ACS Applied Optical Materials最新文献

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Achiral Cation-Induced Chirality Tuning in Cycloalkyl Chiral Cation-Based Quasi-1D and 2D Perovskites 非手性阳离子诱导的环烷基手性阳离子准一维和二维钙钛矿的手性调谐
IF 3.8
ACS Applied Optical Materials Pub Date : 2025-06-20 DOI: 10.1021/acsaom.5c00115
Xinyu Yin, Xiaoyu Zhang, Adewale Joseph Babatunde, Pranab Sarker, Xiaozhou Zheng, Tao Wei and Qiuming Yu*, 
{"title":"Achiral Cation-Induced Chirality Tuning in Cycloalkyl Chiral Cation-Based Quasi-1D and 2D Perovskites","authors":"Xinyu Yin,&nbsp;Xiaoyu Zhang,&nbsp;Adewale Joseph Babatunde,&nbsp;Pranab Sarker,&nbsp;Xiaozhou Zheng,&nbsp;Tao Wei and Qiuming Yu*,&nbsp;","doi":"10.1021/acsaom.5c00115","DOIUrl":"https://doi.org/10.1021/acsaom.5c00115","url":null,"abstract":"<p >Hybrid organic–inorganic perovskites have garnered significant attention in optoelectronics due to their exceptional optical and electrical properties. Among them, low-dimensional chiral perovskites represent a promising class of optoelectronic materials. However, most existing studies focus on chiral organic cations with aromatic structures. In this work, we utilize the cycloalkyl chiral cation (<i>R</i>)-(−)-1-cyclohexylethylammonium (R-CHEA<sup>+</sup>) as a chiral spacer and incorporate achiral alkyl and aryl cations to systematically investigate the impact of molecular rigidity on structural and chiroptical properties of chiral lead iodide perovskites. Structural characterization reveals that the structural rigidity of chiral cations is crucial for efficient chirality transfer across the organic–inorganic interface and for the structural transition from quasi-1D to 2D perovskites. Our findings suggest a strategy to enhance rigidity in chiral cations, improving chirality transfer efficiency. This study provides insights into the mechanism of chirality transfer in chiral perovskites, offering a promising path for future advancements in chiroptoelectronics.</p>","PeriodicalId":29803,"journal":{"name":"ACS Applied Optical Materials","volume":"3 7","pages":"1499–1512"},"PeriodicalIF":3.8,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144808365","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Smart Fluorescence Tuning and Micelle-Stabilized White Light Emission via a Coumarin 102–Rhodamine B System: A Simple Path to Eclectic Color Luminescence for Anti-Counterfeiting Applications 香豆素102 -罗丹明B系统的智能荧光调谐和胶束稳定白光发射:一种用于防伪应用的折衷彩色发光的简单途径
IF 3.8
ACS Applied Optical Materials Pub Date : 2025-06-17 DOI: 10.1021/acsaom.5c00169
Firdaus Ahmad Ahanger, Ayaz Ahmad Manhas, Gousia Ahanger, Tameza Farooq, Showkat Rashid, Saima Sidiq, Sohail Amin Malik, Sahiba Gulzar, Naazim Basheer and Aijaz Ahmad Dar*, 
{"title":"Smart Fluorescence Tuning and Micelle-Stabilized White Light Emission via a Coumarin 102–Rhodamine B System: A Simple Path to Eclectic Color Luminescence for Anti-Counterfeiting Applications","authors":"Firdaus Ahmad Ahanger,&nbsp;Ayaz Ahmad Manhas,&nbsp;Gousia Ahanger,&nbsp;Tameza Farooq,&nbsp;Showkat Rashid,&nbsp;Saima Sidiq,&nbsp;Sohail Amin Malik,&nbsp;Sahiba Gulzar,&nbsp;Naazim Basheer and Aijaz Ahmad Dar*,&nbsp;","doi":"10.1021/acsaom.5c00169","DOIUrl":"https://doi.org/10.1021/acsaom.5c00169","url":null,"abstract":"<p >The pursuit of simple, cost-effective, and emission color-tunable luminescent materials is gaining momentum due to their vast potential in emerging technologies. However, practical systems with high tunability, compatibility, and aqueous stability remain limited. In this work, we report a smart luminescent platform based on two well-known and sensitive organic fluorophores coumarin 102 (C102) and rhodamine B (RhB) that collectively deliver a broad color-tunable emission with minimal material