npj Spintronics最新文献

{"title":"Emergence of exchange bias in van der Waals magnetic alloy CrxPt1−xTe2","authors":"Ryan Bailey-Crandell, Warren L. B. Huey, Archibald J. Williams, Wenyi Zhou, Joshua E. Goldberger, Roland K. Kawakami","doi":"10.1038/s44306-024-00028-1","DOIUrl":"10.1038/s44306-024-00028-1","url":null,"abstract":"CrxPt1−xTe2 is a recently developed van der Waals magnetic alloy noted for its stability under ambient conditions. Here, we report the emergence of an exchange bias effect in CrxPt1−xTe2, without typical exchange bias sources such as an adjacent antiferromagnetic layer. We find that the exchange bias is present for x = 0.45 and absent for x = 0.35, which is correlated to the presence of a Cr modulation where the Cr concentration alternates each vdW layer (modulation period of 2 layers) for x ≥ 0.4. We perform Monte Carlo simulations utilizing exchange parameters from first-principles calculations, which recreate the exchange bias in hysteresis loops of Cr0.45Pt0.55Te2. From our simulations, we infer the source of exchange bias to be magnetic moments locked into free energy minima that resist magnetization reversal. This work presents a way to introduce desirable magnetic properties to van der Waals magnets.","PeriodicalId":501713,"journal":{"name":"npj Spintronics","volume":" ","pages":"1-7"},"PeriodicalIF":0.0,"publicationDate":"2024-07-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s44306-024-00028-1.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141537074","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Spintronics meets orbitronics: Emergence of orbital angular momentum in solids","authors":"Daegeun Jo, Dongwook Go, Gyung-Min Choi, Hyun-Woo Lee","doi":"10.1038/s44306-024-00023-6","DOIUrl":"10.1038/s44306-024-00023-6","url":null,"abstract":"One of the ultimate goals of spintronics is to realize an efficient electrical manipulation of spin for high-speed and low-power nanodevices. A core ingredient for achieving this goal is the relativistic interaction between the electron’s orbital motion and spin, but the properties of the orbital angular momentum itself have remained largely unexplored. However, recent theories and experiments have uncovered that electrons may acquire nonvanishing orbital angular momentum when an external electric field is applied, even without the spin–orbit coupling. These findings have spurred the emergence of a burgeoning field known as orbitronics, which harnesses the orbital angular momentum to manipulate magnetic devices. In this Review, we provide an overview of the recent developments in orbitronics and discuss their implications for spintronics. We then outline future avenues of research at the intersection of spintronics and orbitronics.","PeriodicalId":501713,"journal":{"name":"npj Spintronics","volume":" ","pages":"1-9"},"PeriodicalIF":0.0,"publicationDate":"2024-06-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s44306-024-00023-6.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141537073","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Slow and non-equilibrium dynamics due to electronic ferroelectricity in a strongly-correlated molecular conductor","authors":"Tatjana Thomas, Yassine Agarmani, Steffi Hartmann, Mark Kartsovnik, Natalia Kushch, Stephen M. Winter, Sebastian Schmid, Peter Lunkenheimer, Michael Lang, Jens Müller","doi":"10.1038/s44306-024-00022-7","DOIUrl":"10.1038/s44306-024-00022-7","url":null,"abstract":"Ferroelectricity, where electronic degrees of freedom determine the polar order—thereby enabling fast switching and phase control—is an important research field in current condensed-matter physics. Using a combination of resistance noise and dielectric spectroscopy we investigate the nature of relaxor-type electronic ferroelectricity in the organic conductor κ-(BETS)2Mn[N(CN)2]3, a system that represents a wider class of materials of correlated electron systems for which functionalities for organic spintronics recently have been discussed. The two complementary spectroscopies reveal a distinct low-frequency dynamics on different length scales, namely (i) an intrinsic relaxation that is typical for relaxor ferroelectrics which classifies the system as a possible new multiferroic, and (ii) two-level processes which we identify as fluctuating polar nanoregions (PNR), i.e., clusters of quantum electric dipoles that fluctuate collectively. The PNR preform above the metal insulator (MI) transition. Upon cooling through TMI, a drastic increase of the low-frequency 1/f-type fluctuations and slowing down of the charge carrier dynamics is accompanied by the onset of strong non-equilibrium dynamics indicating a glassy transition of interacting dipolar clusters. The freezing of PNR and non-equilibrium dynamics is suggested to be a common feature of organic relaxor-type electronic ferroelectrics.","PeriodicalId":501713,"journal":{"name":"npj Spintronics","volume":" ","pages":"1-11"},"PeriodicalIF":0.0,"publicationDate":"2024-06-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s44306-024-00022-7.