Jin-Mok Hur, Jungho Hur, Yung-Zun Cho, Chang Hwa Lee
{"title":"Thermodynamic study on the separation of strontium and barium from LWR spent fuel","authors":"Jin-Mok Hur, Jungho Hur, Yung-Zun Cho, Chang Hwa Lee","doi":"10.1016/j.net.2024.08.050","DOIUrl":"10.1016/j.net.2024.08.050","url":null,"abstract":"<div><div>The separation of high heat load fission products, such as alkaline earth metals, from nuclear spent fuel can significantly reduce the burden of spent fuel disposal. This study investigates the feasibility of separating strontium and barium from light water reactor spent fuel through non-aqueous processes. Process flows were developed for treating spent nuclear fuel by heating it at high temperatures to remove volatile nuclides, followed by chlorination with a chlorinating agent. The chlorinated products were then treated with a precipitating agent in LiCl-KCl molten salt for further separation. The remaining liquid was distilled to recover strontium and barium. Thermodynamic equilibrium calculations were conducted for the process flows. Under the conditions of the process flows, the chlorinating agents MgCl<sub>2</sub> and NH<sub>4</sub>Cl both converted SrO and BaO entirely into SrCl<sub>2</sub> and BaCl<sub>2</sub>, respectively. The precipitating agent Li<sub>2</sub>CO<sub>3</sub> exhibited superior separation effectiveness compared to Li<sub>3</sub>PO<sub>4</sub>. Thermodynamic calculations indicate that strontium and barium recovered by MgCl<sub>2</sub> chlorination, Li<sub>2</sub>CO<sub>3</sub> precipitation, and distillation will contain 0.18 %, 1.06 %, and 0.32 % impurities in terms of mass, radioactivity, and decay heat, respectively.</div></div>","PeriodicalId":19272,"journal":{"name":"Nuclear Engineering and Technology","volume":"57 2","pages":"Article 103181"},"PeriodicalIF":2.6,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142207229","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Qianxu Wang , Yuanlai Xie , Huihui Hong , Yang Zhu , Fang Wang , Kun Tian , Bin Li
{"title":"Analysis and optimization of LN2 two-phase flow in CRAFT NNBI cryopump","authors":"Qianxu Wang , Yuanlai Xie , Huihui Hong , Yang Zhu , Fang Wang , Kun Tian , Bin Li","doi":"10.1016/j.net.2024.08.047","DOIUrl":"10.1016/j.net.2024.08.047","url":null,"abstract":"<div><div>As an important component of Negative ion based Neutral Beam Injector (NNBI), the cryopump mainly provides a suitable vacuum environment for beam generation and transmission. In the paper, Liquid nitrogen (LN2) pipe structure models of two cryopumps were established for simulation and experimental studies. Thermal analysis of the thermal radiation shielding baffle (LN2 cooling) was carried out by Ansys steady-state thermal analysis software, while Fluent was used to simulate the two-phase flow in the LN2 pipeline, then the pressure drops, temperature, velocity, gas-phase volume fraction, and other parameters of the two pipeline structures were analyzed and compared. The simulation results show that the optimized structure B can reduce the pressure drop by 3 bar, the outlet temperature of structure A is 78.8 K, the outlet temperature of structure B is 79.2 K, the temperature difference is 0.4 K. The outlet velocity increases from 2.067 m/s to 4.947 m/s for Structure A, and from 1.096 m/s to 6.614 m/s for Structure B. The experiment results show that the outlet temperature of structure A is 79.4 K, meanwhile the outlet temperature of structure B is 80.1 K, the optimized structure B can reduce the pressure drop about 3 bar.</div></div>","PeriodicalId":19272,"journal":{"name":"Nuclear Engineering and Technology","volume":"57 2","pages":"Article 103178"},"PeriodicalIF":2.6,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142207241","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Do Yun Kim , Han-Seop Song , Jae-Ho Jeong , Seung-Hwan Yu
{"title":"Development of CFD porous model parameters of Korean PWR spent nuclear fuel assemblies for thermal analysis","authors":"Do Yun Kim , Han-Seop Song , Jae-Ho Jeong , Seung-Hwan Yu","doi":"10.1016/j.net.2024.09.014","DOIUrl":"10.1016/j.net.2024.09.014","url":null,"abstract":"<div><div>This study focused on developing and validating porous model parameters to accurately estimate the thermal behavior of spent nuclear fuel assemblies for computational fluid dynamics simulations. These assemblies are stored in Korean pressurized water reactors (PWRs) under dry storage conditions. Korean PWR fuel assemblies were categorized into four distinct types based on their configuration, facilitating the calculation of effective thermal conductivities and flow resistance coefficients. These parameters are