Xi Hu, Nan Wang, Xia Guo, Zeyu Liang, Heng Sun, Hongwei Liao, Fan Xia, Yunan Guan, Jiyoung Lee, Daishun Ling, Fangyuan Li
{"title":"A Sub-Nanostructural Transformable Nanozyme for Tumor Photocatalytic Therapy","authors":"Xi Hu, Nan Wang, Xia Guo, Zeyu Liang, Heng Sun, Hongwei Liao, Fan Xia, Yunan Guan, Jiyoung Lee, Daishun Ling, Fangyuan Li","doi":"10.1007/s40820-022-00848-y","DOIUrl":"10.1007/s40820-022-00848-y","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000 <ul>\u0000 <li>\u0000 <p>An internal sub-nanostructural transformation of sub-nanostructural transformable gold@ceria (STGC-PEG) is initiated by the conversion between CeO<sub>2</sub> and electron-rich state of CeO<sub>2−x</sub>, and active oxygen vacancies generation via the hot-electron injection from gold to ceria.</p>\u0000 </li>\u0000 <li>\u0000 <p>The sub-nanostructural transformation of STGC-PEG enhances the peroxidase-like activity and activates the plasmon-promoted oxidase-like activity, resulting in an augmented reactive oxygen species output.</p>\u0000 </li>\u0000 <li>\u0000 <p>STGC-PEG successfully achieves excellent low power (50 mW cm<sup>−2</sup>) near-infrared light-activated photocatalytic ablation of tumors in vivo.</p>\u0000 </li>\u0000 </ul>\u0000 \u0000 </div></div>","PeriodicalId":48779,"journal":{"name":"Nano-Micro Letters","volume":null,"pages":null},"PeriodicalIF":26.6,"publicationDate":"2022-04-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-022-00848-y.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"4481555","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Hanxiao Xu, Guozheng Zhang, Yi Wang, Mingqiang Ning, Bo Ouyang, Yang Zhao, Ying Huang, Panbo Liu
{"title":"Size-Dependent Oxidation-Induced Phase Engineering for MOFs Derivatives Via Spatial Confinement Strategy Toward Enhanced Microwave Absorption","authors":"Hanxiao Xu, Guozheng Zhang, Yi Wang, Mingqiang Ning, Bo Ouyang, Yang Zhao, Ying Huang, Panbo Liu","doi":"10.1007/s40820-022-00841-5","DOIUrl":"10.1007/s40820-022-00841-5","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000 <ul>\u0000 <li>\u0000 <p>The size of metal organic frameworks (MOFs) derivatives was manipulated by a spatial confined growth strategy.</p>\u0000 </li>\u0000 <li>\u0000 <p>Dielectric polarization is the dominant dissipation mechanism due to the phase hybridization based on size dependent oxidation motion.</p>\u0000 </li>\u0000 <li>\u0000 <p>The specific reflection loss of synthesized Co/Co<sub>3</sub>O<sub>4</sub> hollow carbon nanocages surpasses most reported MOFs derived counterparts for practical microwave absorption applications.</p>\u0000 </li>\u0000 </ul>\u0000 \u0000 </div></div>","PeriodicalId":48779,"journal":{"name":"Nano-Micro Letters","volume":null,"pages":null},"PeriodicalIF":26.6,"publicationDate":"2022-04-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-022-00841-5.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"4480817","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Arpana Parihar, Ayushi Singhal, Neeraj Kumar, Raju Khan, Mohd. Akram Khan, Avanish K. Srivastava
{"title":"Next-Generation Intelligent MXene-Based Electrochemical Aptasensors for Point-of-Care Cancer Diagnostics","authors":"Arpana Parihar, Ayushi Singhal, Neeraj Kumar, Raju Khan, Mohd. Akram Khan, Avanish K. Srivastava","doi":"10.1007/s40820-022-00845-1","DOIUrl":"10.1007/s40820-022-00845-1","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000 <ul>\u0000 <li>\u0000 <p>Shed light on MXene-based electrochemical aptasensors for the detection of cancer biomarkers.</p>\u0000 </li>\u0000 <li>\u0000 <p>Strategies for the design and synthesis of biomarker-specific aptamer are presented.</p>\u0000 </li>\u0000 <li>\u0000 <p>The properties such as electrical conductivity, chemical stability, mechanical properties, and the hydrophilic–hydrophobic nature of MXenes are discussed.</p>\u0000 </li>\u0000 <li>\u0000 <p>Brief insight on futuristic sensing applications along with challenges are highlighted.</p>\u0000 </li>\u0000 </ul>\u0000 \u0000 </div></div>","PeriodicalId":48779,"journal":{"name":"Nano-Micro Letters","volume":null,"pages":null},"PeriodicalIF":26.6,"publicationDate":"2022-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-022-00845-1.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"4444803","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Tianhao Wu, Xiao Liu, Xinhui Luo, Hiroshi Segawa, Guoqing Tong, Yiqiang Zhang, Luis K. Ono, Yabing Qi, Liyuan Han
