IF 39.8 1区材料科学

Joule Pub Date : 2024-10-08 DOI: 10.1016/j.joule.2024.09.004

Chen Zhao, Heonjae Jeong, Inhui Hwang, Tianyi Li, Yang Wang, Jianming Bai, Luxi Li, Shiyuan Zhou, Chi Cheung Su, Wenqian Xu, Zhenzhen Yang, Manar Almazrouei, Cheng-Jun Sun, Lei Cheng, Gui-Liang Xu, Khalil Amine

{"title":"Polysulfide-incompatible additive suppresses spatial reaction heterogeneity of Li-S batteries","authors":"Chen Zhao, Heonjae Jeong, Inhui Hwang, Tianyi Li, Yang Wang, Jianming Bai, Luxi Li, Shiyuan Zhou, Chi Cheung Su, Wenqian Xu, Zhenzhen Yang, Manar Almazrouei, Cheng-Jun Sun, Lei Cheng, Gui-Liang Xu, Khalil Amine","doi":"10.1016/j.joule.2024.09.004","DOIUrl":"https://doi.org/10.1016/j.joule.2024.09.004","url":null,"abstract":"Rational electrolyte engineering for practical pouch cells remains elusive because the correlation between the cathode/solid-electrolyte interphase layer and cell-level reaction behavior is poorly understood. Here, by combining multiscale characterization and computational modeling, we show that—counter to the conventional perception of polysulfide-incompatible additives—the spontaneous reaction of sparingly solvated polysulfides with Lewis acid additives (LAAs) can induce in situ formation of a homogeneous interphase on thick and tortuous S cathode. Multiscale synchrotron X-ray characterization consistently affirms that such interface design could effectively eliminate the notorious problems of polysulfide shuttle and lithium corrosion and, more importantly, provide an interconnected “ion transport highway” to alleviate the uneven ion transport within the tortuous S cathode. Hence, this design dramatically reduces the reaction heterogeneity of lithium-sulfur (Li-S) pouch cells under lean electrolyte conditions. This work resolves controversy around the role of polysulfide-incompatible additives in high-energy Li-S pouch cells and highlights the importance of suppressing reaction heterogeneity for practical batteries.","PeriodicalId":343,"journal":{"name":"Joule","volume":"44 1","pages":""},"PeriodicalIF":39.8,"publicationDate":"2024-10-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142384828","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Carbon abatement costs of green hydrogen across end-use sectors 绿色氢气在各最终使用部门的碳减排成本

IF 39.8 1区材料科学

Joule Pub Date : 2024-10-08 DOI: 10.1016/j.joule.2024.09.003

Roxana T. Shafiee, Daniel P. Schrag

引用次数: 0

A reversible four-electron Sn metal aqueous battery 可逆式四电子锰金属水电池

IF 39.8 1区材料科学

Joule Pub Date : 2024-09-27 DOI: 10.1016/j.joule.2024.09.002

Jianbo Wang, Sofia K. Catalina, Zhelong Jiang, Xin Xu, Qin Tracy Zhou, William C. Chueh, J. Tyler Mefford

{"title":"A reversible four-electron Sn metal aqueous battery","authors":"Jianbo Wang, Sofia K. Catalina, Zhelong Jiang, Xin Xu, Qin Tracy Zhou, William C. Chueh, J. Tyler Mefford","doi":"10.1016/j.joule.2024.09.002","DOIUrl":"https://doi.org/10.1016/j.joule.2024.09.002","url":null,"abstract":"Sn is a promising metal anode for aqueous batteries, with up to four-electron redox available per atom (903 mAh g−1Sn). However, practically harnessing the four-electron Sn(OH)62−/Sn reversibility remains challenging due to limited mechanistic understanding. Here, we reveal a kinetically asymmetric redox pathway involving a successive four-electron plating and a stepwise 2 + 2 electron stripping through a Sn(OH)3− intermediate. The crossover of Sn(OH)3− induces a reversible self-discharge that reduces Coulombic efficiency but does not impact cyclability, demonstrated by four-electron Sn-Ni full cells that sustain >800 h of stable cycling. By tuning the ion selectivity of the separator to suppress Sn(OH)3− crossover while allowing OH− transport, we further demonstrate high Sn utilization (67%) and high energy density (143.1 Wh L−1cell). The results provide key understandings of the tradeoffs in engineering reversible multi-electron metal anodes and define a new benchmark for practical energy density that exceeds any Sn-based aqueous batteries to date.","PeriodicalId":343,"journal":{"name":"Joule","volume":"38 1","pages":""},"PeriodicalIF":39.8,"publicationDate":"2024-09-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142325326","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Single-source pulsed laser-deposited perovskite solar cells with enhanced performance via bulk and 2D passivation 通过块体和二维钝化提高性能的单源脉冲激光沉积过氧化物太阳能电池

