Jack D Briscoe, Danielle Pizzey, Steven A Wrathmall and Ifan G Hughes
{"title":"Indirect measurement of atomic magneto-optical rotation via Hilbert transform","authors":"Jack D Briscoe, Danielle Pizzey, Steven A Wrathmall and Ifan G Hughes","doi":"10.1088/1361-6455/ad5e24","DOIUrl":"https://doi.org/10.1088/1361-6455/ad5e24","url":null,"abstract":"The Kramers–Kronig relations are a pivotal foundation of linear optics and atomic physics, embedding a physical connection between the real and imaginary components of any causal response function. A mathematically equivalent, but simpler, approach instead utilises the Hilbert transform. In a previous study, the Hilbert transform was applied to absorption spectra in order to infer the sole refractive index of an atomic medium in the absence of an external magnetic field. The presence of a magnetic field causes the medium to become birefringent and dichroic, and therefore it is instead characterised by two refractive indices. In this study, we apply the same Hilbert transform technique to independently measure both refractive indices of a birefringent atomic medium, leading to an indirect measurement of atomic magneto-optical rotation. Key to this measurement is the insight that inputting specific light polarisations into an atomic medium induces absorption associated with only one of the refractive indices. We show this is true in two configurations, commonly referred to in literature as the Faraday and Voigt geometries, which differ by the magnetic field orientation with respect to the light wavevector. For both cases, we measure the two refractive indices independently for a Rb thermal vapour in a magnetic field, finding excellent agreement with theory. This study further emphasises the application of the Hilbert transform to the field of quantum and atomic optics in the linear regime.","PeriodicalId":16826,"journal":{"name":"Journal of Physics B: Atomic, Molecular and Optical Physics","volume":null,"pages":null},"PeriodicalIF":1.6,"publicationDate":"2024-08-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141937009","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"What future for attophysics?","authors":"Pierre Agostini","doi":"10.1088/1361-6455/ad6383","DOIUrl":"https://doi.org/10.1088/1361-6455/ad6383","url":null,"abstract":"","PeriodicalId":16826,"journal":{"name":"Journal of Physics B: Atomic, Molecular and Optical Physics","volume":null,"pages":null},"PeriodicalIF":1.5,"publicationDate":"2024-07-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141802761","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Doppler sensitivity and resonant tuning of Rydberg atom-based antennas","authors":"Peter B Weichman","doi":"10.1088/1361-6455/ad6385","DOIUrl":"https://doi.org/10.1088/1361-6455/ad6385","url":null,"abstract":"Radio frequency antennas based on Rydberg atom vapor cells can in principle reach sensitivities beyond those of any conventional wire antenna, especially at lower frequencies where very long wires are needed to accommodate the increasing wavelength. They also have other desirable features such as consisting of nonmetallic, hence lower profile, elements. This paper presents a detailed theoretical investigation of Rydberg antenna sensitivity, elucidating parameter regimes that could cumulatively lead to a sensitivity increase 2–3 orders of magnitude beyond that of currently tested configurations. The key insight is to optimally combine the advantages of two well-studied approaches: (i) three laser ‘2D star configuration’ setups that, when enhanced with increased laser power, to some degree compensate for atom motion-induced Doppler broadening, and (ii) resonant coupling between a pair of near-degenerate Rydberg levels, tuned via a local oscillator to the incident signal of interest. The advantage of the star setup is subtle because it only restores the overall sensitivity to the expected Doppler-limited value, compensating for additional significant off-resonance reductions where differently moving atom sub-populations destructively interfere with each other in the net signal. An additional unique advantage of local oscillator tuning is that it leads to vastly narrower line widths, as low as ∼10 kHz set by the intrinsic Rydberg state lifetimes, rather than the typical ∼10 MHz scale set by the core state lifetimes. Intuitively, with this setup the two Rydberg states may be tuned to act as an independent high-q cavity, a point of view supported by a study of the frequency-dependence of the antenna resonant response. There are a number of practical experimental advances, especially larger ∼1 cm laser beam widths, required to suppress various extrinsic line broadening effects and to fully exploit this ‘Rydberg superheterodyne’ response.","PeriodicalId":16826,"journal":{"name":"Journal of Physics B: Atomic, Molecular and Optical Physics","volume":null,"pages":null},"PeriodicalIF":1.6,"publicationDate":"2024-07-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141782045","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
R Hassaine, F Gauchet, F Iacob, J Zs Mezei, E Roueff, J Tennyson and I F Schneider
{"title":"Dissociative recombination of NS+ in collision with slow electrons","authors":"R Hassaine, F Gauchet, F Iacob, J Zs Mezei, E Roueff, J Tennyson and I F Schneider","doi":"10.1088/1361-6455/ad5e20","DOIUrl":"https://doi.org/10.1088/1361-6455/ad5e20","url":null,"abstract":"Cross sections and rate coefficients for the dissociative recombination (DR) of the NS+ ion induced by collisions with low-energy electrons are reported for temperatures between 10 and 1000 K, relevant to a large range of interstellar cloud temperatures. Uncertainties are discussed for these rates. Comparisons are made with DR rates for the isovalent NO+ molecular ion which are found to be much faster. The present findings lead to a moderate dissociative reaction rate coefficient, smaller by a factor of 2 than the current estimates reported in the different kinetic databases for a temperature of 10 K. We consider that our rate coefficients obtained through multichannel quantum defect theory for NS+ are likely to be better than those displayed in the different kinetic databases.","PeriodicalId":16826,"journal":{"name":"Journal of Physics B: Atomic, Molecular and Optical Physics","volume":null,"pages":null},"PeriodicalIF":1.6,"publicationDate":"2024-07-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141737444","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
