Biogeosciences discussions : (BGD)最新文献

{"title":"Influence of land use and occupation on the water quality of a\u0000microbasin in the southwestern Amazon","authors":"A. Mendonça, Josilena De Jesus Laureano, Daíse Da Silva Lopes, Lindolaine Machado de Sousa, T. Lima, Ana Lúcia Denardin da Rosa, B. M. Gomes, I. D. Costa, E. L. Nascimento","doi":"10.5194/BG-2020-485","DOIUrl":"https://doi.org/10.5194/BG-2020-485","url":null,"abstract":"Abstract. Water resource management in Brazil is constantly evolving, and greater knowledge about this resource allows better planning and more sustainable uses. In Brazil, the improvement of water resource management faces the difficulty of implementing the instruments of the National Water Resources Policy, such as classification of water bodies. Thus, to help improve the water management instruments in the country's northern region, the objective of the present study was to diagnose the influence of land use and occupation on the water quality of the Igarapé Nazaré microbasin. For this purpose, indirect methods of landscape analysis were applied based on the processing of remote sensing images in a GIS. For the water quality analysis, 10 collection points were selected in the watershed, with samples collected at each one in four periods (high water; HW/LW transition; low water; LW/HW transition). In the collected samples, 14 parameters were analyzed, namely: temperature, pH, electrical conductivity; turbidity; water transparency and depth; dissolved oxygen; chlorophyll a, ammonia, nitrite, nitrate, total phosphorus and dissolved phosphorus; total coliforms and E. coli. The spatial analysis showed that the microbasin has about 84 % anthropized territory, with emphasis on agriculture, and sources of pollution from industries, fish farming and domestic sewage. Parameter analyses showed high values of total phosphorus (0.005–27.55 mg.L−1), total coliforms (4,103–1,09,106 CFU) and E. coli (0–5.8,105 CFU), and low DO concentration (0.0–8.33 mg.L−1), below the official limit established in all periods analyzed The water quality of the Igarapé Nazaré microbasin was found to suffer strong anthropic interference, requiring improvement of the sanitary infrastructure of city of Ji-Paraná, for maintenance of the watershed in class 2.\u0000","PeriodicalId":89897,"journal":{"name":"Biogeosciences discussions : (BGD)","volume":" ","pages":"1-23"},"PeriodicalIF":0.0,"publicationDate":"2021-02-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"47773226","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Tritium activity concentration and behaviour in coastal\u0000regions of Fukushima in 2014","authors":"M. Aoyama, S. Charmasson, Y. Hamajima, C. Duffa, D. Tsumune, Y. Tateda","doi":"10.5194/BG-2021-10","DOIUrl":"https://doi.org/10.5194/BG-2021-10","url":null,"abstract":"Abstract. We observed 3H activity concentrations and the 137Cs activity concentrations during the SoSo 5 rivers cruise in 2014 and at the Tomioka port in 2014–2018. The 3H activity concentrations at coastal stations located close to the Fukushima coast ranged from 90 Bq m−3 to 175 Bq m−3, and decreased between 67 Bq m−3 to 83 Bq m−3 at the stations located 12–16 km from the coast. The 3H activity concentration at the estuaries and ports, except at 56 north canal of the FNPP1 site, are around 200–500 Bq m−3 and slightly lower than the 3H activity concentration of 500–600 Bq m−3 observed in the rivers. These gradients of the 3H activity concentrations in the coastal region might indicate the large effect of 3H flux through the rivers. On the other hand, the 3H activity concentration at 56N of the FNPP1 site was significantly high compared to the 3H activity concentration in surrounding waters both north and south of the FNPP1 site and in river waters. It should also be noted that the 3H activity concentrations were similar at the stations located both north and south of the FNPP1 site, while the 137Cs activity concentrations were lower at the stations north of the FNPP1 site and higher at the stations south of the FNPP1 site. This indicated that the major sources of 137Cs could be the FNPP1 site as the point source while the source of 3H should be more diffuse and linked to riverine inputs located north and south of the FNPP1 site. The 3H / 137Cs activity