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First-principles study of structural, elastic, electronic and optical properties of XRbCl3 (X = Ca, Ba) perovskite compounds
IF 4.4 2区 物理与天体物理
Results in Physics Pub Date : 2025-02-17 DOI: 10.1016/j.rinp.2025.108163
Norah Algethami , Aiman Jehan , Nasir Rahman , Saima Naz Khan , Wafa Mohammed Almalki , Mudasser Husain , Vineet Tirth , Hanan A. Althobaiti , Yazen M. Alawaideh , Khamael M. Abualnaja , Ghaida Alosaimi
{"title":"First-principles study of structural, elastic, electronic and optical properties of XRbCl3 (X = Ca, Ba) perovskite compounds","authors":"Norah Algethami ,&nbsp;Aiman Jehan ,&nbsp;Nasir Rahman ,&nbsp;Saima Naz Khan ,&nbsp;Wafa Mohammed Almalki ,&nbsp;Mudasser Husain ,&nbsp;Vineet Tirth ,&nbsp;Hanan A. Althobaiti ,&nbsp;Yazen M. Alawaideh ,&nbsp;Khamael M. Abualnaja ,&nbsp;Ghaida Alosaimi","doi":"10.1016/j.rinp.2025.108163","DOIUrl":"10.1016/j.rinp.2025.108163","url":null,"abstract":"<div><div>We report on DFT calculations of electronic, elastic and optical properties of XRbCl<sub>3</sub> (X = Ca, Ba) perovskites using the FP-LAPW method. The investigated compounds crystallize in a cubic structure, with structural optimization performed using the Birch-Murnaghan equation of state. The optimized lattice parameters were determined to be 5.83 Å and 5.77 Å for XRbCl<sub>3</sub> (X = Ca, Ba), respectively. The elastic properties, including cubic elastic constants, Poisson’s ratio (ν), elastic moduli, anisotropy factor, and Pugh’s ratio (B/G), were computed using the highly precise IRelast package integrated within the WIEN2k software. The analysis confirms that these materials exhibit mechanical stability, ductility, and elastic anisotropy. The electronic band structures of CaRbCl<sub>3</sub> and BaRbCl<sub>3</sub> were accurately determined using DFT calculations with the TB-mBJ approximation, revealing direct band gaps of 1.51 eV and 2.76 eV, respectively, at the Γ-Γ high-symmetry points. The optical properties, including the absorption coefficient, refractive index n(ω), reflectivity, and optical conductivity, were analyzed within the energy range of 0–15 eV, offering valuable insights into their response to varying photon energies. The favorable optical characteristics of these compounds highlight their potential for advancements in light-based technologies and energy-related applications.</div></div>","PeriodicalId":21042,"journal":{"name":"Results in Physics","volume":"70 ","pages":"Article 108163"},"PeriodicalIF":4.4,"publicationDate":"2025-02-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143444939","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Nonlinear drift waves and their role in Saturn’s B-ring: implications of rotation-induced dispersive dust drift waves and plasma parameter effects on spokes
IF 4.4 2区 物理与天体物理
Results in Physics Pub Date : 2025-02-15 DOI: 10.1016/j.rinp.2025.108149
S. Hassan , N. Batool , W. Masood , P.H. Yoon
{"title":"Nonlinear drift waves and their role in Saturn’s B-ring: implications of rotation-induced dispersive dust drift waves and plasma parameter effects on spokes","authors":"S. Hassan ,&nbsp;N. Batool ,&nbsp;W. Masood ,&nbsp;P.H. Yoon","doi":"10.1016/j.rinp.2025.108149","DOIUrl":"10.1016/j.rinp.2025.108149","url":null,"abstract":"<div><div>Both linear and nonlinear dispersive dust drift waves are investigated in a magnetized, rotating plasma in the presence of Cairns and kappa-distributed ions by using the two fluid model. In the linear regime, dispersion relation is obtained. In the nonlinear regime, nonlinear partial differential equation (NLPDE) is solved to obtain the exact solitary solution by using the functional variable method. Parameters of Saturn’s B-ring are used for the graphical analysis. Graphical illustrations show that the solved NLPDE admits both compressive and rarefactive solitary solution depending on the velocity of the solitary structure. 