Shengzhi Sun, Zhonghui Cheng, Juan Song, Chaoyue Yan, T.P.M. Man, G. Dong, B. Qian, Jianrong Qiu
{"title":"Low‐Power‐Consumption, Reversible 3D Optical Storage Based on Selectively Laser‐Induced Photoluminescence Degradation in CsPbBr3 Quantum Dots Doped Glass","authors":"Shengzhi Sun, Zhonghui Cheng, Juan Song, Chaoyue Yan, T.P.M. Man, G. Dong, B. Qian, Jianrong Qiu","doi":"10.1002/admt.202200470","DOIUrl":"https://doi.org/10.1002/admt.202200470","url":null,"abstract":"In recent years, inorganic lead halide perovskite quantum dots have been used in various optoelectronic fields for their excellent luminescence properties, such as narrow emission bands, ultra‐wide tunable emission wavelength, and high quantum efficiency. In this paper, different from luminescence optimization in most research, luminescence degradation of perovskite quantum dots is addressed by femtosecond laser irradiation and successfully used for three‐dimensional data storage in CsPbBr3 quantum dots doped glass. Photoluminescence (PL) degradation can be finely modulated by adjusting the laser parameters. PL degradation mechanism, investigated by optical spectroscopy and morphology characterization, is attributed to laser‐induced decomposition, recrystallization, and defection of CsPbBr3 quantum dots. Laser‐induced PL degradation and the followed PL recovery by heat treatment are repeated for several cycles, showing good reversibility. Multilayer PL degradation patterns are written into the glass and read out without crosstalk, indicating high‐reliability 3D optical storage characteristics. Amazingly, PL degradation can be induced by just a low‐energy single laser pulse with estimated subpicosecond writing time per bit, demonstrating its potential in high‐speed, low‐power consumption 3D optical storage.","PeriodicalId":7200,"journal":{"name":"Advanced Materials & Technologies","volume":"20 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2022-08-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"79059377","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Near‐Infrared to Visible Light Converter by Integrating Graphene Transistor into Perovskite Quantum Dot Light Emitting Diodes (Adv. Mater. Technol. 8/2022)","authors":"Wei Zhao, Sheng Bi, Chengming Jiang, Jinhui Song","doi":"10.1002/admt.202270048","DOIUrl":"https://doi.org/10.1002/admt.202270048","url":null,"abstract":"A near-infrared to visible light converter (NVLC) which could emit visible light according to external NIR is fabricated in article number 2200043 by Sheng Bi ,Jinhui Song, and co-workers. The NVLC is an integration of an inverted perovskite QLED and a hybrid PbS quantum dots/graphene transistor. Further, the micron-scale NVLCs are integrated into a matrix device that could sense NIR image and display it into visible light image.","PeriodicalId":7200,"journal":{"name":"Advanced Materials & Technologies","volume":"31 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2022-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"72874586","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Conjugated Polymer‐Wrapped Single‐Wall Carbon Nanotubes for High‐Mobility Photonic/Electrical Fully Modulated Synaptic Transistor","authors":"Maina Moses Mburu, Kuan‐Ting Lu, Nathaniel Prine, Ai-Nhan Au-Duong, Wei‐Hung Chiang, X. Gu, Y. Chiu","doi":"10.1002/admt.202101506","DOIUrl":"https://doi.org/10.1002/admt.202101506","url":null,"abstract":"Although synaptic devices have already demonstrated their operability through electric or photonic signals or a combination thereof, current challenges include developing a single hardware synaptic device that is independently fully operational through either photonic or electric signals to improve device versatility. Additionally, most previously reported devices are fabricated using multiple technical processes—which impede device implementation—while the low‐output current triggered in most such devices limits the possible integration of auxiliary gadgets. Therefore, by spontaneously wrapping a conjugated block copolymer around single‐walled carbon nanotubes (SWCNTs), a thin‐film transistor memory device comprising single‐layered poly(9,9‐dioctylfluorene)‐b‐polyisoprene (PF‐b‐PI)‐wrapped‐SWCNTs—which function as both a semiconductor and an electret layer—to simplify the device structure and fabrication is designed. Owing to the robust SWCNT charge carrier mobility (≈11.3 cm2 V−1 s−1), a high output current (10−4 to 10−3 A) can be achieved and because PF is a photoactive conjugated polymer, the photonic signal can also be modulated. The designed memory device independently exhibits both voltage‐ and light‐controllable switching, thereby mimicking biological synaptic behavior such as short‐ and long‐term plasticity, spike‐time, and spike‐rate‐dependent plasticity. This study may provide a suitable basis for developing more‐convenient, economical, highly versatile synaptic devices.","PeriodicalId":7200,"journal":{"name":"Advanced Materials & Technologies","volume":"15 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2022-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"74431671","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Lingying Li, Wanli Li, Xuying Liu, Mizuki Tenjimbayashi, H. Segawa, C. Niikura, T. Nakayama, T. Minari
