{"title":"Synergistic effects of indigenous bacterial consortia on heavy metal tolerance and reduction.","authors":"Rahel Khidr, Karzan Qurbani, Vania Muhammed, Sazgar Salim, Shajwan Abdulla, Hevy Wsw","doi":"10.1007/s10653-025-02392-1","DOIUrl":"10.1007/s10653-025-02392-1","url":null,"abstract":"<p><p>Heavy metal contamination represents a critical environmental and public health challenge, necessitating effective remediation approaches. This study examines the bioremediation potential of three indigenous bacterial strains Aeromonas caviae KQ_21, Aeromonas hydrophila AUoR_24, and Shewanella putrefaciens SUoR_24 evaluated both individually and in consortia for their capacity to remove heavy metals. Tolerance assessments demonstrated that the coculture of these strains exhibited superior resistance to copper (Cu), zinc (Zn), and nickel (Ni), with optimal growth observed up to 6 mM for Cu, 9 mM for Zn, and 5 mM for Ni, outperforming the monocultures. The co-culture system also achieved higher metal reduction efficiencies, with reductions of 47.02% for Cu, 61.49% for Ni, and 61.93% for Zn, in contrast to lower reductions observed in individual strains. The study further explored the impact of environmental conditions on bioremediation efficiency. Optimal temperature for both monoculture and coculture setups was found to be 30 °C. pH and salt concentration variations significantly affected bacterial growth and metal reduction, highlighting the necessity of tailored conditions for enhanced bioremediation. In terms of metal removal mechanisms, the results demonstrated that nickel (Ni) removal occurred primarily through bioaccumulation, while copper (Cu) removal involved both biosorption and bioaccumulation. Zinc (Zn) removal was facilitated through biosorption, bioaccumulation, and biotransformation. These findings underscore the effectiveness of bacterial consortia, particularly indigenous strains, in improving heavy metal tolerance and reduction through synergistic interactions and cooperative metabolic processes. This research offers valuable insights into optimizing bacterial consortia for environmental cleanup and advances the application of indigenous bacteria in bioremediation strategies. Future investigations should focus on exploring additional microbial species and further elucidating the molecular mechanisms that contribute to enhanced bioremediation efficacy.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"47 3","pages":"79"},"PeriodicalIF":3.2,"publicationDate":"2025-02-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143448585","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Soil heavy metals assessment of the Zhoukou riparian zone base of Shaying river basin, China: spatial distribution, source analysis and ecological risk.","authors":"Yimei Ying, Meng Shang, Xu Wang, Xinrui Cui, Ruijie Huang, Zhixin Song, Yunjiao Han","doi":"10.1007/s10653-025-02391-2","DOIUrl":"10.1007/s10653-025-02391-2","url":null,"abstract":"<p><p>The riparian zone serves as an ecological transition area between aquatic and terrestrial environments. Understanding the spatial distribution and origins of heavy metals within this zone is crucial for studying riverine ecosystems. In this research, we assessed the occurrence forms and spatial patterns of heavy metals in the riparian zone of the Shaying River Basin in Zhoukou City. Environmental risks were preliminarily evaluated using indices such as I<sub>geo</sub>, RI, and PLI, and the sources of heavy metals were identified through PMF. The results revealed that the overall ecological risk associated with eight analyzed heavy metals (Cd, Co, Cr, Cu, Mn, Ni, Pb, Zn) in this region was low. However, Cd is marked enriched and represents a significant factor contributing to the potential ecological risk within the riparian zone of the basin. The high bioavailability of Cd and Mn in the soils of nine more contaminated sites showed moderate to very high ecological risk. The PMF model identified four pollution primary sources in this region: agricultural and industrial activities (29.4%), upstream water pollution (21.1%), natural sources (26.5%), and transport-related source (23.1%). These findings establish a scientific foundation for the conservation and management of the ecological environment in the riparian zone of the Shaying River Basin in Zhoukou City. Additionally, they will serve as a reference for future research on soil heavy metal migration and sources within the Huaihe River Basin, China.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"47 3","pages":"77"},"PeriodicalIF":3.2,"publicationDate":"2025-02-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143440284","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Rodrigo Queiroz de Alcântara, Jéssica Frontino Paulino, Felippe Ceraso Gonçalves, Ricardo Gonçalves Cesar, Rodolfo Santos Barboza, Lívia Gonçalves Leida Soares, Manuel Castro Carneiro, Fernanda Veronesi Marinho Pontes
