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Realization of elastic Weyl semimetal phases with skyrmion spin textures 用skyrmion自旋织构实现弹性Weyl半金属相。
IF 21.1 1区 综合性期刊
Science Bulletin Pub Date : 2026-04-15 Epub Date: 2026-02-26 DOI: 10.1016/j.scib.2026.02.039
Yuang Pan , Liang Si , Miao Yang , Ning Han , Li Zhang , Qiaolu Chen , Rui Zhao , Fujia Chen , Yudong Ren , Wenhao Li , Yuze Hu , Mingyu Tong , Xinrui Li , Junyao Wu , Ronghao Bao , Weiqiu Chen , Yang Long , Bin Wu , Hongsheng Chen , Baile Zhang , Yihao Yang
{"title":"Realization of elastic Weyl semimetal phases with skyrmion spin textures","authors":"Yuang Pan , Liang Si , Miao Yang , Ning Han , Li Zhang , Qiaolu Chen , Rui Zhao , Fujia Chen , Yudong Ren , Wenhao Li , Yuze Hu , Mingyu Tong , Xinrui Li , Junyao Wu , Ronghao Bao , Weiqiu Chen , Yang Long , Bin Wu , Hongsheng Chen , Baile Zhang , Yihao Yang","doi":"10.1016/j.scib.2026.02.039","DOIUrl":"10.1016/j.scib.2026.02.039","url":null,"abstract":"","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":"71 7","pages":"Pages 1602-1606"},"PeriodicalIF":21.1,"publicationDate":"2026-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147455115","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Young adulthood adiposity in relation to all-cause and cause-specific mortality: a prospective study of 0.5 million Chinese adults 青年肥胖与全因和特定原因死亡率的关系:一项50万中国成年人的前瞻性研究。
IF 21.1 1区 综合性期刊
Science Bulletin Pub Date : 2026-04-15 Epub Date: 2026-02-26 DOI: 10.1016/j.scib.2026.02.036
Lei Fan , Andri Iona , Shixian Feng , Gang Zhou , Huarong Sun , Pang Yao , Canqing Yu , Yiping Chen , Dianjianyi Sun , Pei Pei , Ling Yang , Mingshu Yan , Xiaoming Yang , Jun Lv , Junshi Chen , Liming Li , Zhengming Chen , Huaidong Du
{"title":"Young adulthood adiposity in relation to all-cause and cause-specific mortality: a prospective study of 0.5 million Chinese adults","authors":"Lei Fan ,&nbsp;Andri Iona ,&nbsp;Shixian Feng ,&nbsp;Gang Zhou ,&nbsp;Huarong Sun ,&nbsp;Pang Yao ,&nbsp;Canqing Yu ,&nbsp;Yiping Chen ,&nbsp;Dianjianyi Sun ,&nbsp;Pei Pei ,&nbsp;Ling Yang ,&nbsp;Mingshu Yan ,&nbsp;Xiaoming Yang ,&nbsp;Jun Lv ,&nbsp;Junshi Chen ,&nbsp;Liming Li ,&nbsp;Zhengming Chen ,&nbsp;Huaidong Du","doi":"10.1016/j.scib.2026.02.036","DOIUrl":"10.1016/j.scib.2026.02.036","url":null,"abstract":"<div><div>Obesity is a well-established risk factor for early death, but the exact shapes of associations between young adulthood body mass index (BMI) and mortality in later life were not well characterised. Using data from the prospective China Kadoorie Biobank study of 430,373 participants (∼57% being women, with a median follow-up duration of 12 years), Cox regression analysis was performed to yield adjusted hazard ratios (HRs) relating BMI at ∼25 years old (BMI<sub>25</sub>) with different mortality outcomes including total mortality (<em>n</em> = 36,814), cardiovascular mortality (<em>n</em> = 13,620), cancer mortality (<em>n</em> = 13,394) and respiratory mortality (<em>n</em> = 2929). Mean BMI<sub>25</sub> of participants was 21.9 (SD = 2.5) kg/m<sup>2</sup>, and 1.9% participants were obese at young adulthood (i.e., BMI<sub>25</sub> ≥28.0 kg/m<sup>2</sup>). Independent of baseline BMI, higher BMI<sub>25</sub> was associated with much higher levels of blood glucose and diabetes prevalence at baseline. After adjusting for potential confounders e.g., age, smoking, and baseline measured BMI, BMI<sub>25</sub> had a strong positive log-linear association with all above-mentioned mortality outcomes, those being obese at young adulthood had a HR of 1.85 (95% CI: 1.75–1.95), 1.85 (1.71–2.00), 1.40 (1.26–1.56) and 2.34 (1.96–2.81), respectively, compared with participants having BMI<sub>25</sub> of 18.5–20.0 kg/m<sup>2</sup>. The association with cancer mortality was more pronounced in men than in women, but no such heterogeneity was observed for total, cardiovascular diseases (CVD), and respiratory mortality. To conclude, the observed strong monotonically positive associations between young adulthood BMI and various mortality outcomes, independent of BMI in later life, support the need for early and stringent body weight control to prevent early death.</div></div>","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":"71 7","pages":"Pages 1760-1770"},"PeriodicalIF":21.1,"publicationDate":"2026-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147430159","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Single-frame motion vector imaging with phonon-engineered perovskite optoelectronic synapses for neuromorphic visual perception 声子工程钙钛矿光电突触单帧运动矢量成像用于神经形态视觉感知。
