Petroleum SciencePub Date : 2024-10-01DOI: 10.1016/j.petsci.2024.02.019
{"title":"Characterization of chemical composition of high viscosity heavy oils: Macroscopic properties, and semi-quantitative analysis of molecular composition using high-resolution mass spectrometry","authors":"","doi":"10.1016/j.petsci.2024.02.019","DOIUrl":"10.1016/j.petsci.2024.02.019","url":null,"abstract":"<div><div>Heavy oil is an important resource in current petroleum exploitation, and the chemical composition information of heavy oil is crucial for revealing its viscosity-inducing mechanism and solving practical exploitation issues. In this study, the techniques of high-temperature gas chromatography and high-resolution mass spectrometry equipped with an electrospray ionization source were applied to reveal the chemical composition of typical heavy oils from western, central, and eastern China. The results indicate that these heavy oils display significant variations in their bulk properties, with initial boiling points all above 200 °C. Utilizing pre-treatment and ESI high-resolution mass spectrometry, an analysis of the molecular composition of saturated hydrocarbons, aromatic hydrocarbons, acidic oxygen compounds, sulfur compounds, basic nitrogen compounds, and neutral nitrogen compounds within the heavy oil was conducted. Ultimately, a semi-quantitative analysis of the molecular composition of the heavy oil was achieved by integrating the elemental content. The semi-quantitative analysis results of Shengli-J8 heavy oil and a conventional Shengli crude oil show that Shengli-J8 heavy oil lacks alkanes and low molecular weight aromatic hydrocarbons, which contributes to its high viscosity. Additionally, characteristic molecular sets for different heavy oils were identified based on the semi-quantitative analysis of molecular composition. The semi-quantitative analysis of molecular composition in heavy oils may provide valuable reference data for establishing theoretical models on the viscosity-inducing mechanism in heavy oils and designing viscosity-reducing agents for heavy oil exploitation.</div></div>","PeriodicalId":19938,"journal":{"name":"Petroleum Science","volume":null,"pages":null},"PeriodicalIF":6.0,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140044634","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Petroleum SciencePub Date : 2024-10-01DOI: 10.1016/j.petsci.2024.05.014
{"title":"Optimal depth of in-situ pressure-preserved coring in coal seams considering roadway excavation and drilling disturbance","authors":"","doi":"10.1016/j.petsci.2024.05.014","DOIUrl":"10.1016/j.petsci.2024.05.014","url":null,"abstract":"<div><div>Using pressure-preserved coring technique to determine in-situ gas content provides a more precise assessment of gas resource reserves and safeguard of mining safety in coal seams. How coring technique and depth affect the determination of gas content is unclear due to borehole zoning rupture caused by roadway excavation and drilling disturbance. To this end, a proposed coupling model of stress distribution and gas migration was simulated and validated by FLAC<sup>3D</sup> and COMSOL Multiphysics considering superposition effects of roadway excavation and drilling disturbance. The findings indicate that the roadway surrounding rock displays distinct zoning features including stress relief zone, stress concentration zone that is composed of plastic zone, elastic zone, and original stress zone; and the broken situations depending on the borehole peeping are consistent with the corresponding simulation results. On this basis, this study proposes a set of drilling coring depth calculation and prediction model for the gas desorption affected area under engineering disturbance. Optimal depth of coring drilling is not only approach to the in-situ coal bulk, but also can get the balance of the drilling workload and cost controlling. According to the typical mine site geological conditions and the numerical simulation results in this study, if the roadway excavation time is ∼1 year, it is recommended that the pressure-preserved coring depth should be greater than 17 m.</div></div>","PeriodicalId":19938,"journal":{"name":"Petroleum Science","volume":null,"pages":null},"PeriodicalIF":6.0,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141140238","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Petroleum SciencePub Date : 2024-10-01DOI: 10.1016/j.petsci.2024.08.001