3-D representation of compressive and rarefactive solitary structuresd appear as the spokes like structures (dark and bright, respectively) which are wider at the base and become narrower as the radial distance increases. This observation further supports the hypothesis that nonlinear drift waves may indeed correspond to the spokes observed in Saturn’s B-ring. It is noted that bright and dark spokes exhibit distinct behaviors in response to variations in the plasma parameters. By applying plasma parameters typical of those found in Saturn’s B-ring, it is demonstrated that the theoretically predicted spatiotemporal scale lengths align closely with the observations of the spokes made by various space missions and the Hubble Space Telescope (HST).</div></div>","PeriodicalId":21042,"journal":{"name":"Results in Physics","volume":"70 ","pages":"Article 108149"},"PeriodicalIF":4.4,"publicationDate":"2025-02-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143420690","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Novel hafnium oxide doped G-T-B Glass: Structural, physical, mechanical, optical, and radiation shielding investigation
IF 4.4 2区 物理与天体物理
Results in Physics Pub Date : 2025-02-15 DOI: 10.1016/j.rinp.2025.108161
M.H.A. Mhareb , Kawa M. Kaky , K.A. Mahmoud , M.I. Sayyed , Abed Jawad Kadhim , Yasser Maghrbi
{"title":"Novel hafnium oxide doped G-T-B Glass: Structural, physical, mechanical, optical, and radiation shielding investigation","authors":"M.H.A. Mhareb ,&nbsp;Kawa M. Kaky ,&nbsp;K.A. Mahmoud ,&nbsp;M.I. Sayyed ,&nbsp;Abed Jawad Kadhim ,&nbsp;Yasser Maghrbi","doi":"10.1016/j.rinp.2025.108161","DOIUrl":"10.1016/j.rinp.2025.108161","url":null,"abstract":"<div><div>Three glasses were fabricated using a common melting and annealing process. Hafnium oxide-doped tellurite germanate borate glasses have been investigated for radiation shielding. A series of three glasses with the formula of (35-x) B<sub>2</sub>O<sub>3</sub>-20TeO<sub>2</sub>-10GeO<sub>2</sub>-35MgO-xHfO<sub>2</sub> (x = 1.25, 2.5, and 3.75 mol%). X-ray diffraction (XRD) pattern investigated the glassy phase of the samples. The Makishima-Mackenzie model was employed to evaluate the mechanical features of synthetic glasses. The dissociation energy (G<sub>t</sub>) and packing density (V<sub>t</sub>) are determined using the related formulas. The optical features of the manufactured glasses were determined using a number of formulas and the UV absorption edge. The energy band gap (E<sub>g</sub>) was found using the Mott and Davis relation. The refractive index and Urbach energy (E<sub>U</sub>) were computed using the related relationships. Many optical features, like metallization (M), transmission (T), reflection loss (R), optical basicity (Λ), optical polarizability (α<sub>0</sub>), and optical electronegativity (χ), were computed and reported in this work. Monte Carlo simulation was employed to investigate the gamma-ray shielding parameters over an energy interval that extends from 0.015 MeV to 10 MeV. The increase in HfO<sub>2</sub> content within the concentration rage of 1.25–3.75 mol% increases the linear attenuation coefficient of the prepared glasses across the ranges of 107.510–134.277 cm<sup>−1</sup> (at 0.015 MeV) 1.282–1.593 cm<sup>−1</sup> (at 0.15 MeV), and 0.183–0.191 cm<sup>−1</sup> (at 1.5 MeV). The increase in HfO<sub>2</sub> concentrations is also accompanied by a decrease in the half-value thickness, thickness equivalent lead, and the transmission factor for the synthesized glass samples.</div></div>","PeriodicalId":21042,"journal":{"name":"Results in Physics","volume":"70 ","pages":"Article 108161"},"PeriodicalIF":4.4,"publicationDate":"2025-02-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143454577","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Investigation of a novel exact wave solution structure in nonlinear thermoelasticity using modern techniques
