ACS Catalysis 最新文献

筛选
英文 中文
IF 11.3 1区 化学
ACS Catalysis Pub Date : 2025-06-20
Jan Fingerhut, Jessalyn A. DeVine, Rongrong Yin, Mark E. Bernard, Alice Bremer, Dmitriy Borodin, Kai Golibrzuch, Theofanis N. Kitsopoulos, Daniel J. Auerbach, Hua Guo and Alec M. Wodtke*, 
{"title":"","authors":"Jan Fingerhut, Jessalyn A. DeVine, Rongrong Yin, Mark E. Bernard, Alice Bremer, Dmitriy Borodin, Kai Golibrzuch, Theofanis N. Kitsopoulos, Daniel J. Auerbach, Hua Guo and Alec M. Wodtke*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":"15 12","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":11.3,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acscatal.5c01448","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429059","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 11.3 1区 化学
ACS Catalysis Pub Date : 2025-06-20
Yanwei Li, Jie Chen and Yi Shen*, 
{"title":"","authors":"Yanwei Li, Jie Chen and Yi Shen*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":"15 12","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":11.3,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acscatal.4c06137","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429063","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 11.3 1区 化学
ACS Catalysis Pub Date : 2025-06-20
Yang Chen, Diwen Zhou*, Yongli Chang, Yunzhao Xu, Hongqiao Lin, Lizhi Wu, Yu Tang, Chengyi Dai, Xingang Li, Lisheng Guo*, Ting Qiu and Li Tan*, 
{"title":"","authors":"Yang Chen, Diwen Zhou*, Yongli Chang, Yunzhao Xu, Hongqiao Lin, Lizhi Wu, Yu Tang, Chengyi Dai, Xingang Li, Lisheng Guo*, Ting Qiu and Li Tan*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":"15 12","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":11.3,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acscatal.5c01701","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429067","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 11.3 1区 化学
ACS Catalysis Pub Date : 2025-06-20
Francesco Falcioni*, Luke Humphreys*, Richard C. Lloyd*, Hao Wu, Isamir Martinez, Jonathan Jones, Shane McKenna, Katharina Neufeld, Ryan M. Phelan, Tay Rosenthal, Christophe J. Szczepaniak, Kumiko Yamamoto, Scott P. France and Anna Fryszkowska, 
{"title":"","authors":"Francesco Falcioni*, Luke Humphreys*, Richard C. Lloyd*, Hao Wu, Isamir Martinez, Jonathan Jones, Shane McKenna, Katharina Neufeld, Ryan M. Phelan, Tay Rosenthal, Christophe J. Szczepaniak, Kumiko Yamamoto, Scott P. France and Anna Fryszkowska, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":"15 12","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":11.3,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acscatal.5c01646","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429077","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 11.3 1区 化学
ACS Catalysis Pub Date : 2025-06-20
Antara Bhowmick, Sanjana Srinivas, Junyan Zhang, Jorge Moncada, Charles J. Titus, Bruce Ravel, Cherno Jaye, Daniel A. Fischer, Genevieve Yarema, Song Luo, Yuying Shu, Kewei Yu, Akash Warty, Sooyeon Hwang, Stavros Caratzoulas, Dionisios G. Vlachos*, Evan P. Jahrman* and Dongxia Liu*, 
{"title":"","authors":"Antara Bhowmick, Sanjana Srinivas, Junyan Zhang, Jorge Moncada, Charles J. Titus, Bruce Ravel, Cherno Jaye, Daniel A. Fischer, Genevieve Yarema, Song Luo, Yuying Shu, Kewei Yu, Akash Warty, Sooyeon Hwang, Stavros Caratzoulas, Dionisios G. Vlachos*, Evan P. Jahrman* and Dongxia Liu*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":"15 12","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":11.3,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acscatal.5c00494","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429086","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 11.3 1区 化学
ACS Catalysis Pub Date : 2025-06-20
Yuan-Xiang Yang, Yi-Fan Wang, Guo-Qiang Lin and Zhi-Tao He*, 
{"title":"","authors":"Yuan-Xiang Yang, Yi-Fan Wang, Guo-Qiang Lin and Zhi-Tao He*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":"15 12","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":11.3,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acscatal.5c01798","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429087","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 11.3 1区 化学
ACS Catalysis Pub Date : 2025-06-20
Wen-Hao Deng, Harry Lewin, Rong-Zhen Liao* and Edina Rosta*, 
{"title":"","authors":"Wen-Hao Deng, Harry Lewin, Rong-Zhen Liao* and Edina Rosta*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":"15 12","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":11.3,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acscatal.5c01682","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429098","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 11.3 1区 化学
ACS Catalysis Pub Date : 2025-06-20
Varanasi Sai Subhankar, Charan R. Nallapareddy, C. Buddie Mullins and Thomas C. Underwood*, 
