Journal of The Mechanics and Physics of Solids最新文献

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Mechanochemical patterning and wave propagation in multicellular tubes 多细胞管中的机械化学模式和波传播
IF 5 2区 工程技术
Journal of The Mechanics and Physics of Solids Pub Date : 2024-07-30 DOI: 10.1016/j.jmps.2024.105801
{"title":"Mechanochemical patterning and wave propagation in multicellular tubes","authors":"","doi":"10.1016/j.jmps.2024.105801","DOIUrl":"10.1016/j.jmps.2024.105801","url":null,"abstract":"<div><p>Multicellular tubes are fundamental tissues for transporting and distributing liquids and gases in living organisms. Although the molecular, cellular and mechanical aspects in tube formation have been addressed experimentally, how these factors are coupled to control tube patterning and dynamics at the tissue level remains incompletely understood. Here, we propose a three-dimensional (3D) vertex model that incorporates a mechanochemical feedback loop correlating cell deformation and actomyosin signaling pathway to probe the morphodynamics of multicellular tubes. We show that diverse patterns, including ring, helix, double helix, and labyrinth, are generated in tubes through pitchfork bifurcation, where spatial fluctuations of both biochemical signaling and 3D cell deformation are remarkably involved. The mechanochemical feedback loop enables cell oscillations via Hopf bifurcation, which induces the mechanical and chemical patterns to propagate successively as either traveling or pulse waves while their spatial configurations are maintained, strikingly distinct from the classical Turing instability. Our simulations, together with stability analysis of a minimal model, uncover the essential role of mechanochemical principles in sculpting biological tubes.</p></div>","PeriodicalId":17331,"journal":{"name":"Journal of The Mechanics and Physics of Solids","volume":null,"pages":null},"PeriodicalIF":5.0,"publicationDate":"2024-07-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141915033","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Towards stable End Notched Flexure (ENF) tests 实现稳定的端面缺口挠曲 (ENF) 试验
IF 5 2区 工程技术
Journal of The Mechanics and Physics of Solids Pub Date : 2024-07-29 DOI: 10.1016/j.jmps.2024.105795
{"title":"Towards stable End Notched Flexure (ENF) tests","authors":"","doi":"10.1016/j.jmps.2024.105795","DOIUrl":"10.1016/j.jmps.2024.105795","url":null,"abstract":"<div><p>Mode II fracture toughness of interfaces in laminated structures is usually assessed through standardized tests. Standards are based on samples featuring regular shapes and uniform cross-sections, in which mode II propagation happens to be unstable. We explore here, via a semi-analytical approach, the potential of more complex geometry and shapes for stabilizing the crack propagation. Results demonstrate that an end-notch flexure (ENF) sample with increasing width along the propagation direction possesses a more stable fracture compared to the classical configuration. This leads to the conceptualization of a width-tapered ENF (WTENF) that can address the instability issue encountered by the classical ENF samples. The closed-form solution of WTENF is derived, including the compliance and energy release rate of the system, based on which, the stability status diagram of WTENF has been provided. A systematic validation is performed by numerical and physical experiments, confirming the validity and the accuracy of the associated data reduction model. The WTENF can be a robust method with enhanced stability for measuring the mode II delamination toughness. Beyond solving the WTENF, the derived equations hold significant potential for other applications, such as probing the length-scale effect for delamination of fiber-reinforced composites and guiding the design of toughening strategies for interfaces.</p></div>","PeriodicalId":17331,"journal":{"name":"Journal of The Mechanics and Physics of Solids","volume":null,"pages":null},"PeriodicalIF":5.0,"publicationDate":"2024-07-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141915226","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Modeling the electro-chemo-mechanical failure at the lithium-solid electrolyte interface: Void evolution and lithium penetration 锂-固体电解质界面的电-化学-机械失效建模:空洞演化和锂渗透
IF 5 2区 工程技术
Journal of The Mechanics and Physics of Solids Pub Date : 2024-07-27 DOI: 10.1016/j.jmps.2024.105799