incompatibility. C102 exhibits polarity and pH-dependent fluorescence shifts, while RhB responds sensitively to temperature changes, enabling multimodal modulation of emission through solvent polarity, pH, and temperature variations. A precise molar ratio (C102: RhB = 4:10) yields stable white-light emission (CIE: 0.33, 0.33) in an aqueous medium. Furthermore, the system offers multistate fluorescence switching driven by pH and thermal stimuli, enabling its use in reversible, water-based fluorescent security inks for concealment, revelation, and erasure-based encryption. Embedding the fluorophores within sodium dodecyl sulfate (SDS) micelles ensures emission stability and facilitates efficient Förster resonance energy transfer (FRET) (∼94%) from C102 to RhB in acidic aqueous environments. This eco-friendly and tunable system holds significant promise for next-generation anticounterfeiting, display, and biosensing technologies.</p>","PeriodicalId":29803,"journal":{"name":"ACS Applied Optical Materials","volume":"3 6","pages":"1451–1460"},"PeriodicalIF":3.8,"publicationDate":"2025-06-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144808260","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High-Purity Deep Red Emission of Cr3+-Doped YAlO3 Solid Solution with Perovskite Structure for Plant Growth 具有钙钛矿结构的Cr3+掺杂YAlO3固溶体在植物生长中的高纯度深红色发射
IF 3.8
ACS Applied Optical Materials Pub Date : 2025-06-16 DOI: 10.1021/acsaom.5c00163
Mengyu Zhang, Chong Li, Wenzhi Su, Chuancheng Zhang, Haitang Hu, Yong Zou, Wenpeng Liu, Qingli Zhang and Shoujun Ding*, 
{"title":"High-Purity Deep Red Emission of Cr3+-Doped YAlO3 Solid Solution with Perovskite Structure for Plant Growth","authors":"Mengyu Zhang,&nbsp;Chong Li,&nbsp;Wenzhi Su,&nbsp;Chuancheng Zhang,&nbsp;Haitang Hu,&nbsp;Yong Zou,&nbsp;Wenpeng Liu,&nbsp;Qingli Zhang and Shoujun Ding*,&nbsp;","doi":"10.1021/acsaom.5c00163","DOIUrl":"https://doi.org/10.1021/acsaom.5c00163","url":null,"abstract":"<p >Efficient and homogeneous doping of Cr<sup>3+</sup> (1 at. %) in yttrium–aluminum perovskite (YAlO<sub>3</sub>, YAP) solid solution was successfully achieved using a high-temperature melting method. The cell structure figure indicates the formation of orthogonally distorted perovskite structure (space group Pbnm) after the substitution of Cr<sup>3+</sup> for Al<sup>3+</sup> sites, and the Goldschmidt tolerance factor (<i>t</i> = 0.88) reveals the inevitability of the lattice distortion, while Raman spectroscopy confirms the significant enhancement of the local structural disorder. Excitation and emission spectra show that YAP: Cr<sup>3+</sup> exhibits bilinear state far-red emission at 724 and 731 nm with 100% color purity, which perfectly matches the absorption peaks (730 nm) of the phytochrome far-red (P<sub>FR</sub>), which is required for plant photosynthesis. Variable-temperature spectroscopy confirms that the luminescence intensity of the material at 420 K is 48.4% of that at 300 K, with <i>E</i><sub>a</sub> = 0.12 eV, good thermal stability, and a fluorescence lifetime of 29 ms, which is significantly better than that of the conventional garnet system (such as YAG: Cr<sup>3+</sup>, τ ≈ 3 ms). This finding demonstrates that the high color purity, excellent thermal stability, and luminescence properties of YAP: Cr<sup>3+</sup> have great potential for full-spectrum illumination and plant growth control light sources.</p>","PeriodicalId":29803,"journal":{"name":"ACS Applied Optical Materials","volume":"3 6","pages":"1443–1450"},"PeriodicalIF":3.8,"publicationDate":"2025-06-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144808170","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Unveiling the Optical Properties of Micropattern-Based Fluorescent Gold Nanoclusters and Plasmonic Nanoparticles in Polymer Thin Films 揭示聚合物薄膜中基于微图的荧光金纳米团簇和等离子体纳米粒子的光学性质