IF 39.8 1区材料科学

Joule Pub Date : 2024-09-25 DOI: 10.1016/j.joule.2024.09.001

Tatiana Soto-Montero, Suzana Kralj, Randi Azmi, Manuel A. Reus, Junia S. Solomon, Daniel M. Cunha, Wiria Soltanpoor, Drajad Satrio Utomo, Esma Ugur, Badri Vishal, Martin Ledinsky, Peter Müller-Buschbaum, Finn Babbe, Do Kyoung Lee, Carolin M. Sutter-Fella, Erkan Aydin, Stefaan De Wolf, Monica Morales-Masis

{"title":"Single-source pulsed laser-deposited perovskite solar cells with enhanced performance via bulk and 2D passivation","authors":"Tatiana Soto-Montero, Suzana Kralj, Randi Azmi, Manuel A. Reus, Junia S. Solomon, Daniel M. Cunha, Wiria Soltanpoor, Drajad Satrio Utomo, Esma Ugur, Badri Vishal, Martin Ledinsky, Peter Müller-Buschbaum, Finn Babbe, Do Kyoung Lee, Carolin M. Sutter-Fella, Erkan Aydin, Stefaan De Wolf, Monica Morales-Masis","doi":"10.1016/j.joule.2024.09.001","DOIUrl":"https://doi.org/10.1016/j.joule.2024.09.001","url":null,"abstract":"Single-source vapor deposition of halide perovskites has, to date, remained challenging due to the dissimilar volatilities of the precursors, limiting the controlled transfer of multiple elements at once. Here, we demonstrate that pulsed laser deposition (PLD) addresses the rate-control challenges of single-source evaporation, enabling perovskite solar cells with power conversion efficiencies above 19% after passivation. Combining dry mechanochemical synthesis and PLD, we fabricated (Cl-passivated) MA1−xFAxPbI3 films from a single-source target. These films grow on hole-selective self-assembled monolayers, initially forming a thin PbI2-rich layer, which fully converts to perovskite. An oleylammonium iodide (OAmI) post-treatment is then applied to passivate the perovskite’s top surface by forming a 2D perovskite film. Incorporating PbCl2 in the target and applying OAmI-based 2D passivation results in a remarkable 19.7% efficiency for p-i-n perovskite solar cells with enhanced device stability. This highlights the appeal of PLD to fully unlock the potential of single-source vapor-deposited perovskites.","PeriodicalId":343,"journal":{"name":"Joule","volume":"35 1","pages":""},"PeriodicalIF":39.8,"publicationDate":"2024-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142317334","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Impact of the valence band energy alignment at the hole-collecting interface on the photostability of wide band-gap perovskite solar cells 空穴收集界面价带能量排列对宽带隙过氧化物太阳能电池光稳定性的影响

IF 38.6 1区材料科学

Joule Pub Date : 2024-09-18 DOI: 10.1016/j.joule.2024.06.017

Luis Victor Torres Merino , Christopher E. Petoukhoff , Oleksandr Matiash , Anand Selvin Subbiah , Carolina Villamil Franco , Pia Dally , Badri Vishal , Sofiia Kosar , Diego Rosas Villalva , Vladyslav Hnapovskyi , Esma Ugur , Sahil Shah , Francisco Peña Camargo , Orestis Karalis , Hannes Hempel , Igal Levine , Rakesh R. Pradhan , Suzana Kralj , Nikhil Kalasariya , Maxime Babics , Stefaan De Wolf

