International Journal of Radiation Applications and Instrumentation. Part A. Applied Radiation and Isotopes最新文献

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Estimation of uncertainties in stopping-power ratios using Monte Carlo methods 用蒙特卡罗方法估计停止功率比的不确定性
P. Andreo, A. Fransson
{"title":"Estimation of uncertainties in stopping-power ratios using Monte Carlo methods","authors":"P. Andreo, A. Fransson","doi":"10.1016/0883-2889(92)90021-6","DOIUrl":"10.1016/0883-2889(92)90021-6","url":null,"abstract":"","PeriodicalId":14288,"journal":{"name":"International Journal of Radiation Applications and Instrumentation. Part A. Applied Radiation and Isotopes","volume":"43 11","pages":"Pages 1425-1426"},"PeriodicalIF":0.0,"publicationDate":"1992-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1016/0883-2889(92)90021-6","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"77350331","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 3
Ion chromatographic analysis of high specific activity 18FDG preparations and detection of the chemical impurity 2-deoxy-2-chloro-d-glucose 高比活性18FDG制备的离子色谱分析及化学杂质2-脱氧-2-氯-葡萄糖的检测
David L. Alexoff, Rosangela Casati , Joanna S. Fowler, Alfred P. Wolf, Colleen Shea, David J. Schlyer, Chyng-Yann Shiue
{"title":"Ion chromatographic analysis of high specific activity 18FDG preparations and detection of the chemical impurity 2-deoxy-2-chloro-d-glucose","authors":"David L. Alexoff,&nbsp;Rosangela Casati ,&nbsp;Joanna S. Fowler,&nbsp;Alfred P. Wolf,&nbsp;Colleen Shea,&nbsp;David J. Schlyer,&nbsp;Chyng-Yann Shiue","doi":"10.1016/0883-2889(92)90002-V","DOIUrl":"10.1016/0883-2889(92)90002-V","url":null,"abstract":"<div><p>Because of the widespread use of 2-deoxy-2-[<sup>18</sup>F]fluoro-<span>d</span>-glucose (FDG) prepared by the “Julich” method or its variants it was decided necessary to determine the major chemical impurities present in the final product. An analytical system for quantifying FDG was developed using pulsed amperometry after separation by high-performance anion exchange chromatography. With this system a heretofore unidentified impurity, 2-deoxy-2-chloro-<span>d</span>-glucose (ClDG, <em>ca</em> 20–2000 μg; typically &lt; 100 μg), was found in our preparation and in those from other laboratories using the “Julich” method. ClDG arises from Cl<sup>−</sup> ion displacement during the labeling procedure where Cl<sup>−</sup> ion comes from several sources, and Cl<sup>−</sup> ion displacement from the HCl used in the hydrolysis step. FDG mass was present in the same preparations at a level of <em>ca</em> 1–40 μg. Other major chemical constituents were glucose (<em>ca</em> 1–6 mg) and mannose (<em>ca</em> 10–18 μg). Glycerol, arising from sterilizing filters, was also detected in most preparations.</p><p>Although ClDG is a chemical impurity which has not been detected previously in nca FDG preparations, its biochemical and pharmacological properties are similar to FDG and 2-deoxy-<span>d</span>-glucose. Thus it is unlikely that the presence of small quantities of ClDG found in typical FDG preparations (<em>ca</em> 100 μg) would have adverse pharmacological or toxicological consequences that would limit continued application of this radiopharmaceutical in basic and clinical studies.</p></div>","PeriodicalId":14288,"journal":{"name":"International Journal of Radiation Applications and Instrumentation. Part A. Applied Radiation and Isotopes","volume":"43 11","pages":"Pages 1313-1322"},"PeriodicalIF":0.0,"publicationDate":"1992-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1016/0883-2889(92)90002-V","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"12507297","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 45
The role of diffusion, migration and long-range interaction in energy transfer and quenching processes in an organic liquid scintillator 有机液体闪烁体中扩散、迁移和远程相互作用在能量传递和猝灭过程中的作用
B.G. Math, G.C. Chikkur , G.H. Malimath