crucial for simulating heat transfer and determining the peak cladding temperature (PCT), ensuring the thermal safety of stored nuclear fuel. The validation of the proposed porous model against explicit two-dimensional and three-dimensional simulations demonstrated its efficacy and reliability in enhancing the thermal analysis of spent fuel assemblies, highlighting the significance of accurately calculating the porous model parameters in the safety assessment of nuclear fuel storage. Furthermore, the study assessed the sensitivity of variables influencing temperature during spent nuclear fuel storage, focusing on flow resistance coefficients, control rod effect, and basket size. The findings revealed that variations in flow resistance and the presence of control rods minimally impacted PCT, whereas basket size significantly influenced temperature, underscoring its importance in the thermal analysis of nuclear fuel storage systems.</div></div>","PeriodicalId":19272,"journal":{"name":"Nuclear Engineering and Technology","volume":"57 2","pages":"Article 103211"},"PeriodicalIF":2.6,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143099601","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Analysis of Naturally Occurring Radioactive Material (NORM) in shifting earth layers in Piyungan, Bantul","authors":"Iqbal Nurrahim , Andang Widi Harto , Yohannes Sardjono , Isman Mulyadi Triatmoko , Zuhdi Ismail , Gede Sutresna Wijaya","doi":"10.1016/j.net.2024.08.055","DOIUrl":"10.1016/j.net.2024.08.055","url":null,"abstract":"<div><div>In recent decades, understanding the correlation between radon gas emissions and geodynamic processes has been pivotal in enhancing geophysical monitoring. This study advances current methodologies by refining radon data analysis and employing mathematical models to further elucidate this relationship. We developed a radon well geometry for Piyungan using Finite Element Method principles, and conducted simulations via GNU Octave to assess normal and anomalous conditions. The results indicate a basal radon concentration of 2.2420 Bq/L at a depth of 14.2308 m. Notably, radon levels inversely correlate with the water volume and diffusivity, yet proportionally increase with soil moisture. These findings offer a nuanced understanding of radon behavior in response to geodynamic activity, paving the way for improved environmental monitoring.</div></div>","PeriodicalId":19272,"journal":{"name":"Nuclear Engineering and Technology","volume":"57 2","pages":"Article 103186"},"PeriodicalIF":2.6,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143099929","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Differentiated influences of perceived benefit types of nuclear power on its acceptance: Evidence from South Korea","authors":"Jin Won Lee , Hailin Zhang , Seungkook Roh","doi":"10.1016/j.net.2024.09.017","DOIUrl":"10.1016/j.net.2024.09.017","url":null,"abstract":"<div><div>Perceived benefits and risk of nuclear power have received considerable attention as influencing factors in public acceptance of nuclear power. The validation of the differential effects of these perceptions across contexts can provide implications for public communication strategies. This study is based on the similarity and dissimilarity between nuclear benefits and risk in their consequences. It posits that the pattern of the effect of environmental benefit perception on nuclear power acceptance is more similar to that of risk perception than to that of energy supply benefit perception, which is another type of benefit perception. Upon analyzing a national survey data from South Korea, we discovered the following: (1) regarding nuclear power as a non-dispreferred option, all the benefit perceptions and the risk perception exhibited a significant effect; (2) however, regarding nuclear power as the favorite option, the perception of environmental benefit and that of risk demonstrated a significant effect, but that of energy supply benefit did not. These findings have implications for both public communication strategies and theoretical considerations in future studies.</div></div>","PeriodicalId":19272,"journal":{"name":"Nuclear Engineering and Technology","volume":"57 2","pages":"Article 103214"},"PeriodicalIF":2.6,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143099940","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Ayman M. Sharaf , M.A. El-Nahal , Islam M. Nabil , I.H. Saleh , Mohamed Elsafi