IF 3.8
ACS Applied Optical Materials Pub Date : 2025-06-15 DOI: 10.1021/acsaom.5c00103
Quang Truong Pham, Isabelle Ledoux-Rak and Ngoc Diep Lai*, 
{"title":"Unveiling the Optical Properties of Micropattern-Based Fluorescent Gold Nanoclusters and Plasmonic Nanoparticles in Polymer Thin Films","authors":"Quang Truong Pham,&nbsp;Isabelle Ledoux-Rak and Ngoc Diep Lai*,&nbsp;","doi":"10.1021/acsaom.5c00103","DOIUrl":"https://doi.org/10.1021/acsaom.5c00103","url":null,"abstract":"<p >Gold nanoclusters (Au NCs) and gold nanoparticles (Au NPs) are directly created within a polymer matrix by employing a direct laser writing (DLW) technique. The excitation of a continuous-wave 532 nm laser inside a hybrid metal complex/photoresist material optically induces a localized thermal effect, resulting in the formation of polymeric voxels containing either strongly fluorescent Au NCs, or plasmonic Au NPs, depending on the exposure dose. Furthermore, this DLW technique allowed us to fabricate multidimensional micropatterns of Au NCs within a polymer matrix by controlling the movement of the laser focus, achieving a feature size of 1 μm and a minimum periodicity of 1.5 μm. The direct creation of Au NCs and/or Au NPs inside a photoresist film offers a simple and low-cost approach for advancing the field of plasmonic nanofabrication and opens applications such as Au fluorescence-based lasers or Au quantum dots for quantum light generation.</p>","PeriodicalId":29803,"journal":{"name":"ACS Applied Optical Materials","volume":"3 6","pages":"1324–1329"},"PeriodicalIF":3.8,"publicationDate":"2025-06-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144808218","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Polarization-Sensitive Scattering from Tunable Hybrid Au–Si Nanoantennas for Anticounterfeiting Applications 用于防伪的可调谐混合金硅纳米天线极化敏感散射
IF 3.8
ACS Applied Optical Materials Pub Date : 2025-06-12 DOI: 10.1021/acsaom.5c00156
Pavel Kustov*, Vitaly Yaroshenko, Martin Sandomirskii, Elena Petrova, Maria Fedorova, Eduard Ageev, Ivan Mukhin and Dmitry Zuev*, 
{"title":"Polarization-Sensitive Scattering from Tunable Hybrid Au–Si Nanoantennas for Anticounterfeiting Applications","authors":"Pavel Kustov*,&nbsp;Vitaly Yaroshenko,&nbsp;Martin Sandomirskii,&nbsp;Elena Petrova,&nbsp;Maria Fedorova,&nbsp;Eduard Ageev,&nbsp;Ivan Mukhin and Dmitry Zuev*,&nbsp;","doi":"10.1021/acsaom.5c00156","DOIUrl":"https://doi.org/10.1021/acsaom.5c00156","url":null,"abstract":"<p >Polarization of light provides an additional degree of freedom in nanostructure-light interactions and delivers a wide variety of physical phenomena and applications. While relatively well-described for plasmonics and high-refractive-index nanosystems, the potential for polarization-dependent control of optical properties in hybrid nanostructures composed of two or more materials remains not fully unlocked. Here, we study the polarization-dependent scattering behavior of resonant hybrid gold–silicon nanostructures lacking inversion symmetry. We adjust the geometrical configuration and material phase of the nanostructure components through precise femtosecond laser irradiation to induce polarization-dependent changes of scattering spectra. By evaluating the color change using the color-difference (Δ<i>E</i>*) formula, we demonstrate Δ<i>E</i>* values of approximately 9.7 and 3.9 for TE- and TM-polarized oblique illumination, respectively. Notably, the latter value is close to the just noticeable difference threshold of 2.3 calculated for the studied nanosystems. Numerical simulations and semianalytical multipole decomposition techniques are applied to investigate this polarization-dependent scattering behavior, revealing that for the studied hybrid nanosystem, this phenomenon occurs at illumination angles ranging from 57° to 75°. Finally, we developed an effective defense mechanism against counterfeiting. The achieved results hold significant potential for further research into hybrid nanophotonic systems and for the development of optical chips, sensors, and anticounterfeit systems.