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Dielectric-barrier-stabilized solution plasma for high-nitrogen, few-layer graphene via low-temperature CN radical polymerization 通过低温CN自由基聚合制备高氮、少层石墨烯的介质势垒稳定溶液等离子体
IF 11.6 2区 材料科学
Carbon Pub Date : 2025-10-03 DOI: 10.1016/j.carbon.2025.120914
Jiangqi Niu , Pinli Diao , Shan Ding , Fei Qi , Chayanaphat Chokradjaroen , Rusen Zhou , Sibudjing Kawi
{"title":"Dielectric-barrier-stabilized solution plasma for high-nitrogen, few-layer graphene via low-temperature CN radical polymerization","authors":"Jiangqi Niu ,&nbsp;Pinli Diao ,&nbsp;Shan Ding ,&nbsp;Fei Qi ,&nbsp;Chayanaphat Chokradjaroen ,&nbsp;Rusen Zhou ,&nbsp;Sibudjing Kawi","doi":"10.1016/j.carbon.2025.120914","DOIUrl":"10.1016/j.carbon.2025.120914","url":null,"abstract":"<div><div>Nitrogen-doped graphene (NG) with high crystallinity and elevated nitrogen content is highly desirable for energy and catalytic applications, yet conventional high-temperature methods suffer from nitrogen volatilization, structural degradation, and metal contamination. Here, we report a dielectric-barrier-assisted criss-cross electrode configuration for solution plasma (SP) synthesis that achieves stable, low-temperature glow discharge in a benzene–DMF mixture. Finite-element simulations and optical diagnostics reveal that the dielectric barrier suppresses electron avalanches, producing a spatially uniform CN-rich plasma (∼2505 K) while minimizing C<sub>2</sub> formation, thereby preserving aromatic integrity and limiting nitrogen loss. Compared to the conventional pin-to-pin SP, which generates high-temperature (∼5280 K), C<sub>2</sub>-dominated abnormal glow, the dielectric-stabilized system yields few-layer NG with markedly reduced defect density (I<sub>D</sub>/I<sub>G</sub> = 0.133), narrower 2D band (FWHM = 70 cm<sup>−1</sup>), and higher crystallinity. XPS analysis shows a nitrogen content of 12.22 at% with a high fraction of quaternary N (32.6 %), achieved without detectable metal carbide impurities. Mechanistic analysis suggests that the CN-rich plasma environment promotes polymerization of nitrogen-containing oligomers (e.g., CN·, C<sub>6</sub>H<sub>5</sub>·) into ordered graphene frameworks, providing a controllable pathway for tailoring both the structural and chemical properties of NG. Additional precursor tests (σ-bonded aliphatic, π-bonded aromatic, and extended conjugated molecules) further confirm the generality of this CN-driven mechanism. This work establishes a scalable, low-temperature, in-liquid plasma strategy for producing high-purity, nitrogen-rich graphene with tunable functionalities.</div></div>","PeriodicalId":262,"journal":{"name":"Carbon","volume":"246 ","pages":"Article 120914"},"PeriodicalIF":11.6,"publicationDate":"2025-10-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145218166","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Enhanced catalyst nucleation for vertically grafted CNTs in 3D heterostructures on defect-free 2D materials 无缺陷二维材料上三维异质结构垂直接枝碳纳米管的催化剂成核增强
IF 11.6 2区 材料科学
Carbon Pub Date : 2025-10-02 DOI: 10.1016/j.carbon.2025.120908
Benwu Xin, Jiaxu Ding, Hongyu Liu, Shiwen Li, Qinglin Yuan, Qian Chen, Yang Wang, Dongyan Liu, Zengqin Song, Jinjing Li
{"title":"Enhanced catalyst nucleation for vertically grafted CNTs in 3D heterostructures on defect-free 2D materials","authors":"Benwu Xin,&nbsp;Jiaxu Ding,&nbsp;Hongyu Liu,&nbsp;Shiwen Li,&nbsp;Qinglin Yuan,&nbsp;Qian Chen,&nbsp;Yang Wang,&nbsp;Dongyan Liu,&nbsp;Zengqin Song,&nbsp;Jinjing Li","doi":"10.1016/j.carbon.2025.120908","DOIUrl":"10.1016/j.carbon.2025.120908","url":null,"abstract":"<div><div>A rationally designed three-dimensional (3D) heterostructure integrating anisotropic low-dimensional materials (such as one-dimensional nanotubes and two-dimensional crystals) exhibits synergistic properties unattainable in individual components. By combining the axial anisotropy of 1D materials with the in-plane characteristics of 2D materials, such architectures offer broad application prospects in areas such as