International Journal of Greenhouse Gas Control最新文献

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A million scenarios to identify conditions for robust bioenergy carbon capture in Sweden 一百万个场景来确定瑞典强大的生物能源碳捕获的条件
IF 4.6 3区 工程技术
International Journal of Greenhouse Gas Control Pub Date : 2025-05-29 DOI: 10.1016/j.ijggc.2025.104411
Oscar Stenström, Tharun Roshan Kumar, Magnus Rydén
{"title":"A million scenarios to identify conditions for robust bioenergy carbon capture in Sweden","authors":"Oscar Stenström,&nbsp;Tharun Roshan Kumar,&nbsp;Magnus Rydén","doi":"10.1016/j.ijggc.2025.104411","DOIUrl":"10.1016/j.ijggc.2025.104411","url":null,"abstract":"<div><div>Large-scale bioenergy carbon capture and storage (BECCS) could be realized without escalating biomass use - under the right conditions. We apply robust decision-making theory to frame carbon capture as a decision problem. We then search for conditions of low costs and energy penalties by modelling the capture decision across a million scenarios of already-existing plants in Sweden. Mining the scenario data reveals that annual plant utilization, heat recovery via heat pumps and electricity prices constitute key conditions for combined heat and power plants. For pulp mills, key conditions are site-specific, but the availability of low-pressure steam and electricity prices are generally important. A sensitivity analysis supports these findings, but also identifies capture rates as key. About 19 MtCO<sub>2</sub> could be captured annually from the 113 plants studied while combusting zero additional biomass. Under the identified conditions, this would entail reduced power and district heating generation of 5.1-7.9 TWh per year – a modest penalty relative to the 220 TWh generated annually in Sweden.</div></div>","PeriodicalId":334,"journal":{"name":"International Journal of Greenhouse Gas Control","volume":"145 ","pages":"Article 104411"},"PeriodicalIF":4.6,"publicationDate":"2025-05-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144168556","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Flow2Quake, an integrated multiphase flow, geomechanical and seismicity model for efficient forecasting of injection and extraction induced earthquakes Flow2Quake是一个集成多相流、地质力学和地震活动性模型,用于有效预测注入和抽取引起的地震
IF 4.6 3区 工程技术
International Journal of Greenhouse Gas Control Pub Date : 2025-05-28 DOI: 10.1016/j.ijggc.2025.104388
Mateo Acosta , Thomas Ledevin , Guillaume Salha , Charles Forestier , Lucie Michelin , Xiaojing Fu , Jean-Philippe Avouac
{"title":"Flow2Quake, an integrated multiphase flow, geomechanical and seismicity model for efficient forecasting of injection and extraction induced earthquakes","authors":"Mateo Acosta ,&nbsp;Thomas Ledevin ,&nbsp;Guillaume Salha ,&nbsp;Charles Forestier ,&nbsp;Lucie Michelin ,&nbsp;Xiaojing Fu ,&nbsp;Jean-Philippe Avouac","doi":"10.1016/j.ijggc.2025.104388","DOIUrl":"10.1016/j.ijggc.2025.104388","url":null,"abstract":"<div><div>Efforts to secure and decarbonize the energy sector are driving various subsurface reservoir operations. These operations carry a risk of inducing surface deformation and earthquakes. To assess these risks, modeling tools integrating fluid flow, geomechanical and seismicity modeling are needed. Here, we demonstrate the use of an efficient Vertical Flow Equilibrium (VFE) multiphase fluid flow model in an integrated framework for deformation and seismicity modeling both under fluid extraction or injection configurations. The VFE-computed spatio-temporal pressure evolution is fed to a geomechanical module to compute surface deformation and stress changes in and around the reservoir. Stress changes feed a seismicity module to calculate earthquake probabilities. First, we apply the benchmarked model to gas extraction from Groningen. There, we can reduce the variance of pressure measurements by <span><math><mo>∼</mo></math></span>38% with respect to a pre-existing single phase flow model while remaining computationally efficient. The surface deformation and seismicity simulations show remarkable agreement with observed data. Second, we study induced seismicity due to CO<span><math><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub></math></span> sequestration in the Decatur phase 1 project. We find that, for the Decatur phase 1 project, poroelastic stress changes can account for most of the non-clustered observed seismicity within modeling uncertainties. Finally we simulate scenarios for CO<span><math><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub></math></span> sequestration using the Quest field. The sloping reservoir topography significantly impacts the predicted position of the CO<span><math><msub><mrow></mrow><mrow><mn>2</mn></mrow></msub></math></span> plume but the effects on geomechanical deformation (and seismicity) are minimal. Incorporating VFE models with geomechanical and seismicity forecasts with real-world case applications can allow real-time hazard assessment and mitigation procedures.