{"title":"Modeling the electro-chemo-mechanical failure at the lithium-solid electrolyte interface: Void evolution and lithium penetration","authors":"","doi":"10.1016/j.jmps.2024.105799","DOIUrl":"10.1016/j.jmps.2024.105799","url":null,"abstract":"<div><p>The solid-solid contact interface is crucial for the reliability of solid-state energy storage systems. The contact condition becomes more complicated when lithium (Li) metal is used as the anode. The contact between solid electrolyte (SE) and Li metal is inferior compared to the liquid/solid interface in conventional Li-ion batteries. Experimental evidence has shown that improper operating conditions of solid-state batteries can lead to electro-chemo-mechanical failures at the Li/SE interface, including the formation of voids and the penetration of Li. In this study, a unified phase-field model is developed to investigate these two mechanisms. The model considers the coupled electro-chemo-mechanical processes including void diffusion, lattice annihilation, stripping and plating reactions, and plastic deformation of Li metal. The study begins with a revisit of the deformation-mechanism map for Li metal under a wide range of temperatures, stress, and deformation rates. This map serves as the basis for the mechanical characterization in the phase-field model. The large inelastic deformation of Li is considered by introducing an advection term into the Allen-Cahn equation, which is used to describe the dynamic evolution of the Li and void phases. The effects of current density and stack pressure on void evolution and Li penetration are studied based on the model predictions. By combining the simulation results with the experimental data from publications, we obtain the stable operation zone of stack pressure and applied current density. In this zone, the Li/SE interface can enable stable stripping and plating of Li metal. The same phase-field modeling framework is transferred to investigate the Li-Mg alloy/SE interface considering Li-Mg alloy is also used as the anode. The fundamental difference between Li/SE and Li-Mg/SE is analyzed accordingly. This study provides a useful tool for the design, manufacturing, and management of next-generation batteries by providing important scientific insights into the electro-chemo-mechanical processes of different anode materials under various operational conditions.</p></div>","PeriodicalId":17331,"journal":{"name":"Journal of The Mechanics and Physics of Solids","volume":null,"pages":null},"PeriodicalIF":5.0,"publicationDate":"2024-07-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S0022509624002655/pdfft?md5=09ae07d76b9943a188036487f2cedd8c&pid=1-s2.0-S0022509624002655-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141847490","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Twinning, slip and size effect of phase-transforming ferroelectric nanopillars 相变铁电纳米柱的孪晶、滑移和尺寸效应
IF 5 2区 工程技术
Journal of The Mechanics and Physics of Solids Pub Date : 2024-07-26 DOI: 10.1016/j.jmps.2024.105796
{"title":"Twinning, slip and size effect of phase-transforming ferroelectric nanopillars","authors":"","doi":"10.1016/j.jmps.2024.105796","DOIUrl":"10.1016/j.jmps.2024.105796","url":null,"abstract":"<div><p>Ferroelectric materials are widely used in energy applications due to their field-driven multiferroic properties. The stress-induced phase transformation plays an important role in the functionality over repeated and consecutive operation cycles, especially at the micro/nanoscales. Here we report a systematic in-situ uniaxial compression tests on cuboidal Barium titanate (BaTiO<span><math><msub><mrow></mrow><mrow><mn>3</mn></mrow></msub></math></span>) nanopillars with size varying from 100 nm to 3000 nm, by which we explore the stress-induced transformation and its interplay with plastic deformation. We confirm the superelasticity achieved in pillars by martensitic phase transformation from tetragonal to orthorhombic. There exists a critical size, 330 nm, for the yield stress. Above 330 nm, martensitic phase transformation aids slip along the plane with a low Schmid factor, in turn, the pseudo-compatible twins form within the shear band. The scaling exponent of size-dependent yield strength is found to be exactly 1. For nanopillars smaller than 330 nm, no twins form, only slips with large Schmid factors are activated, and size effect vanishes. All pillars with sizes from 100 nm to 300 nm achieve the theoretical yield limit around 9 GPa. Our experimental results uncover the interplay between twins and slips in BaTiO<span><math><msub><mrow></mrow><mrow><mn>3</mn></mrow></msub></math></span> nanopillars, which pave the way for the optimization of microstructure design of ferroelectric materials for microelectronic applications at small scales.</p></div>","PeriodicalId":17331,"journal":{"name":"Journal of The Mechanics and Physics of Solids","volume":null,"pages":null},"PeriodicalIF":5.0,"publicationDate":"2024-07-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141838674","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A multiscale mechanics model for disordered biopolymer gels containing junction zones with variable length 含有长度可变接合区的无序生物聚合物凝胶的多尺度力学模型
IF 5 2区 工程技术
Journal of The Mechanics and Physics of Solids Pub Date : 2024-07-25 DOI: 10.1016/j.jmps.2024.105792
