Scripta Materialia最新文献

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Boosting energy storage at moderate fields in Sr₀.₇Bi₀.₂TiO₃ weakly polar relaxor via BiNi2/3Ta1/3O₃-induced ferroelectric-paraelectric composite structure 助推Sr 0 .₇Bi 0中等规模油田储能。通过bini2 / 3ta1 / 30o₃诱导的铁电-准电复合结构的2 TiO₃弱极性弛豫剂
IF 5.6 2区 材料科学
Scripta Materialia Pub Date : 2026-03-01 Epub Date: 2025-11-15 DOI: 10.1016/j.scriptamat.2025.117101
Yuming Mao , Jingji Zhang , Mo Chen , Min Fang , Ning Yan , Zhihao Lou , Yun Zhou
{"title":"Boosting energy storage at moderate fields in Sr₀.₇Bi₀.₂TiO₃ weakly polar relaxor via BiNi2/3Ta1/3O₃-induced ferroelectric-paraelectric composite structure","authors":"Yuming Mao ,&nbsp;Jingji Zhang ,&nbsp;Mo Chen ,&nbsp;Min Fang ,&nbsp;Ning Yan ,&nbsp;Zhihao Lou ,&nbsp;Yun Zhou","doi":"10.1016/j.scriptamat.2025.117101","DOIUrl":"10.1016/j.scriptamat.2025.117101","url":null,"abstract":"<div><div>The weakly polar relaxor Sr₀.₇Bi₀.₂TiO₃ is renowned for its exceptional energy efficiency but suffers from low maximum polarization. To overcome this trade-off, we introduce BiNi<sub>2/3</sub>Ta<sub>1/3</sub>O₃ to design a composite structure of coexisting ferroelectric A<sub>4</sub>B<sub>3</sub>O<sub>12</sub> and paraelectric ABO₃ phases. With increasing dopant, the A<sub>4</sub>B<sub>3</sub>O<sub>12</sub> phase is progressively replaced by paraelectric ABO₃ and pyrochlore Bi<sub>2</sub>Ti<sub>2</sub>O<sub>7</sub>, raising the phase-transition temperature. The optimal composition comprises 70.67% <em>P</em>4/<em>mbm</em> ABO₃, 28.49% <em>Fmmm</em> A<sub>4</sub>B<sub>3</sub>O<sub>12</sub>, 0.75% <em>Fd</em>3<em>m</em> Bi<sub>2</sub>Ti<sub>2</sub>O<sub>7</sub>, and 0.09% <em>Pnna</em> BiTaO<sub>4</sub>, forming polar clusters and a coherent boundary between the ABO₃ and A<sub>4</sub>B<sub>3</sub>O<sub>12</sub> phases. This yields a high energy storage density of 5.12 J cm<sup>-3</sup> an ultrahigh efficiency of 97.13% at a high breakdown strength of 460 kV cm<sup>-1</sup><strong>,</strong> together with a figure of merit of 175.90 J cm<sup>-3</sup> and environment-independent stability. These results establish the composite as a highly promising candidate for high-performance dielectric energy-storage devices.</div></div>","PeriodicalId":423,"journal":{"name":"Scripta Materialia","volume":"273 ","pages":"Article 117101"},"PeriodicalIF":5.6,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145527331","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Temperature-dependent deformation mechanisms and transition of fracture behaviors in polycrystalline Sn 多晶锡的温度变形机制及断裂行为转变
IF 5.6 2区 材料科学
Scripta Materialia Pub Date : 2026-03-01 Epub Date: 2025-11-24 DOI: 10.1016/j.scriptamat.2025.117112
Xiaoliang Ji , Yiping Xia , Jian Lin , Longxiao Huang , Yishu Wang , Fu Guo
{"title":"Temperature-dependent deformation mechanisms and transition of fracture behaviors in polycrystalline Sn","authors":"Xiaoliang Ji ,&nbsp;Yiping Xia ,&nbsp;Jian Lin ,&nbsp;Longxiao Huang ,&nbsp;Yishu Wang ,&nbsp;Fu Guo","doi":"10.1016/j.scriptamat.2025.117112","DOIUrl":"10.1016/j.scriptamat.2025.117112","url":null,"abstract":"<div><div>The low-temperature embrittlement of β-Sn poses a critical reliability challenge for Sn-based solders in cryogenic electronics. In this work, a comparative investigation was conducted by quasi-in-situ EBSD at 77 K and 293 K to elucidate the deformation mechanisms accounting for the ductile-to-brittle transition of β-Sn. It is found that the deformation mechanisms shift from dislocation-dominated to twinning-dominated as the temperature decreases. Dynamic recovery and continuous dynamic recrystallization were suppressed at 77 K, while discontinuous dynamic recrystallization occurred around the crack propagation path. The intergranular fracture at cryogenic temperature could be attributed to the failure of twin-twin transmission across grain boundaries. Molecular dynamics simulations further verified that the twin-twin transmission could accommodate the local strain, correlating its failure with the intergranular cracking. These findings offer new insights into the cryogenic brittleness of β-Sn, helping design Sn-based solders with enhanced cryogenic reliability.