IF 21.1 1区 综合性期刊
Science Bulletin Pub Date : 2026-04-15 Epub Date: 2026-01-21 DOI: 10.1016/j.scib.2026.01.047
Hao Wang , Tianhua Liu , Yongle Pan , Junjie Zhou , Junfang Wang , Xu Wang , Shiwei Zhang , Enhao Cui , Shuyang Wang , Ziquan Yuan , Zengsheng Li , Yashuai Qi , Le Huang , Yang Chai , Xiangyue Meng
{"title":"Single-frame motion vector imaging with phonon-engineered perovskite optoelectronic synapses for neuromorphic visual perception","authors":"Hao Wang ,&nbsp;Tianhua Liu ,&nbsp;Yongle Pan ,&nbsp;Junjie Zhou ,&nbsp;Junfang Wang ,&nbsp;Xu Wang ,&nbsp;Shiwei Zhang ,&nbsp;Enhao Cui ,&nbsp;Shuyang Wang ,&nbsp;Ziquan Yuan ,&nbsp;Zengsheng Li ,&nbsp;Yashuai Qi ,&nbsp;Le Huang ,&nbsp;Yang Chai ,&nbsp;Xiangyue Meng","doi":"10.1016/j.scib.2026.01.047","DOIUrl":"10.1016/j.scib.2026.01.047","url":null,"abstract":"","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":"71 7","pages":"Pages 1612-1616"},"PeriodicalIF":21.1,"publicationDate":"2026-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146117401","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Conjugated organic polymer enables external-sacrificial-agent-free photocatalytic uranium extraction with efficiency boosted by oxygen pre-activation 共轭有机聚合物可以实现无外部牺牲剂的光催化铀萃取,并通过氧预活化提高了效率。
IF 21.1 1区 综合性期刊
Science Bulletin Pub Date : 2026-04-15 Epub Date: 2026-02-13 DOI: 10.1016/j.scib.2026.02.024
Xuefeng Tian , Jipeng Li , Xuewen Cao , Jiacheng Zhang , Rui Huang , Peng Lin , Ning Wang , Yihui Yuan
{"title":"Conjugated organic polymer enables external-sacrificial-agent-free photocatalytic uranium extraction with efficiency boosted by oxygen pre-activation","authors":"Xuefeng Tian ,&nbsp;Jipeng Li ,&nbsp;Xuewen Cao ,&nbsp;Jiacheng Zhang ,&nbsp;Rui Huang ,&nbsp;Peng Lin ,&nbsp;Ning Wang ,&nbsp;Yihui Yuan","doi":"10.1016/j.scib.2026.02.024","DOIUrl":"10.1016/j.scib.2026.02.024","url":null,"abstract":"<div><div>Efficient extraction of uranium from seawater is critical for sustainable nuclear energy. Photocatalysis offers a promising route, while the reliance on sacrificial agents and the limited extraction capacity necessitate the development of new photocatalysts. Here, we report the first conjugated organic polymer (COP), BB-COP-AO, that enables external-sacrificial-agent-free photocatalytic uranium extraction from natural seawater. Rational incorporation of benzothiadiazole and pyridine units optimizes the band structure, enhances intramolecular donor–acceptor interactions, and facilitates charge separation, endowing it with high photocatalytic activity. Pyridine nitrogen atoms benefit dissolved oxygen adsorption and pre-activation to promote ·O<sub>2</sub><sup>−</sup> generation, boosting the uranium recovery efficiency. Furthermore, the suitable valence band enables photogenerated holes to oxidize H<sub>2</sub>O to H<sub>2</sub>O<sub>2</sub>, thereby eliminating the need for external sacrificial agents. Concurrently, amidoxime functionalities ensure selective uranyl binding. Consequently, BB-COP-AO drives selective conversion of the uranyl ions into highly stable metastudtite via a dual-pathway mechanism coupling dissolved oxygen activation and water oxidation. Benefiting from these synergistic effects, BB-COP-AO exhibits an outstanding uranium extraction capacity of 19.80 mg g<sup>−1</sup> in natural seawater within 7 d, along with excellent selectivity and recyclability. This work expands the application scope of COP-based materials and offers a generalizable molecular design strategy for developing multifunctional photocatalysts toward sustainable uranium recovery from seawater.</div></div>","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":"71 7","pages":"Pages 1686-1694"},"PeriodicalIF":21.1,"publicationDate":"2026-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147371986","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Non-progressive orogenesis of the Southern Tibetan Plateau. 青藏高原南部的非进动造山作用。
