Journal of Environmental Management最新文献

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Integrated impacts of land use changes and climate dynamics on hydrological components in the Munneru River basin, India.
IF 8 2区 环境科学与生态学
Journal of Environmental Management Pub Date : 2025-03-27 DOI: 10.1016/j.jenvman.2025.125096
Kotapati Narayana Loukika, Venkata Reddy Keesara, Eswar Sai Buri, Venkataramana Sridhar, Bloodless Dzwairo, Suzana Montenegro
{"title":"Integrated impacts of land use changes and climate dynamics on hydrological components in the Munneru River basin, India.","authors":"Kotapati Narayana Loukika, Venkata Reddy Keesara, Eswar Sai Buri, Venkataramana Sridhar, Bloodless Dzwairo, Suzana Montenegro","doi":"10.1016/j.jenvman.2025.125096","DOIUrl":"https://doi.org/10.1016/j.jenvman.2025.125096","url":null,"abstract":"<p><p>Effective water management and adaptation plans depend on understanding how changing Land Use and Land Cover (LU&LC) and Climate Change (CC) will affect future spatiotemporal water availability in a river basin. However, a major challenge in hydrological modelling is accurately integrating both LU&LC and climate projections to address uncertainties in future water availability. This study evaluates how LU&LC and climate change together affect hydrology of the basin for future climate change scenarios. The future LU&LCs are projected using the Dyna-CLUE model for three user-defined scenarios such as past trend, drastic change in built-up and barren land, and restricted agricultural land. CMIP6 climate data was used under three scenarios SSP245, SSP370 and SSP585 which was then ensemble using the Reliable Ensemble Averaging (REA) method at each grid for both precipitation and temperature. The SUFI2 algorithm in SWAT-CUP tool is used to calibrate and validate the SWAT model for the years 1983-2017. The average monthly streamflow is projected for both LU&LC and SSP climate change scenarios during the baseline period (1983-2014), as well as for three future periods.: the near-future (2025-2040), mid-future (2041-2070) and far-future (2071-2100). Streamflow, total aquifer recharge and evapotranspiration increase in the three selected future periods when compared to baseline period in all three SSP scenarios. When combining both LU&LC and climate change scenarios, the LU&LC scenario 2 exhibits more change in streamflow, surface runoff, total aquifer recharge compared to the climate change scenario alone. In the near-future the streamflow was increased the most in the months of July by 56.13 % for climate change scenario SSP370 with LU&LC scenario 2 in the near-future period compared to the baseline period. Similarly, in the mid-future, the maximum increase was observed in June by 67.52 % for the combined impact of SSP585 and LU&LC scenario 2. In the far-future period, the maximum increase is in the month of July by 133.4 % for the combined impact of SSP585 and LU&LC2. Increasing precipitation under future climate scenarios is expected to significantly enhance streamflows, particularly from August to November, with October consistently experiencing peak flows, highlighting the need for improved flood management strategies in response to intensifying hydrological extremes. This study addresses key methodological challenges by integrating dynamic LU&LC projections, ensemble climate model data processing, and advanced calibration techniques to improve hydrological predictions. In light of projected LU&LC under climate change scenarios, the findings can be used to plan and develop short-term and long-term integrated water management strategies for the basin. Other basins in comparable physiographic regions all over the globe can use this methodology.</p>","PeriodicalId":356,"journal":{"name":"Journal of Environmental Management","volume":"380 ","pages":"125096"},"PeriodicalIF":8.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143741713","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Development of a graphene based anodic membrane for efficient electrocatalytic oxidation of typical antibiotics from water.