Rui-Shuai Ma , Ji-Yuan Zhang , Qi-Hong Feng , Xue-Ying Zhang , Yan-Hui Yang
{"title":"Effect of cyclic hydraulic stimulation on pore structure and methane sorption characteristics of anthracite coal: A case study in the Qinshui Basin, China","authors":"Rui-Shuai Ma , Ji-Yuan Zhang , Qi-Hong Feng , Xue-Ying Zhang , Yan-Hui Yang","doi":"10.1016/j.petsci.2024.08.001","DOIUrl":"10.1016/j.petsci.2024.08.001","url":null,"abstract":"<div><div>The cyclic hydraulic stimulation (CHS) has proven as a prospective technology for enhancing the permeability of unconventional formations such as coalbeds. However, the effects of CHS on the microstructure and gas sorption behavior of coal remain unclear. In this study, laboratory tests including the nuclear magnetic resonance (NMR), low-temperature nitrogen sorption (LTNS), and methane sorption isotherm measurement were conducted to explore changes in the pore structure and methane sorption characteristics caused by CHS on an anthracite coal from Qinshui Basin, China. The NMR and LTNS tests show that after CHS treatment, meso- and macro-pores tend to be enlarged, whereas micro-pores with larger sizes and transition-pores may be converted into smaller-sized micro-pores. After the coal samples treated with 1, 3, 5 and 7 hydraulic stimulation cycles, the total specific surface area (TSSA) decreased from 0.636 to 0.538, 0.516, 0.505, and 0.491 m<sup>2</sup>/g, respectively. Fractal analysis based on the NMR and LTNS results show that the surface fractal dimensions increase with the increase in the number of hydraulic stimulation cycles, while the volume fractal dimensions exhibit an opposite trend to the surface fractal dimensions, indicating that the pore surface roughness and pore structure connectivity are both increased after CHS treatment. Methane sorption isothermal measurements show that both the Langmuir volume and Langmuir pressure decrease significantly with the increase in the number of hydraulic stimulation cycles. The Langmuir volume and the Langmuir pressure decrease from 33.47 cm<sup>3</sup>/g and 0.205 MPa to 24.18 cm<sup>3</sup>/g and 0.176 MPa after the coal samples treated with 7 hydraulic stimulation cycles, respectively. The increments of Langmuir volume and Langmuir pressure are positively correlated with the increment of TSSA and negatively correlated with the increments of surface fractal dimensions.</div></div>","PeriodicalId":19938,"journal":{"name":"Petroleum Science","volume":null,"pages":null},"PeriodicalIF":6.0,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142180077","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Petroleum SciencePub Date : 2024-10-01DOI: 10.1016/j.petsci.2024.04.002
{"title":"Efficient anti-aliasing and anti-leakage Fourier transform for high-dimensional seismic data regularization using cube removal and GPU","authors":"","doi":"10.1016/j.petsci.2024.04.002","DOIUrl":"10.1016/j.petsci.2024.04.002","url":null,"abstract":"<div><div>Seismic data is commonly acquired sparsely and irregularly, which necessitates the regularization of seismic data with anti-aliasing and anti-leakage methods during seismic data processing. We propose a novel method of 4D anti-aliasing and anti-leakage Fourier transform using a cube-removal strategy to address the combination of irregular sampling and aliasing in high-dimensional seismic data. We compute a weighting function by stacking the spectrum along the radial lines, apply this function to suppress the aliasing energy, and then iteratively pick the dominant amplitude cube to construct the Fourier spectrum. The proposed method is very efficient due to a cube removal strategy for accelerating the convergence of Fourier reconstruction and a well-designed parallel architecture using CPU/GPU collaborative computing. To better fill the acquisition holes from 5D seismic data and meanwhile considering the GPU memory limitation, we developed the anti-aliasing and anti-leakage Fourier transform method in 4D with the remaining spatial dimension looped. The entire workflow is composed of three steps: data splitting, 4D regularization, and data merging. Numerical tests on both synthetic and field data examples demonstrate the high efficiency and effectiveness of our approach.</div></div>","PeriodicalId":19938,"journal":{"name":"Petroleum Science","volume":null,"pages":null},"PeriodicalIF":6.0,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140778175","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Petroleum SciencePub Date : 2024-10-01DOI: 10.1016/j.petsci.2024.05.019