</div></div>","PeriodicalId":334,"journal":{"name":"International Journal of Greenhouse Gas Control","volume":"145 ","pages":"Article 104388"},"PeriodicalIF":4.6,"publicationDate":"2025-05-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144154385","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
The role of impurities in CCS from pilot capture plants to sequestration sites—A review 从中试捕集厂到封存点,杂质在CCS中的作用综述
IF 4.6 3区 工程技术
International Journal of Greenhouse Gas Control Pub Date : 2025-05-27 DOI: 10.1016/j.ijggc.2025.104410
Eleni G. Nikolaidou , Evie Nessi , Panos Seferlis , Athanasios I. Papadopoulos
{"title":"The role of impurities in CCS from pilot capture plants to sequestration sites—A review","authors":"Eleni G. Nikolaidou ,&nbsp;Evie Nessi ,&nbsp;Panos Seferlis ,&nbsp;Athanasios I. Papadopoulos","doi":"10.1016/j.ijggc.2025.104410","DOIUrl":"10.1016/j.ijggc.2025.104410","url":null,"abstract":"<div><div>We investigate the presence and effects of impurities in the carbon capture, transportation and sequestration (CCS) technology chain. We start from the composition of flue gases and investigate the subsequent treatment methods, the technical and operating characteristics of solvent-based CO<sub>2</sub> capture pilot plants, the compositions of the absorber and desorber outlet streams and the CO<sub>2</sub> stream specifications for downstream compression, transportation and storage processes. We present public data from 40 campaigns in large capture pilot plants and 20 sets of specifications for CO<sub>2</sub> transportation and underground storage from national agencies, companies and projects worldwide. We identify and categorize the impurities depending on the flue gas source and the solvent type. The most commonly identified emissions in the treated gas are ammonia (NH<sub>3</sub>) and the solvent used in each plant. Monoethanolamine (MEA) emissions are higher compared to those of the other amine solvents. Sulfur and nitrogen oxides (SO<sub>x</sub>, NO<sub>x</sub>) are the most investigated impurities, whereas oxalate and formate are the most reported degradation products. Regardless of the solvent used, NO<sub>x</sub>, NH<sub>3</sub> and aldehydes are reported in the CO<sub>2</sub> gas product stream of most campaigns. The specifications for transportation and sequestration have similarities, with those of Northern Lights being stricter.</div></div>","PeriodicalId":334,"journal":{"name":"International Journal of Greenhouse Gas Control","volume":"145 ","pages":"Article 104410"},"PeriodicalIF":4.6,"publicationDate":"2025-05-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144154386","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Interactions of CO2 with sedimentary blue carbon: the fate of leaked CO2 from a geological storage site 二氧化碳与沉积蓝碳的相互作用:从地质储存地点泄漏的二氧化碳的命运
IF 4.6 3区 工程技术
International Journal of Greenhouse Gas Control Pub Date : 2025-05-19 DOI: 10.1016/j.ijggc.2025.104408
Malini Kallingal , Tom Kettlety , Christopher Batchelor-McAuley , Rosalind E.M. Rickaby
{"title":"Interactions of CO2 with sedimentary blue carbon: the fate of leaked CO2 from a geological storage site","authors":"Malini Kallingal ,&nbsp;Tom Kettlety ,&nbsp;Christopher Batchelor-McAuley ,&nbsp;Rosalind E.M. Rickaby","doi":"10.1016/j.ijggc.2025.104408","DOIUrl":"10.1016/j.ijggc.2025.104408","url":null,"abstract":"<div><div>One of the main considerations in terms of carbon dioxide removal techniques is the net carbon storage potential, i.e. whether the amount of carbon that can be stored, significantly outweighs the carbon footprint of the process of storage. Here we assess the potential for disruption of blue carbon stored in sediments, and interactions with leaked CO<sub>2</sub> above a sub-seafloor geological storage site. Blue carbon is carbon stored within the ocean which, in this