ratios in coastal waters were 1.2–2.2 as obtained via the slopes by standardised major axis regressions between the 3H activity concentration and the 137Cs activity concentration of SoSo samples and Tomioka Port observed in 2014–2018, which is significantly high compared to that of the released radionuclides derived from the FNPP1 site, which was 0.01 in 2011 just after the accident. The open-water 3H activity concentration contribution to coastal waters was estimated to be 67 ± 20 Bq m−3 and 66 ± 17 Bq m−3 as the intercepts also by standardised major axis regressions. These estimates are consistent with 50 Bq m−3 obtained at the Kuroshio region as the background levels of 3H activity concentration in open water. The 3H and 137Cs fluxes to the coastal region of Fukushima based on the open-water movement, freshwater flux from the rivers based on their respective catchment, and mean monthly precipitation were estimated. The largest 3H flux is the open-water inflow from the north of the FNPP1 site and it reaches 52 GBq day−1, while the rivers north of the FNPP1 site showed 3–5 GBq day−1 fluxes. We obtained a 3H flux as 1.9–4.5 GBq day−1 of 3H using the 3H activity concentration in the port, which is comparable with the fluxes obtained from the rivers located north of the FNPP1 site. While using 3H activity concentration at the 56 north canal of FNPP1, we obtained 28–86 GBq day−1 fluxes, which is one order of magnitude larger than those estimated using 3H activity concentration in the FNPP1 port. One ","PeriodicalId":89897,"journal":{"name":"Biogeosciences discussions : (BGD)","volume":"1 1","pages":"1-29"},"PeriodicalIF":0.0,"publicationDate":"2021-02-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"45829921","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Temporal patterns and biophysical controls on methane emissions\u0000from a small eutrophic reservoir: insights from two years of eddy\u0000covariance monitoring","authors":"Sarah Waldo, J. Beaulieu, W. Barnett, D. A. Balz, M. Vanni, T. Williamson, J. Walker","doi":"10.5194/BG-2021-36","DOIUrl":"https://doi.org/10.5194/BG-2021-36","url":null,"abstract":"Abstract. Waters impounded behind dams (i.e. reservoirs) are important sources of greenhouses gases, especially methane (CH4), but their contribution is not well constrained due to high spatial and temporal variability, limitations in monitoring methods to characterize hot spot and hot moment emissions, and the limited number of studies that investigate diurnal, seasonal, and interannual patterns in emissions. In this study, we investigate the temporal patterns and biophysical drivers of CH4 emissions from Acton Lake, a small eutrophic reservoir, using a combination of methods: eddy covariance monitoring, continuous warm-season ebullition measurements, spatial emission surveys, and measurements of key drivers of CH4 production and emission. We used an artificial neural network to gap-fill the eddy covariance time series and to explore the relative importance of biophysical drivers on the inter-annual timescale. Acton Lake had cumulative areal emission rates of 40.6 ± 5.9 and 71.4 ±  4.2 g CH4 m−2 in 2017 and 2018, respectively, or 97.4 ± 14 and 171 ± 10 Mg CH4 in 2017 and 2018 across the whole 2.4 km2 area of the lake. The main difference between years was a period of elevated emissions lasting less than two weeks in the spring of 2018, which contributed 17 % of the total annual emissions, and was likely due to favourable sediment temperature and algal carbon substrate availability in 2018 compared to 2017. CH4 emissions only displayed diurnal patterns 18.5 % of the monitoring period, suggesting that factors that do not follow a diurnal pattern (e.g. substrate availability) may be driving emissions. Combining spatially extensive measurements with temporally continuous monitoring enabled us to quantify aspects of the spatial and temporal variability in CH4 emission. We found that the relationships between CH4 emissions and sediment T depended on location within the reservoir and observed a clear spatio-temporal offset in maximum CH4 emissions as a function of reservoir depth. These findings suggest a strong spatial pattern in CH4 biogeochemistry within this relatively small (2.4 km2) reservoir. In addressing the need for a better