Aerosol and Air Quality Research最新文献

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Effects of Precipitation on the Air Quality Index, PM2.5 Levels and on the Dry Deposition of PCDD/Fs in the Ambient Air 降水对空气质量指数、PM2.5水平及环境空气中PCDD/Fs干沉降的影响
IF 4 4区 环境科学与生态学
Aerosol and Air Quality Research Pub Date : 2023-01-01 DOI: 10.4209/aaqr.220417
Ruoxin Wang, Kangping Cui, Hwey-Lin Sheu, Lin-Chi Wang, Xueyan Liu
{"title":"Effects of Precipitation on the Air Quality Index, PM2.5 Levels and on the Dry Deposition of PCDD/Fs in the Ambient Air","authors":"Ruoxin Wang, Kangping Cui, Hwey-Lin Sheu, Lin-Chi Wang, Xueyan Liu","doi":"10.4209/aaqr.220417","DOIUrl":"https://doi.org/10.4209/aaqr.220417","url":null,"abstract":"The effects of 9 precipitation events in Suzhou City in Anhui Province, China, on the air quality index (AQI), PM2.5, and dry deposition flux of PCDD/Fs (polydibenzo-p-dioxins and polydibenzofurans) were investigated. A total of 7 precipitation events were positive contributes to the reduction of AQI;among them, the AQI were between 23 and 216, with an average of 75, the PM2.5 concentrations were between 5.0 and 169 mu g m-3, with an average of 25 mu g m-3, while the total-PCDD/F-TEQ dry deposition flux ranged from 149 to 1034 pg WHO2005-TEQ m-2 day-1 and averaged 315 pg WHO2005-TEQ m-2 day-1. By comparing the average AQI and PM2.5, respectively, during and after rainfall with that before rainfall, the results indicated that the average reduction fractions of AQI were 26% and 44%, respectively, while those of PM2.5 were 58% and 43%. In addition, the effect of precipitation on the average reduction fraction of total PCDD/F-TEQ dry deposition flux was 31%. However, in the other 2 AQI elevation events, the AQI were between 23 and 100, and averaged 51;when comparing the average AQI and PM2.5 concentrations, during and after the rain with that before the rain, the increases in AQI were 42% and 49%, respectively, while the increases in PM2.5 concentration were 26% and 29%, respectively. The above results show that, on the whole, rain and snow improved the air quality. This is because rainwater removes particles or dissolved gaseous pollutants from the atmosphere and brings aerosols to the ground. However, in some cases, the increase of source emissions and atmospheric vertical convection, the effect of precipitation or air humidity increased the AQI and elevated the concentration of PM2.5, and dry deposition flux of PCDD/Fs. The results of this study provide useful information for both scientific communities and air quality management.","PeriodicalId":7402,"journal":{"name":"Aerosol and Air Quality Research","volume":"1 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"70295300","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Multisite Scenarios of Black Carbon and Biomass Burning Aerosol Characteristics in India 印度炭黑和生物质燃烧气溶胶特征的多站点情景
IF 4 4区 环境科学与生态学
Aerosol and Air Quality Research Pub Date : 2023-01-01 DOI: 10.4209/aaqr.220435
Vivek Kumar, P. Devara, V. Soni
{"title":"Multisite Scenarios of Black Carbon and Biomass Burning Aerosol Characteristics in India","authors":"Vivek Kumar, P. Devara, V. Soni","doi":"10.4209/aaqr.220435","DOIUrl":"https://doi.org/10.4209/aaqr.220435","url":null,"abstract":"Black Carbon (BC) aerosols are not only substantial climate-forcing drivers but also impact human health. The spatial distribution of BC aerosols depends on the combination of anthropogenic activities and meteorological conditions. In this study, we used the India Meteorological Department (IMD) Black Carbon Observational Network datasets to assess the diurnal, seasonal, and long-term BC trends for the period, 2016–2021. The majority of the IMD’s BC monitoring stations show an overall declining trend in the BC mass concentration during the study period in India. Maximum BC concentrations are observed in the post-monsoon and winter seasons due to the stubble-burning activity and lower values of Atmospheric Boundary Layer Height (ABLH). Minimum concentrations are observed at all stations in the monsoon season due to the wet