study, is in the form of sedimentary calcium carbonate, or organic carbon. CO<sub>2</sub> injected into sub-sea bed geological storage sites can be effectively trapped and retained. Despite the perceived safety of geological CO<sub>2</sub> storage, it is imperative to thoroughly evaluate and address the risks of carbon loss either through disturbance of sea bed carbon with infrastructure, or through the impacts of potential CO<sub>2</sub> leakage from the storage reservoir. This study aims to quantify the amount of blue carbon, and its different components, which is at risk of loss above a proposed CO<sub>2</sub> reservoir in the North Sea. Second we investigate the impact of CO<sub>2</sub> leakage from the reservoir on sediment-stored blue carbon through laboratory based experiments. The sediments in the North Sea were found to contain minimal organic carbon but a significant variable fraction of biogenic calcite in the form of shells. The leaked CO<sub>2</sub> was found to act as an acid titrating away the CO<sub>3</sub><sup>2-</sup> ion in seawater to drive undersaturation with respect to calcite until equilibration occurs between the CO<sub>2</sub> stream and the calcite. The study infers that sites abundant in particulate inorganic carbon (PIC) face a heightened risk of blue carbon depletion in the event of leakage, but with considerable potential for re-sequestration of the escaped CO<sub>2</sub> into solution as the HCO<sub>3</sub><sup>-</sup> ion, as a result of enhanced dissolution of seafloor calcium carbonates and release of buffering alkalinity. This aqueous storage of any released CO<sub>2</sub> will be limited under low rates of release, due to the titration of the carbon dioxide with the alkalinity already present in the sediment pore water. Conversely, at higher release rates the re-sequestration of the escaped CO<sub>2</sub> is controlled by the solubility of the calcium carbonate under near CO<sub>2</sub> saturated conditions, such that the proportion of resequestered CO<sub>2</sub> can be quantified through a thermodynamic framework. Locales rich in particulate organic carbon (POC) tend to exhibit a reduced susceptibility to blue carbon loss, yet have a reduced neutralization potential for CO<sub>2</sub> leakage.</div></div>","PeriodicalId":334,"journal":{"name":"International Journal of Greenhouse Gas Control","volume":"145 ","pages":"Article 104408"},"PeriodicalIF":4.6,"publicationDate":"2025-05-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144084040","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
A review of modeling approaches for CO2 injection into depleted gas reservoirs: Coupling transient wellbore and reservoir dynamics 枯竭气藏CO2注入建模方法综述:瞬态井筒与储层动力学耦合
IF 4.6 3区 工程技术
International Journal of Greenhouse Gas Control Pub Date : 2025-05-17 DOI: 10.1016/j.ijggc.2025.104406
Behnam Tavagh Mohammadi , Ashkan Jahanbani Ghahfarokhi , Alv-Arne Grimstad
{"title":"A review of modeling approaches for CO2 injection into depleted gas reservoirs: Coupling transient wellbore and reservoir dynamics","authors":"Behnam Tavagh Mohammadi ,&nbsp;Ashkan Jahanbani Ghahfarokhi ,&nbsp;Alv-Arne Grimstad","doi":"10.1016/j.ijggc.2025.104406","DOIUrl":"10.1016/j.ijggc.2025.104406","url":null,"abstract":"<div><div>This paper reviews the current state of modeling the transient wellbore-reservoir coupling for CO<sub>2</sub> injection into depleted gas reservoirs (DGRs). It explores methodologies applied to CO<sub>2</sub> injection modeling, emphasizing recent advancements and unresolved challenges to provide an overview for researchers and industry professionals. A comprehensive perspective of the coupled wellbore-reservoir modeling system is offered, with detailed discussions on each aspect of the model including well modeling, reservoir modeling, wellbore-reservoir coupling schemes, and thermodynamic modeling. These components interact in complex ways during transient operations like injection start-up and shut-in. Inadequate modeling of these processes can lead to serious operational risks, such as wellbore damage from excessive cooling and inaccurate prediction of injection rates. Understanding these interactions is crucial for safe and efficient CO<sub>2</sub> storage operations. Future research should focus on developing more accurate two-phase wellbore models and addressing critical factors such as hydrate formation, as well as geochemical and geomechanical effects in the near-wellbore region, to enhance the accuracy of predictions for CO<sub>2</sub> injection into depleted gas reservoirs. The availability of real-world field measurements is essential for validating these models and improving their ability to predict complex transient behaviors effectively.