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Projectile Coherence Effects in Twisted Electron Ionization of Helium 氦扭曲电子电离中的抛射相干效应
IF 1.8
Atoms Pub Date : 2023-05-03 DOI: 10.3390/atoms11050079
A. Harris
{"title":"Projectile Coherence Effects in Twisted Electron Ionization of Helium","authors":"A. Harris","doi":"10.3390/atoms11050079","DOIUrl":"https://doi.org/10.3390/atoms11050079","url":null,"abstract":"Over the last decade, it has become clear that for heavy ion projectiles, the projectile’s transverse coherence length must be considered in theoretical models. While traditional scattering theory often assumes that the projectile has an infinite coherence length, many studies have demonstrated that the effect of projectile coherence cannot be ignored, even when the projectile-target interaction is within the perturbative regime. This has led to a surge in studies that examine the effects of the projectile’s coherence length. Heavy-ion collisions are particularly well-suited to this because the projectile’s momentum can be large, leading to a small deBroglie wavelength. In contrast, electron projectiles that have larger deBroglie wavelengths and coherence effects can usually be safely ignored. However, the recent demonstration of sculpted electron wave packets opens the door to studying projectile coherence effects in electron-impact collisions. We report here theoretical triple differential cross-sections (TDCSs) for the electron-impact ionization of helium using Bessel and Laguerre-Gauss projectiles. We show that the projectile’s transverse coherence length affects the shape and magnitude of the TDCSs and that the atomic target’s position within the projectile beam plays a significant role in the probability of ionization. We also demonstrate that projectiles with large coherence lengths result in cross-sections that more closely resemble their fully coherent counterparts.","PeriodicalId":8629,"journal":{"name":"Atoms","volume":null,"pages":null},"PeriodicalIF":1.8,"publicationDate":"2023-05-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"45786518","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Enhanced Acetone Sensing Based on Group-11 Metal (Cu, Ag, and Au) Nanoparticles Embedded in Graphitic Carbon Nitride (gCN) 基于嵌入石墨氮化碳(gCN)的11族金属(Cu、Ag和Au)纳米粒子的增强丙酮传感
IF 1.8
Atoms Pub Date : 2023-05-01 DOI: 10.3390/atoms11050078
Nihal, R. Sharma, Navjot Kaur, Mamta Sharma, B. Choudhary, J. Goswamy
{"title":"Enhanced Acetone Sensing Based on Group-11 Metal (Cu, Ag, and Au) Nanoparticles Embedded in Graphitic Carbon Nitride (gCN)","authors":"Nihal, R. Sharma, Navjot Kaur, Mamta Sharma, B. Choudhary, J. Goswamy","doi":"10.3390/atoms11050078","DOIUrl":"https://doi.org/10.3390/atoms11050078","url":null,"abstract":"In this work, a group-11 metal nanoparticle-embedded, graphitic carbon nitride-based, resistive-type sensor was developed for room temperature acetone sensing. We synthesized pure and group-11 transition metal (Cu, Ag and Au) nanoparticles embedded in graphitic carbon nitride (gCN) by thermal polycondensation and chemical reduction methods. The synthesized material was characterized using UV/visspectroscopy, FTIRspectroscopy, XRD, HRTEM, FESEM, and EDS techniques. Sensing properties such as response, response/recovery time, selectivity, and stability were calculated. This study confirms that Ag/gCN is the best material for room temperature sensing of acetone compared to Cu/gCN, Au/gCN, and pure gCN. The response of Ag/gCN for 20 ppm acetone at room temperature is 28%. The response/recovery time is 42.05/37.09 s. Moreover, the response of Ag/gCN is stable for 10 days.","PeriodicalId":8629,"journal":{"name":"Atoms","volume":null,"pages":null},"PeriodicalIF":1.8,"publicationDate":"2023-05-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"47417866","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Fragmentation Dynamics of CO2q+ (q = 2, 3) in Collisions with 1 MeV Proton CO2q+(q=2,3)与1MeV质子碰撞的碎裂动力学
IF 1.8
Atoms Pub Date : 2023-04-23 DOI: 10.3390/atoms11050075
Avijit Duley, A. Kelkar