out-of-plane electrical conduction and 3D thermal diffusion. In this study, a 3D chemically bonded heterostructure comprising vertically aligned carbon nanotubes (VA-CNTs) and defect-free graphite was synthesized via optimized Al<sub>2</sub>O<sub>3</sub>/Fe/graphite catalytic system, forming a 3D VA-CNTs/graphite allotropic heterostructure without an intermediate dielectric layer. Experiments have proved that the presence of amorphous Al<sub>2</sub>O<sub>3</sub> effectively confines lateral migration of Fe nanoparticles and suppresses their ripening, thereby reducing the size dispersion of the catalyst particles, ultimately facilitating an ordered growth of VA-CNTs. Furthermore, this confinement mechanism shows its applicability to other 2D materials like h-BN, which broadens its potential applications. This reveals a new way of developing novel anisotropic 3D nanostructures based on hierarchical CNT grafting, allowing the utilization of the intrinsic properties of both nanomaterials, with potential applications in various fields.</div></div>","PeriodicalId":262,"journal":{"name":"Carbon","volume":"246 ","pages":"Article 120908"},"PeriodicalIF":11.6,"publicationDate":"2025-10-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145218232","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A review of strategies to produce a fast-charging graphite anode in lithium-ion batteries 锂离子电池中快速充电石墨阳极生产策略综述
IF 11.6 2区 材料科学
Carbon Pub Date : 2025-10-01 DOI: 10.1016/j.carbon.2025.120801
Jin Liang , Ze Qin , Zhong Quan , Jing Hao , Xian-ying Qin , Bao-hua Li , Fei-yu Kang
{"title":"A review of strategies to produce a fast-charging graphite anode in lithium-ion batteries","authors":"Jin Liang ,&nbsp;Ze Qin ,&nbsp;Zhong Quan ,&nbsp;Jing Hao ,&nbsp;Xian-ying Qin ,&nbsp;Bao-hua Li ,&nbsp;Fei-yu Kang","doi":"10.1016/j.carbon.2025.120801","DOIUrl":"10.1016/j.carbon.2025.120801","url":null,"abstract":"","PeriodicalId":262,"journal":{"name":"Carbon","volume":"245 ","pages":"Article 120801"},"PeriodicalIF":11.6,"publicationDate":"2025-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145216738","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Lithium-ion pre-doping of graphite electrodes using lithium naphthalenide derivatives with electron-donating substituents 含供电子取代基的萘化锂衍生物石墨电极的锂离子预掺杂
IF 11.6 2区 材料科学
Carbon Pub Date : 2025-10-01 DOI: 10.1016/j.carbon.2025.120753
Yuu Watanabe , Hiroyuki Matsuura
{"title":"Lithium-ion pre-doping of graphite electrodes using lithium naphthalenide derivatives with electron-donating substituents","authors":"Yuu Watanabe ,&nbsp;Hiroyuki Matsuura","doi":"10.1016/j.carbon.2025.120753","DOIUrl":"10.1016/j.carbon.2025.120753","url":null,"abstract":"","PeriodicalId":262,"journal":{"name":"Carbon","volume":"245 ","pages":"Article 120753"},"PeriodicalIF":11.6,"publicationDate":"2025-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145216333","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Modifying the pore structure of biomass-derived porous carbon for use in energy storage systems 修饰生物质衍生多孔碳的孔隙结构,用于储能系统
IF 11.6 2区 材料科学
Carbon Pub Date : 2025-10-01 DOI: 10.1016/j.carbon.2025.120807
Bin Xie , Xin-ya Zhao , Zheng-dong Ma , Yi-jian Zhang , Jia-rong Dong , Yan Wang , Qiu-hong Bai , Ye-hua Shen
{"title":"Modifying the pore structure of biomass-derived porous carbon for use in energy storage systems","authors":"Bin Xie ,&nbsp;Xin-ya Zhao ,&nbsp;Zheng-dong Ma ,&nbsp;Yi-jian Zhang ,&nbsp;Jia-rong Dong ,&nbsp;Yan Wang ,&nbsp;Qiu-hong Bai ,&nbsp;Ye-hua Shen","doi":"10.1016/j.carbon.2025.120807","DOIUrl":"10.1016/j.carbon.2025.120807","url":null,"abstract":"","PeriodicalId":262,"journal":{"name":"Carbon","volume":"245 ","pages":"Article 120807"},"PeriodicalIF":11.6,"publicationDate":"2025-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145217010","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Microstructure-mechanism-performance relationships in hard carbon anode materials for sodium-ion batteries 钠离子电池硬碳负极材料的微观结构-机理-性能关系
IF 11.6 2区 材料科学
Carbon Pub Date : 2025-10-01 DOI: 10.1016/j.carbon.2025.120806