IF 4.4 2区 物理与天体物理
Results in Physics Pub Date : 2025-02-15 DOI: 10.1016/j.rinp.2025.108148
Wafaa B. Rabie , Hamdy M. Ahmed , Mohamed F. Ismail , Abdul-Majid Wazwaz , Abdallah A. Syied , Assmaa Abd-Elmonem , Nesreen Sirelkhtam Elmki Abdalla , W. Abbas , M.A. Ibrahim
{"title":"Investigation of a novel exact wave solution structure in nonlinear thermoelasticity using modern techniques","authors":"Wafaa B. Rabie ,&nbsp;Hamdy M. Ahmed ,&nbsp;Mohamed F. Ismail ,&nbsp;Abdul-Majid Wazwaz ,&nbsp;Abdallah A. Syied ,&nbsp;Assmaa Abd-Elmonem ,&nbsp;Nesreen Sirelkhtam Elmki Abdalla ,&nbsp;W. Abbas ,&nbsp;M.A. Ibrahim","doi":"10.1016/j.rinp.2025.108148","DOIUrl":"10.1016/j.rinp.2025.108148","url":null,"abstract":"<div><div>This study introduces an enhanced methodology to investigate the complex interactions within temperature-dependent thermoelastic systems, particularly under the Dual-Phase-Lag (DPL) model. Motivated by the challenges posed by nonlinear thermoelasticity, where thermal loads significantly influence material geometry and properties, the research aims to bridge the gap in accurately modeling such phenomena. Real-world applications, including the behavior of materials under extreme thermal conditions and thermal stresses in large-scale structures, necessitate precise methodologies to capture these intricate couplings between thermal and mechanical effects. To this end, the study introduces an enhanced approach, the improved modified extended tanh function technique (IMETFT). The analysis reveals a variety of solutions, such as dark soliton, bright soliton, singular soliton, hyperbolic, rational, Jacobi elliptic, polynomial, and exponential solutions. Graphical depictions of some of the extracted solutions are included to aid readers in physically understanding the obtained solutions’ behavior and characteristics.</div></div>","PeriodicalId":21042,"journal":{"name":"Results in Physics","volume":"70 ","pages":"Article 108148"},"PeriodicalIF":4.4,"publicationDate":"2025-02-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143420692","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Generic mobility edges in a class of non-Hermitian quasicrystals
IF 4.4 2区 物理与天体物理
Results in Physics Pub Date : 2025-02-12 DOI: 10.1016/j.rinp.2025.108146
Xiang-Ping Jiang , Mingdi Xu , Lei Pan
{"title":"Generic mobility edges in a class of non-Hermitian quasicrystals","authors":"Xiang-Ping Jiang ,&nbsp;Mingdi Xu ,&nbsp;Lei Pan","doi":"10.1016/j.rinp.2025.108146","DOIUrl":"10.1016/j.rinp.2025.108146","url":null,"abstract":"<div><div>We present approximate solutions for the mobility edge (ME) in a specific class of one-dimensional non-Hermitian (NH) quasicrystals delineating between localized and extended states. These NH quasicrystals exhibit a combination of nonreciprocal hopping terms and imaginary phase factors. Our analytical approach is supported by rigorous numerical calculations, demonstrating significant accuracy. Furthermore, our ansatz aligns closely with the established limiting cases of the NH Aubry–André–Harper (AAH) and Ganeshan–Pixley–Das Sarma (GPD) models, which possess exact results, thereby enhancing the credibility of our approach. Additionally, we have examined their dynamic properties and identified distinct behaviors in different regimes. Our research offers a practical methodology for estimating the position of MEs in a category of NH quasicrystals that break duality.</div></div>","PeriodicalId":21042,"journal":{"name":"Results in Physics","volume":"70 ","pages":"Article 108146"},"PeriodicalIF":4.4,"publicationDate":"2025-02-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143395192","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Pore-scale evaluation on hydrothermal performance in a microtube with homogeneous microporous media by lattice Boltzmann method
IF 4.4 2区 物理与天体物理
