International Journal of Adhesion and Adhesives最新文献

{"title":"Evaluating the differences of adhesion strength between mussel-inspired and conventional soy protein adhesives: A critical review","authors":"Mulya Supianto ,&nbsp;Eko Setio Wibowo ,&nbsp;Muhammad Adly Rahandi Lubis ,&nbsp;Sukma Surya Kusumah ,&nbsp;Jajang Sutiawan ,&nbsp;Sumit Manohar Yadav ,&nbsp;Byung-Dae Park","doi":"10.1016/j.ijadhadh.2025.104059","DOIUrl":"10.1016/j.ijadhadh.2025.104059","url":null,"abstract":"<div><div>The quest for sustainable and high-performance adhesives has driven extensive research into bio-based alternatives, with soy protein (SP) emerging as a promising candidate. Inspired by the remarkable adhesion mechanisms of marine mussels, recent studies have explored biomimetic strategies—such as dual crosslinking, organic-inorganic hybridization, and sacrificial bond mechanisms—to enhance the bonding strength and water resistance of SP-based adhesives. This review examines the effectiveness of these mussel-inspired modifications compared to conventional crosslinking approaches in SP adhesives. Surprisingly, the improvements in adhesive performance, particularly in terms of bonding strength and water resistance, were only marginally superior to those achieved through non-biomimetic modifications. This finding suggests that while mussel-inspired strategies offer valuable insights, further refinement is necessary to fully harness their potential. Specific technical directions, such as designing SP-specific mussel-inspired peptide segments, incorporating catechol-functionalized crosslinkers, and optimizing redox-responsive or pH-sensitive bonding mechanisms, represent promising routes for improvement. By critically evaluating these approaches, this review also highlights opportunities for advancing SP-based adhesives through novel crosslinking techniques, cost-effective formulations, and processing methods. The insights provided herein pave the way for future innovations in bio-based adhesives.</div></div>","PeriodicalId":13732,"journal":{"name":"International Journal of Adhesion and Adhesives","volume":"141 ","pages":"Article 104059"},"PeriodicalIF":3.2,"publicationDate":"2025-05-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144083711","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Numerical analysis of the structural performance of adhesive T-joints under bending loads","authors":"L.M. Ferreira ,&nbsp;R.D.S.G. Campilho ,&nbsp;M. Muñoz-Reja ,&nbsp;P.N.B. Reis","doi":"10.1016/j.ijadhadh.2025.104064","DOIUrl":"10.1016/j.ijadhadh.2025.104064","url":null,"abstract":"<div><div>T-joints are a good alternative to conventional adhesive joints, such as single-lap joints, due to their ability to efficiently transfer bending, compressive, shear, and tensile loads between the T-profile stiffener and the base plate, all while maintaining cost-effectiveness. However, for widespread adoption, a comprehensive understanding of the joint strength and damage mechanisms is essential. Therefore, this study aims to numerically analyse the structural performance of adhesive T-joints subjected to 3-point bending loads using two-dimensional (2D) finite element models, and cohesive zone modelling (CZM) to simulate the behaviour of the adhesive. CZM validation was also accomplished by comparing the joints' behaviour with experimental data. Numerically, peaks of peel stresses at the overlap edges were observed, with sharp gradients toward the inner bond region, as well as shear stresses due to the geometric discontinuity. Adhesives with higher stiffness provide higher peak values of peel and shear stresses, while more ductile ones lead to higher peak loads. The CZM was successfully validated with experiments, and a correlation was observed between energy dissipation and damage propagation, according to a non-symmetrical pattern, and for conditions that minimize the system's functional energy.</div></div>","PeriodicalId":13732,"journal":{"name":"International Journal of Adhesion and Adhesives","volume":"141 ","pages":"Article 104064"},"PeriodicalIF":3.2,"publicationDate":"2025-05-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144071561","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Bonding behavior of graphene-based enhanced restorative materials: a systematic review and meta-analysis","authors":"Priscila Toninatto Alves de Toledo ,&nbsp;Gabriel Pereira Nunes ,&nbsp;Mayra Fernanda Ferreira ,&nbsp;Tamires Passadori Martins ,&nbsp;Geórgia Rondó Peres ,&nbsp;Diana Gabriela Soares ,&nbsp;Marcella Esteves-Oliveira","doi":"10.1016/j.ijadhadh.2025.104046","DOIUrl":"10.1016/j.ijadhadh.2025.104046","url":null,"abstract":"<div><h3>Objective</h3><div>This systematic review and meta-analysis (SRM) aimed to investigate the efficacy of graphene-based materials on dentin adhesion in resin composites.