IF 8 2区 环境科学与生态学
Journal of Environmental Management Pub Date : 2025-03-27 DOI: 10.1016/j.jenvman.2025.125131
Yulu Shi, Wangli Yao, Xiaotie Shen, Ruiyi Li, Baoliang Chen, Xiaoying Zhu
{"title":"Development of a graphene based anodic membrane for efficient electrocatalytic oxidation of typical antibiotics from water.","authors":"Yulu Shi, Wangli Yao, Xiaotie Shen, Ruiyi Li, Baoliang Chen, Xiaoying Zhu","doi":"10.1016/j.jenvman.2025.125131","DOIUrl":"https://doi.org/10.1016/j.jenvman.2025.125131","url":null,"abstract":"<p><p>Traditional membrane separation processes were ineffective at degrading pollutant molecules, while catalytic reactors often faced inefficiencies due to their inability to simultaneously retain and concentrate reactant molecules. To address these challenges, we synthesized an anodic electrocatalyst (Ti<sub>4</sub>O<sub>7</sub>/SnO<sub>2</sub>-Sb) and combined it with reduced graphene oxide (rGO) sheets to develop a high-performance anodic electrocatalytic membrane (AOM). The AOM's tailored interlayer spacing facilitated simultaneous concentration and electrooxidation of antibiotic pollutants, enabling efficient degradation. At a permeate flux of 7.4 L m<sup>-2</sup>·h<sup>-1</sup>, the AOM achieved ∼95 % degradation of chloramphenicol (CAP, 20 mg L<sup>-1</sup>). The corresponding degradation rate constant (k) of 199.70 min<sup>-1</sup> was two orders of magnitude higher than that of a conventional reactor without retention capability (1.06 min<sup>-1</sup>). Moreover, the AOM exhibited exceptional energy efficiency and long-term stability, highlighting its potential for advanced wastewater treatment. This innovative design, which leveraged pollutant concentration via the size-sieving effects of confined interlayer spaces, marked a significant advancement in high-performance water treatment technologies.</p>","PeriodicalId":356,"journal":{"name":"Journal of Environmental Management","volume":"380 ","pages":"125131"},"PeriodicalIF":8.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143741785","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Regeneration of spent NCM622 into high performance cathode materials with exposed {010} planes via an efficient closed-loop recycling strategy.
IF 8 2区 环境科学与生态学
Journal of Environmental Management Pub Date : 2025-03-27 DOI: 10.1016/j.jenvman.2025.125051
Yongfan Xie, Ya Sun, Fangya Guo, Youxiang Zhang
{"title":"Regeneration of spent NCM622 into high performance cathode materials with exposed {010} planes via an efficient closed-loop recycling strategy.","authors":"Yongfan Xie, Ya Sun, Fangya Guo, Youxiang Zhang","doi":"10.1016/j.jenvman.2025.125051","DOIUrl":"https://doi.org/10.1016/j.jenvman.2025.125051","url":null,"abstract":"<p><p>The recycling of the spent cathode materials of lithium-ion batteries is crucial to address the resource shortage and environmental pollution issues. In this article, the spent LiNi<sub>0.6</sub>Co<sub>0.2</sub>Mn<sub>0.2</sub>O<sub>2</sub> polycrystal cathode materials were regenerated to the monodispersed rod-shaped cathode materials with exposed {010} planes by a recycling method that combines the selective extraction and solid-state calcination. Such a selective extraction involves the treatment of spent cathode materials in an oxalic-urea mixed solution under hydrothermal reaction, which ensures the complete decomposition and reduction of spent cathode materials, further promoting the uniform precipitation of Ni, Co and Mn elements. The regenerated LiNi<sub>0.6</sub>Co<sub>0.2</sub>Mn<sub>0.2</sub>O<sub>2</sub> cathode materials are obtained by the subsequent calcination that exhibit excellent electrochemical performance in terms of Li<sup>+</sup> ions diffusivity, rate capability and long-term cycling performance. This deconstructive and remanufacturing recycling method could provide a guidance for the upcycling of spent ternary cathode materials.</p>","PeriodicalId":356,"journal":{"name":"Journal of Environmental Management","volume":"380 ","pages":"125051"},"PeriodicalIF":8.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143741733","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A critical review on bioaugmentation assisted anaerobic digestion for methane production: Performances, microbiome-functionalities and challenges.