IF 21.1 1区 综合性期刊
Science Bulletin Pub Date : 2026-04-15 DOI: 10.1016/j.scib.2026.04.033
Xiaoyu Guo, Hengcheng Ying, Lin Chen, Rui Gao, Xiaofan Deng, Zhanwu Lu, Hongda Liang, Bo Xiang, Michael Murphy, Wenhui Li, Xiao Xu
{"title":"Non-progressive orogenesis of the Southern Tibetan Plateau.","authors":"Xiaoyu Guo, Hengcheng Ying, Lin Chen, Rui Gao, Xiaofan Deng, Zhanwu Lu, Hongda Liang, Bo Xiang, Michael Murphy, Wenhui Li, Xiao Xu","doi":"10.1016/j.scib.2026.04.033","DOIUrl":"https://doi.org/10.1016/j.scib.2026.04.033","url":null,"abstract":"<p><p>The Lhasa Terrane (LT), a ∼2000-km-long orogenic belt within the Neo-Tethyan tectonic domain, constitutes the southern Tibetan Plateau (STP). Geochronological data reveal non-progressive (multi-phase) surface uplift, initiating in the central LT rather than the southern LT adjacent to the collisional front. To resolve the geodynamic drivers of this uplift pattern, we present an integrated analysis of a 345-km-long N-S deep seismic reflection profile traversing the entire LT. This unified transect reveals a critical structural continuity invisible to isolated studies: the non-reflective crust in the southern LT transitions to a continuous north-dipping crystalline basement wedge that tapers progressively northward from the central to northern LT. Integration of multi-disciplinary data with geodynamic modeling supports a three-phase orogenic evolution, suggesting that while the evolving Neo-Tethyan slab dynamics and subsequent Indian collision provided the external geodynamic drivers, the inherited across-strike crustal strength heterogeneity acted as the internal template. Initially, early-stage subduction induced northward basement tilting and early uplift. Subsequently, slab rollback (<70 Ma) drove juvenile crustal accretion and magmatic softening in the southern LT, causing delayed uplift upon Indian indentation. Finally, Late Oligocene-Miocene passive roof thrust systems modified the relief. These validated processes demonstrate that external tectonic forcing interacted with inherited crustal structures to fundamentally affect the spatial progression of thickening, thereby establishing the STP's non-progressive orogenic framework.</p>","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":21.1,"publicationDate":"2026-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147758932","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Anchoring phase change interface enhances solar thermal energy storage. 锚定相变界面增强了太阳能热能的储存。
IF 21.1 1区 综合性期刊
Science Bulletin Pub Date : 2026-04-14 DOI: 10.1016/j.scib.2026.04.024
Qiao Xu, Jingwen Zhu, Yan Wang, Xianglei Liu, Tao Wang, Jianguo Wang, Shushan Lv, Yongliang Li
{"title":"Anchoring phase change interface enhances solar thermal energy storage.","authors":"Qiao Xu, Jingwen Zhu, Yan Wang, Xianglei Liu, Tao Wang, Jianguo Wang, Shushan Lv, Yongliang Li","doi":"10.1016/j.scib.2026.04.024","DOIUrl":"https://doi.org/10.1016/j.scib.2026.04.024","url":null,"abstract":"<p><p>Solar thermal energy storage based on phase change materials (PCMs) provides a compact, near-isothermal pathway toward decarbonizing thermal energy supplies. However, the intrinsic recession of the solid-liquid interface away from the irradiated surface leads to gradually increasing thermal resistance and decaying charging rate with time. To address this challenge, we demonstrate that anchoring the phase change interface achieves rapid, efficient, and continuous solar thermal charging. This is enabled by dynamically circulating photothermal core-shell composite phase change particles (CPCPs) to continuously renew the irradiated surface. Scalable CPCPs, fabricated via extrusion-spheronization, consist