibility and performance of this system were conclusively validated by successfully molding polystyrene (PS) microlens arrays. The produced components exhibited exceptional weight repeatability, with a deviation of merely 0.614 ‰, meeting the requirements for precision injection molding, and optical testing confirmed uniform focusing and imaging performance. This self-adaptive clamping method provides a practical and robust solution for high-precision injection molded products, overcoming mold deflection caused by clamping system errors to adapt the mold precision.</div></div>","PeriodicalId":7186,"journal":{"name":"Advanced Industrial and Engineering Polymer Research","volume":"9 2","pages":"Pages 385-398"},"PeriodicalIF":12.0,"publicationDate":"2026-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147584271","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Hydra's scenes of per- and polyfluoroalkyl substances (PFAS): Occurrence and removal across environments Hydra的全氟烷基和多氟烷基物质(PFAS)场景:在不同环境中的发生和去除
IF 12
Advanced Industrial and Engineering Polymer Research Pub Date : 2026-04-01 Epub Date: 2026-01-06 DOI: 10.1016/j.aiepr.2025.12.007
Weiwei Zhu , Qingqing Liang , Wenjuan Gu , Hao Wang , Yukang Xu , Yuxin Li
{"title":"Hydra's scenes of per- and polyfluoroalkyl substances (PFAS): Occurrence and removal across environments","authors":"Weiwei Zhu ,&nbsp;Qingqing Liang ,&nbsp;Wenjuan Gu ,&nbsp;Hao Wang ,&nbsp;Yukang Xu ,&nbsp;Yuxin Li","doi":"10.1016/j.aiepr.2025.12.007","DOIUrl":"10.1016/j.aiepr.2025.12.007","url":null,"abstract":"<div><div>Per- and polyfluoroalkyl substances (PFAS) have been widely utilized across various industrial and consumer applications due to their exceptional chemical and thermal stability, as well as combined hydrophobic-oleophobic properties. Representative applications include non-stick cookware coatings, water-repellent textile agents, industrial lubricants, and high-temperature sealing materials. Despite their functional advantages, the extreme environmental persistence of PFAS has raised growing concerns regarding their adverse impacts on ecosystems and human health. Owing to strong C–F bonds, PFAS exhibit extreme resistance to degradation, environmental persistence, and bio accumulative potential, leading to widespread ecological consequences. Human exposure to PFAS is associated with multiple health risks, including immunosuppression, endocrine disruption, hepatotoxicity, nephrotoxicity, and increased cancer risk, primarily through the ingestion of contaminated water and food. Current removal strategies mainly include adsorption, chemical degradation, membrane separation, and microbial degradation. However, these approaches often face significant challenges under real-world environmental conditions due to the complexity of environmental matrices. Natural aquatic systems typically contain a variety of coexisting constituents, such as inorganic salts, heavy metals, and natural organic matter, which compete for adsorption sites or interfere with degradation pathways, thereby reducing PFAS removal efficiency. Although numerous laboratory-scale studies have demonstrated high removal efficiencies, their applicability to complex environmental settings remains uncertain. Hence, tailoring PFAS removal strategies to specific environmental contexts is imperative. In situ evaluation of both removal mechanisms and environmental variables will be critical for identifying optimal remediation pathways. This review comprehensively examines the major sources, environmental distribution, and potential risks of PFAS. It focuses on comparative analysis of removal technologies and underlying mechanisms under various environmental conditions, with particular emphasis on the impact of environmental factors on PFAS removal efficiency. Furthermore, the review explores strategies to leverage these environmental variables to optimize remediation processes, thereby achieving more efficient and sustainable PFAS remediation.</div></div>","PeriodicalId":7186,"journal":{"name":"Advanced Industrial and Engineering Polymer Research","volume":"9 2","pages":"Pages 245-280"},"PeriodicalIF":12.0,"publicationDate":"2026-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147584504","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Kaolin-group and sepiolite–palygorskite-group clay minerals as next-generation platforms for polymer nanocomposites 高岭土组和海泡石-坡面石组粘土矿物作为下一代聚合物纳米复合材料的平台
IF 12