</div></div>","PeriodicalId":334,"journal":{"name":"International Journal of Greenhouse Gas Control","volume":"145 ","pages":"Article 104406"},"PeriodicalIF":4.6,"publicationDate":"2025-05-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144070323","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Biogenic carbon capture at pulp mills via sodium spiking and oxy-fuel calcination 在纸浆厂通过钠喷淋和氧燃料煅烧进行生物碳捕获
IF 4.6 3区 工程技术
International Journal of Greenhouse Gas Control Pub Date : 2025-05-16 DOI: 10.1016/j.ijggc.2025.104409
Edgar Carrejo , Hasan Jameel , Sunkyu Park , William Joe Sagues
{"title":"Biogenic carbon capture at pulp mills via sodium spiking and oxy-fuel calcination","authors":"Edgar Carrejo ,&nbsp;Hasan Jameel ,&nbsp;Sunkyu Park ,&nbsp;William Joe Sagues","doi":"10.1016/j.ijggc.2025.104409","DOIUrl":"10.1016/j.ijggc.2025.104409","url":null,"abstract":"<div><div>Over 13 million metric tons of biogenic carbon dioxide (CO<sub>2</sub>) are mineralized yearly in United States (US) pulp mill recovery boilers as molten sodium carbonate. The mineralized CO<sub>2</sub> is released downstream in the rotary lime kiln where it can be captured at a relatively low cost for permanent sequestration. The use of biocarbon and bioenergy at pulp mills enables the possibility for atmospheric carbon removal when biogenic CO<sub>2</sub> is captured and sequestered. We demonstrate the feasibility of capturing biogenic CO<sub>2</sub> via sodium spiking coupled with oxy-fuel calcination in the rotary lime kiln at existing kraft pulp mills. Sodium (Na) spiking elevates the Na ion loading in the kraft chemical looping process by replacing chlorine-based bleaching with a highly alkaline bleaching sequence. Chemical pulping processes are modeled and simulated to understand the technical limits of implementing sodium spiking in existing pulp mills. Each 1 % of sodium added to the bleaching operations increases the rate of CO<sub>2</sub> mineralization by 4 %, and the maximum increase in sodium content in the kraft process is 9 %. Without sodium spiking, estimated CO<sub>2</sub> capture costs are $131 and $107/mt CO<sub>2</sub> for air and oxy-fuel combustion, respectively. With the implementation of sodium spiking, the cost of CO<sub>2</sub> captured decreases by 27 % and 31 %, showing costs of $96 and $74/mt CO<sub>2</sub> for air and oxy-fuel combustion, respectively. Oxy-fuel combustion reduces the costs of CO<sub>2</sub> capture compared to air combustion, but merged deployment with sodium spiking seems to be the most cost-effective pathway to integrate carbon capture.</div></div>","PeriodicalId":334,"journal":{"name":"International Journal of Greenhouse Gas Control","volume":"145 ","pages":"Article 104409"},"PeriodicalIF":4.6,"publicationDate":"2025-05-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144070322","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dissolved oxygen depletion catalyzed by amino acids in piperazine 哌嗪中氨基酸催化的溶解氧耗竭
IF 4.6 3区 工程技术
International Journal of Greenhouse Gas Control Pub Date : 2025-05-15 DOI: 10.1016/j.ijggc.2025.104405
James I. Obute, Gary T. Rochelle
{"title":"Dissolved oxygen depletion catalyzed by amino acids in piperazine","authors":"James I. Obute,&nbsp;Gary T. Rochelle","doi":"10.1016/j.ijggc.2025.104405","DOIUrl":"10.1016/j.ijggc.2025.104405","url":null,"abstract":"<div><div>Dissolved oxygen (DO) significantly influences the oxidative degradation of amine solvents used for CO<sub>2</sub> capture from oxygen-containing gases. Amino acids are major degradation products in pilot testing of piperazine (PZ) solvent. This study used oxygen depletion to investigate the effect of metal ions and amino acids on amine oxidation in 5 m PZ. DO consumption was catalyzed by Fe<sup>3+</sup> with a half-order dependency on Fe<sup>3+</sup>. A reaction order breakpoint occurred at 0.05 mM Fe³⁺, beyond which excess Fe³⁺ likely formed inactive clusters. Amino acids enhance the effective solubility and availability of monomeric Fe³⁺, amplifying its catalytic effect. Adding 0.05 mM ethylenediaminetetraacetic acid (EDTA) with 