Process Safety and Environmental Protection最新文献

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An avalanche transistor-based Marx circuit pulse generator with sub-nanosecond, high frequency and high-voltage for pathogenic Escherichia coli ablation 基于雪崩晶体管的马克思电路脉冲发生器,具有亚纳秒、高频率和高电压,可用于致病性大肠杆菌消融术
IF 6.9 2区 环境科学与生态学
Process Safety and Environmental Protection Pub Date : 2024-09-26 DOI: 10.1016/j.psep.2024.09.095
{"title":"An avalanche transistor-based Marx circuit pulse generator with sub-nanosecond, high frequency and high-voltage for pathogenic Escherichia coli ablation","authors":"","doi":"10.1016/j.psep.2024.09.095","DOIUrl":"10.1016/j.psep.2024.09.095","url":null,"abstract":"<div><div>Pathogenic Escherichia coli, which will easily cause environmental pollution, is a potentially hazardous microorganism that enters the environment through various routes such as biological feces. The presence of this bacterium poses a serious health risk, especially in water sources. When consuming water containing excessive amounts of pathogenic Escherichia coli, both humans and animals may experience severe health issues, such as diarrhea and gastrointestinal infections. However, current treatment methods for this bacterium are not ideal, and traditional means sometimes struggle to completely eliminate these stubborn microorganisms. In recent years, the scientific community has been exploring new sterilization techniques to address this challenge without causing secondary environmental pollution. Among them, pulsed electric field (PEF) technology has garnered significant attention. By applying high-intensity electric field pulses, PEF technology can have a fatal impact on microbial cells in a very short period of time. Studies have shown that this technology can cause cell membrane perforation, destroying the integrity of the cell and leading to cell death. This method is not only capable of decomposing organic pollutants, but also has a significant bactericidal effect. Nevertheless, despite the theoretical potential of PEF technology, there is still relatively little research on its application, especially in terms of treating pathogenic Escherichia coli. Further studies and experimental verification are needed. This article investigates the bioelectromagnetic effects of electric pulses on pathogenic Escherichia coli in sewage through a self-developed pulse source device (capable of providing a voltage range from 1.7 kV to 2.2 kV, with a rise time of 190 ps and a maximum repetition rate of 20 kHz). The feasibility of using a pulsed electric field to purify water bodies is verified in this report.</div></div>","PeriodicalId":20743,"journal":{"name":"Process Safety and Environmental Protection","volume":null,"pages":null},"PeriodicalIF":6.9,"publicationDate":"2024-09-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142322055","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Fabrication of heterogeneous catalyst for production of biodiesel form municipal sludge 制造用于以市政污泥为原料生产生物柴油的异相催化剂
IF 6.9 2区 环境科学与生态学
Process Safety and Environmental Protection Pub Date : 2024-09-25 DOI: 10.1016/j.psep.2024.09.101
{"title":"Fabrication of heterogeneous catalyst for production of biodiesel form municipal sludge","authors":"","doi":"10.1016/j.psep.2024.09.101","DOIUrl":"10.1016/j.psep.2024.09.101","url":null,"abstract":"<div><div>Sewage sludge, a semi-solid byproducts of municipal wastewater treatment processes, offers a sustainable and cost-effective feedstock for biodiesel production through the synthesis of catalytic heterogeneous catalysts. In this study, we developed a novel heterogeneous catalyst by impregnating aluminum nitrate and calcite, obtained from carbon dioxide-sequestering bacteria, onto DigSBiochar (Biochar derived from digested sewage sludge). The produced catalyst was subsequently immobilized with the lipase enzyme isolated from <em>Bacillus</em> sp., creating a bioactive material for the transesterification of lipids in sewage sludge. Comprehensive characterization of the biocatalysts was conducted using Energy Dispersive Spectroscopy (EDS), Fourier Transform Infrared Spectroscopy (FTIR), and Field Emission Scanning Electron Microscopy (FE-SEM). Gas Chromatography-Mass Spectrometry (GC-MS) analysis of the resulting fatty acid methyl esters (FAMEs) demonstrated that the highest yield was achieved with the enzyme immobilized on the activated heterogeneous catalyst using methanol (99 %), followed by the activated heterogeneous catalyst with methanol (96 %), and methanol with Sulfuric acid (82 %). This study underscores the potential of utilizing municipal sewage sludge as a valuable resource for producing efficient heterogeneous catalysts, thereby advancing sustainable waste management practices and promoting renewable energy production.