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Structural insights into soft matter materials via spin echo small angle neutron scattering and small angle neutron scattering 通过自旋回波小角中子散射和小角中子散射洞察软物质材料的结构
Nuclear Analysis Pub Date : 2024-08-16 DOI: 10.1016/j.nucana.2024.100128
Tingting Wang
{"title":"Structural insights into soft matter materials via spin echo small angle neutron scattering and small angle neutron scattering","authors":"Tingting Wang","doi":"10.1016/j.nucana.2024.100128","DOIUrl":"10.1016/j.nucana.2024.100128","url":null,"abstract":"<div><p>The recent advancements in neutron scattering technologies in China, with the development of China's first Spin-Echo Small-Angle Neutron Scattering (SESANS) spectrometer at China Mianyang Research Reactor (CMRR) and the integration of a Very Small Angle Neutron Scattering (VSANS) instrument at China Spallation Neutron Source (CSNS), have significantly bolstered the nation's scientific capabilities. This review aims to highlight the distinctive features and applications of SESANS and SANS, and to offer a valuable contribution by demonstrating how SESANS and SANS can be leveraged for the study of soft matters and solid-state materials, with a particular emphasis on the benefits of techniques such as chain labeling, contrast variation, and contrast matching. We also aim to illustrate what types of information can be gleaned from these methods. The review is structured to first introduce the general concepts of SANS and SESANS, followed by a discussion on the information these techniques can provide. Then the applications of these techniques, in combination with other techniques, on various material investigations will be demonstrated. The review concludes with a summary and future perspectives, aiming to inspire further interdisciplinary research and collaboration, and beneficial to a broader audience.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 3","pages":"Article 100128"},"PeriodicalIF":0.0,"publicationDate":"2024-08-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000284/pdfft?md5=35c8e99ee7a1b6e9645a922724fdd3ac&pid=1-s2.0-S2773183924000284-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142040717","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Gold nanoparticle effect on dose and DNA damage enhancement in the vicinity of gold nanoparticles 金纳米粒子对剂量和金纳米粒子附近 DNA 损伤增强的影响
Nuclear Analysis Pub Date : 2024-08-13 DOI: 10.1016/j.nucana.2024.100126
Adil Bardane , Nabil Maalej , El Mahjoub Chakir , El Mehdi Al Ibrahmi
{"title":"Gold nanoparticle effect on dose and DNA damage enhancement in the vicinity of gold nanoparticles","authors":"Adil Bardane ,&nbsp;Nabil Maalej ,&nbsp;El Mahjoub Chakir ,&nbsp;El Mehdi Al Ibrahmi","doi":"10.1016/j.nucana.2024.100126","DOIUrl":"10.1016/j.nucana.2024.100126","url":null,"abstract":"<div><p>This study uses Monte Carlo simulations to examine the dose enhancement effect of gold nanoparticles (AuNPs) in radiation therapy and its effects on DNA damage. Using the GATE- 9.0 and Geant4-DNA packages, Monte Carlo simulations were used to simulate a mathematical phantom and determine the energy deposition in the vicinity of AuNP. The simulations were conducted for various photon beam energies (50, 100, 250, and 6000 keV) with and without the presence of different-size AuNPs (10, 30, 50 and 100 nm). The dose enhancement factor (DER) was evaluated using Geant4-DNA to examine the effects AuNP sizes and photon beam energies on DNA damage. A multi-scale Monte Carlo simulation was conducted to evaluate enhanced DNA damage owing to nanoparticles in the proximity of cancer cells. The Monte Carlo simulations indicated that AuNPs boost the dose delivery, resulting in enhanced energy deposition and subsequent DNA damage. The DER analysis revealed a significant increase in the dose deposition within DNA, leading to single or double-strand breaks. Geant4-DNA simulations revealed information on the dosage enhancement factor for various AuNP sizes and photon beam intensities, enabling a deeper comprehension of the underlying mechanics. The outcomes of this study emphasize the potential of AuNPs as effective radiosensitizers in radiation therapy and contribute to the growing body of research on the use of nanotechnology in enhancing cancer treatment outcomes. Further investigations and experimental validations are necessary to optimize the usage of AuNPs for improved radiation therapy.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 4","pages":"Article 100126"},"PeriodicalIF":0.0,"publicationDate":"2024-08-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000260/pdfft?md5=28fbf1d35df9f3b5d4b49c66adb0a166&pid=1-s2.0-S2773183924000260-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142011368","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Fusion mechanism involved in the synthesis of superheavy element Z>118 using Mn projectiles 利用锰射弹合成超重元素 Z>118 所涉及的聚变机制
