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Upcycling of Air-Degraded Ni-Rich Cathodes via In Situ Surface Reconstruction 通过原位表面重建的空气降解富镍阴极的升级回收
IF 22 1区 材料科学
ACS Energy Letters Pub Date : 2025-06-13 DOI: 10.1021/acsenergylett.5c00581
Mengshan Xu, Mei Zhao, Min Hong, Mengting Zheng, Jianwei Nai, Xinyong Tao, Tiefeng Liu
{"title":"Upcycling of Air-Degraded Ni-Rich Cathodes via In Situ Surface Reconstruction","authors":"Mengshan Xu, Mei Zhao, Min Hong, Mengting Zheng, Jianwei Nai, Xinyong Tao, Tiefeng Liu","doi":"10.1021/acsenergylett.5c00581","DOIUrl":"https://doi.org/10.1021/acsenergylett.5c00581","url":null,"abstract":"Ni-rich cathodes are well-known for their high specific capacity but require extremely dry conditions for prolonged storage due to their inherent sensitivity to tiny amounts of moisture in the atmosphere. Once LiOH/Li<sub>2</sub>CO<sub>3</sub> is formed from exposure to moisture on the cathode surface, these impurities unavoidably obstruct Li insertion into/extraction out of bulk electrodes and simultaneously cause a further loss of the active Li source. In this work, we propose to convert the LiOH/Li<sub>2</sub>CO<sub>3</sub> layer on spent NCM82 particles (S-NCM82) into a high-kinetic Li<sub>3</sub>PO<sub>4</sub>/LiF interphase via a simple phosphide reaction in aqueous LiPO<sub>2</sub>F<sub>2</sub> solution. Meanwhile, such a conformal interphase prevents side reactions with electrolytes and alleviates structural strain during the service. The regenerated NCM82 electrode (R-NCM82) demonstrates a high specific capacity of 102 mAh/g at 5C, surpassing the 79 mAh/g observed in the pristine NCM82 (P-NCM82). Additionally, the R-NCM82//Gr full-cell exhibits 76% of its initial capacity after 300 cycles at 1C. This conversion process is easily scalable and could inspire the development of upcycling techniques for regenerating various spent electrodes.","PeriodicalId":16,"journal":{"name":"ACS Energy Letters ","volume":"25 1","pages":""},"PeriodicalIF":22.0,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144278766","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 19.3 1区 材料科学
ACS Energy Letters Pub Date : 2025-06-13
Kang Wu, Lihua Mo, Tiancheng Yi, Zhigang Zhang, Yoshihiro Kuroiwa, Sangwook Kim, Peilin Ran, Wen Yin, Fangwei Wang, Quanzhi Yu*, Tianjiao Liang*, Jinkui Zhao* and Enyue Zhao*, 
{"title":"","authors":"Kang Wu,&nbsp;Lihua Mo,&nbsp;Tiancheng Yi,&nbsp;Zhigang Zhang,&nbsp;Yoshihiro Kuroiwa,&nbsp;Sangwook Kim,&nbsp;Peilin Ran,&nbsp;Wen Yin,&nbsp;Fangwei Wang,&nbsp;Quanzhi Yu*,&nbsp;Tianjiao Liang*,&nbsp;Jinkui Zhao* and Enyue Zhao*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":16,"journal":{"name":"ACS Energy Letters ","volume":"10 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":19.3,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsenergylett.5c00828","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144355109","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 19.3 1区 材料科学
ACS Energy Letters Pub Date : 2025-06-13
Shiyu Wang, Kang Ji, Shuyun Yao, Yingjie Ji, Jingxian Li, Yuanming Liu, Weijie Fu, Jinghua Yang, Ruilong Liu, Jiangzhou Xie, Ningning Wu*, Zhiyu Yang* and Yi-Ming Yan*, 
{"title":"","authors":"Shiyu Wang,&nbsp;Kang Ji,&nbsp;Shuyun Yao,&nbsp;Yingjie Ji,&nbsp;Jingxian Li,&nbsp;Yuanming Liu,&nbsp;Weijie Fu,&nbsp;Jinghua Yang,&nbsp;Ruilong Liu,&nbsp;Jiangzhou Xie,&nbsp;Ningning Wu*,&nbsp;Zhiyu Yang* and Yi-Ming Yan*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":16,"journal":{"name":"ACS Energy Letters ","volume":"10 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":19.3,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsenergylett.5c00836","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144424930","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 19.3 1区 材料科学
ACS Energy Letters Pub Date : 2025-06-13
Lakshminarayana Polavarapu*,  and , Narayan Pradhan*, 
{"title":"","authors":"Lakshminarayana Polavarapu*,&nbsp; and ,&nbsp;Narayan Pradhan*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":16,"journal":{"name":"ACS Energy Letters ","volume":"10 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":19.3,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsenergylett.5c01173","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144424931","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 19.3 1区 材料科学
ACS Energy Letters Pub Date : 2025-06-13
Xusheng Zhang, Huican Mao, Zhao Chen, Lin Zhou, Lilu Liu, Mingxuan Wu, Zilong Lv, Zhihao Zhang, Yukun Zhong, Yong-Sheng Hu and Junmei Zhao*, 