IF 8 2区 环境科学与生态学
Journal of Environmental Management Pub Date : 2025-03-27 DOI: 10.1016/j.jenvman.2025.125127
Le Chen, Shuangshuang Li, Jiasheng Zhang, Feng Zhen, Zezhou Shang, Miao Yan, Yajie Zhang, Panyue Zhang, Yongming Sun, Ying Li
{"title":"A critical review on bioaugmentation assisted anaerobic digestion for methane production: Performances, microbiome-functionalities and challenges.","authors":"Le Chen, Shuangshuang Li, Jiasheng Zhang, Feng Zhen, Zezhou Shang, Miao Yan, Yajie Zhang, Panyue Zhang, Yongming Sun, Ying Li","doi":"10.1016/j.jenvman.2025.125127","DOIUrl":"https://doi.org/10.1016/j.jenvman.2025.125127","url":null,"abstract":"<p><p>Bioaugmentation technology is considered as a straightforward approach to improve anaerobic digestion performances, with advantages of high efficiency and sustainability. However, the mechanisms and challenges of bioaugmentation in anaerobic digestion have yet to been well reviewed. In this review, the advantages of bioaugmentation in anaerobic digestion are systematically identified and discussed, covering enhancing anaerobic digestion process, relieving toxic inhibition of ammonia, and overcoming limitation of psychrophilic anaerobic digestion. This review find that the underlying mechanisms of bioaugmentation enhancing anaerobic digestion are the improvement of microbial community metabolism activity, interspecies electron transfer, and microbial adaptability to environment stress. In addition, future challenges and research directions are discussed from theoretical and practical perspectives, including preparation of bioaugmentation microorganisms, immobilization of bioaugmentation microorganisms, and economic feasibility of bioaugmentation technology. This review contributes to understanding the positive effect of bioaugmentation on anaerobic digestion and promoting the applicability of bioaugmentation technology in anaerobic digestion.</p>","PeriodicalId":356,"journal":{"name":"Journal of Environmental Management","volume":"380 ","pages":"125127"},"PeriodicalIF":8.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143741929","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
An improved sulfur iodine cycle for sour gas purification and hydrogen fuel production for better environment.
IF 8 2区 环境科学与生态学
Journal of Environmental Management Pub Date : 2025-03-27 DOI: 10.1016/j.jenvman.2025.124921
Muhammad Ishaq, Ibrahim Dincer
{"title":"An improved sulfur iodine cycle for sour gas purification and hydrogen fuel production for better environment.","authors":"Muhammad Ishaq, Ibrahim Dincer","doi":"10.1016/j.jenvman.2025.124921","DOIUrl":"https://doi.org/10.1016/j.jenvman.2025.124921","url":null,"abstract":"<p><p>The conventional sulfur-iodine (S-I) thermochemical cycle developed for sour gas purification and hydrogen production from H<sub>2</sub>S stoichiometrically produces 2 moles of H<sub>2</sub>. The present work aims to develop an improved sulfur-iodine cycle, here called the five-step sulfur-iodine cycle, that replaces direct sulfur oxidation with a reaction between metallic oxygen carrier (OC) and elemental S to produce hydrogen. This new cycle does not only produce more H<sub>2</sub>, but also produces extra H<sub>2</sub>SO<sub>4</sub>. The process is followed by a hydrolysis reaction to regenerate OC and produce additional hydrogen. Hydrogen sulfide from the flue gas is considered the major feedstock for the developed system. The stoichiometry of the cycle is also studied to ensure that all the reactants follow the cyclic pathways. The cycle is then modeled in the Aspen Plus process simulation software under steady-state conditions, and a comprehensive thermodynamic analysis of the entire system is conducted using energy and exergy methods, evaluating energy and exergy efficiencies, as well as the exergy destruction rates of major components. Furthermore, several parameters are thoroughly examined to better investigate the system peformance. The proposed cycle demonstrates a significant improvement in hydrogen yield, and produces 4 moles of H<sub>2</sub> per mole of H<sub>2</sub>S. This represents a 100 % increase in hydrogen production efficiency compared to the conventional S-I cycle, which either produces 1 mole of H<sub>2</sub> or 2 moles of H<sub>2</sub> per mole of H<sub>2</sub>S. The hydrolysis and Claus reactors exhibit the highest exergy destruction rates accounting for 33.19 % and 16.69 % of the total exergy destruction rates, respectively. The energy and exergy efficiencies of the CBD section are found to be 72.89 % and 48.54 % respectively. The overall energy and exergy efficiencies of the new cycle configuration are found to be 74.72 % and 62.46 % respectively.</p>","PeriodicalId":356,"journal":{"name":"Journal of Environmental Management","volume":"380 ","pages":"124921"},"PeriodicalIF":8.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143741937","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Electric field as an activator of inoculated Bacillus clausii enhances humification during electric field-assisted aerobic composting.