Nuclear Analysis Pub Date : 2024-08-06 DOI: 10.1016/j.nucana.2024.100124
H.S. Anushree , N. Sowmya , H.C Manjunatha , S. Shubha
{"title":"Fusion mechanism involved in the synthesis of superheavy element Z>118 using Mn projectiles","authors":"H.S. Anushree ,&nbsp;N. Sowmya ,&nbsp;H.C Manjunatha ,&nbsp;S. Shubha","doi":"10.1016/j.nucana.2024.100124","DOIUrl":"10.1016/j.nucana.2024.100124","url":null,"abstract":"&lt;div&gt;&lt;div&gt;We conducted an in-depth investigation of Mn-induced fusion reactions aimed at synthesizing superheavy elements with atomic numbers Z=119 to Z=123. Our analysis considers the total potential, which combines Coulomb and nuclear potentials. The nuclear potential was calculated using the Thomas–Fermi approach, a valuable method for modeling the behavior of nucleons in atomic nuclei. within the framework of advanced statistical model, the evaporation residue cross-sections were determined. At optimal energies, we have calculated capture, fusion, and evaporation residue cross-sections for the reactions of all the projectile–target combinations. All &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;53&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Mn isotopes with larger half-lives were taken into consideration as projectiles. Fusion reactions between &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;53&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Mn projectiles with &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;238&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;242&lt;/mn&gt;&lt;mo&gt;,&lt;/mo&gt;&lt;mn&gt;244&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Pu, &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;241&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;243&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Am, &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;242&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;248&lt;/mn&gt;&lt;mo&gt;,&lt;/mo&gt;&lt;mn&gt;250&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Cm, &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;247&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;249&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Bk, and &lt;span&gt;&lt;math&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;248&lt;/mn&gt;&lt;mo&gt;−&lt;/mo&gt;&lt;mn&gt;254&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;/math&gt;&lt;/span&gt;Cf. Detailed investigations were made and promising reactions viz. &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;241&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Pu&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;293&lt;/sup&gt;119, &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;242&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Am&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;294&lt;/sup&gt;120, &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;247&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Cm&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;299&lt;/sup&gt;121, &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;248&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Bk&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;55&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;300&lt;/sup&gt;122 and &lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;251&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Cf&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt; (&lt;span&gt;&lt;math&gt;&lt;mrow&gt;&lt;msup&gt;&lt;mrow&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mn&gt;53&lt;/mn&gt;&lt;/mrow&gt;&lt;/msup&gt;&lt;mi&gt;Mn&lt;/mi&gt;&lt;/mrow&gt;&lt;/math&gt;&lt;/span&gt;, 3n)&lt;sup&gt;301&lt;/sup&gt;123 with maximum &lt;span&gt;&lt;math&gt;&lt;msub&gt;&lt;mrow&gt;&lt;mi&gt;σ&lt;/mi&gt;&lt;/mrow&gt;&lt;mrow&gt;&lt;mi&gt;E&lt;/mi&gt;&lt;mi&gt;R&lt;/mi&gt;&lt;/mrow&gt;&lt;/msub&gt;&lt;/math&gt;&lt;/span&gt; are found to be 415.1 fb at 240 MeV, 115.4 fb at 244 MeV, 36.5 fb at 245 MeV, 13.6 fb at 249 MeV, 5.4 fb at 250 MeV for Z=119-123 respectively. Th","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 4","pages":"Article 100124"},"PeriodicalIF":0.0,"publicationDate":"2024-08-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142327640","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Evaluation of Potassium-40 and Uranium-238 activities and radiological risk in Missour, Morocco soils using gamma spectrometry 利用伽马能谱仪评估摩洛哥米苏尔土壤中钾-40 和铀-238 的放射性活度及辐射风险