</div></div>","PeriodicalId":423,"journal":{"name":"Scripta Materialia","volume":"273 ","pages":"Article 117112"},"PeriodicalIF":5.6,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145621340","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Distinct impacts of hydrogen and carbon on thermally activated dislocation motion in Fe-Cr-Ni austenitic steel 氢和碳对Fe-Cr-Ni奥氏体钢热激活位错运动的显著影响
IF 5.6 2区 材料科学
Scripta Materialia Pub Date : 2026-03-01 Epub Date: 2025-11-22 DOI: 10.1016/j.scriptamat.2025.117111
Haruki Nishida , Yuhei Ogawa , Akinobu Shibata
{"title":"Distinct impacts of hydrogen and carbon on thermally activated dislocation motion in Fe-Cr-Ni austenitic steel","authors":"Haruki Nishida ,&nbsp;Yuhei Ogawa ,&nbsp;Akinobu Shibata","doi":"10.1016/j.scriptamat.2025.117111","DOIUrl":"10.1016/j.scriptamat.2025.117111","url":null,"abstract":"<div><div>Plastic flow behavior and strain rate sensitivity, <em>S</em>, of Fe-15Cr-15Ni (mass%) austenitic steel, alloyed with either hydrogen or carbon, were evaluated by tensile and stress relaxation tests at ambient temperature. The effects of these two interstitial elements on solid solution-hardening and thermally activated dislocation motion were compared in terms of <em>Haasen plot</em>—<em>S</em> versus flow stress. Both hydrogen and carbon exhibited solid solution-hardening of the same order of magnitude, increasing <em>S</em> proportionally with their concentrations. However, their ability to increase <em>S</em> was distinct. Hydrogen caused a much steeper increase in <em>S</em>, acting as extremely localized obstacles resisting dislocation motion. In contrast, despite exhibiting comparable solid solution-hardening, carbon led to an order of magnitude smaller increase in <em>S</em> than hydrogen. This result demonstrates a relatively long-range and less rate-sensitive nature of carbon, which is totally different from hydrogen in its obstacle character.</div></div>","PeriodicalId":423,"journal":{"name":"Scripta Materialia","volume":"273 ","pages":"Article 117111"},"PeriodicalIF":5.6,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145621339","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Thermoelectric properties of semiconducting approximant crystals in the Al–Ge–Ru system Al-Ge-Ru体系中半导体近似晶体的热电性质
IF 5.6 2区 材料科学
Scripta Materialia Pub Date : 2026-03-01 Epub Date: 2025-11-17 DOI: 10.1016/j.scriptamat.2025.117100
Yutaka Iwasaki , Yasuhiro Niwa , Koichi Kitahara , Kaoru Kimura , Ryuji Tamura
{"title":"Thermoelectric properties of semiconducting approximant crystals in the Al–Ge–Ru system","authors":"Yutaka Iwasaki ,&nbsp;Yasuhiro Niwa ,&nbsp;Koichi Kitahara ,&nbsp;Kaoru Kimura ,&nbsp;Ryuji Tamura","doi":"10.1016/j.scriptamat.2025.117100","DOIUrl":"10.1016/j.scriptamat.2025.117100","url":null,"abstract":"<div><div>Semiconducting quasicrystals and their approximant crystals (ACs) have attracted significant attention because of their potential applications as thermoelectric materials. Herein, we report the synthesis of a semiconducting AC in the Al–Ge–Ru system and its thermoelectric properties. The Al–Ge–Ru AC exhibited a band gap of approximately 0.25 eV. Notably, we observed a negative Seebeck coefficient, which reached a maximum magnitude of 200 µV K<sup>−1</sup>, marking the first example of an n-type semiconducting AC. The Al<sub>74</sub>Ge<sub>4</sub>Ru<sub>22</sub> AC exhibiting degenerate semiconductor behavior reached a dimensionless figure of merit of 0.28 at a peak temperature of 473 K. This represents the highest figure of merit achieved to date for a quasicrystalline-based thermoelectric material.</div></div>","PeriodicalId":423,"journal":{"name":"Scripta Materialia","volume":"273 ","pages":"Article 117100"},"PeriodicalIF":5.6,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145577437","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Microstructural transition across interlayer ultrasonic impact peened interfaces in hybrid additive manufacturing of 316L stainless steel 混合增材制造316L不锈钢层间超声冲击强化界面的微观组织转变