{"title":"Fragmentation Dynamics of CO2q+ (q = 2, 3) in Collisions with 1 MeV Proton","authors":"Avijit Duley, A. Kelkar","doi":"10.3390/atoms11050075","DOIUrl":"https://doi.org/10.3390/atoms11050075","url":null,"abstract":"The fragmentation dynamics of the CO2q+ (q = 2, 3) molecular ions formed under the impact of 1 MeV protons is studied using a recoil ion momentum spectrometer equipped with a multi-hit time- and position-sensitive detector. Both two-body and three-body fragmentation channels arising from the doubly and triply ionized molecular ions of CO2 are identified and analyzed. Kinetic energy release (KER) distributions have been obtained for various channels. With the help of Dalitz plots and Newton diagrams concerted and sequential processes have been assigned to observed fragmentation channels. In addition, angular correlations are used to determine the molecular geometry of the precursor molecular ion. It is found that the symmetric breakup into C+ + O+ + O+ involves asymmetric stretching of the molecular bonds in CO23+ prior to dissociation via concerted decay implying the fact that collisions with 1 MeV proton induces an asynchronous decay in CO2.","PeriodicalId":8629,"journal":{"name":"Atoms","volume":null,"pages":null},"PeriodicalIF":1.8,"publicationDate":"2023-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"48674463","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Theoretical Investigation of Electron–Ion Recombination Process of Mg-like Gold 类镁金电子-离子复合过程的理论研究
IF 1.8
Atoms Pub Date : 2023-04-23 DOI: 10.3390/atoms11050076
L. Xie, Wenliang He, Shengbo Niu, J. Rui, Yulong Ma, C. Dong
{"title":"Theoretical Investigation of Electron–Ion Recombination Process of Mg-like Gold","authors":"L. Xie, Wenliang He, Shengbo Niu, J. Rui, Yulong Ma, C. Dong","doi":"10.3390/atoms11050076","DOIUrl":"https://doi.org/10.3390/atoms11050076","url":null,"abstract":"The L-shell dielectronic and trielectronic recombinations of highly charged Mg-like gold ions (Au67+) in the ground state 2s22p63s2 1S0 have been studied systematically. The recombination cross-sections and rate coefficients are carefully calculated for ∆n = 1 (2s/2p → 3l) transitions using a flexible atomic code based on the relativistic configuration interaction method and considering the Breit and QED corrections. Detailed resonance energies and resonance strengths are presented for the stronger resonances of the LMn (n = 3–12) series. It is found that the contributions of the trielectronic recombination to the total cross-section is about 13.75%, which cannot be neglected. For convenience of application, the plasma rate coefficients are also calculated and fitted to a semiempirical formula, and in the calculations, the contributions from the higher excited resonance groups n ≥ 13 are evaluated by an extrapolation method, which is about 2.93% of the total rate coefficient.","PeriodicalId":8629,"journal":{"name":"Atoms","volume":null,"pages":null},"PeriodicalIF":1.8,"publicationDate":"2023-04-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"46721824","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Signatures of Quantum Chaos of Rydberg-Dressed Bosons in a Triple-Well Potential 三阱势中rydberg修饰玻色子的量子混沌特征
IF 1.8
Atoms Pub Date : 2023-04-19 DOI: 10.3390/atoms11060089
T. Yan, M. Collins, R. Nath, Weibin Li
{"title":"Signatures of Quantum Chaos of Rydberg-Dressed Bosons in a Triple-Well Potential","authors":"T. Yan, M. Collins, R. Nath, Weibin Li","doi":"10.3390/atoms11060089","DOIUrl":"https://doi.org/10.3390/atoms11060089","url":null,"abstract":"We studied signatures of quantum chaos in dynamics of Rydberg-dressed bosonic atoms held in a one-dimensional triple-well potential. Long-range nearest-neighbor and next-nearest-neighbor interactions, induced by laser dressing atoms to strongly interacting Rydberg states, drastically affect mean-field and quantum many-body dynamics. By analyzing the mean-field dynamics, classical chaos regions with positive and large Lyapunov exponents were identified as a function of the potential well tilting and dressed interactions. In the quantum regime, it was found that level statistics of the eigen-energies gain a Wigner–Dyson distribution when the Lyapunov exponents are large, giving rise to signatures of strong quantum chaos. We found that both the time-averaged entanglement entropy and survival probability of the initial state have distinctively large values in the quantum chaos regime. We further showed that population variances could be used as an indicator of the emergence of quantum chaos. This might provide a way to directly probe quantum chaotic dynamics through analyzing population dynamics in individual potential wells.","PeriodicalId":8629,"journal":{"name":"Atoms","volume":null,"pages":null},"PeriodicalIF":1.8,"publicationDate":"2023-04-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"49102922","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Rydberg Interaction-Induced Distortion of the Autler–Townes Spectra in Cold Lithium Atoms 冷锂原子中奥德勒-汤光谱的Rydberg相互作用诱导畸变
