Hongtao Hu, Tobias Flöry, Vinzenz Stummer, Audrius Pugzlys, Markus Zeiler, Xinhua Xie, Aleksei Zheltikov, Andrius Baltuška
{"title":"Hyper spectral resolution stimulated Raman spectroscopy with amplified fs pulse bursts.","authors":"Hongtao Hu, Tobias Flöry, Vinzenz Stummer, Audrius Pugzlys, Markus Zeiler, Xinhua Xie, Aleksei Zheltikov, Andrius Baltuška","doi":"10.1038/s41377-023-01367-0","DOIUrl":"10.1038/s41377-023-01367-0","url":null,"abstract":"<p><p>We present a novel approach for Stimulated Raman Scattering (SRS) spectroscopy in which a hyper spectral resolution and high-speed spectral acquisition are achieved by employing amplified offset-phase controlled fs-pulse bursts. We investigate the method by solving the coupled non-linear Schrödinger equations and validate it by numerically characterizing SRS in molecular nitrogen as a model compound. The spectral resolution of the method is found to be determined by the inverse product of the number of pulses in the burst and the intraburst pulse separation. The SRS spectrum is obtained through a motion-free scanning of the offset phase that results in a sweep of the Raman-shift frequency. Due to high spectral resolution and fast motion-free scanning the technique is beneficial for a number SRS-based applications such as gas sensing and chemical analysis.</p>","PeriodicalId":18093,"journal":{"name":"Light, science & applications","volume":"13 1","pages":"61"},"PeriodicalIF":19.4,"publicationDate":"2024-02-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10901837/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139990529","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Yao Xiao, Jun Wang, Heng Liu, Pei Miao, Yudan Gou, Zhicheng Zhang, Guoliang Deng, Shouhuan Zhou
{"title":"Multi-junction cascaded vertical-cavity surface-emitting laser with a high power conversion efficiency of 74.","authors":"Yao Xiao, Jun Wang, Heng Liu, Pei Miao, Yudan Gou, Zhicheng Zhang, Guoliang Deng, Shouhuan Zhou","doi":"10.1038/s41377-024-01403-7","DOIUrl":"10.1038/s41377-024-01403-7","url":null,"abstract":"<p><p>High electro-optical conversion efficiency is one of the most distinctive features of semiconductor lasers as compared to other types of lasers. Its further increase remains a significant objective. Further enhancing the efficiency of edge-emitting lasers (EEL), which represent the highest efficiency among semiconductor lasers at present, is challenging. The efficiency of vertical cavity surface emitting lasers (VCSELs) has always been relatively low compared to EEL. This paper, combining modeling with experiments, demonstrates the potential of multi-junction cascaded VCSELs to achieve high efficiency beyond that of EELs, our simulations show, that a 20-junction VCSEL can achieve an efficiency of more than 88% at room temperature. We fabricated VCSEL devices with different numbers of junctions and compared their energy efficiency. 15-junction VCSELs achieved a maximum efficiency of 74% at room temperature under nanosecond driving current, the corresponding differential quantum efficiency exceeds 1100%, being the largest electro-optical conversion efficiency and differential quantum efficiency reported until now for VCSELs.</p>","PeriodicalId":18093,"journal":{"name":"Light, science & applications","volume":"13 1","pages":"60"},"PeriodicalIF":19.4,"publicationDate":"2024-02-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10899599/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139983229","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Elena Erben, Weida Liao, Antonio Minopoli, Nicola Maghelli, Eric Lauga, Moritz Kreysing
{"title":"Opto-fluidically multiplexed assembly and micro-robotics.","authors":"Elena Erben, Weida Liao, Antonio Minopoli, Nicola Maghelli, Eric Lauga, Moritz Kreysing","doi":"10.1038/s41377-024-01406-4","DOIUrl":"10.1038/s41377-024-01406-4","url":null,"abstract":"<p><p>Techniques for high-definition micromanipulations, such as optical tweezers, hold substantial interest across a wide range of disciplines. However, their applicability remains constrained by material properties and laser exposure. And while microfluidic manipulations have been suggested as an alternative, their inherent capabilities are limited and further hindered by practical challenges of implementation and control. Here we show that the iterative application of laser-induced, localized flow fields can be used for the relative positioning of multiple micro-particles, irrespectively of their material properties. Compared to the standing theoretical proposal, our method keeps particles mobile, and we show that