{"title":"The role of diffusion, migration and long-range interaction in energy transfer and quenching processes in an organic liquid scintillator","authors":"B.G. Math,&nbsp;G.C. Chikkur ,&nbsp;G.H. Malimath","doi":"10.1016/0883-2889(92)90007-2","DOIUrl":"10.1016/0883-2889(92)90007-2","url":null,"abstract":"<div><p>The energy transfer rate parameter <em>K</em><sub>3</sub> and the quenching rate parameter <em>K</em><sub>7b</sub> are determined in a liquid scintillator system consisting of 2,5-di-[5-tertbutyl-2-benzoxazolyl)-thiophene (BBOT) as solute, toluene as solvent and bromobenzene as external solvent quencher in three different media; neat toluene (TN), dilute mixture 1:9 by volume fraction to toluene to cyclohexane (TC) and toluene to liquid paraffin (TP), in the temperature range 20°–70°C (viscosity range 0.35–39.0 cp). The results are discussed in terms of the role of diffusion, migration and long-range dipole-dipole interaction of Forster type in these three systems.</p></div>","PeriodicalId":14288,"journal":{"name":"International Journal of Radiation Applications and Instrumentation. Part A. Applied Radiation and Isotopes","volume":"43 11","pages":"Pages 1349-1354"},"PeriodicalIF":0.0,"publicationDate":"1992-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1016/0883-2889(92)90007-2","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"77986893","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Decay data of 123Tem 123Tem的衰变数据
H. Janßen, E. Schönfeld, R. Klein
{"title":"Decay data of 123Tem","authors":"H. Janßen,&nbsp;E. Schönfeld,&nbsp;R. Klein","doi":"10.1016/0883-2889(92)90001-U","DOIUrl":"10.1016/0883-2889(92)90001-U","url":null,"abstract":"<div><p>Measurements of coincidences between conversion electrons of the 88 keV transition in the <sup>123</sup>Te<sup>m</sup> decay and subsequent 159 keV quanta have been made with a 4πβ-γ coincidence system equipped with a pressurized proportional counter (PPC) in the beta channel. With <sup>123</sup>Te<sup>m</sup> sources prepared for activity determination, a detection probability for conversion electrons, ϵ, very close to ϵ = 1 was achieved. The following data have been derived from the slope of a polynomial fit to <em>n</em><sub>β</sub><em>n</em><sub>γ</sub>/<em>n</em><sub>c</sub> vs (1 − ϵ)/ϵ by varying ϵ by discrimination and taking into account the γ sensitivity of the PPC (<em>n</em><sub>β</sub>, <em>n</em><sub>γ</sub>, <em>n</em><sub>c</sub> are the counting rates in the β, γ and coincidence channel): the total conversion coefficient of the 159 keV transition α<sub>t</sub> = 0.1895(13), the γ-ray emission probability of the 159 keV photons <em>p</em> = 0.8407(9). These data agree with the theoretically calculated values, and with less accurate values determined experimentally by other authors.</p></div>","PeriodicalId":14288,"journal":{"name":"International Journal of Radiation Applications and Instrumentation. Part A. Applied Radiation and Isotopes","volume":"43 11","pages":"Pages 1309-1312"},"PeriodicalIF":0.0,"publicationDate":"1992-11-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1016/0883-2889(92)90001-U","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"85521984","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Efficiency of transfer of stored energy from gamma-irradiated NaCl in aqueous ammonium nitrate solution γ辐照NaCl在硝酸铵水溶液中储存能量的转移效率
C.D. Kalkar, V.M. Raut, R.N. Raut
{"title":"Efficiency of transfer of stored energy from gamma-irradiated NaCl in aqueous ammonium nitrate solution","authors":"C.D. Kalkar,&nbsp;V.M. Raut,&nbsp;R.N. Raut","doi":"10.1016/0883-2889(92)90196-L","DOIUrl":"10.1016/0883-2889(92)90196-L","url":null,"abstract":"<div><p>The reduction of nitrate to nitrite is studied by the transfer of energy stored in γ-irradiated NaCl crystals to aqueous ammonium nitrate solution. The G(NO<sub>2</sub><sup>−</sup>) values are evaluated under varying conditions of energy transfer from γ-irradiated NaCl crystals. Similarly, the G(NO<sub>2</sub><sup>−</sup>) value for direct radiolysis of 0.1 M aqueous ammonium nitrate solution is determined. The efficiency of energy transfer is the ratio of the G-values of the two pathways. The efficiency is 60% at low doses. It is explained on the basis of two processes. The first process depends upon the extent to which the energy can be stored in irradiated NaCl crystals, while the second process of energy transfer is governed by various parameters which limit the yield of nitrite.</p></div>","PeriodicalId":14288,"journal":{"name":"International Journal of Radiation Applications and Instrumentation. Part A. Applied Radiation and Isotopes","volume":"43 10","pages":"Pages 1207-1210"},"PeriodicalIF":0.0,"publicationDate":"1992-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1016/0883-2889(92)90196-L","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"78377467","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