{"title":"Characteristics, preservation mechanisms, and significance of aragonite in lacustrine shale: A case study from the Jiyang Depression, Bohai Bay Basin","authors":"","doi":"10.1016/j.petsci.2024.05.019","DOIUrl":"10.1016/j.petsci.2024.05.019","url":null,"abstract":"<div><div>Aragonite is a metastable mineral, which is easily transformed into calcite, and generally difficult to preserve in the stratum. However, large amounts of aragonites were found in the Paleogene shale of the Jiyang Depression. The characteristics and preservation mechanisms of these aragonites were analyzed through a series of analytical methods, including cathodoluminescence, field-emission scanning electron microscopy (FESEM), laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS), micro-area carbon and oxygen isotopes, Sr isotopes, and dissolution simulation experiments under high temperature and high pressure. The research results show that: ①Aragonite in the Paleogene shale of the Jiyang Depression is related to algal microbial fossils, primarily composed of coccoliths and characterized by two emission peaks at 420 nm and 480 nm in cathodoluminescence; ②The primary factor allowing biological aragonite to be preserved is the immaturity of the organic matter and the deficiency of abundant organic acids necessary for its dissolution or transformation, which is confirmed by the evidence of organic matter maturity and simulation experiments of organic acid dissolution on aragonite under high-temperature and high-pressure conditions. Additional factors that may aid in the preservation of aragonite are the ideal sedimentation conditions, the defense of organic coating, and the enclosed environment with tiny pores, low porosity, and low permeability; ③These aragonite-rich shales, characterized by coccolithophores, provide a solid evidence for seawater intrusion into terrestrial lake basin, and have a significant implication for the source and storage of shale oil.</div></div>","PeriodicalId":19938,"journal":{"name":"Petroleum Science","volume":null,"pages":null},"PeriodicalIF":6.0,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141138172","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Petroleum SciencePub Date : 2024-10-01DOI: 10.1016/j.petsci.2024.05.023
Cheng Liu , Biao Zhou , Bing-Shan Wang , Huan Wang , Qing You , Guang Zhao , Cai-Li Dai
{"title":"Synthesis of temperature and salt resistance silicon dots for effective enhanced oil recovery in tight reservoir","authors":"Cheng Liu , Biao Zhou , Bing-Shan Wang , Huan Wang , Qing You , Guang Zhao , Cai-Li Dai","doi":"10.1016/j.petsci.2024.05.023","DOIUrl":"10.1016/j.petsci.2024.05.023","url":null,"abstract":"<div><div>The intensive development of tight reservoirs has positioned them as a strategic alternative to conventional oil and gas resources. Existing enhanced oil recovery (EOR) methods struggle to effectively exploring reservoir oil, resulting in low recovery rates. Novel and effective means of developing tight reservoirs are urgently needed. Nanomaterials have shown promising applications in improving water flooding efficiency, with in-depth research into mechanisms that lower injection pressure and increase water injection volumes. However, the extent of improvement remains limited. In this study, a silicon quantum dots (Si-QDs) material was synthesized via a hydrothermal synthesis method and used to prepare a nanofluid for the efficient recovery of tight reservoir. The Si-QDs, with an approximate diameter of 3 nm and a spherical structure, were surface functionalized with benzenesulfonic acid groups to enhance the performance. The developed nanofluid demonstrated stability without aggregation at 120 °C and a salinity of 60000 mg/L. Core flooding experiments have demonstrated the attractive EOR capabilities of Si-QDs, shedding light of the EOR mechanisms. Si-QDs effectively improve the wettability of rocks, enhancing the sweeping coefficient of injected fluids and expanding sweeping area. Within this sweeping region, Si-QDs efficiently stripping adsorbed oil from the matrix, thus increasing sweeping efficiency. Furthermore, Si-QDs could modify the state of pore-confined crude oil, breaking it down into smaller particles that are easier to displacement in subsequent stages. Si-QDs exhibit compelling EOR potential, positioning them as a promising approach for effectively developing tight oil reservoirs.