0.05 mM Fe³⁺ increased the rate constant for oxygen depletion from 0.53 h⁻¹ (clean 5 m PZ) to 6.5 h⁻¹. A plateau in DO consumption rate was seen at a critical Fe³⁺ concentration for each tested amino acid, beyond which additional Fe³⁺ became inactive. At lower Fe<sup>3+</sup> (0.025 mM), amino acids such as nitrilotriacetic acid (NTA) sequestered Fe³⁺, reducing catalytic potential, while others enhanced it. This suggests that the role of amino acids is more complex than previously understood. Amino acids were ranked by their ability to increase DO consumption with 1 mM Fe³⁺ in 5 m PZ: 1 mM EDTA &gt; 20 mM 1,2-di(piperazin-1-yl)ethan-1-one (PZAAPZ+) &gt; 15 mM NTA &gt; 15 mM <em>N-</em>(2-aminoethyl)glycine (AEG+) &gt; 15 mM ethylenediaminediacetic acid (EDDA) &gt; 15 mM glycine (GLY) &gt; 15 mM iminodiacetic acid (IDA). In a degraded solvent sample from pilot plant testing, degradation products complex metal ions, enhancing their catalytic effects.</div></div>","PeriodicalId":334,"journal":{"name":"International Journal of Greenhouse Gas Control","volume":"145 ","pages":"Article 104405"},"PeriodicalIF":4.6,"publicationDate":"2025-05-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143946667","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Developing a preliminary site selection method for direct air capture and CO2 storage technology with a case study in the North Germany 以德国北部为例,开发直接空气捕获和二氧化碳储存技术的初步选址方法
IF 4.6 3区 工程技术
International Journal of Greenhouse Gas Control Pub Date : 2025-05-14 DOI: 10.1016/j.ijggc.2025.104392
Yifan Xu , Mrityunjay Singh , Cornelia Schmidt-Hattenberger , Márton Pál Farkas , Wolfgang Weinzierl , Tomas Fernandez-Steeger
{"title":"Developing a preliminary site selection method for direct air capture and CO2 storage technology with a case study in the North Germany","authors":"Yifan Xu ,&nbsp;Mrityunjay Singh ,&nbsp;Cornelia Schmidt-Hattenberger ,&nbsp;Márton Pál Farkas ,&nbsp;Wolfgang Weinzierl ,&nbsp;Tomas Fernandez-Steeger","doi":"10.1016/j.ijggc.2025.104392","DOIUrl":"10.1016/j.ijggc.2025.104392","url":null,"abstract":"<div><div>Achieving global net-zero emission targets requires substantial CO<sub>2</sub> removal, with Direct Air Capture and Carbon Storage (DACCS) emerging as a pivotal technology. Addressing a knowledge gap in systematically selecting optimal geological sites for CO<sub>2</sub> storage for DACCS, this study introduces a novel and adaptable multicriteria site selection and ranking methodology. By coupling the Analytical Hierarchy Process (AHP) with multicriteria decision-making, we quantitatively evaluate and prioritize potential storage sites, providing a scalable framework applicable to sedimentary basins worldwide. As a case study, we compiled and standardized publicly available geological data to build a comprehensive underground storage database for the North German Basin (NGB), categorizing geological features into five key criteria: storage capacity, injectivity, trapping mechanism, containment, and cost. Representative parameters under each criterion were harmonized for data resolution and quality. Our findings not only highlight promising sites in the German North Sea and the state of Brandenburg but also demonstrate the methodology's effectiveness in systematically identifying optimal sites for DACCS implementation. The developed criteria-based ranking system incorporates weighting factors determined by experts, effectively quantifying the importance of each criterion while accounting for uncertainties in both parameters and weighting factors. This approach addresses the global site selection necessity for CO₂ storage by providing a transparent, reproducible, and adaptable framework.</div></div>","PeriodicalId":334,"journal":{"name":"International Journal of Greenhouse Gas Control","volume":"145 ","pages":"Article 104392"},"PeriodicalIF":4.6,"publicationDate":"2025-05-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143946780","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Chemical monitoring for shallow-water subsea CCS: Anomaly detection and sensor coverage 浅水海底CCS的化学监测:异常检测和传感器覆盖
IF 4.6 3区 工程技术
International Journal of Greenhouse Gas Control Pub Date : 2025-05-14 DOI: 10.1016/j.ijggc.2025.104407
J. Greenwood , M. Mongin , E. Van Ooijen , A.S. Ross , C. Jenkins , D. Slawinski