IF 8 2区 环境科学与生态学
Journal of Environmental Management Pub Date : 2025-03-27 DOI: 10.1016/j.jenvman.2025.125132
Jiahuan Tang, Huan Mi, Chang Shen, Keren Ding, Shuqun Zhang, Huayuan Shangguan, Tao Fu, Jie Ye, Hao Lin
{"title":"Electric field as an activator of inoculated Bacillus clausii enhances humification during electric field-assisted aerobic composting.","authors":"Jiahuan Tang, Huan Mi, Chang Shen, Keren Ding, Shuqun Zhang, Huayuan Shangguan, Tao Fu, Jie Ye, Hao Lin","doi":"10.1016/j.jenvman.2025.125132","DOIUrl":"https://doi.org/10.1016/j.jenvman.2025.125132","url":null,"abstract":"<p><p>A novel electric field-assisted aerobic composting (EAC) method effectively facilitates compost disposal by applying a low electric field to conventional aerobic composting (CAC). The humification effect of inoculation with Bacillus clausii in the EAC system was better than that in the CAC system, so this study focused on the enhancement effect of microbial inoculation in the EAC system. Compared with EAC, EAC with microbial inoculation (AMI-EAC) increased the degradation of cellulose, hemicellulose, and lignin. Furthermore, AMI-EAC improved the humification index by 42.89 % relative to EAC. AMI-EAC also increased the relative abundance of Bacillus, enriched thermophilic and electroactive microorganisms, and enhanced the activity of associated degradative enzymes, which promoted the decomposition and humification of organic matter. Partial least squares-path model analysis showed that Bacillus inoculation during AMI-EAC enhanced the direct positive effect of microorganisms on enzyme activity and strengthened the positive impacts of substance degradation and enzyme activity on compost maturation. This study provided new insights for inoculating microbial agents to enhance composting efficiency in future engineering applications of EAC.</p>","PeriodicalId":356,"journal":{"name":"Journal of Environmental Management","volume":"380 ","pages":"125132"},"PeriodicalIF":8.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143741802","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Can digitalization break the political resource curse? A study on political connections and corporate green innovation.
IF 8 2区 环境科学与生态学
Journal of Environmental Management Pub Date : 2025-03-27 DOI: 10.1016/j.jenvman.2025.124992
Neng Shen, Lin Zhang, Hao Huang, Guoping Zhang, Jing Zhang, Jingwen Zhou
{"title":"Can digitalization break the political resource curse? A study on political connections and corporate green innovation.","authors":"Neng Shen, Lin Zhang, Hao Huang, Guoping Zhang, Jing Zhang, Jingwen Zhou","doi":"10.1016/j.jenvman.2025.124992","DOIUrl":"https://doi.org/10.1016/j.jenvman.2025.124992","url":null,"abstract":"<p><p>Digitalization and greening are inexorable trends in enterprise development today. Based on data from Chinese listed companies from 2008 to 2020, this study examines the relationship between political connections and firms' green innovation, exploring whether digitalization can break the political resource curse and promote green innovation. We find that political connections hinder firms' green innovation, indicating the existence of the political resource curse. Our moderating effect analysis shows that the higher the degree of digitalization of firms, the more significant the decrease in the negative effect of political connections on green innovation, thereby breaking the political resource curse. Heterogeneity analysis shows that the positive moderating effect of digitalization is higher on private firms and firms with more redundant resources. Finally, mechanistic analysis indicates that political connections hinder firms' green innovation by reducing operational efficiency.</p>","PeriodicalId":356,"journal":{"name":"Journal of Environmental Management","volume":"380 ","pages":"124992"},"PeriodicalIF":8.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143741772","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Mapping bird and bat assemblage vulnerability for predicting wind energy impact.