</div></div>","PeriodicalId":20743,"journal":{"name":"Process Safety and Environmental Protection","volume":null,"pages":null},"PeriodicalIF":6.9,"publicationDate":"2024-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142326990","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Soil utilization analysis of synergistic pyrolysis products of flue gas desulfurization gypsum and biomass 烟气脱硫石膏和生物质协同热解产物的土壤利用分析
IF 6.9 2区 环境科学与生态学
Process Safety and Environmental Protection Pub Date : 2024-09-25 DOI: 10.1016/j.psep.2024.09.103
{"title":"Soil utilization analysis of synergistic pyrolysis products of flue gas desulfurization gypsum and biomass","authors":"","doi":"10.1016/j.psep.2024.09.103","DOIUrl":"10.1016/j.psep.2024.09.103","url":null,"abstract":"<div><div>Flue gas desulfurization gypsum (FGDG) is one of the typical bulk solid wastes. With its vast production and considerable storage capacity, it accumulates in substantial quantities, occupies an extensive amount of land, and poses a severe pollutant threat to the ecological environment. To achieve large-scale consumption of FGDG, this study puts forward a method for the soil utilization and ecological reconstruction involving the co-pyrolysis of FGDG and biomass. The main emphasis is placed on exploring the alterations in leaching toxicity and plant-available elements under diverse conditions of temperature, biomass addition, and pyrolysis time. The co-pyrolysis parameters were optimized, and the changes in mineral composition of FGDG and biomass under different pyrolysis circumstances were investigated using XRD and SEM characterization methods. The experimental outcomes demonstrated that the optimal pyrolysis conditions were a temperature of 700 °C, a biomass content of 60 %, and a pyrolysis time of 5 h. The toxic and harmful substances within FGDG were solidified and stabilized, achieving a harmless treatment of FGDG. Simultaneously, the usable elements for plants were released. Through the analysis of mineral composition and microstructure, it was discovered that the pyrolysis products contain a considerable amount of CaSO<sub>4</sub> and C, and the microstructure mainly consists of porous aggregates. The reason for the reduced leaching efficiency of toxic and harmful substances might be attributed to the formation of stable minerals such as heavy metals through crystallization and vitrification mineralization after the removal of crystal water from FGDG. Under the reduction effect of C, the available elements for plants are liberated. This study furnishes a theoretical basis for the industrial application of FGDG and biomass for large-scale soil utilization treatment.</div></div>","PeriodicalId":20743,"journal":{"name":"Process Safety and Environmental Protection","volume":null,"pages":null},"PeriodicalIF":6.9,"publicationDate":"2024-09-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142327107","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dispersion and explosion characteristics of multi-phase fuel with different charge structure 不同装料结构的多相燃料的分散和爆炸特性
IF 6.9 2区 环境科学与生态学
Process Safety and Environmental Protection Pub Date : 2024-09-24 DOI: 10.1016/j.psep.2024.09.096