Jin-ting Li , Nurbiye Sawu , Yi-chu Zhao , Ping Liu , Yan-xia Wang , Yu-liang Cao
{"title":"Microstructure-mechanism-performance relationships in hard carbon anode materials for sodium-ion batteries","authors":"Jin-ting Li ,&nbsp;Nurbiye Sawu ,&nbsp;Yi-chu Zhao ,&nbsp;Ping Liu ,&nbsp;Yan-xia Wang ,&nbsp;Yu-liang Cao","doi":"10.1016/j.carbon.2025.120806","DOIUrl":"10.1016/j.carbon.2025.120806","url":null,"abstract":"","PeriodicalId":262,"journal":{"name":"Carbon","volume":"245 ","pages":"Article 120806"},"PeriodicalIF":11.6,"publicationDate":"2025-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145216588","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Carbon materials for smart batteries 智能电池用碳材料
IF 11.6 2区 材料科学
Carbon Pub Date : 2025-10-01 DOI: 10.1016/j.carbon.2025.120804
Jun-yi Zhou , Hong-hui Du , Xue-tao Wang , Xin-ru Cao , Lin-jie Zhi
{"title":"Carbon materials for smart batteries","authors":"Jun-yi Zhou ,&nbsp;Hong-hui Du ,&nbsp;Xue-tao Wang ,&nbsp;Xin-ru Cao ,&nbsp;Lin-jie Zhi","doi":"10.1016/j.carbon.2025.120804","DOIUrl":"10.1016/j.carbon.2025.120804","url":null,"abstract":"","PeriodicalId":262,"journal":{"name":"Carbon","volume":"245 ","pages":"Article 120804"},"PeriodicalIF":11.6,"publicationDate":"2025-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145216740","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Compilation and characterization of the visual appearance of alkali metal graphite intercalation compounds 碱金属石墨插层化合物视觉外观的合成与表征
IF 11.6 2区 材料科学
Carbon Pub Date : 2025-10-01 DOI: 10.1016/j.carbon.2025.120754
Rika Matsumoto , Masato Oshima , Katsumi Yamada , Tokio Yukiya , Masaomi Sanekata
{"title":"Compilation and characterization of the visual appearance of alkali metal graphite intercalation compounds","authors":"Rika Matsumoto ,&nbsp;Masato Oshima ,&nbsp;Katsumi Yamada ,&nbsp;Tokio Yukiya ,&nbsp;Masaomi Sanekata","doi":"10.1016/j.carbon.2025.120754","DOIUrl":"10.1016/j.carbon.2025.120754","url":null,"abstract":"","PeriodicalId":262,"journal":{"name":"Carbon","volume":"245 ","pages":"Article 120754"},"PeriodicalIF":11.6,"publicationDate":"2025-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145216648","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Separating the effects of the electrolyte and solid electrolyte interphase on alkali metal ion transer resistance in non-graphitizable carbon 分离了电解质和固体电解质界面相对非石墨化碳中碱金属离子转移电阻的影响
IF 11.6 2区 材料科学
Carbon Pub Date : 2025-10-01 DOI: 10.1016/j.carbon.2025.120758
Shota Tsujimoto , Yasuyuki Kondo , Changhee Lee , Yuko Yokoyama , Yuto Miyahara , Kohei Miyazaki , Takeshi Abe
{"title":"Separating the effects of the electrolyte and solid electrolyte interphase on alkali metal ion transer resistance in non-graphitizable carbon","authors":"Shota Tsujimoto ,&nbsp;Yasuyuki Kondo ,&nbsp;Changhee Lee ,&nbsp;Yuko Yokoyama ,&nbsp;Yuto Miyahara ,&nbsp;Kohei Miyazaki ,&nbsp;Takeshi Abe","doi":"10.1016/j.carbon.2025.120758","DOIUrl":"10.1016/j.carbon.2025.120758","url":null,"abstract":"","PeriodicalId":262,"journal":{"name":"Carbon","volume":"245 ","pages":"Article 120758"},"PeriodicalIF":11.6,"publicationDate":"2025-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145216736","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Carbon-based electrodes and sensors for miniaturized blood gas analyzers 用于小型血气分析仪的碳基电极和传感器
IF 11.6 2区 材料科学
Carbon Pub Date : 2025-10-01 DOI: 10.1016/j.carbon.2025.120750
Akiko Yoshida , Tetsuji Itoh , Hirotomo Nishihara
{"title":"Carbon-based electrodes and sensors for miniaturized blood gas analyzers","authors":"Akiko Yoshida ,&nbsp;Tetsuji Itoh ,&nbsp;Hirotomo Nishihara","doi":"10.1016/j.carbon.2025.120750","DOIUrl":"10.1016/j.carbon.2025.120750","url":null,"abstract":"","PeriodicalId":262,"journal":{"name":"Carbon","volume":"245 ","pages":"Article 120750"},"PeriodicalIF":11.6,"publicationDate":"2025-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145216330","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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