IF 5.6 2区 材料科学
Scripta Materialia Pub Date : 2026-03-01 Epub Date: 2025-11-19 DOI: 10.1016/j.scriptamat.2025.117107
Kossi Loic M. Avegnon , Ronan Henry , Michael Sealy , Fabrice Barbe , Benoit Vieille
{"title":"Microstructural transition across interlayer ultrasonic impact peened interfaces in hybrid additive manufacturing of 316L stainless steel","authors":"Kossi Loic M. Avegnon ,&nbsp;Ronan Henry ,&nbsp;Michael Sealy ,&nbsp;Fabrice Barbe ,&nbsp;Benoit Vieille","doi":"10.1016/j.scriptamat.2025.117107","DOIUrl":"10.1016/j.scriptamat.2025.117107","url":null,"abstract":"<div><div>While additive manufacturing generally involves building components layer by layer, hybrid additive manufacturing in this context refers to a process that combines printing with interlayer cold working. Although cold working induces plastic deformation, the subsequent microstructural evolution in the newly printed layers is largely dictated by the thermal input of the printing process. Hence, the objective of this study was to characterize the microstructural evolution at the interface of interlayer ultrasonic impact peened 316 L stainless steel manufactured by laser powder bed fusion. Ultrasonic treatment was applied intensively over five consecutive layers, and the resulting interface was mapped through microstructural analysis and hardness testing across multiple length scales. The results revealed a succession from highly deformed grains in treated regions to recrystallized equiaxed structures, and finally remelted columnar features in the subsequent layers. This transition was driven by the rapid cooling rate and steep thermal gradient of the printing process.</div></div>","PeriodicalId":423,"journal":{"name":"Scripta Materialia","volume":"273 ","pages":"Article 117107"},"PeriodicalIF":5.6,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145577408","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
RECIPIENTS OF THE 2024 ACTA MATERIALIA, INC. STUDENT AWARDS 2024年材料学报的接受者,inc。学生奖
IF 5.6 2区 材料科学
Scripta Materialia Pub Date : 2026-03-01 Epub Date: 2025-11-21 DOI: 10.1016/j.scriptamat.2025.117091
{"title":"RECIPIENTS OF THE 2024 ACTA MATERIALIA, INC. STUDENT AWARDS","authors":"","doi":"10.1016/j.scriptamat.2025.117091","DOIUrl":"10.1016/j.scriptamat.2025.117091","url":null,"abstract":"","PeriodicalId":423,"journal":{"name":"Scripta Materialia","volume":"273 ","pages":"Article 117091"},"PeriodicalIF":5.6,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145690475","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Direct atomic observation of large-angle lattice rotation in Cu3Pd Cu3Pd中大角度晶格旋转的直接原子观察
IF 5.6 2区 材料科学
Scripta Materialia Pub Date : 2026-03-01 Epub Date: 2025-11-13 DOI: 10.1016/j.scriptamat.2025.117099
Yujie Song , Huichao Duan , Tao Zheng , Qianning Dai , Kui Du
{"title":"Direct atomic observation of large-angle lattice rotation in Cu3Pd","authors":"Yujie Song ,&nbsp;Huichao Duan ,&nbsp;Tao Zheng ,&nbsp;Qianning Dai ,&nbsp;Kui Du","doi":"10.1016/j.scriptamat.2025.117099","DOIUrl":"10.1016/j.scriptamat.2025.117099","url":null,"abstract":"<div><div>Grain rotation plays a critical role in grain growth of nanocrystalline materials, yet the underlying atomic-scale mechanisms, especially for large-angle rotation, remain poorly understood. Here, we report a 62.4° lattice rotation in Cu<sub>3</sub>Pd nanocrystals by <em>in-situ</em> atomic resolution transmission electron microscopy (TEM) images. This rotation proceeds via a sequential two-step mechanism: double-shear-driven structural transition followed by atomic shuffling. The large-angle rotation suggests a potential coalescence between adjacent grains and provides an atomic-scale explanation for abnormal grain growth in intermetallic nanocrystals. These experiments establish a novel shear-shuffle paradigm for grain rotation, offering a new framework for understanding the structural evolution and nanocrystal coalescence.