{"title":"Chemical monitoring for shallow-water subsea CCS: Anomaly detection and sensor coverage","authors":"J. Greenwood ,&nbsp;M. Mongin ,&nbsp;E. Van Ooijen ,&nbsp;A.S. Ross ,&nbsp;C. Jenkins ,&nbsp;D. Slawinski","doi":"10.1016/j.ijggc.2025.104407","DOIUrl":"10.1016/j.ijggc.2025.104407","url":null,"abstract":"<div><div>Chemical monitoring of dissolved carbon dioxide (CO<sub>2</sub>) in seawater provides assurance for subsea carbon capture and storage (CCS) but can be confounded by high natural variability, and rapid dilution of any anomalous additions, placing strict limits on leak detection. In this study, we demonstrate how pre-injection baseline monitoring data can be combined with a plume dispersal model to provide guidelines for monitoring design, using a proposed CCS shallow water location on the Australian continental shelf as an example. This avoids the need to accurately simulate background CO<sub>2</sub> variability in an ecosystem model for the purpose of performing CO<sub>2</sub> leak simulations. In the test region, unusually steep spatial concentration gradients associated with the model simulated CO<sub>2</sub> leak plume means that higher frequency chemical sensor sampling is expected to improve anomaly detection. We determine that any leak in the test region should be detectable by chemical monitoring of pH by sampling at a minimum rate of 4 hr<sup>-1</sup> within the area affected by a drop in pH of at least 0.01 over a 60-day monitoring period. The leak-affected area depends on the leak rate and is shown to increase over time due to variable flow direction and decrease with average water velocity due to higher rates of dilution. The dimensions of the leak-affected area are reported for leak rates between 5 and 50 t CO<sub>2</sub>d<sup>-1</sup> providing critical information for monitoring design in the region.</div></div>","PeriodicalId":334,"journal":{"name":"International Journal of Greenhouse Gas Control","volume":"145 ","pages":"Article 104407"},"PeriodicalIF":4.6,"publicationDate":"2025-05-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143942504","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Carbon capture utilisation and storage (CCUS) and public perceptions: A systematic literature review 碳捕集利用与封存(CCUS)与公众认知:系统文献综述
IF 4.6 3区 工程技术
International Journal of Greenhouse Gas Control Pub Date : 2025-05-13 DOI: 10.1016/j.ijggc.2025.104393
Raquel Tardin-Coelho, Bishal Bharadwaj, Peta Ashworth
{"title":"Carbon capture utilisation and storage (CCUS) and public perceptions: A systematic literature review","authors":"Raquel Tardin-Coelho,&nbsp;Bishal Bharadwaj,&nbsp;Peta Ashworth","doi":"10.1016/j.ijggc.2025.104393","DOIUrl":"10.1016/j.ijggc.2025.104393","url":null,"abstract":"<div><div>Over time, carbon capture utilisation and storage (CCUS) projects have faced limited public acceptance, with projects being delayed due to public and policy opposition. Public concerns tend to focus on the perceived efficacy, potential risks, costs and benefits of CCUS projects. It highlights a need for further discussion and reflection on the various aspects of CCUS technologies and their implications for local host communities and the broader public. This systematic literature review utilises the Technology Acceptance Framework by Huijts, Molin and Steg (2012) to study public perceptions of CCUS globally, based on 88 peer-reviewed papers published between 2016 – 2024. It offers an updated perspective on positive, neutral and negative perceptions towards CCUS and the factors influencing them. Different public groups and aspects of the technologies are considered. Our findings suggest that positive perceptions are underpinned by trust in government and developers, as well as the establishment of fair and transparent decision-making processes alongside benefit sharing for local host communities. It confirms that knowledge and awareness of CCUS technologies may affect support. For CCUS projects to be validated in society, more transparent decision-making and proactive engagement about the technological options to reduce emissions in the battle against climate change will be required.</div></div>","PeriodicalId":334,"journal":{"name":"International Journal of Greenhouse Gas Control","volume":"145 ","pages":"Article 104393"},"PeriodicalIF":4.6,"publicationDate":"2025-05-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143934961","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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