{"title":"Pedogeochemical mobility of metals from fluorescent lamp waste and human health risk assessment.","authors":"Rodrigo Queiroz de Alcântara, Jéssica Frontino Paulino, Felippe Ceraso Gonçalves, Ricardo Gonçalves Cesar, Rodolfo Santos Barboza, Lívia Gonçalves Leida Soares, Manuel Castro Carneiro, Fernanda Veronesi Marinho Pontes","doi":"10.1007/s10653-025-02385-0","DOIUrl":"10.1007/s10653-025-02385-0","url":null,"abstract":"<p><p>The management of fluorescent lamps wastes is a challenge, and its disposal in soils may cause harmful effects on human health and edaphic biota due to the presence of Hg and other potentially toxic metals. However, the pedogeochemical behavior of metals from fluorescent lamps is still rarely studied in the tropics. An Oxisol sample was contaminated in the laboratory using a dosage of 6.5% fluorescent lamp powder relative to the mass of soil. The mobility of metals was assessed through a sequential extraction protocol of the Community Bureau of Reference. To assess potential risks, a mathematical model of Human Health Risk Assessment was employed, based on human exposure on metal-contaminated groundwater from soil contamination. Evaluation of metal mobility showed that 6% of Ni and 30% of Cu in contaminated soil were in the potentially bioavailable fraction. The slightly acidic pH of the contaminated soil seems to influence the mobility of Ni and Cu. Zn and Pb were mainly found in the residual fraction, suggesting low geochemical availability. However, over time, metals may be leached, highlighting the importance of monitoring disposal areas. When these results are compared to the mobility profile found in extractions applied to pure fluorescent lamps waste, the data suggest that soil properties tend to reduce metal mobility. Human Health Risk Assessment showed significant risks associated with the human consumption of Cu-contaminated groundwater, considering a scenario of metal leaching from the soil. This study highlights the need for proper fluorescent lamps disposal in tropical terrestrial systems to prevent ecological and public health risks.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"47 3","pages":"78"},"PeriodicalIF":3.2,"publicationDate":"2025-02-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143440280","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Ensuring food safety by combining phytoremediation and food crop cultivation: a case study in farmlands near a lead-zinc mine in Southwest China.","authors":"Wenting Liu, Ming Li, Landry Soh Tamehe, Yuhong Tang, Yujiao Shi, Lishan Huang","doi":"10.1007/s10653-025-02377-0","DOIUrl":"10.1007/s10653-025-02377-0","url":null,"abstract":"<p><p>Environmental pollution by heavy metals (HMs) in mining areas is a major concern worldwide since it pollutes the surrounding surface water, groundwater, and farmland soils. Once in the food chain, HMs can cause mild to life-threatening side effects thereby negatively affecting the environment and human health. To remedy this situation, cost-effective and environmentally friendly remediation approaches are needed to ensure food safety. Phytoremediation is a remediation technique that meets these criteria; however, it is still unclear whether co-cultivation of food crops during phytoremediation can produce crops that meet the required safety standards. In this study, we investigate the effectiveness of phytoremediation and food crop co-cultivation to produce \"HM-free\" crops from farmland soils in Sidi village in Xingping Town of Guangxi Zhuang Autonomous Region in China, contaminated by HMs from a lead-zinc mine. Our results show that (1) After 19 months of phytoremediation, the redistribution of HMs (cadmium, lead, and arsenic) from acidic to slightly acidic, neutral, and mostly weakly alkaline soils was promoted. This resulted in a reduction in HMs availability and consequently the amount absorbed by food crops. (2) The concentrations of important nutrients including nitrogen, phosphorus, and potassium were significantly increased during phytoremediation. This translated to increased plant biomass in Celosia Argentea L. (26.09%), Sedum erythrostictum Migo (18.52%), and Amaranthus cruentus L. (21.67, 33.33, and 66.67%, for consecutive harvests). (3) Co-cultivation of maize crops with low HM accumulator plants in slightly and moderately polluted sites or a rotation of rapeseed-sunflower plants with hyperaccumulator plants in the highly polluted site ensured 100% compliance with the food crop and feed safety standards. Our findings can provide an important reference for studies aimed at managing polluted sites and ensuring food safety.