Advanced Industrial and Engineering Polymer Research Pub Date : 2026-04-01 Epub Date: 2025-11-14 DOI: 10.1016/j.aiepr.2025.11.001
Georgy Lazorenko, Anton Kasprzhitskii
{"title":"Kaolin-group and sepiolite–palygorskite-group clay minerals as next-generation platforms for polymer nanocomposites","authors":"Georgy Lazorenko,&nbsp;Anton Kasprzhitskii","doi":"10.1016/j.aiepr.2025.11.001","DOIUrl":"10.1016/j.aiepr.2025.11.001","url":null,"abstract":"<div><div>This work provides a systematic review of recent advances in polymer-matrix nanocomposites containing kaolin group and sepiolite–palygorskite group clay minerals such as kaolinite (Kln), halloysite (Hly), sepiolite (Sep) and palygorskite (Plg), as well as their derivatives fabricated via surface reactions with organic and inorganic substances. The study analyzes research hotspots, frontiers, and emerging trends in this field, as well as quantitatively and qualitatively evaluates the impact of institutions, countries, and researchers. The review summarizes the surface chemistry and physical characteristics of these clay minerals, along with key design approaches and methods used to prevent poor dispersion and agglomeration of filler particles in the fabrication of high-performance clay-polymer nanocomposites (CPNs) for various applications. Finally, a comprehensive analysis of the industrial, economic, and developmental aspects of fabricating such CPNs is provided.</div></div>","PeriodicalId":7186,"journal":{"name":"Advanced Industrial and Engineering Polymer Research","volume":"9 2","pages":"Pages 189-207"},"PeriodicalIF":12.0,"publicationDate":"2026-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147584449","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Printing 2D MXene-Based chipless radio frequency identification tags to enable plastic waste sorting for recycling 打印2D基于mxene的无芯片射频识别标签,使塑料废物分类回收
IF 12
Advanced Industrial and Engineering Polymer Research Pub Date : 2026-04-01 Epub Date: 2025-11-28 DOI: 10.1016/j.aiepr.2025.11.007
Kevin W. Sun , Fátima Villa-González , Dheeban Govindan , Mengqiang Zhao , Rahul Bhattacharyya
{"title":"Printing 2D MXene-Based chipless radio frequency identification tags to enable plastic waste sorting for recycling","authors":"Kevin W. Sun ,&nbsp;Fátima Villa-González ,&nbsp;Dheeban Govindan ,&nbsp;Mengqiang Zhao ,&nbsp;Rahul Bhattacharyya","doi":"10.1016/j.aiepr.2025.11.007","DOIUrl":"10.1016/j.aiepr.2025.11.007","url":null,"abstract":"<div><div>Plastic recycling is limited by mis-sorting across polymer families and additives. Current identification methods, such as SPI resin codes, labels, and visible/near-infrared/Fourier Transform infrared (VIS/NIR/FTIR) sorting, often fail for dark or filled plastics, multilayer materials, and contaminated packaging. We introduce a printable, chipless radio frequency identification (RFID) tag based on high-conductivity MXene traces protected by an ultrathin polyvinyl alcohol (PVA) film. The tag provides robust, remote identification, yet detaches/disperses in the standard alkaline, elevated-temperature wash already used in recycling processing, preventing contaminant carryover. We engineer resonant geometries for RFID readability, quantify oxidation-limited drift, and show that an ultrathin PVA film slows oxygen ingress to preserve conductivity and read range over storage and use. In simulated wash lines (1–2% NaOH, 60–85 °C), both MXene and PVA dissolve rapidly, yielding effective removal and negligible residue on flakes. This approach enables accurate pre-recycling sortation without compromising downstream polymer quality, offering a practical path to efficient and higher-purity recycled streams.</div></div>","PeriodicalId":7186,"journal":{"name":"Advanced Industrial and Engineering Polymer Research","volume":"9 2","pages":"Pages 346-354"},"PeriodicalIF":12.0,"publicationDate":"2026-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147584505","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Interfacial engineering of Poly(Ionic Liquid)-based composite electrolyte via ionic liquid modification for high-performance solid-state lithium batteries 高性能固态锂电池用离子液体改性聚离子液体基复合电解质界面工程研究
IF 12
Advanced Industrial and Engineering Polymer Research Pub Date : 2026-01-01 Epub Date: 2025-09-25 DOI: 10.1016/j.aiepr.2025.09.007
Qingfeng Liu , Yang Li , Qiufeng Huang , Lewen Yang , Caixia Zhang , Hucan Hong , Xugang Shu , Mingqiu Zhang , Wenhong Ruan , Fujie Yang