Results in Physics Pub Date : 2025-02-12 DOI: 10.1016/j.rinp.2025.108155
Saboura Yousefi , Mostafa Mahdavi , Seyed Soheil Mousavi Ajarostaghi , Mohsen Sharifpur , Magda Abd El-Rahman
{"title":"Pore-scale evaluation on hydrothermal performance in a microtube with homogeneous microporous media by lattice Boltzmann method","authors":"Saboura Yousefi ,&nbsp;Mostafa Mahdavi ,&nbsp;Seyed Soheil Mousavi Ajarostaghi ,&nbsp;Mohsen Sharifpur ,&nbsp;Magda Abd El-Rahman","doi":"10.1016/j.rinp.2025.108155","DOIUrl":"10.1016/j.rinp.2025.108155","url":null,"abstract":"<div><div>This study investigates the heat transfer and flow behavior of Al<sub>2</sub>O<sub>3</sub>-water nanofluid in micro-scale systems, using the lattice Boltzmann method (LBM) for numerical simulations. To implement the LBM code, FORTRAN home-made programming is employed. The research focuses on a three-dimensional microtube (500 μm diameter and 6,000 μm length) subjected to a uniform wall heat flux, with Reynolds numbers between 40 and 100. Spherical particles of varying sizes and quantities are introduced into the flow path to investigate the impact of porosity on thermophysical properties. The study explores the relatively unexamined application of the LBM to curved boundaries. Results indicate that introducing 6–10 spherical objects at Re = 40 increases the average Nusselt number by about 23.61 % and 25.83 %, respectively, whereas larger spheres in smaller quantities exhibit minimal or negative effects on heat transfer. Although the lattice Boltzmann method is gaining traction in fluid dynamics, its application to curved boundaries remains limited. This study advances the field by analyzing flow dynamics in a microtube with spherical inserts, integrating curved boundaries, nanofluids, and porous structures, thereby providing valuable insights into thermophysical studies.</div></div>","PeriodicalId":21042,"journal":{"name":"Results in Physics","volume":"70 ","pages":"Article 108155"},"PeriodicalIF":4.4,"publicationDate":"2025-02-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143420852","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Electrostatic action promotes bonding efficacy of DNA-modified nanoparticle self-assembly in solution
IF 4.4 2区 物理与天体物理
Results in Physics Pub Date : 2025-02-11 DOI: 10.1016/j.rinp.2025.108153
Qiuyan Yu , Jinhong Huang , Mengyuan Liu
{"title":"Electrostatic action promotes bonding efficacy of DNA-modified nanoparticle self-assembly in solution","authors":"Qiuyan Yu ,&nbsp;Jinhong Huang ,&nbsp;Mengyuan Liu","doi":"10.1016/j.rinp.2025.108153","DOIUrl":"10.1016/j.rinp.2025.108153","url":null,"abstract":"<div><div>Our study aims to develop a foundational framework for simulating DNA-modified nanoparticle (DNA-NP) self-assembly in salt solutions, focusing on electrostatic and bonding interactions. We employ a sophisticated coarse-grained model to explore bonding efficacy and thermodynamic analysis across various density systems by molecular dynamics method. Notably, in low-density systems, bonding percentage <em>p</em><sub>h</sub> is minimal at <em>T</em> = 1.2. By increasing cation concentration <em>c</em><sup>+</sup>, controlling temperature, optimizing grafting number <em>n</em> and linker length, <em>p</em><sub>h</sub> can be significantly improved. For instance, at <em>c</em><sup>+</sup> = 0.5, the maximum <em>p</em><sub>h</sub> reaches 0.4 for <em>n</em> = 60, surpassing that for <em>n</em> = 100. Although higher DNA loadings can significantly influence nanotherapeutics and biological detection, an optimal grafting number (<em>n</em> = 60) is crucial for peak bonding efficacy at temperatures <em>T</em> = 1.08 ∼ 1.23. The peak value <em>p</em><sub>h, max</sub> is observed near <em>t</em> = 3 × 10<sup>6</sup>. The required bonding strength varies depending on the application field. For crystalline lattice formation, optimal linker length <em>n</em><sub>l</sub> is equal to 3. For probes or medical diagnostics, longer linker chains is recommended to enhance bonding strength and probe sensitivity. In higher density systems, there exist different optimization conditions. These insights are valuable for rational design of DNA-NP for targeted drug delivery and diagnostics among other biomedical applications.