{"title":"Development of simplified treatment methods for removal of Ra-226 and Ra-228 from sludge waste produced in natural gas processing plants","authors":"Ayman M. Sharaf , M.A. El-Nahal , Islam M. Nabil , I.H. Saleh , Mohamed Elsafi","doi":"10.1016/j.net.2024.08.044","DOIUrl":"10.1016/j.net.2024.08.044","url":null,"abstract":"<div><div>The present study aims to establish a new treatment method for removing or reducing the concentration of <sup>226</sup>Ra and <sup>228</sup>Ra in sludge waste produced due to natural gas production at natural gas processing Plants. The main radionuclides present in sludge waste of natural gas processing are Radium and its daughters due to their low solubility in the water they can form compounds with sulfate ions, carbonate ions, silicate ions, then precipitation scale or sludge. The suggested method is designed to be simple, applicable, economically beneficial, and environmentally safe, by using internal available resources like emitted hydrogen sulfide and sodium hydroxide, also reduction of chemicals that used in radioactivity treatment to be sulfuric acid or sodium hydroxide instead of multiple different chemicals that used in other treatment procedures. The effects of the used chemical reagents sulfuric acid and sodium hydroxide in various concentrations at different reaction temperatures on the sludge waste to extract the radium isotopes have been studied, evaluated, and compared. The study proved that removing radium isotopes is increased by elevating the reagents concentration and sludge temperature. The removal effects of the used reagents are approximately similar.</div></div>","PeriodicalId":19272,"journal":{"name":"Nuclear Engineering and Technology","volume":"57 2","pages":"Article 103175"},"PeriodicalIF":2.6,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143099941","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Fluence-to-dose conversion coefficients in a voxel rat model for external neutron irradiation","authors":"Xiaomin Zhang , Xu Xu , Yong Yuan, Jing Ning, Dawei Li, Yunlong Ji","doi":"10.1016/j.net.2024.08.056","DOIUrl":"10.1016/j.net.2024.08.056","url":null,"abstract":"<div><div>Fluence-to-dose conversion coefficients based on a developed rat model have been calculated for neutrons with energies <20 MeV using Monte Carlo N-particle code (MCNP), for the purpose of neutron radiation effect evaluation. The calculation was conducted respectively for 27 monodirectional monoenergetic neutron beams in the energy range 10<sup>−9</sup> MeV to 20 MeV, under four different irradiation conditions: left lateral, right lateral, dorsal–ventral and ventral–dorsal. The neutron fluence-to-dose conversion coefficients for selected organs were presented in the study and can be used to determine the organ dose of the rats experimentally exposed to external neutron irradiation. The results in this work were compared with the published data based on a mouse model to investigate the effect of size and weight difference on neutron organ dose. The comparison results showed the fluence-to-dose conversion coefficients of the rat model have the similar energy dependency and sensitivity to irradiation conditions compared with that of the mouse model, and the weight and size difference in individuals could lead to different levels of neutron organ dose difference depending on neutron energy, irradiation conditions as well as the location of organs.</div></div>","PeriodicalId":19272,"journal":{"name":"Nuclear Engineering and Technology","volume":"57 2","pages":"Article 103187"},"PeriodicalIF":2.6,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142226264","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
S.Y. Zhang , Y.B. Nie , Y.Y. Ding , Q. Zhao , K.Z. Xu , X.Y. Pan , H.T. Chen , Q. Sun , Z. Wei
{"title":"Accurate pulse time distribution determination using MLEM algorithm in integral experiments","authors":"S.Y. Zhang , Y.B. Nie , Y.Y. Ding , Q. Zhao , K.Z. Xu , X.Y. Pan , H.T. Chen , Q. Sun , Z. Wei","doi":"10.1016/j.net.2024.08.060","DOIUrl":"10.1016/j.net.2024.08.060","url":null,"abstract":"<div><div>Integral experiments play a crucial role in advancing nuclear science and technology by providing critical data that validate theoretical models and enhance reactor designs. This study presents a novel approach to accurately determine pulse time distribution in integral experiments conducted with pulsed accelerators. By strategically placed monitors and shields at angles of 0° and 90° relative to the beam direction, neutron flight times from the target are measured, and a response matrix for neutron emission at different times is constructed through simulation. The Maximum Likelihood Expectation Maximization (MLEM) algorithm is employed for pulse time reconstruction, with the gamma ray flight time spectrum from monitors used as the initial spectrum to streamline the computational process. Experimental validation using a standard polyethylene sample and n-p scattering cross-sections confirms the accuracy of the method. Results are compared across multiple nuclear databases such as CENDL-3.2, ENDF/B-VIII.0, JENDL-5.0, and JEFF-3.3 libraries. The developed method significantly enhances the precision of pulse time distribution determination, thereby improving the quality and reliability of experimental data obtained from integral experiments conducted with pulsed accelerators.