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"47 3","pages":"76"},"PeriodicalIF":3.2,"publicationDate":"2025-02-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143406362","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"The coexistence characteristics of microplastics and heavy metals in rhizomes of traditional Chinese medicine in mulch planting area.","authors":"Cong Xiao, Jiabin Zhou, Wen Xiong, Xiaochuan Ye","doi":"10.1007/s10653-025-02393-0","DOIUrl":"10.1007/s10653-025-02393-0","url":null,"abstract":"<p><p>Rhizomatous traditional Chinese medicines (RTCMs) are widely crushed into powder and swallowed directly as medicine and food or health products to treat various diseases; however, they may contain toxic microplastics (MPs) and heavy metals. Currently, there are no reports on the detection of MPs and MP-heavy metal synergies in RTCMs. In this study, we selected eight representative RTCMs to investigate the abundance, types, sizes, and polymers of MP and heavy metals and to assess the level of contamination of MPs and synergies between MPs and heavy metals in RTCMs. The abundance of MPs in different RTCM ranged from 20.83 to 43.65 items/g. The dominant type was fragment (95.43%), and the dominant particle size was < 0.5 mm (73.72%) in MPs. Polyurethane (PU) (29.21%) and acrylics (ACR 13.53%) were the dominant polymers of MP. MP polymers showed obvious correlations with type and particle size: PU was enriched in 0-50-mm and 100-300-mm fragments, whereas ethylene vinyl acetate and ACR were enriched in 0-30-mm fibers. The heavy metals arsenic (As), lead (Pb), and chromium (Cr) were found to be more susceptible to synergistic contamination with MPs in RTCMs compared to other heavy metals. The estimated daily intake (EDI) of the MPs and heavy metals for RG (Rehmannia glutinosa) and RAY (Rhizoma atractylodis) were higher than others. The results showed that MP pollution is common in RTCMs and carries the potential risk of heavy metal or MP poisoning in humans who consume RTCMs.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"47 3","pages":"74"},"PeriodicalIF":3.2,"publicationDate":"2025-02-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143398716","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Groundwater quality and hydrogeochemical challenges in the Sarakhs Plain, NE Iran: a call for sustainable management.","authors":"Maryam Tajbakhshian","doi":"10.1007/s10653-025-02371-6","DOIUrl":"10.1007/s10653-025-02371-6","url":null,"abstract":"<p><p>The physicochemical analysis of 292 groundwater samples from the Sarakhs Plain revealed significant variations in water quality, influenced by natural factors. The pH values ranged from 6.4 to 8.6, with an average of 7.97, indicating that most of the samples (98.97%) meet WHO drinking water standards. However, electrical conductivity (EC) levels were alarmingly high, ranging from 1020 to 37,500 μS cm<sup>-1</sup>, making all samples unsuitable for drinking. Ca<sup>2+</sup> and Mg<sup>2+</sup> concentrations were within acceptable limits for approximately 88.39% and 61.09% of the samples, respectively. Spatial distribution analysis showed that higher salinity levels were concentrated in the western and central regions, while the eastern areas benefited from fresher water due to the influence of the Harirud River, which enhances groundwater quality through natural dilution processes. Hydrogeochemical assessments indicated a predominance of mixed-type water, with significant intrusion processes affecting chemical composition. The Gibbs diagram highlighted evaporation as a major factor influencing water chemistry. Groundwater quality index (GWQI) indicated that nearly half of the samples were classified as unsuitable for drinking, while agricultural suitability varied significantly. Although salinity was a critical concern, many samples were deemed suitable for irrigation based on specific ion concentrations. Overall, this study addressed the necessity for sustainable groundwater management practices in the Sarakhs Plain to mitigate salinity issues and enhance water quality for both human consumption and agricultural use.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"47 3","pages":"75"},"PeriodicalIF":3.2,"publicationDate":"2025-02-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143398743","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Dragan Čakmak, Veljko Perović, Dragana Pavlović, Marija Matić, Darko Jakšić, Samat Tanirbergenov, Pavle Pavlović