The gamma-ray response of clear polymethylmethacrylate dosimeter radix RN15® 透明聚甲基丙烯酸甲酯剂量计基数RN15®的伽马射线响应
T. Kojima, N. Haneda, S. Mitomo, H. Tachibana, R. Tanaka
{"title":"The gamma-ray response of clear polymethylmethacrylate dosimeter radix RN15®","authors":"T. Kojima,&nbsp;N. Haneda,&nbsp;S. Mitomo,&nbsp;H. Tachibana,&nbsp;R. Tanaka","doi":"10.1016/0883-2889(92)90194-J","DOIUrl":"10.1016/0883-2889(92)90194-J","url":null,"abstract":"<div><p>Basic characteristics of different batches of Radix RN15® dosimeter, a commercially available undyed polymethylmethacrylate dosimeter, was studied for its application to process control of radiation sterilization. Radix has relatively small deviation of thickness, optical absorption spectrum, and optical density values before irradiation. The response curves, in terms of net optical density per unit thickness (ΔOD/mm) as a function of absorbed dose, D<sub>PMMA</sub>, are nearly linear up to 15 kGy and become sublinear at higher doses. Scattering of dose response in 5 dosimeter replicates is ± 1% (1 σ). The dose-response slope at 25 kGy while held at irradiation temperatures in the range 0–60°C, relative to those under 25°C, increases with temperature up to 40°C, the maximum point, and decreases at higher temperatures. Over the temperature range of 10–50°C, the variation with temperature of evaluated dose derived from the calibration curve at 25°C is less than 5% when using a dose rate of 6 kGy/h. At lower dose rates (e.g. 0.7 kGy/h) the irradiation temperature dependence is negligible over this temperature range. The temperature dependence at 40 kGy is less severe than that at 25 kGy. The post-irradiation stability of dose response is less than 5% for more than 100 h after 25 kGy irradiation and storage at 0–35°C. The change in optical density of unirradiated dosimeters 3 years after manufacturing is negligible when the dosimeters are stored at controlled laboratory conditions of temperature (25°C) and relative humidity (40%). The 3-year-old dosimeters by irradiation to a dose of 25 kGy show about 2% lower response than that at 25 kGy at the beginning of the 3-year period.</p></div>","PeriodicalId":14288,"journal":{"name":"International Journal of Radiation Applications and Instrumentation. Part A. Applied Radiation and Isotopes","volume":"43 10","pages":"Pages 1197-1202"},"PeriodicalIF":0.0,"publicationDate":"1992-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1016/0883-2889(92)90194-J","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"82913726","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 5
Radioactive isotope and isomer separation using the light induced drift effect 利用光诱导漂移效应分离放射性同位素和异构体
C. Hradecny, J. Slovak , T. Tethal , I.M. Yermolayev , A.M. Shalagin
{"title":"Radioactive isotope and isomer separation using the light induced drift effect","authors":"C. Hradecny,&nbsp;J. Slovak ,&nbsp;T. Tethal ,&nbsp;I.M. Yermolayev ,&nbsp;A.M. Shalagin","doi":"10.1016/0883-2889(92)90204-R","DOIUrl":"10.1016/0883-2889(92)90204-R","url":null,"abstract":"<div><p>Isotope separation with using light induced drift (LID) is discussed. Two basic theoretical characteristics of the method are deduced. I, separation simultaneously with an arbitrary high enrichment and without significant losses; 2, high separation productivity up to 100 μg/h. These characteristics are sufficient and very convenient for the separation of expensive radioactive isotopes and isomers for applications in medicine and science. The first experimental separation of the radioactive isotopes (<sup>22,24</sup>Na) using the LID effect is reported.</p></div>","PeriodicalId":14288,"journal":{"name":"International Journal of Radiation Applications and Instrumentation. Part A. Applied Radiation and Isotopes","volume":"43 10","pages":"Pages 1259-1264"},"PeriodicalIF":0.0,"publicationDate":"1992-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1016/0883-2889(92)90204-R","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"76265305","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 4