</div></div><div><h3>Methods</h3><div>This SRM was conducted following the PRISMA statement and was registered in PROSPERO (CRD42024614838). A systematic search was conducted in Medline/Web of Science/Scopus/Embase/Cochrane Library, for articles published until September 2024. Eligible studies included <em>in vitro</em> studies evaluating the use of graphene-based materials in resin-dentin adhesion, excepting those without controls, on animals, non-dentine-focused, material-only, or reviews. Data were extracted and Meta-analysis was performed using Rev Man software. A modified Joanna Briggs Institute's Checklist was used for risk of bias assessment.</div></div><div><h3>Results</h3><div>Of the 694 records screened, 9 studies were included. Graphene-based materials exhibited effects on the improvement of bond strength to dentin. Dentin shear bond strength was significantly enhanced, particularly at 1 % (MD[95 % CI] = 2.30[1.88; 2.72], P &lt; 0.00001) and 2 % (MD[95 % CI] = 20.41 [7.86; 32.95], Р = 0.001) concentrations, while lower concentration 0.25 % (MD[95 % CI] = 3.25 [-8.30; 14.79], P = 0.58) had minimal effect. Microtensile bond strength showed mixed results, with lower initial bond strength but comparable performance to conventional materials over time. Push-out bond strength varied, with one study showing improved bonding and another showing no difference. Graphene incorporation reduced adhesive failure and cohesive failure, and some materials exhibited less microleakage. Overall, the studies presented a low risk of bias.</div></div><div><h3>Conclusions</h3><div>Graphene-based materials have shown promise in enhancing dentin adhesion and bond strength <em>in vitro</em>, suggesting their potential to improve adhesive restoration outcomes in clinical practice. However, variability in protocols and limited long-term data, including aging by water storage, prevent definitive clinical conclusions. Future research should focus on standardizing methods, evaluating long-term performance, and assessing biocompatibility.</div></div>","PeriodicalId":13732,"journal":{"name":"International Journal of Adhesion and Adhesives","volume":"141 ","pages":"Article 104046"},"PeriodicalIF":3.2,"publicationDate":"2025-05-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143937217","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Effects of a novel tungsten alloy (W-Mn-Cu-Sn) particles, produced through powder metallurgy, on the mechanical and failure characterization of adhesively single-lap bonded GFRP joints","authors":"Mikail Aslan ,&nbsp;M. Veysel Çakır ,&nbsp;Ahmed Elmossa","doi":"10.1016/j.ijadhadh.2025.104043","DOIUrl":"10.1016/j.ijadhadh.2025.104043","url":null,"abstract":"<div><div>The impact of novel tungsten-manganese-copper-tin (W-Mn-Cu-Sn) alloy nanoparticles on the shear strength of adhesively bonded single lap joints (SLJs) using glass fiber reinforced polymer (GFRP) substrates was examined in this study. The W-Mn-Cu-Sn alloy particles were produced via mechanical alloying (MA). MA is a process that involves repeated cycles of cold welding, fracturing, and re-welding of powder particles, producing fine, homogeneous materials with improved properties. This technique plays a vital role in uniformly dispersing particles within the tungsten matrix, thereby enhancing the alloy's mechanical properties. The mean diameters of each sample were determined from statistical analysis of 33 measurements using ImageJ software, resulting in an average diameter of 245 nm. Furthermore, the particle size distribution predominantly ranged from 121 to 439 nm. The crystallographic characteristics of the powders were analyzed using X-ray diffraction (X'Pert PRO, Malvern PANalytical) with CuKα radiation (λ = 0.15406 nm). In all samples, the most prominent diffraction peak corresponds to the W phase and the nanoparticles were dispersed in Araldite 2014 using a combination of probe sonication and high-speed mechanical mixing. Single-lap shear tests were applied to SLJs prepared with 1.0 %, 3.0 %, 5.0 %, and 7.0 % tungsten alloy (WAs) additive ratios by weight. The results show that incorporating W-Mn-Cu-Sn nanoparticles enhances the adhesive's mechanical properties, as evidenced by increased shear strength and toughness. The maximum shear strength was observed in specimens with 5.0 wt% W-Mn-Cu-Sn nanoparticles, which exhibited a 21.7 % improvement compared to the neat adhesive. The failure modes of the joints changed from mixed-mode failure to cohesive failure with increasing nanoparticle content, indicating improved adhesion and load transfer between the adhesive and the GFRP substrates. The SEM images indicate that the fracture surfaces of tungsten alloy (WAs) modified specimens exhibited ductile failure modes. Due to the formation of plastic voids and mechanisms for crack deviation, the fracture toughness and shear strength of the modified adhesive have improved. These findings highlight the potential of W-Mn-Cu-Sn nanoparticles as effective reinforcements to enhance the performance of adhesively bonded joints (ABJs) in polymer applications.