{"title":"Microflow Manipulation by Velocity Field Gradient: Spontaneous Patterning of Silver Nanowires for Tailored Flexible Transparent Conductors (Adv. Mater. Technol. 8/2022)","authors":"Lingying Li, Wanli Li, Xuying Liu, Mizuki Tenjimbayashi, H. Segawa, C. Niikura, T. Nakayama, T. Minari","doi":"10.1002/admt.202270046","DOIUrl":"https://doi.org/10.1002/admt.202270046","url":null,"abstract":"","PeriodicalId":7200,"journal":{"name":"Advanced Materials & Technologies","volume":"52 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2022-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"84682947","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
S. Glinšek, Longfei Song, V. Kovacova, M. A. Mahjoub, Nicolas Godard, S. Girod, Jean‐Luc Biagi, R. Quintana, T. Schleeh, Matthieu Guédra, M. Rupin, E. Defay
{"title":"Inkjet‐Printed Piezoelectric Thin Films for Transparent Haptics","authors":"S. Glinšek, Longfei Song, V. Kovacova, M. A. Mahjoub, Nicolas Godard, S. Girod, Jean‐Luc Biagi, R. Quintana, T. Schleeh, Matthieu Guédra, M. Rupin, E. Defay","doi":"10.1002/admt.202200147","DOIUrl":"https://doi.org/10.1002/admt.202200147","url":null,"abstract":"Transparent thin‐film piezoelectric transducers are attractive for haptic displays. However, for their widespread use in consumer electronics, innovative and cost‐effective processing methods need to be developed. In this contribution the effectiveness of the deposition of lead zirconate titanate thin films by inkjet printing for the fabrication of haptic devices is demonstrated. The 1,3‐propanediol solvent is used to prepare effective inkjet‐printing inks from chemical solution deposition solutions. The printed thin‐film structures on fused silica glass substrates are 900 nm thick and strongly {100} oriented perovskite phase is detected in X‐ray diffraction patterns. To fabricate devices, interdigitated capacitors and SU‐8 insulation layers are deposited on top of the printed lead zirconate titanate. Dimensions of the final device are 15.7 × 3.4 mm2. A standing antisymmetric Lamb wave is observed at 63.3 kHz, with out‐of‐plane displacement reaching 2 µm at an applied voltage of 100 V. This value exceeds the limit at which the texture rendering function can be induced in the device. Good functional performance of the device is linked with good electromechanical properties of the printed piezoelectric, with permittivity ε ′ and piezoelectric coefficient e33,f values of 1000 and 7.7 C m−2, respectively, which are comparable to films prepared by standard spin‐coating process.","PeriodicalId":7200,"journal":{"name":"Advanced Materials & Technologies","volume":"35 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2022-08-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"84677157","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Zehuan Wang, Jin Cheng, Yan Xie, Yunhan Wang, Zhonghui Yu, Shuai Li, Liuting Li, S. Dong, Hong Wang
{"title":"Lead‐Free Piezoelectric Composite Based on a Metamaterial for Electromechanical Energy Conversion","authors":"Zehuan Wang, Jin Cheng, Yan Xie, Yunhan Wang, Zhonghui Yu, Shuai Li, Liuting Li, S. Dong, Hong Wang","doi":"10.1002/admt.202200650","DOIUrl":"https://doi.org/10.1002/admt.202200650","url":null,"abstract":"Additive manufacturing of arbitrary shapes and unique architecture provides remarkable flexibility and simplicity for the preparation of highly complex conformal electronics. This drives up demand for electronic materials with excellent process ability and functionality from one‐step molding of microminiature to large‐scale devices. Herein, a novel method is introduced for fabricating high‐performance barium titanate (BaTiO3)‐polydimethylsiloxane composites based on three‐dimensional (3D)‐printing‐ordered structure of a metamaterial skeleton. When subjected to external mechanical stress, the metamaterial structure facilitates effective stress transfer, resulting in a significantly