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Spectral Hole-Burning and Related Spectroscopies: Science and Applications最新文献

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Spectral Hole Burning and Fluorescence Line Narrowing of Si Center in CVD Diamond CVD金刚石中Si中心的光谱烧孔和荧光线变窄
Spectral Hole-Burning and Related Spectroscopies: Science and Applications Pub Date : 1900-01-01 DOI: 10.1364/shbs.1994.wd54
A. Gorokhovsky, A. Turukhin, R. Alfano, W. Phillips
{"title":"Spectral Hole Burning and Fluorescence Line Narrowing of Si Center in CVD Diamond","authors":"A. Gorokhovsky, A. Turukhin, R. Alfano, W. Phillips","doi":"10.1364/shbs.1994.wd54","DOIUrl":"https://doi.org/10.1364/shbs.1994.wd54","url":null,"abstract":"In this presentation we report on several spectral features associated with Si impurity in diamond related to spectral hole-burning. Diamond, with its hardness and high temperature stability, is a potentially useful material for high temperature hole-burning storage. The first hole-burning in bulk diamonds [1] was observed from color centers in the spectra of N3 at 415 nm, H4 at 496 nm, N-V at 637 nm, and GR1 at 741 nm. Recently, hole-burning was observed for color centers N-V at 637 nm and 574 nm of electron irradiated chemical-vapor deposited (CVD) diamonds [2].","PeriodicalId":443330,"journal":{"name":"Spectral Hole-Burning and Related Spectroscopies: Science and Applications","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"1900-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"133582908","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Coherent erasure and processing in time-domain optical storage 时域光存储中的相干擦除与处理
Spectral Hole-Burning and Related Spectroscopies: Science and Applications Pub Date : 1900-01-01 DOI: 10.1364/shbs.1994.wc4
U. Elman, S. Kröll
{"title":"Coherent erasure and processing in time-domain optical storage","authors":"U. Elman, S. Kröll","doi":"10.1364/shbs.1994.wc4","DOIUrl":"https://doi.org/10.1364/shbs.1994.wc4","url":null,"abstract":"Persistent spectral hole-burning and photon echoes can provide insight into the dynamics of amorphous and crystalline materials on the molecular/atomic level. Part of the current interest in these methods, however, is also caused by the existence of potential applications in optical data storage and processing. At present it may be difficult to specify exactly at what applications these techniques should try to target but, based on current research efforts and results, it appears that persistent spectral hole burning is a possible candidate for high density, possibly long time, volumetric storage, while photon echoes have properties more attractive for short time storage or storage connected to processing applications.","PeriodicalId":443330,"journal":{"name":"Spectral Hole-Burning and Related Spectroscopies: Science and Applications","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"1900-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"133115268","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Single Molecule Spectroscopy of Novel Crystalline and Polymeric Systems 新型晶体和聚合物体系的单分子光谱
Spectral Hole-Burning and Related Spectroscopies: Science and Applications Pub Date : 1900-01-01 DOI: 10.1364/shbs.1994.wb3
T. Basché, S. Kummer, R. Kettner, J. Tittel, C. Bräuchle
{"title":"Single Molecule Spectroscopy of Novel Crystalline and Polymeric Systems","authors":"T. Basché, S. Kummer, R. Kettner, J. Tittel, C. Bräuchle","doi":"10.1364/shbs.1994.wb3","DOIUrl":"https://doi.org/10.1364/shbs.1994.wb3","url":null,"abstract":"Single molecule spectroscopy in solids at low temperature is a very rapidly growing field which due to the sensitivity of a single molecule to its truly local environment yields new insights in the structure and dynamics of crystalline and amorphous solids [1,2]. In the first years of SMS a lot of different experimental techniques have been applied to only a few well selected systems. These were the mixed crystalline system pentacene in p-terphenyl, and perylene and terrylene in poly(ethylene). Very recently, it was recognized by several groups that it is important to find new systems to demonstrate the more general applicability of this new and exciting spectroscopy. While there are several - well known - stringent requirements for any specific system to observe single molecule spectra with the fluorescence excitation technique, recent successful experiments proved that there is still a wide variety of systems where SMS can be pursued. Two new systems introduced lately were terrylene in the Shpol’skii matrix hexadecane [3] and Rhodamine 640 in (poly)ethylene [4]. In our group we investigated new crystalline as well as new polymeric systems.","PeriodicalId":443330,"journal":{"name":"Spectral Hole-Burning and Related Spectroscopies: Science and Applications","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"1900-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"133555029","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Near-field Time-Resolved Fluorescence Spectroscopy of Single Molecules 单分子近场时间分辨荧光光谱
Spectral Hole-Burning and Related Spectroscopies: Science and Applications Pub Date : 1900-01-01 DOI: 10.1364/shbs.1994.fc2