{"title":"A multiscale mechanics model for disordered biopolymer gels containing junction zones with variable length","authors":"","doi":"10.1016/j.jmps.2024.105792","DOIUrl":"10.1016/j.jmps.2024.105792","url":null,"abstract":"<div><p>Disordered biopolymer gels, such as those synthesized from polysaccharide and gelatin, play an important role in biomedical applications, particularly in tissue engineering. During the gelation process of these gels, polymer chains associate in the presence of gelling agents, forming physical cross-links known as the junction zones. In contrast to rubber-like networks, the resulting network comprises two main regions: the ordered region due to the junction zones and the amorphous region due to the unassociated chains. Under thermal fluctuations and/or external loading, the number and locations of junction zones can change leading to “zipping” (lengthening, i.e., expansion of the junction zones) and “unzipping” (shortening, i.e., shrinkage of the junction zones). This gives rise to intriguing features in biopolymer gels such as healing and damage-like energy dissipation. Despite the recognition of zipping and unzipping in such gels, the development of mathematical models that incorporate the microscopic mechanisms into the material’s macroscopic mechanical properties is still in its early stages. In this paper, we provide a systematic framework for such multiscale modeling. Several critical steps are taken to equip the eight-chain network model with a previously developed micromechanics model for a coil–rod structure, where the coil represents an unassociated chain and the rod represents a junction zone. Most importantly, for a network of coil–rod structures under zero stress, the rigidity induced by the rod leads to an end-to-end distance (<span><math><msub><mrow><mi>r</mi></mrow><mrow><mn>0</mn></mrow></msub></math></span>) for the coil–rod which is different from a classical result for a Gaussian coil: <span><math><mrow><msqrt><mrow><mi>n</mi></mrow></msqrt><mi>b</mi></mrow></math></span> where <span><math><mi>b</mi></math></span> is the Kuhn length and <span><math><mi>n</mi></math></span> is the number of Kuhn segments in the coil. By relaxing the incompressible assumption in the original eight-chain model, <span><math><msub><mrow><mi>r</mi></mrow><mrow><mn>0</mn></mrow></msub></math></span> is determined for the gel network, which depends on the length of the junction zone. Consequently, as the junction zone extends/shrinks following zipping/unzipping under an external load, an irreversible deformation can occur after unloading, consistent with experimentally observed “permanent set”. The extension/shrinkage of the junction zone is captured by statistical mechanics analysis in the grand canonical ensemble, which allows the exchange of segments between the coil and the rod, driven by the binding energy of polymer chain association. The model also includes explicit consideration of swelling and the influence of solvent molecules as a result of their mixing with the polymer chains in the gel network. With physically reasonable parameters, the proposed model is shown to provide good matching with experimental data on the uniaxial testing ","PeriodicalId":17331,"journal":{"name":"Journal of The Mechanics and Physics of Solids","volume":null,"pages":null},"PeriodicalIF":5.0,"publicationDate":"2024-07-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S0022509624002588/pdfft?md5=5e37b967195cf157f4f20fa4d6182358&pid=1-s2.0-S0022509624002588-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141840988","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Pressurized membranes between walls: Thermodynamic process changes force and stiffness 墙壁之间的加压膜:热力学过程改变力和刚度
IF 5 2区 工程技术
Journal of The Mechanics and Physics of Solids Pub Date : 2024-07-24 DOI: 10.1016/j.jmps.2024.105798
{"title":"Pressurized membranes between walls: Thermodynamic process changes force and stiffness","authors":"","doi":"10.1016/j.jmps.2024.105798","DOIUrl":"10.1016/j.jmps.2024.105798","url":null,"abstract":"<div><p>Pressurized solids are ubiquitous in nature. Mechanical properties of biological tissues arise from cell turgor pressure and membrane elasticity. Flat contact between cells generate nonlinear forces. In this work, cells are idealized as pressurized elastic membranes in frictionless contact with one another. Contact forces are experimentally measured on rubber-like membranes and computed using finite element analysis (FEA). FEA matches experimental force-indentation relationships from small to large indentations. With the chosen dimensionless numbers, data gather on a master curve. The isobaric force exhibits a 4/3 power law over 1.5 decades of indentation. Forces for other thermodynamic processes (adiabatic, isothermal/osmotic and isochoric) are interpolated from isobaric data. Regarding stiffness, the isochoric process is superlinear contrary to the sublinear isobaric stiffness. Simple force-indentation relationships are given for each process.</p></div>","PeriodicalId":17331,"journal":{"name":"Journal of The Mechanics and Physics of Solids","volume":null,"pages":null},"PeriodicalIF":5.0,"publicationDate":"2024-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141851995","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A comprehensive study of nonlinear perturbations in the dynamics of planar crack fronts 平面裂缝前沿动力学中的非线性扰动综合研究