{"title":"","authors":"Varanasi Sai Subhankar, Charan R. Nallapareddy, C. Buddie Mullins and Thomas C. Underwood*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":"15 12","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":11.3,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acscatal.5c01772","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144429633","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Thermochemical and Kinetic Correlations of Redox and Lewis Sites on Cobalt–Molybdenum Oxides: Illustrated with Alkanol-O2 Catalysis 钴钼氧化物上氧化还原和路易斯位点的热化学和动力学相关性:以醇-氧催化为例
IF 12.9 1区 化学
ACS Catalysis Pub Date : 2025-06-20 DOI: 10.1021/acscatal.5c01633
Guangming Cai, Ya-Huei Cathy Chin
{"title":"Thermochemical and Kinetic Correlations of Redox and Lewis Sites on Cobalt–Molybdenum Oxides: Illustrated with Alkanol-O2 Catalysis","authors":"Guangming Cai, Ya-Huei Cathy Chin","doi":"10.1021/acscatal.5c01633","DOIUrl":"https://doi.org/10.1021/acscatal.5c01633","url":null,"abstract":"Electronic properties of redox and Lewis acid sites on bifunctional metal oxides are inherently correlated to each other, a phenomenon that has long been recognized but not yet explicitly and quantitatively illustrated. Using alkanol oxidative dehydrogenation (ODH) and inter- and intramolecular dehydration (inter- and intra-DEH) kinetics as the respective thermochemical/electronic proxies for redox and Lewis acid sites, we elucidate the thermochemical and electronic correlations of these two types of sites on Co<sub><i>y</i></sub>MoO<sub><i>x</i></sub> domains with Co-to-Mo atomic ratio (<i>y</i>) varying from 0 to 1. At redox sites (O*), alkanol ODH occurs via a late, kinetically relevant C<sub>α</sub>–H scission transition state [O···<b>H···</b>RH<b>C</b>O···M<sup><i>n</i>+</sup>]<sup>‡</sup>, involving a net H atom (H<sup>•</sup>), arising from an electron (e<sup>–</sup>) and a proton (H<sup>+</sup>) transfer to a redox site, making hydrogen addition energy (HAE) as the kinetic descriptor, encapsulating the negative of electron (–EA<sub>MO</sub>) and proton (–PA<sub>O<sup>–</sup></sub>) affinities of catalysts. At Lewis acid sites, alkanol inter-DEH proceeds via S<sub>N</sub>2-type substitution with the [O<sup>δ−</sup>···<b>H···</b>RH<sub>2</sub>C<b>O···C</b>H<sub>2</sub>R<b>···O</b>H···M<sup>δ+</sup>]<sup>‡</sup> transition state, while intra-DEH, whether uni- or bimolecular, occurs via E2-type elimination through the [O<sup>δ−</sup>···<b>H···</b>R′H<b>C</b>H<sub>2</sub><b>C</b><sup><b>⊕</b></sup><b>···</b><sup><b>⊖</b></sup><b>O</b>H···M<sup>δ+</sup>]<sup>‡</sup> and [RH<sub>2</sub>C(H)O<sup>δ−</sup>···<b>H···</b>R′H<b>C</b>H<sub>2</sub><b>C</b><sup><b>⊕</b></sup><b>···</b><sup><b>⊖</b></sup><b>O</b>H···M<sup>δ+</sup>]<sup>‡</sup> transition states. These DEH pathways involve C–O scission in their respective transition states, where an electron and a <sup>•</sup>OH radical transfer as a <sup>⊖</sup>OH group to the Lewis acid center (<b>M</b><sup><b>δ+</b></sup>–O<sup>δ–</sup>). Consequently, the negative <sup>⊖</sup>OH affinity (–HA<sub>⊖OH</sub>) serves as an incomplete kinetic descriptor, encapsulating the same negative electron affinity and the negative <sup>•</sup>OH affinity (–HA<sub>•OH</sub>) of catalysts. The common electron transfer during the evolution of all these transition states in alkanol ODH and DEH entails the electron affinity of metal oxides to determine their relative activation enthalpies. On Co<sub><i>y</i></sub>MoO<sub><i>x</i></sub>, introducing Co cations as electronic perturbators increases the electron affinity of these oxides, thereby reducing both HAE at redox sites and –HA<sub>⊖OH</sub> at Lewis acid sites, which proportionally decreases the activation enthalpies for C<sub>α</sub>–H scission in methanol, ethanol, <i>n</i>-propanol, and <i>n</i>-butanol ODH; C–O formation in methanol and ethanol inter-DEH; and C<sub>β</sub>–H scission in uni- and bimolecular <i>n</i>-propanol and <i>n</i>-butanol intra-DEH, as th","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":"4 1","pages":""},"PeriodicalIF":12.9,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144335214","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
IF 11.3 1区 化学
ACS Catalysis Pub Date : 2025-06-20
Le-Cheng Wang, Hefei Yang, Qiangwei Li and Xiao-Feng Wu*, 
{"title":"","authors":"Le-Cheng Wang, Hefei Yang, Qiangwei Li and Xiao-Feng Wu*, ","doi":"","DOIUrl":"","url":null,"abstract":"","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":"15 12","pages":"XXX-XXX XXX-XXX"},"PeriodicalIF":11.3,"publicationDate":"2025-06-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/pdf/10.1021/acscatal.5c02925","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"144353613","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
0
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
相关产品
×
本文献相关产品
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信