{"title":"","authors":"Xusheng Zhang,&nbsp;Huican Mao,&nbsp;Zhao Chen,&nbsp;Lin Zhou,&nbsp;Lilu Liu,&nbsp;Mingxuan Wu,&nbsp;Zilong Lv,&nbsp;Zhihao Zhang,&nbsp;Yukun Zhong,&nbsp;Yong-Sheng Hu and Junmei Zhao*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":16,"journal":{"name":"ACS Energy Letters ","volume":"10 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":19.3,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsenergylett.5c00653","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144424937","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 19.3 1区 材料科学
ACS Energy Letters Pub Date : 2025-06-13
Xin-Yu Zhang, Ling-Yi Kong, Junjie Ding, Yan-Fang Zhu*, Jia-Yang Li, Zhuang-Chun Jian, Hanshen Xin*, Meng-Ying Li, Peng Tan*, Wei Kong Pang, Shi-Xue Dou and Yao Xiao*, 
{"title":"","authors":"Xin-Yu Zhang,&nbsp;Ling-Yi Kong,&nbsp;Junjie Ding,&nbsp;Yan-Fang Zhu*,&nbsp;Jia-Yang Li,&nbsp;Zhuang-Chun Jian,&nbsp;Hanshen Xin*,&nbsp;Meng-Ying Li,&nbsp;Peng Tan*,&nbsp;Wei Kong Pang,&nbsp;Shi-Xue Dou and Yao Xiao*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":16,"journal":{"name":"ACS Energy Letters ","volume":"10 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":19.3,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsenergylett.5c01161","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144424942","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 19.3 1区 材料科学
ACS Energy Letters Pub Date : 2025-06-13
Simon Rufer, Tal Joseph, Zara Aamer and Kripa K. Varanasi*, 
{"title":"","authors":"Simon Rufer,&nbsp;Tal Joseph,&nbsp;Zara Aamer and Kripa K. Varanasi*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":16,"journal":{"name":"ACS Energy Letters ","volume":"10 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":19.3,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsenergylett.5c00893","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144424963","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Photoelectrochemical Solar Fuels: What’s Next? 光电化学太阳能燃料：下一步是什么？
IF 22 1区 材料科学
ACS Energy Letters Pub Date : 2025-06-13 DOI: 10.1021/acsenergylett.5c01404
Kevin Sivula
{"title":"Photoelectrochemical Solar Fuels: What’s Next?","authors":"Kevin Sivula","doi":"10.1021/acsenergylett.5c01404","DOIUrl":"https://doi.org/10.1021/acsenergylett.5c01404","url":null,"abstract":"Figure 1. Abstract illustration of a PEC cell. Text-to-image generation from Microsoft Bing image creator was used, in part, to create this image. Figure 2. Simplified schematics of some typical semiconductor electrode architectures: (a) classic n-type semiconductor photoanode, (b) cocatalyst decorated photoanode, (c) a protected photoelectrode with a wide band gap semiconductor overlayer, and (d) a heterojunction photoanode. Electrode structures with continuous metal overlayers (with a work function Φ<sub>M</sub> that controls the band bending/photopotential in the semiconductor) are also shown: (e) Schottky junction-biased electrode and (f) PV-biased electrode. This article references 14 other publications. Early View Article. This article has not yet been cited by other publications.","PeriodicalId":16,"journal":{"name":"ACS Energy Letters ","volume":"27 1","pages":""},"PeriodicalIF":22.0,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144278772","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 19.3 1区 材料科学
ACS Energy Letters Pub Date : 2025-06-13
Zhigao Chen, Ruigeng Du, Chenyang Liu, Ji Kong, Zihao Li, Yiran Ying*, Chao Shen, Ting Jin* and Keyu Xie*, 
{"title":"","authors":"Zhigao Chen,&nbsp;Ruigeng Du,&nbsp;Chenyang Liu,&nbsp;Ji Kong,&nbsp;Zihao Li,&nbsp;Yiran Ying*,&nbsp;Chao Shen,&nbsp;Ting Jin* and Keyu Xie*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":16,"journal":{"name":"ACS Energy Letters ","volume":"10 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":19.3,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsenergylett.5c00593","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144355104","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 19.3 1区 材料科学
ACS Energy Letters Pub Date : 2025-06-13
Rui Li, Yanpei Fan, Xiaotong Liu, Jiewen Li, Haodong Zhang, Lin Lin, Zhenbin Wang and Bohua Wen*, 
{"title":"","authors":"Rui Li,&nbsp;Yanpei Fan,&nbsp;Xiaotong Liu,&nbsp;Jiewen Li,&nbsp;Haodong Zhang,&nbsp;Lin Lin,&nbsp;Zhenbin Wang and Bohua Wen*,&nbsp;","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":16,"journal":{"name":"ACS Energy Letters ","volume":"10 6","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":19.3,"publicationDate":"2025-06-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acsenergylett.5c00174","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144424918","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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