IF 1.8
Atoms Pub Date : 2023-04-13 DOI: 10.3390/atoms11040073
S. Saakyan, N. Morozov, V. Sautenkov, B. Zelener
{"title":"Rydberg Interaction-Induced Distortion of the Autler–Townes Spectra in Cold Lithium Atoms","authors":"S. Saakyan, N. Morozov, V. Sautenkov, B. Zelener","doi":"10.3390/atoms11040073","DOIUrl":"https://doi.org/10.3390/atoms11040073","url":null,"abstract":"In this article, effects of the strong long-range interaction of Rydberg atoms on the Autler–Townes splitting spectrum are investigated. Preliminary results are obtained for various excitation times and Rydberg atom densities. The 2S1/2 and 2P1/2 levels of lithium-7 are coupled with strong laser field and probed by another laser via excitation into a 70S Rydberg level. Interactions between Rydberg atoms excited by the probe beam lead to the broadening of the Autler–Townes spectra. At high concentrations of Rydberg atoms, a suppression of the excitation of the Autler–Townes peak at red detuning is observed.","PeriodicalId":8629,"journal":{"name":"Atoms","volume":null,"pages":null},"PeriodicalIF":1.8,"publicationDate":"2023-04-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"41927970","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Temporal Response of Atoms Trapped in an Optical Dipole Trap: A Primer on Quantum Computing Speed 被困在光偶极子阱中的原子的时间响应:量子计算速度入门
IF 1.8
Atoms Pub Date : 2023-04-10 DOI: 10.3390/atoms11040072
S. Baral, R. Easwaran, J. José, Aarthi Ganesan, P. Deshmukh
{"title":"Temporal Response of Atoms Trapped in an Optical Dipole Trap: A Primer on Quantum Computing Speed","authors":"S. Baral, R. Easwaran, J. José, Aarthi Ganesan, P. Deshmukh","doi":"10.3390/atoms11040072","DOIUrl":"https://doi.org/10.3390/atoms11040072","url":null,"abstract":"An atom confined in an optical dipole trap is a promising candidate for a qubit. Analyzing the temporal response of such trapped atoms enables us to estimate the speed at which quantum computers operate. The present work models an atom in an optical dipole trap formed using crossed laser beams and further examines the photoionization time delay from such confined atoms. We study noble gas atoms, such as Ne (Z = 10), Ar (Z = 18), Kr (Z = 36), and Xe (Z = 54). The atoms are considered to be confined in an optical dipole trap using X-ray Free Electron Lasers (XFEL). The present work shows that the photoionization time delay of the trapped atoms is different compared with that of the free atoms. This analysis alerts us that while talking about the speed of quantum computing, the temporal response of the atoms in the trapped environment must also be accounted for.","PeriodicalId":8629,"journal":{"name":"Atoms","volume":null,"pages":null},"PeriodicalIF":1.8,"publicationDate":"2023-04-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"46276957","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Indigenisation of the Quantum Clock: An Indispensable Tool for Modern Technologies 量子钟的本土化:现代技术不可或缺的工具
IF 1.8
Atoms Pub Date : 2023-04-10 DOI: 10.3390/atoms11040071
S. De, Arijit Sharma
{"title":"Indigenisation of the Quantum Clock: An Indispensable Tool for Modern Technologies","authors":"S. De, Arijit Sharma","doi":"10.3390/atoms11040071","DOIUrl":"https://doi.org/10.3390/atoms11040071","url":null,"abstract":"Time and frequency (T&F) measurement with unprecedented accuracy is the backbone for several sophisticated technologies, commensurate with the evolution of human civilisation in the 20th century in terms of communication, positioning, navigation, and precision timing. This necessity drove researchers in the early 1950s to build atomic clocks that have now evolved to a state-of-the-art level, operating at optical wavelengths as optical atomic clocks, which use cold and trapped samples of atomic/ionic species and various other sophisticated diagnostic test techniques. Such ultrahigh-precision accurate clocks have made it possible to probe fundamental aspects of science through