{"title":"Heterogeneous FASnI3 Absorber with Enhanced Electric Field for High-Performance Lead-Free Perovskite Solar Cells","authors":"Tianhao Wu, Xiao Liu, Xinhui Luo, Hiroshi Segawa, Guoqing Tong, Yiqiang Zhang, Luis K. Ono, Yabing Qi, Liyuan Han","doi":"10.1007/s40820-022-00842-4","DOIUrl":"10.1007/s40820-022-00842-4","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000 <ul>\u0000 <li>\u0000 <p>A novel strategy to further improve the efficiency of lead-free tin perovskite solar cells by carefully controlling the built-in electric field in the absorber is described.</p>\u0000 </li>\u0000 <li>\u0000 <p>A promising efficiency of 13.82% was obtained based on the formamidinium tin iodide (FASnI<sub>3</sub>) perovskite solar cells with a vertical Sn<sup>2+</sup> gradient and an enhanced electric field.</p>\u0000 </li>\u0000 <li>\u0000 <p>The solar cell with a heterogeneous FASnI<sub>3</sub> absorber is ultrastable, maintaining over 13% efficiency after operation under 1-sun illumination for 1,000 h in air.</p>\u0000 </li>\u0000 </ul>\u0000 \u0000 </div></div>","PeriodicalId":48779,"journal":{"name":"Nano-Micro Letters","volume":null,"pages":null},"PeriodicalIF":26.6,"publicationDate":"2022-04-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-022-00842-4.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"4645202","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Building Ultra-Stable and Low-Polarization Composite Zn Anode Interface via Hydrated Polyzwitterionic Electrolyte Construction","authors":"Qiong He, Guozhao Fang, Zhi Chang, Yifang Zhang, Shuang Zhou, Miao Zhou, Simin Chai, Yue Zhong, Guozhong Cao, Shuquan Liang, Anqiang Pan","doi":"10.1007/s40820-022-00835-3","DOIUrl":"10.1007/s40820-022-00835-3","url":null,"abstract":"<div><p>Aqueous zinc metal batteries are noted for their cost-effectiveness, safety and environmental friendliness. However, the water-induced notorious issues such as continuous electrolyte decomposition and uneven Zn electrochemical deposition remarkably restrict the development of the long-life zinc metal batteries. In this study, zwitterionic sulfobetaine is introduced to copolymerize with acrylamide in zinc perchlorate (Zn(ClO<sub>4</sub>)<sub>2</sub>) solution. The designed gel framework with hydrophilic and charged groups can firmly anchor water molecules and construct ion migration channels to accelerate ion transport. The in situ generated hybrid interface, which is composed of the organic functionalized outer layer and inorganic Cl<sup>−</sup> containing inner layer, can synergically lower the mass transfer overpotential, reduce water-related side reactions and lead to uniform Zn deposition. Such a novel electrolyte configuration enables Zn//Zn cells with an ultra-long cycling life of over 3000 h and a low polarization potential (~ 0.03 V) and Zn//Cu cells with high Coulombic efficiency of 99.18% for 1000 cycles. Full cells matched with MnO<sub>2</sub> cathodes delivered laudable cycling stability and impressive shelving ability. Besides, the flexible quasi-solid-state batteries which are equipped with the anti-vandalism ability (such as cutting, hammering and soaking) can successfully power the LED simultaneously. Such a safe, processable and durable hydrogel promises significant application potential for long-life flexible electronic devices. </p><figure><div><div><div><picture><source><img></source></picture></div></div></div></figure></div>","PeriodicalId":48779,"journal":{"name":"Nano-Micro Letters","volume":null,"pages":null},"PeriodicalIF":26.6,"publicationDate":"2022-04-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-022-00835-3.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"4234318","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Yulin Gao, Zhenghui Pan, Jianguo Sun, Zhaolin Liu, John Wang