scavenging of aerosols by rain. There is a clear decrease in the BC mass concentration from winter to monsoon months and an increase in the post-monsoon months. Regional emissions from crop residue burning in the post-harvesting seasons are the main contributing factor for extremely high levels of BC mass concentration. Low wind speed and shallow mixed layer were found to be the main reasons for high levels of aerosol concentration during the winter season. There is an increasing trend in Biomass Burning (BB) at most of the stations except for Thiruvananthapuram, where a prominent decreasing trend in BC concentration is also noticed. In the present study, the impact of local meteorological parameters such as wind, temperature, rainfall and Atmospheric Boundary Layer Height on BC mass concentration is investigated. The results show a negative correlation with rainfall, relative humidity, wind speed, temperature and ABL height. Both local activity and long-range transport at each study site are also found to be responsible for the significant changes in BC mass concentration.","PeriodicalId":7402,"journal":{"name":"Aerosol and Air Quality Research","volume":"1 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"70295825","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Impact of the Contamination Method on the Disinfection of N95 Respirators: Drops versus Aerosols 污染方法对N95口罩消毒的影响:滴剂与气溶胶
IF 4 4区 环境科学与生态学
Aerosol and Air Quality Research Pub Date : 2023-01-01 DOI: 10.4209/aaqr.230018
Mirna Alameddine, Oluchi Okoro, Loïc Wingert, Geneviève Marchand, Benoit Barbeau
{"title":"Impact of the Contamination Method on the Disinfection of N95 Respirators: Drops versus Aerosols","authors":"Mirna Alameddine, Oluchi Okoro, Loïc Wingert, Geneviève Marchand, Benoit Barbeau","doi":"10.4209/aaqr.230018","DOIUrl":"https://doi.org/10.4209/aaqr.230018","url":null,"abstract":"The recent surge in the use of filtering facepiece respirators (FFRs) during the SARS-CoV-2 pandemic triggered economic and environmental concerns with regards to their safe reuse and/or disposal. Their decontamination through ultraviolet (UV) irradiation has proven efficient in bench tests. Nevertheless, no study has yet investigated to what extent the decontamination method’s performance was impacted by the contamination method. In this study, Bacillus subtilis spores were inoculated in three suspensions used to contaminate coupons of FFRs via aerosols nebulisation or 2 µ L drops deposition. The contaminated coupons were then exposed to UV irradiation in a monochromatic UVC lamp collimated beam reactor. The results revealed that contamination and decontamination were more efficient for drops (maximum 0.72 log losses and 3 log inactivation at 150 mJ cm –2 ) than for aerosols (maximum 2.47 log losses and 1.75 log inactivation at 150 mJ cm –2 ). Inactivation was greater in coupons contaminated using artificial saliva, followed by phosphate buffer solution, and finally artificial saliva with mucin which also presented the highest fraction of resistant spores, based on kinetic modeling. Disinfection was determined sensitive to the method of contamination ( p < 0.001). However, the composition of the contaminating suspension was the most important performance predictor for decontamination by UV irradiation ( p = 9.2 × 10 –10 ).","PeriodicalId":7402,"journal":{"name":"Aerosol and Air Quality Research","volume":"1 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"70296171","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Calibration of Low-cost Sensors for Measurement of Indoor Particulate Matter Concentrations via Laboratory/Field Evaluation 通过实验室/现场评估校准用于测量室内颗粒物浓度的低成本传感器
IF 4 4区 环境科学与生态学
Aerosol and Air Quality Research Pub Date : 2023-01-01 DOI: 10.4209/aaqr.230097
Doheon Kim, Dongmin Shin, Jungho Hwang