IF 5 2区 工程技术
Journal of The Mechanics and Physics of Solids Pub Date : 2024-07-24 DOI: 10.1016/j.jmps.2024.105788
{"title":"A comprehensive study of nonlinear perturbations in the dynamics of planar crack fronts","authors":"","doi":"10.1016/j.jmps.2024.105788","DOIUrl":"10.1016/j.jmps.2024.105788","url":null,"abstract":"<div><p>The interaction of crack fronts with asperities is central to fracture criteria in heterogeneous materials and for predicting fracture surface formation. It is known how dynamic crack fronts respond to small, 1st-order, perturbations. However, large and localized disturbances to crack motion induce dynamic and geometric nonlinear effects beyond the existing linear theories. Because the determination of the 3D elastic fields surrounding perturbed crack fronts is a necessary step toward any theoretical study of crack front dynamics, we develop a 2nd-order perturbation theory for the asymptotic fields of planar crack fronts. Based on previous work, we consider two models of fracture: (1) Fracture in a scalar elastic solid which is an analog of antiplane shear fracture (Mode III). In this model, the near-crack fields are obtained via matched asymptotic expansions. (2) Tensile Mode I fracture, in which a self-consistent expansion is used to resolve the fields near the crack front. These methods can be readily extended to higher perturbation orders. The main results of this work are the <em>explicit</em> 2nd-order expressions of the <em>local</em> dynamic energy-release-rates for arbitrary perturbations of straight fronts. The formulae recover the known energy-release-rates of curved quasi-static fronts and of simple 2D cracks. We show that the expressions are separable as a product of a dynamical prefactor that only depends on the instantaneous local normal front velocity, and a history functional that integrates past front configurations. To gain insight, the energy-release-rates in the two models are computed for a traveling wave perturbation. While similar at low wave velocities, the two theories behave differently for fast waves. In scalar elasticity, the 2nd-order contributions are always sub-dominant. However, in the Mode I theory, the 2nd-order correction becomes the dominant term at the crack front wave velocity, where the 1st-order term is zero. We discuss employing the energy-release-rate expressions to predict crack front dynamics via energy balance with dissipation.</p></div>","PeriodicalId":17331,"journal":{"name":"Journal of The Mechanics and Physics of Solids","volume":null,"pages":null},"PeriodicalIF":5.0,"publicationDate":"2024-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141947062","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The adjustable adhesion strength of multiferroic composite materials via electromagnetic loadings and shape effect of punch 通过电磁加载和冲头形状效应调节多铁氧体复合材料的粘附强度
IF 5 2区 工程技术
Journal of The Mechanics and Physics of Solids Pub Date : 2024-07-24 DOI: 10.1016/j.jmps.2024.105794
{"title":"The adjustable adhesion strength of multiferroic composite materials via electromagnetic loadings and shape effect of punch","authors":"","doi":"10.1016/j.jmps.2024.105794","DOIUrl":"10.1016/j.jmps.2024.105794","url":null,"abstract":"<div><p>Tunable and reversible dry adhesion possess great potential in a wide range of applications including transfer printing, climbing robots, wearable devices/electronics, and gripping in pick-and-place operations. Multiferroic composite materials offer new routines and approaches to achieve tunable adhesion due to their multi-field coupling effects. In this paper, the classical Johnson-Kendall-Roberts (JKR) adhesion model is extended to investigate the adhesive contact problem of a multiferroic composite half-space indented by an axisymmetric power-law shaped punch, whose shape index is denoted by <em>n</em>. The JKR-<em>n</em> adhesion models under the action of the power-law shaped punches with four different electromagnetic properties are set up by means of the total energy method. The explicit analytical expressions relating the indentation load and indentation depth to the contact radius are obtained, which can include the existing results in open literature as special cases. The generalized Tabor parameter and the interfacial adhesion strength applicable to multiferroic composite materials are defined. The effects of the shape index and the electromagnetic loadings on adhesion behaviors are revealed. It is found that both of them have prominent influences on the relationships among the indentation load, indentation depth and contact radius, the contact radius and indentation depth at self-equilibrium state, and the critical contact radius and indentation depth at pull-off moment. The pull-off force under the action of the conducting spherical punch subjected to non-zero electromagnetic loadings is dependent on material properties, which is different from the classical JKR result. More importantly, our analysis indicates that the pull-off force and the interfacial adhesion strength can be adjusted via altering the electromagnetic loadings and the shape index of the punch, which provides new approaches to achieve tunable adhesion.