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141537086","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Formation of chirality in propagating spin waves","authors":"Cody Trevillian, Vasyl Tyberkevych","doi":"10.1038/s44306-024-00026-3","DOIUrl":"10.1038/s44306-024-00026-3","url":null,"abstract":"A general approach to quantify chirality, or absence of parity symmetry, of spin waves has been developed and applied to spin waves propagating in obliquely magnetized ferromagnetic films. Using theoretical arguments and numerical calculations, it is shown that, upon increasing spin wave wavevector, initially achiral spin waves develop chiral properties through the “parity exchange” mechanism, which implies, in particular, that chiral spin waves appear in pairs. The most striking example of the parity exchange mechanism is the simultaneous formation of two chiral waves: the magnetostatic surface wave and the recently discovered heterosymmetric spin wave, which were previously considered independent of each other. Another manifestation of the parity exchange is the formation of strongly chiral waves near the anti-crossings of spin wave branches of unequal symmetry. These findings illustrate viable paths to engineering spin wave systems with prescribed chiral spectra that had not previously been considered.","PeriodicalId":501713,"journal":{"name":"npj Spintronics","volume":" ","pages":"1-8"},"PeriodicalIF":0.0,"publicationDate":"2024-06-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s44306-024-00026-3.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141537076","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Author Correction: Antiferromagnetic tunnel junctions for spintronics","authors":"Ding-Fu Shao, Evgeny Y. Tsymbal","doi":"10.1038/s44306-024-00037-0","DOIUrl":"10.1038/s44306-024-00037-0","url":null,"abstract":"","PeriodicalId":501713,"journal":{"name":"npj Spintronics","volume":" ","pages":"1-1"},"PeriodicalIF":0.0,"publicationDate":"2024-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s44306-024-00037-0.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141435708","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Celebrating 1 year of npj Spintronics","authors":"Elke Arenholz","doi":"10.1038/s44306-024-00032-5","DOIUrl":"10.1038/s44306-024-00032-5","url":null,"abstract":"","PeriodicalId":501713,"journal":{"name":"npj Spintronics","volume":" ","pages":"1-1"},"PeriodicalIF":0.0,"publicationDate":"2024-06-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s44306-024-00032-5.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141304305","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Multiferroic kinks and spin-flop transition in Ni2InSbO6 from first principles","authors":"Ryota Ono, Igor Solovyev, Sergey Artyukhin","doi":"10.1038/s44306-024-00020-9","DOIUrl":"10.1038/s44306-024-00020-9","url":null,"abstract":"Magnetoelectric multiferroics are key materials for next-generation spintronic devices due to their entangled magnetic and ferroelectric properties. Spiral multiferroics possess ferroelectric polarization and are particularly promising for electric control of magnetism and magnetic control of ferroelectricity. In this work, we uncover long-period incommensurate states characterized by unique multiferroic kinks in corundum nickelate Ni2InSbO6, a member of a promising family of polar magnets. Utilizing a 2-orbital S = 1 model, we derive formulas for Heisenberg and anisotropic magnetic exchanges and magnetically-induced polarization, enabling their calculations from first principles. We use these parameters in Monte Carlo and Landau theory-based calculations to reproduce experimentally observed magnetic structures and polarization dependence on the magnetic field. We predict magnetic phase transitions between flat spiral, conical spiral, canted antiferromagnetic and ferromagnetic states under increasing magnetic fields. Kinks in the spiral phases repel each other through a Yukawa-like potential arising from exchange of massive magnons. We also find that suitably directed electric fields can be used to stabilize the ferromagnetic and spiral states. The findings open a new pathway to predictive first-principles modelling of multiferroics and will inspire experiments and technological applications based on multiferroic kinks.","PeriodicalId":501713,"journal":{"name":"npj Spintronics","volume":" ","pages":"1-10"},"PeriodicalIF":0.0,"publicationDate":"2024-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s44306-024-00020-9.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141246220","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"High-temperature Néel skyrmions in Fe3GaTe2 stabilized by Fe intercalation into the van der Waals gap","authors":"Rana Saha, Holger L. Meyerheim, Börge Göbel, Ingrid Mertig, Stuart S. P. Parkin","doi":"10.1038/s44306-024-00024-5","DOIUrl":"10.1038/s44306-024-00024-5","url":null,"abstract":"Two-dimensional (2D) van der Waals (vdW) magnets that exhibit ferromagnetism at ambient temperature show great promise for spintronic applications. However, until now, only a few pristine or doped 2D magnets have demonstrated the ability to host non-collinear spin textures, thereby limiting their potential applications. Here we directly observe Néel-type skyrmions in the metallic vdW magnetic compound Fe3GaTe2 (FGaT) up to temperatures well above room temperature (≈340 K) in the absence of any external magnetic field. We show that the presence of defects in the structure of FGaT make its structure acentric and therefore compatible with hosting skyrmions that would otherwise not be possible. Indeed, in this regard it is very similar to the closely related compound Fe3GeTe2 (FGT), whose structure with the same space group P3m1 is also realized by defects. Interestingly, however, FGaT accommodates a significantly higher concentration of Fe within the vdW gaps, likely accounting for its enhanced Curie temperature (TC). In addition to the Néel skyrmions observed in the temperature range of 250–340 K, we also detect type-I and -II Bloch-type skyrmionic bubbles in the temperature range of 100–200 K due to an enhanced magnitude of dipole-dipole interactions relative to the Dzyaloshinskii-Moriya exchange interaction. Self-intercalation is thus a highly interesting property of vdW magnets that considerably modifies their fundamental properties.","PeriodicalId":501713,"journal":{"name":"npj Spintronics","volume":" ","pages":"1-7"},"PeriodicalIF":0.0,"publicationDate":"2024-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s44306-024-00024-5.