ACS ES&T engineering最新文献

{"title":"","authors":"Kehan Li, Wenji Feng, Ao Zhong, Haiqiang Wang* and Zhongbiao Wu, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.4c00910","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144423818","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"","authors":"Ke-Lin Yu, Xiaojun Wang, Chunying Wang, Shaohua Chen, Sheng-Peng Sun*, John C. Crittenden and Yao-Yin Lou*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.4c00943","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144423796","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"","authors":"Yaqiong Luo, Jiacheng Bao, Xin Yan, Lei Shi, Fei Wang, Xin Sun*, Kai Li* and Ping Ning, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.4c00951","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144423800","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"","authors":"Boyu Jia, Siyu Zhang, Lijuan Zhang*, Weijia Li, Qunying Wang, Juanjuan Wan, Wanqing Zeng, Simona Rossetti, Bo Yan* and Xintai Su, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.5c00005","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144423922","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"","authors":"Jun-du Zhou, Wen-hui An, Lu-ming Ma and Yan Liu*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.4c00952","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144423931","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Activation of High-Valent Metal Oxidants on Carbon Catalysts: Mechanisms, Applications and Challenges","authors":"Yonghui Fan,&nbsp;Qiming Zhang,&nbsp;Yu Peng,&nbsp;Jinwen Zeng,&nbsp;Wei Ren*,&nbsp;Xiao Xiao and Xubiao Luo*,&nbsp;","doi":"10.1021/acsestengg.5c0016410.1021/acsestengg.5c00164","DOIUrl":"https://doi.org/10.1021/acsestengg.5c00164https://doi.org/10.1021/acsestengg.5c00164","url":null,"abstract":"<p >High-valent metal oxidants (HVMOs) have attracted considerable attention in advanced oxidation processes (AOPs) due to their high selectivity for oxidizing organic pollutants. However, the pursuit of green and efficient activators, together with the clarification of external factors affecting HVMO performance, remains a major challenge in practical applications. In this review, we present a comprehensive overview of the chemical properties of HVMOs, with a particular emphasis on their oxidation characteristics, focusing on permanganate (MnO₄^–), ferrate (FeO₄^–), dichromate (Cr₂O₇^2–). We further analyze energy changes and redox potential variations during the oxidation process. Recent advances in the activation of HVMOs by metal-free carbon materials are summarized, and the potential effects of common coexisting substances in environmental matrices, such as H⁺, OH^–, inorganic anions, metal ions, and natural organic matter (NOM), are critically examined. Moreover, potential risks associated with residual HVMOs after organic pollutant oxidation are discussed, along with relevant separation and purification strategies. This review aims to deepen the understanding of HVMOs in environmental catalysis, explore their potential for resource recovery, and provide perspectives on future research directions and practical applications.</p>","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 6","pages":"1338–1356 1338–1356"},"PeriodicalIF":7.4,"publicationDate":"2025-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144269587","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Unveiling Stainless-Steel Corrosion in the Drinking Water Distribution System: Interdisciplinary Insights on Water Quality and Anticorrosion Design","authors":"Xinyu Pan,&nbsp;Yumeng Zhao*,&nbsp;Xuhui Dang,&nbsp;Meng Sun,&nbsp;Gang Liu*,&nbsp;Gang Wen,&nbsp;Xinlei Li,&nbsp;Ao Chen,&nbsp;Chotiwat Jantarakasem,&nbsp;Federick Pinongcos,&nbsp;Linda Li and Jun Ma,&nbsp;","doi":"10.1021/acsestengg.5c0026010.1021/acsestengg.5c00260","DOIUrl":"https://doi.org/10.1021/acsestengg.5c00260https://doi.org/10.1021/acsestengg.5c00260","url":null,"abstract":"<p >Drinking water distribution system (DWDS) necessitates sustainable, durable, and nonpolluting materials for enhanced water quality of the end-users. Stainless steel (SS) is gaining momentum in DWDS, particularly in end-point distribution facilities such as secondary water storage tanks, pumps, and household water pipes due to its high chemical stability and robust mechanical strength. However, SS’s susceptibility to corrosion in given defect areas is of great concern, and there is a lack of fundamental insight on SS corrosion from an interdisciplinary perspective of materials science and environmental science. Herein, the SS corrosion in the DWDS environment is critically assessed, encompassing the basic science of SS corrosion occurrence, its cascading influence on water quality, and anticorrosion strategies. Electrochemical corrosion mechanisms of SS corrosion are specifically differentiated, particularly those initiated at given SS defects, including welding points, grain boundaries, and areas with tensile stress. It is shown that SS corrosion influences water quality by destroying the Cr-rich passive film and releasing Cr, Fe, and other heavy metals from the corrosion scale. The critical factors influencing SS corrosion are subsequently identified, namely, SS elemental composition, SS manufacturing process (e.g., heat-affected zone, stress concentration), and water condition in DWDS (e.g., chlorine, oxygen, sulfate, hydraulic shock, pH). Corresponding strategies are elucidated to facilitate the anticorrosion resistance of SS and improve the water quality, including SS alloying enhancement, SS dispersion strengthening, SS surface treatment/modification, and tuning water condition in DWDS. Overall, this review highlights the importance of controlling SS corrosion, which could provide guidance on the rational design and utilization of SS in DWDS to enhance the ultimate water quality of the end-users and the overall resilience of the DWDS.