David Stevens, Aaditya Datar, Z. Cheong, J. P. Sullivan
{"title":"Low energy elastic and inelastic scattering of positrons from formic acid","authors":"David Stevens, Aaditya Datar, Z. Cheong, J. P. Sullivan","doi":"10.1088/1361-6455/ad636a","DOIUrl":"https://doi.org/10.1088/1361-6455/ad636a","url":null,"abstract":"\u0000 This paper presents a detailed study of low energy positron scattering from formic acid, examining elastic scattering, electronic excitation and ionisation processes. Through detailed comparisons with previous experimental and theoretical data, it is clear that the picture for positron scattering from this target remains incomplete, with significant disagreement between experiment and theory in the comparisons of differential cross section data. Calculations of elastic electron scattering are unexpectedly in better agreement with the positron scattering experiments, and give some hints as to potential areas for improvement in the modelling of scattering for targets which tend to be dominated by dipole interactions.","PeriodicalId":16826,"journal":{"name":"Journal of Physics B: Atomic, Molecular and Optical Physics","volume":null,"pages":null},"PeriodicalIF":1.5,"publicationDate":"2024-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141648955","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Daniel Thima, A. Niggas, Matthias Werl, G. L. Szabo, Paul-Friedmar Laux, Mike Schmidt, Günter Zschornack, F. Aumayr, R. Wilhelm
{"title":"A compact electron beam ion source for highly charged ion experiments at large-scale user facilities","authors":"Daniel Thima, A. Niggas, Matthias Werl, G. L. Szabo, Paul-Friedmar Laux, Mike Schmidt, Günter Zschornack, F. Aumayr, R. Wilhelm","doi":"10.1088/1361-6455/ad6384","DOIUrl":"https://doi.org/10.1088/1361-6455/ad6384","url":null,"abstract":"\u0000 Probing and manipulating of 2D materials and their heterostructures using slow highly charged ions (HCIs) is currently a hot topic due to the ultimate surface sensitivity of electronic sputtering with profound implications for fundamental research and technological applications. To study surface modifications without the complications of sample transport from ion irradiation to complex microscopic or spectroscopic analysis tools, the development of compact and thus portable ion sources is essential. In this paper we present the first results of the Electron Beam Ion Source - Compact version 1 (EBIS-C1), a novel and highly compact source for highly charged ions manufactured by D.I.S Germany GmbH. The main focus of this paper is to demonstrate the suitability of the EBIS-C1 as an ideal source for ion scattering experiments at surfaces and at gas/liquid jet targets by presenting the first charge state spectra of extracted neon, argon and xenon ions. The results highlight the potential of this portable EBIS to become a versatile platform for the study of HCI-surface interactions, allowing investigations to be carried out at user terminals in different laboratory environments.","PeriodicalId":16826,"journal":{"name":"Journal of Physics B: Atomic, Molecular and Optical Physics","volume":null,"pages":null},"PeriodicalIF":1.5,"publicationDate":"2024-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141645664","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Geometric and electronic properties of anionic precious metal gold doped boron clusters AuBn\u0000 - (n = 10-20)","authors":"Peixin Fu, Bole Chen, Kewei Ding, Cheng Lu","doi":"10.1088/1361-6455/ad636b","DOIUrl":"https://doi.org/10.1088/1361-6455/ad636b","url":null,"abstract":"\u0000 Recently, the Au-B covalent bonds in gold doped boron clusters has attracted great attention. However, there are fewer theoretical reports on exploration their ground state structures and stabilities, especially for The medium sizes. Here, we study the structural evolution and electronic properties of the anionic Au doped boron clusters with medium sizes of n from 10 to 20 using the unbiased cluster structural searches combined with density functional theory (DFT) calculations. The results reveal that the quasi-planar AuB18\u0000 - (1A, C1) cluster shows excellent stability and a large vertical separation energy (VDE) of 4.25 eV. The good consistency between the computationally simulated photoelectron spectra and the experimental spectra strongly supports the correctness of our low-lying structures. Further bonding analyses show that the well-stabilized aromatic AuB18\u0000 - cluster is due to the active σ interactions between Au atom (6s orbitals) and B units (2p orbitals), as well as the large number of σ-bonds in the B18\u0000 - moiety with π-aromaticity. These findings enriched the family of Au-B alloy clusters and metal-doped boron-based aromatic clusters, which provide valuable information for the experimental characterization and preparation of boron-rich alloy nanoclusters in the future.","PeriodicalId":16826,"journal":{"name":"Journal of Physics B: Atomic, Molecular and Optical Physics","volume":null,"pages":null},"PeriodicalIF":1.5,"publicationDate":"2024-07-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141644918","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}