{"title":"High-Energy Batteries: Beyond Lithium-Ion and Their Long Road to Commercialisation","authors":"Yulin Gao, Zhenghui Pan, Jianguo Sun, Zhaolin Liu, John Wang","doi":"10.1007/s40820-022-00844-2","DOIUrl":"10.1007/s40820-022-00844-2","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000 <ul>\u0000 <li>\u0000 <p>Fundamental rationalisation for high-energy batteries.</p>\u0000 </li>\u0000 <li>\u0000 <p>Newly emerging and the state-of-the-art high-energy batteries vs. incumbent lithium-ion batteries: performance, cost and safety.</p>\u0000 </li>\u0000 <li>\u0000 <p>Closing the gap between academic research and commercialisation of emerging high-energy batteries, and examination of the remaining challenges.</p>\u0000 </li>\u0000 </ul>\u0000 \u0000 </div></div>","PeriodicalId":48779,"journal":{"name":"Nano-Micro Letters","volume":null,"pages":null},"PeriodicalIF":26.6,"publicationDate":"2022-04-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-022-00844-2.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"4237051","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Nanozymes: Versatile Platforms for Cancer Diagnosis and Therapy","authors":"Xiaodong Zhang, Xiaokai Chen, Yanli Zhao","doi":"10.1007/s40820-022-00828-2","DOIUrl":"10.1007/s40820-022-00828-2","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000 <ul>\u0000 <li>\u0000 <p>This review introduces nanozymes that exhibit different enzymatic activities and emphasizes the advantages of nanozymes over natural enzymes.</p>\u0000 </li>\u0000 <li>\u0000 <p>The roles of nanozymes in different cancer diagnostic and therapeutic technologies are summarized, explained by representative examples.</p>\u0000 </li>\u0000 <li>\u0000 <p>The potential challenges of nanozyme-based cancer theranostics are outlined, and future research directions are outlooked.</p>\u0000 </li>\u0000 </ul>\u0000 \u0000 </div></div>","PeriodicalId":48779,"journal":{"name":"Nano-Micro Letters","volume":null,"pages":null},"PeriodicalIF":26.6,"publicationDate":"2022-04-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-022-00828-2.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"4233597","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Jingya Liu, Zhen Wen, Hao Lei, Zhenqiu Gao, Xuhui Sun
{"title":"A Liquid–Solid Interface-Based Triboelectric Tactile Sensor with Ultrahigh Sensitivity of 21.48 kPa−1","authors":"Jingya Liu, Zhen Wen, Hao Lei, Zhenqiu Gao, Xuhui Sun","doi":"10.1007/s40820-022-00831-7","DOIUrl":"10.1007/s40820-022-00831-7","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000 <ul>\u0000 <li>\u0000 <p>A self-powered liquid–solid interface ferrofluid-based triboelectric tactile sensor with immediately formed spike-shaped microstructure is proposed.</p>\u0000 </li>\u0000 <li>\u0000 <p>Due to the high spike microstructure, low Young’s modulus of ferrofluid and efficient solid–liquid interface contact-electrification, an ultrahigh sensitivity of 21.48 kPa<sup>−1</sup> for the triboelectric sensors can be achieved.</p>\u0000 </li>\u0000 <li>\u0000 <p>A strategy for personalized password lock with high security level is demonstrated.</p>\u0000 </li>\u0000 </ul>\u0000 \u0000 </div></div>","PeriodicalId":48779,"journal":{"name":"Nano-Micro Letters","volume":null,"pages":null},"PeriodicalIF":26.6,"publicationDate":"2022-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-022-00831-7.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"4002009","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Meifang Jiang, Pengzhou Mu, Huanrui Zhang, Tiantian Dong, Ben Tang, Huayu Qiu, Zhou Chen, Guanglei Cui
{"title":"An Endotenon Sheath-Inspired Double-Network Binder Enables Superior Cycling Performance of Silicon Electrodes","authors":"Meifang Jiang, Pengzhou Mu, Huanrui Zhang, Tiantian Dong, Ben Tang, Huayu Qiu, Zhou Chen, Guanglei Cui","doi":"10.1007/s40820-022-00833-5","DOIUrl":"10.1007/s40820-022-00833-5","url":null,"abstract":"<div><h2>Highlights</h2><div>\u0000 \u0000 \u0000 <ul>\u0000 <li>\u0000 <p>The double-network binder shows excellent adhesive and self-healing abilities, which help suppress electrode volume expansion and stabilize the electrode interface upon cycling.</p>\u0000 </li>\u0000 <li>\u0000 <p>This binder induces a Li<sub>3</sub>N/LiF-rich solid electrolyte interface layer, which can suppress continuous electrolyte decomposition.</p>\u0000 </li>\u0000 <li>\u0000 <p>Superior electrochemical performance can be achieved in Si/Li half cells and LiNi<sub>0.8</sub>Co<sub>0.1</sub>Mn<sub>0.1</sub>O<sub>2</sub>/Si full cells, even with a high loading of Si electrode.</p>\u0000 </li>\u0000 </ul>\u0000 \u0000 </div></div>","PeriodicalId":48779,"journal":{"name":"Nano-Micro Letters","volume":null,"pages":null},"PeriodicalIF":26.6,"publicationDate":"2022-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40820-022-00833-5.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"4001122","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}