</p>","PeriodicalId":29803,"journal":{"name":"ACS Applied Optical Materials","volume":"3 6","pages":"1432–1442"},"PeriodicalIF":3.8,"publicationDate":"2025-06-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144808085","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Multimode Ultrasensitive Optical Temperature Sensing Based on Upconversion Luminescence in BaNb2O6 Phosphor 基于BaNb2O6荧光粉上转换发光的多模超灵敏光学温度传感
IF 3.8
ACS Applied Optical Materials Pub Date : 2025-06-12 DOI: 10.1021/acsaom.5c00153
Xi Chen, Jing Li*, Li Chen, Xing Liu, Xuechen Jiao, Yaru Peng, Yuxin Huang and Guangyong Jin*, 
{"title":"Multimode Ultrasensitive Optical Temperature Sensing Based on Upconversion Luminescence in BaNb2O6 Phosphor","authors":"Xi Chen,&nbsp;Jing Li*,&nbsp;Li Chen,&nbsp;Xing Liu,&nbsp;Xuechen Jiao,&nbsp;Yaru Peng,&nbsp;Yuxin Huang and Guangyong Jin*,&nbsp;","doi":"10.1021/acsaom.5c00153","DOIUrl":"https://doi.org/10.1021/acsaom.5c00153","url":null,"abstract":"<p >Multimode and highly sensitive optical temperature measurements are the key technology to improve the temperature monitor. In this work, doping-concentration-optimized BaNb<sub>2</sub>O<sub>6</sub> materials show excellent temperature measurement performance, achieving multimode temperature measurement with self-calibration function upon a 980 nm laser diode pump. Four models of optically ultrasensitive temperature measurement are achieved in BaNb<sub>2</sub>O<sub>6</sub>: Yb<sup>3+</sup>/Er<sup>3+</sup> and Yb<sup>3+</sup>/Ho<sup>3+</sup> phosphors by making use of thermal coupling energy levels (Er<sup>3+</sup>: <sup>2</sup>H<sub>11/2</sub>/<sup>4</sup>S<sub>3/2</sub> and Ho<sup>3+</sup>: <sup>5</sup>F<sub>5</sub>) and nonthermal coupling energy levels (Er<sup>3+</sup>: <sup>2</sup>H<sub>11/2</sub>/<sup>4</sup>S<sub>3/2</sub>, <sup>4</sup>F<sub>9/2</sub> and Ho<sup>3+</sup>: <sup>5</sup>F<sub>5</sub>, <sup>5</sup>F<sub>4</sub>/<sup>5</sup>S<sub>2</sub>). In the BaNb<sub>2</sub>O<sub>6</sub>: 7.0% Yb<sup>3+</sup>/5.0% Er<sup>3+</sup> sample, we obtained maximum relative sensitivities (<i>S</i><sub>r</sub>) of <i>S</i><sub>r-g</sub> = 1.64% K<sup>–1</sup> and <i>S</i><sub>r-Er</sub> = 1.48% K<sup>–1</sup> at 298 K and maximum absolute sensitivities (<i>S</i><sub>a</sub>) of <i>S</i><sub>a-g</sub> = 0.33% K<sup>–1</sup> and <i>S</i><sub>a-Er</sub> = 0.113% K<sup>–1</sup> at 573 K corresponding to thermal coupling and nonthermal coupling energy levels, respectively. In the BaNb<sub>2</sub>O<sub>6</sub>: 7.0% Yb<sup>3+</sup>/0.5% Ho<sup>3+</sup> sample, maximum <i>S</i><sub>r</sub> levels of <i>S</i><sub>r-r</sub> = 0.64% K<sup>–1</sup> and <i>S</i><sub>r-Ho</sub> = 1.39% K<sup>–1</sup> at 298 K and maximum <i>S</i><sub>a</sub> levels of <i>S</i><sub>a-r</sub> = 0.375% K<sup>–1</sup> (298 K) and <i>S</i><sub>a-Ho</sub> = 1.25% K<sup>–1</sup> (498 K) are obtained simultaneously. Throughout all the modes in the testing temperature range, excellent temperature resolution is exhibited, achieving an optimal value of 0.016 K. The four optical temperature sensors are validated to own excellent resolution, repeatability, and accuracy. All the studies demonstrate that BaNb<sub>2</sub>O<sub>6</sub> is a promising candidate in the field of high-precision self-referencing multimode optical temperature measurements.</p>","PeriodicalId":29803,"journal":{"name":"ACS Applied Optical Materials","volume":"3 6","pages":"1410–1421"},"PeriodicalIF":3.8,"publicationDate":"2025-06-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144808032","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