of a MnFe<sub>2</sub>O<sub>4</sub> photothermal shell and an MgO/h-BN/NaCl-KCl core integrating broadband photon absorption with high thermal conductivity within a single particle. The MnFe<sub>2</sub>O<sub>4</sub> shell delivers a solar-weighted absorptance of 91.1%, facilitated by near-surface photon confinement and internal multiple scattering. Within the core, a percolated MgO skeleton combined with in-plane h-BN phonon transport pathways forms a hierarchical ceramic network. The interfacial phonon-spectrum overlap in this structure reduces Kapitza resistance, elevating the effective thermal conductivity to 6.84 W m<sup>-1</sup> K<sup>-1</sup>, while maintaining a high energy storage density of 844.7 kJ kg<sup>-1</sup>. By matching the incident solar flux with particle stream mass flow rates, the system attains a charging power of 0.54 kW under 1.08 kW solar input. This yields a solar thermal storage efficiency of 49.7%, a 26-fold improvement over conventional diffusion-limited approaches (1.9%). This work introduces a paradigm shift from the conventional diffusion-limited \"material-static, interface-retreating\" mode to \"material-moving, interface-anchoring\" mode, leading to rapid, efficient, and continuous solar thermal energy storage.</p>","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":21.1,"publicationDate":"2026-04-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147758981","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Quantum tunneling effects on hydrogen transport in lanthanum trihydrides. 三氢化镧中氢输运的量子隧穿效应。
IF 21.1 1区 综合性期刊
Science Bulletin Pub Date : 2026-04-14 DOI: 10.1016/j.scib.2026.04.026
Chunlei Yang, Luhao Zhang, Cui Zhang, Qiuhao Xu, Qunfang Gu, Yunzhe Jia, Wei Fang, Sheng Meng, Enge Wang
{"title":"Quantum tunneling effects on hydrogen transport in lanthanum trihydrides.","authors":"Chunlei Yang, Luhao Zhang, Cui Zhang, Qiuhao Xu, Qunfang Gu, Yunzhe Jia, Wei Fang, Sheng Meng, Enge Wang","doi":"10.1016/j.scib.2026.04.026","DOIUrl":"https://doi.org/10.1016/j.scib.2026.04.026","url":null,"abstract":"<p><p>Ionic conductivity in solids is a topic of great interest in the fields of physics, materials science, and energy applications. Previous studies have primarily focused on the activation energy of ion transport based on classical transition state theory, lacking considerations from the perspective of nuclear quantum effects. Herein, by considering the effects of zero-point energy and quantum tunneling, we examine the quantum behaviors of hydrogen migration in lanthanum trihydrides (LaH<sub>3</sub>), through the two dominant pathways-concerted migration and single-ion migration. Our first-principles calculations based on instanton rate theory indicate that the quantum rate constants diverge significantly from their classical counterparts at low temperatures. We predict that quantum tunneling becomes dominant over thermal diffusion for concerted hydrogen migration at liquid nitrogen temperature, and emerges even at room temperature when concerted transport is suppressed. We also demonstrate the tuning of migration rates by strain, and the sensitivity of the quantum tunneling rate to the energy barrier geometry. Our findings depict a complete quantum picture of hydrogen transport in lanthanide hydrides and provide a new perspective on ionic conductivity of solid materials.</p>","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":21.1,"publicationDate":"2026-04-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147758941","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Exploring geographical modal and its implications to support geographical integration. 探索地理模态及其支持地理整合的意义。
IF 21.1 1区 综合性期刊
Science Bulletin Pub Date : 2026-04-11 DOI: 10.1016/j.scib.2026.04.011
Zhuo Sun, Tianyu Sheng, Kai Wu, Peilong Ma, Zihao Tang, Dichen Liu, Min Chen, Guonian Lü