understanding of GHG emissions from reservoirs, there is a trade-off in intensive measurement of one water body versus short-term and/or spatially limited measurements in many water bodies. The insights from multi-year, continuous, spatially extensive studies like this one can be used to inform both the study design and emission upscaling from spatially or temporally limited results, specifically the importance of trophic status and intra-lake variability in assumptions about upscaling CH4 emissions.","PeriodicalId":89897,"journal":{"name":"Biogeosciences discussions : (BGD)","volume":"1 1","pages":"1-40"},"PeriodicalIF":0.0,"publicationDate":"2021-02-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"46153964","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Drought effects on leaf fall, leaf flushing and stem growth in\u0000Neotropical forest; reconciling remote sensing data and field\u0000observations","authors":"T. Janssen, Y. van der Velde, F. Hofhansl, S. Luyssaert, K. Naudts, B. Driessen, K. Fleischer, H. Dolman","doi":"10.5194/BG-2021-30","DOIUrl":"https://doi.org/10.5194/BG-2021-30","url":null,"abstract":"Abstract. Large amounts of carbon flow through tropical ecosystems every year, from which a part is sequestered in biomass through tree growth. However, the effects of ongoing warming and drying on tree growth and carbon sequestration in tropical forest is still highly uncertain. Field observations are sparse and limited to a few sites while remote sensing analysis shows diverging growth responses to past droughts that cannot be interpreted with confidence. To reconcile data from field observations and remote sensing, we collated in situ measurements of stem growth and leaf litterfall from inventory plots across the Neotropics. This data was used to train two machine learning models and to evaluate model performance on reproducing stem growth and litterfall rates. The models utilized multiple climatological variables and other geospatial datasets as explanatory variables. The output consisted of monthly estimates of leaf litterfall (R2 = 0.67, NRMSE = 9.5 %) and stem growth (R2 = 0.51, NRMSE = 11.2 %) across the neotropics from 1982 to 2019 at a high spatial resolution (0.1°). Modelled time series allowed to assess the impacts of the 2005 and 2015 droughts in the Amazon basin on regional scales. Both droughts were estimated to have caused widespread declines in stem growth (−0.6σ ~ −1.8σ), coinciding with enhanced leaf fall (+0.7σ ~ +0.9σ). Regions in the Amazon basin that flushed leaves at the onset of both droughts (+1.1σ ~ +1.9σ), showed positive anomalies in remotely sensed enhanced vegetation index, while sun-induced fluorescence and vegetation optical depth were reduced. The previously observed counterintuitive response of canopy green-up during drought in the Amazon basin detected by many remote sensing analyses can therefore be explained by enhanced leaf flushing at the onset of a drought. The long-term estimates of leaf litterfall and stem growth point to a decline of stem growth and a simultaneous but weaker increase in leaf litterfall in the Amazon basin since 1982 that is not observed in long-term inventory plots. These trends are associated with increased warming and drying of the Amazonian climate.\u0000","PeriodicalId":89897,"journal":{"name":"Biogeosciences discussions : (BGD)","volume":" ","pages":"1-41"},"PeriodicalIF":0.0,"publicationDate":"2021-02-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"48436084","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Changes in population depth distribution and oxygen stratification are involved in the current low condition of the eastern Baltic Sea cod (Gadus morhua)","authors":"M. Casini, Martin Hansson, Alessandro Orio, K. Limburg","doi":"10.5194/BG-18-1321-2021","DOIUrl":"https://doi.org/10.5194/BG-18-1321-2021","url":null,"abstract":"Abstract. During the past twenty years, hypoxic areas have expanded exponentially in the Baltic Sea, which has become one of the largest marine dead zones in the world. At the same time, the most important commercial fish population of the region, the Eastern Baltic cod, has experienced a drastic reduction in mean body condition, but the processes relating hypoxia to condition remain elusive. Here we use extensive long-term