</div></div>","PeriodicalId":19938,"journal":{"name":"Petroleum Science","volume":null,"pages":null},"PeriodicalIF":6.0,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141781352","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Evaluation of the combined influence of geological layer property and in-situ stresses on fracture height growth for layered formations","authors":"Peng Tan , Zhao-Wei Chen , Liu-Ke Huang , Qing Zhao , Sha-Rui Shao","doi":"10.1016/j.petsci.2024.07.014","DOIUrl":"10.1016/j.petsci.2024.07.014","url":null,"abstract":"<div><div>Fracture geometry is important when stimulating low-permeability reservoirs for natural gas or oil production. The geological layer (GL) properties and contrasts in in-situ stress are the two most important parameters for determination of the vertical fracture growth extent and containment in layered rocks. However, the method for assessing the cumulative impact on growth in height remains ambiguous. In this research, a 3D model based on the cohesive zone method is used to simulate the evolution of hydraulic fracture (HF) height in layered reservoirs. The model incorporates fluid flow and elastic deformation, considering the friction between the contacting fracture surfaces and the interaction between fracture components. First, an analytical solution that was readily available was used to validate the model. Afterwards, a quantitative analysis was performed on the combined impacts of the layer interface strength, coefficient of interlayer stress difference, and coefficient of vertical stress difference. The results indicate that the observed fracture height geometries can be categorized into three distinct regions within the parametric space: blunted fracture, crossed fracture, and T-shaped fracture. Furthermore, the results explained the formation mechanism of the low fracture height in the deep shale reservoir of the Sichuan Basin, China, as well as the distinction between fracture network patterns in mid-depth and deep shale reservoirs.</div></div>","PeriodicalId":19938,"journal":{"name":"Petroleum Science","volume":null,"pages":null},"PeriodicalIF":6.0,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141691111","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Petroleum SciencePub Date : 2024-10-01DOI: 10.1016/j.petsci.2024.06.014
Hong-Yong Yan
{"title":"Seismic modeling by combining the finite-difference scheme with the numerical dispersion suppression neural network","authors":"Hong-Yong Yan","doi":"10.1016/j.petsci.2024.06.014","DOIUrl":"10.1016/j.petsci.2024.06.014","url":null,"abstract":"<div><div>Seismic finite-difference (FD) modeling suffers from numerical dispersion including both the temporal and spatial dispersion, which can decrease the accuracy of the numerical modeling. To improve the accuracy and efficiency of the conventional numerical modeling, I develop a new seismic modeling method by combining the FD scheme with the numerical dispersion suppression neural network (NDSNN). This method involves the following steps. First, a training data set composed of a small number of wavefield snapshots is generated. The wavefield snapshots with the low-accuracy wavefield data and the high-accuracy wavefield data are paired, and the low-accuracy wavefield snapshots involve the obvious numerical dispersion including both the temporal and spatial dispersion. Second, the NDSNN is trained until the network converges to simultaneously suppress the temporal and spatial dispersion. Third, the entire set of low-accuracy wavefield data is computed quickly using FD modeling with the large time step and the coarse grid. Fourth, the NDSNN is applied to the entire set of low-accuracy wavefield data to suppress the numerical dispersion including the temporal and spatial dispersion. Numerical modeling examples verify the effectiveness of my proposed method in improving the computational accuracy and efficiency.</div></div>","PeriodicalId":19938,"journal":{"name":"Petroleum Science","volume":null,"pages":null},"PeriodicalIF":6.0,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141936657","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Petroleum SciencePub Date : 2024-10-01DOI: 10.1016/j.petsci.2024.03.020