{"title":"Dispersion and explosion characteristics of multi-phase fuel with different charge structure","authors":"","doi":"10.1016/j.psep.2024.09.096","DOIUrl":"10.1016/j.psep.2024.09.096","url":null,"abstract":"<div><div>The fuel dispersion and explosion laws are important for safety design of fuel charge, concentration prediction of accidental release vapor cloud and prevention of fire and explosion accidents. The charge structure is an important factor in determining the fuel dispersion and explosion performance. Experiments and numerical simulations are carried out for cylindrical, square and fan-shaped charge structures. The dispersion process, concentration distribution, explosion overpressure, component reaction and safety radius of 11 kg solid-liquid-gas propylene oxide (PO) are obtained. The results show that square and fan-shaped structure have local enhancement effect. Compared with cylindrical structure, the dispersion distance of square at 0° and fan-shape at 45° increase by 10.13 % and 14.39 % respectively. The peak overpressure increased by 8.85 % and 4.73 %. At 4 m, the remaining fuel of the three structures is 39.13 %, 22.34 % and 17.20 %, respectively. The equivalent safety radius is 14.20 m, 14.80 m and 14.27 m respectively.</div></div>","PeriodicalId":20743,"journal":{"name":"Process Safety and Environmental Protection","volume":null,"pages":null},"PeriodicalIF":6.9,"publicationDate":"2024-09-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142319136","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Optimizing multivariate alarm systems: A study on joint false alarm rate, and joint missed alarm rate using linear programming technique 优化多元报警系统:利用线性规划技术研究联合误报率和联合漏报率
IF 6.9 2区 环境科学与生态学
Process Safety and Environmental Protection Pub Date : 2024-09-23 DOI: 10.1016/j.psep.2024.09.078
{"title":"Optimizing multivariate alarm systems: A study on joint false alarm rate, and joint missed alarm rate using linear programming technique","authors":"","doi":"10.1016/j.psep.2024.09.078","DOIUrl":"10.1016/j.psep.2024.09.078","url":null,"abstract":"<div><div>In modern complex industrial systems, multiple process variables interact with one another. The role of alarm systems in ensuring the safety of these systems is of utmost importance. Consequently, there is an increasing value placed on the assessment of the performance of multivariate alarm systems. As the dimensions of the system and the number of variables grow, designing optimal parameters for the multivariate alarm system using traditional approaches such as probability density function estimation becomes increasingly convoluted. In this paper, an approximate method is proposed for calculating two indices known as the Joint False Alarm Rate (JFAR) and Joint Missed Alarm Rate (JMAR), which are used to evaluate the performance of multivariate alarm systems. These indices are computed using the multivariate Markov chain method. The Markov chain is constructed by solving an optimal Linear Programming (LP) problem. Subsequently, joint indices are defined based on steady state estimations of a multivariate Markov chain. To validate the theoretical results obtained on the JFAR and JMAR and to demonstrate the proposed performance assessment and alarm system design procedures, numerical example and an industrial case study are provided.</div></div>","PeriodicalId":20743,"journal":{"name":"Process Safety and Environmental Protection","volume":null,"pages":null},"PeriodicalIF":6.9,"publicationDate":"2024-09-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142322051","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A new catalyst derived from the sulfur-doped metal-organic framework for Fenton-like reaction 源自掺硫金属有机框架的新型催化剂,可用于类芬顿反应
IF 6.9 2区 环境科学与生态学
Process Safety and Environmental Protection Pub Date : 2024-09-21 DOI: 10.1016/j.psep.2024.09.082
{"title":"A new catalyst derived from the sulfur-doped metal-organic framework for Fenton-like reaction","authors":"","doi":"10.1016/j.psep.2024.09.082","DOIUrl":"10.1016/j.psep.2024.09.082","url":null,"abstract":"<div><div>Fenton-like reaction exhibits considerable advantages in the remediation of pollutants. To fabricate an efficient catalyst becomes an issue concerning the performance enhancement in Fenton-like reaction. Herein, S-Fe-MOF-400 which was derived from a sulfur-doped metal-organic framework (Fe-MOF), was newly prepared and exhibited high ability for H<sub>2</sub>O<sub>2</sub> activation during Fenton-like reaction. The results showed that the sulfurization effectively reduced the charge transfer resistance (<em>R</em><sub><em>ct</em></sub>) of S-Fe-MOF-400, and facilitated the charge transfer, consequently enhancing the catalytic performance