improved voltage output. In comparison to traditional low‐dimensional ceramic polymer composites, metamaterial‐structured BaTiO3 composites exhibit excellent electromechanical energy conversion properties, thereby enabling tactile imitation applications and mechanical energy harvesting. This study proposes a novel strategy for biological signal identification and implantable self‐powered electronic applications.","PeriodicalId":7200,"journal":{"name":"Advanced Materials & Technologies","volume":"48 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2022-07-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"86053440","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Flexible Copper Metal Circuits via Desktop Laser Printed Masks","authors":"R. Ghosh, Xiaoya Liu, M. Z. Yates","doi":"10.1002/admt.202200400","DOIUrl":"https://doi.org/10.1002/admt.202200400","url":null,"abstract":"A novel process is demonstrated that produces patterns of electrically conductive copper on a flexible polyimide film substrate using standard desktop laser printed toner and near room temperature aqueous chemistry. The laser toner acts as a mask to selectively block the ion exchange self‐metallization (IESM) reduction reaction that forms nanoscale silver or palladium coatings at the polyimide surface. The silver or palladium IESM coating is then used as a catalyst for electroless deposition of copper. Under appropriate conditions, the copper is deposited selectively on top of the catalyst layer. The resulting copper layer has a measured sheet resistance as low as 0.3 Ohms/sq. Electrical isolation is measured between copper traces spaced as close as 300 microns, and high conductivity is measured along traces with widths as low as 200 microns. The minimum pattern size appears to be limited primarily by the resolution of the laser toner pattern, as the IESM metal layer is observed to follow the contours of individual toner particles. The process avoids the use of high temperature, vacuum, and organic solvents and is thus suitable for very low cost prototyping or distributed manufacturing of simple electronic devices.","PeriodicalId":7200,"journal":{"name":"Advanced Materials & Technologies","volume":"56 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2022-07-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"83478017","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
H. Yoon, Seokgyu Ko, Ashok Chhetry, Chani Park, Sudeep Sharma, Sanghyuk Yoon, Dongkyun Kim, Shipeng Zhang, D. Kim, J. Park
{"title":"Ultra‐Sensitive and Quick‐Responsive Hybrid‐Supercapacitive Iontronic Pressure Sensor for Intuitive Electronics and Artificial Tactile Applications","authors":"H. Yoon, Seokgyu Ko, Ashok Chhetry, Chani Park, Sudeep Sharma, Sanghyuk Yoon, Dongkyun Kim, Shipeng Zhang, D. Kim, J. Park","doi":"10.1002/admt.202101743","DOIUrl":"https://doi.org/10.1002/admt.202101743","url":null,"abstract":"Recent advances in supercapacitive pressure sensors based on iontronic film have a significant capacitive response and a low detection limit due to their large capacitance change resulting from electrical double layer (EDL) and these pressure sensors are used to detect a wide range of pressure with high resolution for various applications such as prosthesis, wearable devices, and robotics. Thus, the enhancements to the EDL capacitive response are significantly important challenges for advanced applications with outstanding performances. Herein, an ultra‐sensitive and quick‐responsive hybrid‐supercapacitive iontronic pressure sensor using a novel sensing mechanism and facile fabrication technique is reported to overcome the limitations of the existing iontronic pressure sensors. As a sensing material, conductive polymer and carbon nanotube are incorporated into the iontronic film, as pseudo‐ and EDL‐capacitive material, respectively. Moreover, vinyl silica nanoparticle (VSNP) is used to decrease the recovery time by making the iontronic film quick‐response. The developed hybrid‐supercapacitive pressure sensor exhibited an ultra‐high sensitivity of 301.5 kPa−1 over a wide pressure range of up to 63.3 kPa along with a fast recovery time of ≈32 ms. It is believed that the proposed hybrid‐supercapacitive mechanism in iontronic film will significantly enhance the performance of conventional iontronic pressure sensors.","PeriodicalId":7200,"journal":{"name":"Advanced Materials & Technologies","volume":"6 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2022-07-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"87478048","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}