Nuclear Analysis Pub Date : 2024-08-05 DOI: 10.1016/j.nucana.2024.100125
Abdessamad Didi , Hamid Bounouira , Abir Adnane , Soumaia El Khamsi Chahd , Hamid Amsil , Abdelwahab Badague , Iliasse Aarab
{"title":"Evaluation of Potassium-40 and Uranium-238 activities and radiological risk in Missour, Morocco soils using gamma spectrometry","authors":"Abdessamad Didi ,&nbsp;Hamid Bounouira ,&nbsp;Abir Adnane ,&nbsp;Soumaia El Khamsi Chahd ,&nbsp;Hamid Amsil ,&nbsp;Abdelwahab Badague ,&nbsp;Iliasse Aarab","doi":"10.1016/j.nucana.2024.100125","DOIUrl":"10.1016/j.nucana.2024.100125","url":null,"abstract":"<div><p>The objective of this study is to assess natural activity in soil to estimate potential radiological risks for the population. Given that soil is inherently radioactive and can reach hazardous levels, it is crucial to determine the activities of radionuclides such as Potassium-40 and Uranium-238 descendants at different depths and geographical positions. For this work, gamma spectrometry method was employed to analyze soil samples collected at three different positions in the Missour region. Each position was sampled at five different depths, spaced 5 cm apart, resulting in a total of 15 samples. The activity of Potassium-40 and Uranium238 descendants in the soil was accurately assessed using Lvis software, enabling the estimation of radiological doses.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 3","pages":"Article 100125"},"PeriodicalIF":0.0,"publicationDate":"2024-08-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000259/pdfft?md5=b064fa8f6785305a19ec020d1f7ebcfe&pid=1-s2.0-S2773183924000259-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141964342","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Compound nucleus formation probability of heavy and superheavy nuclei synthesized using heavy ion fusion reactions 利用重离子聚变反应合成的重核和超重核的复合核形成概率
Nuclear Analysis Pub Date : 2024-07-31 DOI: 10.1016/j.nucana.2024.100123
Reddi Rani L. , N. Sowmya , H.C. Manjunatha , M.M. Armstrong Arasu
{"title":"Compound nucleus formation probability of heavy and superheavy nuclei synthesized using heavy ion fusion reactions","authors":"Reddi Rani L. ,&nbsp;N. Sowmya ,&nbsp;H.C. Manjunatha ,&nbsp;M.M. Armstrong Arasu","doi":"10.1016/j.nucana.2024.100123","DOIUrl":"10.1016/j.nucana.2024.100123","url":null,"abstract":"<div><div>The role of entrance channel parameters such as <span><math><mrow><msup><mrow><mi>Z</mi></mrow><mrow><mn>2</mn></mrow></msup><mo>/</mo><mi>A</mi></mrow></math></span>, charge asymmetry <span><math><msub><mrow><mi>α</mi></mrow><mrow><mi>z</mi></mrow></msub></math></span>, mass-asymmetry (<span><math><msub><mrow><mi>η</mi></mrow><mrow><mi>A</mi></mrow></msub></math></span>), charge product (<span><math><mrow><msub><mrow><mi>Z</mi></mrow><mrow><mn>1</mn></mrow></msub><msub><mrow><mi>Z</mi></mrow><mrow><mn>2</mn></mrow></msub></mrow></math></span>), mean fissility <span><math><msub><mrow><mi>χ</mi></mrow><mrow><mi>m</mi></mrow></msub></math></span>, Coulomb interaction parameter and <span><math><mrow><mrow><mo>(</mo><mi>N</mi><mo>−</mo><mi>Z</mi><mo>)</mo></mrow><mo>/</mo><mrow><mo>(</mo><mi>N</mi><mo>+</mo><mi>Z</mi><mo>)</mo></mrow></mrow></math></span> on compound nucleus formation of actinide nuclei using heavy ion fusion reactions were investigated. For the formation of compound nuclei, the considered atomic number range of the projectile varies between <span><math><mrow><mn>5</mn><mo>≤</mo><mi>Z</mi><mo>≤</mo><mn>14</mn></mrow></math></span> and the mass number lies between <span><math><mrow><mn>10</mn><mo>≤</mo><mi>A</mi><mo>≤</mo><mn>34</mn></mrow></math></span>. Similarly, the studied target atomic number varies between <span><math><mrow><mn>78</mn><mo>≤</mo><mi>Z</mi><mo>≤</mo><mn>92</mn></mrow></math></span> and the mass number range is <span><math><mrow><mn>197</mn><mo>≤</mo><mi>A</mi><mo>≤</mo><mn>238</mn></mrow></math></span>. Among these entrance channel parameters, <span><math><msub><mrow><mi>P</mi></mrow><mrow><mi>C</mi><mi>N</mi></mrow></msub></math></span> is more systematic for <span><math><mfrac><mrow><mrow><mo>(</mo><mi>N</mi><mo>−</mo><mi>Z</mi><mo>)</mo></mrow></mrow><mrow><mrow><mo>(</mo><mi>N</mi><mo>+</mo><mi>Z</mi><mo>)</mo></mrow></mrow></mfrac></math></span>, <span><math><mrow><msup><mrow><mi>Z</mi></mrow><mrow><mn>2</mn></mrow></msup><mo>/</mo><mi>A</mi></mrow></math></span> and <span><math><msub><mrow><mi>α</mi></mrow><mrow><mi>z</mi></mrow></msub></math></span>. In addition to entrance channel parameters, the <span><math><msub><mrow><mi>E</mi></mrow><mrow><mi>c</mi><mi>m</mi></mrow></msub></math></span> and <span><math><msub><mrow><mi>E</mi></mrow><mrow><mi>B</mi><mi>a</mi><mi>s</mi><mi>s</mi></mrow></msub></math></span> also play a significant role in the prediction of <span><math><msub><mrow><mi>P</mi></mrow><mrow><mi>C</mi><mi>N</mi></mrow></msub></math></span>. The proposed empirical formulae are applicable to the compound nuclei from Fr to Sg. These findings are significant for the <span><math><msub><mrow><mi>P</mi></mrow><mrow><mi>C</mi><mi>N</mi></mrow></msub></math></span> prediction from Fr to Sg.</div></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 4","pages":"Article 100123"},"PeriodicalIF":0.0,"publicationDate":"2024-07-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142358342","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Feasibility of producing 225Ac via thermal neutron irradiation of 226Ra: A systematic theoretical study 通过热中子辐照 226Ra 生产 225Ac 的可行性:系统理论研究
Nuclear Analysis Pub Date : 2024-07-20 DOI: 10.1016/j.nucana.2024.100122
Long Qiu , Jinsong Zhang , Tu Lan , Jiali Liao , Yuanyou Yang , Feize Li , Ning Liu
{"title":"Feasibility of producing 225Ac via thermal neutron irradiation of 226Ra: A systematic theoretical study","authors":"Long Qiu ,&nbsp;Jinsong Zhang ,&nbsp;Tu Lan ,&nbsp;Jiali Liao ,&nbsp;Yuanyou Yang ,&nbsp;Feize Li ,&nbsp;Ning Liu","doi":"10.1016/j.nucana.2024.100122","DOIUrl":"10.1016/j.nucana.2024.100122","url":null,"abstract":"<div><p>With a suitable half-life and abundant radiolabeling strategy, <sup>225</sup>Ac has become one of the most promising radionuclides in the area of targeted alpha therapy. However, limited radionuclide supply is threatening the development of <sup>225</sup>Ac related endoradiotherapy dramatically. As the parent nuclide of <sup>225</sup>Ac, <sup>229</sup>Th can be produced via <sup>226</sup>Ra(3n, 2β)<sup>229</sup>Th reaction in a nuclear reactor. However, related practice has not been conducted in large scale, since the nuclear reaction pathway for producing <sup>229</sup>Th is complicated. In this work, the feasibility of producing <sup>225</sup>Ac/<sup>229</sup>Th in a reactor was confirmed by systematic theoretical calculations, and a procedure that combines irradiation with separation process was proposed. The results show that 176 MBq of <sup>229</sup>Th can be produced by irradiating 1.0 g of <sup>226</sup>Ra with a neutron flux density of 1 × 10<sup>15</sup> n cm<sup>−2</sup> s<sup>−1</sup> for 90 days. This will generate 150 MBq of <sup>225</sup>Ac monthly from a radionuclide generator, which is sufficient for the single treatment cycle of 200 patients each year considering the radioactivity loss in radiochemical separation, transfer and radiolabeling process. In addition, this irradiation process will also produce 37.8 GBq <sup>227</sup>Ac for the preparation of <sup>227</sup>Ac-<sup>227</sup>Th-<sup>223</sup>Ra generator. In general, the production of <sup>225</sup>Ac by neutron irradiation of <sup>226</sup>Ra in reactor is practicable and holds potential to alleviate the shortage of current supply of <sup>225</sup>Ac.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 3","pages":"Article 100122"},"PeriodicalIF":0.0,"publicationDate":"2024-07-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000223/pdfft?md5=459ab0fb9ccb924e8ab5a6fed4199880&pid=1-s2.0-S2773183924000223-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141839148","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Radiological impact of hydrocarbon waste release on drinking water of ughievwen and udu communities, delta state Nigeria 碳氢化合物废物排放对尼日利亚三角洲州 Ughievwen 和 Udu 社区饮用水的辐射影响
Nuclear Analysis Pub Date : 2024-07-16 DOI: 10.1016/j.nucana.2024.100121
Oghenevovwero Emmanuel Esi