</div></div>","PeriodicalId":19272,"journal":{"name":"Nuclear Engineering and Technology","volume":"57 2","pages":"Article 103191"},"PeriodicalIF":2.6,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142207216","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Estimation of neutral beam injector power transferred to KSTAR plasmas","authors":"Jong-Gu Kwak, J.H. Jeong, S.C. Hong","doi":"10.1016/j.net.2024.08.057","DOIUrl":"10.1016/j.net.2024.08.057","url":null,"abstract":"<div><div>KSTAR shows the long pulse capability based on superconducting magnet and NBI plays a crucial role in sustaining the plasma via plasma heating and current driving. So, the accurate NBI power measurement transferred to KSTAR plasma is important for the analysis of plasma transport as well as plasma performance parameters. In a long pulse operation, the water coolant temperature is at the steady state condition in longer pulse more than 20s and the coupled neutral beam power to KSTAR plasma during the tokamak experiments is rechecked by using water flow calorimetric method after the experiment. The effect of beam duct scraper loss which was not considered at the neutral beam power calibration process is less than 5 % in terms of neutral beam power. However, in long pulse operation of NBI in KSTAR experiments, high strength of stray PF affects the beam path, the neutral beam power registered on mds + using beam current method is over estimated and it is calculated up to a few percent in terms of neutral beam power using calorimetric method. Therefore, it is necessary to consider the beam power variation by PF effect to interpret the plasma performance degradation in long pulse operation. Lastly. when the ion source tun on or turn off in condition other ion sources are operated, the beam transmission power is also affected because of sharing the beam box for ion sources so that the careful power estimation is necessary for such kind of beam power modulation experiments in KSTAR.</div></div>","PeriodicalId":19272,"journal":{"name":"Nuclear Engineering and Technology","volume":"57 2","pages":"Article 103188"},"PeriodicalIF":2.6,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142207221","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Enhanced formula-based method to estimate burnup, initial enrichment, and cooling time using limited gamma-ray source data of reference PWR spent nuclear fuel assemblies","authors":"Sang Hyeok Lee, Jae Hak Cheong","doi":"10.1016/j.net.2024.09.025","DOIUrl":"10.1016/j.net.2024.09.025","url":null,"abstract":"<div><div>This study proposes a framework to develop a model for estimating burnup (BU), initial enrichment (IE), and cooling time (CT) of spent nuclear fuel (SNF) overcoming the limitations of existing models in determining IE. Database (DB) of gamma-ray sources for PWR SNF was generated using ORIGAMI. Target gamma radionuclides were selected based on the ease and credibility of measurement. The concept of Product of Powers of Radioactivity (PPR) was suggested, and PPRs for modeling were selected through evaluation of all possible PPRs. Functions established for PPRs were applied to estimate BU, IE, and CT (BIC) of PWR SNF assemblies. Optimized PPR combinations for estimating BU, IE, and CT respectively, as well as three variables simultaneously with the highest accuracy, were suggested. The estimation model proposed in this study enhanced IE estimations, maintaining the reliability of BU and CT estimations. The above framework enables construction of intuitive BIC estimation models using only a small amount of data. This can help hasten the development of estimation models for SNF from various reactor types. Consequently, it is expected to contribute to the safety and safeguards of SNF management by improving the verification that SNF meets acceptance criteria and conforms to the declared information.</div></div>","PeriodicalId":19272,"journal":{"name":"Nuclear Engineering and Technology","volume":"57 2","pages":"Article 103222"},"PeriodicalIF":2.6,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143099582","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}