</div></div>","PeriodicalId":13732,"journal":{"name":"International Journal of Adhesion and Adhesives","volume":"141 ","pages":"Article 104043"},"PeriodicalIF":3.2,"publicationDate":"2025-05-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143936837","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Evaluating adhesive failures in hybrid resin-ceramic restorations: A systematic review of laboratory studies and clinical trials","authors":"Venkata Suresh Venkataiah ,&nbsp;Deepak Mehta ,&nbsp;Jogikalmat Krithikadatta ,&nbsp;Marcelo Giannini ,&nbsp;Salvatore Sauroe ,&nbsp;Vishwas Gowda","doi":"10.1016/j.ijadhadh.2025.104048","DOIUrl":"10.1016/j.ijadhadh.2025.104048","url":null,"abstract":"<div><h3>Background</h3><div>Adhesive failures in hybrid resin-ceramic restorations remain a critical challenge in restorative dentistry. Despite advancements in materials and techniques, achieving reliable and durable bonds between hybrid ceramics and tooth structures continues to be problematic. Understanding the impact of various adhesion protocols, primers, adhesives, resin cements, and surface pre-treatment are essential to improve clinical outcomes.</div></div><div><h3>Aim</h3><div>The purpose of this systematic review was to evaluate the adhesive failures in hybrid ceramic restorations and compare the effectiveness of different adhesion protocols, materials, and surface pre-treatment.</div></div><div><h3>Methods</h3><div>A comprehensive review of 19 in vitro studies and 2 randomized controlled trials was conducted. Failure rates and causes of adhesive failures were analyzed and categorized based on adhesion protocols, primers, adhesives, resin cements, and surface pre-treatment.</div></div><div><h3>Results</h3><div>Adhesive failures were frequently observed at the interface between the restoration and tooth structure. Failure rates ranged from 7 % to 15 % across different adhesion protocols. Grit-blasting combined with silane coupling agents showed failure rates of 7–15 %, while hydrofluoric acid etching combined with silane coupling agents had failure rates of 10–15 %. Universal adhesives exhibited failure rates of 8–14 %. Self-adhesive resin cements showed failure rates of 8–13 %, total-etch techniques had rates of 7–14 %, and thermocycling resulted in failure rates of 9–15 %. Long-term water storage led to failure rates of 7–15 %. Substrate pre-treatment methods of tooth structure also significantly influenced adhesive failures, with hydrofluoric acid etching and grit-blasting being the most effective but also prone to degradation over time.</div></div><div><h3>Conclusion</h3><div>Adhesive failures in hybrid ceramic restorations are significantly influenced by the choice of adhesion protocols, primers, adhesives, resin cements, and surface pre-treatment. Optimizing these factors and choosing the best techniques and materials are crucial for enhancing bond strength and durability. The inability to perform a meta-analysis due to variability in study designs and outcomes underscores the need for standardized research methodologies in future studies.</div></div>","PeriodicalId":13732,"journal":{"name":"International Journal of Adhesion and Adhesives","volume":"141 ","pages":"Article 104048"},"PeriodicalIF":3.2,"publicationDate":"2025-05-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144071565","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Mechanical behaviour and durability of an epoxy adhesive for structural glass-to-steel connections in a ship","authors":"Danie Wium ,&nbsp;Bert Van Lancker ,&nbsp;Jan Belis ,&nbsp;Evert Lataire","doi":"10.1016/j.ijadhadh.2025.104050","DOIUrl":"10.1016/j.ijadhadh.2025.104050","url":null,"abstract":"<div><div>The luxury yacht industry demands increased vessel transparency by enlarging glazed areas. Structurally integrating glass into yacht structures offers a solution to this. However, this requires a rigid and reliable connection between glass and metal components, which needs to be validated. Consequently, an epoxy adhesive is tested experimentally to evaluate its structural performance for such applications. First, tensile tests on dumbbell specimens are conducted at crosshead speeds of 0.1, 1, 10 and 50 mm/min and temperatures of −20, 23, 50 and 80 °C. Results show that both stiffness and strength increase with strain rate but decrease with increasing temperature, with significant loss at 80 °C. Second, shear tests on double-lap glass-to-steel specimens evaluate adhesion, using a bond thickness of 7 mm to accommodate geometric tolerances in a ship. This thickness is significantly larger than what is recommended by the manufacturer for maximum bond strength. Third, ageing tests are performed on dumbbell and double-lap specimens stored at 50 °C ± 1 °C and 94 ± 1 % relative humidity for six weeks. After ageing, tensile strength and stiffness of the epoxy reduced by 24 % and 51 %, respectively. While double-lap specimens exhibited reduced stiffness after ageing, the scatter on results could not be used to quantify stiffness and strength reduction. During the ageing period the amount of water absorbed by dumbbell specimens was estimated by weighing the specimens periodically. A correlation was found between amount of absorbed water and degraded properties. Based on its high strength and stiffness, epoxy has potential for structural glass-to-steel bonding. However, its viscoelastic behaviour makes it susceptible to temperature and load rate variations.