their precision manipulation is non-linearly accelerated via the multiplexing of temperature stimuli below the heat diffusion limit. The resulting flow fields are topologically rich and mathematically predictable. They represent unprecedented microfluidic control capabilities that are illustrated by the actuation of humanoid micro-robots with up to 30 degrees of freedom, whose motions are sufficiently well-defined to reliably communicate personal characteristics such as gender, happiness and nervousness. Our results constitute high-definition micro-fluidic manipulations with transformative potential for assembly, micro-manufacturing, the life sciences, robotics and opto-hydraulically actuated micro-factories.</p>","PeriodicalId":18093,"journal":{"name":"Light, science & applications","volume":"13 1","pages":"59"},"PeriodicalIF":19.4,"publicationDate":"2024-02-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10897173/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139972488","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Hang Wei, Jinxin Gu, Tao Zhao, Zhiyuan Yan, He-Xiu Xu, Shuliang Dou, Cheng-Wei Qiu, Yao Li
{"title":"Tunable VO<sub>2</sub> cavity enables multispectral manipulation from visible to microwave frequencies.","authors":"Hang Wei, Jinxin Gu, Tao Zhao, Zhiyuan Yan, He-Xiu Xu, Shuliang Dou, Cheng-Wei Qiu, Yao Li","doi":"10.1038/s41377-024-01400-w","DOIUrl":"10.1038/s41377-024-01400-w","url":null,"abstract":"<p><p>Optical materials capable of dynamically manipulating electromagnetic waves are an emerging field in memories, optical modulators, and thermal management. Recently, their multispectral design preliminarily attracts much attention, aiming to enhance their efficiency and integration of functionalities. However, the multispectral manipulation based on these materials is challenging due to their ubiquitous wavelength dependence restricting their capacity to narrow wavelengths. In this article, we cascade multiple tunable optical cavities with selective-transparent layers, enabling a universal approach to overcoming wavelength dependence and establishing a multispectral platform with highly integrated functions. Based on it, we demonstrate the multispectral (ranging from 400 nm to 3 cm), fast response speed (0.9 s), and reversible manipulation based on a typical phase change material, vanadium dioxide. Our platform involves tandem VO<sub>2</sub>-based Fabry-Pérot (F-P) cavities enabling the customization of optical responses at target bands independently. It can achieve broadband color-changing capacity in the visible region (a shift of ~60 nm in resonant wavelength) and is capable of freely switching between three typical optical models (transmittance, reflectance, and absorptance) in the infrared to microwave regions with drastic amplitude tunability exceeding 0.7. This work represents a state-of-art advance in multispectral optics and material science, providing a critical approach for expanding the multispectral manipulation ability of optical systems.</p>","PeriodicalId":18093,"journal":{"name":"Light, science & applications","volume":"13 1","pages":"54"},"PeriodicalIF":19.4,"publicationDate":"2024-02-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10879493/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139912935","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Jiaqi Hu, Gina Jinna Chen, Chenlong Xue, Pei Liang, Yanqun Xiang, Chuanlun Zhang, Xiaokeng Chi, Guoying Liu, Yanfang Ye, Dongyu Cui, De Zhang, Xiaojun Yu, Hong Dang, Wen Zhang, Junfan Chen, Quan Tang, Penglai Guo, Ho-Pui Ho, Yuchao Li, Longqing Cong, Perry Ping Shum
{"title":"RSPSSL: A novel high-fidelity Raman spectral preprocessing scheme to enhance biomedical applications and chemical resolution visualization.","authors":"Jiaqi Hu, Gina Jinna Chen, Chenlong Xue, Pei Liang, Yanqun Xiang, Chuanlun Zhang, Xiaokeng Chi, Guoying Liu, Yanfang Ye, Dongyu Cui, De Zhang, Xiaojun Yu, Hong Dang, Wen Zhang, Junfan Chen, Quan Tang, Penglai Guo, Ho-Pui Ho, Yuchao Li, Longqing Cong, Perry Ping Shum","doi":"10.1038/s41377-024-01394-5","DOIUrl":"10.1038/s41377-024-01394-5","url":null,"abstract":"<p><p>Raman spectroscopy has tremendous potential for material analysis with its molecular fingerprinting capability in many branches of science and technology. It is also an emerging omics technique for metabolic profiling to shape precision medicine. However, precisely attributing vibration peaks coupled with specific environmental, instrumental, and specimen noise is problematic. Intelligent Raman spectral preprocessing to remove statistical bias noise and sample-related