{"title":"Impact of the valence band energy alignment at the hole-collecting interface on the photostability of wide band-gap perovskite solar cells","authors":"Luis Victor Torres Merino , Christopher E. Petoukhoff , Oleksandr Matiash , Anand Selvin Subbiah , Carolina Villamil Franco , Pia Dally , Badri Vishal , Sofiia Kosar , Diego Rosas Villalva , Vladyslav Hnapovskyi , Esma Ugur , Sahil Shah , Francisco Peña Camargo , Orestis Karalis , Hannes Hempel , Igal Levine , Rakesh R. Pradhan , Suzana Kralj , Nikhil Kalasariya , Maxime Babics , Stefaan De Wolf","doi":"10.1016/j.joule.2024.06.017","DOIUrl":"10.1016/j.joule.2024.06.017","url":null,"abstract":"<div>This work discusses the need to enhance charge carrier collection to minimize halide segregation in wide band-gap (WBG) perovskites. Here, we systematically elucidate the impact of valence band maximum (VBM) offsets and energetic barriers formed at the hole transport layer (HTL)/perovskite interface on charge accumulation, its influence on halide segregation, and ultimately on perovskite solar cell (PSC) long-term photostability. To this end, we precisely tune the VBM-HTL energetic levels by employing blends of self-assembled monolayers (SAMs; MeO-2PACz and Br-2PACz) to fabricate customized HTLs for PSCs with three different WBG perovskite photoabsorbers (1.69, 1.81, and 2.00 eV), commonly used in various tandem configurations. We find that optimized energetic alignment at the SAM HTL/perovskite interface significantly enhances the long-term photostability of the WBG PSCs. Our results show that photostability of devices can be predicted when comparing HTL/perovskite interfaces using photoluminescence’s evolution and transient surface photovoltage spectroscopies of half-stacks (glass/metal oxide/HTL/perovskite) in correlation with halide segregation.</div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"8 9","pages":"Pages 2585-2606"},"PeriodicalIF":38.6,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141631765","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Temperature excavation to boost machine learning battery thermochemical predictions 温度挖掘促进机器学习电池热化学预测

IF 38.6 1区材料科学

Joule Pub Date : 2024-09-18 DOI: 10.1016/j.joule.2024.07.002

Yu Wang , Xuning Feng , Dongxu Guo , Hungjen Hsu , Junxian Hou , Fangshu Zhang , Chengshan Xu , Xiang Chen , Li Wang , Qiang Zhang , Minggao Ouyang

{"title":"Temperature excavation to boost machine learning battery thermochemical predictions","authors":"Yu Wang , Xuning Feng , Dongxu Guo , Hungjen Hsu , Junxian Hou , Fangshu Zhang , Chengshan Xu , Xiang Chen , Li Wang , Qiang Zhang , Minggao Ouyang","doi":"10.1016/j.joule.2024.07.002","DOIUrl":"10.1016/j.joule.2024.07.002","url":null,"abstract":"<div>Advancing battery technologies requires precise predictions of thermochemical reactions among multiple components to efficiently exploit the stored energy and conduct thermal management. Recently, machine learning (ML) promised to address this complex thermochemical prediction task; however, it failed due to the huge gap between high problem complexity and extremely limited experimental data available for model training. Here, we innovate and validate the temperature excavation (TE) method that interprets the kinetic preferences of thermochemical reactions within minimal experiments into millions of training data. With the help of the TE method, we build the first universally applicable battery thermal runaway model, which achieves high prediction accuracy across a 500°C range on 15 distinct commercial and advanced chemistries with different battery formats and covers all normal working conditions. The TE method also demonstrates broad adaptability and training stability on various ML algorithms, opening new interdisciplinary opportunities for ML in thermochemistry and all thermal-related studies.</div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"8 9","pages":"Pages 2639-2651"},"PeriodicalIF":38.6,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141764481","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Thermochromic polymer blends 热致变色聚合物混合物