One-Step Synthesis of Amine-Functionalized White-Light-Emitting Carbon Dots and Temperature-Dependent Photoluminescence Studies 氨基功能化白光发光碳点的一步合成及温度依赖性光致发光研究
IF 3.8
ACS Applied Optical Materials Pub Date : 2025-06-11 DOI: 10.1021/acsaom.5c00063
Muniappan Kalipriyadharshini,  and , Shanmugam Easwaramoorthi*, 
{"title":"One-Step Synthesis of Amine-Functionalized White-Light-Emitting Carbon Dots and Temperature-Dependent Photoluminescence Studies","authors":"Muniappan Kalipriyadharshini,&nbsp; and ,&nbsp;Shanmugam Easwaramoorthi*,&nbsp;","doi":"10.1021/acsaom.5c00063","DOIUrl":"https://doi.org/10.1021/acsaom.5c00063","url":null,"abstract":"<p >We synthesized amine-functionalized, white-light-emitting (WLE) carbon quantum dots using amino acid <span>l</span>-3,4-dihydroxyphenylalanine (DOPA) as a carbon precursor via a one-step, slow, low-temperature oxidative pyrolysis reaction. The synthesized carbon dots (<b>DP-CD</b>) were well-characterized by different spectral techniques, including XRD, XPS, FTIR, contact angle measurement, and steady-state and time-resolved fluorescence spectroscopic techniques. This single precursor containing carbon, nitrogen, and oxygen ensures nitrogen doping in the frameworks and is also responsible for different functional groups, such as amine, carboxyl, and amide, on the surface. An excitation-wavelength-dependent emission, along with intense white-light emission under UV excitation in the solution and thin film state, makes these materials single-component WLE phosphors. The origin of white-light emission is understandably the simultaneous emission from multiple chromophoric species in the carbon dots (CDs) covering the entire visible spectral region. The excitation-resolved area-normalized spectra (ERANES) and time-resolved area-normalized spectra (TRANES) exhibit isoemissive points ascertaining the presence of multiple chromophoric species. The surface amino groups on the <b>DP-CD</b> are essential to maintain the fluorescence properties because their reaction with aldehydes leads to diminished fluorescence quantum yields. The temperature-dependent fluorescence spectra exhibit a linear relationship between the temperature and emission intensity at longer excitation wavelengths and could make them candidates for luminescent temperature sensor applications.</p>","PeriodicalId":29803,"journal":{"name":"ACS Applied Optical Materials","volume":"3 6","pages":"1245–1253"},"PeriodicalIF":3.8,"publicationDate":"2025-06-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144808128","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Terahertz Self-Induced Dynamic Slow-Light Behavior in Metasurfaces 超表面中太赫兹自激动态慢光行为
IF 3.8
ACS Applied Optical Materials Pub Date : 2025-06-11 DOI: 10.1021/acsaom.5c00135
Soumyajyoti Mallick, Nityananda Acharyya, Vineet Gupta, Shreeya Rane, Koijam Monika Devi, Ashutosh Sharma, József A. Fülöp* and Dibakar Roy Chowdhury*, 
{"title":"Terahertz Self-Induced Dynamic Slow-Light Behavior in Metasurfaces","authors":"Soumyajyoti Mallick,&nbsp;Nityananda Acharyya,&nbsp;Vineet Gupta,&nbsp;Shreeya Rane,&nbsp;Koijam Monika Devi,&nbsp;Ashutosh Sharma,&nbsp;József A. Fülöp* and Dibakar Roy Chowdhury*,&nbsp;","doi":"10.1021/acsaom.5c00135","DOIUrl":"https://doi.org/10.1021/acsaom.5c00135","url":null,"abstract":"<p >Dynamically reconfigurable metasurfaces are complex to realize because they require exotic materials, external stimuli, or both. However, with the advent of intense THz transients, these conventional preconditions can be