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141246232","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Perspective: There is plenty of room for magnetic straintronics in the analog domain","authors":"Supriyo Bandyopadhyay","doi":"10.1038/s44306-024-00018-3","DOIUrl":"10.1038/s44306-024-00018-3","url":null,"abstract":"Magnetic straintronics made its debut more than a decade ago as an extremely energy-efficient paradigm for implementing a digital switch for digital information processing. The switch consists of a slightly elliptical nano-sized magnetostrictive disk in elastic contact with a poled ultrathin piezoelectric layer (forming a two-phase multiferroic system). Because of the elliptical shape, the nanomagnet’s magnetization has two stable (mutually antiparallel) orientations along the major axis, which can encode the binary bits 0 and 1. A voltage pulse of sub-ns duration and amplitude few to few tens of mV applied across the piezoelectric generates enough strain in the nanomagnet to switch its magnetization from one stable state to the other by virtue of the inverse magnetostriction (or Villari) effect, with an energy expenditure that is roughly an order of magnitude smaller than what it takes to switch a modern-day electronic transistor. That possibility, along with the fact that such a switch is non-volatile unlike the conventional transistor, generated significant excitement. However, it was later tempered by the realization that straintronic switching is also extremely error-prone, which may preclude many digital applications, particularly in Boolean logic. In this perspective, we offer the view that there is plenty of room for magnetic straintronics in the analog domain, which is much more forgiving of switching errors, and where the excellent energy-efficiency and non-volatility are a boon. Analog straintronics can have intriguing applications in many areas, such as a new genre of aggressively miniaturized electromagnetic antennas that defy the Harrington limits on the gain and radiation efficiency of conventional antennas, analog arithmetic multipliers (and ultimately vector matrix multipliers) for non-volatile deep learning networks with very small footprint and excellent energy-efficiency, and relatively high-power microwave oscillators with output frequency in the X-band. When combined with spintronics, analog straintronics can also implement a new type of spin field effect transistor employing quantum materials such as topological insulators, and they have unusual transfer characteristics which can be exploited for analog tasks such as frequency multiplication using just a single transistor. All this hints at a world of new possibilities in the analog domain that deserves serious attention.","PeriodicalId":501713,"journal":{"name":"npj Spintronics","volume":" ","pages":"1-15"},"PeriodicalIF":0.0,"publicationDate":"2024-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s44306-024-00018-3.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141246208","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Inducing a tunable skyrmion-antiskyrmion system through ion beam modification of FeGe films","authors":"M. B. Venuti, Xiyue S. Zhang, Eric J. Lang, Sadhvikas J. Addamane, Hanjong Paik, Portia Allen, Peter Sharma, David Muller, Khalid Hattar, Tzu-Ming Lu, Serena Eley","doi":"10.1038/s44306-024-00013-8","DOIUrl":"10.1038/s44306-024-00013-8","url":null,"abstract":"Skyrmions and antiskyrmions are nanoscale swirling textures of magnetic moments formed by chiral interactions between atomic spins in magnetic noncentrosymmetric materials and multilayer films with broken inversion symmetry. These quasiparticles are of interest for use as information carriers in next-generation, low-energy spintronic applications. To develop skyrmion-based memory and logic, we must understand skyrmion-defect interactions with two main goals—determining how skyrmions navigate intrinsic material defects and determining how to engineer disorder for optimal device operation. Here, we introduce a tunable means of creating a skyrmion-antiskyrmion system by engineering the disorder landscape in FeGe using ion irradiation. Specifically, we irradiate epitaxial B20-phase FeGe films with 2.8 MeV Au4+ ions at varying fluences, inducing amorphous regions within the crystalline matrix. Using low-temperature electrical transport and magnetization measurements, we observe a strong topological Hall effect with a double-peak feature that serves as a signature of skyrmions and antiskyrmions. These results are a step towards the development of information storage devices that use skyrmions and antiskyrmions as storage bits, and our system may serve as a testbed for theoretically predicted phenomena in skyrmion-antiskyrmion crystals.","PeriodicalId":501713,"journal":{"name":"npj Spintronics","volume":" ","pages":"1-10"},"PeriodicalIF":0.0,"publicationDate":"2024-06-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s44306-024-00013-8.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141246215","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}