IF 38.6 1区材料科学

Joule Pub Date : 2024-09-18 DOI: 10.1016/j.joule.2024.07.020

Sreehari K. Saju , Anand B. Puthirath , Shancheng Wang , Thierry Tsafack , Lucas K. Beagle , Andrey Baydin , Nithya Chakingal , Natsumi Komatsu , Fuyang Tay , Arvin Sharma , Rohini Sreenivasan , Junichiro Kono , Robert Vajtai , Nicholas R. Glavin , Yi Long , Pulickel M. Ajayan

{"title":"Thermochromic polymer blends","authors":"Sreehari K. Saju , Anand B. Puthirath , Shancheng Wang , Thierry Tsafack , Lucas K. Beagle , Andrey Baydin , Nithya Chakingal , Natsumi Komatsu , Fuyang Tay , Arvin Sharma , Rohini Sreenivasan , Junichiro Kono , Robert Vajtai , Nicholas R. Glavin , Yi Long , Pulickel M. Ajayan","doi":"10.1016/j.joule.2024.07.020","DOIUrl":"10.1016/j.joule.2024.07.020","url":null,"abstract":"<div>Smart windows using thermochromic materials provide an excellent thermal management system over broad temperature ranges, leading to significant energy savings. Existing thermochromic materials face challenges, including difficulty in application, degradation during use, and limited durability. Here, we report a simple salted polymer blend system, consisting of poly(dimethylsiloxane), poly(ethylene oxide), and lithium perchlorate, that shows excellent thermochromic properties across an accessible temperature window and remarkable durability. The reversible temperature dependence of optical transmittance of the films arises due to the miscibility of the constituent polymers at room temperature, leading to high transparency, and the gradual phase separation and opaqueness with temperature rise. The easy-to-fabricate, stable polymer system can be a viable and cost-effective alternative to inorganic thermochromic materials such as vanadium dioxide for many applications.</div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"8 9","pages":"Pages 2696-2714"},"PeriodicalIF":38.6,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141981051","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Wavelength-selective solar photovoltaic systems to enhance spectral sharing of sunlight in agrivoltaics 波长选择性太阳能光伏系统，提高农业光伏领域的太阳光光谱共享水平

IF 38.6 1区材料科学

Joule Pub Date : 2024-09-18 DOI: 10.1016/j.joule.2024.08.006

Silvia Ma Lu , Stefano Amaducci , Shiva Gorjian , Matthew Haworth , Carl Hägglund , Tao Ma , Sebastian Zainali , Pietro Elia Campana

{"title":"Wavelength-selective solar photovoltaic systems to enhance spectral sharing of sunlight in agrivoltaics","authors":"Silvia Ma Lu , Stefano Amaducci , Shiva Gorjian , Matthew Haworth , Carl Hägglund , Tao Ma , Sebastian Zainali , Pietro Elia Campana","doi":"10.1016/j.joule.2024.08.006","DOIUrl":"10.1016/j.joule.2024.08.006","url":null,"abstract":"<div>Agrivoltaic systems offer a solution to the debate over using agricultural land for food production or energy conversion. Conventional silicon solar panels often shade plants excessively, impacting growth. Wavelength-selective photovoltaic (WSPV) technologies address this by allowing the transmission of beneficial wavelengths for photosynthesis while converting less useful ones into electricity. Wavelength selectivity can be achieved through various methods, such as by tuning photoactive layers, applying colored semi-transparent layers, utilizing mirrors and lenses, or designing spectrally selective luminophores. While evidence suggests that these technologies effectively share sunlight, many of them are yet to be fully implemented and evaluated. This review covers current WSPV technologies, discussing their classification, status, and future prospects. It also provides appropriate PV performance metrics for WSPV technologies in agricultural applications and advocates for standardized reporting practices in crop experiments conducted under WSPV systems, accompanied by practical suggestions. Solar cell efficiency limits under spectral sharing for crop production and the optimal band gap under varying levels of photosynthetically active radiation for crop growth are further examined as guidance for future development.</div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"8 9","pages":"Pages 2483-2522"},"PeriodicalIF":38.6,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2542435124003726/pdfft?md5=f2b70c9d9b6b8fc129bca38df8c001c7&pid=1-s2.0-S2542435124003726-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142142909","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