of S-Fe-MOF-400 in the Fenton-like reaction. XRD analysis revealed that FeS<sub>2</sub> was the predominant reactive component in S-Fe-MOF-400 with a regular cubic structure and pronounced crystallinity. Additionally, the presence of low-valent sulfur ensured the availability of Fe (II), thereby facilitating the occurrence of the Fenton reaction. Under optimal conditions, the removal efficiency of pollutants reached 86.7 % within 60 min, resulting in total organic carbon (TOC) removal efficiency at 40.6 %. Quenching experiments and electron paramagnetic resonance (EPR) detections revealed that <sup>•</sup>OH, <sup>1</sup>O<sub>2</sub>, and <span><math><msubsup><mrow><mtext>O</mtext></mrow><mrow><mn>2</mn></mrow><mrow><mtext>•</mtext><mo>−</mo></mrow></msubsup></math></span> synergistically participated in the Fenton-like reaction<sup>,</sup> with <sup>•</sup>OH being the primary active species. The activation process of H<sub>2</sub>O<sub>2</sub> induced by S-Fe-MOF-400 mainly yielded hydroxyl radicals and superoxide radicals. The <sup>1</sup>O<sub>2</sub> was generated through two following pathways: (i) the transformation of superoxide and hydroxyl radicals, and (ii) the conversion of natural oxygen molecules (O<sub>2</sub>). This current study illustrated the significant potential for the application of sulfur-modified Fe-MOF in the Fenton-like reaction for pollutant removal.</div></div>","PeriodicalId":20743,"journal":{"name":"Process Safety and Environmental Protection","volume":null,"pages":null},"PeriodicalIF":6.9,"publicationDate":"2024-09-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142314989","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Exploring the composition and function profiles of bacteria from wood- and soil-feeding termites for effective degradation of lignin-based aromatics 探索食木白蚁和食土白蚁细菌的组成和功能特征,以有效降解木质素类芳香烃
IF 6.9 2区 环境科学与生态学
Process Safety and Environmental Protection Pub Date : 2024-09-20 DOI: 10.1016/j.psep.2024.09.081
{"title":"Exploring the composition and function profiles of bacteria from wood- and soil-feeding termites for effective degradation of lignin-based aromatics","authors":"","doi":"10.1016/j.psep.2024.09.081","DOIUrl":"10.1016/j.psep.2024.09.081","url":null,"abstract":"<div><div>Lignocellulosic biomass (LCB) in the form of agricultural, forestry, and agro-industrial wastes is globally generated in large volumes every year. The chemical components of lignocellulosic biomass render them a substrate valuable for biofuel production. However, the rigid association of lignin, cellulose, and hemicellulose component of LCB forms a complex, hierarchical, and recalcitrant structure, which inhibits the solubilization of LCB resources for biofuel production. The learning from termites (wood-feeding and soil-feeding) and further application of their gut bacteria for lignin degradation and bioconversion remain unexplored or at its early stage. With reference to this scientific knowledge gap, this study seeks to highlight the culturable gut bacterial community in soil- and wood-feeding termites, namely <em>Pericapritermes nitobei</em> and <em>Microcerotermes</em> sp., respectively to design a future biorefinery and bioremediation technologies. In this study, a total of 40 and 67 bacterial isolates were indeed identified from <em>Pericapritermes nitobei</em> and <em>Microcerotermes</em> sp., respectively. The identified isolates from both termite species were actually classified into four different phyla: Actinobacteria, Proteobacteria, Firmicutes, and Bacteroidetes, where the phylum Actinobacteria dominated gut bacteria isolates identified from <em>P. nitobei</em> at 47.5 % while Proteobacteria were dominant in wood-feeding termite, <em>Microcerotermes</em> sp. at 46.27 %. At the genus level, the bacterial isolates enriched from the gut of <em>Microcerotermes</em> sp. belonged to 17 different genera, among which the bacterial genus <em>Streptomyces</em> (28 %) was most prevalent, followed by <em>Enterobacter</em> (11 %). Meanwhile, 9 genera were recorded for gut bacterial isolates from <em>P. nitobei</em> and were dominated by <em>Streptomyces</em> (37.5 %), followed by <em>Acinetobacter</em> (25 %). In general, the gut bacterial symbionts from both termites showed a congruency at the phyla level but were more diverged at a lower classification, inferring that different termite species evolved a unique repertoire of gut bacteria. Moreover, 61 % and 55 % of the gut bacterial isolates from the wood- and soil-feeding termites demonstrated a significant and multifunctional role in the hydrolysis of three lignocellulolytic substrates, including carboxymethyl cellulose, beechwood xylan, and aniline blue dye, indicating their unique functions and assistance to the host for the degradation of lignocellulose or other xenobiotic compounds from soil.