{"title":"Development of optimisation methods to identify sources of pollution and assess potential health risks in the vicinity of antimony mines.","authors":"Dragan Čakmak, Veljko Perović, Dragana Pavlović, Marija Matić, Darko Jakšić, Samat Tanirbergenov, Pavle Pavlović","doi":"10.1007/s10653-025-02369-0","DOIUrl":"10.1007/s10653-025-02369-0","url":null,"abstract":"<p><p>After elevated levels of lead (Pb) were found in the blood of children living near the antimony (Sb) mine and battery smelter in Zajača, Republic Serbia, studies were carried out to determine the health risk assessment (HRA) effects of the soil. In this study, for the first time a combination of Network Analysis, CoDA (Compositional Data Analysis) and receptor modelling was used to determine the geopedological and atmospheric origin of PTEs in soil and their historical significance. It was found that arsenic (As) and Pb are the main pollutants in the area. The largest contribution to the environmental risk (Er) was made by Pb. In addition to perception methods Network Analysis (NA) was used to determine the source of pollution and, for the first time, the strength of the positive and negative connections of the network nodes of the mutual influence of PTE. Lead pollution was found to originate from two sources: historical and present, and As was found to originate from a wider area. For the child population, an unacceptable risk for the occurrence of chronic diseases with a probability of 95% was found, with As and Pb accounting for the highest percentage. Similarly, As has the greatest impact on occurrence of cancer at the unacceptable risk level, while Pb is at the notable risk level. The historical exposure to Pb is slightly lower and the difference is slightly more pronounced for total pollution for HRA.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"47 3","pages":"73"},"PeriodicalIF":3.2,"publicationDate":"2025-02-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11814042/pdf/","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143390526","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Archi Mishra, Shamsh Pervez, Yasmeen Fatima Pervez, Madhuri Verma, Princy Dugga, Sushant Ranjan Verma, Indrapal Karbhal, Kallol K Ghosh, Manas Kanti Deb, Manmohan L Satnami, Kamlesh Shrivas
{"title":"Particulate toxic elements' oxidative potential and gastrointestinal bioaccessibility features in the vicinities of coal-fired mineral processing industries, India.","authors":"Archi Mishra, Shamsh Pervez, Yasmeen Fatima Pervez, Madhuri Verma, Princy Dugga, Sushant Ranjan Verma, Indrapal Karbhal, Kallol K Ghosh, Manas Kanti Deb, Manmohan L Satnami, Kamlesh Shrivas","doi":"10.1007/s10653-025-02388-x","DOIUrl":"10.1007/s10653-025-02388-x","url":null,"abstract":"<p><p>Particulate matter (PM) poses significant health risks due to its ability to generate reactive oxygen species (ROS) and transport toxic metal(loid)s into the human body. In this study, an in vitro physiologically based extraction test (PBET) method, allowing the simulation of the gastric phase (GPh) and intestinal phase (IPh) of human digestion, was applied to evaluate bioaccessibility of eleven potentially toxic elements (Al, As, Cd, Co, Cr, Cu, Fe, Mn, Ni, Pb, and Zn) in airborne particulate matter (APM) samples collected from an urban-residential area in Chhattisgarh, India. Additionally, oxidative potential (OP) was assessed using the dithiothreitol (DTT) assay for a comprehensive understanding of PM toxicity. The bioaccessibility of metal(loid)s varied significantly across phases, with gastric phase solubility upto ~ 75%, attributed to its lower pH enhancing metal dissolution. Elevated DTT responses were recorded for PM<sub>10</sub> and PM<sub>2.5</sub>, driven primarily by Fe, Zn, and Pb, underlining their pivotal role in oxidative stress generation. Correlation analyses demonstrated strong associations between bioaccessible fractions and OP, especially in the GPh. The findings advance understanding by linking bioaccessibility with ROS generation and highlight the importance of particle size and solubility in assessing the health risks posed by PM. These insights provide a foundation for improved risk assessments and mitigation strategies targeting emissions from high-temperature processing industries, and vehicular activities, on a global scale.