</div></div>","PeriodicalId":13732,"journal":{"name":"International Journal of Adhesion and Adhesives","volume":"141 ","pages":"Article 104050"},"PeriodicalIF":3.2,"publicationDate":"2025-05-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143943189","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Effect of laser patterned microscale interlocking features on aluminum adhesive-bonded single lap joints","authors":"F. Musiari,&nbsp;F. Moroni,&nbsp;A. Lutey","doi":"10.1016/j.ijadhadh.2025.104047","DOIUrl":"10.1016/j.ijadhadh.2025.104047","url":null,"abstract":"<div><div>Many attempts have been made to enhance the strength or toughness of adhesive-bonded joints by fabricating macroscopic interlocking features on adherends or resorting to 3D-printing to produce microscale surface structures. Laser ablation has recently been proposed as a method to manufacture serrated surface profiles on aluminum single lap joints with the aim of improving strength; however, increases have so far been limited due to joint failure resulting from peeling phenomena at the end of the overlap, making enhancements in mechanical interlocking ineffective in the loading direction. The present work seeks to overcome these limitations, increasing the role of interlocking in strengthening laser patterned joints by employing deeper tooth-like features to increase geometric interlocking and thicker substrates to minimize the effect of bending-induced peeling on the initiation and development of failure. Several different patterns have been produced and tested, including both symmetrical (identical adherends) and asymmetrical (complementary adherends) with different feature orientations with respect to the loading direction. The results have revealed that, on single lap joints with thicker adherends, by using deeper asymmetrical features, the strength can be increased by 40 % compared to that obtained with flat adherends.</div></div>","PeriodicalId":13732,"journal":{"name":"International Journal of Adhesion and Adhesives","volume":"141 ","pages":"Article 104047"},"PeriodicalIF":3.2,"publicationDate":"2025-05-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143943188","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Fatigue crack growth analysis of a ductile structural acrylic adhesive under constant-amplitude load control at various loading conditions","authors":"Yu Sekiguchi ,&nbsp;Kazumasa Shimamoto ,&nbsp;Keiji Houjou ,&nbsp;Chiaki Sato","doi":"10.1016/j.ijadhadh.2025.104049","DOIUrl":"10.1016/j.ijadhadh.2025.104049","url":null,"abstract":"<div><div>The fatigue behavior of adhesives depends on the type of adhesive and loading conditions. Highly ductile adhesives, such as structural acrylic adhesives, are excellent under static conditions; however, their fatigue crack growth (FCG) is not yet well understood. Especially when ductile adhesives are used to bond large structures, the joints are subjected to cyclic creep, a combination of fatigue and creep. Therefore, it is important to understand the contribution of creep to FCG clearly.</div><div>The fatigue double cantilever beam tests of a structural acrylic adhesive were conducted by varying mean loads to investigate the effect of creep on FCG. Calculating the equivalent crack length from compliance, the FCG was found to be divided into three stages, similar to the creep curve. The relationships between FCG rate and energy release rate (ERR) and between ERR and the number of cycles until the FCG onset, i.e., the FCG relationship and G−N curve, were investigated using several ERR parameters. A parameter <span><math><mrow><msubsup><mi>G</mi><mrow><mo>Δ</mo><mi>P</mi></mrow><mrow><mn>1</mn><mo>−</mo><mi>γ</mi></mrow></msubsup><mo>·</mo><msubsup><mi>G</mi><mtext>mean</mtext><mi>γ</mi></msubsup></mrow></math></span>, which is a combination of ERRs represented by <span><math><mrow><mo>Δ</mo><mi>P</mi><mo>=</mo><msub><mi>P</mi><mi>max</mi></msub><mo>−</mo><msub><mi>P</mi><mi>min</mi></msub></mrow></math></span> and <span><math><mrow><msub><mi>P</mi><mtext>mean</mtext></msub><mo>=</mo><mrow><mrow><mo>(</mo><mrow><msub><mi>P</mi><mi>max</mi></msub><mo>+</mo><msub><mi>P</mi><mi>min</mi></msub></mrow><mo>)</mo></mrow><mo>/</mo><mn>2</mn></mrow></mrow></math></span>, was found to be the most suitable crack driving force, and was therefore used to discuss fatigue and creep contributions. For the adhesive tested, the creep contribution was slightly greater in the load control than in the displacement control. Furthermore, the effect of R ratio on the FCG relationships of <span><math><mrow><msub><mi>G</mi><mi>max</mi></msub></mrow></math></span> and <span><math><mrow><mo>Δ</mo><mi>G</mi></mrow></math></span> was discussed in relation to the fatigue and creep contributions.