</div></div>","PeriodicalId":20743,"journal":{"name":"Process Safety and Environmental Protection","volume":null,"pages":null},"PeriodicalIF":6.9,"publicationDate":"2024-09-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142314990","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Chloridizing roasting studies of spent NdFeB magnets for recovery of rare earth values 回收稀土价值的废钕铁硼磁体氯化焙烧研究
IF 6.9 2区 环境科学与生态学
Process Safety and Environmental Protection Pub Date : 2024-09-19 DOI: 10.1016/j.psep.2024.09.053
{"title":"Chloridizing roasting studies of spent NdFeB magnets for recovery of rare earth values","authors":"","doi":"10.1016/j.psep.2024.09.053","DOIUrl":"10.1016/j.psep.2024.09.053","url":null,"abstract":"<div><p>The increased demand for rare earth elements in advanced technological applications and supply shortages call for metal recovery from secondary sources. Permanent magnet (Nd<sub>2</sub>Fe<sub>14</sub>B or NdFeB) may serve as a potential secondary source due to its high rare earth (Nd+Pr+Dy: ∼30 %) content and its vast application. The present study utilizes a chloridizing roasting (CaCl<sub>2</sub>.2 H<sub>2</sub>O) pre-treatment process followed by water leaching, acid leaching (0.5 M HCl, S/L =1/10 g/ml, 90 °C, 3 h), oxalic acid precipitation and calcination (850 °C, 2 h) to obtain mixed rare earth oxides. The process was optimized based on temperature (400–700 °C), dosage (CaCl<sub>2</sub>.2H<sub>2</sub>O: NdFeB=0.5:1–2.5:1), and time (30–120 min) on the rare earth dissolution. The theoretical activation energy for the chloridizing roasting process is estimated as 22.3 (OFW) and 16.7 kJ/mol (KAS), while the experimental activation energy for Nd and Dy dissolution was determined to ∼29.3 and ∼17.7 kJ/mol, respectively depicting product layer diffusion-controlled kinetics. Higher dosages of CaCl<sub>2</sub>.2H<sub>2</sub>O (1.5:1 and 2:1) favored NdOCl formation, thereby, higher dissolution; however, further higher dosage (2.5:1) leads to reduced Nd dissolution due to higher CaO formation and acid consumption by Ca during leaching. Incomplete oxidation at lower temperatures (400 °C) and iron dissolution impair the Nd dissolution and selectivity. Excessive oxidation at &gt;700 °C favors the formation of NdFeO<sub>3</sub>, decreasing Nd dissolution. The maximum dissolution of Nd was ∼89 %, while for Dy, it was ∼88 % at optimum conditions of 600 °C, 90 min, 2:1. Water leaching post-roasting leads to ∼87 % Ca removal and the precipitation efficiency of rare earth oxalates was 99 %. The overall extraction for rare earth elements was ∼89 %, and 1 kg of NdFeB powder can yield ∼285 g of rare earth oxides (∼239 g Nd<sub>2</sub>O<sub>3</sub>, ∼14 g Dy<sub>2</sub>O<sub>3</sub>) with 96 % purity. Further, this study demonstrates that using CaCl<sub>2</sub>.2 H<sub>2</sub>O as a solid chlorinating agent in chlorination roasting enhances recovery rates of mixed rare earth oxides while providing a safer and more environment-friendly alternative for industrial applications.</p></div>","PeriodicalId":20743,"journal":{"name":"Process Safety and Environmental Protection","volume":null,"pages":null},"PeriodicalIF":6.9,"publicationDate":"2024-09-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142274297","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Enhanced selectivity of reactive intermediates by modifying electrodes with layered materials for the green high-salinity wastewater treatment 利用层状材料改性电极提高反应中间体的选择性,实现绿色高盐度废水处理
IF 6.9 2区 环境科学与生态学
Process Safety and Environmental Protection Pub Date : 2024-09-19 DOI: 10.1016/j.psep.2024.09.075