</p></div>","PeriodicalId":17331,"journal":{"name":"Journal of The Mechanics and Physics of Solids","volume":null,"pages":null},"PeriodicalIF":5.0,"publicationDate":"2024-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141849437","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Intrinsic fracture toughness of a soft viscoelastic adhesive 软粘弹性粘合剂的内在断裂韧性
IF 5 2区 工程技术
Journal of The Mechanics and Physics of Solids Pub Date : 2024-07-23 DOI: 10.1016/j.jmps.2024.105797
{"title":"Intrinsic fracture toughness of a soft viscoelastic adhesive","authors":"","doi":"10.1016/j.jmps.2024.105797","DOIUrl":"10.1016/j.jmps.2024.105797","url":null,"abstract":"<div><p>The fracture toughness of inelastic materials consists of an intrinsic component associated with the crack tip fracture process and a dissipative component due to bulk dissipation. Experimental characterization of the intrinsic component of fracture toughness is important for understanding the fracture mechanism and predictive modeling of the fracture behavior. Here we present an experimental study on the intrinsic toughness of a soft viscoelastic adhesive. We first obtained full-field and full-history data of the displacement and deformation fields in pure shear fracture tests using a particle tracking method. By combining these data with a nonlinear constitutive model, we extracted the intrinsic toughness through an energy balance analysis. A two-stage crack propagation behavior was observed in our fracture experiments: under monotonic loading the crack first underwent a slow propagation stage and then suddenly entered a fast propagation stage. We found that the intrinsic toughness was highly scattered for the slow propagation stage, but remained consistent for the fast propagation stage. Further examination of the fracture surface and the onset of fast propagation revealed that transition from the slow to the fast propagation stage was governed by the applied stretch and was likely due to a change in the crack tip fracture process.</p></div>","PeriodicalId":17331,"journal":{"name":"Journal of The Mechanics and Physics of Solids","volume":null,"pages":null},"PeriodicalIF":5.0,"publicationDate":"2024-07-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141839439","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Magneto-mechanically derived diffusion processes in ultra-soft biological hydrogels 超软生物水凝胶中的磁力学扩散过程
IF 5 2区 工程技术
Journal of The Mechanics and Physics of Solids Pub Date : 2024-07-22 DOI: 10.1016/j.jmps.2024.105791
{"title":"Magneto-mechanically derived diffusion processes in ultra-soft biological hydrogels","authors":"","doi":"10.1016/j.jmps.2024.105791","DOIUrl":"10.1016/j.jmps.2024.105791","url":null,"abstract":"<div><p>Magneto-active hydrogels (MAHs) consist of a polymeric network doped with magnetic particles that enable the material to mechanically respond to magnetic stimuli. This multifunctionality allows for modulation of mechanical properties in a remote and dynamic manner. These characteristics combined with the biocompatibility of hydrogels, make MAHs excellent for drug delivery and biological scaffolds. In this work, ultra-soft biological MAHs with strong magnetostriction are fabricated from human blood plasma (<span><math><mo>∼</mo></math></span>20 Pa). The material is experimentally tested using a novel <em>in-house</em> device that allows for a precise control of magnetic actuation conditions, enabling the hydrogel modulation in terms of mechanical deformation and stiffness. We study the impact of magnetic actuation on the solvent expulsion and diffusion dynamics within the polymeric network. To further elucidate the mechanisms driving solvent diffusion processes, a computational framework for modeling the diffusion process of two different species within a magneto-responsive material is proposed. These experimental and computational outcomes open exciting new opportunities for the use of ultra-soft MAHs in bioengineering applications.</p></div>","PeriodicalId":17331,"journal":{"name":"Journal of The Mechanics and Physics of Solids","volume":null,"pages":null},"PeriodicalIF":5.0,"publicationDate":"2024-07-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S0022509624002576/pdfft?md5=27b4ae15a38c082dda872e1152f7c04d&pid=1-s2.0-S0022509624002576-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141843269","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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