A polymer bilayer hole transporting layer architecture for high-efficiency and stable organic solar cells 用于高效稳定有机太阳能电池的聚合物双层空穴传输层结构

IF 38.6 1区材料科学

Joule Pub Date : 2024-09-18 DOI: 10.1016/j.joule.2024.06.013

{"title":"A polymer bilayer hole transporting layer architecture for high-efficiency and stable organic solar cells","authors":"","doi":"10.1016/j.joule.2024.06.013","DOIUrl":"10.1016/j.joule.2024.06.013","url":null,"abstract":"<div>All-solution-processed organic photovoltaic (OPV) cells allow cost- and energy-effective fabrication methods for large-area devices. Despite significant progress on laboratory-scale devices, there is still a lack of interface materials that can be solution processed on top of the active layer, are compatible with novel non-fullerene acceptors (NFAs), and also provide sufficient long-term stability. We developed a novel interface layer concept, where alcohol-based organic polymer nanoparticles can be processed on top of a polymer-NFA active layer and doped to achieve a quasi-Ohmic hole contact. Moreover, poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) is processed as a second layer, forming a bilayer solution-processed hole transporting layer (HTL), providing an industrially relevant inverted architecture with a protective PEDOT:PSS layer on top. Most importantly, exceptional stability is observed. PM6:Y6 devices with the bilayer HTL are demonstrated to maintain 93% of their initial efficiency for 1,800 h under continuous solar cell operation at 60°C.</div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"8 9","pages":"Pages 2570-2584"},"PeriodicalIF":38.6,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2542435124002897/pdfft?md5=cf339e8642c2fba921a3f5cf7b1f77a4&pid=1-s2.0-S2542435124002897-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141561689","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

Ultralow thermal conductivity and high ZT of Cu2Se-based thermoelectric materials mediated by TiO2−n nanoclusters 以 TiO2-n 纳米团簇为介质的 Cu2Se 基热电材料的超低热导率和高 ZT

IF 38.6 1区材料科学

Joule Pub Date : 2024-09-18 DOI: 10.1016/j.joule.2024.06.007

{"title":"Ultralow thermal conductivity and high ZT of Cu2Se-based thermoelectric materials mediated by TiO2−n nanoclusters","authors":"","doi":"10.1016/j.joule.2024.06.007","DOIUrl":"10.1016/j.joule.2024.06.007","url":null,"abstract":"<div>Cu2Se is a promising p-type thermoelectric material for energy harvesting due to its intrinsically low thermal conductivity arising from the liquid-like Cu ions, leaving very limited room for regulation of phonon propagation. Herein, the thermal conductivity of superionic Cu2Se is efficiently mediated by titanium oxide nanoclusters, leading to an exceptionally high thermoelectric figure of merit (ZT) at high temperatures. By controlling the oxygen deficiency, the sophisticated TiO2−n architectures can be constructed with optimized phase composition and electrical properties. The presence of p-n junctions helps to reduce carrier concentration without degrading mobility, and the complex heterogeneous interfaces generated by TiO2−n nanoclusters give rise to huge interfacial thermal resistance. Benefiting from the suppressed electrical transport and enhanced phonon scattering, the total thermal conductivity shows a reduction of at least 36%, contributing to a high ZT value of 2.8 at 973 K. This work demonstrates a paradigm of modulating thermal transport through the self-assembly design.</div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"8 9","pages":"Pages 2652-2666"},"PeriodicalIF":38.6,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141489795","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

引用次数: 0

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