errors should provide a powerful tool for valuable information extraction. Here, we propose a novel Raman spectral preprocessing scheme based on self-supervised learning (RSPSSL) with high capacity and spectral fidelity. It can preprocess arbitrary Raman spectra without further training at a speed of ~1 900 spectra per second without human interference. The experimental data preprocessing trial demonstrated its excellent capacity and signal fidelity with an 88% reduction in root mean square error and a 60% reduction in infinite norm ([Formula: see text]) compared to established techniques. With this advantage, it remarkably enhanced various biomedical applications with a 400% accuracy elevation (ΔAUC) in cancer diagnosis, an average 38% (few-shot) and 242% accuracy improvement in paraquat concentration prediction, and unsealed the chemical resolution of biomedical hyperspectral images, especially in the spectral fingerprint region. It precisely preprocessed various Raman spectra from different spectroscopy devices, laboratories, and diverse applications. This scheme will enable biomedical mechanism screening with the label-free volumetric molecular imaging tool on organism and disease metabolomics profiling with a scenario of high throughput, cross-device, various analyte complexity, and diverse applications.</p>","PeriodicalId":18093,"journal":{"name":"Light, science & applications","volume":"13 1","pages":"52"},"PeriodicalIF":19.4,"publicationDate":"2024-02-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10876988/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139905963","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Versatile photonic molecule switch in multimode microresonators.","authors":"Zihan Tao, Bitao Shen, Wencan Li, Luwen Xing, Haoyu Wang, Yichen Wu, Yuansheng Tao, Yan Zhou, Yandong He, Chao Peng, Haowen Shu, Xingjun Wang","doi":"10.1038/s41377-024-01399-0","DOIUrl":"10.1038/s41377-024-01399-0","url":null,"abstract":"<p><p>Harnessing optical supermode interaction to construct artificial photonic molecules has uncovered a series of fundamental optical phenomena analogous to atomic physics. Previously, the distinct energy levels and interactions in such two-level systems were provided by coupled microresonators. The reconfigurability is limited, as they often require delicate external field stimuli or mechanically altering the geometric factors. These highly specific approaches also limit potential applications. Here, we propose a versatile on-chip photonic molecule in a multimode microring, utilizing a flexible regulation methodology to dynamically control the existence and interaction strength of spatial modes. The transition between single/multi-mode states enables the \"switched-off/on\" functionality of the photonic molecule, supporting wider generalized applications scenarios. In particular, \"switched-on\" state shows flexible and multidimensional mode splitting control in aspects of both coupling strength and phase difference, equivalent to the a.c. and d.c. Stark effect. \"Switched-off\" state allows for perfect low-loss single-mode transition (Q<sub>i</sub> ~ 10 million) under an ultra-compact bend size (FSR ~ 115 GHz) in a foundry-based silicon microring. It breaks the stereotyped image of the FSR-Q factor trade-off, enabling ultra-wideband and high-resolution millimeter-wave photonic operations. Our demonstration provides a flexible and portable solution for the integrated photonic molecule system, extending its research scope from fundamental physics to real-world applications such as nonlinear optical signal processing and sixth-generation wireless communication.</p>","PeriodicalId":18093,"journal":{"name":"Light, science & applications","volume":"13 1","pages":"51"},"PeriodicalIF":19.4,"publicationDate":"2024-02-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10876944/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139905993","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Maxim Makhonin, Anthonin Delphan, Kok Wee Song, Paul Walker, Tommi Isoniemi, Peter Claronino, Konstantinos Orfanakis, Sai Kiran Rajendran, Hamid Ohadi, Julian Heckötter, Marc Assmann, Manfred Bayer, Alexander Tartakovskii, Maurice Skolnick, Oleksandr Kyriienko, Dmitry Krizhanovskii