</div></div>","PeriodicalId":423,"journal":{"name":"Scripta Materialia","volume":"273 ","pages":"Article 117099"},"PeriodicalIF":5.6,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145527333","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Acta Biomaterialia Gold Medal 2026 生物材料学报金牌2026
IF 5.6 2区 材料科学
Scripta Materialia Pub Date : 2026-03-01 Epub Date: 2025-11-06 DOI: 10.1016/j.scriptamat.2025.117031
{"title":"Acta Biomaterialia Gold Medal 2026","authors":"","doi":"10.1016/j.scriptamat.2025.117031","DOIUrl":"10.1016/j.scriptamat.2025.117031","url":null,"abstract":"","PeriodicalId":423,"journal":{"name":"Scripta Materialia","volume":"273 ","pages":"Article 117031"},"PeriodicalIF":5.6,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145690548","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Acta Materialia Gold Medal 2026 《材料学报》第2026期
IF 5.6 2区 材料科学
Scripta Materialia Pub Date : 2026-03-01 Epub Date: 2025-11-05 DOI: 10.1016/j.scriptamat.2025.117029
{"title":"Acta Materialia Gold Medal 2026","authors":"","doi":"10.1016/j.scriptamat.2025.117029","DOIUrl":"10.1016/j.scriptamat.2025.117029","url":null,"abstract":"","PeriodicalId":423,"journal":{"name":"Scripta Materialia","volume":"273 ","pages":"Article 117029"},"PeriodicalIF":5.6,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145690547","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Pressure-induced phase transitions of amorphous silicon nanoparticles 非晶硅纳米颗粒的压力诱导相变
IF 5.6 2区 材料科学
Scripta Materialia Pub Date : 2026-03-01 Epub Date: 2025-11-21 DOI: 10.1016/j.scriptamat.2025.117106
Haotian Zhu , Shuai Liu , Di Peng , Fujun Lan , Yuxin Liu , Guangrun Zhong , Hongbo Lou , Qiaoshi Zeng , Zhidan Zeng
{"title":"Pressure-induced phase transitions of amorphous silicon nanoparticles","authors":"Haotian Zhu ,&nbsp;Shuai Liu ,&nbsp;Di Peng ,&nbsp;Fujun Lan ,&nbsp;Yuxin Liu ,&nbsp;Guangrun Zhong ,&nbsp;Hongbo Lou ,&nbsp;Qiaoshi Zeng ,&nbsp;Zhidan Zeng","doi":"10.1016/j.scriptamat.2025.117106","DOIUrl":"10.1016/j.scriptamat.2025.117106","url":null,"abstract":"<div><div>Amorphous silicon (a-Si) plays a significant role in various modern technologies. Therefore, understanding its stability is of both fundamental and technological importance. While pressure-induced phase transitions in a-Si have been extensively studied, the effect of domain size remains unclear. In this study, we synthesized amorphous silicon nanoparticles (a-SiNPs) with an average size of ∼9 nm and investigated their pressure-induced phase transitions using <em>in situ</em> high-pressure Raman spectroscopy and synchrotron X-ray diffraction. These results reveal that a-SiNPs transform into β-Sn phase at ∼10.8 GPa, rather than a previously reported high-density amorphous phase. Upon decompression, the β-Sn phase reverts to a-Si. The phase transition pathway and transition pressure are similar to those observed in bulk a-Si, indicating that domain size is not a determining factor for inducing polyamorphism in a-Si. These findings bring new insights into the thermodynamics and kinetics of phase transitions in a-SiNPs and provide experimental constraints for theoretical studies of a-Si.</div></div>","PeriodicalId":423,"journal":{"name":"Scripta Materialia","volume":"273 ","pages":"Article 117106"},"PeriodicalIF":5.6,"publicationDate":"2026-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145577410","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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