{"title":"Calibration of Low-cost Sensors for Measurement of Indoor Particulate Matter Concentrations via Laboratory/Field Evaluation","authors":"Doheon Kim, Dongmin Shin, Jungho Hwang","doi":"10.4209/aaqr.230097","DOIUrl":"https://doi.org/10.4209/aaqr.230097","url":null,"abstract":"Recently, low-cost sensors (LCSs) have been widely used in monitoring particulate matter (PM) mass concentrations. Maintaining the accuracy of the sensors is important and requires rigorous calibration and performance evaluation. In this study, two commercial LCSs, Plantower PMS3003 and Plantower PMS7003, were evaluated in the laboratory and in the field using a reference-grade PM monitor (GRIMM 11-D). Laboratory evaluation was conducted with polystyrene latex (PSL) particles in a 1 m 3 chamber at 20 ° C with a relative humidity of 20%. Each LCS indicated higher mass concentrations than GRIMM 11-D for small-sized PSL particles (0.56 µ m); however, the LCSs indicated lower mass concentrations than GRIMM 11-D for PSL particles larger than 0.56 µ m. In addition, the difference in mass concentrations between the LCS and GRIMM 11-D became higher with particle sizes greater than 0.56 µ m. Nonetheless, a high correlation (R 2 > 0.9) between each LCS and GRIMM 11-D was obtained. Field evaluation was conducted at Yonsei University (Seoul, South Korea) from February 12 to March 31, 2022. The LCSs showed generally higher PM mass concentrations than GRIMM 11-D; however, some data points of the LCSs revealed different trends. We observed that outdoor PM 10 /PM 2.5 and relative humidity had notable impacts on the LCS data; in addition, LCS sensitivity depended on whether the PM concentration was low or high. Based on these observations, regression-based calibration models were constructed using the selected independent variables (outdoor PM 10 /PM 2.5 and relative humidity) after dividing the PM concentration into low and high sections. Consequently, the accuracy of the LCSs was significantly enhanced. Therefore, using LCSs with the calibration models can replace the use of expensive reference PM monitors, resulting in cost savings.","PeriodicalId":7402,"journal":{"name":"Aerosol and Air Quality Research","volume":"1 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"70297102","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Impacts of the “Coal to Gas” Policy on Rural Air VOC Level and Ozone Potentials in North China “煤改气”政策对华北农村空气VOC水平和臭氧潜能值的影响
IF 4 4区 环境科学与生态学
Aerosol and Air Quality Research Pub Date : 2023-01-01 DOI: 10.4209/aaqr.230136
Zhiyong Li, Chen Liu, Chengjing Cao, Z. Zhai, Changtao Huang, Zhuangzhuang Ren, Jixiang Liu, Lan Chen, Songtao Guo, Ding-Guor Yang
{"title":"Impacts of the “Coal to Gas” Policy on Rural Air VOC Level and Ozone Potentials in North China","authors":"Zhiyong Li, Chen Liu, Chengjing Cao, Z. Zhai, Changtao Huang, Zhuangzhuang Ren, Jixiang Liu, Lan Chen, Songtao Guo, Ding-Guor Yang","doi":"10.4209/aaqr.230136","DOIUrl":"https://doi.org/10.4209/aaqr.230136","url":null,"abstract":"A unique study was enacted during the heating season (HS) in 2020 and 2021 at a rural site in the Beijing-Tianjin-Hebei region to evaluate the policy impacts of “Coal to Gas” (CTG) on ambient volatile organic compounds (VOCs). A total of 58 VOCs in air and flue gas from wall-mounted gas stoves (WMGS) were concurrently analyzed. The total VOCs decreased from 38.6 µ g m –3 in 2020 to 32.8 µ g m –3 in 2021, indicating the CTG played a positive role. However, the ozone formation potentials (OFPs) increased from 31.5 to 44.9 µ g m –3 . Toluene, vinylidene chloride, ethylbenzene, o, m, p-xylene, 4-methyl-2-pentanone, n-butylbenzene, trans-1,2-dichloroethylene, and 1,2,4-trimethylbenzene were the main contributors to the OFPs. Halohydrocarbons contributed the most to ∑ 58 VOCs of 54.8% and 54.4% in 2020 and 2021, respectively. It should be noted that the sustained CTG made WMGS the largest VOC source, replacing coal combustion (CC) in 2020. The CC contributions decreased from 33.2% in 2020 to 28.7% in 2021, while the WMGS far increased from 22.5% to 35.6%. Potential source contribution function (PSCF) modelling showed that the WMGS originated mainly from local emissions. High VOCs appeared surprisingly in clean days, because the WMGS and advanced coal-burning stoves with low particle emission prevailed in heating modes. The