Transport for the nuclear industry 核工业的运输
Gustav Kafka
{"title":"Transport for the nuclear industry","authors":"Gustav Kafka","doi":"10.1016/0883-2889(92)90212-W","DOIUrl":"10.1016/0883-2889(92)90212-W","url":null,"abstract":"","PeriodicalId":14288,"journal":{"name":"International Journal of Radiation Applications and Instrumentation. Part A. Applied Radiation and Isotopes","volume":"43 10","pages":"Page 1303"},"PeriodicalIF":0.0,"publicationDate":"1992-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1016/0883-2889(92)90212-W","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"79268172","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Ion exchangers in radioactive waste management—V. A case of efficient removal of Ba(II) from aqueous solutions by TiO2 powder—radiotracer study 离子交换剂在放射性废物管理中的应用。TiO2粉末-放射性示踪剂对水溶液中Ba(II)的高效去除研究
Shuddhodan P. Mishra, N. Srinivasu, Dhanesh Tiwary
{"title":"Ion exchangers in radioactive waste management—V. A case of efficient removal of Ba(II) from aqueous solutions by TiO2 powder—radiotracer study","authors":"Shuddhodan P. Mishra,&nbsp;N. Srinivasu,&nbsp;Dhanesh Tiwary","doi":"10.1016/0883-2889(92)90203-Q","DOIUrl":"10.1016/0883-2889(92)90203-Q","url":null,"abstract":"<div><p>The adsorption behaviour of Ba(II) on titanium(IV) oxide in an aqueous solution was studied by means of batch technique as a function of Ba(II) concentration, temperature and solution pH using Ba-140 as radiotracer. The results show that adsorption is essentially complete in <em>ca</em> 2 h and that the steady state values of adsorption at various concentrations agree well with the classical Freundlich isotherm and follow first order kinetics. The pH and temperature of the solution markedly affect the extent of adsorption. The nature and mechanism of adsorption are discussed.</p></div>","PeriodicalId":14288,"journal":{"name":"International Journal of Radiation Applications and Instrumentation. Part A. Applied Radiation and Isotopes","volume":"43 10","pages":"Pages 1253-1257"},"PeriodicalIF":0.0,"publicationDate":"1992-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1016/0883-2889(92)90203-Q","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"83008735","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 13
Calibration method in isotopic carbon analysis 同位素碳分析中的校正方法
Zhang Weicheng, Li Liwu
{"title":"Calibration method in isotopic carbon analysis","authors":"Zhang Weicheng,&nbsp;Li Liwu","doi":"10.1016/0883-2889(92)90206-T","DOIUrl":"10.1016/0883-2889(92)90206-T","url":null,"abstract":"<div><p>Unlike neutrons or gamma-rays, charged particles readily lose energy when they penetrate matter; thus, the main difficulty in its calculation is, perhaps, the complication introduced in its mathematical treatment. In our experiments, determination of <sup>13</sup>C in breath test samples by proton-induced gamma-ray emission, interesting regularities were found that allowed drastic simplification in the theoretical treatment of the problem, and led to the derivation from first principles of a simple, sufficiently accurate basic equation which proved reliable for the determination of the isotopic abundance ratio <span><math><msup><mi></mi><mn>13</mn></msup><mtext>C</mtext><msup><mi></mi><mn>12</mn></msup><mtext>C</mtext></math></span> by low-energy proton bombardment of biological samples with simultaneous prompt gamma spectrometry.</p></div>","PeriodicalId":14288,"journal":{"name":"International Journal of Radiation Applications and Instrumentation. Part A. Applied Radiation and Isotopes","volume":"43 10","pages":"Pages 1275-1278"},"PeriodicalIF":0.0,"publicationDate":"1992-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1016/0883-2889(92)90206-T","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"78898831","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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