{"title":"Interfacial engineering of Poly(Ionic Liquid)-based composite electrolyte via ionic liquid modification for high-performance solid-state lithium batteries","authors":"Qingfeng Liu ,&nbsp;Yang Li ,&nbsp;Qiufeng Huang ,&nbsp;Lewen Yang ,&nbsp;Caixia Zhang ,&nbsp;Hucan Hong ,&nbsp;Xugang Shu ,&nbsp;Mingqiu Zhang ,&nbsp;Wenhong Ruan ,&nbsp;Fujie Yang","doi":"10.1016/j.aiepr.2025.09.007","DOIUrl":"10.1016/j.aiepr.2025.09.007","url":null,"abstract":"<div><div>This study addresses the critical challenges of low ionic conductivity in polymer-based composite electrolytes for solid-state lithium batteries (SSLBs) arising from high interfacial impedance. A poly(ionic liquid) (PIL)-based composite electrolyte was engineered by modifying Li<sub>7</sub>La<sub>3</sub>Zr<sub>2</sub>O<sub>12</sub> (LLZO) nanowire surfaces with pyridine-functionalized ionic liquid via electrostatic adsorption. This interfacial strategy constructs efficient Li<sup>+</sup> transport pathways at the PIL/LLZO interface, significantly enhancing PIL chain segmental motion. The optimized electrolyte membrane achieves a high ionic conductivity of 2.79 × 10<sup>−4</sup> S cm<sup>−1</sup> at 25 °C. Symmetrical Li||Li cells demonstrate stable plating/stripping for 600 h, while the assembled LiFePO<sub>4</sub>||Li half cell delivers 169.81 mAh g<sup>−1</sup> at 55 °C (0.5C rate) with 77.35 % capacity retention after 400 cycles, outperforming the unmodified system. This interfacial engineering approach provides a scalable strategy for developing high-performance SSLB electrolytes.</div></div>","PeriodicalId":7186,"journal":{"name":"Advanced Industrial and Engineering Polymer Research","volume":"9 1","pages":"Pages 63-73"},"PeriodicalIF":12.0,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146057549","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Role of fluorinated-component positioning in Li metal battery performance 氟化组件定位在锂金属电池性能中的作用
IF 12
Advanced Industrial and Engineering Polymer Research Pub Date : 2026-01-01 Epub Date: 2025-10-28 DOI: 10.1016/j.aiepr.2025.10.002
Linglan He , Junshi Zhang , Yue Ma , Mingfu Ye , Dawei Song , Hongzhou Zhang , Xixi Shi , Lianqi Zhang
{"title":"Role of fluorinated-component positioning in Li metal battery performance","authors":"Linglan He ,&nbsp;Junshi Zhang ,&nbsp;Yue Ma ,&nbsp;Mingfu Ye ,&nbsp;Dawei Song ,&nbsp;Hongzhou Zhang ,&nbsp;Xixi Shi ,&nbsp;Lianqi Zhang","doi":"10.1016/j.aiepr.2025.10.002","DOIUrl":"10.1016/j.aiepr.2025.10.002","url":null,"abstract":"<div><div>To boost electrochemical performance, fluorine-containing constituents are often introduced into lithium metal batteries (LMBs) to achieve superior properties. However, the underlying mechanism governing positional effects of fluorinated species remains unclear. Herein, three typical gel polymer electrolytes: fluorinated solvent-dominated (FSD), fluorinated polymer-dominated (FPD), and dual-site fluorinated-dominated (DFD) are systematically fabricated to investigate the related influence. Ionic conductivity, XPS characterization and molecular dynamics confirm the contribution of fluorinated solvent to the formation of stable and anion-derived inorganic-rich solid electrolyte interphase (SEI) layer. Density functional theory (DFT) results demonstrate that fluorinated polymer exhibits enhanced interaction energies, leading to increased free ion concentration. While Consistent conclusions can be drawn from diffusion coefficient analysis and distribution of relaxation times (DRT) results. By synergistically combining the merits of fluorinated solvents and fluorinated polymer, an ionic conductivity of 1.19 mS cm<sup>−1</sup> is obtained for DFD and a minor polarization of 12 mV is achieved over 8000 h at 1 mA cm<sup>−1</sup> in Li//Li battery. After assembling with LiFePO<sub>4</sub>, capacity retentions of 91.3 % and 91.6 % are maintained after 200 cycles at 1C under 25 °C and 60 °C, showing exceptional cycling stability, respectively, particularly under elevated-temperature operating conditions.</div></div>","PeriodicalId":7186,"journal":{"name":"Advanced Industrial and Engineering Polymer Research","volume":"9 1","pages":"Pages 147-156"},"PeriodicalIF":12.0,"publicationDate":"2026-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146057294","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
0
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
相关产品
×
本文献相关产品
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信
小红书