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"47 3","pages":"72"},"PeriodicalIF":3.2,"publicationDate":"2025-02-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143381933","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Organic-inorganic interplay and paleoenvironmental reconstruction of Asia's largest opencast lignite mine deposits.","authors":"B Preethi, T Subramani, T Nathiya, Zaixing Huang","doi":"10.1007/s10653-025-02384-1","DOIUrl":"10.1007/s10653-025-02384-1","url":null,"abstract":"<p><p>Asia's largest opencast lignite mines, located in Neyveli, Tamil Nadu, India, were studied to evaluate the organic and inorganic characteristics and reconstruct the paleo-depositional environment of the lignite deposits. The investigation involved advanced geochemical and analytical techniques, including X-ray fluorescence, field emission scanning electron microscopy (FE-SEM), as well as proximate and ultimate analyses. The physical properties of the lignite revealed a moisture content ranging from a minimum of 7.5% to a maximum of 25%, with an average of 14.4%. The ash content varied between 2.6 and 19%, with an average of 6.6%, suggesting the low mineral impurity levels in the lignite deposits. Volatile matter ranged from 38.2 to 48.9%, while fixed carbon content was observed between 31.4 and 40.3%. The ultimate analysis identified carbon content ranging from 51.93 to 78.58%, with moderate levels of hydrogen (< 5%), nitrogen (< 5%), and sulfur (< 1%). Variations in the Gross Calorific Value (4608-5882 kcal/kg) reflect the heterogeneous nature of the lignite, emphasizing the necessity of utilization strategies based on energy density. Major oxide analysis demonstrated strong correlations among SiO<sub>2</sub>, Al<sub>2</sub>O<sub>3</sub>, and TiO<sub>2</sub> with ash yield, suggesting a shared origin and close association with the inorganic constituents of the lignite. Trace elements revealed significant associations among elements such as Zr, V, Sr, Nb, Ga, and Cr, providing the geochemical composition of Neyveli lignite. Microstructural investigation via FE-SEM revealed a fine-grained morphology, distinct mineral phases, and porosity characteristics. Weathering indices and alteration studies pointed to a felsic to intermediate igneous provenance for the inorganic components. The study situates the Neyveli lignite deposits within a deltaic depositional system formed during the late Cretaceous to early Tertiary periods. This paleoenvironment was characterized by dynamic hydrological regimes, as evidenced by sedimentary structures and interbedded lignite layers.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"47 3","pages":"70"},"PeriodicalIF":3.2,"publicationDate":"2025-02-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143373925","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Yindi Peng, Yamin Zhao, Ning Gao, Dan Sheng, Shaoyan Tang, Shan Zheng, Minzhen Wang
{"title":"Spatiotemporal evolution of PM<sub>2.5</sub> and its components and drivers in China, 2000-2023: effects of air pollution prevention and control actions in China.","authors":"Yindi Peng, Yamin Zhao, Ning Gao, Dan Sheng, Shaoyan Tang, Shan Zheng, Minzhen Wang","doi":"10.1007/s10653-025-02375-2","DOIUrl":"10.1007/s10653-025-02375-2","url":null,"abstract":"<p><p>This study evaluated the Air Pollution Prevention and Control Action Plan (APPCAP) in China using 2000-2023 data. The average annual PM<sub>2.5</sub> concentration dropped from 46.11 ± 16.18 µg/m<sup>3</sup> to 31.75 ± 14.22 µg/m<sup>3</sup> (P < 0.05) after APPCAP, with components showing a similar decline. Temporal analysis via Mann-Kendall test indicated a decreasing trend (Z < 0, P < 0.05), seasonally peaking in winter and lowest in summer. Spatially, APPCAP reduced concentration distribution, with key regions improving but areas like Shandong and Henan still facing severe pollution. The main PM<sub>2.5</sub> driver shifted from human (e.g., population density) to meteorological (e.g., temperature) factors post-APPCAP, and anthropogenic influence varied across regions. In summary, APPCAP has curbed PM<sub>2.5</sub> pollution, yet SO<sub>4</sub><sup>2-</sup>, NO<sub>3</sub><sup>-</sup>, and NH<sub>4</sub><sup>+</sup> remain relatively high, and the increasing human impact in central and southeastern China demands attention in future policies.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"47 3","pages":"69"},"PeriodicalIF":3.2,"publicationDate":"2025-02-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143373926","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}