</div></div>","PeriodicalId":21042,"journal":{"name":"Results in Physics","volume":"70 ","pages":"Article 108153"},"PeriodicalIF":4.4,"publicationDate":"2025-02-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143420693","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Thermodynamic properties and the confinement frequency for Second Pὃschl-Teller potential
IF 4.4 2区 物理与天体物理
Results in Physics Pub Date : 2025-02-10 DOI: 10.1016/j.rinp.2025.108144
C.A. Onate , I.B. Okon , E. Omugbe , E.S. Eyube , K.O. Emeje
{"title":"Thermodynamic properties and the confinement frequency for Second Pὃschl-Teller potential","authors":"C.A. Onate ,&nbsp;I.B. Okon ,&nbsp;E. Omugbe ,&nbsp;E.S. Eyube ,&nbsp;K.O. Emeje","doi":"10.1016/j.rinp.2025.108144","DOIUrl":"10.1016/j.rinp.2025.108144","url":null,"abstract":"<div><div>The study of thermodynamic properties for different potentials as a function of temperature and maximum quantum state have been widely reported. In the present study, the authors examined the effect of the total confinement frequency (which is a combination of a confinement frequency <span><math><msub><mi>ω</mi><mn>0</mn></msub></math></span> and cyclotron frequency <span><math><msub><mi>ω</mi><mi>c</mi></msub></math></span>) on some thermodynamic properties such as the vibrational enthalpy, the vibrational Gibbs free energy and the vibrational entropy. The energy level of the Second Pὃschl-Teller potential model is obtained using supersymmetric approach and shape invariance formalism. Then, the vibrational partition function is calculated from the energy level of the Second Pὃschl-Teller potential model using the Poisson summation formula. The vibrational thermodynamic properties are calculated from the partition function and its derivative. The result shows that the presence of the total confinement frequency lowers the vibrational enthalpy and entropy but reduces the negativity of the Gibbs free energy. The result also showcases that the magnetic field which is the main term in the cyclotron frequency has less decreasing effect on the enthalpy and entropy compared to the frequency as part of the total confinement frequency.</div></div>","PeriodicalId":21042,"journal":{"name":"Results in Physics","volume":"70 ","pages":"Article 108144"},"PeriodicalIF":4.4,"publicationDate":"2025-02-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143376610","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A random fiber laser with multiple bidirectional Rayleigh scattering provided by dual-ring sub-cavity structure
IF 4.4 2区 物理与天体物理
Results in Physics Pub Date : 2025-02-10 DOI: 10.1016/j.rinp.2025.108151
Shaode Li , Wei He , Qiongyue Zhang , Xingpeng Fei
{"title":"A random fiber laser with multiple bidirectional Rayleigh scattering provided by dual-ring sub-cavity structure","authors":"Shaode Li ,&nbsp;Wei He ,&nbsp;Qiongyue Zhang ,&nbsp;Xingpeng Fei","doi":"10.1016/j.rinp.2025.108151","DOIUrl":"10.1016/j.rinp.2025.108151","url":null,"abstract":"<div><div>In this study, a simple and effective method for enhancing Rayleigh scattering (RS) intensity is proposed and experimentally validated, enabling stable output with exceptionally low-frequency noise across each wavelength channel of random fiber lasers (RFLs). The design employs two segments of single-mode fibers (SMFs) symmetrically arranged in dual-ring sub-cavity. This unique structural configuration facilitates multiple bidirectional RS interactions, providing sufficient random distributed feedback (R-DFB) for the laser system. Initially, random