recognition of WMGS was achieved by coefficients of correlation and divergence between the positive matrix factorization (PMF) identified factor and field measured profiles of WMGS. This study firstly evidenced that the use of WMGS was becoming a major VOC source in rural north China. Meanwhile, the coal combustion for heating was still serious in rural area despite the “Coal Prohibition” law. The study was expected to provide some novel strategies for further VOC control and air quality improvement in rural area.","PeriodicalId":7402,"journal":{"name":"Aerosol and Air Quality Research","volume":"1 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"70297812","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Assessments of the Emission Contributions from an Ultra-Supercritical Coal-Fired Power Plant to Ambient PM2.5 in Taiwan 台湾超超临界燃煤电厂排放对环境PM2.5贡献之评估
4区 环境科学与生态学
Aerosol and Air Quality Research Pub Date : 2023-01-01 DOI: 10.4209/aaqr.230059
Yi-Cheng Lin, Fang-Yi Cheng, Yi-Ju Lee, Thi-Thuy-Nghiem Nguyen, Chuen-Jinn Tsai, Huan-Cheng Wen, Cheng-Hung Wu, Wei-Chieh Chang, Chung-Chi Huan
{"title":"Assessments of the Emission Contributions from an Ultra-Supercritical Coal-Fired Power Plant to Ambient PM2.5 in Taiwan","authors":"Yi-Cheng Lin, Fang-Yi Cheng, Yi-Ju Lee, Thi-Thuy-Nghiem Nguyen, Chuen-Jinn Tsai, Huan-Cheng Wen, Cheng-Hung Wu, Wei-Chieh Chang, Chung-Chi Huan","doi":"10.4209/aaqr.230059","DOIUrl":"https://doi.org/10.4209/aaqr.230059","url":null,"abstract":"An ultra-supercritical (USC) coal-fired power plant was built to replace the old subcritical (SC) unit in the Linkou power plant (LPP) in northern Taiwan and has been in operation since 2016. Compared to the old SC power generator, the renovated unit (USC + emission control) can reduce SOx, NOx, and TSP emissions by 65%, 87% and 77%, respectively. Enhancing thermal efficiency can significantly reduce air pollutant emissions; however, its impact on ambient air pollutant concentrations under various meteorological conditions is rarely studied. To clarify the issue, we utilized the Community Multiscale Air Quality (CMAQ) model to estimate the contributions of the emissions from old and renovated LPP on the ambient PM2.5 concentrations in Taiwan. During the one-month study period, the LPP upgrade can reduce the PM2.5 concentrations to more than 10 μg m-3 for a severe PM2.5 episode when the weak wind persisted for several days. The reductions were most significant in northern Taiwan. Even with the substantial emission reductions through the advanced USC units, the LPP emissions contribute considerably to the PM2.5 concentrations, with a maximum reaching 5.1 μg m-3 (10.3%). This study quantitatively assesses the environmental burden that a USC coal-fired power plant places on the ambient PM2.5 concentrations.","PeriodicalId":7402,"journal":{"name":"Aerosol and Air Quality Research","volume":"1 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"135653425","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Estimation of PM10 and PM2.5 Using Backscatter Coefficient of Ceilometer and Machine Learning 基于Ceilometer后向散射系数和机器学习的PM10和PM2.5估算
4区 环境科学与生态学
Aerosol and Air Quality Research Pub Date : 2023-01-01 DOI: 10.4209/aaqr.230033
Bu-Yo Kim, Joo Wan Cha, Yong Hee Lee
{"title":"Estimation of PM10 and PM2.5 Using Backscatter Coefficient of Ceilometer and Machine Learning","authors":"Bu-Yo Kim, Joo Wan Cha, Yong Hee Lee","doi":"10.4209/aaqr.230033","DOIUrl":"https://doi.org/10.4209/aaqr.230033","url":null,"abstract":"Air quality issues, including health and environmental challenges, have recently become more relevant in urban areas with large populations and active industries. Therefore, particulate matter (PM) estimation with high accuracy using various methods is required. In this study, PM 10 and PM 2.5 in Cheongju city, South Korea, were estimated using the attenuated backscatter coefficient of the ceilometer and meteorological observation data from an automatic weather station with supervised machine learning (ML). The backscatter coefficient data were obtained from the vertical