{"title":"Radiological impact of hydrocarbon waste release on drinking water of ughievwen and udu communities, delta state Nigeria","authors":"Oghenevovwero Emmanuel Esi","doi":"10.1016/j.nucana.2024.100121","DOIUrl":"10.1016/j.nucana.2024.100121","url":null,"abstract":"<div><p>Well water quality has been characterized with constant and continuous changes via the interaction of rock, soil and natural nano-filters which terminates at the aquiferous layer for clean well-water collection. The continuous exploration and production of crude oil has resulted significant increase of unwanted elements such as naturally occurring radionuclides in the water-bed which necessitates this study. The study determines the radionuclides based health impact or hazards associated with drinking water from crude oil exploration/production release in Ughievwen and Udu communities of Delta State, Nigeria. Sixty well water samples (three samples from each community) were collected and analyzed using sodium iodide (Nal (Tl)) detector. The obtained mean values of <sup>238</sup>U, <sup>232</sup>Th and <sup>40</sup>K are 6.91 <span><math><mrow><mo>±</mo></mrow></math></span> 1.62BqL<sup>−1</sup>, 4.39 <span><math><mrow><mo>±</mo></mrow></math></span> 1.47 BqL<sup>−1</sup> and 24.54 <span><math><mrow><mo>±</mo></mrow></math></span> 1.59 BqL<sup>−1</sup> respectively. The <sup>238</sup>U, <sup>232</sup>Th and <sup>40</sup>K results showed that the measured values are higher than the world standard (UNSCEAR; WHO) and the control values The mean values of total annual effective dose of different age groups are: 11.08 mSvy<sup>−1</sup>, 2.54 mSvy<sup>−1</sup>, 1.93 mSvy<sup>−1</sup>, 2.52 mSvy<sup>−1</sup>, 7.03 mSvy<sup>−1</sup> and 1.12 mSvy<sup>−1</sup> respectively. While the mean committed effective dose of adult is 55.94 mSvy<sup>−1</sup>. The total annual effective dose, committed effective dose, cancer risks and hereditary effects are all lower than recommended limit (WHO; ICRP; USEPA) and reported scientific values except 11.08 mSvy<sup>−1</sup> and 7.03 mSvy<sup>−1</sup> that are higher than limit. It is evident from obtained results that the drinking water may not be radiologically safe for use by the public, which necessitates routine monitoring and caution to circumvent increase in radiation and the radiological of the studied communities’ drinking water. This is to avoid long term radiological risk arising from accumulation of such release in the studied communities.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 3","pages":"Article 100121"},"PeriodicalIF":0.0,"publicationDate":"2024-07-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000211/pdfft?md5=869ab386a09f2b2eca91c3c05f0eb686&pid=1-s2.0-S2773183924000211-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141850667","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Temperature distribution in the PGAA system: Collimator, shutter, and filter in TRIGA Mark II reactor PGAA 系统中的温度分布:TRIGA Mark II 反应器中的准直器、快门和过滤器
Nuclear Analysis Pub Date : 2024-07-09 DOI: 10.1016/j.nucana.2024.100120
Jamila Yousfi , Abdessamad Didi , Hamane Lemziouka , Lamiae Mrharrab , Hamid Amsil , Otman Jai , Hamid Bounouira , Khalid Larakil
{"title":"Temperature distribution in the PGAA system: Collimator, shutter, and filter in TRIGA Mark II reactor","authors":"Jamila Yousfi ,&nbsp;Abdessamad Didi ,&nbsp;Hamane Lemziouka ,&nbsp;Lamiae Mrharrab ,&nbsp;Hamid Amsil ,&nbsp;Otman Jai ,&nbsp;Hamid Bounouira ,&nbsp;Khalid Larakil","doi":"10.1016/j.nucana.2024.100120","DOIUrl":"https://doi.org/10.1016/j.nucana.2024.100120","url":null,"abstract":"<div><p>This article examines the impact of temperature on the steel collimator cap and the primary beam shutter. These components will be used to implement the Prompt Gamma Activation Analysis (PGAA) technique in the Moroccan TRIGA Mark-II research reactor. The steel collimator plug is essential for forming the neutron beam, while the main role of the shutter is to stop the beam when the channel is inactive. This study analyzes the effect of temperature on the collimator and shutter system, particularly focusing on the variation in maximum temperature over a month of operation with 8-h cycles per day, the behavior of temperature over 24 h, the total heat flux as a function of the length of the experimental device, the temperature distribution in mild steel (E235) and 304L stainless steel materials, and the total displacement and strain gradient as a function of temperature. All calculations were performed using COMSOL Multiphysics simulation software, based on the finite element method.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 3","pages":"Article 100120"},"PeriodicalIF":0.0,"publicationDate":"2024-07-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S277318392400020X/pdfft?md5=ed234df0ea998ce112ebc55e0b3b6931&pid=1-s2.0-S277318392400020X-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141607678","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Exploring the impact of anode material on X-ray photon fluence and characteristics: A Monte Carlo simulation study 探索阳极材料对 X 射线光子通量和特性的影响:蒙特卡罗模拟研究