monitoring data on cod biology and distribution as well as on hydrological variations, to investigate the processes that relate deoxygenation and cod condition during the autumn season. Our results show that the depth distribution of cod has increased during the past four decades at the same time of the expansion, and shallowing, of the waters with an oxygen concentration known to be detrimental for cod performance. This has resulted in a spatial overlap between the cod population and low-oxygenated waters after the mid-1990s, which relates with the observed decline in cod mean body condition. Complementary analyses on fish otolith microchemistry also revealed that since the mid-1990s, cod individuals with low condition were indeed exposed to low-oxygen waters during their life. This study helps to shed light on the processes that have led to a decline of the Eastern Baltic cod body condition, which can aid the management of this population currently in distress. Further studies should focus on understanding why the cod population has moved to deeper waters in autumn and on analysing the overlap with low-oxygen waters in other seasons to quantify the potential effects of the variations in physical properties on cod biology throughout the year.","PeriodicalId":89897,"journal":{"name":"Biogeosciences discussions : (BGD)","volume":"18 1","pages":"1321-1331"},"PeriodicalIF":0.0,"publicationDate":"2021-02-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"45244549","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Response of tropical marine benthic diatoms exposed to elevated\u0000irradiance and temperature","authors":"Sazlina Salleh, A. McMinn","doi":"10.5194/BG-2021-18","DOIUrl":"https://doi.org/10.5194/BG-2021-18","url":null,"abstract":"Abstract. Shallow tropical marine environments are likely to experience future water temperatures that will challenge the ability of life to survive. Changes in temperature and irradiance during tidal cycles in the Tanjung Rhu estuary, Langkawi, Malaysia in 2007 did not significantly affect the benthic diatom communities, although, higher photosynthetic parameters, such as maximum relative electron transport rate (rETRmax), photosynthetic efficiency (α), maximum quantum yield (Fv/Fm) and effective quantum yield (∆F/Fm'), were recorded at high tide when the temperatures were lower. However, when benthic diatoms were experimentally exposed to irradiances of 1800 µmol photons m−2 s−1, they were only able to photosynthesize at temperatures","PeriodicalId":89897,"journal":{"name":"Biogeosciences discussions : (BGD)","volume":" ","pages":"1-25"},"PeriodicalIF":0.0,"publicationDate":"2021-02-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"41680454","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Anthropogenic CO2-mediated freshwater acidification limits survival,\u0000calcification, metabolism, and behaviour in stress-tolerant freshwater\u0000crustaceans","authors":"A. Quijada-Rodriguez, Pou-Long Kuan, Po-Hsuan Sung, Mao-Ting Hsu, G. J. Allen, P. Hwang, Yung‐Che Tseng, D. Weihrauch","doi":"10.5194/BG-2021-34","DOIUrl":"https://doi.org/10.5194/BG-2021-34","url":null,"abstract":"Abstract. Dissolution of anthropogenic CO2 is chronically acidifying aquatic ecosystems. Studies indicate that ocean acidification will cause marine life, especially calcifying species, to suffer at the organismal and ecosystem levels. In comparison, freshwater acidification has received less attention rendering its consequences unclear. Here, juvenile Chinese mitten crabs, Eriocheir sinensis, were used as a calcifying model to investigate the impacts of CO2-mediated freshwater acidification. Our integrative approach investigating changes in the animal's acid-base homeostasis, metabolism, calcification, locomotory behaviour, and survival rate indicate that the crab will face energetic consequences from future freshwater acidification. These energetic trade-offs allow the animal to maintain its acid-base homeostasis at the cost of reduced metabolic activity, exoskeletal calcification, and locomotion reducing the animal's overall fitness and increasing its mortality. Results suggest that present-day calcifying invertebrates could be heavily affected by freshwater acidification similar to their marine organisms and emphasizes the importance in understanding the long-term implications of freshwater acidification on species fitness.