layer with the highest correlation with PM 10 and PM 2.5 . The estimation methods utilized were tree, vector, neural, and regularization-based supervised ML. The extreme gradient boosting method yielded the highest PM estimation accuracy. The estimation of PM 10 and PM 2.5 for the test data set was more accurate than that in previous studies that used satellite and ground-based meteorological data (bias = 0.10 µ g m –3 , root mean square error (RMSE) = 14.44 µ g m –3 , and R = 0.92 for PM 10 ; and bias = 0.12 µ g m –3 , RMSE = 7.16 µ g m –3 , and R = 0.91 for PM 2.5 ). Particularly, the correlation coefficient was the highest for the estimation results for strong haze cases (1 km < visibility ≤ 5 km) ( R = 0.95 for PM 10 ; R = 0.89 for PM 2.5 ). Therefore, PM estimation using meteorological observation data can help obtain meteorological and PM information simultaneously, making it useful for air quality monitoring.","PeriodicalId":7402,"journal":{"name":"Aerosol and Air Quality Research","volume":"25 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"134882992","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Impacts of Floods on the Indoor Air Microbial Burden 洪水对室内空气微生物负荷的影响
4区 环境科学与生态学
Aerosol and Air Quality Research Pub Date : 2023-01-01 DOI: 10.4209/aaqr.230191
Akila Muthalagu, Yang Lian, Rekha M. Ravindran, Asif Qureshi
{"title":"Impacts of Floods on the Indoor Air Microbial Burden","authors":"Akila Muthalagu, Yang Lian, Rekha M. Ravindran, Asif Qureshi","doi":"10.4209/aaqr.230191","DOIUrl":"https://doi.org/10.4209/aaqr.230191","url":null,"abstract":"Floods create a conducive environment for the proliferation of microbes in the indoor air by providing nutrients and moisture and by introducing new microbes from outdoors to indoors. Thus, it is important to better understand the level of proliferation and the characteristics of microbes in the indoor air of flooded built environments. In this work, we address these aspects in a flooded environment in India and investigate the changes in the indoor air microbial burden by comparing with the control (non-flooded) houses. Flooded houses within one month of water recession were compared with control houses. Microbes (bacteria, fungi) were characterized and endotoxins were quantified. Microbial concentrations were significantly higher in flooded houses than the control houses ( p < 0.05). The potential infectious bacterial genera Pantoea , Acinetobacter , and fungal genera Aspergillus and Penicillium were found dominant in the indoor air of flooded houses. Though these fungal genera were also present in the control houses, concentrations were higher ( p < 0.05) in the flooded houses. Multivariable regression analysis revealed that indoor air microbial burden was significantly and positively associated with outdoor air and outdoor soil. Further, antibiotic resistant bacteria (ARB) were found in both indoor air, and outdoor water sources (wells) of flooded houses. In our chlorine tests, the bacteria showed resistance to concentrations above 100 ppm, far exceeding those found in national and international guidelines. Bacteria were resistant to common antibiotics such as penicillin and ciprofloxacin.","PeriodicalId":7402,"journal":{"name":"Aerosol and Air Quality Research","volume":"1 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"134883004","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The Role of Sulfur Emission from the Petroleum Industry on Ultrafine Particle Number Concentration in Singapore 新加坡石油工业硫排放对超细颗粒数浓度的影响
IF 4 4区 环境科学与生态学
Aerosol and Air Quality Research Pub Date : 2023-01-01 DOI: 10.4209/aaqr.220265
Suyi Hou, Weihan Li, Liudongqing Yang, Guorong Chen, Yilin Zhang, M. Kuwata