bypassed. Strong THz fields are capable of invoking modulation of the electronic configuration in materials through impact ionization. In this context, we report the diligent intertwining of strong THz field-induced nonlinearities and the structural interactions of near-field coupled metastructures. We experimentally demonstrate a well-established metal-on-silicon metasurface framework to achieve reconfigurability that is devoid of any exotic materials or external stimuli. Aided by meta-geometry, intense THz transients modify the dispersion of the silicon substrate, leading to self-induced nonlinear modulations in conductivities. Altering the conductivity through impact ionization results in dynamically reconfigurable electromagnetically induced transparency (EIT) effects in a self-sustained manner, controlling the slow-light characteristics (group delay and the group velocity) by more than 6 times. These outcomes could potentially enable versatile applications in upcoming 6G technologies and on-chip silicon-based integrated photonics.</p>","PeriodicalId":29803,"journal":{"name":"ACS Applied Optical Materials","volume":"3 6","pages":"1357–1364"},"PeriodicalIF":3.8,"publicationDate":"2025-06-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144808120","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Picometer-Scale Optical Electrohydrodynamic Sensing Method Based on F–P Interferometry 基于F-P干涉测量的皮米尺度光学电流体动力传感方法
IF 3.8
ACS Applied Optical Materials Pub Date : 2025-06-09 DOI: 10.1021/acsaom.5c00109
Li Wang, Liang Wang, Lin Fu, Fouad Belhora and Jia-Wei Zhang*, 
{"title":"Picometer-Scale Optical Electrohydrodynamic Sensing Method Based on F–P Interferometry","authors":"Li Wang,&nbsp;Liang Wang,&nbsp;Lin Fu,&nbsp;Fouad Belhora and Jia-Wei Zhang*,&nbsp;","doi":"10.1021/acsaom.5c00109","DOIUrl":"https://doi.org/10.1021/acsaom.5c00109","url":null,"abstract":"<p >Accurate measurement of propulsion generated by electrohydrodynamics (EHD) contributes to the assessment of the thrust efficiency of drones and electric aircraft and may provide benefits in sustainability and stability. Here, we propose an electrohydrodynamic (EHD) measurement system based on an optical Fabry–Perot (F–P) sensor which senses the EHD thrust generated by a bipolar corona discharge via an elastic sensitive element. Static calibration experiments of the sensor were performed under such a pin-plate corona discharge system. The dynamic output characteristics of the sensors were tested under corona discharges with different polarities and discharge distances. The results show that the sensor has a linear operating region of 4–7 kV, a linearity of 99.6%, and a sensitivity of 257.7 pm/kV. Negative corona discharge leads to a higher spectral offset of the sensor compared with positive corona discharge. Continuous and simultaneous ionic wind sensing via an optical EHD sensor should provide accurate information about the performance of the propulsion system and contribute to the enhancement of the dynamic stability of the EHD actuator system.</p>","PeriodicalId":29803,"journal":{"name":"ACS Applied Optical Materials","volume":"3 6","pages":"1350–1356"},"PeriodicalIF":3.8,"publicationDate":"2025-06-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144809146","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Photophysical Insights and Polarity Dynamics of 4-Diethylamino Salicylaldehyde-Based Fluorescent Molecules and Their Application as Mitochondrial and Endoplasmic Reticulum Tracker Agents 4-二乙胺水杨醛基荧光分子的光物理性质和极性动力学及其在线粒体和内质网跟踪剂中的应用
IF 3.8
ACS Applied Optical Materials Pub Date : 2025-06-04 DOI: 10.1021/acsaom.5c00089
Ramakrishnan AbhijnaKrishna, Shu-Pao Wu and Sivan Velmathi*, 
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