</p>","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 6","pages":"1357–1372 1357–1372"},"PeriodicalIF":7.4,"publicationDate":"2025-05-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144269613","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Carbonic Anhydrase-Integrated Silk Hydrogels for Efficient Microalgae Growth and Carbon Fixation","authors":"Taoqing He,&nbsp;Yawen Yin,&nbsp;XingXing Li,&nbsp;Lei Zhu,&nbsp;Zhaozhu Zheng,&nbsp;Gang Li,&nbsp;Xiaoqin Wang* and David L. Kaplan,&nbsp;","doi":"10.1021/acsestengg.4c0083110.1021/acsestengg.4c00831","DOIUrl":"https://doi.org/10.1021/acsestengg.4c00831https://doi.org/10.1021/acsestengg.4c00831","url":null,"abstract":"<p >Microalgae can capture CO₂ from the air and convert it into biomass and valuable byproducts, positioning these organisms as the key in terms of sustainable carbon fixation technologies. However, cultivating microalgae efficiently and cost-effectively remains a significant challenge. In this study, we enhanced the cultivation of microalgal cells within a silk/alginate hydrogel, shielded by CO₂ adsorption/desorption functional fabrics, to generate an innovative sandwich-structured composite system. Additionally, carbonic anhydrase-encapsulated silk fibroin nanoparticles were synthesized and co-embedded with the microalgae in the hydrogel. This silk-based microencapsulation sustained enzymatic activity, improving the conversion of CO₂ to bicarbonate and providing vital inorganic carbon for microalgal growth. The integration of microchannels within the gel facilitated continuous flow of culture medium via a microinjection pump, addressing nutrient deficiencies during prolonged exposure to air. Our findings indicate that microalgae cultivated in this system exhibit a significantly higher growth rate and carbon fixation rate compared to control setups, highlighting their potential as a carbon fixation system.</p>","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 6","pages":"1373–1384 1373–1384"},"PeriodicalIF":7.4,"publicationDate":"2025-05-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144269528","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Recent Advances in Engineering Functional Catalysts toward Multicomponent VOC Purification under Reality","authors":"Jicheng Liu,&nbsp;Yani Wu,&nbsp;Chunli Zheng*,&nbsp;Mingjiao Tian,&nbsp;Zeyu Jiang*,&nbsp;Reem Albilali and Chi He*,&nbsp;","doi":"10.1021/acsestengg.5c0015910.1021/acsestengg.5c00159","DOIUrl":"https://doi.org/10.1021/acsestengg.5c00159https://doi.org/10.1021/acsestengg.5c00159","url":null,"abstract":"<p >Volatile organic compounds (VOCs) have caused serious harm to human health and the ecological environment. As a promising strategy, the catalytic oxidation of VOCs into harmless products such as H₂O and CO₂ has been widely employed. Although many catalysts have been developed for VOC decomposition, the design and synthesis of functional catalysts toward multicomponent VOC purification in industrial exhaust gas under reality remains a great challenge. In the actual vent, the composition of multicomponent VOCs is complex and impurities such as NO_<i>x</i>, SO₂, and H₂O are also present. Traditional catalysts often suffer from poor stability, deactivation by impurities, and inefficient oxidation of complex VOC mixtures in industrial settings. Addressing these challenges requires a deeper understanding of the fundamental mechanisms and advanced catalyst design strategies. Therefore, elucidating the mechanism of multicomponent VOC oxidation and revealing the influential behavior of impurities are urgently required to guide researchers on how to synthesize effective and stable catalysts proactively for multicomponent VOC purification under reality. Accordingly, this review systematically summarizes the recent advances in the engineering of highly active and durable catalysts for the oxidation of multicomponent VOCs. The experimental and theoretical studies revealing the mixing effects occurring in the catalytic oxidation process of multicomponent VOCs are also highlighted. Further development of and research on catalysts to be adopted in multipollutant controlling are proposed. This review can help researchers to better understand the catalytic elimination of multicomponent VOCs and provide a great foundation for future design and practical industrial application of VOC oxidation catalysts.</p>","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 6","pages":"1316–1337 1316–1337"},"PeriodicalIF":7.4,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144269912","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"","authors":"Lianghui Xia,&nbsp;Yujie Liu,&nbsp;Kang Hui Lim,&nbsp;Qiyuan Liu,&nbsp;Meizan Jing*,&nbsp;Yanfei Jian,&nbsp;Jingjing Wang,&nbsp;He Xu,&nbsp;Mudi Ma*,&nbsp;Shouning Chai,&nbsp;Reem Albilali and Chi He*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":7008,"journal":{"name":"ACS ES&T engineering","volume":"5 5","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":7.4,"publicationDate":"2025-05-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsestengg.4c00861","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144452039","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}