{"title":"Nonlinear Rydberg exciton-polaritons in Cu<sub>2</sub>O microcavities.","authors":"Maxim Makhonin, Anthonin Delphan, Kok Wee Song, Paul Walker, Tommi Isoniemi, Peter Claronino, Konstantinos Orfanakis, Sai Kiran Rajendran, Hamid Ohadi, Julian Heckötter, Marc Assmann, Manfred Bayer, Alexander Tartakovskii, Maurice Skolnick, Oleksandr Kyriienko, Dmitry Krizhanovskii","doi":"10.1038/s41377-024-01382-9","DOIUrl":"10.1038/s41377-024-01382-9","url":null,"abstract":"<p><p>Rydberg excitons (analogues of Rydberg atoms in condensed matter systems) are highly excited bound electron-hole states with large Bohr radii. The interaction between them as well as exciton coupling to light may lead to strong optical nonlinearity, with applications in sensing and quantum information processing. Here, we achieve strong effective photon-photon interactions (Kerr-like optical nonlinearity) via the Rydberg blockade phenomenon and the hybridisation of excitons and photons forming polaritons in a Cu2O-filled microresonator. Under pulsed resonant excitation polariton resonance frequencies are renormalised due to the reduction of the photon-exciton coupling with increasing exciton density. Theoretical analysis shows that the Rydberg blockade plays a major role in the experimentally observed scaling of the polariton nonlinearity coefficient as ∝ n<sup>4.4±1.8</sup> for principal quantum numbers up to n = 7. Such high principal quantum numbers studied in a polariton system for the first time are essential for realisation of high Rydberg optical nonlinearities, which paves the way towards quantum optical applications and fundamental studies of strongly correlated photonic (polaritonic) states in a solid state system.</p>","PeriodicalId":18093,"journal":{"name":"Light, science & applications","volume":"13 1","pages":"47"},"PeriodicalIF":19.4,"publicationDate":"2024-02-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10847413/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139697818","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Continuous-wave operation of 1550 nm low-threshold triple-lattice photonic-crystal surface-emitting lasers.","authors":"Ziye Wang, Xia Liu, Pinyao Wang, Huanyu Lu, Bo Meng, Wei Zhang, Lijie Wang, Yanjing Wang, Cunzhu Tong","doi":"10.1038/s41377-024-01387-4","DOIUrl":"10.1038/s41377-024-01387-4","url":null,"abstract":"<p><p>Benefitting from narrow beam divergence, photonic crystal surface-emitting lasers are expected to play an essential role in the ever-growing fields of optical communication and light detection and ranging. Lasers operating with 1.55 μm wavelengths have attracted particular attention due to their minimum fiber loss and high eye-safe threshold. However, high interband absorption significantly decreases their performance at this 1.55 μm wavelength. Therefore, stronger optical feedback is needed to reduce their threshold and thus improve the output power. Toward this goal, photonic-crystal resonators with deep holes and high dielectric contrast are often used. Nevertheless, the relevant techniques for high-contrast photonic crystals inevitably complicate fabrication and reduce the final yield. In this paper, we demonstrate the first continuous-wave operation of 1.55 μm photonic-crystal surface-emitting lasers by using a 'triple-lattice photonic-crystal resonator', which superimposes three lattice point groups to increase the strength of in-plane optical feedback. Using this geometry, the in-plane 180° coupling can be enhanced threefold compared to the normal single-lattice structure. Detailed theoretical and experimental investigations demonstrate the much lower threshold current density of this structure compared to 'single-lattice' and 'double-lattice' photonic-crystal resonators, verifying our design principles. Our findings provide a new strategy for photonic crystal laser miniaturization, which is crucial for realizing their use in future high-speed applications.</p>","PeriodicalId":18093,"journal":{"name":"Light, science & applications","volume":"13 1","pages":"44"},"PeriodicalIF":19.4,"publicationDate":"2024-02-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11251162/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139681327","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Mapping super-resolution image quality.","authors":"Megan A Steves, Ke Xu","doi":"10.1038/s41377-024-01379-4","DOIUrl":"10.1038/s41377-024-01379-4","url":null,"abstract":"<p><p>The local quality of super-resolution microscopy images can be assessed and mapped by rolling Fourier ring correlation, even when image quality varies within a single image.</p>","PeriodicalId":18093,"journal":{"name":"Light, science & applications","volume":"13 1","pages":"39"},"PeriodicalIF":19.4,"publicationDate":"2024-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC10830463/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139651026","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}