laser (RL) outputs at 1560 nm were achieved using both ring-cavity and single-ring sub-cavity structures. These systems exhibited frequency noise exceeding 1.21 Hz/√Hz and wavelength and output power fluctuations of 0.79 nm and 1.52 dB, respectively. Subsequently, the laser system was upgraded to a dual-ring sub-cavity configuration, and its output performance was re-evaluated. The experimental results show that the wavelength and output power fluctuations are reduced to 0.28 nm and 0.26 dB, respectively. Benefiting from the enhanced R-DFB and superior filtering properties of the dual-ring sub-cavity, the frequency noise of the lasing output decreased significantly to 0.03 Hz/√Hz, the lowest value reported to date. In addition, the importance of sufficient R-DFB for RFL is demonstrated by measuring frequency amplitude, output linewidth, and slope efficiency.</div></div>","PeriodicalId":21042,"journal":{"name":"Results in Physics","volume":"70 ","pages":"Article 108151"},"PeriodicalIF":4.4,"publicationDate":"2025-02-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143395193","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Laser-induced photochemical reduction for the production of gold and silver nanoparticles on gold nanostructures
IF 4.4 2区 物理与天体物理
Results in Physics Pub Date : 2025-02-10 DOI: 10.1016/j.rinp.2025.108152
Naushad Ahmad Khan , Yi-Han Kuo , Shang-Yang Yu , Yun-Cheng Ku , Kuo-Yung Hung , Jiunn-Woei Liaw
{"title":"Laser-induced photochemical reduction for the production of gold and silver nanoparticles on gold nanostructures","authors":"Naushad Ahmad Khan ,&nbsp;Yi-Han Kuo ,&nbsp;Shang-Yang Yu ,&nbsp;Yun-Cheng Ku ,&nbsp;Kuo-Yung Hung ,&nbsp;Jiunn-Woei Liaw","doi":"10.1016/j.rinp.2025.108152","DOIUrl":"10.1016/j.rinp.2025.108152","url":null,"abstract":"<div><div>This research explores two methods for the photo-chemical reduction of gold and silver ions, utilizing either a continuous-wave (CW) laser or a femtosecond laser, in conjunction with plasmon-assisted hot electrons. The study focuses on the photoreduction of chloroauric acid (HAuCl<sub>4</sub>) and silver nitrate (AgNO<sub>3</sub>) solutions containing gold nanostructures under irradiation from either CW or femtosecond laser. Specifically, we employed a 445 nm CW laser to irradiate gold nanowires, formed through the photo-driven self-assembly of gold nanorods, in HAuCl<sub>4</sub> solution. Through this photoreduction process, we observed the newly formed gold nanoparticles on the surface of gold nanowires. In addition, we also used 445 nm to irradiate gold triangular nanoplates in AgNO<sub>3</sub> solution with ascorbic acid as a reducing agent. We observed that silver nanoparticles clearly formed and attached to the edges of a gold triangular nanoplate. In another approach, an 800 nm femtosecond laser was used to irradiate gold nanorods, gold triangular/hexagonal nanoplates and a gold nanofilm in AgNO<sub>3</sub> solution with a reducing agent under inverted microscopy. For instance, silver nanoparticles were observed to attach to the edges of the gold triangular and hexagonal nanoplates, facilitating the growth of the nanoplates. The formation of photochemically reduced nanoparticles was confirmed using energy-dispersive X-ray spectroscopy. Notably, 3D silver dendritic structures were synthesized with the femtosecond laser and deposited onto the gold nanofilm, a process attributed to two-photon absorption effect. The high sensitivity of these immobilized dendrites for surface-enhanced Raman scattering applications was also demonstrated.</div></div>","PeriodicalId":21042,"journal":{"name":"Results in Physics","volume":"70 ","pages":"Article 108152"},"PeriodicalIF":4.4,"publicationDate":"2025-02-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143420691","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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