X. S. Xie, R. Dunn
{"title":"Near-field Time-Resolved Fluorescence Spectroscopy of Single Molecules","authors":"X. S. Xie, R. Dunn","doi":"10.1364/shbs.1994.fc2","DOIUrl":"https://doi.org/10.1364/shbs.1994.fc2","url":null,"abstract":"Fluorescence lifetime measurements on single dye molecules with nanometer spatial resolution are achieved by incorporating time-correlated single photon counting with a near-field fluorescence microscope.","PeriodicalId":443330,"journal":{"name":"Spectral Hole-Burning and Related Spectroscopies: Science and Applications","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"1900-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"122093934","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Fragile Systems: a Comparative Study of Glassy and Crystalline Phases 脆弱系统:玻璃相和结晶相的比较研究
Spectral Hole-Burning and Related Spectroscopies: Science and Applications Pub Date : 1900-01-01 DOI: 10.1364/shbs.1994.wd36
J. Kikas
{"title":"Fragile Systems: a Comparative Study of Glassy and Crystalline Phases","authors":"J. Kikas","doi":"10.1364/shbs.1994.wd36","DOIUrl":"https://doi.org/10.1364/shbs.1994.wd36","url":null,"abstract":"A full understanding of the strycture and dynamics of different condensed phases of matter (liquids, glasses, crystals) is hardly possible without addressing the processes of their mutual transformations and the interrelations between different phases. This view has become more and more common in the condensed matter research. A well-known example concerns the studies of the liquid-glass transition.","PeriodicalId":443330,"journal":{"name":"Spectral Hole-Burning and Related Spectroscopies: Science and Applications","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"1900-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"124772564","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Wavelength and polarization dependence of hole-burning properties in highly oriented J-aggregates 高取向j -聚集体中孔燃烧特性的波长和偏振依赖性
Spectral Hole-Burning and Related Spectroscopies: Science and Applications Pub Date : 1900-01-01 DOI: 10.1364/shbs.1994.wd47
K. Misawa, Takayoshi Kobayashi, S. Machida, K. Horie
{"title":"Wavelength and polarization dependence of hole-burning properties in highly oriented J-aggregates","authors":"K. Misawa, Takayoshi Kobayashi, S. Machida, K. Horie","doi":"10.1364/shbs.1994.wd47","DOIUrl":"https://doi.org/10.1364/shbs.1994.wd47","url":null,"abstract":"J-aggregates of cyanine dyes show a sharp absorption peak, called J- band, below the transition band of monomers [1,2]. The band is due to the transition of excitons delocalized over an aggregate by intermolecular dipole interaction. A simple model of N identical molecules aligned in a one- dimensional chain has been proposed to explain the optical spectrum of the J- aggregates [3-5]. Recently, we have developed a new method, named \"vertical spin-coating\", to prepare highly oriented J-aggregates dispersed in polymer films [6]. Linear dichroic spectra, and electro-absorption spectra have been measured to study the optical properties of one-dimensional excitons in J- aggregates [7,8].","PeriodicalId":443330,"journal":{"name":"Spectral Hole-Burning and Related Spectroscopies: Science and Applications","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"1900-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"125419438","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Programmable pulse delays by phase controlled frequency swept cw holograms 可编程脉冲延迟的相位控制扫频连续波全息图
Spectral Hole-Burning and Related Spectroscopies: Science and Applications Pub Date : 1900-01-01 DOI: 10.1364/shbs.1994.wd8
S. Altner, S. Bernet, E. Maniloff, Felix Graf, A. Renn, U. Wild
{"title":"Programmable pulse delays by phase controlled frequency swept cw holograms","authors":"S. Altner, S. Bernet, E. Maniloff, Felix Graf, A. Renn, U. Wild","doi":"10.1364/shbs.1994.wd8","DOIUrl":"https://doi.org/10.1364/shbs.1994.wd8","url":null,"abstract":"The spectroscopic technique of photon echoes has been proven to be a versatile tool to obtain information about dephasing times and related parameters of materials [1]. In addition, applications within the framework of time domain optical data storage and processing have been discussed [2].","PeriodicalId":443330,"journal":{"name":"Spectral Hole-Burning and Related Spectroscopies: Science and Applications","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"1900-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"132148314","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Optically Detected Nuclear Magnetic Resonance of Co2+ in LiGa5O8 LiGa5O8中Co2+的光学检测核磁共振
Spectral Hole-Burning and Related Spectroscopies: Science and Applications Pub Date : 1900-01-01 DOI: 10.1364/shbs.1994.wd6
R. Wannemacher, S. Magnien, W. Grill