\u0000","PeriodicalId":89897,"journal":{"name":"Biogeosciences discussions : (BGD)","volume":" ","pages":"1-21"},"PeriodicalIF":0.0,"publicationDate":"2021-02-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"48716003","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Blue Carbon Stocks and Exchanges Along the Pacific West Coast","authors":"M. Ward, T. Hill, C. Souza, Tessa Filipczyk, A. Ricart, Sarah Merolla, L. Capece, B. O’Donnell, K. Elsmore, W. Oechel, Kathryn M. Beheshti","doi":"10.5194/BG-2021-27","DOIUrl":"https://doi.org/10.5194/BG-2021-27","url":null,"abstract":"Abstract. Salt marshes and seagrass meadows can sequester and store high quantities of organic carbon (OC) in their sediments relative to other marine and terrestrial habitats. Assessing carbon stocks, carbon sources, and the transfer of carbon between habitats within coastal seascapes are each integral in identifying the role of blue carbon habitats in coastal carbon cycling. Here, we quantified carbon stocks, sources, and exchanges in seagrass meadows, salt marshes, and unvegetated sediments in six bays along the Pacific coast of California. The salt marshes studied here contained approximately twice as much OC as did seagrass meadows, 23.51 ± 1.77 kg OC m−3 compared to 11.01 ± 1.18 kg OC m−3, respectively. Both seagrass and salt marsh sediment carbon stocks were higher than previous estimates from this region but lower than global and U.S.-wide averages, respectively. Seagrass-derived carbon was deposited annually into adjacent marshes during fall seagrass senescence. However, isotope mixing models estimate that negligible amounts of this seagrass material were ultimately buried in underlying sediment. Rather, the vast majority of OC in sediment across sites was likely derived from planktonic/benthic diatoms and C3 salt marsh plants.","PeriodicalId":89897,"journal":{"name":"Biogeosciences discussions : (BGD)","volume":" ","pages":"1-36"},"PeriodicalIF":0.0,"publicationDate":"2021-02-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"47165952","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Weekly reconstruction of pH and total alkalinity in an upwelling-dominated coastal ecosystem through neural networks (ATpH-NN): The case of Ría de Vigo (NW Spain) \u0000between 1992 and 2019","authors":"Daniel Broullón, F. F. Pérèz, M. D. Doval","doi":"10.5194/BG-2021-33","DOIUrl":"https://doi.org/10.5194/BG-2021-33","url":null,"abstract":"Abstract. Short and long-term variability of seawater carbon dioxide (CO2) system shows large differences between different ecosystems which are derived from the characteristic processes of each area. The high variability of coastal ecosystems, their ecological and economic significance, the anthropogenic influence on them and their behavior as sources or sinks of atmospheric CO2, highlight the relevance to better understand the processes that underlie the variability and the alterations of the CO2 system at different spatiotemporal scales. To confidently achieve this purpose, it is necessary to have high-frequency data sustained over several years in different regions. In this work, we contribute to this need by configuring and training two neural networks with the capacity to model the weekly variability of pH and total alkalinity (AT) in the upper 50 m of the water column of the Ria de Vigo (NW Spain), with an error of 0.031 pH units and 10.9 µmol kg−1 respectively. With these networks, we generated weekly time series of pH and AT in seven locations of the Ria de Vigo in three depth ranges (0–5 m, 5–10 m and 10–15 m), which adequately represent independent discrete measurements. In a first analysis of the time series, a high short-term variability is observed, being larger for the inner stations of the Ria de Vigo. The lowest values of pH and AT were obtained for the inner zone, showing a progressive increase towards the outer/middle zone of the ria. The mean seasonal cycle also reflects the gradient between both zones, with a larger amplitude and variability for both variables in the inner zone. On the other hand, the long-term trends derived from the time series of pH show a higher acidification than that obtained for the open