{"title":"Enhanced selectivity of reactive intermediates by modifying electrodes with layered materials for the green high-salinity wastewater treatment","authors":"","doi":"10.1016/j.psep.2024.09.075","DOIUrl":"10.1016/j.psep.2024.09.075","url":null,"abstract":"<div><p>Improving the selectivity of the reactive intermediates such as <span><math><msup><mrow><mi>ClO</mi></mrow><mrow><mo>−</mo></mrow></msup></math></span> and <span><math><mrow><mi>•</mi><mi>OH</mi></mrow></math></span> by modifying nickel foam electrodes with ion exchangeable layered materials would greatly enhance the efficiency of high-salinity wastewater treatment. A universal pattern was verified herein that through functioning as a permeable overlayer regulating the transport of cations/anions, <span><math><msup><mrow><mi>ClO</mi></mrow><mrow><mo>−</mo></mrow></msup></math></span> and <span><math><mrow><mi>•</mi><mi>OH</mi></mrow></math></span> could be the predominant intermediates in the anionic/cationic layered material modified electrode. The significance of selectivity enhancement includes improving electrochemical efficiency and reducing the usage of chemical reagents. For instance, it is demonstrated that electrochemically degrading high salinity azo wastewater using decorated electrodes would be as effective as chemical treatment. Furthermore, electrochemical oxidation using cation layered material modified electrode could reduce the pKa of the oxidized cellulose filter paper as effectively as using <span><math><msub><mrow><msub><mrow><mi>H</mi></mrow><mrow><mn>2</mn></mrow></msub><mi>O</mi></mrow><mrow><mn>2</mn></mrow></msub></math></span>.</p></div>","PeriodicalId":20743,"journal":{"name":"Process Safety and Environmental Protection","volume":null,"pages":null},"PeriodicalIF":6.9,"publicationDate":"2024-09-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142274482","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Study on the purification of aquaculture tailwater under Sulfamethoxazole stress using algae-bacteria biofilms: Nutrient removal efficiency, microbial community, and ARGs 利用藻菌生物膜净化磺胺甲噁唑胁迫下的水产养殖尾水的研究:营养物去除效率、微生物群落和 ARGs
IF 6.9 2区 环境科学与生态学
Process Safety and Environmental Protection Pub Date : 2024-09-19 DOI: 10.1016/j.psep.2024.09.067
{"title":"Study on the purification of aquaculture tailwater under Sulfamethoxazole stress using algae-bacteria biofilms: Nutrient removal efficiency, microbial community, and ARGs","authors":"","doi":"10.1016/j.psep.2024.09.067","DOIUrl":"10.1016/j.psep.2024.09.067","url":null,"abstract":"<div><p>This study explored the dynamic processes of algae-bacteria biofilms in the remediation of aquaculture pond effluents as a novel treatment strategy. The purification capacity of the biofilms, changes in community composition, and their impact on the dissemination of antibiotic resistance genes (ARGs) were investigated under the application of <em>sul</em>famethoxazole (SMX) at concentrations ranging from 100 to 1000 μg/L. The study also considered the factors influencing the abundance and diversity of ARGs and mobile genetic elements (MGEs) across different seasons, including the roles of environmental parameters and microbial community structure.The results showed that, although exposure to SMX reduced nutrient removal efficiency, photosynthetic activity, and increased oxidative stress levels, the biofilms maintained relatively high purification efficiency (with nutrient removal rates ranging from 67.62 % to 93.23 % and SMX removal rate reaching 50.13 % ± 12.34 %), demonstrating adaptability to SMX stress. Network analysis identified key microbial carriers responsible for ARG dissemination, highlighting the complex interactions between environmental factors, microbial communities, and resistance gene propagation. These findings enhance our understanding of biofilm-based water treatment systems and the seasonal factors affecting the dynamics of ARGs and MGEs.</p></div>","PeriodicalId":20743,"journal":{"name":"Process Safety and Environmental Protection","volume":null,"pages":null},"PeriodicalIF":6.9,"publicationDate":"2024-09-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142274379","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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