{"title":"Morphological complexity and azimuthal disorder of evolving pore space in low-maturity oil shale during in-situ thermal upgrading and impacts on permeability","authors":"","doi":"10.1016/j.petsci.2024.03.020","DOIUrl":"10.1016/j.petsci.2024.03.020","url":null,"abstract":"<div><div>In-situ thermal upgrading is used to tune the pore system in low-maturity oil shales. We introduce fractal dimension (<em>D</em>), form factor (<em>ff</em>) and stochastic entropy (<em>H</em>) to quantify the heating-induced evolution of pore morphological complexity and azimuthal disorder and develop a model to estimate the impact on seepage capacity via permeability. Experiments are conducted under recreated in-situ temperatures and consider anisotropic properties—both parallel and perpendicular to bedding. Results indicate that azimuthal distribution of pores in the bedding-parallel direction are dispersed, while those in the bedding-perpendicular direction are concentrated. <em>D</em> values indicate that higher temperatures reduce the uniformity of the pore size distribution (PSD) in the bedding-parallel direction but narrow the PSD in the bedding-perpendicular direction. The greater <em>ff</em> (> 0.7) values in the bedding-parallel direction account for a large proportion, while the dominated in the bedding-perpendicular direction locates within 0.2–0.7, for all temperatures. The <em>H</em> value of the bedding-parallel sample remains stable at ∼0.925 during heating, but gradually increases from 0.808 at 25 °C to 0.879 at 500 °C for the bedding-perpendicular sample. Congruent with a mechanistic model, the permeability at 500 °C is elevated ∼1.83 times (bedding-parallel) and ∼6.08 times (bedding-perpendicular) relative to that at 25 °C—confirming the effectiveness of thermal treatment in potentially enhancing production from low-maturity oil shales.</div></div>","PeriodicalId":19938,"journal":{"name":"Petroleum Science","volume":null,"pages":null},"PeriodicalIF":6.0,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140399314","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Petroleum SciencePub Date : 2024-10-01DOI: 10.1016/j.petsci.2024.04.010
{"title":"3D rock physics template-based probabilistic estimation of tight sandstone reservoir properties","authors":"","doi":"10.1016/j.petsci.2024.04.010","DOIUrl":"10.1016/j.petsci.2024.04.010","url":null,"abstract":"<div><div>Quantitative prediction of reservoir properties (e.g., gas saturation, porosity, and shale content) of tight reservoirs is of great significance for resource evaluation and well placements. However, the complex pore structures, poor pore connectivity, and uneven fluid distribution of tight sandstone reservoirs make the correlation between reservoir parameters and elastic properties more complicated and thus pose a major challenge in seismic reservoir characterization. We have developed a partially connected double porosity model to calculate elastic properties by considering the pore structure and connectivity, and to analyze these factors' influences on the elastic behaviors of tight sandstone reservoirs. The modeling results suggest that the bulk modulus is likely to be affected by the pore connectivity coefficient, while the shear modulus is sensitive to the volumetric fraction of stiff pores. By comparing the model predictions with the acoustic measurements of the dry and saturated quartz sandstone samples, the volumetric fraction of stiff pores and the pore connectivity coefficient can be determined. Based on the calibrated model, we have constructed a 3D rock physics template that accounts for the reservoir properties’ impacts on the P-wave impedance, S-wave impedance, and density. The template combined with Bayesian inverse theory is used to quantify gas saturation, porosity, clay content, and their corresponding uncertainties from elastic parameters. The application of well-log and seismic data demonstrates that our 3D rock physics template-based probabilistic inversion approach performs well in predicting the spatial distribution of high-quality tight sandstone reservoirs in southwestern China.</div></div>","PeriodicalId":19938,"journal":{"name":"Petroleum Science","volume":null,"pages":null},"PeriodicalIF":6.0,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140762172","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}