ocean, with surface trends ranging from −0.020 pH units per year in the outer/middle zone to −0.032 pH units per year in the inner zone. In addition, positive long-term trends of AT were obtained ranging from 0.39 µmol kg−1 per year in the outer/middle zone to 2.86 µmol kg−1 per year in the inner zone. The results presented in this study show the changing conditions both in the short and long-term variability as well as the spatial differentiation between the inner and outer/middle zone to which the organisms of the Ria de Vigo are subjected. The neural networks and the database provided in this study offer the opportunity to evaluate the CO2 system in an environment of high ecological and economic relevance, to validate high-resolution regional biogeochemical models and to evaluate the impacts on organisms of the Ria de Vigo by refining the ranges of the biogeochemical variables included in experiments.","PeriodicalId":89897,"journal":{"name":"Biogeosciences discussions : (BGD)","volume":" ","pages":"1-36"},"PeriodicalIF":0.0,"publicationDate":"2021-02-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"44029893","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}

{"title":"Impact of typhoons on particulate and dissolved 137Cs activities in seawater off the Fukushima Prefecture: results from the SOSO 5 Rivers cruise (October 2014)","authors":"M. Aoyama, S. Charmasson, Y. Hamajima, C. Duffa","doi":"10.5194/BG-2020-491","DOIUrl":"https://doi.org/10.5194/BG-2020-491","url":null,"abstract":"Abstract. Cruise SoSo 5 Rivers took place during October 2014 off the coast of Fukushima Prefecture shortly after the passage of two typhoons. Detection of dissolved 134Cs and 137Cs in all samples reflected contamination caused by accidental releases of radiocaesium from the Fukushima Dai-ichi Nuclear power plant (FNPP1) accident. The dissolved activities were generally higher at coastal sites and decreased with distance from shore, and they were higher in the surface than in the bottom water. The tendency of 137Cs activities to decrease with distance from the coast reflected mixing of coastal water and open-ocean water of which 137Cs activity concentration was ~1.5 Bq m−3. At stations very close to the coast, we observed high particulate 137Cs activity concentration that exceeded dissolved 137Cs activity concentration. 137Cs activities were generally 1–2 orders of magnitudes lower in organic particles than in dissolved form, and the ratios of 137Cs activity concentration in organic particles to 137Cs activity concentration in dissolved form ranged from 0.01 ± 0.00 to 0.12 ± 0.01. The ratio of 137Cs to 134Cs activity concentrations in organic particles did not change with distance from shore or with 137Cs activity concentration and generally remained around 1, even in samples collected far from the coast. This pattern indicated that the organic particles had come from rivers or a source very close to the coast. The 137Cs / 134Cs activity ratio in dissolved form north of FNPP1 region was estimated to be 1.074 ± 0.015, a ratio that is in good agreement with the 137Cs / 134Cs activity ratio in the core of Unit 1 of the FNPP1 while the 137Cs / 134Cs activity ratio at Tomioka port which located south of FNPP1 was 0.998 ± 0.017. Therefore we can conclude the source of radiocaesium in seawater in the coastal region north of FNPP1 was deposited radiocaesium released from the core of Unit 1 of FNPP1, while the source of radiocaesium observed in the coastal region south of FNPP1 was a mixture of deposited radiocaesium released from the core of Unit 2 and the core of Unit 1 of FNPP1. During September–October of each year, the typhoon season in Japan, the 137Cs activity concentration generally increased at Ukedo port, Tomioka port, FNPP1, and Iwasawa beach, and showed a good relationship with the 7-day modified antecedent precipitation index (API) while there is less correlation between the modified API and 137Cs activity concentration near the outlet of canal from unit 5 and 6 of FNPP1 to the sea.","PeriodicalId":89897,"journal":{"name":"Biogeosciences discussions : (BGD)","volume":"1 1","pages":"1-33"},"PeriodicalIF":0.0,"publicationDate":"2021-02-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"41856225","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}