IF 8 2区 环境科学与生态学
Journal of Environmental Management Pub Date : 2025-03-27 DOI: 10.1016/j.jenvman.2025.124961
Jon Morant, Lara Naves-Alegre, Henar Macías García, Elena Tena, Sonia Sánchez-Navarro, Jesús Nogueras, Carlos Ibáñez, Esther Sebastián-González, Juan Manuel Pérez-García
{"title":"Mapping bird and bat assemblage vulnerability for predicting wind energy impact.","authors":"Jon Morant, Lara Naves-Alegre, Henar Macías García, Elena Tena, Sonia Sánchez-Navarro, Jesús Nogueras, Carlos Ibáñez, Esther Sebastián-González, Juan Manuel Pérez-García","doi":"10.1016/j.jenvman.2025.124961","DOIUrl":"https://doi.org/10.1016/j.jenvman.2025.124961","url":null,"abstract":"<p><p>The drive towards decarbonization has led countries to seek renewable energy sources to mitigate global warming. Wind energy is an attractive option due to its low cost and sustainability, but it poses significant risks to birds and bats through collisions and barotrauma with wind turbines. We examined the main ecological traits linked to wind turbine mortality in 214 bird and 19 bat species in peninsular Spain. We assessed the vulnerability of bird and bat assemblages to help understand the potential impact of wind energy development on the most vulnerable assemblages. Our findings indicate that bird and bat casualties were driven by morphological and ecological traits. For birds, scavenger species, those with partial migratory patterns, and aerial lifestyles were most affected by turbine collisions. We also found that vulnerability was positively correlated with observed mortality rates at the province level, but the effect was weaker for birds. Sensitive areas for birds and bats are located in southern, south-eastern, and central Spain, with birds showing additional vulnerability in western and northern regions, while future wind energy development affects bats more in eastern Spain. Our research highlights the importance of mitigating impacts on vulnerable bird and bat species, as well as abundant species. The study highlights the potential risk of ecosystem function loss for bird and bat assemblages due to wind energy projects. We provide spatial tools to identify high-vulnerability areas, guiding energy development to minimize ecological impacts. This work calls on authorities to implement measures to protect species and preserve essential ecosystem functions.</p>","PeriodicalId":356,"journal":{"name":"Journal of Environmental Management","volume":"380 ","pages":"124961"},"PeriodicalIF":8.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143741730","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Bacteria isolated from soil degrade low-density polyethylene for growth and polyhydroxyalkanoate synthesis.