{"title":"The Role of Sulfur Emission from the Petroleum Industry on Ultrafine Particle Number Concentration in Singapore","authors":"Suyi Hou, Weihan Li, Liudongqing Yang, Guorong Chen, Yilin Zhang, M. Kuwata","doi":"10.4209/aaqr.220265","DOIUrl":"https://doi.org/10.4209/aaqr.220265","url":null,"abstract":"Ultrafine particles, defined as particles with a diameter ( d p ) smaller than 100 nm, serve as an important component of cloud condensation nuclei, in addition to impacting human health. The dominant sources of ultrafine particles include traffic emissions and nucleation. Singapore is a tropical city that hosts petrochemical industries. To identify the sources of ultrafine particles, a year-long observation of the number size distribution was conducted in Singapore in 2018 and 2019. The concentrations of CO, CO 2 , CH 4 , and SO 2 were also monitored. The particle number concentration during the southwest monsoon season was high, while that during the northeast monsoon period was relatively low. The CO concentration increased during the morning traffic rush hours, which was associated with relatively minor enhancements in ultrafine particle number concentration. The events for a high number concentration of the Aitken mode particles ( d p < 50 nm) were identified during high SO 2 concentration periods. The SO 2 concentration was high during the afternoon because the sea breeze transported the emissions from the coastal industrial area to the observation site. The enhancements in CH 4 from its background level ( Δ CH 4 ) and SO 2 had a quasi-inverse relationship, as the major emission sources of these two chemical species were different. The particle number concentration ( d p > 50 nm) correlated with the enhancements in CO concentration ( Δ CO) for CH 4 -dominant air masses, suggesting that incomplete combustion processes, such as traffic emission, are important for the size range. Conversely, the number concentration of the Aitken mode particles ( d p < 50 nm) increased for SO 2 -dominant air masses, suggesting the importance of industrial plume.","PeriodicalId":7402,"journal":{"name":"Aerosol and Air Quality Research","volume":"1 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"70294114","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Improved Pulsed-Jet Cleaning of Pleated Cone Filter Cartridges Using a Diffusion Nozzle 利用扩散喷嘴改进的脉冲射流清洗折叠锥形滤芯
IF 4 4区 环境科学与生态学
Aerosol and Air Quality Research Pub Date : 2023-01-01 DOI: 10.4209/aaqr.220324
Jianlong Li, W. Xie, Quanquan Wu, Da-Ren Chen, Ding-kun Shi, Qin Chen, Zhifei Ma, Daishe Wu
{"title":"Improved Pulsed-Jet Cleaning of Pleated Cone Filter Cartridges Using a Diffusion Nozzle","authors":"Jianlong Li, W. Xie, Quanquan Wu, Da-Ren Chen, Ding-kun Shi, Qin Chen, Zhifei Ma, Daishe Wu","doi":"10.4209/aaqr.220324","DOIUrl":"https://doi.org/10.4209/aaqr.220324","url":null,"abstract":"A pleated filter cartridge with an additional pleated filter cone installed on the cartridge base, i.e., a pleated cone filter cartridge, has been proposed to increase the filtration area and to improve medium regeneration by reverse pulsed-jet cleaning. In this study, the pulsed-jet cleaning performance of a pleated cone filter cartridge in a dust collector was investigated using a diffusion nozzle (as compared to that of a round nozzle). The effects of tank pressure ( TP ), jet distance ( JD ), and inner cone height ( HC ) on the distribution of static pressure acting on the inner surfaces of the cone filter cartridges were evaluated. The filtration pressure drops and emitted dust concentration of cartridges during the dust collector operation were also measured. It was found that, using a diffusion nozzle, the pulsed-jet pressure at the upper portion of the filter cartridges was increased, compared to that of a round nozzle, particularly for cartridges with a low HC and a short JD setting (e.g., a factor of 7.0 was observed when HC = 560 mm and at a JD setting of 150 mm). The pulsed-jet cleaning of a pleated cone filter cartridge using a diffusion nozzle can decrease the residual filtration pressure drop, prolong the cleaning interval, and reduce the average dust concentration emission from cone filter cartridges.","PeriodicalId":7402,"journal":{"name":"Aerosol and Air Quality Research","volume":"1 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"70294490","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
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