incredibly sensitive measurements. On the other hand, they meet the T&F synchronisation standards for classical and emerging quantum technologies at the desired level of accuracy. Considering the impact of optical atomic clocks in the second quantum revolution (quantum 2.0), they have been identified as an indispensable critical technology in worldwide quantum missions, including in India. This article reviews the present international scenario regarding optical atomic clocks and their related technologies and draws a roadmap for their indigenisation over the next decade.","PeriodicalId":8629,"journal":{"name":"Atoms","volume":null,"pages":null},"PeriodicalIF":1.8,"publicationDate":"2023-04-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"46672806","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Fine-Tuning of Atomic Energies in Relativistic Multiconfiguration Calculations 相对论多重组态计算中原子能的精细调谐
IF 1.8
Atoms Pub Date : 2023-04-08 DOI: 10.3390/atoms11040070
Yanting Li, G. Gaigalas, Wenxian Li, Chongyang Chen, P. Jönsson
{"title":"Fine-Tuning of Atomic Energies in Relativistic Multiconfiguration Calculations","authors":"Yanting Li, G. Gaigalas, Wenxian Li, Chongyang Chen, P. Jönsson","doi":"10.3390/atoms11040070","DOIUrl":"https://doi.org/10.3390/atoms11040070","url":null,"abstract":"Ab initio calculations sometimes do not reproduce the experimentally observed energy separations at a high enough accuracy. Fine-tuning of diagonal elements of the Hamiltonian matrix is a process which seeks to ensure that calculated energy separations of the states that mix are in agreement with experiment. The process gives more accurate measures of the mixing than can be obtained in ab initio calculations. Fine-tuning requires the Hamiltonian matrix to be diagonally dominant, which is generally not the case for calculations based on jj-coupled configuration state functions. We show that this problem can be circumvented by a method that transforms the Hamiltonian in jj-coupling to a Hamiltonian in LSJ-coupling for which fine-tuning applies. The fine-tuned matrix is then transformed back to a Hamiltonian in jj-coupling. The implementation of the method into the General Relativistic Atomic Structure Package is described and test runs to validate the program operations are reported. The new method is applied to the computation of the 2s21S0−2s2p1,3P1 transitions in C III and to the computation of Rydberg transitions in B I, for which the 2s2p22S1/2 perturber enters the 2s2ns2S1/2 series. Improved convergence patterns and results are found compared with ab initio calculations.","PeriodicalId":8629,"journal":{"name":"Atoms","volume":null,"pages":null},"PeriodicalIF":1.8,"publicationDate":"2023-04-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"44754334","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Resonance States of Negative Hydrogen-like Ions in Quantum Plasmas 负类氢离子在量子等离子体中的共振态
IF 1.8
Atoms Pub Date : 2023-04-07 DOI: 10.3390/atoms11040069
Suya Yao, Zishi Jiang, S. Kar
{"title":"Resonance States of Negative Hydrogen-like Ions in Quantum Plasmas","authors":"Suya Yao, Zishi Jiang, S. Kar","doi":"10.3390/atoms11040069","DOIUrl":"https://doi.org/10.3390/atoms11040069","url":null,"abstract":"We studied the 1Se and 1,3Po resonance states of negative hydrogen-like ions immersed in quantum plasmas. The exponential cosine screened Coulomb potential was considered to model the quantum plasma environment. The correlated exponential wave functions in which the exponents were generated by a pseudo-random technique were applied to represent the correlation effects between the charged particles. The stabilization method was used to calculate the resonance parameters (position and width). The resonance parameters (position and width) for Ps−, Mμ−, π−, 1H−, D−, T− and ∞H− embedded in quantum plasmas are reported for various screening parameters. The 1Se resonance parameters for Mμ−, π−, 1H−, D−, T− ions and 1,3 Po states for Ps−, Mμ−, π−, 1H−, D−, T− and ∞H− of the proposed systems are reported for the first time in the literature.","PeriodicalId":8629,"journal":{"name":"Atoms","volume":null,"pages":null},"PeriodicalIF":1.8,"publicationDate":"2023-04-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"43785773","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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