IF 8 2区 环境科学与生态学
Journal of Environmental Management Pub Date : 2025-03-27 DOI: 10.1016/j.jenvman.2025.125072
Intira Khumthong, Wilailak Siripornadulsil, Surasak Siripornadulsil
{"title":"Bacteria isolated from soil degrade low-density polyethylene for growth and polyhydroxyalkanoate synthesis.","authors":"Intira Khumthong, Wilailak Siripornadulsil, Surasak Siripornadulsil","doi":"10.1016/j.jenvman.2025.125072","DOIUrl":"https://doi.org/10.1016/j.jenvman.2025.125072","url":null,"abstract":"<p><p>The low-density polyethylene (LDPE) used in food packaging contributes significantly to the environmental accumulation of microplastics and plastic waste. The aim of this study was to identify and characterize bacteria from plastic waste-contaminated soils that degrade LDPEs. After 16 weeks of degradation, the greatest percentage of LDPE weight loss were achieved with the bacterial consortium and Chitinophaga oryzae NT1-2 (21.97 ± 8.81 % and 16.14 ± 0.46 %, respectively). After bacteria were exposed to LDPE, numerous new functional groups, including aldehydes, ketones, and carboxylic acids, were identified by Fourier transform infrared spectroscopy (FTIR) analysis, while field emission scanning electron microscopy showed that the treated LDPE film surface had more grooves and cracks and was rougher than the control LDPE film surface. The highest total (1781.20 ± 42 U/min/mL) and specific (2.53 ± 0.06 U/min/mg protein) activities of alkane hydroxylase were detected in Bothriochloa intermedia MK2-8, whereas the total and specific alcohol dehydrogenase activities of the MK2-8 strain were 95.57 ± 4.16 U/min/mL and 0.14 ± 0.01 U/min/mg protein, respectively. In Pseudomonas aeruginosa CB1-2, the highest total and specific lipase activities were 10.00 ± 0.20 U/min/mL and 0.10 ± 0.03 U/min/mg protein, respectively. These LDPE-degrading bacteria produced polyhydroxyalkanoate (PHA), with C. oryzae NT1-2 giving the highest yield of 26.27 ± 8.40 mg PHA/g-glucose. Thus, bacteria isolated from plastic contaminated soil possess the capability to enzymatically degrade LDPE and convert it into the PHA biopolymer, thereby contributing to environmental sustainability and resource efficiency.</p>","PeriodicalId":356,"journal":{"name":"Journal of Environmental Management","volume":"380 ","pages":"125072"},"PeriodicalIF":8.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143741764","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Catalytic effects of cations on selenium conversion and distribution by peroxydisulfate in FGD slurry: A combined study.
IF 8 2区 环境科学与生态学
Journal of Environmental Management Pub Date : 2025-03-27 DOI: 10.1016/j.jenvman.2025.125133
Qiyu Weng, Yuqun Zhuo, Pengbo Hu
{"title":"Catalytic effects of cations on selenium conversion and distribution by peroxydisulfate in FGD slurry: A combined study.","authors":"Qiyu Weng, Yuqun Zhuo, Pengbo Hu","doi":"10.1016/j.jenvman.2025.125133","DOIUrl":"https://doi.org/10.1016/j.jenvman.2025.125133","url":null,"abstract":"<p><p>The toxic trace element of selenium, emitted from coal combustion in power plants and enriched in flue gas desulfurization (FGD) slurry, is easily purified in the liquid phase. In order to make as much selenium gathered in the liquid phase of FGD slurry as possible, it is necessary to investigate how peroxydisulfate, the key oxidant in FGD slurry, affects conversion and distribution of selenium with active cations involved. Experiments on the simulated FGD slurry find that Cu<sup>2+</sup> & Fe<sup>2+</sup> have positive effects on oxidation of selenite to selenate by peroxydisulfate via different routes, Co<sup>2+</sup> presents nearly neutral effects and Mn<sup>2+</sup> shows negative effects. Density functional theory (DFT) calculations verify the experimental results by comparing dissociation energy change of peroxydisulfate with different cations added. With the laboratory experiments and DFT calculations combined, selenium distribution in the real FGD slurry sample with peroxydisulfate and copper ion added shows that selenite adsorbed in the gypsum can be quickly oxidized to selenate by the additives and then sent back to the liquid phase without causing damage to the gypsum. This study supplies adequate mechanism explanation and direct technical guidance for selenium purification in FGD slurry.</p>","PeriodicalId":356,"journal":{"name":"Journal of Environmental Management","volume":"380 ","pages":"125133"},"PeriodicalIF":8.0,"publicationDate":"2025-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143741780","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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