</div></div>","PeriodicalId":13732,"journal":{"name":"International Journal of Adhesion and Adhesives","volume":"140 ","pages":"Article 104049"},"PeriodicalIF":3.2,"publicationDate":"2025-05-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143905873","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Additive manufacturing of surface structured metal parts for high strength lightweight injection overmolded polymer-metal hybrid joints","authors":"G.H.M. Oliveira ,&nbsp;V.F. Sciuti ,&nbsp;R.B. Canto ,&nbsp;S. Arneitz ,&nbsp;L. Minkowitz ,&nbsp;S.T. Amancio-Filho ,&nbsp;L.B. Canto","doi":"10.1016/j.ijadhadh.2025.104045","DOIUrl":"10.1016/j.ijadhadh.2025.104045","url":null,"abstract":"<div><div>Polymer-metal hybrid structures (PMH) are increasingly used in the automotive and aerospace industries for lightweight applications. In this study, we investigate the integration of emerging additive manufacturing with injection overmolding to produce high-strength lightweight hybrid joints. AlSi10Mg substrates, with and without submillimeter-sized mushroom-shaped surface structures, were additively manufactured using laser powder bed fusion (L-PBF), followed by injection overmolding (IOM) with polycarbonate (PC). Overlap joints with structured metal substrates demonstrated remarkable joining strength (20.5 ± 3.8 MPa), primarily attributed to the micro-mechanical interlocking between the consolidated polymer and the metal surface structure. Fracture analysis revealed two primary modes of cohesive failure (stretching and shear) in the mushroom-shaped structures, contingent on their location on the metal surface. This behavior was attributed to a combination of interfacial shear stress and secondary bending, as elucidated by digital image correlation (DIC) analysis. The fatigue life of hybrid joints was determined to be 38 % of the joining strength at 10⁶ cycles, indicating excellent mechanical performance and high potential for engineering applications.</div></div>","PeriodicalId":13732,"journal":{"name":"International Journal of Adhesion and Adhesives","volume":"141 ","pages":"Article 104045"},"PeriodicalIF":3.2,"publicationDate":"2025-05-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144071562","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Nano-reinforced adhesives: Effects of graphene, silica, and cellulose on mechanical properties of laminated wood materials","authors":"Huseyin Pelit ,&nbsp;Mustafa Korkmaz ,&nbsp;Esra Davaz","doi":"10.1016/j.ijadhadh.2025.104044","DOIUrl":"10.1016/j.ijadhadh.2025.104044","url":null,"abstract":"<div><div>This study investigated the effects of graphene, silica, and cellulose nanoparticles on the mechanical properties of laminated wood specimens using polyvinyl acetate (PVAc), urea-formaldehyde (UF), and epoxy (EPX) adhesives. Poplar (<em>Populus nigra</em>) and beech (<em>Fagus sylvatica</em>) veneers (4 mm thick) were bonded using adhesives enhanced with varying concentrations of nanoparticles: graphene (0.25 % and 0.50 %), silica (1 % and 2 %), and cellulose (1 % and 2 %). The laminated wood specimens were tested for modulus of elasticity (MOE), modulus of rupture (MOR), compressive strength (CS) and bonding strength (BS). The results showed that the EPX yielded the highest mechanical strength, followed by UF, while PVAc exhibited the lowest. The addition of all nanoparticles improved performance compared to the base adhesives. Graphene additions significantly improved MOE, MOR, and CS, while cellulose and silica primarily enhanced BS strength. Generally, increasing nanoparticle concentration enhanced mechanical properties, with the exception of BS, which decreased with higher silica concentration. These results demonstrate the potential for tailoring laminated wood properties by selecting specific nanoparticle types and concentrations, offering opportunities for optimized and potentially more sustainable material utilization across diverse applications, from furniture to structural components.</div></div>","PeriodicalId":13732,"journal":{"name":"International Journal of Adhesion and Adhesives","volume":"140 ","pages":"Article 104044"},"PeriodicalIF":3.2,"publicationDate":"2025-04-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143902106","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}