{"title":"Exploring geographical modal and its implications to support geographical integration.","authors":"Zhuo Sun, Tianyu Sheng, Kai Wu, Peilong Ma, Zihao Tang, Dichen Liu, Min Chen, Guonian Lü","doi":"10.1016/j.scib.2026.04.011","DOIUrl":"https://doi.org/10.1016/j.scib.2026.04.011","url":null,"abstract":"","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":21.1,"publicationDate":"2026-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147758830","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
B-site regulated Ru-based pyrochlores for acidic water oxidation. b位调控的ru基焦绿石用于酸性水氧化。
IF 21.1 1区 综合性期刊
Science Bulletin Pub Date : 2026-04-11 DOI: 10.1016/j.scib.2026.04.025
Yueying Yan, Yang Yang, Bohan Yao, Yuting Chen, Huanhuan Xing, Yanchao Xu, Dongxu Jiao, Zhicai Xing, Dewen Wang, Xiurong Yang
{"title":"B-site regulated Ru-based pyrochlores for acidic water oxidation.","authors":"Yueying Yan, Yang Yang, Bohan Yao, Yuting Chen, Huanhuan Xing, Yanchao Xu, Dongxu Jiao, Zhicai Xing, Dewen Wang, Xiurong Yang","doi":"10.1016/j.scib.2026.04.025","DOIUrl":"https://doi.org/10.1016/j.scib.2026.04.025","url":null,"abstract":"<p><p>Ruthenium (Ru)-based pyrochlores have shown significant potential for oxygen evolution reaction (OER) in acidic media. However, their further application is severely limited by insufficient structural stability and moderate activity under harsh acidic conditions. Herein, density functional theory (DFT) calculations were performed to investigate the effects of 3d transition metals doping on the intrinsic activity and stability of Y<sub>2</sub>Ru<sub>2</sub>O<sub>7-</sub><sub>δ</sub>. Guided by theoretical predictions, a series of Y<sub>2</sub>Ru<sub>2-</sub><sub>x</sub>M<sub>x</sub>O<sub>7-</sub><sub>δ</sub> (M = Sc, Ti, V, Cr, Mn, Fe, Co, Ni, Cu, and Zn) materials was synthesized, and Y<sub>2</sub>Ru<sub>1.8</sub>Zn<sub>0.2</sub>O<sub>7-</sub><sub>δ</sub> (YRZO) was identified as the optimal candidate. Both theoretical and experimental results demonstrate that Zn doping and cation vacancies synergistically optimize the adsorption energies of OER intermediates and stabilize high-valence Ru sites in YRZO, thereby accelerating reaction kinetics and reducing OER overpotentials. Meanwhile, Zn incorporation enhances the covalency of Ru-O bonds, which not only suppresses Ru dissolution but also delays the formation of surface reconstruction layers, thus significantly improving the long-term durability of the electrocatalyst. In situ characterizations verify that the OER process on YRZO proceeds via the adsorption evolution mechanism (AEM). The optimized YRZO exhibits a low overpotential of 272 mV at 10 mA cm<sup>-2</sup> and can reach 1000 mA cm<sup>-2</sup> at 1.597 V in a proton exchange membrane water electrolysis (PEMWE) device with exceptional stability over 1000 h. This work provides a rational strategy for designing highly active and stable acidic OER electrocatalysts by 3d transition metal doping of Y<sub>2</sub>Ru<sub>2</sub>O<sub>7-</sub><sub>δ</sub>-based pyrochlores.</p>","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":21.1,"publicationDate":"2026-04-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147759013","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Efficient paired indirect electrosynthesis of adipic acid from phenol using polyoxometalate electrolytes. 用多金属氧酸盐电解质从苯酚中高效成对间接电合成己二酸。
IF 21.1 1区 综合性期刊
Science Bulletin Pub Date : 2026-04-10 DOI: 10.1016/j.scib.2026.04.023
Wensi Tang, Zhongling Lang, Ruiqi Yao, Tianyu Qiu, Yonghui Wang, Huaqiao Tan, Wei Liu, Zhen Sun, Zhichao Sun, Yingqi Li, Yangguang Li, Yulin Deng
{"title":"Efficient paired indirect electrosynthesis of adipic acid from phenol using polyoxometalate electrolytes.","authors":"Wensi Tang, Zhongling Lang, Ruiqi Yao, Tianyu Qiu, Yonghui Wang, Huaqiao Tan, Wei Liu, Zhen Sun, Zhichao Sun, Yingqi Li, Yangguang Li, Yulin Deng","doi":"10.1016/j.scib.2026.04.023","DOIUrl":"https://doi.org/10.1016/j.scib.2026.04.023","url":null,"abstract":"","PeriodicalId":421,"journal":{"name":"Science Bulletin","volume":" ","pages":""},"PeriodicalIF":21.1,"publicationDate":"2026-04-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147758773","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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