Nuclear Analysis Pub Date : 2024-06-01 DOI: 10.1016/j.nucana.2024.100112
Hassan Ouhadda , Mustapha Zerfaoui , Karim Bahhous , Yassine Oulhouq , Abdessamad Didi , Abdeslem Rrhioua , Dikra Bakari
{"title":"Exploring the impact of anode material on X-ray photon fluence and characteristics: A Monte Carlo simulation study","authors":"Hassan Ouhadda ,&nbsp;Mustapha Zerfaoui ,&nbsp;Karim Bahhous ,&nbsp;Yassine Oulhouq ,&nbsp;Abdessamad Didi ,&nbsp;Abdeslem Rrhioua ,&nbsp;Dikra Bakari","doi":"10.1016/j.nucana.2024.100112","DOIUrl":"10.1016/j.nucana.2024.100112","url":null,"abstract":"<div><p>This study investigates the critical significance of anode material selection in defining the energy spectrum and properties of X-ray photons in medical physics applications. Using the GATE platform and Monte Carlo simulations, a direct relationship between anode material atomic number and photon fluence is demonstrated. As the atomic number increases from Z = 29 (Copper) to Z = 74 (Tungsten), photon fluence rises by 62 %, indicating a substantial impact on X-ray production. Furthermore, the X-ray spectrum is affected by this material-driven changes, revealing a noticeable shift towards higher energy values: the mean energy of the continuous spectrum rises from 46.97 keV for Copper to 49.0 keV for Tungsten. The thermal properties of the material affect the temperature increase at the focal point. Rhodium and Molybdenum have a higher temperature rise than Copper (Cu) and Tungsten (W), because Cu and W have a greater thermal diffusion compared to other materials. These findings underscore the significance of anode material choice in optimizing X-ray systems which may enhance diagnostic accuracy and efficiency in diverse applications.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 2","pages":"Article 100112"},"PeriodicalIF":0.0,"publicationDate":"2024-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000120/pdfft?md5=9a7db82a57fbdb3212adfe5d2e27cfe0&pid=1-s2.0-S2773183924000120-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141139792","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Simulating the impact of electron beam energy deposition on lead target temperature 模拟电子束能量沉积对铅靶温度的影响
Nuclear Analysis Pub Date : 2024-06-01 DOI: 10.1016/j.nucana.2024.100113
Walid Oueslati
{"title":"Simulating the impact of electron beam energy deposition on lead target temperature","authors":"Walid Oueslati","doi":"10.1016/j.nucana.2024.100113","DOIUrl":"https://doi.org/10.1016/j.nucana.2024.100113","url":null,"abstract":"<div><p>This study delves into the thermal dynamics induced by an electron beam sourced from the CIRCE III accelerator, focusing on a lead target previously employed at the National Centre for Nuclear Science and Technology (CNSTN) in Tunisia for neutron and photon production. Leveraging FLUKA software, we simulate the intricate interplay between electrons and the target surface, analyzing variations in deposited energy across different target thicknesses. Beyond elucidating the electron-target interaction, our investigation extends to predicting crucial parameters such as the maximum operational threshold and surface temperature distribution of the target. To achieve this, a computational model harnessing the finite volume method is employed, offering insights into the thermal response dynamics and paving the way for optimized operational protocols and target design refinements. Through this comprehensive analysis, we aim to advance the understanding of thermal phenomena in electron-target interactions, thereby bolstering the efficiency and safety of particle accelerator operations in diverse scientific applications.</p></div>","PeriodicalId":100965,"journal":{"name":"Nuclear Analysis","volume":"3 2","pages":"Article 100113"},"PeriodicalIF":0.0,"publicationDate":"2024-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773183924000132/pdfft?md5=649bffd1aa4b7288312b8b309793fef4&pid=1-s2.0-S2773183924000132-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141324561","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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