{"title":"Optically Detected Nuclear Magnetic Resonance of Co2+ in LiGa5O8","authors":"R. Wannemacher, S. Magnien, W. Grill","doi":"10.1364/shbs.1994.wd6","DOIUrl":"https://doi.org/10.1364/shbs.1994.wd6","url":null,"abstract":"Optical spectral hole-burning has proven to be a valuable tool for the detection of hyperfine [1] as well as superhyperfine [2] interactions in ground and optically excited states of rare earth ions. In cases where the hole-burning mechanism is population storage in hyperfine or superhyperfine levels of the electronic ground state, the application of an rf-magnetic field resonant with the splittings changes the depth of the spectral hole, which can be monitored either in absorption or in fluorescence [3]. This double resonance technique, commonly termed 'Optically Detected Magnetic Resonance', ODMR (for an overview of applications to rare earth ions see [1]), is in principle able to detect hyperfine as well as superhyperfine [4] splittings of ground and excited [5] states separately. Moreover, the resolution of this technique is determined by the linewidth of the nuclear magnetic resonance and not by the laser linewidth, which only needs to be smaller than the splittings in order to enable spectral hole-burning.","PeriodicalId":443330,"journal":{"name":"Spectral Hole-Burning and Related Spectroscopies: Science and Applications","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"1900-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"130833667","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Inorganic and Hybrid (organic-inorganic) Sol-Gel Glasses doped with Organic Molecules: Fluorescence Line Narrowing, Persistent Hole-Burning and Spectral Diffusion 掺杂有机分子的无机和杂化(有机-无机)溶胶-凝胶玻璃:荧光线变窄、持续烧孔和光谱扩散
Spectral Hole-Burning and Related Spectroscopies: Science and Applications Pub Date : 1900-01-01 DOI: 10.1364/shbs.1994.fb3
J. Galaup, A. Veret-lemarinier, S. Kulikov, S. Arabei, J. Boilot, F. Chaput
{"title":"Inorganic and Hybrid (organic-inorganic) Sol-Gel Glasses doped with Organic Molecules: Fluorescence Line Narrowing, Persistent Hole-Burning and Spectral Diffusion","authors":"J. Galaup, A. Veret-lemarinier, S. Kulikov, S. Arabei, J. Boilot, F. Chaput","doi":"10.1364/shbs.1994.fb3","DOIUrl":"https://doi.org/10.1364/shbs.1994.fb3","url":null,"abstract":"We used spectral line narrowing techniques (site selection spectroscopy and persistent spectral hole-burning) to investigate the vibronic visible spectra of different porphyrins included in various sol-gel matrices. Also, quinizarin and a quinizarin derivative have been studied. The main aim of this work is to compare pure inorganic matrices and hybrid (organic-inorganic) matrices in which organic groups are permanently attached to the inorganic squeleton.","PeriodicalId":443330,"journal":{"name":"Spectral Hole-Burning and Related Spectroscopies: Science and Applications","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"1900-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"123658734","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High Pressure Hole-Burning Studies of Transport Dynamics in Photosynthetic Protein Complex 光合蛋白复合体的高压孔燃烧转运动力学研究
Spectral Hole-Burning and Related Spectroscopies: Science and Applications Pub Date : 1900-01-01 DOI: 10.1364/shbs.1994.thd2
G. Small, N. Reddy, R. Jankowiak
{"title":"High Pressure Hole-Burning Studies of Transport Dynamics in Photosynthetic Protein Complex","authors":"G. Small, N. Reddy, R. Jankowiak","doi":"10.1364/shbs.1994.thd2","DOIUrl":"https://doi.org/10.1364/shbs.1994.thd2","url":null,"abstract":"Hole burning spectroscopies have proven to be powerful tools for the elucidation of the excited state (Qy) electronic structure and transport (energy, charge) dynamics of photosynthetic protein-chlorophyll complexes.1-3 Furthermore, hole burning has proven that such complexes are glass-like on a microscopic scale, which results in inhomogeneous broadenings of ~50-150 cm-1 (ΓI) for the Qy←S0 Chi absorption transitions. Importantly, it has also been shown that the zero-phonon line (ZPL) frequency distribution functions for different Qy-states of the same complex are uncorrelated, meaning that the widths of the distribution functions for energy gaps relevant to energy and electron transfer are ~21/2 ΓI. This raises the possibility that the kinetics for transport could be dispersive.4 Whether or not they are turns out to be dependent on the .strength of the electron-phonon coupling associated with the transport process. Fortunately, hole burning has proven to be capable of characterizing the nature and strength of this coupling. Required was the development of an accurate theory for entire hole profile (zero-phonon hole [ZPH] plus phonon sideband holes) applicable for arbitrarily strong electron-phonon coupling in the low temperature limit. More recently, this theory5 has been extended to arbitrary temperature.6 A key point is that the ZPH is only one small part of the entire profile. It is the entire hole profile that is important to the problem of transport dynamics in the photosynthetic unit. Thus it is that single molecule (complex) detection would be of little consequence to the problem of energy and electron transfer.","PeriodicalId":443330,"journal":{"name":"Spectral Hole-Burning and Related Spectroscopies: Science and Applications","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"1900-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"124922940","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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